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Am. Chem. Soc.<\/strong>\u4e0a<\/strong>\u53d1\u8868\u4e86\u9898\u4e3a\u201cTunable Magnetism and Extraordinary Sunlight Absorbance in Indium TriphosphideMonolayer<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u5728\u8fd9\u7bc7\u6587\u7ae0\u4e2d\uff0c\u7814\u7a76\u5de5\u4f5c\u8005\u901a\u8fc7\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u7b49\u65b9\u6cd5\u9884\u6d4b\u4e86\u4e00\u79cd\u65b0\u578b\u534a\u5bfc\u4f532D\u6750\u6599\u2014\u2014\u4e09\u78f7\u5316\u94df\uff08InP3<\/sub>\uff09\u5355\u5c42\u5e76\u7cfb\u7edf\u7814\u7a76\u4e86\u5176\u76f8\u5173\u6027\u80fd\u30022D 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eV\uff09\u5e76\u4e14\u8868\u73b0\u51fa\u9ad8\u7535\u5b50\u8fc1\u79fb\u7387\uff081919 cm2<\/sup>V-1<\/sup>s-1<\/sup>\uff09\u3002\u7814\u7a76\u8868\u660e\uff0c2D InP3<\/sub>\u6676\u4f53\u5728\u5176\u5e26\u7ed3\u6784\u4e2d\u663e\u793a\u51fa\u7535\u5b50\u4e0d\u7a33\u5b9a\u6027\uff0c\u5373\u8d39\u7c73\u80fd\u7ea7\u9644\u8fd1\u6709\u7c7bMexican-hat\u80fd\u5e26\u548cvan Hove\u5947\u70b9\uff0c\u8fd9\u5bfc\u81f4\u4e86\u538b\u7f29\u548c\u62c9\u4f38\u5e94\u53d8\u5bf9\u5176\u7535\u5b50\u7ed3\u6784\u7684\u975e\u5355\u8c03\u54cd\u5e94\u3002\u7531\u4e8e\u8fd9\u4e9b\u5e26\u7279\u5f81\uff0c\u53ef\u4ee5\u901a\u8fc7p\u578b\u63ba\u6742\uff08\u7a7a\u7a74\u6d53\u5ea6\u4ece5.04\u00d71013<\/sup>\u52301.72\u00d71014<\/sup> cm-2<\/sup>\uff09\u6216\u5f15\u5165\u7f3a\u9677\uff08\u7528Ge\u53d6\u4ee3P\u539f\u5b50\uff09\u6765\u8bf1\u5bfc\u548c\u8c03\u8282\u94c1\u78c1\u548c\u534a\u91d1\u5c5e\u6001\u3002\u5728InP3<\/sub>\u5355\u5c42\u7535\u5b50\u6216\u9ad8\u6d53\u5ea6\u7a7a\u7a74\u63ba\u6742\u4e0b\uff0c\u4f1a\u53d1\u751f\u534a\u5bfc\u4f53-\u91d1\u5c5e\u8f6c\u53d8\u3002\u6b64\u5916\uff0cInP3<\/sub>\u5355\u5c42\u5177\u6709\u8d85\u5f3a\u7684\u5149\u5438\u6536\u6027\u80fd\uff08105<\/sup> 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Am. Chem. Soc., 2017, DOI: 10.1021\/jacs.7b05133\uff09<\/p>\n \u672c\u6587\u7684\u7b2c\u4e00\u53ca\u901a\u8baf\u4f5c\u8005\u5355\u4f4d\u7686\u4e3a\u5317\u4eac\u822a\u7a7a\u822a\u5929\u5927\u5b66\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u7f2a\u5976\u534e\u526f\u6559\u6388\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u5b59\u5fd7\u6885\u6559\u6388\u3002\u7f2a\u5976\u534e\u526f\u6559\u6388\u4e8e2015\u5e74\u83b7\u5f97\u6bd4\u5229\u65f6\u5217\u65e5\u5927\u5b66\u7269\u7406\u5b66\u535a\u58eb\u5b66\u4f4d\uff0c2016\u5e74\u5165\u9009\u5317\u822a\u201c\u5353\u8d8a\u767e\u4eba\u201d\u8ba1\u5212\uff0c\u957f\u671f\u4ece\u4e8b\u6750\u6599\u7269\u6027\u7684\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u548c\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u7b49\uff0c\u76f8\u5173\u5de5\u4f5c\u53d1\u8868\u5728JACS\uff0cACS Nano, Nano Energy\uff0cAPL\uff0cJPCC\u7b49\u671f\u520a\u4e0a\u3002\u5b59\u5fd7\u6885\u6559\u6388\u591a\u5e74\u6765\u4e00\u76f4\u4ece\u4e8b\u8ba1\u7b97\u6750\u6599\u5b66\u3001\u6750\u6599\u5236\u5907\u4e0e\u8868\u5f81\u3001\u6750\u6599\u7ed3\u6784\u4e0e\u6027\u80fd\u5173\u7cfb\u7b49\u65b9\u9762\u7684\u7814\u7a76\u5de5\u4f5c\uff0c\u5728\u76f8\u53d8\/\u963b\u53d8\u5b58\u50a8\u6750\u6599\u53ca\u4e8c\u7ef4\u6750\u6599\u7684\u8bbe\u8ba1\u3001\u6a21\u62df\u548c\u5236\u5907\u8868\u5f81\u7814\u7a76\u4e2d\u53d6\u5f97\u4e86\u663e\u8457\u8fdb\u5c55\uff0c\u5728PNAS\uff0cPhys. Rev. Lett.\uff0cJACS\uff0cNano Lett.\uff0cACS Nano\uff0cAppl.Phys. Lett.\uff0cPhys. Rev. B\uff0cActa. Mater.\uff0cNano Energy\u7b49SCI\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587140\u4f59\u7bc7\u3002<\/p>\n \u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u8ba1\u7b97\u6750\u6599\u7ec4daoke\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n \u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n \u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u4e0a\u6d4b\u8bd5\u8c37!<\/a><\/p>\n \u76f8\u5173\u6587\u732e\u63a8\u8350\uff1a<\/strong><\/p>\n \u8fd1\u5e74\u8be5\u56e2\u961f\u5728\u4e8c\u7ef4\u6676\u4f53MXene\u65b9\u9762\u6587\u7ae0\u63a8\u8350\uff1a<\/p>\n Chen Si et.al.<\/em>, Nano Lett.<\/em><\/strong><\/a>, 2016, 16 (10), pp 6584\u20136591.<\/p>\n Zhonglu Guo et.al.<\/em>, J. Mater. Chem. A<\/em><\/strong><\/a>, 2016,\u00a0 4<\/strong>, 11446-11452.<\/p>\n
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