{"id":82826,"date":"2017-05-27T06:30:24","date_gmt":"2017-05-26T22:30:24","guid":{"rendered":"\/\/m.iemloyee.com\/?p=82826"},"modified":"2017-05-24T08:56:57","modified_gmt":"2017-05-24T00:56:57","slug":"angew-chem-int-ed-%ef%bc%9a%e7%a1%bc%e3%80%81%e6%b0%ae%e5%85%b1%e6%8e%ba%e5%a4%9a%e5%ad%94%e7%9f%b3%e5%a2%a8%e7%83%af%e6%ad%a3%e6%9e%81%e5%ae%9e%e7%8e%b0li-co2%e7%94%b5%e6%b1%a0%e9%ab%98%e6%95%88","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=82826","title":{"rendered":"Angew. Chem. Int. Ed.\uff1a\u787c\u3001\u6c2e\u5171\u63ba\u591a\u5b54\u77f3\u58a8\u70ef\u6b63\u6781\u5b9e\u73b0Li-CO2\u7535\u6c60\u9ad8\u6548\u53ef\u5145\u7535"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u5728\u8fc7\u53bb\u4e8c\u5341\u5e74\u91cc\uff0c\u9502\u79bb\u5b50\u7535\u6c60\u5360\u9886\u4e86\u4fbf\u643a\u5f0f\u7535\u5b50\u5e02\u573a\uff0c\u7136\u800c\uff0c\u76ee\u524d\u7684\u9502\u79bb\u5b50\u7535\u6c60\u80fd\u91cf\u5bc6\u5ea6\u975e\u5e38\u6709\u9650\u3002\u4e3a\u4e86\u6ee1\u8db3\u957f\u8ddd\u79bb\u7535\u52a8\u6c7d\u8f66\u4e25\u683c\u7684\u80fd\u91cf\u5bc6\u5ea6\u8981\u6c42\uff0c\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\uff0c\u7279\u522b\u662f\u9502\u7a7a\u7535\u6c60(\u4f8b\u5982\uff0cLi-O2<\/sub>\u7535\u6c60\u7406\u8bba\u80fd\u91cf\u5bc6\u5ea6\u7ea6\u4e3a3500Wh\u2009 kg\u22121<\/sup>)\u5f15\u8d77\u4e86\u6781\u5927\u5173\u6ce8\u3002Li(Na)-CO2<\/sub>\u7535\u6c60\u4f7f\u7528\u6e29\u5ba4\u6c14\u4f53\u4e8c\u6c27\u5316\u78b3\u4f5c\u4e3a\u6b63\u6781\u7684\u6d3b\u6027\u7269\u8d28\uff0c\u63d0\u4f9b\u4e86\u4e8c\u6c27\u5316\u78b3\u6355\u83b7\u7684\u65b0\u65b9\u6cd5\uff0c\u4ee3\u8868\u4e86\u4e0b\u4e00\u4ee3\u7535\u5316\u5b66\u50a8\u80fd\u7cfb\u7edf\u7684\u53d1\u5c55\u3002\u7136\u800c\uff0c\u4e8c\u6c27\u5316\u78b3\u4e0e\u9502\u8d1f\u6781\u7684\u7535\u5316\u5b66\u53cd\u5e94\u53ef\u80fd\u5bfc\u81f4\u7edd\u7f18Li2<\/sub>CO3<\/sub>\u7684\u4e0d\u53ef\u9006\u5f62\u6210\uff0c\u4f7f\u5f97\u7535\u6c60\u96be\u4ee5\u518d\u6b21\u5145\u7535\uff0c\u5373\u4f7f\u53ef\u4ee5\u5145\u7535\u4e5f\u8868\u73b0\u51fa\u6709\u9650\u7684\u5faa\u73af\u6027\u80fd\uff0c\u5177\u6709\u6781\u5927\u7684\u6781\u5316\u6027\u548c\u8f83\u5dee\u7684\u500d\u7387\u6027\u80fd\u3002\u6240\u4ee5\u5f00\u53d1\u4e8c\u6c27\u5316\u78b3\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u7684\u9ad8\u6548\u50ac\u5316\u5242\u5e76\u7814\u7a76Li-CO2<\/sub>\u7535\u6c60\u7684\u7535\u5316\u5b66\u884c\u4e3a\u81f3\u5173\u91cd\u8981\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/b><\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u51ef\u65af\u897f\u50a8\u5927\u5b66\u7684\u6234\u9ece\u660e\u6559\u6388\u548c\u7f8e\u56fd\u5b87\u822a\u5c40\u5170\u5229\u7814\u7a76\u4e2d\u5fc3\u7684Yi Lin\u535a\u58eb\u3001John W Connell\u535a\u58eb<\/strong>(\u5171\u540c\u901a\u8baf\u4f5c\u8005)\u7b49\u4eba\u5728Angew. Chem. Int. Ed.<\/strong>\u4e0a\u53d1\u8868\u4e86\u4e00\u7bc7\u540d\u4e3a\u201cHighly Rechargeable Lithium-CO2<\/sub>\u00a0Batteries with a Boron and Nitrogen-Codoped Holey-Graphene Cathode\u201d<\/strong>\u7684\u6587\u7ae0\uff0c\u7814\u7a76\u4eba\u5458\u5229\u7528B\u3001N\u5171\u63ba\u591a\u5b54\u77f3\u58a8\u70ef\u4f5c\u4e3a\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u548c\u6c27\u5316\u53cd\u5e94\u7684\u9ad8\u6548\u50ac\u5316\u5242\uff0c\u83b7\u5f97\u4e86\u9ad8\u53ef\u9006\u6027\u7684\u53ef\u5145\u7535Li-CO2<\/sub>\u7535\u6c60\u3002\u56e0\u4e3a\u72ec\u7279\u7684\u591a\u5b54\u7eb3\u7c73\u7ed3\u6784\u548c\u6b63\u6781\u7684\u9ad8\u50ac\u5316\u6d3b\u6027\uff0c\u6240\u5236\u5907\u7684Li-CO2<\/sub>\u7535\u6c60\u57281.0A g–<\/sup>1<\/sup>\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u4ecd\u7136\u5177\u6709\u9ad8\u53ef\u9006\u6027\uff0c\u4f4e\u6781\u5316\u6027\uff0c\u4f18\u5f02\u7684\u500d\u7387\u6027\u80fd\u548c\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1 <\/b><\/strong>\u5177\u6709BN<\/b><\/strong>–<\/b><\/strong>hG<\/b>\u6b63\u6781\u7684Li<\/b><\/strong>–<\/b><\/strong>CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u7535\u6c60<\/b><\/strong>\u7684\u7535\u5316\u5b66\u8fc7\u7a0b\u793a\u610f\u56fe\u548c<\/b><\/strong>BN<\/b><\/strong>–<\/b><\/strong>hG<\/b><\/strong>\u7684\u5f62\u8c8c\u7ed3\u6784\u5206\u6790<\/b><\/strong><\/p>\n

\"\"\u00a0<\/p>\n

a) \u5177\u6709BN-hG\u6b63\u6781\u7684Li-CO2<\/sub>\u7535\u6c60\u793a\u610f\u56fe\uff1b<\/p>\n

b) BN-hG\u6b63\u6781\u4e0a\u76f8\u5e94\u7684CO2<\/sub>\u8fd8\u539f\u548c\u6c27\u5316\u53cd\u5e94\uff1b<\/p>\n

c) BN-hG\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

d) hG\u548cBN-hG\u7684N2<\/sub>\u5438\u9644-\u89e3\u5438\u7b49\u6e29\u7ebf\u548c\u5b54\u5f84\u5206\u5e03(PSD\uff0c\u63d2\u56fe)\uff1b<\/p>\n

e) hG\u548cBN-hG\u7684\u5206\u6790XPS\u5149\u8c31\uff1b<\/p>\n

f-g) N1s\u548cBN-hG\u7684\u9ad8\u5206\u8fa8\u7387\u5149\u8c31\u3002<\/p>\n

\u56fe2 hG\u548cBN-hG\u7535\u6781\u5bf9CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f\u548c\u6c27\u5316\u53cd\u5e94\u50ac\u5316\u6d3b\u6027\u7684\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u00a0a)\u00a0\u5728\u7535\u538b\u4e3a0\u301c4.5V\uff0c\u7535\u6d41\u5bc6\u5ea6\u4e3a0.3Ag–<\/sup>1<\/sup>\u7684\u60c5\u51b5\u4e0b\uff0c\u5177\u6709hG\u548cBN-hG\u6b63\u6781\u7684Li-CO2<\/sub>\u7535\u6c60\u7684\u5168\u653e\u7535\/\u5145\u7535\u66f2\u7ebf\uff1b<\/p>\n

b) \u9996\u6b21\u653e\u7535\u540ehG\u548cBN-hG\u7535\u6781\u7684XRD\u56fe\u3002<\/p>\n

\u56fe3 BN-hG\u7535\u6781\u5bf9CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f\u548c\u6c27\u5316\u8fc7\u7a0b\u7684\u53ef\u9006\u6027\u8868\u5f81<\/b><\/strong>
\n<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

a-b) \u5b8c\u5168\u653e\u7535(\u653e\u7535\u81f32.0V)BN-hG\u7535\u6781\u7684TEM\u56fe\u548c\u76f8\u5e94\u9009\u533a\u7535\u5b50\u884d\u5c04(SAED)\u56fe\uff1b<\/p>\n

c) \u5b8c\u5168\u518d\u5145\u7535(\u518d\u5145\u7535\u81f35V)BN-hG\u7535\u6781\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

d) BN-hG\u7535\u6781\u7684XRD\u56fe\uff1b<\/p>\n

e) \u5177\u6709BN-hG\u7535\u6781\u7684Li-CO2<\/sub>\u7535\u6c60\u7684\u539f\u59cb\u3001\u5b8c\u5168\u653e\u7535\u548c\u5b8c\u5168\u5145\u7535\u72b6\u6001\u7684\u963b\u6297\u8c31\u3002<\/p>\n

\u56fe4 \u5177\u6709hG\u548cBN-hG<\/b>\u6b63\u6781\u7684Li-CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u7535\u6c60\u7684<\/b><\/strong>\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong>\u8868\u5f81<\/b><\/strong>
\n<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

a) \u5177\u6709BN-hG\u6b63\u6781\u7684Li-CO2<\/sub>\u7535\u6c60\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u653e\u7535\/\u5145\u7535\u66f2\u7ebf((b)\u4e2d\u500d\u7387\u6d4b\u8bd5\u7684\u7b2c2\u30015\u30018\u300111\u300114\u548c17\u5468\u671f)\uff1b<\/p>\n

b) \u653e\u7535\u7ec8\u6b62\u7535\u538b\uff1b<\/p>\n

c) \u6781\u5316\uff1b<\/p>\n

d) \u5177\u6709hG\u548cBN-hG\u6b63\u6781\u7684Li-CO2<\/sub>\u7535\u6c60\u7684\u957f\u671f\u5faa\u73af\u6027\u80fd\uff0c\u524d\u4e24\u4e2a\u5faa\u73af\u7684\u5bc6\u5ea6\u4e3a1A g–<\/sup>1<\/sup>\uff0c\u540e\u7eed\u5faa\u73af\u4e3a1.0A g–<\/sup>1<\/sup>\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u672c\u6587\u4e2d\uff0c\u7814\u7a76\u4eba\u5458\u5c06\u591a\u5b54B\u3001N\u5171\u63ba\u591a\u5b54\u77f3\u58a8\u70ef\u7528\u4f5c\u53ef\u518d\u5145\u7535Li-CO2<\/sub>\u7535\u6c60\u7684\u6b63\u6781\u50ac\u5316\u5242\u3002\u56e0\u4e3a\u72ec\u7279\u7684\u591a\u5b54\u7eb3\u7c73\u7ed3\u6784\u548c\u9ad8\u50ac\u5316\u6d3b\u6027\uff0c\u65b0\u5f00\u53d1\u7684Li-CO2<\/sub>\u7535\u6c60\u6781\u5316\u73b0\u8c61\u663e\u8457\u964d\u4f4e\uff0c\u901f\u7387\u6027\u80fd\u4f18\u5f02\uff0c\u57281.0 A g–<\/sup>1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u53ef\u4ee5\u7a33\u5b9a\u5faa\u73af\u8d85\u8fc7200\u6b21\u2014\u2014\u80dc\u8fc7\u5df2\u62a5\u5bfc\u7684\u6240\u6709Li-CO2<\/sub>\u751a\u81f3Li-O2<\/sub>\/CO2<\/sub>\u7535\u6c60\u3002\u8fd9\u9879\u5de5\u4f5c\u5c55\u793a\u4e86\u4f4e\u6210\u672c\u65e0\u91d1\u5c5e\u3001\u53cc\u5b98\u80fd\u56e2\u78b3\u9634\u6781\u50ac\u5316\u5242\u514b\u670dLi-CO2<\/sub>\u7535\u6c60\u5faa\u73af\u4e0d\u7a33\u5b9a\u95ee\u9898\u7684\u53ef\u80fd\u6027\uff0c\u5e76\u5c06\u5176\u63a8\u5411\u5546\u4e1a\u5316\u3002\u8fd9\u5bf9\u4e0b\u4e00\u4ee3\u7535\u5316\u5b66\u50a8\u80fd\u7cfb\u7edf\u7684\u53d1\u5c55\u548c\u4e8c\u6c27\u5316\u78b3\u7684\u6355\u83b7\u90fd\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Highly Rechargeable Lithium<\/u>–<\/u>CO<\/u>2<\/sub><\/u>\u00a0Batteries with a Boron and Nitrogen<\/u>–<\/u>Codoped Holey<\/u>–<\/u>Graphene Cathode<\/u><\/a>(Angew. Chem. Int. Ed.,2017,DIO:10.1002\/anie.201701826)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u7ec4 deer \u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065952\u201d\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8\u5927\u5bb6\u5ead<\/a>\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1axiaofire-18\uff0c\u5434\u73ab\uff0c\u6211\u4eec\u4f1a\u62c9\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/b><\/strong><\/p>\n

\u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u627e<\/b><\/strong>\u6750\u6599\u4eba<\/b><\/strong><\/a>\u3001\u4e0a<\/b><\/strong>\u6d4b\u8bd5\u8c37<\/b><\/strong><\/a>\uff01<\/b><\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u5728\u8fc7\u53bb\u4e8c\u5341\u5e74\u91cc\uff0c\u9502\u79bb\u5b50\u7535\u6c60\u5360\u9886\u4e86\u4fbf\u643a\u5f0f\u7535\u5b50\u5e02\u573a\uff0c\u7136\u800c\uff0c\u76ee\u524d\u7684\u9502\u79bb\u5b50\u7535\u6c60\u80fd\u91cf\u5bc6\u5ea6\u975e\u5e38\u6709\u9650\u3002\u4e3a\u4e86\u6ee1\u8db3\u957f\u8ddd\u79bb\u7535\u52a8\u6c7d\u8f66\u4e25\u683c\u7684\u80fd\u91cf\u5bc6\u5ea6\u8981\u6c42\uff0c\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\uff0c\u7279\u522b\u662f…<\/p>\n","protected":false},"author":3706,"featured_media":82827,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[18,1729],"class_list":["post-82826","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-jiedu","tag-xinnengyuan","tag-1729"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/82826"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/3706"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=82826"}],"version-history":[{"count":5,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/82826\/revisions"}],"predecessor-version":[{"id":83132,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/82826\/revisions\/83132"}],"wp:featuredmedia":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/media\/82827"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=82826"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=82826"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=82826"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}