{"id":73282,"date":"2017-03-28T14:00:25","date_gmt":"2017-03-28T06:00:25","guid":{"rendered":"\/\/m.iemloyee.com\/?p=73282"},"modified":"2017-03-27T15:03:21","modified_gmt":"2017-03-27T07:03:21","slug":"adv-funct-mater-%ef%bc%9a%e9%87%8f%e5%ad%90%e7%82%b9%ef%bc%9a%e9%98%b2%e4%bc%aa%e5%8f%91%e5%85%89%e6%9d%90%e6%96%99","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=73282","title":{"rendered":"Adv. Funct. Mater.\uff1a\u91cf\u5b50\u70b9-\u9632\u4f2a\u53d1\u5149\u6750\u6599"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u534a\u5bfc\u4f53\u91cf\u5b50\u70b9\u5177\u6709\u900f\u660e\u6027\u3001\u6eb6\u6db2\u52a0\u5de5\u6027\u3001\u9ad8\u6548\u7387\u548c\u53ef\u8c03\u8282\u5e26\u5bbd\u7b49\u4f18\u826f\u6027\u8d28\uff0c\u8fd9\u4f7f\u5f97\u5176\u5728\u5149\u7535\u5b50\u9886\u57df\u5177\u6709\u826f\u597d\u7684\u5e94\u7528\u524d\u666f\u3002\u4e8c\u5143II-VI \u65cf\u590d\u5408\u7269\uff08\u5982CdS\uff09\u3001III\u2212V\u65cf\u590d\u5408\u7269\uff08\u5982InP\uff09\u548c\u4e09\u5143I-III-VI\uff08CuInS2<\/sub>\uff09\u5df2\u7ecf\u88ab\u5e7f\u6cdb\u5e94\u7528\u4e8eLED\u3001LD\u3001\u592a\u9633\u80fd\u7535\u6c60\u4e2d\u3002\u8fd1\u4e9b\u5e74\uff0c\u4e3a\u4e86\u907f\u514dCd2+<\/sup>\u7684\u6bd2\u6027\u3001\u51cf\u5c11In3+<\/sup>\u7684\u6210\u672c\uff0c\u9499\u949b\u77ff\u91cf\u5b50\u70b9\u5df2\u7136\u6210\u4e3a\u70ed\u70b9\u8bdd\u9898\u3002\u91cf\u5b50\u70b9\u5177\u6709\u7a84\u5e26\u53d1\u5c04\u3001\u5bbd\u5e26\u5438\u6536\u7684\u5149\u8c31\u7279\u5f81\u3002\u7531\u4e8e\u65af\u6258\u514b\u65af\u9891\u79fb\uff0c\u91cf\u5b50\u70b9\u7684\u5149\u8c31\u53d1\u5c04\u548c\u5438\u6536\u5b58\u5728\u91cd\u53e0\u3002\u91cf\u5b50\u70b9\u7684\u5149\u8c31\u7279\u5f81\u53d7\u91cd\u5438\u6536\u7684\u5f71\u54cd\uff0c\u8fd9\u4e00\u91cd\u5438\u6536\u662f\u7531\u80fd\u91cf\u5171\u632f\u8f6c\u79fb\u6548\u5e94\u9020\u6210\u7684\u3002\u53e6\u4e00\u79cd\u6539\u826f\u534a\u5bfc\u4f53\u91cf\u5b50\u70b9\u56fa\u6709\u6027\u8d28\u7684\u65b9\u6cd5\u662f\u5f15\u5165\u63ba\u6742\u7269\u3002\u63ba\u6742\u7269\u4f1a\u5728\u91cf\u5b50\u70b9\u7684\u4e2d\u95f4\u5e26\u533a\u57df\u4ea7\u751f\u65b0\u7684\u7535\u5b50\u6001\uff0c\u4ee5\u6b64\u6539\u53d8\u7535\u8377\u7684\u5206\u79bb\u548c\u590d\u5408\u3002Mn2+<\/sup>\u63ba\u5165CdS\/ZnS\u91cf\u5b50\u70b9\u4ee5\u540e\uff0c\u5176\u5149\u5b66\u6027\u8d28\u4e0e\u63ba\u6742\u4f4d\u7f6e\u6709\u5173\u3002CdS\u7684\u5e26\u8fb9\u91cf\u5b50\u4ea7\u7387\u662f\u5e38\u91cf\uff0c\u800c\u63ba\u5165Mn2+<\/sup>\u4ee5\u540e\uff0c\u91cf\u5b50\u4ea7\u7387\u589e\u52a0\u3002\u8fd9\u8bf4\u660e\u5e26\u8fb9\u53d1\u5c04\u548cMn2<\/sup>+<\/sup>\u4e4b\u95f4\u5b58\u5728\u6709\u6548\u7684\u80fd\u91cf\u4ea4\u4e92\u3002\u7406\u8bba\u4e0a\u5b58\u5728\u80fd\u591f\u8c03\u63a7\u6838\/\u591a\u58f3\u91cf\u5b50\u70b9\u7684PL\u53d1\u5149\u7684\u65b9\u6cd5\uff0c\u5305\u542b\u5e26\u8fb9\u53d1\u5c04\u548c\u7535\u5b50\u8dc3\u8fc1\uff0c\u4f9d\u636e\u4e0d\u540c\u7684\u6fc0\u53d1\u80fd\u91cf\u5c55\u73b0\u4e0d\u540c\u7684\u53d1\u5149\u884c\u4e3a\u3002\u5c06\u53d1\u5149\u6750\u6599\u4e0e\u53ef\u62c9\u4f38\u57fa\u5e95\u96c6\u6210\u5728\u4e00\u8d77\u662f\u5f53\u4eca\u7684\u70ed\u70b9\u8bdd\u9898\u3002\u7136\u800c\uff0c\u76ee\u524d\u5f88\u5c11\u6709\u62a5\u9053\u6d89\u53ca\u53ef\u62c9\u4f38\u7684\u9632\u4f2a\u6750\u6599\uff0c\u4ece\u800c\u5b9e\u73b0\u9ad8\u7aef\u7684\u9632\u4f2a\u529f\u80fd\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6765\u81ea\u5317\u4eac\u79d1\u6280\u5927\u5b66\u7684\u590f\u5fd7\u56fd\u6559\u6388<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09\u3001\u4e2d\u79d1\u9662<\/b><\/strong>\u5317\u4eac\u7eb3\u7c73\u80fd\u6e90\u4e0e\u7cfb\u7edf\u7814\u7a76\u6240\u7684\u6f58\u66f9\u5cf0\u7814\u7a76\u5458<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u7b49\u4eba\u7814\u7a76\u5236\u5907\u51fa\u4e86\u4e00\u79cd\u53ef\u62c9\u4f38\u3001\u900f\u660e\u3001\u989c\u8272\u53ef\u8c03\u7684PDMS\u8584\u819c\uff08LPF\uff09\uff0c\u5e76\u4e14\u63a2\u7d22\u4e86\u5176\u5728\u9632\u4f2a\u53d1\u5149\u65b9\u9762\u7684\u6f5c\u5728\u5e94\u7528\u3002<\/p>\n

\u8fd9\u9879\u5de5\u4f5c\u901a\u8fc7\u81ea\u4e0b\u800c\u4e0a\u7684\u65b9\u6cd5\u5236\u5907LPF\uff0c\u4f7f\u5176\u53ef\u4ee5\u7075\u6d3b\u5730\u8f6c\u79fb\u5230\u5176\u4ed6\u4efb\u4f55\u8f7d\u4f53\u4e0a\u3002\u540c\u65f6\uff0cLPF\u7684\u53ef\u62c9\u4f38\u6027\u548c\u900f\u660e\u6027\u4f7f\u5f97\u5176\u5728\u9632\u4f2a\u9886\u57df\u4e2d\u5f97\u4ee5\u5e7f\u6cdb\u5e94\u7528\u3002LPF\u53ef\u4ee5\u5b8c\u7f8e\u5730\u5408\u5e76\u8f7d\u6d41\u5b50\uff0c\u5e76\u4e14\u4e0d\u4f1a\u5bf9\u8bc6\u522b\u539f\u6709\u7684\u4fe1\u606f\u9020\u6210\u4e0d\u826f\u5f71\u54cd\uff0c\u8fd9\u9884\u793a\u4e86\u65b0\u7684\u8367\u5149\u9632\u4f2a\u529f\u80fd\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1<\/b><\/strong>\u00a0<\/b><\/strong>CdS\/ZnS\/ZnS:Mn<\/b><\/strong>2+<\/b><\/sup><\/strong>\/ZnS<\/b><\/strong>\u6838<\/b><\/strong>\/<\/b><\/strong>\u591a\u91cd\u91cf\u5b50\u70b9\u7684\u5408\u6210\u53ca\u7ed3\u6784\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a)\u00a0\u4e09\u6b65\u5408\u6210\u8bf4\u660e\uff0c\u70ed\u538b\u4f4f\u53cd\u5e94\u8fc7\u7a0b\u548c\u6bcf\u4e00\u6b65\u53cd\u5e94\u6240\u9700\u7684\u539f\u6750\u6599\u90fd\u5df2\u7ed9\u51fa<\/p>\n

(b) \u5236\u5907\u7684CdS,\u00a0CdS\/ZnS\u548cCdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u91cf\u5b50\u70b9\u4ee5\u53ca\u76f8\u5e94\u7684ZnS \u548c\u00a0CdS\u7684\u6807\u51c6XRD\u884d\u5c04\u82b1\u6837<\/p>\n

(c\u3001d\u3001e)\u00a0\u5206\u522b\u4e3aCdS\u3001CdS\/ZnS\u548cCdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u91cf\u5b50\u70b9\u7684\u900f\u5c04\u7535\u955c\u56fe\u50cf\u53ca\u7535\u5b50\u884d\u5c04\u82b1\u6837<\/p>\n

(f)\u00a0CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS \u91cf\u5b50\u70b9\u4e2dZnS\u7684(220)\u548c(111)\u6676\u9762\u7684\u9ad8\u5206\u8fa8\u900f\u5c04\u7535\u5b50\u50cf<\/p>\n

\u56fe2<\/b><\/strong>\u00a0<\/b><\/strong>CdS\/ZnS\/ZnS:Mn<\/b><\/strong>2+<\/b><\/sup><\/strong>\/ZnS <\/b><\/strong>\u6838<\/b><\/strong>\/<\/b><\/strong>\u591a\u91cd\u91cf\u5b50\u70b9\u7684\u53d1\u5149\u6027\u8d28\u548c\u989c\u8272\u53ef\u8c03\u7684\u673a\u7406<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a) \u5149\u81f4\u53d1\u5149\u8c31<\/p>\n

(b) CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS \u91cf\u5b50\u70b9\u5728\u4e0d\u540c\u6fc0\u53d1\u5f3a\u5ea6\u4e0b\u7684\u53d1\u5c04\u5f3a\u5ea6\uff0c\u6700\u5f3a\u7684\u53d1\u5149\u5cf0\u5728590nm\u9644\u8fd1\uff0c\u63d2\u56fe\u6240\u793a\u4e3aCIE 1931 \u8272\u54c1\u56fe\u548c\u8272\u5f69\u5750\u6807\u7cfb<\/p>\n

(c) CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u91cf\u5b50\u70b9\u7684\u84dd\u5149\u548c\u6a59\u5149\u5149\u5f3a\u6bd4\u7684\u53d8\u5316\u4f9d\u8d56\u6fc0\u53d1\u80fd\u91cf\u7684\u53ef\u80fd\u673a\u7406<\/p>\n

(d) \u7d2b\u5916-\u53ef\u89c1\u5149\u5438\u6536\u8c31(\u7ea2\u7ebf) \u548c\u5149\u81f4\u53d1\u5149\u8c31\u00a0(\u84dd\u7ebf)<\/p>\n

(e) \u6d53\u5ea6\u968fCdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u91cf\u5b50\u70b9\u7684\u6a59\u5149\/\u84dd\u5149\u5149\u5f3a\u6bd4\u7684\u53d8\u5316(\u63d2\u56fe\uff1a 365nm\u7684\u5165\u5c04\u5149\u7167\u5c04\u6d53\u5ea6\u5206\u522b\u4e3a 0.0015mg mL–<\/sup>1<\/sup>(1)\u30010.01mg mL–<\/sup>1<\/sup>\u00a0(2)\u548c\u00a00.5mg mL–<\/sup>1<\/sup>\u00a0(3)\u00a0\u7684CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u91cf\u5b50\u70b9\u6eb6\u6db2(f)\u00a0CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u7684RET\u673a\u7406\u793a\u610f\u56fe<\/p>\n

\u56fe3<\/b><\/strong>\u00a0\u542b\u6709\u4e0d\u540c\u6d53\u5ea6\u7684CdS\/ZnS\/ZnS:Mn<\/b><\/strong>2+<\/b><\/sup><\/strong>\/ZnS\u91cf\u5b50\u70b9\u6d53\u5ea6\u7684PDMS\u8584\u819c\u7684PL\u5149\u8c31<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a) 0.001 g mL\u22121<\/sup>\u3001(b) 0.1 g mL\u22121<\/sup>\u548c(c) 0.5 g mL\u22121<\/sup>(\u63d2\u56fe\u6240\u793a\u4e3a\u767d\u5149\uff08\u5de6\u56fe\uff09\u548c365nm\u7d2b\u5916\u5149\uff08\u53f3\u56fe\uff09\u7167\u5c04\u4e0b\u7684PDMS \u8584\u819c\u53d1\u5149\u7167\u7247\uff0c\u6bd4\u4f8b\u5c3a\u4e3a1 cm\u3002\u00a0PDMS\u8584\u819c\u5728\u4e0d\u540c\u6fc0\u53d1\u5f3a\u5ea6\u4e0b\u7684\u84dd\u5149\u548c\u6a59\u5149\u53d1\u5149\u5f3a\u5ea6<\/p>\n

(d-f) PDMS\u8584\u819c\u5728\u4e0d\u540c\u7684\u6fc0\u53d1\u529f\u7387\uff082.66 mJ cm\u22122<\/sup>\u30010.001 g mL\u22121<\/sup>, 7.56 mJ cm\u22122<\/sup>\u30010.1 g mL\u22121<\/sup>\u548c32.6 mJ cm\u22122<\/sup>\u30010.5 g mL\u22121<\/sup>\uff09\u4e0b\u8fbe\u5230\u4e86\u76f8\u540c\u7684\u6fc0\u53d1\u5f3a\u5ea6\u3002\u63d2\u56fe\u6240\u793a\u4e3a\u00a0CIE 1931 \u8272\u54c1\u56fe\u548c\u4e0d\u540c\u6fc0\u53d1\u529f\u7387\u4e0b\u7684PDMS\u7684\u5750\u6807<\/p>\n

\u56fe4<\/b><\/strong>\u00a0<\/b><\/strong>PDMS<\/b><\/strong>\u8584\u819c\u5ac1\u63a5\u5230<\/b><\/strong>CdS\/ZnS\/ZnS:Mn<\/b><\/strong>2+<\/b><\/sup><\/strong>\/ZnS<\/b><\/strong>\u91cf\u5b50\u70b9\u7684\u5236\u5907\u8fc7\u7a0b\u793a\u610f\u56fe\u53ca\u5176\u4f5c\u4e3a\u9632\u4f2a\u6750\u6599\u7684\u673a\u68b0\u548c\u53d1\u5149\u6027\u8d28<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a)\u4e0d\u540c\u529f\u7387\u7684\u6fc0\u5149\u5165\u5c04PDMS\u8584\u819c\u7684\u793a\u610f\u56fe\u548c\u7167\u7247<\/p>\n

(b) LPF\u5236\u5907\u8fc7\u7a0b<\/p>\n

(c\u3001d) LPF\u7684\u626d\u8f6c\u548c\u53ef\u4f38\u7f29\u6027\u80fd<\/p>\n

(e) LPF\u6750\u6599\u5728\u767d\u5149\u548c\u7d2b\u5916\u95ea\u5149\u706f\u7167\u5c04\u4e0b\u7684\u7167\u7247\u3002LPF\u5728\u767d\u5149\u4e0b\u603b\u662f\u900f\u660e\u7684\u3002\u7d2b\u5916\u5149\u7684\u529f\u7387\u901a\u8fc7ND\u6ee4\u5149\u5668\u540e\u8870\u51cf\u4e86\uff0c\u4f5c\u4e3a\u89c2\u6d4b\u7684LPF\u7684\u989c\u8272\u968f\u7740\u4e0d\u540c\u7684\u6fc0\u53d1\u5f3a\u5ea6\u800c\u53d8\u5316\uff0c\u4ee5\u6b64\u63d0\u4f9b\u9632\u4f2a\u4f5c\u7528<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u5728\u672c\u6587\u4e2d\uff0c\u7814\u7a76\u4eba\u5458\u7b2c\u4e00\u6b21\u5236\u5907\u51fa\u5ac1\u63a5\u5230CdS\/ZnS\/ZnS:Mn2+<\/sup>\/ZnS\u6838\/\u591a\u91cd\u91cf\u5b50\u70b9\u4e0a\u7684PDMS\u8584\u819c\uff0c\u8be5\u6750\u6599\u5177\u6709\u72ec\u7279\u7684\u4f9d\u8d56\u6fc0\u53d1\u529f\u7387\u7684\u53d1\u5149\u7279\u6027\u3002LPF\u6750\u6599\u540c\u65f6\u53d1\u84dd\u5149\u548c\u6a59\u5149\uff0c\u5149\u81f4\u53d1\u5149\u7684\u53ef\u8c03\u63a7\u6e90\u4e8e\u4e24\u79cd\u5149\u5f3a\u5ea6\u4e4b\u6bd4\u7684\u53d8\u5316\u3002\u6b64\u5916\uff0c\u886c\u5e95\uff08\u5df1\u70f7\u6216PDMS\uff09\u4e2d\u91cf\u5b50\u70b9\u7684\u6d53\u5ea6\u4e5f\u53ef\u4ee5\u8c03\u63a7\u53d1\u5149\u5f3a\u5ea6\uff0c\u5176\u4e2d\u7684\u673a\u7406\u5df2\u901a\u8fc7\u5b9e\u9a8c\u8bc1\u5b9e\u3002\u5ac1\u63a5\u5230\u63ba\u6742\u6838\/\u58f3\u91cf\u5b50\u70b9\u4e0a\u7684\u67d4\u6027LPF\u6750\u6599\uff0c\u5176\u53d1\u5149\u5f3a\u5ea6\u4f9d\u8d56\u5916\u754c\u7684\u6fc0\u53d1\u80fd\u91cf\u548c\u91cf\u5b50\u70b9\u6d53\u5ea6\uff0c\u8fd9\u5bf9\u4e8e\u6eb6\u6db2\u6cd5\u3001\u989c\u8272\u53ef\u8c03\u7684\u6750\u6599\u548c\u5668\u4ef6\u975e\u5e38\u91cd\u8981\uff0c\u5e76\u4e14\u5728\u6fc0\u5149\u9632\u4f2a\u65b9\u9762\u5177\u6709\u91cd\u5927\u5e94\u7528\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aPhotoluminescence Tuning in Stretchable PDMS\u00a0Film Grafted Doped Core\/Multishell Quantum Dots\u00a0for Anticounterfeiting<\/a><\/b><\/strong>\uff08Adv. Funct. Mater.,\u00a02017,\u00a0DOI: 10.1002\/adfm.201700051)\u00a0<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7535\u5b50\u7535\u5de5\u5b66\u672f\u7ec4\u6674\u96ea\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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