{"id":56683,"date":"2016-12-14T19:27:00","date_gmt":"2016-12-14T11:27:00","guid":{"rendered":"\/\/m.iemloyee.com\/?p=56683"},"modified":"2017-03-04T23:15:36","modified_gmt":"2017-03-04T15:15:36","slug":"jacs%ef%bc%9a%e9%92%a0%e7%a6%bb%e5%ad%90%e7%94%b5%e6%b1%a0%e8%b4%9f%e6%9e%81%e6%9d%90%e6%96%99%e5%8f%af%e9%80%86%e6%99%b6%e6%80%81%e7%9b%b8%e5%8f%98%e7%a0%94%e7%a9%b6%e5%8f%96%e5%be%97%e9%87%8d","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=56683","title":{"rendered":"JACS\uff1a\u94a0\u79bb\u5b50\u7535\u6c60\u8d1f\u6781\u6750\u6599\u53ef\u9006\u6676\u6001\u76f8\u53d8\u7814\u7a76\u91cd\u8981\u8fdb\u5c55"},"content":{"rendered":"<p><span style=\"color: #0000ff;\"><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/span><\/p>\n<p>\u4ee5\u9502\u79bb\u5b50\u7535\u6c60\u4e3a\u4ee3\u8868\u7684\u53ef\u5145\u7535\u7535\u6c60\u5df2\u7ecf\u5728\u4fbf\u643a\u7535\u5b50\u8bbe\u5907\u548c\u7535\u52a8\u6c7d\u8f66\u4e2d\u5f97\u5230\u4e86\u5e7f\u6cdb\u7684\u5e94\u7528\u3002\u7136\u800c\uff0c\u7535\u6c60\u8d1f\u6781\u6750\u6599\u5728\u9502\u79bb\u5b50\u5d4c\u5165\u548c\u89e3\u5d4c\u8fc7\u7a0b\u4e2d\u53d1\u751f\u7684\u5de8\u5927\u4f53\u79ef\u53d8\u5316\u4f1a\u5f15\u8d77\u7535\u6781\u6750\u6599\u7684\u574d\u584c\u548c\u975e\u6676\u5316\uff0c\u9020\u6210\u7535\u6c60\u6027\u80fd\u7684\u5168\u9762\u52a3\u5316\u3002\u5f53\u524d\u7535\u6c60\u8d1f\u6781\u6750\u6599\u7684\u7814\u7a76\u4e3b\u8981\u5173\u6ce8\u4e8e\u89e3\u51b3\u7535\u6781\u7ed3\u6784\u574d\u584c\u7684\u95ee\u9898\uff0c\u5e76\u53d6\u5f97\u4e86\u8f83\u5927\u7684\u8fdb\u5c55\uff0c\u4f46\u5bf9\u7535\u6781\u6750\u6599\u975e\u6676\u5316\u95ee\u9898\u4e00\u76f4\u7f3a\u4e4f\u6709\u6548\u7684\u89e3\u51b3\u65b9\u6848\u3002\u56e0\u94a0\u8d44\u6e90\u66f4\u4e3a\u5ec9\u4ef7\u3001\u6613\u5f97\u7684\u4f18\u52bf\uff0c\u94a0\u79bb\u5b50\u7535\u6c60\u6210\u4e3a\u66ff\u4ee3\u9502\u79bb\u5b50\u7535\u6c60\u7684\u9996\u9009\uff0c\u5e76\u6709\u671b\u5728\u667a\u80fd\u7535\u7f51\u7b49\u89c4\u6a21\u50a8\u80fd\u5e94\u7528\u4e2d\u53d1\u6325\u5de8\u5927\u4f5c\u7528\u3002<\/p>\n<p>\u4f46\u662f\u94a0\u79bb\u5b50\u7684\u534a\u5f84\u4e3a1.02 \u00c5\uff0c\u6bd4\u9502\u79bb\u5b50\u534a\u5f840.76 \u00c5\u5927\u7ea634%\uff0c\u56e0\u6b64\u94a0\u79bb\u5b50\u7535\u6781\u6750\u6599\u5728\u5145\u653e\u7535\u8fc7\u7a0b\u4e2d\u4f1a\u4ea7\u751f\u66f4\u5927\u7684\u4f53\u79ef\u53d8\u5316\uff0c\u8fd9\u4f7f\u5f97\u7535\u6781\u7ed3\u6784\u574d\u584c\u548c\u975e\u6676\u5316\u7684\u95ee\u9898\u66f4\u4e3a\u4e25\u91cd\u3002\u540c\u65f6\uff0c\u4ece\u52a8\u529b\u5b66\u89d2\u5ea6\u6765\u770b\uff0c\u5c3a\u5bf8\u8f83\u5927\u7684\u94a0\u79bb\u5b50\u5728\u8d1f\u6781\u6750\u6599\u4e2d\u7684\u5d4c\u5165\/\u89e3\u5d4c\u901f\u5ea6\u8981\u6bd4\u9502\u79bb\u5b50\u66f4\u6162\u3002\u8fd9\u4e9b\u4e0d\u5229\u56e0\u7d20\u4f7f\u94a0\u79bb\u5b50\u7535\u6c60\u5728\u5faa\u73af\u6027\u80fd\u548c\u529f\u7387\u6027\u80fd\u7684\u63d0\u5347\u66f4\u5177\u6311\u6218\u3002\u800c\u5bf9\u89c4\u6a21\u50a8\u80fd\u6765\u8bf4\uff0c\u7535\u6c60\u7684\u5faa\u73af\u5bff\u547d\u548c\u529f\u7387\u6070\u662f\u6700\u4e3a\u5173\u952e\u7684\u8981\u7d20\u3002<\/p>\n<p><span style=\"color: #0000ff;\"><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/span><\/p>\n<p>\u8fd1\u65e5\uff0c\u540c\u6d4e\u5927\u5b66\u7684\u6768\u91d1\u864e\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u3001\u590d\u65e6\u5927\u5b66\u7684\u8d75\u4e1c\u5143\u9662\u58eb\uff08\u901a\u8baf\u4f5c\u8005\uff09\u548c\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66\u7684\u5f6d\u6210\u4fe1\u535a\u58eb\uff08\u901a\u8baf\u4f5c\u8005\uff09\u5728\u94a0\u79bb\u5b50\u7535\u6c60\u8d1f\u6781\u6750\u6599\u53ef\u9006\u6676\u6001\u76f8\u53d8\u7814\u7a76\u4e2d\u53d6\u5f97\u4e86\u91cd\u8981\u8fdb\u5c55\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201c<em>Direct Superassemblies of Freestanding Metal-Carbon Frameworks Featuring Reversible Crystalline-Phase Transformation for Electrochemical Sodium Storage<\/em>\u201d\u4e3a\u9898\u5728\u7ebf\u53d1\u8868\u5728\u300aJournal of The American Chemical Society\u300b\uff08JACS, <a href=\"http:\/\/pubs.acs.org\/doi\/full\/10.1021\/jacs.6b10782\">2016, DOI: 10.1021\/jacs.6b10782<\/a>\uff0c\u5f71\u54cd\u56e0\u5b50\u4e3a13.038\uff09\u4e0a\u3002\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a\u590d\u65e6\u5927\u5b66\u5b54\u5f6a\u7814\u7a76\u5458\uff08\u9752\u5e74\u5343\u4eba\uff09\u548c\u540c\u6d4e\u5927\u5b66\u535a\u58eb\u7814\u7a76\u751f\u7956\u8fde\u6d77\u3002<\/p>\n<p><span style=\"color: #0000ff;\"><strong>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/span><\/p>\n<p><strong>\u56fe<\/strong><strong>1<\/strong><strong>\u9650\u57df\u8d85\u7ec4\u88c5\u6c14\u76f8\u6c89\u79ef\u6cd5\u4e2d\u91d1\u5c5e<\/strong><strong>&#8211;<\/strong><strong>\u78b3\u9aa8\u67b6\u590d\u5408\u819c\u5f62\u6210\u673a\u5236\u3002<\/strong><\/p>\n<p><a href=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/1-4.jpeg\"><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-56753\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/1-4.jpeg\" alt=\"1\" width=\"650\" height=\"258\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/1-4.jpeg 650w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/1-4-300x119.jpeg 300w\" sizes=\"(max-width: 650px) 100vw, 650px\" \/><\/a><\/p>\n<p>\uff08a\uff09\u9650\u57df\u8d85\u7ec4\u88c5\u6c14\u76f8\u6c89\u79ef\u6cd5\u4e2d\u91d1\u5c5e-\u78b3\u9aa8\u67b6\u590d\u5408\u819c\u5f62\u6210\u673a\u5236\u793a\u610f\u56fe\uff1b<\/p>\n<p>\uff08b\uff09\u5408\u6210\u8def\u7ebf\u56fe\uff1b\uff08c\uff09\u77f3\u82f1\u7ba1\u4e2d\u590d\u5408\u819c\u793a\u610f\u56fe\uff1b<\/p>\n<p>\uff08d\uff09\u590d\u5408\u819c\u626b\u63cf\u7535\u955c\u56fe\uff1b\uff08e-i\uff09\u590d\u5408\u819c\u5728\u4e0d\u540c\u5f2f\u66f2\u548c\u52a0\u5de5\u5904\u7406\u65f6\u7684\u5149\u5b66\u7167\u7247\u3002<\/p>\n<p>\u7814\u7a76\u8005\u91c7\u7528\u4e00\u7cfb\u5217\u542b\u91d1\u5c5e\u4e2d\u5fc3\u7684<strong>\u591a\u82ef\u57fa\u91d1\u5c5e\u5206\u5b50<\/strong>\u4f5c\u4e3a\u5355\u4e00\u53cd\u5e94\u6e90\uff0c\u5229\u7528\u82ef\u73af\u5e73\u9762\u7684<strong>\u03c0-\u03c0<\/strong><strong>\u7ec4\u88c5<\/strong>\u4f5c\u7528\uff08\u56fe1a\uff09\uff0c\u5728\u5c01\u95ed\u7684\u771f\u7a7a\u77f3\u82f1\u7ba1\u4e2d\u901a\u8fc7\u6e29\u63a7\u7a0b\u5e8f\u5c06\u591a\u82ef\u57fa\u5206\u5b50\u5728\u7ba1\u58c1\u539f\u4f4d\u5206\u89e3\u3001\u6c89\u79ef\uff0c\u5f62\u6210\u91d1\u5c5e\u6216\u5408\u91d1\uff08Sb, Bi, Sn, Ge, Sb<sub>89<\/sub>Bi<sub>11<\/sub>\uff09\u7eb3\u7c73\u70b9\uff08\u76f4\u5f84 &lt; 5\u7eb3\u7c73\uff09\u5747\u5300\u5206\u6563\u4e8e\u77f3\u58a8\u5316\u78b3\u9aa8\u67b6\u4e2d\u7684\u4e8c\u5143\u91d1\u5c5e\/\u78b3\u7eb3\u7c73\u590d\u5408\u819c\uff08\u56fe1a\uff0cb\uff09\u3002\u6240\u5236\u5907\u7684\u590d\u5408\u819c\u5177\u6709\u5f88\u597d\u7684\u53ef\u52a0\u5de5\u6027\u80fd\uff08\u56fe1c-g\uff09\uff0c\u4e5f\u5177\u6709\u4e0e\u77f3\u58a8\u76f8\u5f53\u7684\u5bfc\u7535\u6027\uff0c\u53ef\u4e0d\u9700\u5bfc\u7535\u5242\u76f4\u63a5\u7528\u4f5c\u94a0\u79bb\u5b50\u7535\u6c60\u7684\u7535\u6781\u6750\u6599\uff08\u56fe1h\uff0ci\uff09\u3002\u4ee5Sb\/\u78b3\u590d\u5408\u7535\u6781\u4e3a\u4f8b\uff0c\u56e0\u4e3a\u77f3\u58a8\u5316\u78b3\u7eb3\u7c73\u7247\u5bf9Sb\u7eb3\u7c73\u70b9\u7684\u6709\u6548\u9694\u79bb\u4f5c\u7528\uff0cSb\u7eb3\u7c73\u70b9\u5728\u94a0\u5316\uff08\u975e\u6676\u5316\uff09\u540e\u80fd\u4e00\u76f4\u4fdd\u6301\u8d85\u5c0f\u7684\u7eb3\u7c73\u5c3a\u5bf8\uff0c\u8fd9\u4e0d\u4ec5\u5728\u70ed\u529b\u5b66\u4e0a\u8d4b\u4e88\u7eb3\u7c73\u70b9\u66f4\u9ad8\u7684\u8868\u9762\u80fd\u91cf\u3001\u9a71\u52a8\u5176\u5f62\u6210\u4f4e\u80fd\u6001\u7684\u6676\u6001\u76f8\uff0c\u800c\u4e14\u5728\u52a8\u529b\u5b66\u4e0a\u4e5f\u53ef\u4ee5\u907f\u514d\u539f\u5b50\u7ed3\u6676\u8fc7\u7a0b\u4e2d\u7684\u8fdc\u8ddd\u79bb\u6269\u6563\u548c\u8bc6\u522b\u7684\u52bf\u5792\uff08\u56fe2\uff09\u3002\u56e0\u6b64\uff0c\u7535\u6781\u6d3b\u6027\u6750\u6599\u5728\u6bcf\u6b21\u5145\u653e\u7535\u5faa\u73af\u540e\u90fd\u80fd\u5feb\u901f\u4ece\u975e\u6676\u6001\u6062\u590d\u6676\u6001\uff0c\u8fd9\u79cd\u4e0d\u5bfb\u5e38\u7684\u53ef\u9006\u6676\u6001\u76f8\u53d8\u4fdd\u8bc1\u4e86\u7535\u6781\u8d85\u9ad8\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u9ad8\u529f\u7387\u6027\u80fd\uff0c\u5982\u5373\u4f7f\u57285C\u548c7.5C\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af5000\u6b21\u540e\uff0c\u7535\u6c60\u7684\u5bb9\u91cf\u51e0\u4e4e\u6ca1\u6709\u8870\u51cf\uff0c\u7535\u6781\u6750\u6599\u7ed3\u6784\u4e5f\u4f9d\u7136\u6709\u6548\u4fdd\u6301\u3002\u8fd9\u4e9b\u7ed3\u679c\u8868\u660e\uff0c\u91d1\u5c5e\u7eb3\u7c73\u70b9\/\u78b3\u9aa8\u67b6\u590d\u5408\u7535\u6781\u80fd\u591f\u540c\u65f6\u6291\u5236\u7535\u6781\u7ed3\u6784\u574d\u584c\u548c\u975e\u6676\u5316\u3002\u8be5\u7814\u7a76\u5bf9\u53d1\u5c55\u957f\u5bff\u547d\u3001\u9ad8\u529f\u7387\u7684\u94a0\u79bb\u5b50\u7535\u6c60\u5177\u6709\u91cd\u8981\u7684\u501f\u9274\u610f\u4e49\u3002<\/p>\n<p><strong>\u56fe<\/strong><strong>2 Sb-C\u590d\u5408\u819c\u6750\u6599\u5728\u7279\u5b9a\u5145\u653e\u7535\u7535\u52bf\u4e0b\u7684\u4e94\u79cd\u6676\u76f8\u7ed3\u6784<\/strong><\/p>\n<p><a href=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/2-4.jpeg\"><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-56754\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/2-4.jpeg\" alt=\"2\" width=\"650\" height=\"608\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/2-4.jpeg 650w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/2-4-300x281.jpeg 300w\" sizes=\"(max-width: 650px) 100vw, 650px\" \/><\/a><\/p>\n<p>\uff08a\uff09\u4e0d\u540c\u6676\u76f8\/\u6676\u4f53\u7ed3\u6784\uff08Sb\uff0cNaSb\uff0cNa3Sb\uff09\u5728\u7279\u5b9a\u5145\u653e\u7535\u7535\u538b\u4e0b\u5faa\u73af\u671f\u95f4\uff0cSb-C\u9aa8\u67b6\u819c\u9633\u6781\u7684\u4e94\u79cd\u5173\u952e\u72b6\u6001\u793a\u610f\u56fe\uff1b\uff08b,c\uff09\u57281000\u6b21\u5faa\u73af, 7.5C\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u76f8\u5e94\u7684SAED\u56fe\u3002<\/p>\n<p><strong>\u56fe<\/strong><strong>3 Sb-C\u9aa8\u67b6\u590d\u5408\u819c\u7535\u6781\u5728\u5145\u653e\u7535\u5faa\u73af\u8fc7\u7a0b\u4e2d\u53ef\u80fd\u7684\u53ef\u9006\u6676\u6001\u76f8\u53d8\u673a\u7406<\/strong><\/p>\n<p><a href=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/3-3.jpeg\"><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-56755\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/3-3.jpeg\" alt=\"3\" width=\"650\" height=\"429\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/3-3.jpeg 650w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/3-3-300x198.jpeg 300w\" sizes=\"(max-width: 650px) 100vw, 650px\" \/><\/a><a href=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/\u5c01\u9762.png\"><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-56756\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/\u5c01\u9762.png\" alt=\"%e5%b0%81%e9%9d%a2\" width=\"554\" height=\"401\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/\u5c01\u9762.png 554w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/12\/\u5c01\u9762-300x217.png 300w\" sizes=\"(max-width: 554px) 100vw, 554px\" \/><\/a><\/p>\n<p><span style=\"color: #0000ff;\"><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/span><\/p>\n<p>\u901a\u8fc7\u91c7\u7528\u7535\u6781\u6d3b\u6027\u6750\u6599\u5728\u6bcf\u6b21\u5145\u653e\u7535\u5faa\u73af\u540e\u90fd\u80fd\u5feb\u901f\u4ece\u975e\u6676\u6001\u6062\u590d\u6676\u6001\uff0c\u8fd9\u79cd\u4e0d\u5bfb\u5e38\u7684\u53ef\u9006\u6676\u6001\u76f8\u53d8\u4fdd\u8bc1\u4e86\u7535\u6781\u8d85\u9ad8\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u9ad8\u529f\u7387\u6027\u80fd\uff0c\u5982\u5373\u4f7f\u57285C\u548c7.5C\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af5000\u6b21\u540e\uff0c\u7535\u6c60\u7684\u5bb9\u91cf\u51e0\u4e4e\u6ca1\u6709\u8870\u51cf\uff0c\u7535\u6781\u6750\u6599\u7ed3\u6784\u4e5f\u4f9d\u7136\u6709\u6548\u4fdd\u6301\u3002\u8fd9\u4e9b\u7ed3\u679c\u8868\u660e\uff0c\u91d1\u5c5e\u7eb3\u7c73\u70b9\/\u78b3\u9aa8\u67b6\u590d\u5408\u7535\u6781\u80fd\u591f\u540c\u65f6\u6291\u5236\u7535\u6781\u7ed3\u6784\u574d\u584c\u548c\u975e\u6676\u5316\u3002\u8be5\u7814\u7a76\u5bf9\u53d1\u5c55\u957f\u5bff\u547d\u3001\u9ad8\u529f\u7387\u7684\u94a0\u79bb\u5b50\u7535\u6c60\u5177\u6709\u91cd\u8981\u7684\u501f\u9274\u610f\u4e49\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a<\/strong><a href=\"http:\/\/pubs.acs.org\/doi\/full\/10.1021\/jacs.6b10782#showFigures\" target=\"_blank\"><strong>Direct Superassemblies of Freestanding Metal\u2013Carbon Frameworks Featuring Reversible Crystalline-Phase Transformation for Electrochemical Sodium 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