{"id":51000,"date":"2016-11-12T14:00:43","date_gmt":"2016-11-12T06:00:43","guid":{"rendered":"\/\/m.iemloyee.com\/?p=51000"},"modified":"2016-11-11T19:58:30","modified_gmt":"2016-11-11T11:58:30","slug":"adv-energy-mater-%ef%bc%9a%e8%b6%85%e7%96%8f%e6%b0%b4%e5%87%86%e5%9b%ba%e4%bd%93%e7%94%b5%e8%a7%a3%e8%b4%a8%e6%8f%90%e9%ab%98li-o2%e7%94%b5%e6%b1%a0%e6%bd%ae%e6%b9%bf%e7%8e%af%e5%a2%83%e4%b8%ad","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=51000","title":{"rendered":"Adv. Energy Mater.\uff1a\u8d85\u758f\u6c34\u51c6\u56fa\u4f53\u7535\u89e3\u8d28\u63d0\u9ad8Li-O2\u7535\u6c60\u6f6e\u6e7f\u73af\u5883\u4e2d\u5b89\u5168\u6027\u548c\u5faa\u73af\u5bff\u547d"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/span><\/p>\n

\u9502\u7a7a\u7535\u6c60<\/strong><\/span>\uff08\u4e5f\u573a\u88ab\u79f0\u4e3aLi-O2\u7535\u6c60\uff0c\u53ef\u53c2\u8003\u6750\u6599\u725b\u6587\u7ae0\uff1a\u9502\u7a7a\u7535\u6c60\u4e13\u9898\u4e4b\u53cd\u5e94\u539f\u7406\u7814\u7a76\u8fdb\u5c55<\/strong><\/a>\u3011\u57fa\u4e8e\u91d1\u5c5eLi\u548cO2\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u65f6\uff0c\u5316\u5b66\u80fd\u8f6c\u6362\u7535\u80fd\u7684\u7535\u6c60\u3002\u9502\u7535\u5927\u725bPeter G. Bruce<\/span><\/strong>\uff0c\u5bf9\u9502\u786b\u7535\u6c60\u548c\u9502\u7a7a\u7535\u6c60\u66fe\u505a\u4e86\u8f83\u4e3a\u8be6\u5c3d\u7684\u5bf9\u6bd4[1<\/sup>],\u540c\u65f6\u5305\u62ec\u9502\u6c27\u3001\u9502\u786b\u3001\u9502\u79bb\u5b50\u7535\u6c60\u3001\u950c\u7a7a\u7535\u6c60\u6bd4\u5bb9\u91cf\u7684\u5bf9\u6bd4\u3002\u548c\u9502\u786b\u7535\u6c60\u76f8\u4f3c\uff0cLi-O2\u7535\u6c60\u5177\u6709\u76f8\u5f53\u9ad8\u80fd\u91cf\u5bc6\u5ea6(\u22483500 W h kg\u22121<\/sup>)\uff0c\u6210\u4e3a\u5f53\u4e0b\u7684\u7814\u7a76\u70ed\u70b9\u3002<\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/span><\/p>\n

11\u67083\u65e5\uff0cAdvanced Energy Materials\u5728\u7ebf\u53d1\u8868\u9898\u4e3a\u201c\u4e00\u79cd\u7528\u4e8eLi-O2<\/sub>\u7535\u6c60\u7684\u8d85\u758f\u6c34\u51c6\u56fa\u4f53\u7535\u89e3\u8d28\uff1a\u6f6e\u6e7f\u6c14\u6c1b\u4e2d\u6539\u5584\u5b89\u5168\u6027\u548c\u5faa\u73af\u5bff\u547d\u201d\uff08A Super-Hydrophobic Quasi-Solid Electrolyte for Li-O2 Battery with Improved Safety and Cycle Life in Humid Atmosphere\uff09\u7684\u7814\u7a76\u8bba\u6587[3<\/sup>]\uff0c\u5357\u4eac\u5927\u5b66\u5468\u8c6a\u614e<\/span>\u6559\u6388\uff0c\u65e5\u672c\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\uff08<\/strong>AIST<\/strong>\uff09<\/strong>Dr. J. Yi<\/strong>\u4e3a\u5171\u540c\u901a\u8baf\u4f5c\u8005<\/strong>\u3002<\/p>\n

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\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/span><\/p>\n

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\u56fe1\u00a0<\/strong>\u7535\u6c60\u5728\u6f6e\u6e7f\u5927\u6c14\u4e2d\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"figure3\"<\/p>\n

a\u3001b)\u00a0\u7535\u89e3\u8d28a) LiSICON\u819c\u548cb) SHQSE\u819c\u3002<\/p>\n

\u56fe2\u00a0<\/strong>SHQSE<\/strong>\u819c\u7684\u5fae\u89c2\u5f62\u8c8c\u548c\u5b8f\u89c2\u5c3a\u5bf8\u53ca\u5176\u70ed\u7a33\u5b9a\u6027\u3002<\/strong><\/p>\n

\"figure4\"<\/p>\n

a\uff0cb\uff09SHQSE\u819c\u5728a\uff09\u5e73\u5766\u548cb\uff09\u5f2f\u66f2\u6761\u4ef6\u4e0b\u7684\u7167\u7247\u56fe\u50cf\u3002<\/p>\n

c\uff09SHQSE\u819c\u7684SEM\u56fe\u50cf\u3002<\/p>\n

d\uff09SHQSE\u819c\u7684\u70ed\u91cd\u5206\u6790\uff08TGA\uff09\uff0c\u5728\u6d41\u52a8\u7a7a\u6c14\u4e0b\uff0c10\u2103 min-1<\/sup>\u3002<\/p>\n

e\uff0cf\uff09SHQSE\u819c\u5728120\u2103\u5904\u74061\u5c0f\u65f6e\uff09\u4e4b\u524d\u548cf\uff09\u4e4b\u540e\u7684\u7167\u7247\u56fe\u50cf\u3002<\/p>\n

\u56fe3<\/strong>\u00a0SHQSE<\/strong>\u819c\u7684\u63a5\u89e6\u89d2\u548c\u758f\u6c34\u6027\u5b9e\u9a8c\u3002<\/strong><\/p>\n

\"figure5\"<\/p>\n

a\uff09H2O\u63a5\u89e6\u89d2\u548cSHQSE\u819c\u4e0aH2O\u6ef4\u7684\u76f8\u5e94\u5f62\u72b6\u3002<\/p>\n

b\uff0cc\uff09\u4e0d\u540c\u65f6\u95f4\u4e0b\u73bb\u7483\u7ea4\u7ef4\uff08GF\uff09\uff0c\u975e\u7ec7\u9020\u7247\u6750\u548cSHQSE\u819c\u7684\u758f\u6c34\u8bd5\u9a8c\u3002<\/p>\n

d\uff0ce\uff09\u4f7f\u7528\u6eb6\u89e3\u7684FeCl3<\/sub>\u4f5c\u4e3a\u989c\u8272\u6307\u793a\u5242\u76842mL H2O\u7684\u6e17\u900f\u5b9e\u9a8c\uff1ad\uff09GF\u819c\u548ce\uff09SHQSE\u819c\u3002<\/p>\n

\u56fe4<\/strong>\u00a0<\/strong>\u963b\u6297\uff0c<\/strong>LSV<\/strong>\u4e0e\u6052\u7535\u6d41\u5faa\u73af\u6d4b\u8bd5\u3002<\/strong><\/p>\n

\"figure6\"<\/p>\n

a\uff09\u4e0d\u9508\u94a2\uff08SS\uff09\/ SHQSE \/ SS\u7535\u6c60\u7ed3\u6784\uff0c\u901a\u8fc7\u7535\u5316\u5b66\u963b\u6297\u8c31\uff08EIS\uff09\u6d4b\u91cf\u7814\u7a76\u79bb\u5b50\u7535\u5bfc\u7387\uff0cSHQSE\u7684\u5948\u594e\u65af\u7279\u56fe\u3002<\/p>\n

b\uff09\u626b\u901f1 mV s-1<\/sup>\u65f6SHQSE\u7684LSV\u3002<\/p>\n

c\uff09\u6052\u7535\u6d41\u5faa\u73af\u6765\u7814\u7a76Li\u6eb6\u89e3\/\u6c89\u79ef\u8fc7\u7a0b\u7684\u7a33\u5b9a\u6027\u3002\u7535\u6d41\u5bc6\u5ea60.05 mA cm-2<\/sup>\uff0c\u95f4\u9694\u65f6\u95f430\u5206\u949f\u3002<\/p>\n

\u56fe<\/strong>7 <\/strong>\u7535\u6c60\u6027\u80fd\u6d4b\u8bd5<\/strong><\/p>\n

\"figure7\"<\/p>\n

a\uff0cb\uff09\u591a\u6b21\u5faa\u73af\u7684\u5145\u653e\u7535\u7535\u538b\u66f2\u7ebf\uff0ca\uff0cSHQSE\u548cb\uff09\u6db2\u4f53\u7535\u89e3\u8d28\u3002<\/p>\n

c)\u7535\u6c60\u5145\u653e\u7535\u5728150\u5468\u671f\u5185\u7684\u5faa\u73af\u6027\u80fd\u548c\u5e93\u4ed1\u6548\u7387\uff0c\u7535\u6d41\u5bc6\u5ea6500 mA g-2<\/sup>\u3002<\/p>\n

\u3010\u5c55\u671b\u3011<\/strong><\/span><\/p>\n

\u8d85\u758f\u6c34\u6027\u7684\u51c6\u56fa\u4f53\u7535\u89e3\u8d28\u8868\u73b0\u51fa\u5f3a\u8010\u70ed\u6027\uff08\u65e0\u660e\u663e\u5206\u89e3\u4f4e\u4e8e230\u2103\uff09\uff0c\u9ad8\u7535\u5316\u5b66\u7a33\u5b9a\u6027\uff08>5.5V\uff09\uff0c\u79bb\u5b50\u7535\u5bfc\u7387\uff080.91\u00d710-3<\/sup> S cm-1<\/sup>\uff09\u548c\u8d85\u758f\u6c34\u6027\uff08\u63a5\u89e6\u89d2>150\u00b0\uff09\uff0c\u5b9e\u73b0Li-O2<\/sub>\u7535\u6c60\u5728\u6f6e\u6e7f\u7684\u5927\u6c14\u4e2d\u5de5\u4f5c\u7684\u5b89\u5168\u6027\u548c\u957f\u5bff\u547d\u3002\u7ed3\u679c\u8868\u660e\u8d85\u758f\u6c34\u6027\u8d28\u7684\u56fa\u6001\u7535\u89e3\u8d28\u53ef\u4ee5\u963b\u6b62H2<\/sub>O\u4e0e\u91d1\u5c5e\u9633\u6781Li\u4ea4\u53c9\u53cd\u5e94\uff0c\u4e3a\u9502\u7a7a\u7535\u6c60\u7684\u672a\u6765\u5e94\u7528\u8fdb\u884c\u4e86\u6709\u76ca\u63a2\u7d22\uff0c\u4f46Li-O2<\/sub>\u7535\u6c60\u8981\u4f5c\u4e3a\u7535\u52a8\u8f66\u8f86\u7684\u7535\u6e90\uff0c\u8fd8\u9700\u8981\u52aa\u529b\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>A Super-Hydrophobic Quasi-Solid Electrolyte for Li-O2 Battery with Improved Safety and Cycle Life in Humid Atmosphere<\/a> (Adv. Energy Mater. 2016, 1601759\uff0cDOI: 10.1002\/aenm.201601759)<\/p>\n

\u901a\u8baf\u4f5c\u8005<\/strong>\u5468\u8c6a\u614e<\/strong>\u6559\u6388\u7b80\u4ecb\uff1a<\/p>\n

\u5468\u8c6a\u614e<\/strong>\u6559\u6388\uff0c\u5357\u4eac\u5927\u5b66\u73b0\u4ee3\u5de5\u7a0b\u4e0e\u5e94\u7528\u79d1\u5b66\u5b66\u9662\u6559\u6388\u3001\u535a\u58eb\u751f\u5bfc\u5e08\uff0c\u80fd\u6e90\u79d1\u5b66\u4e0e\u5de5\u7a0b\u7cfb\u4e3b\u4efb\u3002\u4e2d\u7ec4\u90e8\u5343\u4eba\u8ba1\u5212\u4e13\u5bb6\uff0c\u6559\u80b2\u90e8\u957f\u6c5f\u6559\u6388\uff0c\u65e5\u672c\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\u4e3b\u4efb\u7814\u7a76\u5458\u3001\u80fd\u6e90\u90e8\u95e8\u9996\u5e2d\u79d1\u5b66\u5bb6\uff08\u517c\uff09\uff0c\u4e1c\u4eac\u5927\u5b66\u5de5\u5b66\u9662\u5ba2\u5ea7\u6559\u6388\uff0c\u56fd\u5bb6\u91cd\u5927\u7814\u7a76\u8ba1\u5212\u9879\u76ee\uff08973\uff09\u9996\u5e2d\u79d1\u5b66\u5bb6\u3002\u4f5c\u4e3a\u9879\u76ee\u8d1f\u8d23\u4eba\u4e3b\u6301\u8fc7NEDO\uff0cJST\uff0cJSPS\u7b49\u65e5\u672c\u56fd\u5bb6\u5927\u578b\u7814\u7a76\u9879\u76ee\u3002\u5728\u5316\u5b66\uff0c\u6750\u6599\u53ca\u80fd\u6e90\u9886\u57df\u6743\u5a01\u5b66\u672f\u520a\u7269\u5982Nature Materials\uff0cNature Communications\uff0cAngew Chemie, JACS, Adv Mater, Nano Letter, ACS Nano, Adv Fun Mater, Adv Energy Mater, Energy Enviroment Sci.\u7b49\u520a\u7269\u4e0a\u53d1\u8868\u7814\u7a76\u8bba\u6587\u8d85\u8fc7230\u7bc7\uff0c\u53d1\u8868\u6587\u7ae0\u4ed6\u5f15\u8d856000\u6b21\uff0c\u5176\u4e2d\u5355\u7bc7\u88ab\u5f15\u7528\u8d85100\u6b21\u7684\u670916\u7bc7\uff0cH\u56e0\u5b5045\u3002\u5df2\u53d6\u5f97\u4e13\u522918\u4ef6\uff1b\u8f6c\u8ba9\u6280\u672f\uff0c\u5e76\u88ab\u63a8\u5411\u4ea7\u4e1a\u7684\u67092\u9879\uff1b\u4e3b\u6301\u4e0e\u65e5\u672c\u7684\u6c7d\u8f66\u3001\u5316\u5de5\u3001\u7535\u529b\u7b49\u9886\u57df\u77e5\u540d\u516c\u53f8\u5408\u4f5c\u7684\u7814\u53d1\u9879\u76ee\u591a\u9879\u3002\u76ee\u524d\u672c\u5b9e\u9a8c\u5ba4\u5728\u7814\u9879\u76ee\u6709\u79d1\u6280\u90e8973\u9879\u76ee\uff08\u9996\u5e2d\uff09\uff0c\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\uff0c\u6c5f\u82cf\u7701\u79d1\u6280\u5385\u9879\u76ee\uff0c\u4f01\u4e1a\u5408\u4f5c\u9879\u76ee\u7b49\u3002<\/p>\n

\u53c2\u8003\u6587\u732e\uff1a<\/strong><\/span><\/p>\n

1\uff0cBruce PG, Freunberger SA, Hardwick LJ, Tarascon J-M. Li-O2 and Li-S batteries with high energy storage<\/a>. Nature materials<\/em> 2012, 11<\/strong>(1):<\/strong> 19-29.<\/p>\n

2\uff0cLiu T, Leskes M, Yu W, Moore AJ, Zhou L, Bayley PM, et al.<\/em> Cycling Li-O2 batteries via LiOH formation and decomposition.<\/a> Science<\/em> 2015, 350<\/strong>(6260):<\/strong> 530-533.<\/p>\n

3\uff0cWu S, Yi J, Zhu K, Bai S, Liu Y, Qiao Y, et al<\/em>.<\/em> A Super-Hydrophobic Quasi-Solid Electrolyte for Li-O2 Battery with Improved Safety and Cycle Life in Humid Atmosphere.<\/a> Advanced Energy Materials<\/em> 2016:<\/strong> DOI: 10.1002\/aenm.201601759.<\/p>\n

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