{"id":40996,"date":"2016-09-15T06:30:58","date_gmt":"2016-09-14T22:30:58","guid":{"rendered":"\/\/m.iemloyee.com\/?p=40996"},"modified":"2016-09-15T10:20:35","modified_gmt":"2016-09-15T02:20:35","slug":"%e4%b8%ad%e7%a7%91%e5%a4%a7adv-mater-%e6%9e%84%e7%ad%91%e4%b8%89%e7%bb%b4%e5%85%b1%e4%bb%b7%e8%bf%9e%e6%8e%a5%e7%9a%84sp2%e6%9d%82%e5%8c%96%e7%a2%b3%e7%ba%b3%e7%b1%b3%e6%9d%90%e6%96%99%e7%94%a8","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=40996","title":{"rendered":"Adv. Mater. \u4e2d\u79d1\u5927\u6784\u7b51\u65b0\u578b\u4e09\u7ef4\u5171\u4ef7\u8fde\u63a5\u7684sp2\u6742\u5316\u7eb3\u7c73\u78b3\u7528\u4e8e\u9502\u786b\u7535\u6c60\u6b63\u8d1f\u6781\u96c6\u6d41\u4f53"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b>
\n\u9502\u786b\u7535\u6c60\u7531\u4e8e\u6781\u9ad8\u7684\u7406\u8bba\u5bb9\u91cf(2567 w h kg-1<\/sup>)\u6210\u4e3a\u76ee\u524d\u9502\u57fa\u7535\u6c60\u7814\u7a76\u7684\u91cd\u70b9\u4e4b\u4e00\u3002\u76ee\u524d\uff0c\u9502\u786b\u7535\u6c60\u9762\u4e34\u7684\u4e3b\u8981\u95ee\u9898\u5305\u62ec\uff1a1) \u786b\u6b63\u6781\u7535\u5bfc\u7387\u4f4e(5 \u00d7 10-30 <\/sup>S cm-1<\/sup>)\u5bfc\u81f4\u500d\u7387\u6027\u80fd\u5dee\uff1b2)\u591a\u786b\u5316\u9502\u6eb6\u4e8e\u7535\u89e3\u6db2\u5bfc\u81f4\u5faa\u73af\u7a33\u5b9a\u6027\u5dee\uff1b3)\u91d1\u5c5e\u9502\u8d1f\u6781\u957f\u5faa\u73af\u540e\u4ea7\u751f\u679d\u6676\u5f15\u8d77\u5b89\u5168\u9690\u60a3\u3002\u9488\u5bf9\u786b\u6b63\u6781\u7684\u95ee\u9898\uff0c\u4e3b\u8981\u901a\u8fc7\u5236\u5907\u78b3\/\u786b\u590d\u5408\u6750\u6599\u7684\u601d\u8def\u6765\u89e3\u51b3\uff0c\u5229\u7528\u78b3\u6750\u6599\u53ef\u63a7\u7684\u7ed3\u6784\u3001\u4f18\u5f02\u7684\u5bfc\u7535\u80fd\u529b\u548c\u5316\u5b66\u7a33\u5b9a\u6027\u6765\u63d0\u9ad8\u786b\u7684\u5bfc\u7535\u80fd\u529b\uff0c\u5e76\u9650\u5236\u591a\u786b\u5316\u7269\u7684\u6eb6\u51fa\u3002\u800c\u9502\u8d1f\u6781\u95ee\u9898\u7684\u89e3\u51b3\u601d\u8def\u5305\u62ec\uff1a\u7535\u89e3\u6db2\u6dfb\u52a0\u5242\uff0c\u5f62\u6210\u9ad8\u6a21\u91cf\u7684\u56fa\u6001\u7535\u89e3\u8d28\u548c\u4eba\u5de5\u6784\u7b51\u7269\u7406\u4fdd\u62a4\u5c42\u7b49\uff0c\u6765\u6291\u5236\u91d1\u5c5e\u9502\u679d\u6676\u7684\u751f\u957f\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u6700\u8fd1\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u5b63\u6052\u661f\u6559\u6388\u8bfe\u9898\u7ec4\u8bbe\u8ba1\u4e86\u7531sp2<\/sup>\u6742\u5316\u78b3\u7eb3\u7c73\u7ed3\u6784\u901a\u8fc7\u5171\u4ef7\u8fde\u63a5\u5f62\u6210\u7684\u4e09\u7ef4\u5bfc\u7535\u7f51\u7edc\uff0c\u6210\u529f\u7684\u5c06\u78b3\u7eb3\u7c73\u7ba1\u9635\u5217\u901a\u8fc7C-C\u952e\u63a5\u679d\u5728\u591a\u5b54\u6ce1\u6cab\u77f3\u58a8(UGF)\u4e0a\u3002\u5728\u5fae\u89c2\u7ed3\u6784\u4e0a\uff0c\u5171\u4ef7\u8fde\u63a5\u6d88\u9664\u4e86\u7eb3\u7c73\u7ed3\u6784\u5355\u5143\u95f4\u7684\u754c\u9762\u7535\u963b\uff0csp2<\/sup>\u6742\u5316\u78b3\u7eb3\u7c73\u7ed3\u6784\u63d0\u4f9b\u4e86\u53ef\u4ee5\u957f\u7a0b\u4f20\u8f93\u7684\u8f7d\u6d41\u5b50\u3002\u5728\u5b8f\u89c2\u7ed3\u6784\u4e0a\uff0c\u8fd9\u79cd\u6750\u6599\u5177\u6709\u5b8c\u6574\u3001\u8fde\u7eed\u7684\u8868\u89c2\u7ed3\u6784\uff0c12.4 mg cm-3<\/sup>\u7684\u5bc6\u5ea6\u3001250 m2<\/sup> g-1<\/sup>\u7684\u6bd4\u8868\u9762\u79ef\u3001\u767e\u5fae\u7c73\u957f\u7684\u7eb3\u7c73\u5b54\u9053\u548c95 wt%\u7684\u78b3\u542b\u91cf\uff0c\u53ef\u540c\u65f6\u7528\u505a\u9502\u786b\u7535\u6c60\u6b63\u3001\u8d1f\u6781\u96c6\u6d41\u4f53\u3002\u5728\u6b63\u6781\u65b9\u9762\uff0c\u5171\u4ef7\u8fde\u63a5\u7684\u7f51\u7edc\u4f7f\u5f97\u786b\u6b63\u6781\u57288C\u500d\u7387\u5faa\u73af\u4e0b\u83b7\u5f97\u9ad8\u8fbe860 mA h g-1<\/sup>\u7684\u6bd4\u5bb9\u91cf\uff0c\u591a\u7ea7\u5b54\u7ed3\u6784\u7684\u5b58\u5728\u6210\u529f\u6291\u5236\u4e86\u201c\u7a7f\u68ad\u6548\u5e94\u201d\u4f7f\u6bcf\u5708\u5bb9\u91cf\u8870\u51cf\u7387\u4f4e\u81f30.063%\u3002\u5728\u8d1f\u6781\u65b9\u9762\uff0c\u4e09\u7ef4\u96c6\u6d41\u4f53\u4f7f\u7535\u6781\u7684\u6709\u6548\u9762\u79ef\u63d0\u9ad8\uff0c\u4f7f\u9502\u679d\u6676\u7684\u6210\u6838\u65f6\u95f4\u589e\u957f\u4e8650\u500d\u3001\u751f\u957f\u901f\u7387\u964d\u4f4e\u81f31\/7\uff0c\u6291\u5236\u4e86\u679d\u6676\u751f\u957f\uff0c\u63d0\u9ad8\u4e86\u7535\u6c60\u5b89\u5168\u6027\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1<\/strong>\uff1aCNT-UGF<\/strong>\u7ed3\u6784\u548c\u7ec4\u5206\u7684\u5206\u6790<\/strong><\/p>\n

\"fig1\"<\/p>\n

(a)\u4e3aUGF(\u5de6\u8fb9)\u548cCNT-UGF(\u53f3\u8fb9)\u7684SEM\u8868\u5f81\u3002<\/p>\n

(b)\u4e3aCNT-UGF\u7684\u5149\u5b66\u7167\u7247\u3002<\/p>\n

(c)\u4e3a\u81ea\u7531\u7535\u5b50\u5728\u4e09\u7ef4\u8fde\u901a\u7684CNT-UGF\u7f51\u7edc\u4f20\u8f93\u7684\u793a\u610f\u56fe\u3002<\/p>\n

(d-f)\u4e3a\u5b9e\u9a8c\u4e2d\u901a\u8fc7\u8c03\u63a7CVD\u5408\u6210\u53c2\u6570\uff0c\u5f97\u5230\u7684\u4e0d\u540c\u957f\u5ea6\u7684\u78b3\u7eb3\u7c73\u7ba1\u9635\u5217\u7684CNT-UGF\u3002<\/p>\n

(g)\u4e3a\u78b3\u7eb3\u7c73\u7ba1\u675f\u7684SEM\u8868\u5f81\u3002<\/p>\n

(h)\u4e3aCNT-UGF\u548cUGF\u7684\u62c9\u66fc\u5149\u8c31\u3002<\/p>\n

(i)\u4e3aUGF\u548cCNT-UGF\u7684\u70ed\u91cd\u66f2\u7ebf\u3002<\/p>\n

(j)\u4e3aCNT-UGF\u7684\u5b54\u5f84\u5206\u5e03\u3002<\/p>\n

(k)\u4e3a\u78b3\u7eb3\u7c73\u7ba1\u7684\u9ad8\u5206\u8fa8TEM\u8868\u5f81\u3002<\/p>\n

\u56fe<\/strong>2<\/strong>\uff1a\u78b3\u7eb3\u7c73\u7ba1\u4e0e\u77f3\u58a8<\/strong>\u5171\u4ef7\u7ed3\u5408\u7684<\/strong>TEM<\/strong>\u5206\u6790<\/strong><\/p>\n

\"fig2\"<\/p>\n

(a)\u4e3a\u901a\u8fc7\u805a\u7126\u79bb\u5b50\u675f\u5236\u5907\u7684CNT-UGF\u7684TEM\u8868\u5f81\u3002<\/p>\n

(b,c)\u4e3a\u9ad8\u5206\u8fa8\u7684\u78b3\u7eb3\u7c73\u7ba1\/\u77f3\u58a8\u7ed3\u5408\u90e8\u4f4d\u7684TEM\u8868\u5f81\u3002<\/p>\n

(d)\u4e3a\u78b3\u7eb3\u7c73\u7ba1\u4e0e\u77f3\u58a8\u4e4b\u95f4\u4e24\u79cd\u4e0d\u540c\u7ed3\u5408\u65b9\u5f0f\u7684\u4ea4\u6d41\u963b\u6297\u5206\u6790\u3002\u5206\u522b\u5bf9\u4e24\u79cd\u6750\u6599\u865a\u90e8\u7535\u5bb9\u5bf9\u7535\u6d41\u9891\u7387\u4f5c\u56fe\uff0c\u7ea2\u7ebf\u4ee3\u8868\u7740\u77f3\u58a8\u548c\u78b3\u7ba1\u4e2d\u95f4\u6709\u4e00\u5c42\u6c27\u5316\u94dd\u7684\u7ed3\u6784\uff0c\u4e3b\u8981\u662f\u5728\u5236\u5907CNT-UGF\u7684\u8fc7\u7a0b\u4e2d\uff0c\u9996\u5148\u6c89\u79ef\u6c27\u5316\u94dd\uff0c\u7136\u540e\u6c89\u79ef\u94c1\u4f5c\u4e3a\u50ac\u5316\u5242\u3002\u9ed1\u7ebf\u4ee3\u8868\u7740CNT\u548c\u77f3\u58a8\u4e4b\u95f4\u662f\u76f4\u63a5\u5171\u4ef7\u7ed3\u5408\u5728\u4e00\u8d77\u7684\u7ed3\u6784\u3002\u4e3b\u8981\u662f\u5728\u5236\u5907CNT-UGF\u7684\u8fc7\u7a0b\u4e2d\uff0c\u9996\u5148\u6c89\u79ef\u94c1\uff0c\u7136\u540e\u6c89\u79ef\u6c27\u5316\u94dd\u3002<\/p>\n

\u56fe<\/strong>3<\/strong>\uff1aS\/CNT-UGF<\/strong>\u4f5c\u4e3a\u9502\u786b\u7535\u6c60\u6b63\u6781\u7684\u7ed3\u6784\u548c\u7535\u5316\u5b66\u5206\u6790<\/strong><\/p>\n

\"fig3\"<\/p>\n

(a)\u4e3aS\/CNT-UGF\u8d1f\u8f7d\u786b\u7684\u542b\u91cf\u901a\u8fc7\u8d1f\u8f7d\u524d\u540e\u8d28\u91cf\u589e\u91cd\u4e0e\u70ed\u91cd\u5206\u6790\u5f97\u5230\u7684\u6570\u503c\u4e4b\u95f4\u5173\u7cfb\u3002<\/p>\n

(b)\u4e3aS\/CNT-UGF\u6b63\u6781\u7684SEM\u8868\u5f81\u548c\u5143\u7d20\u5206\u5e03\u3002<\/p>\n

(c)\u4e3aS\/CNT-UGF\u7684\u9ad8\u5206\u8fa8\u7684TEM\u8868\u5f81\u3002<\/p>\n

(d)\u4e3aS\/CNT-UGF\u6b63\u6781\u7684\u53ef\u9006\u5145\u653e\u7535\u66f2\u7ebf\u3002\u5f53\u7535\u6d41\u5bc6\u5ea6\u4ece0.5C\u5347\u9ad8\u52308C\u662f\uff0c\u7535\u538b\u5e73\u53f0\u5206\u522b\u4ece2.10 V\u964d1.80 V\u3002<\/p>\n

(e)\u4e3aS\/CNT-UGF\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

\u56fe<\/strong>4<\/strong>\uff1a<\/strong>Li\/CNT-UGF<\/strong>\u8d1f\u6781\u7684\u7ed3\u6784\u548c\u7535\u5316\u5b66\u5206\u6790<\/strong><\/p>\n

\"fig4\"<\/p>\n

(a)\u4e3a\u6c89\u79ef\u9502\u540e\u7684CNT-UGF\u5149\u5b66\u56fe\u7247\u3002<\/p>\n

(b,c)\u4e3a\u6c89\u79ef\u9502\u540eCNT-UGF\u7684SEM\u8868\u5f81\u3002<\/p>\n

(d)\u4e3a\u78b3\u7eb3\u7c73\u7ba1\u6c89\u79ef\u91d1\u5c5e\u9502\u540e\u7684TEM\u8868\u5f81\u3002<\/p>\n

(e)\u4e3a\u6c89\u79ef\u9502\u540eCNT-UGF\u5bf9\u79f0\u7684XPS\u5206\u6790\u3002<\/p>\n

(f)\u4e3aLi\u2551Li\u5bf9\u79f0\u7535\u6c60\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002<\/p>\n

(g,h)\u4e3aLi\/CNT-UGF\u8d1f\u6781\u5faa\u73af800\u5c0f\u65f6\u4ee5\u540e\u7684SEM\u8868\u5f81\u3002<\/p>\n

(i,j)\u4e3a\u9502\u7247\u5faa\u73af350\u5c0f\u65f6\u4ee5\u540e\u7684SEM\u8868\u5f81\u3002<\/p>\n

\u56fe<\/strong>5<\/strong>\uff1a<\/strong>S\/CNT-UGF<\/strong>\u4e3a\u6b63\u6781\uff0c<\/strong>Li\/CNT-UGF<\/strong>\u4e3a\u8d1f\u6781\u7ec4\u88c5\u6210\u9502\u786b\u7535\u6c60\u7684\u7535\u5316\u5b66\u5206\u6790<\/strong><\/p>\n

\"fig5\"<\/p>\n

(a)\u4e3aLi\/CNT-UGF\u2551S\/CNT-UGF\u7535\u6c60\u5728\u4e0d\u540c\u500d\u7387\u4e0b\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002\u5f53\u7535\u6d41\u5bc6\u5ea6\u4ece0.5C\u5347\u9ad8\u523012C\u65f6\uff0c\u7535\u538b\u5e73\u53f0\u4ece2.1 V\u4e0b\u964d\u52301.87 V\u3002<\/p>\n

(b)\u4e3aLi\/CNT-UGF\u2551S\/CNT-UGF\u7535\u6c60\u7684\u500d\u7387\u6027\u80fd\uff0c\u8868\u660eCNT-UGF\u5177\u6709\u6781\u9ad8\u7684\u500d\u7387\u5bb9\u91cf\u3002<\/p>\n

(c)\u4e3aLi\/CNT-UGF\u2551S\/CNT-UGF\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6\u548c\u529f\u7387\u5bc6\u5ea6\u56fe\u548c\u5176\u4ed6\u6587\u732e\u4e4b\u95f4\u7684\u6bd4\u8f83\u3002<\/p>\n

(d)\u4e3aLi\/CNT-UGF\u2551S\/CNT-UGF\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

\u56fe<\/strong>6<\/strong>\uff1a<\/strong>CNT-UGF<\/strong>\u4f5c\u4e3a\u9502\u786b\u7535\u6c60\u6b63\u8d1f\u6781\u96c6\u6d41\u4f53\u7684\u7535\u5316\u5b66\u5206\u6790<\/strong><\/p>\n

\"fig6\"<\/p>\n

(a)\u4e3aS\/CNT-UGF\u5728\u4e0d\u540c\u653e\u7535\u5e73\u53f0\u7684\u6bd4\u5bb9\u91cf\u548c\u5b83\u4eec\u4e4b\u95f4\u6570\u503c\u7684\u7684\u6bd4\u3002<\/p>\n

(b)\u4e3aLi\/CNT-UGF\u8d1f\u6781\u548c\u9502\u8d1f\u6781\u5728\u5bf9\u79f0\u7535\u6c60\u4e2d\u7684\u8fc7\u7535\u52bf\u5bf9\u6bd4\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u8be5\u5de5\u4f5c\u901a\u8fc7\u78b3-\u78b3\u5171\u4ef7\u8fde\u63a5\u7684\u65b9\u5f0f\uff0c\u5c06\u78b3\u7eb3\u7c73\u7ba1\u63a5\u679d\u5728\u6ce1\u6cab\u77f3\u58a8\u4e0a\uff0c\u5f62\u6210\u4e86\u4e09\u7ef4\u8fde\u901a\u7684\u5bfc\u7535\u7f51\u7edc\u3002\u5229\u7528CNT-UGF\u591a\u7ea7\u5b54\u7ed3\u6784\u6210\u529f\u6291\u5236\u4e86\u591a\u7559\u5316\u9502\u7684\u201c\u7a7f\u68ad\u6548\u5e94\uff0c\u540c\u65f6\u4e09\u7ef4\u96c6\u6d41\u4f53\u80fd\u63d0\u9ad8\u7535\u6781\u7684\u6709\u6548\u9762\u79ef\uff0c\u6291\u5236\u4e86\u9502\u679d\u6676\u751f\u957f\uff0c\u63d0\u9ad8\u4e86\u7535\u6c60\u5b89\u5168\u6027\u3002\u5176\u6750\u6599\u8bbe\u8ba1\u7b56\u7565\u4e3a\u9502\u786b\u7535\u6c60\u8fdb\u4e00\u6b65\u53d1\u5c55\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aCovalently Connected Carbon Nanostructures for Current Collectors in Both the Cathode and Anode of Li-S Batteries<\/a> (Adv. Mater., 2016, DOI:10.1002\/adma.201602704)<\/p>\n

\u8be5\u79d1\u6280\u65b0\u95fb\u7531\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u5b63\u6052\u661f\u6559\u6388\u8bfe\u9898\u7ec4\u6295\u7a3f\uff0c\u6750\u6599\u4eba\u7f51\u65b0\u80fd\u6e90\u5b66\u672f\u7ec4\u52a0\u5de5\u6574\u7406\uff0c\u6b22\u8fce\u5404\u5927\u8bfe\u9898\u7ec4\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065952\u201d,\u6b22\u8fce\u5173\u6ce8\u5fae\u4fe1\u516c\u4f17\u53f7\uff0c\u5fae\u4fe1\u641c\u7d22\u201c\u65b0\u80fd\u6e90\u524d\u7ebf\u201d\u6216\u626b\u7801\u5173\u6ce8\u3002\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n

\u503c\u6b64\u5927\u4e2d\u534e\u4e2d\u79cb\u4f73\u8282\u4e4b\u9645\uff0c\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5168\u4f53\u8bda\u631a\u5730\u795d\u798f\u6240\u6709\u6750\u6599\u4eba\u65b0\u8001\u7c89\u4e1d\u548c\u5e7f\u5927\u8bfb\u8005\uff1a<\/strong><\/span><\/p>\n

\u5e78\u798f\u7f8e\u6ee1\uff0c\u4e8b\u4e8b\u987a\u5229\uff0c\u5fc3\u60f3\u4e8b\u6210\uff0c\u9616\u5bb6\u6b22\u4e50\uff01<\/strong><\/span><\/p>\n

\u6b22\u5ea6\u4e2d\u79cb\uff0c\u5047\u671f\u6109\u5feb\uff01<\/strong><\/span><\/p>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

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