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<\/p>\n\n\n\n

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\u7814\u7a76\u80cc\u666f<\/strong><\/strong><\/p>\n\n\n\n

<\/a>\u9502\u91d1\u5c5e\u8d1f\u6781\u56e0\u5176\u8d85\u9ad8\u7406\u8bba\u6bd4\u5bb9\u91cf\uff083860 mAh\u00b7g\u207b\u00b9\uff09\u548c\u6700\u4f4e\u7535\u5316\u5b66\u7535\u4f4d\uff08\u22123.04 V vs. SHE\uff09\uff0c\u88ab\u516c\u8ba4\u4e3a\u4e0b\u4e00\u4ee3\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u50a8\u80fd\u4f53\u7cfb\u7684\u7406\u60f3\u6838\u5fc3\u6750\u6599\u3002\u7136\u800c\uff0c\u5176\u65e0\u5bbf\u4e3b\u7279\u6027\u5bfc\u81f4\u9502\u5728\u6c89\u79ef\u8fc7\u7a0b\u4e2d\u6613\u5f62\u6210\u679d\u6676\u6216\u82d4\u85d3\u72b6\u7ed3\u6784\uff0c\u5f15\u53d1\u5267\u70c8\u4f53\u79ef\u81a8\u80c0\u3001\u754c\u9762\u5931\u7a33\u53ca\u7535\u89e3\u6db2\u6301\u7eed\u5206\u89e3\u7b49\u95ee\u9898\uff0c\u4e25\u91cd\u5236\u7ea6\u5b9e\u9645\u5e94\u7528\u3002\u5c3d\u7ba1\u5f53\u524d\u591a\u79cd\u7b56\u7565\uff08\u5982\u4eba\u5de5SEI\u6784\u5efa\u3001\u5408\u91d1\u5316\u5bbf\u4e3b\u8bbe\u8ba1\u53ca\u4e09\u7ef4\u96c6\u6d41\u4f53\u8c03\u63a7\uff09\u901a\u8fc7\u8c03\u8282\u8868\u9762\u5316\u5b66\u6216\u7535\u6d41\u5206\u5e03\u53ef\u90e8\u5206\u6291\u5236\u679d\u6676\u751f\u957f\uff0c\u4f46\u8fd9\u4e9b\u65b9\u6cd5\u591a\u4f9d\u8d56\u7ecf\u9a8c\u6027\u8bbe\u8ba1\uff0c\u7f3a\u4e4f\u4ece\u539f\u5b50\u5c3a\u5ea6\u51fa\u53d1\u534f\u540c\u4f18\u5316\u754c\u9762\u7535\u573a\u3001\u79bb\u5b50\u6d53\u5ea6\u5206\u5e03\u4e0e\u53cd\u5e94\u52a8\u529b\u5b66\u7684\u666e\u9002\u6027\u7406\u8bba\u6846\u67b6\u3002<\/p>\n\n\n\n

\u503c\u5f97\u5173\u6ce8\u7684\u662f\uff0c\u7535\u8d1f\u6027<\/strong>\u2014\u2014\u8868\u5f81\u539f\u5b50\u5438\u5f15\u7535\u5b50\u80fd\u529b\u7684\u57fa\u672c\u7269\u7406\u91cf\u2014\u2014\u5c1a\u672a\u88ab\u7cfb\u7edf\u5f00\u53d1\u4e3a\u9502\u91d1\u5c5e\u7535\u6c60\u754c\u9762\u5de5\u7a0b\u7684\u5b9a\u5411\u8bbe\u8ba1\u53c2\u6570\u3002\u7406\u8bba\u4e0a\uff0c\u63d0\u5347\u8868\u9762\u7aef\u57fa\u7684\u7535\u8d1f\u6027\u53ef\u589e\u5f3a\u9633\u79bb\u5b50\u5438\u9644\u3001\u6392\u65a5\u9634\u79bb\u5b50\uff0c\u4ece\u800c\u52a0\u901fLi\u207a\u53bb\u6eb6\u5242\u5316\u8fc7\u7a0b\uff0c\u5747\u5300\u5316\u754c\u9762\u79bb\u5b50\u901a\u91cf\u5e76\u4fc3\u8fdb\u7a33\u5b9a\u6210\u6838\u3002<\/p>\n\n\n\n

\u5de5\u4f5c\u4ecb\u7ecd<\/strong><\/strong><\/p>\n\n\n\n

\u9488\u5bf9\u4e0a\u8ff0\u95ee\u9898\uff0c\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u90d7\u51ef\u6559\u6388\u56e2\u961f<\/strong>\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u7535\u8d1f\u6027\u8c03\u63a7\u7684\u754c\u9762\u5de5\u7a0b\u7b56\u7565<\/strong>\u3002\u7814\u7a76\u56e2\u961f\u901a\u8fc7\u7cbe\u51c6\u8bbe\u8ba1\u4e8c\u7ef4MXene\u6750\u6599\u7684\u8868\u9762\u7aef\u57fa\uff0c\u6784\u5efa\u51fa\u9ad8\u7535\u8d1f\u6027\u3001\u4eb2\u9502\u6027\u7684\u9650\u57df\u754c\u9762\uff0c\u5b9e\u73b0\u4e86Li\u207a\u901a\u91cf\u7684\u9ad8\u5ea6\u5747\u5300\u5316\uff0c\u6709\u6548\u6291\u5236\u7a7a\u95f4\u7535\u8377\u79ef\u7d2f\uff0c\u5e76\u4fc3\u8fdb\u5bccLi\u2082O SEI\u7684\u539f\u4f4d\u5f62\u6210\u3002\u5f97\u76ca\u4e8e\u8be5\u8bbe\u8ba1\uff0c\u9502\u8d1f\u6781\u57281600\u6b21\u5faa\u73af\u540e\u4ecd\u4fdd\u630199.41%\u7684\u9ad8\u5e93\u4ed1\u6548\u7387\uff0c\u4e14\u914d\u5408\u78f7\u9178\u94c1\u9502\uff08LiFePO\u2084\uff09\u6b63\u6781\u7ec4\u88c5\u76841 Ah\u8f6f\u5305\u7535\u6c60\u5b9e\u73b0\u4e86\u9ad8\u8fbe238.06 Wh\u00b7kg\u207b\u00b9\u7684\u80fd\u91cf\u5bc6\u5ea6\uff0c\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u5feb\u5145\u4e0e\u5faa\u73af\u7a33\u5b9a\u6027\u80fd\u3002<\/p>\n\n\n\n

\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cAccelerating Near-Electrode Li\u207a Transport via High-Electronegativity Substrates for Sustainable Fast-Charging Lithium Metal Batteries\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728\u56fd\u9645\u8457\u540d\u671f\u520a\u300aAdvanced Functional Materials\u300b\u4e0a\u3002\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a<\/strong>\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u5316\u5b66\u5b66\u9662\u535a\u58eb\u751f\u5218\u6625\u4e3d\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u90d7\u51ef\u6559\u6388<\/strong>\u3002<\/p>\n\n\n\n

\u5185\u5bb9\u8868\u8ff0<\/strong><\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u673a\u7406\u56fe<\/strong>.(a) Li\u207a\u4f20\u8d28\u793a\u610f\u56fe\u3002(b) Ti\u2083C\u2082O\u2093\u548c(c) Ti\u2083C\u2082T\u2093\u652f\u67b6\u4e0a\u9502\u6c89\u79ef\u884c\u4e3a\u7684\u793a\u610f\u56fe\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe1. \u7535\u8d1f\u6027\u8c03\u63a7\u7aef\u57fa\u57fa\u56e2\u7684\u8ba1\u7b97\u7b5b\u9009\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a) Ti\u2083C\u2082O\u2093\u3001(b) Ti\u2083C\u2082F\u2093\u3001(c) Ti\u2083C\u2082Cl\u2093\u548c(d) Ti\u2083C\u2082Br\u2093\u7684\u9759\u7535\u52bf\u56fe\u3002<\/p>\n\n\n\n

(e) Ti\u2083C\u2082O\u2093\u3001Ti\u2083C\u2082F\u2093\u3001Ti\u2083C\u2082Cl\u2093\u548cTi\u2083C\u2082Br\u2093\u7684Mulliken\u7535\u8377\u5206\u5e03\u3002<\/p>\n\n\n\n

(f, g) Ti\u2083C\u2082O\u2093\u4e0e\u9502\u539f\u5b50\u7684\u4f18\u5316\u5438\u9644\u6784\u578b\uff08\u4fa7\u89c6\u56fe\u548c\u4fef\u89c6\u56fe\uff09\u3002<\/p>\n\n\n\n

(h) \u9502\u5438\u9644\u540e\u7535\u8377\u5bc6\u5ea6\u5dee\uff08CDD\uff09\u5206\u6790\uff08\u4fa7\u89c6\u56fe\uff09\u3002<\/p>\n\n\n\n

(i) \u4e0d\u540cMXene\u7aef\u57fa\u57fa\u56e2\u5bf9\u9502\u539f\u5b50\u7684\u5438\u9644\u80fd\uff08E\u2090d\uff09\u3002<\/p>\n\n\n\n

(j) \u9502\u539f\u5b50\u4e0eTi\u2083C\u2082O\u2093\u4e4b\u95f4\u952e\u5408\u7279\u6027\u7684\u7535\u5b50\u5c40\u57df\u51fd\u6570\uff08ELF\uff09\u5206\u6790\u3002<\/p>\n\n\n\n

(k) \u539f\u59cb\u53ca\u7aef\u57faMXene\uff08Ti\u2083C\u2082\u3001Ti\u2083C\u2082O\u2093\u3001Ti\u2083C\u2082F\u2093\u3001Ti\u2083C\u2082Cl\u2093\u548cTi\u2083C\u2082Br\u2093\uff09\u7684\u6001\u5bc6\u5ea6\uff08DOS\uff09\u8c31\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe2. \u6750\u6599\u5236\u5907\u4e0e\u7ed3\u6784\u8868\u5f81\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a) \u901a\u8fc7\u9009\u62e9\u6027\u523b\u8680\u548c\u8868\u9762\u7aef\u57fa\u8c03\u63a7\u4eceTi\u2083AlC\u2082\u5408\u6210Ti\u2083C\u2082O\u2093\u7684\u793a\u610f\u56fe\u3002<\/p>\n\n\n\n

(b) Ti\u2083C\u2082O\u2093\u7684\u900f\u5c04\u7535\u955c\uff08TEM\uff09\u56fe\u50cf\uff0c\u63d2\u56fe\u4e3a\u9009\u533a\u7535\u5b50\u884d\u5c04\uff08SAED\uff09\u548c\u9ad8\u5206\u8fa8TEM\uff08HRTEM\uff09\u3002<\/p>\n\n\n\n

(c) HAADF-TEM\u56fe\u50cf\u53ca\u5143\u7d20\u5206\u5e03\u56fe\u3002<\/p>\n\n\n\n

(d) Ti\u2083C\u2082O\u2093\u3001Ti\u2083C\u2082T\u2093\u548cTi\u2083AlC\u2082\u7684X\u5c04\u7ebf\u884d\u5c04\uff08XRD\uff09\u56fe\u8c31\u3002<\/p>\n\n\n\n

(e) Ti\u2083C\u2082O\u2093\u7eb3\u7c73\u7247\u7684\u539f\u5b50\u529b\u663e\u5fae\u955c\uff08AFM\uff09\u56fe\u50cf\u53ca\u9ad8\u5ea6\u5206\u5e03\u3002<\/p>\n\n\n\n

(f) Ti\u2083C\u2082O\u2093\u548cTi\u2083C\u2082T\u2093\u4e2dTi-O\u4e0eC-Ti-O\u2093\/C-Ti-OH\u7684\u7ec4\u6210\u6bd4\u4f8b\u3002<\/p>\n\n\n\n

(g) Ti\u2083C\u2082O\u2093\u548cTi\u2083C\u2082T\u2093\u7684Zeta\u7535\u4f4d\u6d4b\u91cf\u7ed3\u679c\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe3. \u9502\u6c89\u79ef\u5f62\u8c8c\u8868\u5f81\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a, d) Ti\u2083C\u2082O\u2093\u3001(b, e) Ti\u2083C\u2082T\u2093\u548c(c, f) \u65e0\u652f\u67b6\u4f53\u7cfb\u7684\u9502\u6c89\u79ef\u7535\u6d41\u5bc6\u5ea6\u5206\u5e03\u6709\u9650\u5143\u6a21\u62df\u3002<\/p>\n\n\n\n

(g) Ti\u2083C\u2082O\u2093\u548c(h) Ti\u2083C\u2082T\u2093\u652f\u67b6\u4e0a\u9502\u6c89\u79ef\u884c\u4e3a\u7684\u539f\u4f4d\u5149\u5b66\u663e\u5fae\u955c\u56fe\u50cf\u3002<\/p>\n\n\n\n

(i) Ti\u2083C\u2082O\u2093\u548c(j) Ti\u2083C\u2082T\u2093\u652f\u67b6\u57280.25 mA cm\u207b\u00b2\u4e0b\u6c89\u79ef5\u5206\u949f\u540e\u7684\u626b\u63cf\u7535\u955c\uff08SEM\uff09\u56fe\u50cf\u3002<\/p>\n\n\n\n

(k) \u9502\u6c89\u79ef\u540eTi\u2083C\u2082O\u2093\u7684\u9ad8\u5206\u8fa8\u51b7\u51bb\u7535\u955c\uff08Cryo-EM\uff09\u56fe\u50cf\u53caFFT\u5206\u6790\u3002<\/p>\n\n\n\n

(l) Ti\u2083C\u2082O\u2093\uff08\u7ea2\uff09\u548cTi\u2083C\u2082T\u2093\uff08\u84dd\uff09\u652f\u67b6\u4e2dLiO\u207b\u5f3a\u5ea6\u968f\u6e85\u5c04\u65f6\u95f4\u7684\u53d8\u5316\uff0c\u63d2\u56fe\u4e3a3D TOF-SIMS\u7684LiO\u207b\u5206\u5e03\u56fe\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe4. Ti\u2083C\u2082O\u2093\u652f\u67b6\u4fc3\u8fdb\u7684Li\u207a\u4f20\u8f93\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a) Ti\u2083C\u2082O\u2093@Li \u548c Ti\u2083C\u2082T\u2093@Li \u5bf9\u79f0\u7535\u6c60\u7684\u6e29\u5ea6\u4f9d\u8d56\u6027\u7535\u5316\u5b66\u963b\u6297\u8c31\uff08EIS\uff09\u3002<\/p>\n\n\n\n

(b) \u4e24\u79cd\u5bf9\u79f0\u7535\u6c60\u4e2dLi\u207a\u901a\u8fc7\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762\uff08SEI\uff09\u7684\u4f20\u8f93\u963b\u529b\u968f\u6e29\u5ea6\u53d8\u5316\u7684\u963f\u4f26\u5c3c\u4e4c\u65af\u62df\u5408\u66f2\u7ebf\u3002<\/p>\n\n\n\n

(c) \u4e24\u79cd\u5bf9\u79f0\u7535\u6c60\u4e2d\u7535\u8377\u8f6c\u79fb\u8fc7\u7a0b\u963b\u529b\u7684\u963f\u4f26\u5c3c\u4e4c\u65af\u62df\u5408\u66f2\u7ebf\u3002<\/p>\n\n\n\n

(d, e) Li\u207a\u7a7f\u8fc7LiF (200) \u6676\u9762\u548cLi\u2082O (111) \u6676\u9762\u7684\u8fc1\u79fb\u80fd\u5792\u7406\u8bba\u8ba1\u7b97\u3002<\/p>\n\n\n\n

(f) Ti\u2083C\u2082O\u2093@Li \u548c Ti\u2083C\u2082T\u2093@Li \u5bf9\u79f0\u7535\u6c60\u7684\u5854\u83f2\u5c14\u6781\u5316\u66f2\u7ebf\uff0c\u53cd\u6620\u754c\u9762\u53cd\u5e94\u52a8\u529b\u5b66\u5dee\u5f02\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe5. \u9ad8\u7a33\u5b9a\u7684\u9502\u6c89\u79ef\/\u5265\u79bb\u884c\u4e3a\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a) Li||Ti\u2083C\u2082O\u2093\u548cLi||Ti\u2083C\u2082T\u2093\u534a\u7535\u6c60\u7684\u5faa\u73af\u4f0f\u5b89\uff08CV\uff09\u66f2\u7ebf\u3002<\/p>\n\n\n\n

(b) Ti\u2083C\u2082O\u2093\u548cTi\u2083C\u2082T\u2093\u652f\u67b6\u7684\u6210\u6838\u8fc7\u7535\u4f4d\u5bf9\u6bd4\u3002<\/p>\n\n\n\n

(c) \u57fa\u4e8eAurbach\u6cd5\u7684\u5e93\u4ed1\u6548\u7387\u8bc4\u4f30\u3002<\/p>\n\n\n\n

(d) 0.5 mA cm\u207b\u00b2\u4e0b\u957f\u5faa\u73af\u5e93\u4ed1\u6548\u7387\u3002<\/p>\n\n\n\n

(e) \u5faa\u73af10\u6b21\u540e\u9502\u5316\u652f\u67b6\u7684\u8868\u9762\u7c97\u7cd9\u5ea6\u3002<\/p>\n\n\n\n

(f) \u5bf9\u79f0\u7535\u6c60\u57281.0 mA cm\u207b\u00b2\u4e0b\u7684\u7535\u538b\u66f2\u7ebf\uff0c\u63d2\u56fe\u4e3a\u9502\u63a5\u89e6\u89d2\u6d4b\u8bd5\u3002<\/p>\n\n\n\n

(g) \u672c\u5de5\u4f5c\u4e0e\u5df2\u62a5\u9053MXene\u57fa\u8d1f\u6781\u7684\u6027\u80fd\u5bf9\u6bd4\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe6. \u5168\u7535\u6c60\u7535\u5316\u5b66\u6027\u80fd\u3002<\/strong><\/strong><\/p>\n\n\n\n

(a, b) Ti\u2083C\u2082O\u2093@Li||LFP\u548cTi\u2083C\u2082T\u2093@Li||LFP\u7535\u6c60\u57281 C\u4e0b\u7684\u957f\u5faa\u73af\u6027\u80fd\uff08LFP\u8d1f\u8f7d\u91cf\u5206\u522b\u4e3a10.0\u548c20.0 mg cm\u207b\u00b2\uff09\u3002<\/p>\n\n\n\n

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    \u6587\u732e\u4fe1\u606f<\/strong><\/strong><\/p>\n\n\n\n

    Accelerating Near-Electrode Li+<\/sup> Transport via High-Electronegativity Substrates for Sustainable Fast-Charging Lithium Metal Batteries. Adv. Funct. Mater. <\/em>2025, e24392, <\/a>https:\/\/doi.org\/10.1002\/adfm.202524392.<\/p>\n\n\n\n

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