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\u00a0<\/strong>\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u57fa\u4e8e\u6b64\uff0c\u5929\u6d25\u5927\u5b66\u4f55\u6625\u5e74\u6559\u6388\u4e0e\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66<\/strong>Andrew Barnabas Wong<\/strong>\u6559\u6388<\/strong>\u8054\u5408\u8bbe\u8ba1\u4e86\u4e00\u79cd\u5177\u6709\u94f6\u7eb3\u7c73\u9897\u7c92\uff08Ag NP\uff09\u76843D\u4e32\u8054\u50ac\u5316\u5242\u7535\u6781\uff0c\u7528\u4e8e\u5728\u94dc\u7eb3\u7c73\u9488\u9635\u5217\u4e2d\u751f\u6210CO\u4f5c\u4e3a\u4e2d\u95f4\u4ea7\u7269\u3002\u901a\u8fc7\u8fd9\u79cd\u7eb3\u7c73\u7ed3\u6784\u8bbe\u8ba1\uff0c\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a350 mA cm-2<\/sup>\u7684H\u578b\u7535\u89e3\u6c60\u548c\u6d41\u52a8\u6c60\u4e2d\uff0cCO2<\/sub>\u5f62\u6210C2+<\/sub>\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FEC2+<\/sup>\uff09\u5206\u522b\u4e3a64%\u548c70%\uff0c\u8fd9\u662f\u76ee\u524d\u62a5\u9053\u7684\u6700\u9ad8\u503c\u3002\u968f\u540e\u91c7\u7528\u539f\u4f4d\u62c9\u66fc\u5149\u8c31\u548c\u6709\u9650\u5143\u65b9\u6cd5\u8ba1\u7b97\u6765\u9610\u660e\u589e\u5f3a\u9009\u62e9\u6027\u7684\u539f\u56e0\uff0c\u7ed3\u679c\u63ed\u793a\u4e86\u5728\u4e32\u8054\u50ac\u5316\u5242\u7cfb\u7edf\u7684CO2<\/sub>\u8f6c\u5316\u8fc7\u7a0b\u4e2d\u5ef6\u957fCO\u6269\u6563\u8def\u5f84\u957f\u5ea6\u5bf9\u63d0\u9ad8CO\u5229\u7528\u7387\u7684\u5173\u952e\u4f5c\u7528\u3002\u5728\u4e24\u79cd\u4e0d\u540c\u7684\u73af\u5883\uff08H\u578b\u7535\u89e3\u6c60\u548c\u6d41\u52a8\u6c60\uff09\u4e2d\u6709\u5229\u7684CO2<\/sub>RR-FEC2+<\/sup>\u8fdb\u4e00\u6b65\u8bc1\u5b9e\u4e86\u8fd9\u79cd\u4f5c\u7528\u5e76\u4e0d\u5c40\u9650\u4e8e\u7279\u5b9a\u7684\u53cd\u5e94\u5668\u73af\u5883\u3002\u603b\u7684\u6765\u8bf4\uff0c\u8fd9\u9879\u7814\u7a76\u4e3a\u8bbe\u8ba1\u4e32\u8054\u50ac\u5316\u5242\u4ee5\u63d0\u9ad8CO2<\/sub>RR\u5bf9C2+<\/sub>\u4ea7\u7269\u7684\u9009\u62e9\u6027\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cNanoscale Management of CO Transport in CO2<\/sub> Electroreduction: Boosting Faradaic Efficiency to Multicarbon Products via Nanostructured Tandem Electrocatalysts<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u77e5\u540d\u671f\u520aAdv. Funct. Mater.<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

\u672c\u7814\u7a76\u4e3a\u5177\u6709\u9ad8C2+<\/sub>\u9009\u62e9\u6027\u7684CO2<\/sub>RR\u6784\u5efa\u4e86\u4e00\u79cd\u6709\u6548\u7684\u4e32\u8054\u7535\u6781\u7ed3\u6784\uff0c\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a350 mA cm-2<\/sup>\u7684H\u578b\u7535\u89e3\u6c60\u548c\u6d41\u52a8\u6c60\u4e2d\uff0cCO2<\/sub>\u5f62\u6210C2+<\/sub>\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u5206\u522b\u4e3a64%\u548c70%\u3002<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\u56fe<\/strong>1\u00a0 <\/strong>\u50ac\u5316\u5242\u7684\u8868\u5f81<\/strong> \u00a9 2023 The Authors<\/strong><\/p>\n

\uff08a\uff09Cu\u9488-Ag\u50ac\u5316\u5242\u7684\u5408\u6210\u793a\u610f\u56fe\u3002<\/p>\n

\uff08b-d\uff09Cu(OH)2<\/sub>\u9488-Ag\u7684SEM\u56fe\u50cf\u548c\u5bf9\u5e94\u7684EDS\u56fe\u8c31\u3002<\/p>\n

\uff08e-h\uff09Cu(OH)2<\/sub>\u9488-Ag\u7684TEM\u56fe\u50cf\u548c\u5bf9\u5e94\u7684EDS\u56fe\u8c31\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

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\u56fe<\/strong>2 \u00a0Cu<\/strong>\u9488\u548c<\/strong>Cu<\/strong>\u9488<\/strong>-Ag<\/strong>\u7684\u7535\u50ac\u5316\u6027\u80fd<\/strong> \u00a9 2023 The Authors<\/strong><\/p>\n

\uff08a\uff09\u4e0d\u540c\u5916\u52a0\u7535\u538b\u4e0b\u7684\u7535\u6d41\u5bc6\u5ea6\u3002<\/p>\n

\uff08b-c\uff09CO2<\/sub>\u4e3b\u8981\u8fd8\u539f\u4ea7\u7269\u7684FE\u3002<\/p>\n

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\uff08f\uff09\u5728-1.0V(vs. RHE)\u4e0b\uff0c\u4e0d\u540cAg NPs\u8d1f\u8f7d\u7684Cu\u9488-Ag\u50ac\u5316\u5242\u7684\u4e3b\u8981CO2<\/sub>\u8fd8\u539f\u4ea7\u7269\u3002<\/p>\n

\uff08g\uff09\u5728\u6d41\u52a8\u6c60\u4e2d\u6d4b\u8bd5\u7684Cu\u9488-Ag\u4e0a\u4e0d\u540c\u4ea7\u54c1\u7684FE\u3002<\/p>\n

\uff08h\uff09Cu\u9488-Ag\u4e0aC2+<\/sub>\u3001C1<\/sub>\u548cH2<\/sub>\u7684FE\u4e0e\u65bd\u52a0\u7684\u7535\u6d41\u5bc6\u5ea6\u7684\u5173\u7cfb\u3002<\/p>\n

\uff08i\uff09\u4e0e\u5df2\u62a5\u9053\u7684\u6700\u5148\u8fdb\u7684\u94dc\u57fa\u50ac\u5316\u5242\u4e2d\uff0cCu\u9488-Ag\u50ac\u5316\u5242\u5bf9C2+<\/sub>\u4ea7\u7269\u7684\u50ac\u5316\u6027\u80fd\u5728H\u578b\u7535\u89e3\u6c60\u548c\u6d41\u52a8\u7535\u6c60\u7cfb\u7edf\u4e2d\u8f83\u4f18\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

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\u56fe<\/strong>3 \u00a0<\/strong>\u7ed3\u6784\u6548\u5e94\u7814\u7a76<\/strong> \u00a9 2023 The Authors<\/strong><\/p>\n

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\u00a0<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4 \u00a0<\/strong>\u6709\u9650\u5143\uff08<\/strong>FEM<\/strong>\uff09\u8ba1\u7b97\u6a21\u62df<\/strong> \u00a9 2023 The Authors<\/strong><\/p>\n

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\u539f\u6587\u8be6\u60c5<\/strong>\uff1aNanoscale Management of CO Transport in CO2<\/sub> Electroreduction: Boosting Faradaic Efficiency to Multicarbon Products via Nanostructured Tandem Electrocatalysts<\/a> (Adv. Funct. Mater.<\/em> 2023<\/strong>, 2214992)<\/p>\n

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