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\"\"<\/p>\n

\u56fe1. \u65b0\u578b\u787c\u6c2e\u6742\u7a20\u73af\u82b3\u70c3\u8fd1\u7ea2\u5916\u5149\u654f\u5242\uff08BNS<\/strong>\uff09\u5b9e\u73b0\u9ad8\u6027\u80fd\u84dd\u5149\u4e0a\u8f6c\u6362<\/p>\n

\u8fd1\u65e5\uff0c\u5357\u5f00\u5927\u5b66\u738b\u5c0f\u91ce<\/strong>\u7814\u7a76\u5458\u4e0e\u9ec4\u7075<\/strong>\u7814\u7a76\u5458\u5408\u4f5c\uff0c\u62a5\u9053\u4e86\u9996\u4f8b\u5177\u6709\u591a\u91cd\u5171\u632f-\u70ed\u6d3b\u5316\u5ef6\u8fdf\u8367\u5149\uff08MR-TADF\uff09\u7279\u6027\u7684\u787c\u6c2e\u6742\u7a20\u82b3\u70c3\u8fd1\u7ea2\u5916\u5149\u654f\u5242BNS<\/strong>\uff0c\u5176\u5728\u8fd1\u7ea2\u5916\u533a\u5177\u6709\u5f3a\u70c8\u7684\u5438\u6536\uff0c\u5e76\u4e14\u5177\u6709\u8f83\u5c0f\u7684\u0394E<\/em>ST<\/sub>\uff080.14 eV\uff09\u4e0e\u8f83\u957f\u7684\u5ef6\u8fdf\u8367\u5149\u5bff\u547d\uff08115 \u03bcs\uff09\u3002BNS<\/strong>\u4e0e\u84dd\u5149\u6e6e\u706d\u5242\u7684\u7ec4\u5408\u5b9e\u73b0\u4e86\u53cd\u65af\u6258\u514b\u65af\u4f4d\u79fb\u8fbe1.03 eV\u7684TTA-UC\u8fc7\u7a0b\uff0c\u8fd9\u5728\u65e0\u91d1\u5c5e\u8fd1\u7ea2\u5916\u5149\u654f\u5242\u6fc0\u53d1\u7684TTA-UC\u4f53\u7cfb\u4e2d\u521b\u9020\u4e86\u65b0\u7684\u7eaa\u5f55\u3002\u6b64\u5916\uff0c\u8be5\u4f53\u7cfb\u8fd8\u5177\u6709\u9608\u503c\u529f\u7387\u5bc6\u5ea6\u4f4e\uff08125 mW cm-2<\/sup>\uff09\u3001\u4e0a\u8f6c\u6362\u91cf\u5b50\u4ea7\u7387\u9ad8\uff082.9%\uff09\u3001\u6e6e\u706d\u5242\u6d53\u5ea6\u4f4e\uff0850 \u03bcM\uff09\u3001\u6fc0\u53d1\u5149\u7a7f\u900f\u8ddd\u79bb\u6df1\u7b49\u4f18\u52bf\uff0c\u6709\u671b\u5728\u5149\u52a8\u529b\u6cbb\u7597\u4e0e3D\u6253\u5370\u7b49\u6280\u672f\u4e2d\u83b7\u5f97\u91cd\u8981\u7684\u5e94\u7528\u3002<\/p>\n

\"\"<\/p>\n

\u56fe2. \u8fd1\u7ea2\u5916\u5149\u654f\u5242BNS<\/strong>\u7684\u5408\u6210\u8def\u7ebf\uff08a\uff09\u4e0e\u5149\u7269\u7406\u6027\u8d28\u7814\u7a76\uff08b-e\uff09<\/p>\n

BNS<\/strong>\u53ef\u4ece\u5546\u4e1a\u53ef\u5f97\u7684\u539f\u65991<\/strong>\u51fa\u53d1\uff0c\u901a\u8fc7\u4e24\u6b65\u7b80\u6377\u7684\u53cd\u5e94\u9ad8\u6548\u5236\u5907\u3002\u9996\u5148\uff0c\u4f5c\u8005\u901a\u8fc71<\/strong>\u4e0e1,4-\u4e8c\u6eb4\u56db\u6c1f\u82ef\u7684\u82b3\u9999\u4eb2\u6838\u53d6\u4ee3\u53cd\u5e94\uff0c\u4ee592%\u7684\u6536\u7387\u5408\u6210\u524d\u4f53\u5316\u5408\u72692<\/strong>\uff1b\u7136\u540e\uff0c\u901a\u8fc7\u4e00\u9505\u6cd5\u7684\u9502\u5364\u4ea4\u6362-\u4eb2\u6838\u53d6\u4ee3-\u5206\u5b50\u5185\u78b3\u6c22\u787c\u5316\u53cd\u5e94\uff0c\u4ee522%\u7684\u6536\u7387\u83b7\u5f97BNS<\/strong>\u3002BNS<\/strong>\u7684\u5149\u5b66\u80fd\u9699\u4ec5\u4e3a1.68 eV\uff0c\u8fd9\u662fMR-TADF\u6750\u6599\u4e2d\u7684\u6700\u5c0f\u503c\u3002\u6b64\u5916\uff0cBNS<\/strong>\u5728\u8fd1\u7ea2\u5916\u533a\u5177\u6709\u5f3a\u70c8\u7684\u5438\u6536\uff0c\u5e76\u4e14\u5177\u6709\u975e\u5e38\u9ad8\u7684\u8367\u5149\u91cf\u5b50\u4ea7\u7387\uff0882%\uff09\u3001\u8f83\u5c0f\u7684\u0394E<\/em>ST<\/sub>\uff080.14 eV\uff09\u4e0e\u8f83\u957f\u7684\u5ef6\u8fdf\u8367\u5149\u5bff\u547d\uff08115 \u03bcs\uff09\uff0c\u8868\u660eBNS<\/strong>\u6781\u5177\u4f5c\u4e3a\u8fd1\u7ea2\u5916\u5149\u654f\u5242\u7684\u6f5c\u529b\u3002<\/p>\n

\"\"<\/p>\n

\u56fe3. \u8fd1\u7ea2\u5916\u5230\u84dd\u5149TTA-UC\u6027\u8d28\u7814\u7a76\uff08a\uff09BNS<\/strong>\/\u82dd\u548cBNS<\/strong>\/TIPS-BEA<\/strong>\u7ec4\u5408\u7684\u4e0a\u8f6c\u6362\u53d1\u5c04\u5149\u8c31\uff1b\uff08b\uff09BNS<\/strong>\u53d1\u5149\u4e0e\u4e0a\u8f6c\u6362\u53d1\u5149\u7684CIE\u5750\u6807\uff1b\uff08c,d\uff09BNS<\/strong>\/\u82dd\u548cBNS<\/strong>\/TIPS-BEA<\/strong>\u7ec4\u5408\u7684\u4e0a\u8f6c\u6362\u5f3a\u5ea6\u4e0e\u6fc0\u53d1\u5149\u529f\u7387\u5bc6\u5ea6\u5173\u7cfb\u56fe<\/p>\n

\u7531\u4e8eBNS<\/strong>\u5177\u6709\u8f83\u5c0f\u7684\u0394E<\/em>ST<\/sub>\uff0c\u5728TTA-UC\u8fc7\u7a0b\u4e2d\u6781\u5927\u964d\u4f4e\u4e86\u80fd\u91cf\u635f\u5931\uff0c\u5176\u4e0e\u84dd\u5149\u6e6e\u706d\u5242\u82dd\u62169,10-bis((triisopropylsilyl)ethynyl)anthracene \uff08TIPS-BEA<\/strong>\uff09\u7ec4\u5408\uff0c\u5b9e\u73b0\u4e86\u8fd1\u7ea2\u5916\u5230\u84dd\u5149\u7684TTA-UC\u53d1\u5149\uff0c\u53cd\u65af\u6258\u514b\u65af\u4f4d\u79fb\u5206\u522b\u4e3a1.01 eV\u4e0e1.03 eV\uff0c\u8fd9\u662f\u65e0\u91d1\u5c5e\u8fd1\u7ea2\u5916\u5149\u654f\u5242\u6240\u5b9e\u73b0\u7684\u6700\u5927\u503c\u3002BNS<\/strong>\/\u82dd\u548cBNS<\/strong>\/TIPS-BEA<\/strong>\u7ec4\u5408\u5177\u6709\u8f83\u4f4e\u7684\u9608\u503c\u529f\u7387\u5bc6\u5ea6\uff08\u5206\u522b\u4e3a125 mW cm-2<\/sup>\u4e0e165 mW cm-2<\/sup>\uff09\u4e0e\u8f83\u9ad8\u7684\u4e0a\u8f6c\u6362\u91cf\u5b50\u4ea7\u7387\uff08\u5206\u522b\u4e3a1.5%\u4e0e2.9%\uff0c\u7406\u8bba\u4e0a\u9650\u4e3a50%\uff09\u3002\u6b64\u5916\uff0cBNS<\/strong>\/\u82dd\u548cBNS<\/strong>\/TIPS-BEA<\/strong>\u7ec4\u5408\u8fd8\u5177\u6709\u6e6e\u706d\u5242\u6d53\u5ea6\u4f4e\uff08\u5206\u522b\u4e3a210 \u03bcM\u548c50 \u03bcM\uff09\u4e0e\u6fc0\u53d1\u5149\u7a7f\u900f\u8ddd\u79bb\u6df1\u7b49\u4f18\u52bf\uff0c\u4e3a\u8fd1\u7ea2\u5916\u5149\u9a71\u52a8\u7684TTA-UC\u5e94\u7528\u4e8e\u5149\u50ac\u5316\u4e0e3D\u6253\u5370\u7b49\u9886\u57df\u6253\u4e0b\u4e86\u575a\u5b9e\u7684\u57fa\u7840\u3002<\/p>\n

 <\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u5de5\u4f5c\u8bbe\u8ba1\u5408\u6210\u4e86\u9996\u4f8b\u5177\u6709MR-TADF\u7279\u6027\u7684\u787c\u6c2e\u6742\u7a20\u82b3\u70c3\u8fd1\u7ea2\u5916\u5149\u654f\u5242\uff08BNS<\/strong>\uff09\uff0c\u5176\u5177\u6709\u8fd1\u7ea2\u5916\u5438\u5149\u5f3a\u3001\u0394E<\/em>ST<\/sub>\u5c0f\uff080.14 eV\uff09\u3001\u5ef6\u8fdf\u8367\u5149\u5bff\u547d\u957f\uff08115 \u03bcs\uff09\u7b49\u4f18\u70b9\u3002BNS<\/strong>\u4e0e\u84dd\u5149\u6e6e\u706d\u5242TIPS-BEA<\/strong>\u7684\u7ec4\u5408\u5b9e\u73b0\u4e86\u65e0\u91d1\u5c5e\u8fd1\u7ea2\u5916\u5149\u654f\u5242\u6fc0\u53d1\u7684\u8fd1\u7ea2\u5916\u5230\u84dd\u5149TTA-UC\u4f53\u7cfb\u4e2d\u6700\u5927\u7684\u53cd\u65af\u6258\u514b\u65af\u4f4d\u79fb\uff081.03 eV\uff09\u3002\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u4e3a\u65e0\u91d1\u5c5e\u8fd1\u7ea2\u5916\u5149\u654f\u5242\u7684\u5f00\u53d1\u63d0\u4f9b\u4e86\u65b0\u9896\u7684\u8bbe\u8ba1\u7b56\u7565\uff0c\u4e5f\u4e3a\u8fd1\u7ea2\u5916\u5149\u9a71\u52a8\u7684TTA-UC\u6280\u672f\u5e94\u7528\u4e8e\u672a\u6765\u5149\u7535\u4e0e\u751f\u7269\u9886\u57df\u63d0\u4f9b\u4e86\u65b0\u7684\u673a\u9047\u3002<\/p>\n

 <\/p>\n

\u8fd9\u4e00\u6210\u679c\u8fd1\u671f\u53d1\u8868\u5728Angew<\/em><\/strong>. Chem<\/em>. Int<\/em>. Ed<\/em>.<\/strong>\u4e0a\uff0c\u6587\u7ae0\u7684\u7b2c\u4e00\u4f5c\u8005\u662f\u5357\u5f00\u5927\u5b66\u674e\u7ee7\u5764\u535a\u58eb\u4e0e\u535a\u58eb\u7814\u7a76\u751f\u5f20\u94ed\u5b87\uff0c\u901a\u8baf\u4f5c\u8005\u662f\u5357\u5f00\u5927\u5b66\u738b\u5c0f\u91ce\u7814\u7a76\u5458<\/strong>\u4e0e\u9ec4\u7075\u7814\u7a76\u5458<\/strong>\u3002\u8be5\u5de5\u4f5c\u5f97\u5230\u57fa\u91d1\u59d4\u3001\u79d1\u6280\u90e8\u3001\u5929\u6d25\u5e02\u6d77\u6cb3\u5b9e\u9a8c\u5ba4\u53ca\u4e2d\u592e\u9ad8\u6821\u57fa\u672c\u79d1\u7814\u4e1a\u52a1\u8d39\u7684\u652f\u6301\u3002\u5357\u5f00\u5927\u5b66\u5e9e\u4ee3\u6587\u6559\u6388\u5bf9\u8be5\u5de5\u4f5c\u7ed9\u4e88\u4e86\u6089\u5fc3\u6307\u5bfc\u4e0e\u5927\u529b\u652f\u6301\u3002<\/p>\n

 <\/p>\n

 <\/p>\n

\u539f\u6587\u4fe1\u606f\uff1a<\/p>\n

NIR-Absorbing B,N-Heteroarene as Photosensitizer for High-Performance NIR-to-Blue Triplet-Triplet Annihilation Upconversion<\/p>\n

Ji-Kun Li\u2020<\/sup>, Ming-Yu Zhang\u2020<\/sup>, Le Zeng, Ling Huang*, and Xiao-Ye Wang*<\/p>\n

Angew<\/em>. Chem<\/em>. Int<\/em>. Ed<\/em>. 2023<\/strong>, e202303093<\/p>\n

 <\/p>\n

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\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

\"\"<\/p>\n

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\"\"<\/p>\n

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