{"id":249473,"date":"2023-04-17T06:09:31","date_gmt":"2023-04-16T22:09:31","guid":{"rendered":"\/\/m.iemloyee.com\/?p=249473"},"modified":"2023-04-14T11:09:57","modified_gmt":"2023-04-14T03:09:57","slug":"nat-commun%e9%93%82-%e5%af%8c%e5%8b%92%e7%83%af%e7%95%8c%e9%9d%a2%e9%93%82%e4%bd%8d%e7%82%b9%e7%9a%84%e5%a4%9a%e6%a0%b7%e6%80%a7%e5%8a%a0%e9%80%9f%e7%a2%b1%e6%80%a7%e6%9e%90%e6%b0%a2","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=249473","title":{"rendered":"Nat.Commun:\u94c2\/\u5bcc\u52d2\u70ef\u754c\u9762\u94c2\u4f4d\u70b9\u7684\u591a\u6837\u6027\u52a0\u901f\u78b1\u6027\u6790\u6c22"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/span><\/p>\n

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 <\/p>\n

\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/span><\/p>\n

\u00a0 \u00a0\u8fd1\u65e5\uff0c\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66\u6c6a\u78ca\uff08Lei Wang\uff09\u3001Sergey M. Kozlov\u3001\u6d59\u6c5f\u5927\u5b66\u5b59\u6587\u5e73\uff08Wenping Sun\uff09\u7b49\u62a5\u9053\u5c06Pt\u7c07\u951a\u5b9a\u5728\u4e8c\u7ef4\u5bcc\u52d2\u70ef\u7eb3\u7c73\u7247\u4e0a\uff08PtC60<\/sub>\uff09\uff0c\u663e\u8457\u7684\u63d0\u9ad8Pt\u7684\u78b1\u6027HER\u50ac\u5316\u672c\u5f81\u6d3b\u6027\uff0c\u6bd4\u5546\u4e1aPt\/C\u50ac\u5316\u5242\u63d0\u9ad8\u4e8612\u500d\u3002\u76f8\u5173\u7684\u7814\u7a76\u6210\u679c\u4ee5\u201cDiversity of platinum-sites at platinum\/fullerene interface accelerates alkaline hydrogen evolution<\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Communications<\/em><\/strong>\u4e0a\u3002<\/p>\n

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\u00a0 \u00a02<\/strong>\u3001<\/strong>\u8fd9\u9879\u5de5\u4f5c\u53d1\u73b0<\/strong>\u5728<\/strong>PtC60<\/sub>\u7684\u4e0d\u540c\u754c\u9762\u4e0a\u660e\u663e\u5730\u51fa\u73b0\u7535\u8377\u518d\u5206\u5e03\u73b0\u8c61\u3002\u5e76\u4e14\u8be6\u7ec6\u7684<\/strong>\u52a8\u529b\u5b66\u548c\u8ba1\u7b97\u7814\u7a76\u63ed\u793a\u4e86\u589e\u5f3a\u6d3b\u6027\u7684\u8d77\u6e90\u662f\u94c2<\/strong>\/<\/strong>\u5bcc\u52d2\u70ef\u754c\u9762\u5904\u94c2\u4f4d\u70b9\u5bf9<\/strong>HER<\/strong>\u8fc7\u7a0b\u4e2d\u95f4\u4f53\u7684\u6cdb\u7ed3\u5408\u80fd\u7279\u6027\uff0c<\/strong>\u8fd9\u4e3a<\/strong>\u78b1\u6027<\/strong>HER<\/strong>\u4e2d\u7684\u6240\u6709\u57fa\u672c\u6b65\u9aa4<\/strong>\u4ea7\u751f\u4e86<\/strong>\u9ad8\u6d3b\u6027\u4f4d\u70b9\uff0c\u591a\u6b65\u9aa4\u534f\u540c\u63d0\u5347<\/strong>HER<\/strong>\u6027\u80fd<\/strong>\u3002<\/strong><\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011\"\"<\/strong><\/span><\/p>\n

\u56fe<\/strong>1<\/strong> PtC60<\/sub>\u50ac\u5316\u5242\u7684\u5408\u6210\u4e0e\u8868\u5f81\uff1a\uff08a\uff09 PtC60<\/sub>\u7684\u5408\u6210\u8def\u7ebf\u793a\u610f\u56fe\u3002\uff08b\uff09 PtC60<\/sub>\u7684TEM\u56fe\u3002\uff08c\uff09b\u00a0\u4e2d\u533a\u57dfc’\u7684\u76f8\u5e94FFT\u3002\uff08d\uff09\u00a0b\u00a0\u4e2d\u533a\u57dfd’\u76f8\u5e94\u7684\u9006-FFT\u00a0\u3002\uff08e\uff09PtC60<\/sub>\u7684AFM\u56fe\u50cf\u3002\uff08f\uff09\u00a0b\u4e2d\u533a\u57dff’\u7684\u9ad8\u5206\u8fa8\u7387TEM\u56fe\u3002\uff08g\uff09 PtC60<\/sub>\u7684 STEM-EDS\u6620\u5c04\u56fe\u3002 \u00a92023 The Author(s)<\/p>\n

\"\"<\/strong><\/span><\/p>\n

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\"\"<\/strong><\/span><\/p>\n

\u56fe<\/strong>3<\/strong> \u78b1\u6027HER\u6027\u80fd\uff1a\uff08a\uff09\u8d1f\u8f7d\u91cf\u4e3a 0.4 mg cm\u00a0-2<\/sup>\u7684PtC60<\/sub>, Pt\/C\uff0cPt NC\u548c\u7eafC60<\/sub>\u50ac\u5316\u5242\u7684 LSV\u3002(b)\u00a0 a\u4e2d\u50ac\u5316\u5242\u5728 10\u300150\u3001150 mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u8fc7\u7535\u52bf\u3002(c)\u4f4e\u8d1f\u8f7d\u91cf\uff080.004 mg cm-2<\/sup>\uff09\u7684LSV\u3002(d)\u50ac\u5316\u5242\u8d1f\u8f7d\u91cf\u4e3a0.004 mg cm-2<\/sup>\u7684\u50ac\u5316\u5242\u7684TOF\u00a0\u3002(e)\u4ece\u00a0c\u00a0\u4e2d\u7684 LSV \u83b7\u5f97\u7684\u76f8\u5e94Tafel\u56fe\u3002(f)\u50ac\u5316\u5242\u5728-40 mV (RHE) \u4e0b\u7684 EIS\u56fe\u3002\u00a92023 The Author(s)<\/p>\n

\"\"<\/strong><\/span><\/p>\n

\u56fe<\/strong>4 <\/strong>\u7406\u8bba\u5206\u6790\uff1a\uff08a\uff09\u6240\u91c7\u7528\u7684 Pt\/C60<\/sub>\u6a21\u578b\u3002\uff08b\uff09Pt\u548cC60<\/sub>\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u5bfc\u81f4\u7684\u7535\u5b50\u5bc6\u5ea6\u5dee\u5f02\u3002\uff08c\uff09H\uff08\u9876\u90e8\uff09\u3001OH\uff08\u4e2d\u95f4\uff09\u548c H2<\/sub>O\uff08\u5e95\u90e8\uff09\u5728\u65e0\u652f\u6491 Pt NC \u4e0a\u7ed3\u5408\u5409\u5e03\u65af\u81ea\u7531\u80fd\u7684\u5206\u5e03\u3002\uff08d\uff09\u4e0d\u540c\u78b1\u6027HER\u53cd\u5e94\u6b65\u9aa4\u5bf9Pt\/C60<\/sub> (011)\u548cPt\/\u77f3\u58a8\u70ef\u53cd\u5e94\u901f\u7387\u5e38\u6570\uff0c\u76f8\u5bf9\u4e8e\u901a\u8fc7\u6d3b\u5316\u80fd\u4f30\u8ba1\u7684\u65e0\u8d1f\u8f7dPt NCs\u3002\uff08e\uff09\u7531\u5fae\u52a8\u529b\u5b66\u6a21\u578b\u8ba1\u7b97\u7684\u8d1f\u8f7d Pt\/C60<\/sub>\u3001Pt\/\u77f3\u58a8\u70ef\u548c\u672a\u652f\u6301\u7684 Pt NCs \u7684 LSV\u3002\uff08f\uff09\u00a0Pt\/C60<\/sub>\u4e0a\u53cd\u5e94\u6b65\u9aa4\u56fe\u3002\u00a92023 The Author(s)<\/p>\n

\"\"<\/strong><\/span><\/p>\n

\u56fe5 AEM\u7535\u89e3\u69fd\u7684\u6027\u80fd\uff1a\uff08a\uff09\u4f7f\u7528 PtC60<\/sub>\u2009|\u00a0|IrO2<\/sub>\u00a0, PtC |\u00a0|IrO2<\/sub>\u548cPt NCs |\u00a0|IrO2<\/sub>\u7684AEM\u7535\u89e3\u69fd\u7684LSV\u3002\u200b\u200b\uff08b\uff09\u7535\u6d41\u5bc6\u5ea6\u4e3a1 A cm\u00a0\u20132<\/sup>\u65f6\u7684\u7535\u6c60\u7535\u538b\u548c\u76f8\u5e94\u7684\u80fd\u91cf\u6548\u7387\u3002\uff08c\uff09\u00a0AEM\u7535\u89e3\u69fd\u57281 A cm\u00a0\u20132<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u8010\u4e45\u6027\u6d4b\u8bd5\u3002\u00a92023 The Author(s)<\/p>\n

 <\/p>\n

\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/span><\/p>\n

\u00a0 \u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u5408\u7406\u5f00\u53d1\u4e86\u4e8c\u7ef4 C60<\/sub>\u7eb3\u7c73\u7247\uff0c\u5e76\u5c06Pt \u7eb3\u7c73\u56e2\u7c07\u951a\u5b9a\u5728\u7eb3\u7c73\u7247\u4e4b\u4e0a\u3002C60<\/sub>\u548cPt\u4e4b\u95f4\u5f62\u6210\u4e86\u5bf9\u78b1\u6027 HER \u5177\u6709\u9ad8\u6d3b\u6027\u7684\u5f02\u8d28\u7ed3\u6784\u3002\u6b64\u5916\uff0cPtC60<\/sub>\u5728\u819c\u57faAEM\u7535\u89e3\u69fd\u4e2d\u5c55\u73b0\u51fa\u9ad8\u6d3b\u6027\uff0c\u8868\u73b0\u51fa\u9ad8\u8fbe74%\u7684\u9ad8\u80fd\u91cf\u6548\u7387\u548c\u7a33\u5b9a\u6027\uff0c\u4f7f\u5176\u6210\u4e3a\u5b9e\u7528 AEM\u7535\u89e3\u7684\u6709\u524d\u9014\u9634\u6781\u6750\u6599\u5019\u9009\u8005\u4e4b\u4e00\u3002\u53e6\u5916\uff0c\u4f5c\u8005\u63d0\u51fa\u5f15\u5165\u5177\u6709\u5173\u952e\u53cd\u5e94\u4e2d\u95f4\u4f53\u4e0d\u540c\u7ed3\u5408\u80fd\u7684\u5f02\u8d28\u754c\u9762\u7684\u8bbe\u8ba1\u7b56\u7565\u53ef\u4ee5\u5e7f\u6cdb\u5e94\u7528\u4e8e\u4f9d\u8d56\u9ad8\u6027\u80fd\u7535\u50ac\u5316\u7684\u5176\u4ed6\u80fd\u6e90\u53d1\u5c55\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

\u00a0<\/strong><\/p>\n

\u539f\u6587\u8be6\u60c5\uff1a<\/strong>https:\/\/doi.org\/10.1038\/s41467-023-37404-0<\/p>\n

\u672c\u6587\u7531K . L\u64b0\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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