{"id":249282,"date":"2023-03-29T06:25:01","date_gmt":"2023-03-28T22:25:01","guid":{"rendered":"\/\/m.iemloyee.com\/?p=249282"},"modified":"2023-03-27T16:35:21","modified_gmt":"2023-03-27T08:35:21","slug":"%e5%9b%bd%e5%ae%b6%e5%ae%9e%e9%aa%8c%e5%ae%a4%e5%85%88%e8%bf%9b%e5%be%ae%e7%bb%93%e6%9e%84%e5%8d%8f%e5%90%8c%e5%88%9b%e6%96%b0%e4%b8%ad%e5%bf%83%e4%b8%8e%e5%8d%97%e4%ba%ac%e5%a4%a7%e5%ad%a6%ef%bc%9a","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=249282","title":{"rendered":"\u56fd\u5bb6\u5b9e\u9a8c\u5ba4\u5148\u8fdb\u5fae\u7ed3\u6784\u534f\u540c\u521b\u65b0\u4e2d\u5fc3\u4e0e\u5357\u4eac\u5927\u5b66\uff1a\u5206\u5b50\u5c42\u6c89\u79ef\u950c\u916e\u819c\u8bf1\u5bfc\u9502\u91d1\u5c5e\u8d1f\u6781\u5bccLiF\u754c\u9762\u7684\u5f62\u6210"},"content":{"rendered":"<p>\u4e00\u3001 \u3010\u5bfc\u8bfb\u3011\u00a0<\/p>\n<p>\u00a0 \u00a0 \u00a0 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Tank\u53d1\u5e03\u7684\u300a\u4e2d\u56fd\u9502\u79bb\u5b50\u7535\u6c60\u7535\u89e3\u6db2\u884c\u4e1a\u53d1\u5c55\u767d\u76ae\u4e66\uff082022\uff09\u5e74)\u300b\uff0c\u9884\u8ba1\u52302025\u5e74\u5168\u7403\u9502\u79bb\u5b50\u7535\u6c60\u7535\u89e3\u6db2\u9700\u6c42\u91cf\u5c06\u8fbe216.3\u4e07\u5428\uff0c2030\u5e74\u9502\u79bb\u5b50\u7535\u6c60\u7535\u89e3\u6db2\u9700\u6c42\u91cf\u5c06\u8fbe\u5230548.5\u4e07\u5428\uff0c\u5176\u4e2d85%\u4ee5\u4e0a\u7684\u9700\u6c42\u91cf\u5c06\u7531\u4e2d\u56fd\u4f01\u4e1a\u6765\u6ee1\u8db3\u3002<\/p>\n<p>\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/p>\n<p>\u00a0 \u00a0 \u00a0 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\u00a0\u56fd\u5bb6\u5b9e\u9a8c\u5ba4\u5148\u8fdb\u5fae\u7ed3\u6784\u534f\u540c\u521b\u65b0\u4e2d\u5fc3\u4e0e\u5357\u4eac\u5927\u5b66\u5de5\u7a0b\u4e0e\u5e94\u7528\u79d1\u5b66\u5b66\u9662\u7684\u5f20\u4f1a\u521a\u7814\u7a76\u5458\u548c\u674e\u7231\u4e1c\u6559\u6388\u56e2\u961f\uff0c\u5408\u4f5c\u63d0\u51fa\u5229\u7528\u5206\u5b50\u5c42\u6c89\u79ef\u6280\u672f\u539f\u4f4d\u6784\u7b51\u5bcc\u542bLiF\u7684SEI\uff0c\u5b9e\u73b0\u9502\u91d1\u5c5e\u7535\u6c60\u7a33\u5b9a\u5faa\u73af\u3002\u91c7\u7528\u5206\u5b50\u5c42\u6c89\u79ef(MLD)\u6280\u672f\u5728\u4e09\u7ef4\u94dc\u7eb3\u7c73\u7ebf(CuNWs)\u4e0a\u5171\u5f62\u5236\u5907\u4e86\u6c27\u5316\u950c(ZnHQ)\u3002\u6781\u5316\u540e\uff0c\u5177\u6709\u5076\u6781\u77e9\u7684\u950c\u57fa\u5bf9\u82ef\u4e8c\u915a(ZnHQ)\u4e2d\u7684\u542b\u6c27\u5b98\u80fd\u56e2\u53ef\u4ee5\u4f5c\u4e3a\u4eb2\u6838\u57fa\u56e2\uff0c\u63d0\u4f9b\u591a\u4f59\u7684\u7535\u5b50\u52a0\u5feb\u53cc\u4e09\u6c1f\u7532\u78fa\u9170\u80fa\u9502(LiTFSI)\u964d\u89e3\uff0c\u5f97\u5230\u7684\u5bccLiF\u7684SEI\u4fc3\u8fdbLi\u79bb\u5b50\u6269\u6563\uff0c\u5e76\u6291\u5236\u94dc\u8868\u9762\u9502\u679d\u72b6\u751f\u957f\u3002CuNW@ZnHQ\u7684\u5bf9\u79f0\u7535\u6c60\u57281 mA cm<sup>\u22122<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8868\u73b0\u51fa\u8d85\u8fc77000 h\u7684\u9ad8\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u8fd9\u9879\u5de5\u4f5c\u4ee5\u6807\u9898\u4e3a\uff1a\u201cMolecular-Layer-Deposited Zincone Films Induce the Formation of LiF-Rich Interphase for Lithium Metal Anodes\u201d\uff0c\u53d1\u8868\u5728Advanced Energy Materials\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249283\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/0-0.png\" alt=\"\" width=\"1322\" height=\"395\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/0-0.png 1322w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/0-0-300x90.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/0-0-768x229.png 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/0-0-1024x306.png 1024w\" sizes=\"(max-width: 1322px) 100vw, 1322px\" \/><\/p>\n<p>\u00a0\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/p>\n<p>1.\u901a\u8fc7\u8fd9\u79cd\u65b9\u6cd5\uff0cSEI\u4fc3\u8fdb\u4e86Li\u7684\u4f20\u8f93\uff0c\u5207\u65ad\u4e86\u7535\u5b50\u4f20\u5bfc\uff0c\u5e76\u6291\u5236\u4e86\u9502\u679d\u6676\u7684\u751f\u957f\u3002<\/p>\n<p>2.\u6b64\u5916\uff0cZnHQ\u7684\u950c\u539f\u5b50\u7531\u4e8e\u5176\u4eb2\u9502\u6027\u800c\u8bf1\u5bfc\u6709\u5229\u7684Li\u6c89\u79ef\u3002\u7531MLD\u5b9e\u73b0\u7684\u8fd9\u4e9b\u4f18\u70b9\u4f7f\u5f97ZnHQ\u6539\u6027\u7684CuNW(CuNW@ZnHQ)\u6210\u4e3a\u7406\u60f3\u7684Li\u91d1\u5c5e\u9633\u6781\uff0c\u5176\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u5faa\u73af\u80fd\u529b\u3002<\/p>\n<p>\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249284\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-1-2.png\" alt=\"\" width=\"917\" height=\"681\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-1-2.png 917w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-1-2-300x223.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-1-2-768x570.png 768w\" sizes=\"(max-width: 917px) 100vw, 917px\" \/><\/p>\n<p>\u56fe1.\u793a\u610f\u56fe\uff1aa)\u5728\u950c\u916eMLD\u4e2d\u7684\u5316\u5b66\u53cd\u5e94;b)CuNW@ZnHQ\u4e0a\u7684SEI\u5f62\u6210\u548cc)\u5728ZnHQ\u8bf1\u5bfc\u7684\u5bcc\u542bLiF\u7684SEI\u4e0b\u7684\u5747\u5300Li\u6c89\u79ef\u8fc7\u7a0b;d)CuNW\u4e0a\u7684SEI\u5f62\u6210\u548ce)CuNW\u4e0a\u7684\u975e\u5747\u5300Li\u6c89\u79ef\u8fc7\u7a0b\u3002\u00a92023 Advanced Energy Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249285\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2-2-1.png\" alt=\"\" width=\"805\" height=\"837\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2-2-1.png 805w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2-2-1-289x300.png 289w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2-2-1-768x799.png 768w\" sizes=\"(max-width: 805px) 100vw, 805px\" \/><\/p>\n<p>\u56fe2.SEM\u56fe\u50cf:a)3D\u70e7\u7ed3\u94dc\u9884\u6210\u578b, b) CuNW@ZnHQ, c) 3 d CuNW@ZnHQ;d) ZnHQ\u5305\u8986 CuNW\u7684TEM\u56fe\u50cf;e) CuNW@ZnHQ\u7eb3\u7c73\u7ebf\u7684EDS\u5143\u7d20\u6620\u5c04\u56fe\u50cf; f) CuNW@ZnHQ \u7684SEM\u56fe\u50cf;g) P-Cu\u548cCuNW \u7684ECSA;h) P-Cu, CuNW, CuNW@ZnHQ \u7684XRD; i)ZnHQ\u7684\u7ea2\u5916\u5149\u8c31\u8c31\u3002ZnHQ\u7684XPS\u8c31: j) C 1s, k) O 1s, l)Zn 2p\u7684\u4fe1\u53f7\u3002\u00a92023 Advanced Energy Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249286\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-3-1.png\" alt=\"\" width=\"1000\" height=\"728\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-3-1.png 1000w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-3-1-300x218.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-3-1-768x559.png 768w\" sizes=\"(max-width: 1000px) 100vw, 1000px\" \/><\/p>\n<p>\u56fe3 \u00a0P-Cu\u7684\u7535\u5316\u5b66\u6027\u80fd\u548c\u5faa\u73af\u7a33\u5b9a\u6027, CuNW@ZnHQ, CuNW\u3002a)\u7535\u538b\u66f2\u7ebf\u7684\u9540\u9502\u80fd\u529b1 mAh cm<sup>\u22122<\/sup>\u548c0.5 mA cm<sup>\u22122<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u3002CEs\u7684\u9540\u9502\/\u5265\u79bbb)\u57280.5 mA cm<sup>\u22122<\/sup> (1 mAh cm<sup>\u22122<\/sup>)\u548cc)\u5728\u5265\u79bb\u8fc7\u7a0b2 mA cm<sup>\u22122<\/sup> (5 mAh cm<sup>\u22122<\/sup>)\u622a\u6b62\u7535\u538b\u4e3a1.0 V vs Li<sup>+<\/sup> \/Li\u3002d)\u989d\u5b9a\u5bb9\u91cf\u548c\u7535\u538b\u66f2\u7ebf\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u9a6c\u4ece0.5\u52305 mA cm<sup>\u22122<\/sup>\u3002e) CuNW\u548cCuNW@ZnHQ\u5728\u7b2c10\u548c100\u5468\u671f\u7684EIS\u5149\u8c31\u3002\u65f6\u95f4-\u7535\u538b\u66f2\u7ebf\u5728f)\u5bc6\u5ea6\u4e0b5 mA cm<sup>\u22122<\/sup> (15 mAh cm<sup>\u22122<\/sup>)\u548cg, h)1 mA cm<sup>\u22122<\/sup> (1 mAh cm<sup>\u22122<\/sup>)\u3002\u00a92023 Advanced Energy Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249287\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-4-1.png\" alt=\"\" width=\"1000\" height=\"723\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-4-1.png 1000w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-4-1-300x217.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-4-1-768x555.png 768w\" sizes=\"(max-width: 1000px) 100vw, 1000px\" \/><\/p>\n<p>\u56fe4 LiTFSI\u964d\u89e3\u7684\u673a\u7406\u5206\u6790\uff1aCuNW\u548cCuNW@ZnHQ\u7684XPS\u5149\u8c31\uff1aa)C 1s\u548cb)F 1s\u4fe1\u53f7\u3002c)LiTFSI\u548c\u950c\u916e\u5728\u7535\u5b50\u5bc6\u5ea6\u7b49\u503c\u9762\u5904\u7684\u9759\u7535\u52bf\u5206\u5e03\uff0cr = 0.2|e|bohr<sup>-3<\/sup>\u3002d)Cu\u4e0a\u5e26\u8d1f\u7535\u8377\u7684ZnHQ\u7684\u7535\u5b50\u5dee\u793a\u56fe(\u5411\u6676\u80de\u6dfb\u52a0\u4e00\u4e2a\u7535\u5b50\u4ee5\u8bf4\u660e\u8d1f\u7535\u8377)\u3002LiTFSI\u5206\u89e3\u524de)\u548c\u5206\u89e3\u540ef)\u7684\u7535\u5b50\u5dee\u56fe(\u9ec4\u8272\u548c\u9752\u8272\u5206\u522b\u8868\u793a\u7535\u8377\u79ef\u7d2f\u548c\u8017\u5c3d)\u3002\u663e\u793a\u9000\u5316\u52a8\u6001\u7684AIMD\u6a21\u62df\u5feb\u7167\uff1ag)0 fs\uff0ch)150 fs\uff0ci)275 fs\uff0c\u548cj)475 fs(\u6570\u5b57\u8868\u793a\u4e00\u4e2a\u5355\u72ec\u7fa4\u7684\u77ac\u65f6\u8d1d\u5fb7\u7535\u8377\u7684\u603b\u548c)\u3002\u00a92023 Advanced Energy Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249288\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-5-1.png\" alt=\"\" width=\"996\" height=\"703\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-5-1.png 996w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-5-1-300x212.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-5-1-768x542.png 768w\" sizes=\"(max-width: 996px) 100vw, 996px\" \/><\/p>\n<p>\u56fe5 \u4e0d\u540c\u591a\u573a\u4f5c\u7528\u4e0b\u9540\u9502\u7684\u5f62\u8c8c\u53d8\u5316a)CuNW\u3001d)CuNW@ZnHQ\u548cg)\u9540\u9502\u540e\u94dc\u7b94\u7684SEM\u56fe\u50cf\uff0c\u5bb9\u91cf\u4e3a2.0 mAh cm<sup>\u22122<\/sup>\u3002b)\u4f7f\u7528CuNW\u7684Li<sup>+<\/sup>\u901a\u91cf\u7684\u6d41\u7ebf\u65b9\u5411\u4f7f\u7528e)CuNW@ZnHQ\u548ch)Cu\u7b94\u7684\u7535\u89e3\u8d28\u754c\u9762\u5904\u7684Li<sup>+<\/sup>\u901a\u91cf\u7684COMSOL\u6a21\u62df\u3002\u5728\u5177\u6709c)CuNW\u3001f)CuNW@ ZnHQ\u548ci)Cu\u7b94\u7684\u7535\u89e3\u8d28\u754c\u9762\u5904\u7684\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u5206\u5e03\u7684COMSOL\u6a21\u62df\u3002\u00a92023 Advanced Energy Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-249289\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6-6-1.png\" alt=\"\" width=\"740\" height=\"732\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6-6-1.png 740w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6-6-1-300x297.png 300w\" sizes=\"(max-width: 740px) 100vw, 740px\" \/><\/p>\n<p>\u56fe6\u00a0 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cm<sup>\u22122<\/sup>\u4e0b\u5faa\u73af1000\u6b21\uff0c\u5bb9\u91cf\u4fdd\u6301\u7387\u4e3a90%\u3002\u8fd9\u9879\u5de5\u4f5c\u8868\u660e\uff0cMLD\u6539\u6027\u7684\u591a\u5b54\u94dc\u7eb3\u7c73\u7ebf\u4e3a\u6539\u5584\u9502\u91d1\u5c5e\u57fa\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd\u63d0\u4f9b\u4e86\u53e6\u4e00\u79cd\u673a\u4f1a\uff0cMLD\u6280\u672f\u4e3a\u4e0b\u4e00\u4ee3\u9ad8\u80fd\u9502\u91d1\u5c5e\u7535\u6c60\u5e26\u6765\u4e86\u65b0\u7684\u673a\u9047\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>\u539f\u6587\u8be6\u60c5\uff1ahttps:\/\/doi.org\/10. 1002\/aenm.202204002<\/p>\n<p>\u672c\u6587\u7531\u91d1\u7235\u4f9b\u7a3f<\/p>\n<p>&nbsp;<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u4e00\u3001 \u3010\u5bfc\u8bfb\u3011\u00a0 \u00a0 \u00a0 \u00a0 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