{"id":248910,"date":"2023-04-10T06:07:50","date_gmt":"2023-04-09T22:07:50","guid":{"rendered":"\/\/m.iemloyee.com\/?p=248910"},"modified":"2023-04-07T15:11:11","modified_gmt":"2023-04-07T07:11:11","slug":"advanced-functional-materials%ef%bc%9a-%e6%96%b0%e5%8f%91%e7%8e%b0%ef%bc%81%e8%b0%83%e6%8e%a7mos_2%e4%b8%89%e5%85%83%e5%bc%82%e8%b4%a8%e7%bb%93%e6%9e%84%e5%a2%9e%e5%bc%ba%e6%9e%90%e6%b0%a2%e5%82%ac","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=248910","title":{"rendered":"Advanced Functional Materials\uff1a \u65b0\u53d1\u73b0\uff01\u8c03\u63a7MOS_2\u4e09\u5143\u5f02\u8d28\u7ed3\u6784\u589e\u5f3a\u6790\u6c22\u50ac\u5316\u53cd\u5e94\uff01"},"content":{"rendered":"
\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n \u00a0 \u00a0 \u00a0 \u00a0 \u00a0\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u4e8c\u786b\u65cf\u5316\u7269\uff082D-TMDs\uff09\u53ca\u5176\u76f8\u53d8\u5de5\u7a0b\u90fd\u7ecf\u5386\u4e86\u590d\u5174\uff0c\u56e0\u4e3a\u4f7f\u7528\u9502\u5d4c\u5165\u65b9\u6cd5\u4ece\u534a\u5bfc\u4f53MoS2<\/sub>\u4e2d\u83b7\u5f97\u4e86\u91d1\u5c5eMoS2<\/sub>\u3002\u8fd9\u79cd\u5e76\u7f6e\u7684\u6839\u6e90\u5728\u4e8e\uff0c\u7531\u4e8e\u914d\u4f4d\u7ed3\u6784\u7684\u7578\u53d8\uff0c\u4f53\u76f8\u4e09\u68f1\u67f1MoS2<\/sub>\uff082H-MoS2<\/sub>\uff09\u548c\u516b\u9762\u4f53MoS2<\/sub>\uff081T-MoS2<\/sub>\uff09\u4e4b\u95f4\u5b8c\u5168\u4e0d\u540c\u7684\u7535\u5b50\u7535\u5bfc\u7387\uff0c\u5c24\u5176\u662f\u5728\u7535\u5b50\u5668\u4ef6\u3001\u529f\u80fd\u5668\u4ef6\u3001\u50a8\u80fd\u3001\u7535\u50ac\u5316\u7b49\u9886\u57df\u3002\u4e24\u76f8\u53ef\u4ee5\u901a\u8fc7\u786b\u5c5e\u5143\u7d20\u5c42\u5185\u539f\u5b50\u5e73\u9762\u7684\u5e73\u6ed1\u6ed1\u52a8\u8fdb\u884c\u53ef\u9006\u8f6c\u6362\u3002\u4f5c\u4e3a\u4e00\u79cd\u65b0\u578b\u7684\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u7535\u50ac\u5316\u5242\uff0c1T\u6216\u626d\u66f2\u76841T\u76f8\u56e0\u5176\u57fa\u9762\u4e30\u5bcc\u7684\u6d3b\u6027\u4f4d\u70b9\u4ee5\u53ca\u7535\u6781\u548c\u7535\u89e3\u8d28\u754c\u9762\u4e4b\u95f4\u51fa\u8272\u7684\u7535\u8377\u8f6c\u79fb\u80fd\u529b\u800c\u5907\u53d7\u5173\u6ce8\u3002\u7136\u800c\u5728\u5229\u75282D-TMD\u76f8\u53d8\u5de5\u7a0b\u8303\u4f8b\u65f6\u4ecd\u7136\u5b58\u5728\u4e00\u4e9b\u969c\u788d\uff0c\u9996\u5148\uff0c\u7531\u4e8e\u4e0d\u5229\u7684\u70ed\u529b\u5b66\u4e9a\u7a33\u6001\uff0c\u5728\u63d0\u9ad8\u91d1\u5c5e\u76f8\u8f6c\u6362\u542b\u91cf\u6216\u6b65\u8fdb\u7ecf\u6d4e\u65b9\u5f0f\u76f4\u63a5\u5408\u6210\u65b9\u9762\u7684\u6301\u7eed\u52aa\u529b\u7f3a\u4e4f\u5de5\u4e1a\u5e94\u7528\u5fc5\u9700\u7684\u7279\u5f81\uff1b\u5176\u6b21\uff0c\u5c06\u8ba1\u7b97\u548c\u76f4\u89c2\u7684\u5b9e\u9a8c\u65b9\u6cd5\u7ed3\u5408\uff0c\u4e86\u89e3\u76f8\u53d8\u7684\u5b9e\u9645\u673a\u5236\uff0c\u4e3a\u9ad8\u4ea7\u91cf\u5730\u83b7\u5f97\u7a33\u5b9a\u7684\u91d1\u5c5e\u76f8\u5960\u5b9a\u57fa\u7840\u4e5f\u5f88\u8feb\u5207\uff1b\u6700\u540e\uff0c2H\/1T\u30012H\/1T’\u548c1T\/1T’\u4e4b\u95f4\u7684\u5f02\u8d28\u754c\u9762\u5728HER\u8fc7\u7a0b\u4e2d\u4f5c\u4e3a\u6d3b\u6027\u4f4d\u70b9\u7684\u8bc6\u522b\u4ece\u672a\u88ab\u5b9e\u9a8c\u8bc1\u660e\uff0c\u4e5f\u6ca1\u6709\u901a\u8fc7\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8fdb\u884c\u8ba8\u8bba\u3002<\/p>\n \u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n \u00a0 \u00a0 \u00a0 \u00a0 <\/strong>\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u4e8c\u786b\u5316\u7269\uff082D-TMD\uff09\u4ece\u534a\u5bfc\u4f53\uff082H\uff09\u5230\u91d1\u5c5e\uff081T\uff0c1T’\uff09\u76f8\u7684\u76f8\u53d8\u8fc7\u7a0b\u4e3a\u6790\u6c22\u50ac\u5316\u7684\u8fed\u4ee3\u63d0\u4f9b\u4e86\u65b9\u5411\u6027\u3002\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u76f8\u5de5\u7a0b\u65b9\u6cd5\u5f97\u5230\u4e86\u6df1\u5165\u63a2\u7d22\uff0c\u4f5c\u4e3a\u5728\u80fd\u91cf\u5b58\u50a8\u548c\u50ac\u5316\u9886\u57df\u53d1\u73b0\u7528\u4e8e\u7535\u5b50\u548c\u7535\u6781\u8bbe\u5907\u7684\u4f4e\u6210\u672c\u65b0\u578b\u7eb3\u7c73\u6750\u6599\u7684\u5b9e\u7528\u5de5\u5177\u3002\u7136\u800c\uff0c2H\/1T\u30012H\/1T’\u62161T\/1T’\u4e4b\u95f4\u7684\u5f02\u8d28\u7ed3\u6784\u5728\u7535\u50ac\u5316\u8fc7\u7a0b\u4e2d\u4f5c\u4e3a\u5173\u952e\u6d3b\u6027\u4f4d\u70b9\u53d1\u6325\u4f5c\u7528\u800c\u88ab\u5ffd\u89c6\u3002\u6b64\u9879\u7814\u7a76\u62a5\u544a\u4e86\u4e00\u79cd\u7b80\u5355\u7684\u78b3\u63ba\u6742\u8303\u4f8b\uff0c\u80fd\u591f\u589e\u5f3aMoS2<\/sub>\u76f8\u53d8\uff0c\u4ee5\u53ca\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u548c\u89e3\u91ca\u76f8\u53d8\u7684\u53cd\u76f4\u89c9\u65b9\u5411\u6027\u7684\u57fa\u672c\u539f\u7406\u3002\u5b9e\u9a8c\u548c\u6a21\u62df\u7ed3\u679c\u8868\u660e\uff0c\u78b3\u4f5c\u4e3a\u95f4\u9699\u539f\u5b50\u7684\u5b58\u5728\u6bd4\u53d6\u4ee3\u539f\u5b50\u66f4\u6709\u5229\u4e8e\u76f8\u53d8\u7684\u53d1\u751f\uff0c2H\u548c1T\u62161T’\u4e4b\u95f4\u7684\u5f02\u8d28\u754c\u9762\u66f4\u6709\u5229\u4e8e\u7535\u8377\u8f6c\u79fb\u3002\u6b63\u5982\u9884\u671f\uff0c\u4e09\u5143\u5f02\u8d28\u7ed3\u6784\u7eb3\u7c73\u8584\u819c\u5728\u5fae\u7535\u5316\u5b66\u6d4b\u91cf\u548c\u5e38\u89c4\u7535\u89e3\u7535\u6c60\u4e2d\u5747\u663e\u793a\u51fa\u4f18\u5f02\u7684\u7535\u50ac\u5316\u6d3b\u6027\u3002\u8be5\u7ed3\u679c\u4e3a2D-TMDs\u76f8\u53d8\u673a\u5236\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\uff0c\u5e76\u4e3a\u53ef\u6269\u5c55\u751f\u4ea7\u7684\u4e09\u5143\u5f02\u8d28\u7ed3\u6784\u7535\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u6307\u5bfc\u3002<\/p>\n \u00a0 \u00a0 \u00a0 \u00a0 \u9752\u5c9b\u7406\u5de5\u5927\u5b66\u3001\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u548c\u97e9\u56fd\u9996\u5c14\u5927\u5b66\u5171\u540c\u5b8c\u6210\uff0c\u901a\u8baf\u4f5c\u8005\u4e3aJin Wang\u3001Zhongxiao Song\u548cHo Won Jang\u3002<\/strong>\u76f8\u5173\u7814\u7a76\u5de5\u4f5c\u4ee5\u201cModulating Trinary-Heterostructure of MoS2<\/sub><\/strong> via Controllably Carbon Doping for Enhanced Electrocatalytic Hydrogen Evolution Reaction<\/strong>\u201d\u4e3a\u9898\u520a\u767b\u5728\u529f\u80fd\u6750\u6599\u9876\u520aAdvanced Functional Materials<\/em><\/strong>\u4e0a\u3002<\/p>\n \u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n 1\u3001\u5b8c\u6210\u4e86\u78b3\u63ba\u6742-MoS2<\/sub>\u76f8\u53d8\u7684\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u3002<\/p>\n 2\u3001\u9610\u8ff0C+MoS2<\/sub>\u5408\u6210\u4e0e\u7ed3\u6784\u8868\u5f81\uff0c\u5e76\u6d4b\u8bd5C+MoS2<\/sub>\u5bf9HER\u7684\u50ac\u5316\u6d3b\u6027\u4e0e\u7a33\u5b9a\u6027\u3002<\/p>\n 3\u3001\u8fdb\u884cDFT\u8ba1\u7b97\uff0c\u786e\u5b9a\u4e86\u5177\u6709\u591a\u79cd\u8fde\u63a5\u6a21\u5f0f\u7684\u4e0d\u540c\u754c\u9762\u7684\u6700\u4f73\u6c22\u5438\u9644\u4f4d\u70b9\u3002<\/p>\n \u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n \u56fe<\/strong>1 <\/strong>\u78b3\u63ba\u6742-MoS2<\/sub>\u76f8\u53d8\u7684\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u3002\uff08a\uff09MoS1.75<\/sub>C0.25<\/sub>\u4ece2H\u52301T\u76f8\u7684\u6676\u4f53\u7ed3\u6784\u6f14\u5316\u8fc7\u7a0b\u793a\u610f\u56fe\u3002\uff08b\uff09MoS2<\/sub>C0.25<\/sub>\u4ece2H\u52301T\u76f8\u7684\u6676\u4f53\u7ed3\u6784\u6f14\u5316\u8fc7\u7a0b\u793a\u610f\u56fe\u3002\uff08c\uff09MoS2<\/sub>\u3001MoS1.85<\/sub>C0.125<\/sub>\u3001MoS1.75<\/sub>C0.25<\/sub>\u3001MoS2<\/sub>C0.125<\/sub>\u548cMoS2<\/sub>C0.25<\/sub>\u76842H\u548c1T\u4e4b\u95f4\u7684\u80fd\u91cf\u5dee\uff08\u0394E\uff09\u3002\uff08d\uff09MoS2<\/sub>\u3001MoS1.75<\/sub>C0.25<\/sub>\u3001MoS2<\/sub>C0.125<\/sub>\u5728\u7ed3\u6784\u53d8\u5316\u8fc7\u7a0b\u4e2d\u7684\u76f8\u53d8\u52bf\u5792\u3002\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n \u56fe3\u00a0 <\/strong>C+MoS2<\/sub>\u8584\u819c\u7684\u5149\u8c31\u7814\u7a76\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n \u56fe4<\/strong>\u00a0 C+MoS2<\/sub>\u548cMoS2<\/sub>\u8584\u819c\u7684\u7535\u5b50\u663e\u5fae\u955c\u8868\u5f81\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n \u56fe5 \u00a0<\/strong>C+MoS2<\/sub>\u57280.5m\u4e2d\u57fa\u4e8e\u5fae\u7535\u5316\u5b66\u7535\u6c60\u7684\u672c\u5f81\u9178\u6027HER\u6027\u80fd\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n \u56fe6 <\/strong>H\u539f\u5b50\u5438\u9644\u5728\uff08C-doped 1T’\uff09\/2H\u00a0MoS2<\/sub> \u5e26\u4e0a\u4fef\u89c6\u56fe\u548c\u4fa7\u89c6\u56fe\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n \u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n \u00a0 \u00a0 \u00a0 \u00a0 \u00a0\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u5df2\u7ecf\u8bc1\u660e\u901a\u8fc7\u78c1\u63a7\u6e85\u5c04\u5728\u4e2d\u63ba\u6742\u78b3\u7684\u76f8\u53d8\u5de5\u7a0b\u53ef\u4ee5\u663e\u8457\u5f62\u62102H\/1T\u30012H\/1T’\u548c1T\/1T’\u7684\u5f02\u8d28\u754c\u9762\u3002\u5728\u6c89\u79ef\u8fc7\u7a0b\u4e2d\uff0c\u78b3\u63ba\u6742\u5242\u8d77\u7740\u5173\u952e\u4f5c\u7528\uff0c\u8bf1\u5bfc\u4ece2H\u52301T\u62161T’\u7684\u76f8\u53d8\u4ee5\u5f62\u6210\u4e09\u5143\u5f02\u8d28\u7ed3\uff0c\u66f4\u91cd\u8981\u7684\u662f\uff0c\u901a\u8fc7\u5e94\u53d8\u9489\u624e\u6548\u5e94\u7a33\u5b9a\u91d1\u5c5e\u76f8\u3002DFT\u8ba1\u7b97\u8868\u660e\uff0c\u5728\u76f8\u53d8\u521d\u671f\uff0c\u78b3\u63ba\u6742\u7269\u4ee5\u95f4\u9699\u539f\u5b50\u7684\u5f62\u5f0f\u4f4d\u4e8e\u7684\u6676\u683c\u7a7a\u95f4\u4e2d\u3002XAFS\u548cAC-STEM\u5206\u6790\u8868\u5f81\u4e86\u591a\u76f8\u7ed3\u6784\u548c\u591a\u539f\u5b50\u754c\u9762\u7684\u51fa\u73b0\uff0c\u5236\u5907\u7684C+MoS2<\/sub> \u5728\u78b1\u6027\u548c\u9178\u6027\u4ecb\u8d28\u4e2d\u5747\u5bf9HER\u5177\u6709\u51fa\u8272\u7684\u6d3b\u6027\u3002\u6b64\u5916\uff0c\u901a\u8fc7DFT\u7814\u7a76\u8fdb\u4e00\u6b65\u786e\u5b9a\u4e86\u5177\u6709\u591a\u79cd\u8fde\u63a5\u6a21\u5f0f\u7684\u4e0d\u540c\u754c\u9762\u7684\u6700\u4f73\u6c22\u5438\u9644\u4f4d\u70b9\u3002\u957f\u8fdc\u6765\u770b\uff0c\u8fd9\u9879\u5de5\u4f5c\u6709\u671b\u7528\u4e8e\u5927\u89c4\u6a21\u5de5\u4e1a\u4e2d\u5e94\u7528\u7684\u9ad8\u6027\u80fd\u91d1\u5c5eTMD\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u548c\u5236\u9020\u3002<\/p>\n<\/p>\n
<\/p>\n
\u56fe2<\/strong> C+MoS2<\/sub>\u8584\u819c\u7684\u5408\u6210\u4e0e\u8868\u5f81\u00a0\u00a9 2023 Elsevier Inc.<\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n