{"id":248075,"date":"2023-03-21T06:20:24","date_gmt":"2023-03-20T22:20:24","guid":{"rendered":"\/\/m.iemloyee.com\/?p=248075"},"modified":"2023-03-20T11:25:35","modified_gmt":"2023-03-20T03:25:35","slug":"applied-catalysis-b%ef%bc%9a%e7%8e%b0%e5%ae%9e%e7%8e%af%e5%a2%83%e4%b8%8e%e5%ae%9e%e9%aa%8c%e5%ae%a4cu-ssz-13-scr%e5%82%ac%e5%8c%96%e5%89%82%e5%8a%a0%e9%80%9f%e8%80%81%e5%8c%96%e7%9a%84%e5%af%b9","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=248075","title":{"rendered":"Applied Catalysis B\uff1a\u73b0\u5b9e\u73af\u5883\u4e0e\u5b9e\u9a8c\u5ba4Cu\/SSZ-13 SCR\u50ac\u5316\u5242\u52a0\u901f\u8001\u5316\u7684\u5bf9\u6bd4\u7814\u7a76"},"content":{"rendered":"<p>\u5f20\u7199\u7199<\/p>\n<p><strong>\u4e00\u3001 \u3010\u5bfc\u8bfb\u3011\u00a0 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Gao\u901a\u8fc7\u5e7f\u6cdb\u7684\u50ac\u5316\u5242\u8868\u5f81\u65b9\u6cd5\uff0c\u63ed\u793a\u4e86\u5b9e\u9a8c\u5ba4\u52a0\u901f\u8001\u5316\u548c\u73b0\u5b9e\u73af\u5883\u8001\u5316\u4e4b\u95f4\u7684\u5dee\u8ddd\u3002\u5bf96\u79cd\u4ee3\u8868\u6027\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u6df1\u5165\u6bd4\u8f83\u7814\u7a76\uff0c\u4ece\u800c\u83b7\u5f97\u4e0d\u540c\u8001\u5316\u673a\u5236\u4e0b\u539f\u5b50\u6c34\u5e73\u7684Cu\u8f6c\u5316\u76f8\u5173\u7ed3\u8bba\u3002<\/p>\n<p><strong>\u76f8\u5173\u7814\u7a76\u5de5\u4f5c\u4ee5\u201cA comparative study between real-world and laboratory accelerated aging of Cu\/SSZ-13 SCR catalysts\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520aApplied Catalysis B\u4e0a\u3002<\/strong><\/p>\n<p><strong>\u00a0<img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248076\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1.png\" alt=\"\" width=\"1330\" height=\"643\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1.png 1330w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-300x145.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-768x371.png 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/1-1024x495.png 1024w\" sizes=\"(max-width: 1330px) 100vw, 1330px\" \/><\/strong><strong>\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n<p>1.\u4f5c\u8005\u901a\u8fc7\u5e94\u7528\u5e7f\u6cdb\u7684\u50ac\u5316\u5242\u8868\u5f81\u65b9\u6cd5\uff0c\u5bf96\u79cd\u4ee3\u8868\u6027\u50ac\u5316\u5242\u8fdb\u884c\u4e86\u6df1\u5165\u6bd4\u8f83\u7814\u7a76\uff0c\u4ece\u800c\u83b7\u5f97\u4e0d\u540c\u8001\u5316\u673a\u5236\u4e0b\u539f\u5b50\u6c34\u5e73\u7684Cu\u8f6c\u5316\u7ed3\u8bba\uff0c\u63ed\u793a\u4e86\u5b9e\u9a8c\u5ba4\u52a0\u901f\u8001\u5316\u548c\u73b0\u5b9e\u73af\u5883\u8001\u5316\u4e4b\u95f4\u7684\u5dee\u8ddd\u3002<\/p>\n<p>2.\u7814\u7a76\u53d1\u73b0\u786b\u8001\u5316\u5728\u50ac\u5316\u5242\u5728\u5b9e\u9645\u964d\u89e3\u5e94\u7528\u4e2d\u8d77\u7740\u6700\u91cd\u8981\u7684\u4f5c\u7528\uff0c\u5305\u62ec\u5b64\u7acb\u7684Cu<sup>II<\/sup> SCR\u6d3b\u6027\u7269\u79cd\u5bf9CuSO<sub>4<\/sub>\u7c7b\u7269\u79cd\u7684\u76f4\u63a5\u786b\u4e2d\u6bd2\uff0c\u8fd9\u4e9b\u7269\u79cd\u805a\u96c6\u6210\u591a\u6838CuSO<sub>4<\/sub>\u7c07\uff0c\u5e76\u6700\u7ec8\u5728\u8131\u786b\u5904\u7406\u4e2d\u5f62\u6210CuO\u3002\u8fd9\u79cd\u5316\u5b66\u53cd\u5e94\u5c06SCR\u6d3b\u6027\u94dc\u8f6c\u5316\u4e3aSCR\u60f0\u6027\u94dc\uff0c\u540c\u65f6\u4e0d\u4f1a\u4e25\u91cd\u5f71\u54cd\u50ac\u5316\u5242\u8f7d\u4f53\u7684\u5b8c\u6574\u6027\u3002\u8fd9\u4e9b\u7279\u5f81\u5728SOx\u5b58\u5728\u7684\u6c34\u70ed\u8001\u5316\u4e2d\u5f97\u5230\u90e8\u5206\u590d\u5236\uff0c\u4f46\u5355\u72ec\u6c34\u70ed\u8001\u5316\u65f6\u6548\u5f88\u96be\u6a21\u4eff\u3002<\/p>\n<p><strong>\u00a0<\/strong><\/p>\n<p><strong>\u00a0<\/strong><strong>\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011 <\/strong><\/p>\n<p><strong>\u00a0<img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248077\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2.png\" alt=\"\" width=\"646\" height=\"597\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2.png 646w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/2-300x277.png 300w\" sizes=\"(max-width: 646px) 100vw, 646px\" \/><\/strong><\/p>\n<p><strong>\u56fe1 <\/strong><strong>\u5b9e\u9a8c\u5ba4\u52a0\u901f\u8001\u5316\u4e0e\u73b0\u5b9e\u73af\u5883\u8001\u5316Cu\/SSZ-13\u50ac\u5316\u5242<\/strong><strong>\u3002<\/strong><strong>\u00a9<\/strong><strong> 2022 Elsevier B.V.<\/strong><\/p>\n<p><strong><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248078\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3.png\" alt=\"\" width=\"888\" height=\"740\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3.png 888w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-300x250.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/3-768x640.png 768w\" sizes=\"(max-width: 888px) 100vw, 888px\" \/>\u56fe2 (A)\u6807\u51c6SCR\u4e2dCu\/SSZ-13\u50ac\u5316\u5242\u4e0a\u7684NO<sub>x<\/sub>\u8f6c\u5316\u7387\uff0c(B) NH<sub>3<\/sub>\u8f6c\u5316\u7387\uff0c(C) NO<sub>2<\/sub>\u51fa\u53e3\u6d53\u5ea6\u548c(D) N<sub>2<\/sub>O\u51fa\u53e3\u6d53\u5ea6\u968f\u6e29\u5ea6\u7684\u53d8\u5316\u3002\u00a9 2022 Elsevier B.V.<\/strong><\/p>\n<p><strong><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248079\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4.png\" alt=\"\" width=\"894\" height=\"379\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4.png 894w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-300x127.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/4-768x326.png 768w\" sizes=\"(max-width: 894px) 100vw, 894px\" \/>\u56fe3 (A) Cu\/SSZ-13\u50ac\u5316\u5242\u4e0aNH<sub>3<\/sub>\u6c27\u5316\u8fc7\u7a0b\u4e2dNH<sub>3<\/sub>\u8f6c\u5316\u7387\u968f\u6e29\u5ea6\u7684\u53d8\u5316\u3002(B)\u5e72NO\u6c27\u5316\u8fc7\u7a0b\u4e2dCu\/SSZ-13\u50ac\u5316\u5242\u4e0aNO\u8f6c\u5316\u7387\u968f\u6e29\u5ea6\u7684\u53d8\u5316\u3002\u00a9 2022 Elsevier B.V.<\/strong><\/p>\n<p><strong><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248080\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5.png\" alt=\"\" width=\"916\" height=\"720\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5.png 916w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-300x236.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/5-768x604.png 768w\" sizes=\"(max-width: 916px) 100vw, 916px\" \/>\u56fe4 (A)\u4f4e\u6e29NO<sub>x<\/sub>\u8f6c\u6362\u6570\u636e\u5bfc\u51fa\u7684Arrhenius\u56fe\uff0c\u4f7f\u7528\u4e00\u9636\u901f\u7387\u8868\u8fbe\u5f0f\u8fdb\u884c\u6821\u6b63\u3002(B)\u7531Arrhenius\u5206\u6790\u5f97\u51fa\u7684\u76f8\u5e94\u6307\u6570\u524d\u56e0\u5b50\u3002(C)\u7531Arrhenius\u5206\u6790\u5f97\u5230\u7684\u76f8\u5e94\u8868\u89c2\u6d3b\u5316\u80fd\u3002(D)\u53cd\u5e94\u6e29\u5ea6\u4e3a160<\/strong><strong><sup>0<\/sup><\/strong><strong>C<\/strong><strong>\u65f6\u7684SCR\u5468\u8f6c\u7387\uff0c\u4f7f\u7528\u57fa\u4e8e\u4e00\u9636\u901f\u7387\u8868\u8fbe\u5f0f\u7684\u5f52\u4e00\u5316\u901f\u7387\u8ba1\u7b97\uff0c\u4ee5\u53ca\u4eceNO+NH<sub>3<\/sub>\u6ef4\u5b9a\u4e2d\u53ef\u8fd8\u539f\u7684Cu\u542b\u91cf\u3002\u00a9 2022 Elsevier B.V.<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-248081\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6.png\" alt=\"\" width=\"533\" height=\"451\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6.png 533w, \/\/m.iemloyee.com\/wp-content\/uploads\/2023\/03\/6-300x254.png 300w\" sizes=\"(max-width: 533px) 100vw, 533px\" \/><\/p>\n<p><strong>\u56fe5 \u5728operando SCR\u6761\u4ef6\u4e0b\uff0cCu\/SSZ13\u50ac\u5316\u5242EPR\u53ef\u89c1Cu\/\u603bCu\u968f\u6e29\u5ea6\u7684\u53d8\u5316.\u00a9 2022 Elsevier B.V.<\/strong><\/p>\n<p><strong>\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n<p>\u7814\u7a76\u901a\u8fc7\u8be6\u7ec6\u6bd4\u8f83\u4e86\u5546\u4e1aCu\/SSZ-13\u50ac\u5316\u5242\u5728\u52a0\u901f\u5b9e\u9a8c\u5ba4\u8001\u5316\u548c\u73b0\u5b9e\u73af\u5883\u8001\u5316\u7684\u5404\u9879\u6570\u636e\uff0c\u9610\u660e\u4e86\u8fd9\u4e24\u79cd\u65b9\u6cd5\u4e4b\u95f4\u7684\u5dee\u8ddd\u3002\u91c7\u7528\u591a\u79cd\u50ac\u5316\u5242\u8868\u5f81\u65b9\u6cd5\uff0c\u5305\u62ec\u6bd4\u8868\u9762\u79ef\/\u5b54\u9699\u7387\u5206\u6790\uff0cX\u5c04\u7ebf\u884d\u5c04(XRD)\uff0cH<sub>2<\/sub>-\u6e29\u5ea6\u7a0b\u5e8f\u8fd8\u539f\uff0cNH<sub>3<\/sub>-\u6e29\u5ea6\u7a0b\u5e8f\u89e3\u5438\uff0c\u56fa\u4f53\u6838\u78c1(NMR)\uff0c\u539f\u4f4dX\u5c04\u7ebf\u5149\u7535\u5b50(XPS)\u548c\u7535\u5b50\u987a\u78c1\u5171\u632f(EPR)\u8c31\uff0c\u5c06\u7531\u6b64\u83b7\u5f97\u7684Cu\u8f6c\u5316\u7684\u539f\u5b50\u6c34\u5e73\u76f8\u5173\u7ed3\u8bba\u4e0e\u50ac\u5316\u5242\u7684SCR\u3001NH<sub>3<\/sub>\/NO\u6c27\u5316\u52a8\u529b\u5b66\u884c\u4e3a\u8054\u7cfb\u8d77\u6765\u3002\u8bc1\u660e\u4e86\u5728650<sup>0<\/sup>C\uff0c\u65e0SOx\u7684\u60c5\u51b5\u4e0b\uff0c\u6c34\u70ed\u8001\u5316\u4f1a\u5bfc\u81f4ZCuOH\u8f6c\u53d8\u4e3aZ<sub>2<\/sub>Cu 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