{"id":245410,"date":"2023-01-06T06:04:13","date_gmt":"2023-01-05T22:04:13","guid":{"rendered":"\/\/m.iemloyee.com\/?p=245410"},"modified":"2023-01-04T10:04:38","modified_gmt":"2023-01-04T02:04:38","slug":"%e5%b1%b1%e5%a4%a7%e9%ab%98%e7%8f%82%e6%95%99%e6%8e%88%e5%9b%a2%e9%98%9fjoule%ef%bc%9a%e5%88%9b%e9%80%a0%e5%85%a8%e5%b0%8f%e5%88%86%e5%ad%90%e6%9c%89%e6%9c%ba%e5%a4%aa%e9%98%b3%e8%83%bd%e7%94%b5","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=245410","title":{"rendered":"\u5c71\u5927\u9ad8\u73c2\u6559\u6388\u56e2\u961fJoule\uff1a\u521b\u9020\u5168\u5c0f\u5206\u5b50\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60\u6548\u7387\u65b0\u7eaa\u5f55"},"content":{"rendered":"

\u5c71\u5927\u9ad8\u73c2\u6559\u6388\u56e2\u961f<\/strong>Joule<\/em><\/strong>\uff1a\u521b\u9020\u5168\u5c0f\u5206\u5b50\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60\u6548\u7387\u65b0\u7eaa\u5f55<\/strong><\/p>\n

LWB<\/strong><\/p>\n

01<\/strong>\u3001\u5bfc\u8bfb<\/strong><\/p>\n

\u8fd1\u4e9b\u5e74\uff0c\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60\uff08OSC\uff09\u5728\u5149\u4f0f\u6280\u672f\u4e2d\u7684\u8bf1\u4eba\u5e94\u7528\u5f15\u8d77\u4e86\u5e7f\u6cdb\u5173\u6ce8\u3002\u4e0e\u805a\u5408\u7269\u57faOSC\u76f8\u6bd4\uff0c\u5168\u5c0f\u5206\u5b50OSC\uff08ASM OSC\uff09\u6709\u7740\u66f4\u660e\u786e\u7684\u5316\u5b66\u7ed3\u6784\u5e76\u4e14\u6613\u4e8e\u7eaf\u5316\u3001\u91cd\u590d\u6027\u9ad8\uff0c\u6709\u7740\u66f4\u5927\u7684\u5546\u4e1a\u5316\u6f5c\u529b\u3002\u968f\u7740\u975e\u5bcc\u52d2\u70ef\u53d7\u4f53(NFAs)\uff0c\u7279\u522b\u662fY6\u53ca\u5176\u884d\u751f\u7269\u7684\u51fa\u73b0\uff0cASM OSCs\u5f97\u5230\u4e86\u7a81\u98de\u731b\u8fdb\u7684\u53d1\u5c55\u3002\u7136\u800c\uff0c\u7531\u4e8e\u4f9b\u4f53(D)\u548c\u53d7\u4f53(A)\u7684\u5206\u5b50\u7ed3\u6784\u76f8\u4f3c\uff0cASM OSCs\u7684\u6027\u80fd\u4ecd\u7136\u843d\u540e\u4e8e\u5176\u5bf9\u5e94\u7684\u805a\u5408\u7269\uff0c\u8fd9\u5bfc\u81f4\u4e86ASM\u5171\u6df7\u7269\u5f62\u6001\u8c03\u63a7\u6bd4\u8f83\u590d\u6742\u3002\u56e0\u6b64\uff0c\u5408\u7406\u63a7\u5236\u5f62\u8c8c\u6f14\u53d8\uff0c\u8fdb\u4e00\u6b65\u63d0\u9ad8\u5668\u4ef6\u6027\u80fd\u4ecd\u7136\u662fASM OSCs\u9762\u4e34\u7684\u6311\u6218\u3002<\/p>\n

\u5f62\u6001\u5b66\u4e0e\u5668\u4ef6\u7684\u7535\u8377\u4f20\u8f93\u548c\u590d\u5408\u8fc7\u7a0b\u5bc6\u5207\u76f8\u5173\uff0c\u662f\u51b3\u5b9a\u5149\u4f0f\u6027\u80fd\u7684\u5173\u952e\u56e0\u7d20\u3002\u8fd1\u5e74\u6765\uff0c\u4f53\u5f02\u8d28\u7ed3\uff08BHJ\uff09\u6784\u578b\u5728ASM OSC\u7684\u6d3b\u6027\u5c42\u5f62\u6210\u4e2d\u5360\u636e\u4e3b\u5bfc\u5730\u4f4d\uff0c\u6b64\u5916\uff0c\u7814\u7a76\u4eba\u5458\u76ee\u524d\u5df2\u7ecf\u5f00\u53d1\u4e86\u5404\u79cd\u5316\u5b66\u6216\u52a0\u5de5\u7b56\u7565\u6765\u64cd\u7eb5BHJ\u5171\u6df7\u7269\u819c\u5f62\u6001\u3002\u7136\u800c\uff0c\u5b83\u4eec\u7684\u5f62\u8c8c\u63a7\u5236\u76f8\u5f53\u590d\u6742\uff0c\u5c24\u5176\u662f\u5bf9\u4e8e\u4e00\u6b65\u6c89\u79ef\u7684BHJ\u5171\u6df7\u819c\uff0c\u901a\u5e38\u8fd8\u4f1a\u5bfc\u81f4\u663e\u8457\u7684\u91cd\u7ec4\u635f\u5931\u3002\u56e0\u6b64\uff0c\u5bf9\u4e8eASM OSCs\u6765\u8bf4\uff0c\u64cd\u7eb5\u5f62\u6001\u4ee5\u6ee1\u8db3\u5b9e\u73b0\u6700\u5927\u5149\u5b50\u7535\u6d41\u548c\u586b\u5145\u56e0\u5b50\uff08FF\uff09\u8fd9\u4e00\u57fa\u672c\u6311\u6218\u8fdc\u672a\u5b9e\u73b0\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8fde\u7eed\u6c89\u79ef\u7ed9\u4f53\u548c\u53d7\u4f53\u5c42\u4ee5\u6784\u5efa\u9010\u5c42\uff08LbL\uff09\u5668\u4ef6\u5df2\u88ab\u8ba4\u4e3a\u662f\u63a7\u5236\u805a\u5408\u7269OSCs\u5f62\u6001\u7684\u6709\u6548\u65b9\u6cd5\u3002\u4f46\u662f\uff0c\u76ee\u524d\u6587\u732e\u4e2d\u5c1a\u672a\u6709\u5173\u4e8e\u9ad8\u6027\u80fdLbL ASM OSCs\u7684\u62a5\u9053\uff0c\u56e0\u6b64\u76f8\u5173\u7814\u7a76\u975e\u5e38\u6709\u9650\u3002\u5e78\u8fd0\u7684\u662f\uff0c\u7814\u7a76\u5df2\u7ecf\u6210\u529f\u8bc1\u660e\u4e86\u5177\u6709\u03c0\u5171\u8f6d\u5e73\u9762\u7ed3\u6784\u7684\u77f3\u58a8\u7094\u884d\u751f\u7269\u4f5c\u4e3a\u591a\u529f\u80fd\u56fa\u4f53\u6dfb\u52a0\u5242\u53ef\u4ee5\u5fae\u8c03\u5206\u5b50\u5806\u79ef\uff0c\u5e76\u5728\u805a\u5408\u7269OSCs\u4e2d\u5b9e\u73b0\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\uff0c\u8fd9\u4e3a\u540e\u7eed\u76f8\u5173\u7814\u7a76\u63d0\u4f9b\u4e86\u8fdb\u4e00\u6b65\u7684\u5e2e\u52a9\u3002<\/p>\n

02<\/strong>\u3001\u6210\u679c\u63a0\u5f71<\/strong><\/p>\n

\u9274\u4e8e\u6b64\uff0c\u5c71\u4e1c\u5927\u5b66\u7269\u8d28\u521b\u5236\u4e0e\u80fd\u91cf\u8f6c\u6362\u79d1\u5b66\u7814\u7a76\u4e2d\u5fc3\u9ad8\u73c2\u6559\u6388\u3001\u674e\u7389\u826f\u9662\u58eb\u3001\u534e\u5357\u5e08\u8303\u5927\u5b66\u5148\u8fdb\u5149\u7535\u5b50\u7814\u7a76\u9662\u8f87\u7406\u6559\u6388\u7b49\u4eba\u8054\u5408\u62a5\u9053\u4e86\u4e00\u79cd\u9ad8\u6548\u7684ASM OSC\u3002\u7814\u7a76\u4eba\u5458\u901a\u8fc7\u7ed3\u5408LbL\u6c89\u79ef\u548c\u56fa\u4f53\u6dfb\u52a0\u5242\u7532\u6c27\u57fa\u53d6\u4ee3\u77f3\u58a8\u7094\uff08GOMe\uff09\u5904\u7406\u6765\u5408\u7406\u63a7\u5236\u987a\u5e8f\u5f62\u6001\u6f14\u53d8\u548c\u5782\u76f4\u6210\u5206\u5206\u5e03\uff0c\u6700\u7ec8\u83b7\u5f97\u4e86\u4e00\u79cd\u9ad8\u6548\u7684ASM OSCs\u3002\u4e0eBHJ\u5171\u6df7\u7269\u76f8\u6bd4\uff0cLbL\u5904\u7406\u7684\u5171\u6df7\u7269\u5177\u6709\u5e95\u90e8\u7ed9\u4f53\u5bcc\u96c6\u3001\u9876\u90e8\u53d7\u4f53\u5bcc\u96c6\u7684\u6700\u4f73\u5782\u76f4\u5206\u5c42\u3002\u6b64\u5916\uff0c\u7ed3\u679c\u8868\u660e\uff0c\u5c06\u56fa\u4f53\u6dfb\u52a0\u5242GOMe\u6dfb\u52a0\u5230\u7ed9\u4f53\u5c42\u7565\u5fae\u589e\u5f3a\u4e86\u5206\u5b50\u5806\u79ef\u5e76\u589e\u52a0\u4e86\u8868\u9762\u7c97\u7cd9\u5ea6\uff0c\u4ece\u800c\u4e3a\u968f\u540e\u7684\u53d7\u4f53\u6c89\u79ef\u63d0\u4f9b\u4e86\u5408\u9002\u7684\u57fa\u8d28\uff0c\u8fd9\u663e\u8457\u4fc3\u8fdb\u4e86\u53d7\u4f53\u6269\u6563\u4ece\u800c\u5f62\u6210\u4f18\u9009\u7684\u5782\u76f4\u5206\u5e03\u3002\u53e6\u4e00\u4e2a\u65b9\u9762\uff0cGOMe\u5904\u7406\u7684\u53d7\u4f53\u5c42\u663e\u793a\u51fa\u66f4\u7d27\u5bc6\u7684\u5206\u5b50\u5806\u79ef\u3002\u901a\u8fc7\u8fd9\u79cd\u65b9\u6cd5\uff0c\u5408\u7406\u63a7\u5236\u7684\u5171\u6df7\u7269\u5f62\u6001\u540c\u65f6\u5177\u6709\u7d27\u51d1\u7684\u5206\u5b50\u5806\u79ef\u3001\u8db3\u591f\u7684D\/A\u754c\u9762\u548c\u5782\u76f4\u4f20\u8f93\u901a\u9053\uff0c\u4ece\u800c\u5b9e\u73b0\u4e86\u589e\u5f3a\u7684\u6fc0\u5b50\u89e3\u79bb\u548c\u7535\u8377\u4f20\u8f93\u3002\u6700\u7ec8\uff0c\u57fa\u4e8eZnP-TSEH:4TIC:6TIC\u7684\u5668\u4ef6\u83b7\u5f97\u4e8677.31%\u7684FF\uff0c\u4ee5\u53ca17.18%\u7684\u7a81\u7834\u6548\u7387\uff08\u9a8c\u8bc1\u6548\u7387\uff1a17.08%\uff09\uff0c\u663e\u8457\u9ad8\u4e8e\u5bf9\u7167\u5668\u4ef6\u3002<\/p>\n

\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cRational control of sequential morphology evolution and vertical distribution toward 17.18% efficiency all-small-molecule organic solar cells<\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520aJoule<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

03<\/strong>\u3001\u6838\u5fc3\u521b\u65b0\u70b9<\/strong><\/p>\n

1\u3001\u901a\u8fc7\u7ed3\u5408\u5206\u5c42(LbL)\u6c89\u79ef\u548c\u56fa\u4f53\u6dfb\u52a0\u5242\u7532\u6c27\u57fa\u53d6\u4ee3\u77f3\u58a8\u7094(GOMe)\u5904\u7406\u6765\u63a7\u5236\u6d3b\u6027\u5c42\u5f62\u6001\uff0c\u8bc1\u660e\u4e86\u5168\u5c0f\u5206\u5b50\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60(ASM OSC)\u7684\u6548\u7387\u9ad8\u8fbe17.18%\u3002<\/p>\n

2\u3001\u5408\u7406\u63a7\u5236\u3001\u5206\u5b50\u5806\u53e0\u6709\u5e8f\u3001\u5782\u76f4\u5206\u5e03\u7684\u5f62\u6001\u5177\u6709\u53cc\u91cd\u4f18\u52bf\u3002\u57fa\u4e8eZnP-TSEH:4TIC:6TIC\u7684\u5668\u4ef6\u83b7\u5f97\u4e8677.31%\u7684FF\uff0c\u4ee5\u53ca17.18%\u7684\u7a81\u7834\u6548\u7387\uff0c\u8fd9\u662f\u8fc4\u4eca\u4e3a\u6b62\u62a5\u9053\u7684ASM OSCs\u7684\u6700\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387\u3002<\/p>\n

04<\/strong>\u3001\u6570\u636e\u6982\u89c8<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>1 <\/strong>\u5316\u5b66\u7ed3\u6784\uff0c\u539f\u7406\u56fe\uff0c\u5149\u5b66\u6027\u8d28<\/strong> \u00a9 2022 Elsevier Inc.<\/strong><\/p>\n

\uff08A\uff09\u4f9b\u4f53(D, ZnP-TSEH)\uff0c\u53d7\u4f53(A, 4TIC\u548c6TIC)\u548c\u56fa\u4f53\u6dfb\u52a0\u5242(GOMe)\u7684\u5316\u5b66\u7ed3\u6784\uff1b<\/p>\n

\uff08B\uff09BHJ\u548cLbL\u5668\u4ef6\u52a0\u5de5\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08C\uff09D\u548cD+GOMe\uff080.5 wt %\uff09\u8584\u819c\u7684\u5149\u5b66\u6027\u8d28\uff1b<\/p>\n

\uff08D\uff09A\u548cA+GOMe\uff080.5 wt %\uff09\u8584\u819c\u7684\u5149\u5b66\u6027\u8d28\uff1b<\/p>\n

\uff08E\uff09BHJ:D+A\u3001BHJ:D+A+GOMe (1 wt %)\u3001LbL:D\/A\u3001LbL:D+GOMe (0.5 wt %)\/A\u3001GOMe (0.5 wt %)\u8584\u819c\u7684\u5149\u5b66\u6027\u8d28\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>2 <\/strong>\u5f62\u6001\u5b66\u8c03\u67e5<\/strong> \u00a9 2022 Elsevier Inc.<\/strong><\/p>\n

\uff08A-D\uff09BHJ:D+A (A)\u3001BHJ:D+A+GOMe (1 wt %) (B)\u3001LbL:D\/A (C)\u3001LbL:D+GOMe (0.5 wt %)\/A+GOMe (0.5 wt %) (D)\u6d3b\u6027\u5c42\u7684AFM\u9ad8\u5ea6\u56fe\u50cf\uff1b<\/p>\n

\uff08E-H\uff09\u8584\u819c\u7684AFM\u76f8\u4f4d\u56fe\u50cf\uff1b<\/p>\n

\uff08I-L\uff09\u6d3b\u6027\u819c\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>3 <\/strong>\u5f62\u6001\u5b66\u7279\u5f81\u548c\u53ef\u80fd\u7684\u7269\u7406\u52a8\u529b\u5b66<\/strong> \u00a9 2022 Elsevier Inc.<\/strong><\/p>\n

\uff08A-D\uff09\u5bf9\u7167\u548cGOMe\u5904\u7406\u7684BHJ\u548cLbL\u819c\u7684GIXD\u884d\u5c04\u56fe\uff0cBHJ:D+A (A)\u3001BHJ:D+A+GOMe (1 wt %) (B)\u3001LbL:D\/A (C)\u3001LbL:D+GOMe (0.5 wt %)\/A+GOMe (0.5 wt %) (D)\uff1b<\/p>\n

\uff08E\uff09\u6d3b\u6027\u5c42\u7684\u9762\u5916(OOP)\u548c\u9762\u5185(IP)\u66f2\u7ebf\uff1b<\/p>\n

\uff08F\uff09\u5bf9\u4e8eGOMe\u5904\u7406\u7684BHJ\u548cLbL\u819c\uff0cZn2+<\/sup>\u7684ToF-SIMS\u79bb\u5b50\u4ea7\u7387\u4e0e\u6e85\u5c04\u65f6\u95f4\u7684\u5173\u7cfb\uff1b<\/p>\n

\uff08G-J\uff09\u5bf9\u7167\u548cGOMe\u5904\u7406\u7684BHJ\u548cLbL\u819c\u4e2d\u5206\u5b50\u6392\u5217\u548c\u53ef\u80fd\u7684\u7269\u7406\u52a8\u529b\u5b66\u7684\u89c6\u89c9\u8349\u56fe\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4 <\/strong>\u5149\u4f0f\u6027\u80fd\u548c\u7269\u7406\u52a8\u529b\u5b66<\/strong> \u00a9 2022 Elsevier Inc.<\/strong><\/p>\n

\uff08A\uff09\u5bf9\u7167\u548cGOMe\u5904\u7406\u7684BHJ\u548cLbL\u88c5\u7f6e\u7684J-V\u66f2\u7ebf\uff1b<\/p>\n

\uff08B\uff09\u62a5\u544a\u8fc7\u7684ASM OSC\u7684PCE\u603b\u7ed3\uff1b<\/p>\n

\uff08C\uff09\u56db\u4e2aASM OSC\u7684EQE\u66f2\u7ebf\uff1b<\/p>\n

\uff08D\uff09\u5149\u7535\u6d41\u5bc6\u5ea6\u4e0e\u6709\u6548\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08E\uff09Jsc<\/sub>\u7684\u5149\u5f3a\u4f9d\u8d56\u6027\uff1b<\/p>\n

\uff08F\uff09TRPL\u5149\u8c31\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>5 <\/strong>\u98de\u79d2\u77ac\u6001\u5438\u6536\uff08<\/strong>fs-TA<\/strong>\uff09\u5149\u8c31<\/strong> \u00a9 2022 Elsevier Inc.<\/strong><\/p>\n

\uff08A-D\uff09BHJ:D+A (A)\u3001BHJ:D+A+GOMe (1 wt %) (B)\u3001 LbL:D\/A (C)\u3001and LbL:D+GOMe (0.5 wt %)\/A+GOMe (0.5 wt %) (D)\u8584\u819c\u7684fs-TA\u5149\u8c31\u76842D\u5f69\u8272\u56fe\uff1b<\/p>\n

\uff08E-H\uff09BHJ:D+A (E)\u3001BHJ:D+A+GOMe (1 wt %) (F)\u3001LbL:D\/A (G)\u3001LbL:D+GOMe (0.5 wt %)\/A+GOMe (0.5 wt %) (H)\u5728\u7279\u5b9a\u5ef6\u8fdf\u65f6\u95f4\u4e0b\u7684\u4ee3\u8868\u6027TA\u5149\u8c31\uff1b<\/p>\n

05<\/strong>\u3001\u6210\u679c\u542f\u793a<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u5de5\u4f5c\u901a\u8fc7\u56fa\u4f53\u6dfb\u52a0\u5242GOMe\u5904\u7406\u548cLbL\u5904\u7406\u76f8\u7ed3\u5408\uff0c\u6765\u5408\u7406\u63a7\u5236\u987a\u5e8f\u5f62\u6001\u6f14\u53d8\u548c\u5782\u76f4\u5206\u5e03\uff0c\u5f97\u5230\u4e86PCE\u8fbe\u523017.18%\u7684ASM OSCs\u300217.18%\u7684PCE\u662f\u8fc4\u4eca\u4e3a\u6b62\u62a5\u9053\u7684ASM OSC\u7684\u6700\u9ad8\u6548\u7387\u3002\u5c06GOMe\u5904\u7406\u4e0eLbL\u5904\u7406\u76f8\u7ed3\u5408\uff0c\u7cbe\u7ec6\u8c03\u63a7\u8fde\u7eed\u5f62\u6001\u6f14\u53d8\u548c\u5782\u76f4\u5206\u91cf\u5206\u5e03\uff0c\u662f\u8fdb\u4e00\u6b65\u63d0\u9ad8ASM OSCs\u6027\u80fd\u7684\u6709\u6548\u9014\u5f84\u3002\u8fd9\u9879\u5de5\u4f5c\u6709\u671b\u6fc0\u53d1\u76f8\u5173\u9886\u57df\u7684\u7814\u7a76\u70ed\u60c5\uff0c\u63a8\u52a8\u76f8\u5173\u9886\u57df\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002\u968f\u7740\u4e0d\u540c\u5149\u6d3b\u6027\u6750\u6599\u7684\u5f00\u53d1\u548c\u5bf9\u5f62\u6001\u673a\u5236\u7684\u6df1\u5165\u7406\u89e3\uff0c\u76f8\u4fe1\u672a\u6765ASM OSCs\u5c06\u53d6\u5f97\u4e00\u7cfb\u5217\u7a81\u7834\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Rational control of sequential morphology evolution and vertical distribution toward 17.18% efficiency all-small-molecule organic solar cells<\/strong>\uff0c<\/strong>2022<\/strong>\uff0c<\/strong>https:\/\/doi.org\/10.1016\/j.joule.2022.10.005<\/strong>\uff09<\/strong><\/p>\n

 <\/p>\n

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