{"id":245258,"date":"2023-01-12T06:00:48","date_gmt":"2023-01-11T22:00:48","guid":{"rendered":"\/\/m.iemloyee.com\/?p=245258"},"modified":"2023-01-09T12:48:13","modified_gmt":"2023-01-09T04:48:13","slug":"%e4%be%af%e5%89%91%e8%be%89%e9%83%91%e4%bc%97adv-mater-%ef%bc%9azno%e5%b1%82%e7%9a%84%e6%96%b0%e5%88%b6%e5%a4%87%e6%96%b9%e6%b3%95%e5%8a%a9%e5%8a%9b%e9%ab%98%e6%95%88%e7%a8%b3%e5%ae%9a%e6%9c%89","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=245258","title":{"rendered":"\u4faf\u5251\u8f89&\u90d1\u4f17Adv. Mater.\uff1aZnO\u5c42\u7684\u65b0\u5236\u5907\u65b9\u6cd5\u52a9\u529b\u9ad8\u6548\u7a33\u5b9a\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

01<\/strong>\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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02<\/strong>\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u79d1\u9662\u5316\u5b66\u6240\u4faf\u5251\u8f89\u7814\u7a76\u5458<\/strong>\u548c\u5317\u4eac\u79d1\u6280\u5927\u5b66\u90d1\u4f17\u6559\u6388\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u7b80\u5355\u3001\u6709\u6548\u3001\u7ecf\u6d4e\u7684\u65b9\u6cd5\uff0c\u7528\u787c\u9178(BA)\u53bb\u9664\u6eb6\u80f6-\u51dd\u80f6ZnO CIL\u4e2d\u6b8b\u7559\u7684\u80fa\u800c\u4e0d\u635f\u4f24ZnO\u3002BA\u88ab\u7528\u4f5c\u80fa\u6e05\u6d17\u5242\uff0c\u56e0\u4e3a\u5176\u5177\u6709\u5408\u9002\u7684\u9178\u79bb\u89e3\u5e38\u6570(pKa<\/sub>)\u4ee5\u907f\u514dZnO\u5206\u89e3\u3002X\u5c04\u7ebf\u5149\u7535\u5b50\u80fd\u8c31(XPS)\u7ed3\u679c\u8868\u660e\uff0c\u7531\u4e8eBA\u7684\u51b2\u6d17\uff0c\u6b8b\u7559\u7684\u80fa\u53ef\u4ee5\u88ab\u6709\u6548\u5730\u53bb\u9664\u3002ZnO\u7684\u529f\u51fd\u6570(\u03a6)\u53ef\u4ee5\u4ece3.86 eV\u6539\u53d8\u52303.79 eV\uff0c\u5bfc\u81f4\u57fa\u4e8ePBDB-TF:HDO-4Cl:BTP-eC9\u7684OSCs\u7684Voc<\/sub>\u589e\u52a010 meV\u3002\u6b64\u5916\uff0c\u6e05\u6d17\u540e\u7684ZnO CIL\u5728\u7535\u5b50\u63d0\u53d6\u80fd\u529b\u65b9\u9762\u8868\u73b0\u51fa\u660e\u663e\u7684\u6539\u5584\uff0c\u4f8b\u5982BA\u5904\u7406\u7684ZnO\u4e2d\u7684\u7535\u5b50\u63d0\u53d6\u53ef\u4ee5\u572844.29 ns\u5185\u5b8c\u6210(\u6bd4\u539f\u59cbZnO\u5feb33.64%)\u3002\u53e6\u4e00\u65b9\u9762\uff0cZnO CIL\u7684\u7535\u8377\u6536\u96c6\u80fd\u529b\u589e\u5f3a\uff0cZnO CIL\u7684\u529f\u51fd\u6570\u6709\u5229\u4e8e\u5b9e\u73b0\u66f4\u9ad8\u7684Voc<\/sub>\u3002ZnO CIL\u7684\u6539\u8fdb\u6027\u8d28\u5c06PBDB-TF:HDO-4Cl:BTP-eC9 OSC\u7684FF\u4ece75.07%\u63d0\u9ad8\u523078.13%\uff0c\u5e76\u4e14\u5c06PBDB-TF: BTP-eC9 OSC\u7684FF\u4ece73.97%\u63d0\u9ad8\u523077.28%\u3002\u57fa\u4e8e\u4e0a\u8ff0\u7ed3\u679c\uff0c\u4f18\u5316\u7684\u5355\u7ed3OSCs\u7684\u7a33\u5b9a\u6027\u548c\u529f\u7387\u8f6c\u6362\u6548\u7387(PCE)\u540c\u65f6\u63d0\u9ad8\u3002\u6d3b\u6027\u9762\u79ef\u4e3a0.04\u548c1.00 cm2<\/sup>\u7684\u7535\u6c60\u5206\u522b\u8868\u73b0\u51fa18.40%\u548c17.42%\u7684PCEs\u3002\u6b64\u5916\uff0c\u57fa\u4e8eBA\u5904\u7406\u7684ZnO CIL\u7684\u4e32\u8054OSCs\u8868\u73b0\u51fa19.56%\u7684PCE\uff0c\u8bc1\u660e\u4e86\u6240\u63d0\u51fa\u65b9\u6cd5\u7684\u6709\u6548\u6027\u3002<\/p>\n

\u76f8\u5173\u7814\u7a76\u6587\u7ae0\u4ee5\u201cNew Method for Preparing ZnO Layer for Efficient and Stable Organic Solar Cells<\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Adv. Mater.<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

03<\/strong>\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

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04<\/strong>\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\"\"<\/p>\n

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\"\"<\/p>\n

\u56fe\u4e8c\u3001\u5904\u7406\u524dZnO\u548cZnO\/BA\u7684XPS\u5149\u8c31\u3002a) C 1s\uff0cb) N 1s\uff0cc) Zn 2p1\/2<\/sub>\uff0cd) Zn 2p3\/2<\/sub>\uff0ce) O 1s\uff0c\u548cf)B\u4fe1\u53f7\u7684\u5f3a\u5ea6\u3002\u00a9 2022 Wiley<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e09\u3001a)\u7814\u7a76\u7684CILs\u7684UPS\u6570\u636e\u3002b)\u57fa\u4e8e\u6240\u7814\u7a76CILs\u7684\u5668\u4ef6\u7684Mott\u2013Schottky\u56fe\u3002c)\u5728\u6ca1\u6709\u504f\u7f6e\u767d\u5149\u7684\u60c5\u51b5\u4e0b\uff0c\u5728488 nm\u7684\u6fc0\u53d1\u4e0b\uff0c\u5177\u6709\u6240\u7814\u7a76\u7684CILs\u7684\u53cd\u5f0fOSCs\u7684TPC\u3002d)\u5728\u5177\u6709\u4e0d\u540cCILs\u7684OSCs\u4e0a\u6d4b\u91cf\u7684\u963b\u6297\u8c31\u7684\u5948\u594e\u65af\u7279\u56fe\u3002\u6570\u636e\u7531Schottky\u7b49\u6548\u7535\u8def\u6a21\u578b\u62df\u5408\uff0c\u5176\u4e2dRs<\/sub>\u662f\u4e32\u8054\u7535\u963b\uff0cCg<\/sub>\u662f\u51e0\u4f55\u7535\u5bb9\uff0cRt<\/sub>\u662f\u4f20\u8f93\u7535\u963b\uff0cCn<\/sub>\u662f\u5316\u5b66\u7535\u963b\uff0cRrec<\/sub>\u662f\u590d\u5408\u7535\u963b\u3002\u00a9 2022 Wiley<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u56db\u3001a)\u672c\u5de5\u4f5c\u4e2d\u4f7f\u7528\u7684\u7ed9\u4f53\u548c\u53d7\u4f53\u3002b)\u672c\u5de5\u4f5c\u6240\u6d89\u53ca\u6750\u6599\u7684\u80fd\u7ea7\u56fe\u3002c)\u7ecf\u8fc7\u5404\u79cd\u5904\u7406\u7684\u5668\u4ef6\u7684J-V\u66f2\u7ebf\u3002\u6d3b\u6027\u5c42\u4e3aPBDB-TF:HDO-4Cl:BTP-eC9\u3002d)\u57fa\u4e8e\u5177\u6709PBDB-TF:HDO-4Cl:BTP-eC9\u6d3b\u6027\u5c42\u7684CILs\u7684\u6700\u4f73\u5668\u4ef6\u7684EQE\u5149\u8c31\u3002e)\u7ecf\u8fc7\u5404\u79cd\u5904\u7406\u7684\u5668\u4ef6\u7684J-V\u66f2\u7ebf\u3002\u6d3b\u6027\u5c42\u5206\u522b\u662fA: PBDB-TF:BTP-eC9P3HT\uff0cB: PBDB-TF:IT4F\uff0cC: PPDT2FBT:PC71BM\uff0cD: P3HT:PC71BM\u3002f)\u7a7a\u6c14\u7a33\u5b9a\u6027\u3002\u5728AM 1.5G\u4e0b\uff0c\u6807\u51c6\u5316PCE\u4f5c\u4e3aOSCs\u5728\u7a7a\u6c14\u4e2d\u50a8\u5b58\u65f6\u95f4\u7684\u51fd\u6570\u3002\u6e29\u5ea6\u4e3a65\u00b0C\uff0c\u76f8\u5bf9\u6e7f\u5ea6\u4e3a30%\u3002\u4e32\u8054OPV\u7535\u6c60\u7684\u539f\u7406\u56fe\u3001J-V\u66f2\u7ebf\u548cEQE\u66f2\u7ebf\u3002J)\u57fa\u4e8e1.0 cm2<\/sup> PBDB-TF:HDO-4Cl:BTP-eC9\u7535\u6c60\u7684\u5668\u4ef6\u7684J-V\u66f2\u7ebf\u3002\u00a9 2022 Wiley<\/strong><\/p>\n

05<\/strong>\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

\u672c\u5de5\u4f5c\u5c06\u6eb6\u80f6-\u51dd\u80f6ZnO CIL\u4e2d\u6b8b\u7559\u7684\u80fa\u901a\u8fc7\u7528BA\u51b2\u6d17\u6709\u6548\u5730\u53bb\u9664\uff0c\u7559\u4e0b\u5b8c\u6574\u7684\u7ea4\u950c\u77ffZnO\u3002\u8fd9\u79cd\u65b9\u6cd5\u5bf9BHJs\u7684\u7a81\u51fa\u901a\u7528\u6027\u663e\u793a\u4e86\u5728\u672a\u6765\u7684\u5e94\u7528\u4e2d\u7684\u5de8\u5927\u6f5c\u529b\u3002<\/p>\n

\u539f\u6587\u8be6\u60c5\uff1aWang, Y., Zheng, Z., Wang, J., Liu, X., Ren, J., An, C., Zhang, S., Hou, J., New Method for Preparing ZnO Layer for Efficient and Stable Organic Solar Cells. Adv. Mater. 2022, 2208305. https:\/\/doi.org\/10.1002\/adma.202208305<\/strong><\/p>\n

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