{"id":245163,"date":"2022-12-29T06:00:37","date_gmt":"2022-12-28T22:00:37","guid":{"rendered":"\/\/m.iemloyee.com\/?p=245163"},"modified":"2022-12-28T20:38:11","modified_gmt":"2022-12-28T12:38:11","slug":"%e6%b5%99%e6%b1%9f%e5%a4%a7%e5%ad%a6nature-commun%ef%bc%9a%e9%80%9a%e7%94%a8%e7%95%8c%e9%9d%a2%e8%83%bd%e9%87%8f%e8%b0%83%e8%8a%82%e7%ad%96%e7%95%a5%e5%a2%9e%e5%bc%ba%e4%ba%ba%e5%b7%a5%e5%85%89","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=245163","title":{"rendered":"\u6d59\u6c5f\u5927\u5b66Nat.Commun\uff1a\u901a\u7528\u754c\u9762\u80fd\u91cf\u8c03\u8282\u7b56\u7565\u589e\u5f3a\u4eba\u5de5\u5149\u5408\u4f5c\u7528"},"content":{"rendered":"
\u3010\u5bfc\u8bfb\u3011<\/p>\n
\u592a\u9633\u80fd\u88ab\u8ba4\u4e3a\u662f\u89e3\u51b3\u5168\u7403\u65e5\u76ca\u589e\u957f\u7684\u6e05\u6d01\u80fd\u6e90\u9700\u6c42\u548c\u76f8\u5173\u6c14\u5019\u95ee\u9898\u7684\u5173\u952e\u89e3\u51b3\u65b9\u6848\u3002\u4e3a\u4e86\u89e3\u51b3\u592a\u9633\u8f90\u5c04\u7684\u65f6\u7a7a\u6ce2\u52a8\u95ee\u9898\uff0c\u4e00\u4e2a\u7b56\u7565\u662f\u901a\u8fc7\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u5c06\u592a\u9633\u80fd\u6355\u83b7\u4e3a\u53ef\u50a8\u5b58\u548c\u53ef\u8fd0\u8f93\u7684\u592a\u9633\u80fd\u71c3\u6599(\u4f8b\u5982H2<\/sub>\u548cH2<\/sub>O2<\/sub>)\u3002\u5728\u4e3b\u8981\u7684\u5149\u5408\u7cfb\u7edf\u4e2d\uff0c\u9897\u7c92\u5149\u50ac\u5316\u5242\u56e0\u5176\u7b80\u5355\u6027\u548c\u53ef\u6269\u5c55\u6027\u800c\u88ab\u8ba4\u4e3a\u662f\u6700\u5177\u6210\u672c\u6548\u76ca\u7684\u4e00\u79cd\uff0c\u4f46\u5176\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u4ecd\u9700\u63d0\u9ad8\u624d\u80fd\u83b7\u5f97\u53ef\u884c\u7684\u5e94\u7528\u3002\u540c\u65f6\u7531\u4e8e\u9897\u7c92\u5149\u50ac\u5316\u5242\u4e2d\u7684\u7535\u8377\u5206\u79bb\u662f\u7531\u5176\u8fd8\u539f\u4f4d\u70b9\u548c\u6c27\u5316\u4f4d\u70b9\u4e4b\u95f4\u7684\u4e0d\u5bf9\u79f0\u754c\u9762\u80fd\u5b66\u9a71\u52a8\u7684\uff0c\u56e0\u6b64\u589e\u5f3a\u8fd9\u4e00\u8fc7\u7a0b\u9700\u8981\u5728\u4e0d\u635f\u5bb3\u8868\u9762\u53cd\u5e94\u52a8\u529b\u5b66\u548c\u9009\u62e9\u6027\u7684\u524d\u63d0\u4e0b\u5bf9\u754c\u9762\u80fd\u8fdb\u884c\u7eb3\u7c73\u7ea7\u8c03\u6574\u3002<\/p>\n \u3010\u6210\u679c\u63a0\u5f71\u3011<\/p>\n \u8fd1\u65e5\uff0c\u6d59\u6c5f\u5927\u5b66\u891a\u9a70\u6052\u6559\u6388\u901a\u8fc7\u4e00\u79cd\u603b\u4f53\u7b56\u7565\u6765\u5b9e\u73b0\u4e0a\u9762\u7684\u76ee\u6807\uff0c\u8be5\u7b56\u7565\u6d89\u53ca\u5728\u5404\u79cd\u5149\u50ac\u5316\u7cfb\u7edf\u4e0a\u5c55\u793a\u7684\u6838\/\u58f3\u578b\u52a9\u50ac\u5316\u5242\u7684\u5e94\u7528\u3002H2<\/sub>O2<\/sub>\u751f\u6210\u9ad8\u6548\u7387\u9a8c\u8bc1\u4e86\u5bf9\u8c03\u6574\u754c\u9762\u80fd\u91cf\u5b66\u4ee5\u589e\u5f3a\u7535\u8377\u5206\u79bb\u548c\u5149\u5408\u4f5c\u7528\u6027\u80fd\u7684\u89c2\u70b9\u3002\u7279\u522b\u662f\uff0c\u8fd9\u4e00\u7b56\u7565\u5728BiVO4<\/sub>\u7cfb\u7edf\u4e0a\u5f97\u5230\u4e86\u7a81\u51fa\u4f53\u73b0\uff0c\u8be5\u7cfb\u7edf\u7528\u4e8e\u6574\u4f53H2<\/sub>O2<\/sub>\u5149\u5408\u4f5c\u7528\uff0c\u592a\u9633\u80fd\u5230H2<\/sub>O2<\/sub>\u7684\u8f6c\u5316\u7387\u4e3a0.73%\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201cA general interfacial-energetics-tuning strategy for enhanced artificial photosynthesis<\/strong>\u201d\u53d1\u8868\u5728Nature Communications<\/em><\/strong>\u4e0a\u3002\u6d59\u6c5f\u5927\u5b66\u5218\u6dfb\u4e3a\u4e00\u4f5c\uff0c\u6d59\u6c5f\u5927\u5b66\u891a\u9a70\u6052\u6559\u6388\u548c\u65e5\u672c\u4e2d\u592e\u5927\u5b66\u7406\u5de5\u5b66\u9662Zhenhua Pan\u6559\u6388\u4e3a\u5171\u540c\u901a\u8baf\u4f5c\u8005\u3002<\/p>\n \u3010<\/strong>\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n \u672c\u7814\u7a76\u8bc1\u660e\u4e86\u7528\u4e8e\u754c\u9762\u80fd\u91cf\u8c03\u8282\u7684\u6838\/\u58f3\u52a9\u50ac\u5316\u5242\u7ed3\u6784\u7684\u53ef\u884c\u6027\uff0c\u5e76\u4e14\u8bc1\u660e\u4e86\u5176\u5bf9\u4e8e\u589e\u5f3a\u5149\u5408\u4f5c\u7528\u7cfb\u7edf\u4e2d\u7684\u7535\u8377\u5206\u79bb\u548c\u6027\u80fd\u7684\u9ad8\u5ea6\u901a\u7528\u6027\u3002<\/p>\n \u3010\u6570\u636e\u6982\u51b5\u3011<\/p>\n \u56fe1:Ag\/Pd\u6838\/\u58f3\u578b\u8f85\u50ac\u5316\u5242\u5728BiVO4<\/sub>\u4e0a\u7684\u9762\u9009\u62e9\u6027\u8d1f\u8f7d\u548c\u754c\u9762\u80fd\u91cf\u5b66\u8c03\u6574\u3002<\/p>\n a Co\u3001Ag\u548cPd\u5728BiVO4<\/sub>\u4e0a\u7684\u9010\u6b65\u548c\u9762\u9009\u62e9\u6027\u5149\u6c89\u79ef\u3002b\u80fd\u91cf\u8272\u6563x\u5c04\u7ebf\u80fd\u8c31(EDS)\u5143\u7d20\u6620\u5c04\u548c\u7ebf\u5256\u9762\uff0c\u4ee5\u53caCoOx<\/sub>\/BiVO4<\/sub>\/(Ag\/Pd)\u7684\u767d\u8272\u7bad\u5934\u3002c, d\u5728BiVO4<\/sub>\u4e0a\u8d1f\u8f7dAg\/Pd\u7c92\u5b50\u7684\u626b\u63cf\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c(STEM)-EDS\u5143\u7d20\u6620\u5c04\u3002e BiVO4<\/sub>\u3001BiVO4<\/sub>\/Ag\u3001BiVO4<\/sub>\/Pd\u3001BiVO4<\/sub>\/(Ag\/Pd)\u7684\u7d2b\u5916\u5149\u7535\u5b50\u80fd\u8c31(UPS)\u3002f BiVO4<\/sub>\u4e0aAg\/Pd\u6838\/\u58f3\u5171\u50ac\u5316\u5242\u6784\u5efa{010}\u8fd8\u539f\u9762\u754c\u9762\u80fd\u91cf\u5b66\u8c03\u6574\u793a\u610f\u56fe\u3002\u00a92022 Springer Nature<\/p>\n \u56fe2:H2<\/sub>O2<\/sub>\u5149\u5408\u4f5c\u7528\u603b\u91cf\u3002<\/p>\n a\u5149\u50ac\u5316\u751f\u6210H2<\/sub>O2<\/sub>\u7684\u65f6\u95f4\u8fc7\u7a0b\u3002b BiVO4<\/sub>\u3001BiVO4<\/sub>\/Ag\u3001BiVO4<\/sub>\/Pd\u3001BiVO4<\/sub>\/(Ag\/Pd)\u4ea7H2<\/sub>O2<\/sub>\u7684\u9009\u62e9\u6027\u3002c\u5404\u79cd\u6838\u58f3\u8f85\u50ac\u5316\u5242\u7684\u5236\u5907\u53caH2<\/sub>O2<\/sub>\u5149\u5408\u4f5c\u7528\u6027\u80fd\u4e0e\u6838\u7ed3\u91d1\u5c5e\u529f\u51fd\u6570\u7684\u5173\u7cfb\u3002d\u5bcc\u2022OH\u6761\u4ef6\u4e0bCoOx<\/sub>\/BiVO4<\/sub>\/(Ag\/Pd)\u548cC3<\/sub>N4<\/sub>\/Pd H2<\/sub>O2<\/sub>\u5149\u5408\u4f5c\u7528\u6d3b\u6027\u7684\u8870\u51cf\u3002e\u91cd\u590d\u4f7f\u7528CoOx<\/sub>\/BiVO4<\/sub>\/(Ag\/Pd)\u8fdb\u884cH2<\/sub>O2<\/sub>\u5149\u5408\u4f5c\u7528\u3002f CoOx<\/sub>\/Mo:BiVO4<\/sub>\/(Ag\/Pd)\u5149\u50ac\u5316\u751f\u6210H2<\/sub>O2<\/sub>\u7684\u65f6\u95f4\u8fdb\u7a0b\u53ca\u76f8\u5e94\u7684STH\u6548\u7387\u3002g H2<\/sub>O2<\/sub>\u5728CoOx<\/sub>\/Mo:BiVO4<\/sub>\/(Ag\/Pd)\u4e0a\u5149\u5408\u4f5c\u7528\u7684\u8868\u89c2\u91cf\u5b50\u4ea7\u989d(AQY)\u968f\u5165\u5c04\u5149\u6ce2\u957f\u7684\u53d8\u5316\u3002\u00a92022 Springer Nature<\/p>\n \u56fe3:\u8f7d\u6d41\u5b50\u52a8\u529b\u5b66\u3002<\/p>\n a, b\u57282000 nm\u5904\u63a2\u6d4b\u7684\u81ea\u7531\/\u6d45\u4fd8\u83b7\u7535\u5b50\u548c\u5728505 nm\u5904\u63a2\u6d4b\u7684\u4fd8\u83b7\u7a7a\u7a74\u7684\u77ac\u6001\u5206\u5e03\u3002c, d\u5728\u771f\u7a7a\u548cHCOOH\u84b8\u6c7d\u5b58\u5728\u4e0b\uff0c\u5728505 nm\u5904\u63a2\u6d4bc CoOx<\/sub>\/BiVO4<\/sub>\/Pd\u548cd CoOx<\/sub>\/BiVO4<\/sub>\/(Ag\/Pd)\u4fd8\u83b7\u5b54\u7684\u77ac\u6001\u5206\u5e03\u3002e\u901a\u8fc7\u8868\u9762\u80fd\u91cf\u5b66\u8c03\u6574\u589e\u5f3a\u7684\u7535\u8377\u5206\u79bb\u8fc7\u7a0b\u793a\u610f\u56fe\u3002\u00a92022 Springer Nature<\/p>\n \u56fe4:\u5149\u8f7d\u6d41\u5b50\u5206\u5e03\u7684\u6a21\u62df\u3002<\/p>\n a, b BiVO4<\/sub>\u4f5c\u4e3a\u592a\u9633\u80fd\u7535\u6c60\u7684\u793a\u610f\u56fe\u6a21\u578b\u548c\u80fd\u5e26\u56fe\u3002c\u5728\u9634\u6781\u4f4d\u7f6e(\u03a6010)\uff0c\u968f\u7740\u52bf\u5792\u9ad8\u5ea6\uff0c\u7535\u6d41\u5bc6\u5ea6\u4e0e\u5e94\u7528\u7535\u4f4d\u53d8\u5316\u8303\u56f4\u4e3a0\u81f30.4 V(\u7070\u8272\u865a\u7ebf\u7bad\u5934)\u3002d – i BiVO4<\/sub>\u7c92\u5b50\u5149\u7535\u7279\u6027\u7684\u4e8c\u7ef4\u622a\u9762\u56fe\uff0c\u5305\u62ec\u5bfc\u5e26\u80fd\u91cf(eV) (d, e)\u3001\u7535\u5b50\u6d53\u5ea6(f, g)\u548c\u7a7a\u7a74\u6d53\u5ea6(h, i)\u3002j – m\u80fd\u5e26\u56fe(j, k)\u548c\u79fb\u52a8\u8f7d\u6d41\u5b50\u5bc6\u5ea6(l, m)\u7684\u4e00\u7ef4\u56fe\u3002\u00a92022 Springer Nature<\/p>\n \u56fe5:\u589e\u5f3a\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u7684\u754c\u9762-\u80fd\u91cf-\u8c03\u8282\u7b56\u7565\u7684\u901a\u5219\u3002<\/p>\n a C3<\/sub>N4<\/sub>\/Pd\u3001C3<\/sub>N4<\/sub>\/(Ag\/Pd)\uff0cb TiO2<\/sub>\/Pd\u3001TiO2<\/sub>\/(Ag\/Pd)\u5149\u50ac\u5316H2<\/sub>O2<\/sub>\u751f\u6210\u7684\u65f6\u95f4\u8fc7\u7a0b\u3002c\u6709\u6548\u754c\u9762\u80fd\u91cf\u8c03\u8282\u548c\u589e\u5f3a\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u7684\u4e00\u822c\u65b9\u6cd5\u3002\u00a92022 Springer Nature<\/p>\n \u3010\u6210\u679c\u542f\u793a\u3011<\/p>\n \u603b\u4e4b\uff0c\u672c\u7814\u7a76\u9a8c\u8bc1\u4e86\u754c\u9762\u80fd\u91cf\u5b66\u7684\u8c03\u6574\u662f\u589e\u5f3a\u7535\u8377\u5206\u79bb\u7684\u4e00\u79cd\u666e\u904d\u6709\u6548\u7684\u65b9\u6cd5\uff0c\u8fd9\u662f\u8bbe\u8ba1\u9ad8\u6027\u80fd\u5149\u50ac\u5316\u5242\u7684\u4e00\u4e2a\u5173\u952e\u6311\u6218\u3002\u6838\/\u58f3Ag\/Pd\u5171\u50ac\u5316\u5242\u7684\u6784\u5efa\u964d\u4f4e\u4e86BiVO4<\/sub>{010}\u9762\u7684\u8096\u7279\u57fa\u52bf\u5792\uff0c\u800c\u4e0d\u5f71\u54cd\u8868\u9762\u53cd\u5e94\uff0c\u5bfc\u81f4\u80fd\u91cf\u5b66\u548c\u7535\u8377\u5206\u79bb\u7684\u6574\u4f53\u4e0d\u5bf9\u79f0\u6027\u589e\u5f3a\u3002\u901a\u8fc7\u6210\u529f\u8c03\u6574\u754c\u9762\u80fd\u91cf\u5b66\uff0cBiVO4<\/sub>\u751f\u6210\u7684H2<\/sub>O2<\/sub>\u5728\u5168\u5149\u8c31\u4e0bAQY\u4e3a3.0%\uff0cSTH\u6548\u7387\u4e3a0.73%\uff0c\u8fd9\u662f\u65e0\u673a\u534a\u5bfc\u4f53\u4f53\u7cfb\u7684\u65b0\u8bb0\u5f55\u3002\u6b63\u5982BiVO4<\/sub>\u7528\u4e8eH2<\/sub>O2<\/sub>\u4ea7\u751f\u6240\u5f3a\u8c03\u7684\u90a3\u6837\uff0c\u8fd9\u79cd\u8c03\u6574\u754c\u9762\u80fd\u91cf\u5b66\u7684\u7b56\u7565\u4e00\u822c\u53ef\u4ee5\u5e94\u7528\u4e8e\u5176\u4ed6\u5149\u5408\u7cfb\u7edf\uff0c\u4ee5\u4fc3\u8fdb\u592a\u9633\u80fd\u71c3\u6599\u7684\u751f\u4ea7\uff0c\u5982\u6c34\u5206\u89e3\u548c\u4e8c\u6c27\u5316\u78b3\u51cf\u5c11\u3002<\/p>\n <\/p>\n <\/p>\n <\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n
<\/p>\n