{"id":243900,"date":"2022-11-11T06:57:33","date_gmt":"2022-11-10T22:57:33","guid":{"rendered":"\/\/m.iemloyee.com\/?p=243900"},"modified":"2022-11-10T19:57:52","modified_gmt":"2022-11-10T11:57:52","slug":"nature-materials%ef%bc%9a%e5%8f%96%e5%90%91%e7%9b%b8%e7%95%b4%e5%af%b9mg2%e5%b5%8c%e5%85%a5%ce%bb-mno2%e7%94%b5%e5%8c%96%e5%ad%a6%e9%98%b4%e6%9e%81%e7%9a%84%e5%bd%b1%e5%93%8d","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=243900","title":{"rendered":"Nature 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Jian-Min Zuo \u548c Qian Chen\u7684\u56e2\u961f\uff0c\u53d1\u8868\u4e86\u8bba\u6587\u9898\u76ee\u4e3a\uff1a\u201cFormation and impact of nanoscopic oriented phase domains in electrochemical crystalline electrodes\u201d\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243901\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/0-2.png\" alt=\"\" width=\"998\" height=\"547\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/0-2.png 998w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/0-2-300x164.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/0-2-768x421.png 768w\" sizes=\"(max-width: 998px) 100vw, 998px\" 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<sub>t<\/sub>\u76f8\u53d6\u5411\u5171\u5b58\u4e8eNP\u4e2d\uff1b<\/p>\n<p>3\uff1a\u6536\u96c6\u5f97\u5230\u6570\u636e\u96c6\uff0c\u901a\u8fc7\u6570\u636e\u6316\u6398\u65b9\u6cd5\u7814\u7a766\u4e2a\u539f\u59cb\u7684\u7eb3\u7c73\u9897\u7c92\u6a21\u578b\uff0c\u5f97\u5230\u7684\u53d6\u5411\u56fe\u663e\u793a\u5355\u76f8\u53d6\u5411\u7684\u7a7a\u95f4\u5206\u5e03\u662f\u5747\u5300\u7684\u3002<\/p>\n<p>\u3010\u6570\u636e\u6982\u8bba\u3011<\/p>\n<p>\u56fe1 \u6210\u5206\u5747\u5300\u7684\u9634\u6781\u7eb3\u7c73\u9897\u7c92\u4e2d\u7684\u53d6\u5411\u76f8\u7574\u3002a.\u9634\u6781NPs\u5c40\u90e8\u6676\u683c\u7ed3\u6784\u76844D-STEM\u6620\u5c04\u793a\u610f\u56fe;.b.\u653e\u7535\u524dMnO<sub>2<\/sub>\u9634\u6781NP\u7684HAADF\u56fe\u50cf(\u5de6)\u548c\u5bf9\u5e94\u76844D-STEM\u6c47\u603b\u56fe(\u53f3);.c,d.\u6676\u4f53\u5b66\u53d6\u5411<strong>n<\/strong>\u548c(c) \u5e94\u53d8\u5206\u5e03\u03b5<sub>xx<\/sub>\u548c\u03b5<sub>yy<\/sub> (d)\u5728\u539f\u59cbMnO<sub>2<\/sub>\u9634\u6781NP;.e.\u9634\u6781NPs\u7b2c\u4e00\u6b21\u5728\u4e0d\u540c\u622a\u6b62\u7535\u538b\u4e0b\u6052\u6d41\u653e\u7535NP\u4e0e\u5176\u5bf9\u5e94\u7684XRD\u8c31\u56fe;.f.\u5e73\u5747Mn L<sub>3<\/sub>\/L<sub>2<\/sub>\u6bd4\u548c\u6839\u636eEELS\u6620\u5c04\u8ba1\u7b97\u51fa\u7684\u6bcf\u4e2aNP\u7684\u8f6c\u6362Mn\u6c27\u5316\u6001(<em>m<\/em>):\u6570\u636e\u8868\u793a\u4e3a\u5e73\u5747\u503c\u00b1\u6807\u51c6\u5dee;.g.\u9634\u6781NP\u70b9\u7684ADF\u56fe\u50cf; h. \u9634\u6781NP\u5728\u653e\u7535\u7ed3\u675f\u540e\u865a\u62df\u7684ADF\u56fe\u50cf; i-k.Mn\u6c27\u5316\u6001\u56fe\u00a9 2022 Nature Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243912\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/1-7.png\" alt=\"\" width=\"638\" height=\"746\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/1-7.png 638w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/1-7-257x300.png 257w\" sizes=\"(max-width: 638px) 100vw, 638px\" \/><\/p>\n<p>\u56fe2 \u653e\u7535\u7eb3\u7c73\u9897\u7c92\u4e2d\u7684\u53d6\u5411\u76f8\u7574\u5f62\u8c8c\u4ee5\u53ca\u5bf9\u79f0\u6027\u53d8\u5316\u7684\u8d77\u6e90\u3002a,c.\u865a\u62dfADF\u56fe\u50cf\uff0c\u5728\u7535\u89e3\u8d28\u6eb6\u6db2\u4e2d\u9634\u6781NP\u653e\u7535\u7ed3\u675f\u65f6\uff0cC\/10\u7684\u53d6\u5411\u6620\u5c04\u56fe\u548c\u5e94\u53d8\u56fe; d.\u865a\u62dfADF\u56fe\u50cf\uff0c\u9634\u6781NPs\u5728\u653e\u7535\u7ed3\u675f\u65f6\u5728C\/20 \u548cC \/50\u7684\u53d6\u5411\u6620\u5c04\u56fe\u548c\u5e94\u53d8\u56fe; g. \u03b5<sub>yy<\/sub>\u76f4\u65b9\u56fe\u5448\u73b0\u72ec\u7279\u7684\u5256\u9762\u5bf9\u5e94\u4e8ea\u4e2d\u7684\u5b9a\u5411\u76f8\u57df\u5f62\u6001\u3002\u00a9 2022 Nature Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243909\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/2-6.png\" alt=\"\" width=\"636\" height=\"750\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/2-6.png 636w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/2-6-254x300.png 254w\" sizes=\"(max-width: 636px) 100vw, 636px\" \/><\/p>\n<p>\u56fe3 \u00a0\u5728\u6574\u4e2a\u653e\u7535\u8fc7\u7a0b\u4e2d\uff0c\u9634\u6781\u7eb3\u7c73\u9897\u7c92\u5185\u53d6\u5411\u76f8\u7574\u7684\u6210\u6838\u3001\u751f\u957f\u548c\u5408\u5e76\u8fc7\u7a0b\u3002a.\u5728\u4e94\u79cd\u4e0d\u540c\u622a\u6b62\u7535\u538b(V vs Ag\/AgCl)\u4e0b\u6536\u96c6\u7684\u9634\u6781NPs\u7684\u7b2c\u4e00\u6b21\u653e\u7535\u65f6\u53d6\u5411\u6620\u5c04\u56fe; b,c. \u5728\u4e0d\u540c\u622a\u6b62\u7535\u538b\u4e0b\u03c1 (b)\u548c\u9762\u79ef\u5206\u6570(A\/A<sub>0<\/sub>) (c)\u5728\u7edf\u8ba1\u8ba1\u7b97\u7684\u6295\u5f71\u57df\uff0c\u6570\u636e\u8868\u793a\u4e3a\u5e73\u5747\u503c\u00b1\u6807\u51c6\u5dee;d.Mn\u6c27\u5316\u6001\u7684\u53d6\u5411\u56fe\u548cEELS\u56fe;e, g(r) 6\u4e2a\u9634\u6781Nps\u5728\u76f8\u540c\u65b9\u5411\u548c\u4e0d\u540c\u65b9\u5411\u7684\u57df\u3002\u00a9 2022 Nature Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243910\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/3-6.png\" alt=\"\" width=\"691\" height=\"620\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/3-6.png 691w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/3-6-300x269.png 300w\" sizes=\"(max-width: 691px) 100vw, 691px\" \/><\/p>\n<p>\u56fe4 \u4e0d\u540c\u7535\u89e3\u8d28\u6761\u4ef6\u4e0b\u7684\u53d6\u5411\u76f8\u7574\u53ca\u5176\u5bf9\u5e94\u53d8\u68af\u5ea6\u548c\u79bb\u5b50\u6269\u6563\u7684\u5f71\u54cd\u3002a,b.\u56db\u79cd\u5177\u6709\u4ee3\u8868\u6027\u7684\u9634\u6781NPs\u5728\u6e7f\u6709\u673a\u7535\u89e3\u8d28(a)\u548c\u5e72\u6709\u673a\u7535\u89e3\u8d28(b)\u4e2d\u653e\u7535\u540e\u7684\u865aADF\u56fe\u50cf\u3001\u53d6\u5411\u6620\u5c04\u56fe\u3001\u5e94\u53d8\u56fe\u548c\u03b5<sub>yy<\/sub> (\u03b7<sub>yy<\/sub>)\u7684\u5e94\u53d8\u68af\u5ea6\u56fe; c.\u4e0d\u540c\u7535\u89e3\u8d28\u6761\u4ef6\u4e0b\u9634\u6781NPs\u4e8c\u7ef4\u6295\u5f71\u7574\u7684\u5e73\u5747\u6570\u91cf\u5bc6\u5ea6;d.GITT\u6d4b\u91cf\u4e2d\u9634\u6781NPs\u5728\u6e7f\u548c\u5e72\u6709\u673a\u7535\u89e3\u8d28\u4e2d\u7b2c\u4e00\u6b21\u653e\u7535\u65f6\u7684\u7535\u538b\u54cd\u5e94\u3002\u00a9 2022 Nature Materials<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243911\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/4-6.png\" alt=\"\" width=\"912\" height=\"556\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/4-6.png 912w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/4-6-300x183.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/11\/4-6-768x468.png 768w\" sizes=\"(max-width: 912px) 100vw, 912px\" \/><\/p>\n<p>\u3010\u6210\u679c\u5c55\u793a\u3011<\/p>\n<p>\u5728\u6587\u7ae0\u4e2d\uff0c\u901a\u8fc7\u5b9a\u91cf\u5730\u7ed8\u5236\u4e86\u7535\u5316\u5b66\u79bb\u5b50\u63d2\u5165\u8fc7\u7a0b\u4e2d\u53d6\u5411\u76f8\u7574\u7684\u5f62\u6210\u548c\u5e94\u53d8\u68af\u5ea6\u7684\u8fc7\u7a0b\u3002\u91c7\u7528\u5171\u5b9a\u4f4d\u56db\u7ef4\u626b\u63cf\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u548c\u7535\u5b50\u80fd\u91cf\u635f\u5931\u8c31\u65b9\u6cd5\uff0c\u5e76\u7ed3\u5408\u6570\u636e\u6316\u6398\uff0c\u4f7f\u7814\u7a76\u6210\u4e3a\u53ef\u80fd\u3002\u7ed3\u679c\u8868\u660e\uff0c\u5728\u03bb-MnO<sub>2<\/sub>\u7684\u6a21\u578b\u4f53\u7cfb\u4e2d\uff0cMg<sup>2+<\/sup>\u63d2\u5165\u7acb\u65b9\u5c16\u6676\u77f3MnO<sub>2<\/sub>\u7eb3\u7c73\u9897\u7c92\u540e\u53d1\u751f\u76f8\u53d8\uff0c\u5728\u7eb3\u7c73\u5c3a\u5ea6\u4e0a\u5f62\u6210\u5177\u6709\u76f8\u4f3c\u5316\u5b66\u7279\u6027\u4f46\u4e0d\u540c\u53d6\u5411\u7684\u7574\uff0c\u5e76\u9075\u5faa\u6210\u6838\u3001\u751f\u957f\u548c\u5408\u5e76\u8fc7\u7a0b\u3002\u6b64\u5916\uff0c\u5e94\u53d8\u68af\u5ea6\u662f\u7531\u76f8\u7574\u5728\u5176\u8fb9\u754c\u4e0a\u7684\u53d1\u5c55\u5f62\u6210\u7684\uff0c\u5bf9\u5316\u5b66\u6269\u6563\u7cfb\u6570\u7684\u5f71\u54cd\u662f10\u500d\u6216\u66f4\u591a\u3002\u56e0\u6b64\uff0c\u7814\u7a76\u7ed3\u679c\u4e3a\u5fae\u89c2\u7ed3\u6784\u5f62\u6210\u673a\u5236\u53ca\u5176\u5bf9\u79bb\u5b50\u63d2\u5165\u8fc7\u7a0b\u7684\u5f71\u54cd\u63d0\u4f9b\u4e86\u91cd\u8981\u7684\u89c1\u89e3\uff0c\u4e3a\u50a8\u80fd\u6750\u6599\u7684\u8f6c\u53d8\u7ed3\u6784\u63a7\u5236\u63d0\u4f9b\u4e86\u65b0\u7684\u89c4\u5219\u3002<\/p>\n<p>\u53c2\u8003\u6587\u732e<\/p>\n<p>Chen, W., Zhan, X., Yuan, R. et al. Formation and impact of nanoscopic oriented phase domains in electrochemical crystalline electrodes. Nat. Mater. (2022).<\/p>\n<p>\u6587\u732e\u94fe\u63a5https:\/\/www.nature.com\/articles\/s41563-022-01381-4<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u3010\u5bfc\u8bfb\u3011 \u6750\u6599\u7684\u76f8\u662f\u5728\u7279\u5b9a\u53d6\u5411\u7684\u76f8\u7574\u4e2d\u6392\u5217\u5f62\u6210\u7684\uff0c\u8fd9\u79cd\u7cbe\u7ec6\u5fae\u7ed3\u6784\u63a7\u5236\u7740\u6750\u6599\u7684\u7269\u7406\u548c\u529b\u5b66\u6027\u80fd\u3002\u5f53\u7269\u8d28\u7684\u5bf9\u79f0\u6027\u53d1\u751f\u53d8\u5316\u65f6\uff0c\u8fd9\u79cd\u76f8\u53d8\u5fae\u7ed3\u6784\u5e7f\u6cdb\u5b58\u5728\u4e8e\u76f8\u53d8\u56fa\u4f53\u4e2d\uff0c\u5e76\u4e14\u5bf9&#8230;<\/p>\n","protected":false},"author":35611,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-243900","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243900"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/35611"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=243900"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243900\/revisions"}],"predecessor-version":[{"id":243920,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243900\/revisions\/243920"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=243900"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=243900"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=243900"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}