{"id":243253,"date":"2022-10-19T06:55:22","date_gmt":"2022-10-18T22:55:22","guid":{"rendered":"\/\/m.iemloyee.com\/?p=243253"},"modified":"2022-10-18T20:55:48","modified_gmt":"2022-10-18T12:55:48","slug":"%e9%99%88%e5%bf%a0%e4%bc%9f%e4%bd%99%e7%88%b1%e8%90%8d%e7%8e%8b%e6%96%b0nature-energy%ef%bc%9a%e5%88%a9%e7%94%a8co2%e6%ba%b6%e5%87%ba%e8%af%b1%e5%af%bc%e6%b5%81%e5%8a%a8%e7%94%b5%e8%a7%a3%e6%b1%a0","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=243253","title":{"rendered":"\u9648\u5fe0\u4f1f&\u4f59\u7231\u840d&\u738b\u65b0Nature Energy\uff1a\u5229\u7528CO2\u6eb6\u51fa\u8bf1\u5bfc\u6d41\u52a8\u7535\u89e3\u6c60\u8fdb\u884c\u8fde\u7eedCO2\u7535\u89e3\uff01"},"content":{"rendered":"

\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u8fd1\u5e74\u6765\uff0c\u7528\u4e8e\u5e38\u6e29CO2<\/sub>\u8fd8\u539f\u53cd\u5e94\uff08CO2<\/sub>RRs\uff09\u7684\u7535\u50ac\u5316\u6750\u6599\u5728\u50ac\u5316\u5242\u6d3b\u6027\u548c\u9009\u62e9\u6027\u65b9\u9762\u53d6\u5f97\u4e86\u91cd\u5927\u8fdb\u5c55\u3002\u7136\u800c\uff0cCO2<\/sub>RR\u7684\u5de5\u4e1a\u5e94\u7528\u9700\u8981\u52a0\u901f\u53cd\u5e94\u901f\u7387\uff08\u7535\u6d41\u5bc6\u5ea6\u5927\u4e8e1 A \u2009cm-2<\/sup>\uff09\u4ee5\u6700\u5c0f\u5316\u64cd\u4f5c\u6210\u672c\uff0c\u7ec4\u88c5\u5927\u578b\u7ecf\u6d4e\u7535\u89e3\u6c60\uff08\u7535\u6781\u5c3a\u5bf8\u8d85\u8fc7100\u2009cm2<\/sup>\uff09\u4ee5\u6700\u5c0f\u5316\u8d44\u672c\u6210\u672c\u3002\u4f46\u662f\uff0c\u5f53\u7535\u6d41\u5bc6\u5ea6\u8fdb\u4e00\u6b65\u589e\u5927\u65f6\uff0c\u53cd\u5e94\u53d7\u5230\u4f20\u8d28\u7684\u9650\u5236\uff0c\u63d0\u9ad8\u4e86\u6311\u6218\u6027\u3002\u56e0\u6b64\uff0c\u7406\u60f3\u7684\u7535\u6781\u7ed3\u6784\u9700\u8981\u5e73\u8861\u53cd\u5e94\u7269\u8fdb\u6599\u3001\u53cd\u5e94\u52a8\u529b\u5b66\u548c\u4ea7\u7269\u6392\u51fa\uff0c\u540c\u65f6\u51cf\u5c0f\u6d41\u4f53\u52a8\u529b\u6269\u6563\u5c42\u5c40\u90e8\u5fae\u73af\u5883\u4e2d\u5404\u79cd\u7269\u8d28\u7684\u6d53\u5ea6\u68af\u5ea6\u81f3\u5173\u91cd\u8981\u3002\u5728\u7535\u89e3\u69fd\u4e2d\u4f7f\u7528\u6c14\u4f53\u6269\u6563\u7535\u6781\uff08GDEs\uff09\uff0c\u53ef\u4ee5\u63d0\u9ad8CO2<\/sub>\u5728\u50ac\u5316\u5242\u8868\u9762\u7684\u5c40\u90e8\u6d53\u5ea6\uff0c\u6240\u4ee5\u5728\u62a5\u9053\u7684GDE\u7535\u89e3\u6c60\u4e2d\uff0c\u4e00\u822c\u7684\u4e09\u76f8\u754c\u9762\uff08TPBs\uff09\u662f\u901a\u8fc7CO2<\/sub>\u6c14\u76f8\u548c\u6db2\u76f8\u78b1\u6027\u9634\u6781\u6db2\u7684\u540c\u65f6\u8fdb\u6599\u6765\u6784\u5efa\u7684\uff0c\u867d\u7136\u8be5\u7535\u89e3\u6c60\u53ef\u8fbe\u52301.4 A cm-2<\/sup>\u7684\u6700\u5927\u7535\u6d41\u5bc6\u5ea6\uff08J<\/em>max<\/sub>\uff09\uff0c\u4f46\u8f93\u5165\u7684CO2<\/sub>\u53cd\u5e94\u7269\u5c06\u635f\u5931\u6210\u78b3\u9178\u6c22\u76d0\u548c\u78b3\u9178\u76d0\uff0c\u5bfc\u81f4GDE\u7a7a\u9699\u4e2d\u7684\u6c89\u6dc0\u3002\u6b64\u5916\uff0cGDE\u7535\u89e3\u6c60\u4f7f\u7528\u589e\u6e7fCO2<\/sub>\u5165\u53e3\u548c\u819c\u7535\u6781\u7ec4\u4ef6\uff0c\u53ef\u4ee5\u7b80\u5316\u7535\u6c60\u914d\u7f6e\u5e76\u63d0\u9ad8\u7a33\u5b9a\u6027\u3002\u7136\u800c\uff0c\u8fd9\u79cd\u7535\u89e3\u6c60\u7684J<\/em>max<\/sub>\u4ecd\u5f88\u96be\u8d85\u8fc71.0 A cm-2<\/sup>\uff0c\u53ef\u80fd\u4e0e\u79bb\u5b50\u7535\u5bfc\u7387\u964d\u4f4e\u548c\u8d28\u5b50\u5229\u7528\u7387\u4f4e\u6709\u5173\u3002\u56e0\u6b64\uff0c\u9700\u8981\u8fdb\u4e00\u6b65\u63d0\u9ad8\u751f\u4ea7\u901f\u7387\u548c\u7535\u6781\u7ed3\u6784\u7684\u7a33\u5b9a\u6027\uff0c\u7279\u522b\u662f\u5bf9\u89c4\u6a21\u5316\u7535\u89e3\u6c60\u7684\u7ec4\u88c5\u3002<\/p>\n

\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u9648\u5fe0\u4f1f\u9662\u58eb\u548c\u4f59\u7231\u840d\u6559\u6388\u3001\u534e\u5357\u5e08\u8303\u5927\u5b66\u738b\u65b0\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u7535\u89e3\u69fd\uff0c\u8be5\u7535\u89e3\u69fd\u4f7f\u7528\u542b\u6c34CO2<\/sub>\u9971\u548c\u9634\u6781\u6db2\u5728\u591a\u5b54\u7535\u6781\u4e2d\u7684\u5f3a\u5236\u5bf9\u6d41\uff0c\u5229\u7528CO2<\/sub>(g)-\u6db2\u4f53-\u50ac\u5316\u5242\u754c\u9762\u7684\u539f\u4f4d\u5f62\u6210\u6765\u6539\u5584CO2<\/sub>\u3001\u7535\u5b50\u3001\u8d28\u5b50\u548c\u4ea7\u7269\uff08CEPP\uff09\u4f20\u8f93\u8f6c\u79fb\u6765\u8fbe\u5230\u9ad8\u7535\u6d41\u5bc6\u5ea6\u3002\u7531\u4e8e\u5c40\u90e8\u538b\u529b\u964d\u4f4e\u7684\u663e\u8457\u5f71\u54cd\uff0c\u5f53\u6d41\u4f53\u88ab\u8feb\u5728\u591a\u5b54\u7535\u6781\u5185\u6d41\u52a8\u65f6\uff0c\u4f1a\u53d1\u751fCO2<\/sub>(g)\u7684\u6eb6\u51fa\uff0c\u4ece\u800c\u5bfc\u81f4\u539f\u4f4d\u5f62\u6210\u4e09\u76f8\u754c\u9762\uff08TPBs\uff09\u3002\u8fd9\u4e9bTPBs\u968f\u7740\u53cd\u5e94\u7684\u8fdb\u884c\u800c\u52a8\u6001\u518d\u751f\uff0c\u800c\u8fd9\u79cd\u5e26\u6709\u6d41\u52a8\u8bf1\u5bfc\u52a8\u6001TPBs\u7684CO2<\/sub>RR\u7535\u89e3\u69fd\u79f0\u4e3aFTDT-cell\u3002\u968f\u7740\u6269\u6563\u5c42\u539a\u5ea6\uff08\u03b4<\/em>DL<\/sub>\uff09\u51cf\u5c11\u5341\u500d\uff0c\u6253\u7834\u4e86\u8d28\u91cf\u4f20\u8f93\u9650\u5236\u3002\u6b64\u5916\uff0c\u901a\u8fc7\u539f\u4f4d\u7535\u6c89\u79ef\u9634\u6781\u7ea4\u7ef4\u5b8c\u5168\u88ab\u914d\u4f53\u4fee\u9970\u7684Ag\u6d3b\u6027\u4f4d\u70b9\u5305\u88f9\uff0c\u4ece\u800c\u63d0\u4f9b\u4e30\u5bcc\u7684\u6d3b\u6027\u4f4d\u70b9\u5e76\u4fc3\u8fdb\u53cd\u5e94\u52a8\u529b\u5b66\u3002\u5b9e\u9a8c\u6d4b\u8bd5\u53d1\u73b0\uff0c\u4f7f\u7528Ag\u57fa\u50ac\u5316\u5242\u7684FTDT-cell\u7684\u6700\u5927\u7535\u6d41\u5bc6\u5ea6\u8fbe\u5230\u4e863.37 A cm-2<\/sup>\uff0c\u5e76\u7ec4\u88c5\u5f62\u62104\u2009\u00d7\u2009100\u2009cm2<\/sup>\u7535\u5806\uff0c\u4ee590.6 L h-1<\/sup>\u7684\u901f\u7387\u4ea7\u751fCO\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cContinuous CO2<\/sub> electrolysis using a CO2<\/sub> exsolution-induced flow cell\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Energy<\/em>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u3010\u6838\u5fc3\u521b\u65b0\u3011<\/strong><\/p>\n

\u5e26\u6709\u6d41\u52a8\u8bf1\u5bfc\u52a8\u6001TPBs\u7684FTDT-cell\uff0c\u968f\u7740\u6269\u6563\u5c42\u539a\u5ea6\uff08\u03b4<\/em>DL<\/sub>\uff09\u51cf\u5c11\u5341\u500d\uff0c\u6253\u7834\u4e86\u8d28\u91cf\u4f20\u8f93\u9650\u5236\uff0c\u540c\u65f6\u63d0\u5347\u78b3\u6e90\u3001\u7535\u5b50\u3001\u8d28\u5b50\u548c\u4ea7\u7269\u7684\u4f20\u9012\u8f6c\u79fb\uff0c\u5b9e\u73b0\u4e86\u8d85\u9ad8\u4ea7\u7269\u6536\u7387\uff0c\u6b64\u5916\uff0c\u4f7f\u7528Ag\u57fa\u50ac\u5316\u5242\u7684FTDT\u69fd\u7684\u6700\u5927\u7535\u6d41\u5bc6\u5ea6\u8fbe\u5230\u4e863.37 A cm-2<\/sup>\uff0c\u5e76\u7ec4\u88c5\u62104\u2009\u00d7\u2009100\u2009cm2<\/sup>\u7535\u5806\uff0c\u4ee590.6 L h-1<\/sup>\u7684\u901f\u7387\u4ea7\u751fCO\u3002<\/p>\n

\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u6d41\u52a8\u8bf1\u5bfc\u52a8\u6001TPBs\u7684\u5f62\u6210<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09CEPP\u5728\u50ac\u5316\u8868\u9762\u9644\u8fd1\u4e0d\u540c\u5c3a\u5ea6\u4e0a\u7684\u534f\u540c\u8f6c\u79fb\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u5df2\u62a5\u9053\u4e0d\u540c\u7535\u89e3\u69fd\u548c\u4e0d\u540cCO2<\/sub>\u4f9b\u5e94\u65b9\u5f0f\u5b9e\u73b0\u7684\u6700\u5927\u7535\u6d41\u5bc6\u5ea6\uff1b<\/p>\n

\uff08c-d\uff09\u5178\u578b\u7684GDEA\u7535\u89e3\u6c60\u548cGDEM\u7535\u89e3\u6c60\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08e\uff09\u4ece\u52a8\u6001\u5e73\u8861E1\u548cE2\u4e2d\u62bd\u5438CO2<\/sub>\u9971\u548c\u9634\u6781\u6db2\u7684FTDT\u7535\u89e3\u6c60\u7684\u56fe\u793a\uff0c\u5176\u4e2dCO2<\/sub>\u4ece\u591a\u5b54\u7535\u6781\u4e2d\u6790\u51fa\u3002<\/p>\n

\u56fe\u4e8c\u3001FTDT\u7535\u6c60\u7684\u7ed3\u6784\u548c\u673a\u5236<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09FTDT\u7535\u89e3\u6c60\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u78b3\u7ea4\u7ef4\u4e2d\u6c14\u4f53CO2<\/sub>\u548c\u4ea7\u54c1\u6eb6\u51fa\u5bfc\u81f4\u6c14\u6ce1\u5f62\u6210\u8fc7\u7a0b\u7684\u7167\u7247\uff1b<\/p>\n

\uff08c\uff09\u57fa\u4e8e\u540c\u6b65\u8f90\u5c04\u5149\u6e90\u7684X\u5c04\u7ebf\u65ad\u5c42\u626b\u63cf\u6210\u50cf\u6280\u672f\u8868\u5f81CF\u7684\u5185\u90e8\u7ed3\u6784\uff1b<\/p>\n

\uff08d\uff09\u6a21\u62dfCFs\u5b54\u5589\u548c\u5b54\u4f53\u4e2d\u7684CO2<\/sub>(g)\u4f53\u79ef\u5206\u6570\uff1b<\/p>\n

\uff08e\uff09\u6a21\u62df\u03b4<\/em>DL<\/sub>\u548c\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u5bf9\u4e0d\u540cCO2<\/sub>RR\u7535\u6c60CO\u751f\u6210\u7684\u4f9d\u8d56\u6027\uff1b<\/p>\n

\uff08f\uff09\u5728\u5404\u79cd\u7535\u6781\u7ed3\u6784\u4e2d\uff0c\u968f\u7740\u7535\u6d41\u5bc6\u5ea6\u4ece\u8d77\u59cb\u7535\u4f4d\u589e\u52a0\u5230\u6700\u5927\u7535\u4f4d\uff0c\u6a21\u62df\u4e86\u6269\u6563\u5c42\u4e2dCO2<\/sub>\u7684\u6d53\u5ea6\u5206\u5e03\u3002<\/p>\n

\u56fe\u4e09\u3001\u6d41\u52a8\u7ed3\u6784\u7684\u5f71\u54cd<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09\u4e0d\u540c\u6d41\u573a\u4e2d\u6269\u6563\u5c42\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b-c\uff09\u4e0d\u540c\u6d41\u573a\u4e2d\u7535\u6781\u9644\u8fd1pH\u503c\u76842D\u6a21\u62df\u5206\u5e03\uff1b<\/p>\n

\uff08d\uff09\u865a\u7ebf\u6846\u6240\u793a\u533a\u57df\u5185\u7684\u6a21\u62df\u7269\u79cd\u6d41\u5411\uff1b<\/p>\n

\uff08e\uff09\u6a21\u62df\u6269\u6563\u5c42\u4e2d\u7684\u7269\u8d28\u5206\u5e03\u3002<\/p>\n

\u56fe\u56db\u3001FTDT\u7535\u6c60\u7684\u4f18\u5316<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09EA\u4e3a100 cm2<\/sup>\u7684FTDT\u7535\u89e3\u6c60\u7167\u7247\uff1b<\/p>\n

\uff08b\uff09Ag K-\u8fb9\u7f18\u7684\u5085\u91cc\u53f6\u53d8\u6362\u6269\u5c55X\u5c04\u7ebf\u5438\u6536\u7cbe\u7ec6\u7ed3\u6784\u8c31\uff1b<\/p>\n

\uff08c-d\uff091 cm2<\/sup> FTDT\u7535\u89e3\u6c60\u4e2d\u9634\u6781\u539a\u5ea6\u548c\u7ed3\u6784\u5bf9\u7535\u6d41\u5bc6\u5ea6\u548cFECO<\/sub>\u7684\u5f71\u54cd\u3002<\/p>\n

\u56fe\u4e94\u3001FTDT\u7535\u6c60\u7684\u6027\u80fd<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a-b\uff09\u6bd4\u8f83\u4e0d\u540c\u7535\u89e3\u6c60\u7684\u7535\u6d41\u5bc6\u5ea6\u548cFECO<\/sub>\uff1b<\/p>\n

\uff08c-d\uff09\u5bf9\u4e8e\u4e09\u79cd\u4e0d\u540cEAs\u7684FTDT\u7535\u89e3\u6c60\uff1aEA=1\u30014\u548c100 cm2<\/sup>\uff0cFECO<\/sub>\u548c\u7535\u6c60\u7535\u538b\u4e0e\u7535\u6d41\u5bc6\u5ea6\u7684\u5173\u7cfb\u3002<\/p>\n

\uff08e\uff09\u4e0d\u540cEAs\u7684FTDT\u7535\u6c60\u7684\u80fd\u91cf\u6548\u7387\u3002<\/p>\n

\u56fe\u516d\u3001\u6bd4\u8f83FTDT\u7535\u6c60\u7684\u6027\u80fd\u4e0e\u5df2\u62a5\u9053\u6570\u636e\u548c\u7535\u6781\u7a33\u5b9a\u6027\u6d4b\u8bd5<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09\u4e0d\u540cEAs\u4e0bCO\u7684\u4ea7\u7387\uff1b<\/p>\n

\uff08b-d\uff09\u4e0d\u540cEAs\u7535\u89e3\u6db2\u4e2dCO\u7684\u5c40\u90e8\u7535\u6d41\uff1a1 cm2<\/sup>\u30014 cm2<\/sup>\u548c100 cm2<\/sup>\uff1b<\/p>\n

\uff08e\uff091 cm2<\/sup>\u548c100 cm2<\/sup> FTDT\u7535\u6c60\u5728\u4e0d\u540c\u7535\u6c60\u7535\u538b\u4e0b\u7684\u7535\u6781\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002<\/p>\n

\u56fe\u4e03\u3001\u78b3\u9178\u6c22\u76d0\u5728CO2<\/sub>\u4f9b\u5e94\u548c\u4f20\u8f93\u4e2d\u7684\u4f5c\u7528<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\u00a0\uff08a\uff09CO2<\/sub>RR\u4e2d\u78b3\u5faa\u73af\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u6765\u81ea\u4ea7\u751f\u7684\u6c14\u4f53CO\u548c\u6b8b\u4f59CO2<\/sub>\u7684DEMS\u4fe1\u53f7\uff0c\u4f7f\u75280.1 M H13<\/sup>CO3<\/sub>–<\/sup>\u6eb6\u6db2\u4f5c\u4e3a\u7535\u89e3\u8d28\u8fdb\u884c\u4e24\u6b65\u6d4b\u91cf\uff1b<\/p>\n

\uff08c\uff09\u5b9a\u5236AFB\u7535\u89e3\u6c60\u7684\u539f\u4f4d\u62c9\u66fc\u5149\u8c31\u3002<\/p>\n

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\n \"\"\u00a0\uff08a\uff09\u5e26\u6709\u56db\u4e2a\u6a21\u5757\u7684100 cm2<\/sup> FTDT\u7535\u5806\u7684\u7167\u7247\uff1b<\/p>\n

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\u7b2c\u4e00\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

\"\"\u6587\u56fd\u658c\u535a\u58eb\uff0c\u4e8e\u5929\u6d25\u5927\u5b66\u83b7\u5f97\u5b66\u58eb\u3001\u7855\u58eb\u5b66\u4f4d\uff0c\u5728\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u8363\u83b7\u535a\u58eb\u5b66\u4f4d\uff0c\u5bfc\u5e08\u9648\u5fe0\u4f1f\u9662\u58eb\uff0c\u6bd5\u4e1a\u540e\u5728\u9648\u9662\u58eb\u6307\u5bfc\u4e0b\u7ee7\u7eed\u8fdb\u884c\u535a\u58eb\u540e\u7814\u7a76\u3002\u6f5c\u5fc3\u505a\u80fd\u6e90\u7535\u50ac\u5316\uff0c\u96c6\u4e2d\u4e8e\u8de8\u5c3a\u5ea6\u7535\u6781\u7ed3\u6784\u4f18\u5316\u548c\u6a21\u62df\u8f85\u52a9\u8bbe\u8ba1\uff0c\u4e3b\u8981\u7528\u4e8e\u7535\u50ac\u5316CO2<\/sub>\u8fd8\u539f\u8f6c\u5316\uff0c\u7814\u7a76\u7535\u50ac\u5316\u5242\u7684\u534f\u540c\u914d\u4f4d\u8c03\u63a7\u548c\u6d41\u52a8\u7535\u89e3\u6c60\u7684\u7535\u6781\u6784\u7b51\uff0c\u4fc3\u8fdbCO2<\/sub>\u7535\u50ac\u5316\u8f6c\u5316\u53ca\u89c4\u6a21\u5e94\u7528\uff0c\u73b0\u5df2\u53d1\u8868SCI\u6536\u5f55\u8bba\u658735\u4f59\u7bc7\uff0c\u4ee5\u7b2c\u4e00\uff08\u5171\u4e00\uff09\u4f5c\u8005\u5728Nature Energy, Nature Communications, Angewandte Chemie International Edition, Journal of the American Chemical Society, Advanced Energy Materials, Chemistry of Materials\u7b49\u53d1\u8868\u8bba\u65878\u7bc7\u3002
\n \"\"\u4efb\u535a\u534e\u535a\u58eb\uff0c\u5728\u5929\u6d25\u5927\u5b66\u83b7\u5f97\u5b66\u58eb\u5b66\u4f4d\uff0c\u540e\u8fdb\u5165\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u653b\u8bfb\u535a\u58eb\u5b66\u4f4d\uff0c\u535a\u58eb\u5bfc\u5e08Eric Croiset\u6559\u6388\u548cLuis Ricardez Sandoval\u6559\u6388\uff0c\u6bd5\u4e1a\u540e\u5728\u9648\u5fe0\u4f1f\u9662\u58eb\u6307\u5bfc\u4e0b\u8fdb\u884c\u535a\u58eb\u540e\u7814\u7a76\u3002\u7533\u8bf7\u4eba\u4e00\u76f4\u4ece\u4e8b\u975e\u5747\u76f8\u50ac\u5316\u5242\u7406\u8bba\u6a21\u62df\uff08DFT\uff0c\u5fae\u52a8\u529b\u5b66\u548c\u591a\u7269\u7406\u573a\u6a21\u62df\uff09\u4e0e\u5b9e\u9a8c\u8bbe\u8ba1\u7684\u7814\u7a76\uff0c\u5e76\u5bf9\u7535\u50ac\u5316\u53cd\u5e94\u4f53\u7cfb\u7684\u8ba1\u7b97\u5efa\u6a21\u79ef\u7d2f\u4e86\u4e30\u5bcc\u7684\u7814\u7a76\u7ecf\u9a8c\uff0c\u7528\u4e8e\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\uff08CO2<\/sub>RR\uff09\u3001\u6c27\u8fd8\u539f\/\u6790\u51fa\uff08ORR\/OER\uff09\u3001\u4ee5\u53ca\u6790\u6c22\uff08HER\uff09\u529f\u80fd\u50ac\u5316\u5242\u7684\u5f00\u53d1\u7b49\u3002\u4ee5\u7b2c\u4e00\u4f5c\u8005\/\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u5728Nature Energy\u3001Nature Commun.\u3001Angew. Chem.\u3001Adv. Mater.\u3001Adv. Energy Mater.\u3001Nano Energy\u3001J. Catal.\u3001Small\u3001J. Power Sources\u7b49\u9ad8\u6c34\u5e73\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587 14\u7bc7\u3002\u5148\u540e\u83b7\u5f97\u201c\u56fd\u5bb6\u4f18\u79c0\u81ea\u8d39\u7559\u5b66\u751f\u5956\u5b66\u91d1\u201d\u3001\u201c\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u7eb3\u7c73\u6280\u672f\u7814\u7a76\u5956\u5b66\u91d1\u201d\uff08\u8fde\u7eed\u4e24\u5e74\uff09\u7b49\u4f17\u591a\u5956\u52b1\u3002<\/p>\n

\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

\"\"\u00a0\u738b\u65b0\u6559\u6388\uff1a\u534e\u5357\u5e08\u8303\u5927\u5b66\u7814\u7a76\u5458\uff0c\u5e7f\u4e1c\u7701\u6770\u51fa\u9752\u5e74<\/strong>\u3002\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u65b0\u80fd\u6e90\u6750\u6599\u4e0e\u5668\u4ef6\u3002\u4e3b\u6301\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u5e7f\u4e1c\u7701\u6770\u51fa\u9752\u5e74\u57fa\u91d1\uff0c\u5e7f\u4e1c\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u5e7f\u4e1c\u7701\u65b0\u578b\u7814\u53d1\u673a\u6784\u7b49\u9879\u76ee\uff1b\u83b7\u5f97\u6559\u80b2\u90e8\u81ea\u7136\u79d1\u5b66\u5956\u4e00\u7b49\u5956\uff1b\u7533\u8bf7\u4e13\u522966\u4ef6\uff0c\u6388\u6743\u53d1\u660e\u4e13\u522936\u4ef6\uff0c\u4ee5\u7b2c\u4e00\u4f5c\u8005\u6216\u901a\u8baf\u4f5c\u8005\u53d1\u8868\u8bba\u658790\u4f59\u7bc7\uff0c\u88ab\u5f155900\u4f59\u6b21\uff0cH-index\u6307\u657041\u3002\u76f8\u5173\u4ee3\u8868\u6027\u7814\u7a76\u6210\u679c\u4ee5\u7b2c\u4e00\u4f5c\u8005\u6216\u901a\u8baf\u4f5c\u8005\u53d1\u8868\u5728Nat. Energy, Nat. Commun., J. Am. Chem. Soc., Angew. Chem. Int. Ed., Adv. Mater., Adv. Energy Mater., Adv. Funct. Mater, Appl. Catal. B, Energy Storage Mater.\u7b49\u671f\u520a\u4e0a\u3002<\/p>\n

\"\"\u4f59\u7231\u840d\u6559\u6388\uff1a\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u6559\u6388\uff0cNSERC\u6388\u4e88\u8457\u540d\u76842020 E.W.R. Steacie\u7eaa\u5ff5\u5956<\/strong>\u3002\u62c5\u4efbChemical Engineering Journal (IF = 10.65) \u7684\u526f\u4e3b\u7f16\u3002\u7814\u7a76\u96c6\u4e2d\u5728\u80fd\u91cf\u5b58\u50a8\u548c\u8f6c\u6362\u7684\u6750\u6599\u5f00\u53d1\uff0c\u5149\u50ac\u5316\u5242\u548c\u7eb3\u7c73\u590d\u5408\u6750\u6599\u3002\u8fd1\u5e74\u6765\u53d1\u8868\u4e86160\u591a\u7bc7\u671f\u520a\u8bba\u6587\uff0c\u62e5\u6709\u4e03\u9879\u7eb3\u7c73\u6750\u6599\u6216\u5668\u4ef6\u5f00\u53d1\u7684\u4e13\u5229\uff0c\u5176\u4e2d\u4e24\u9879\u5df2\u6388\u6743\u7ed9\u516c\u53f8\uff0c\u88ab\u5f15\u7528\u8d85\u8fc725000\u6b21\uff0cH-index\u6307\u657077\u3002<\/p>\n

\"\"\u00a0\u9648\u5fe0\u4f1f\u9662\u58eb\uff1a\u52a0\u62ff\u5927\u7687\u5bb6\u79d1\u5b66\u9662\u9662\u58eb\uff0c\u52a0\u62ff\u5927\u5de5\u7a0b\u9662\u9662\u58eb<\/strong>\uff0c\u6ed1\u94c1\u5362\u5927\u5b66\u5316\u5b66\u5de5\u7a0b\u5b66\u9662\u548c\u7eb3\u7c73\u6280\u672f\u5de5\u7a0b\u4e2d\u5fc3\u6559\u6388\uff0c\u6ed1\u94c1\u5362\u5927\u5b66\u7535\u5316\u5b66\u80fd\u6e90\u4e2d\u5fc3\u4e3b\u4efb\uff0c\u5e94\u7528\u7eb3\u7c73\u6750\u6599\u4e0e\u6e05\u6d01\u80fd\u6e90\u5b9e\u9a8c\u5ba4\u4e3b\u4efb\uff0c\u52a0\u62ff\u5927\u56fd\u5bb6\u9996\u5e2d\u79d1\u5b66\u5bb6(CRC-Tier 1)\uff0c\u56fd\u9645\u7535\u5316\u5b66\u80fd\u6e90\u79d1\u5b66\u9662\uff08IAOEES\uff09\u526f\u4e3b\u5e2d\u3002\u62c5\u4efbRenewables\u4e3b\u7f16\uff08\u5165\u9009\u201c2021\u5e74\u5ea6\u4e2d\u56fd\u79d1\u6280\u671f\u520a\u5353\u8d8a\u884c\u52a8\u8ba1\u5212\u9ad8\u8d77\u70b9\u65b0\u520a\u201d\u9879\u76ee\uff09\u3001\u7f8e\u56fd\u5316\u5b66\u5b66\u4f1a\u65d7\u4e0b\u671f\u520aACS Applied Materials & Interfaces\u526f\u4e3b\u7f16\u3002\u9648\u5fe0\u4f1f\u9662\u58eb\u4eab\u6709\u6781\u9ad8\u7684\u5168\u7403\u5b66\u672f\u5f71\u54cd\u529b\uff0c\u8fde\u7eed\u591a\u5e74\u88ab\u79d1\u777f\u552f\u5b89\u8bc4\u9009\u4e3a\u201c\u9ad8\u88ab\u5f15\u5b66\u8005\u201d\uff0c\u4e5f\u662f\u52a0\u62ff\u5927\u3001\u7f8e\u56fd\u548c\u4e2d\u56fd\u7b49\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u4e0e\u6280\u672f\u7b49\u91cd\u8981\u57fa\u91d1\u8bc4\u59d4\uff0c\u591a\u6b21\u62c5\u4efb\u91cd\u8981\u56fd\u9645\u5b66\u672f\u4f1a\u8bae\u4e3b\u5e2d\uff0c\u5e76\u591a\u6b21\u505a\u7279\u9080\u5927\u4f1a\u62a5\u544a\u3002\u9648\u5fe0\u4f1f\u9662\u58eb\u5e26\u9886\u4e00\u652f\u7ea670\u4eba\u7684\u7814\u7a76\u56e2\u961f\u5e38\u5e74\u81f4\u529b\u4e8e\u71c3\u6599\u7535\u6c60\uff0c\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\uff0c\u9502\u79bb\u5b50\u7535\u6c60\uff0c\u9502\u786b\u7535\u6c60\uff0c\u9502\u7845\u7535\u6c60\uff0c\u5168\u56fa\u6001\u7535\u6c60\uff0c\u6db2\u6d41\u7535\u6c60\uff0c\u4e8c\u6c27\u5316\u78b3\u56de\u6536\u8f6c\u5316\u7b49\u50a8\u80fd\u5668\u4ef6\u548c\u80fd\u6e90\u6750\u6599\u7684\u7814\u53d1\u548c\u4ea7\u4e1a\u5316\u3002\u8fd1\u5e74\u6765\u5728Nat. Energy, Nat. Nanotech., Nat. Commun., Angew. Chem., J. Am. Chem. Soc., Adv. Mater., Energy. Environ. Sci.\u7b49\u671f\u520a\u53d1\u8868SCI\u8bba\u6587500\u4f59\u7bc7\uff0c\u88ab\u5f1548000\u4f59\u6b21\uff0cH-index\u6307\u6570110\uff0c\u53e6\u5916\uff0c\u7f16\u84573\u90e8\uff0c\u7ae0\u828211\u7ae0\uff0c\u7533\u8bf7\/\u6388\u6743\u7f8e\u56fd\u3001\u4e2d\u56fd\u548c\u56fd\u9645\u4e13\u522960\u4f59\u9879\uff0c\u591a\u9879\u6210\u679c\u5b9e\u73b0\u4ea7\u4e1a\u5316\u8f6c\u5316\u548c\u5e94\u7528\u3002<\/p>\n

\u8bfe\u9898\u7ec4\u4e3b\u9875\uff1ahttp:\/\/chemeng.uwaterloo.ca\/zchen\/.<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aContinuous CO2<\/sub> electrolysis using a CO2<\/sub> exsolution-induced flow cell<\/a><\/strong>. Nature Energy<\/em>, 2022<\/strong>, DOI: 10.1038\/s41560-022-01130-6.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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