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\/><\/p>\n<p><strong>\u56fe2<\/strong><strong>\u00a0<\/strong>\u81ea\u7531\u57fa\u8870\u8001\u5047\u8bf4\u793a\u610f\u56fe\u3002\uff08\u56fe\u7247\u6765\u6e90\u4e8e\u7f51\u7edc\uff09<\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>\u56db\u3001<\/b><\/strong><strong><b>\u81ea\u7531\u57fa\u5316\u5b66<\/b><\/strong><\/p>\n<p>\u81ea\u7531\u57fa\u5316\u5b66\u7684\u8bde\u751f\u4e3a\u5316\u5b66\u9886\u57df\u5f00\u8f9f\u4e86\u4e00\u4e2a\u91cd\u8981\u7684\u5206\u652f\uff0c\u5b83\u5b8c\u5584\u4e86\u8bb8\u591a\u5316\u5b66\u57fa\u7840\u7406\u8bba\uff0c\u4e3a\u81ea\u7531\u57fa\u53cd\u5e94\u673a\u7406\u63d0\u4f9b\u4e86\u91cd\u8981\u7684\u7406\u8bba\u652f\u6491\u3002\u7531\u4e8e\u81ea\u7531\u57fa\u7684\u7535\u5b50\u7ed3\u6784\u7684\u72ec\u7279\u6027\u4e3a\u81ea\u7531\u57fa\u53cd\u5e94\u63d0\u4f9b\u4e86\u826f\u597d\u7684\u53cd\u5e94\u6761\u4ef6\u3002<strong>\u81ea\u7531\u57fa\u53cd\u5e94<\/strong>\u6709\u5982\u4e0b\u51e0\u4e2a\u7279\u5f81\uff1a<\/p>\n<p>\uff081\uff09\u81ea\u7531\u57fa\u53cd\u5e94\u6d3b\u6027\u9ad8\uff0c\u80fd\u5792\u4f4e\uff0c\u53cd\u5e94\u901f\u7387\u5feb\uff1b<\/p>\n<p>\uff082\uff09\u81ea\u7531\u57fa\u5728\u6eb6\u6db2\u4e2d\u8fdb\u884c\u53cd\u5e94\u65f6\uff0c\u6eb6\u6db2\u7684\u9178\u6027\u3001\u78b1\u6027\u548c\u6781\u6027\u5bf9\u81ea\u7531\u57fa\u7684\u5f71\u54cd\u8f83\u5c0f\uff1b<\/p>\n<p>\uff083\uff09\u81ea\u7531\u57fa\u53cd\u5e94\u53d1\u751f\u9700\u8981\u6709\u660e\u786e\u7684\u5f15\u53d1\u5242\uff1b<\/p>\n<p>\uff084\uff09\u5bf9\u4e8e\u542b\u6709\u6d3b\u6cfc\u6c22\u7c7b\u7684\u7269\u8d28\uff08\u4f8b\u5982\uff1a\u82ef\u915a\u7c7b\u548c\u82b3\u9999\u8102\u80fa\uff09\u80fd\u591f\u4f7f\u81ea\u7531\u57fa\u7684\u53cd\u5e94\u901f\u7387\u51cf\u6162\uff0c\u751a\u81f3\u4f7f\u81ea\u7531\u57fa\u53cd\u5e94\u5b8c\u5168\u88ab\u6291\u5236<sup>[6]<\/sup>\u3002<\/p>\n<p>\u81ea\u7531\u57fa\u805a\u5408\u53cd\u5e94\u662f\u81ea\u7531\u57fa\u53cd\u5e94\u7684\u4e00\u4e2a\u91cd\u8981\u7684\u53cd\u5e94\u7c7b\u578b\uff0c\u5e7f\u6cdb\u7684\u5e94\u7528\u4e8e\u70ed\u5851\u6027\u5851\u6599\u3001\u7c98\u5408\u5242\u3001\u5305\u88c5\u3001\u6cb9\u58a8\u3001\u6d82\u6599\u3001\u7259\u79d1\u4fee\u590d\u6750\u6599\u548c3D\u6253\u5370\u7b49\u591a\u4e2a\u9886\u57df\u3002\u5728\u5178\u578b\u7684\u81ea\u7531\u57fa\u805a\u5408\u53cd\u5e94\u4e2d\uff0c\u4e00\u822c\u4f1a\u7ecf\u5386\u94fe\u5f15\u53d1\uff0c\u94fe\u589e\u957f\u548c\u94fe\u7ec8\u6b62\u4e09\u4e2a\u8fc7\u7a0b\uff08\u5982\u56fe3\uff09<sup>[7]<\/sup>\u3002\u81ea\u7531\u57fa\u901a\u5e38\u662f\u901a\u8fc7\u70ed\u5206\u89e3\u3001\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u3001\u7535\u79bb\u8f90\u5c04\u548c\u5149\u89e3\u53cd\u5e94\u5f15\u53d1\u3002\u5728\u4f53\u7cfb\u4e2d\u5f15\u53d1\u540e\uff0c\u5355\u4f53\u6216\u8005\u4f4e\u4ea4\u8054\u805a\u5408\u7269\u5e76\u5728\u53cd\u5e94\u65e9\u671f\u5f62\u6210\u8f83\u5927\u7684\u5927\u5206\u5b50\u805a\u5408\u7269\uff0c\u8fd9\u4e2a\u8fc7\u7a0b\u4e2d\u4f53\u7cfb\u662f\u653e\u70ed\u53cd\u5e94\u3002\u8fd9\u4e9b\u5927\u5206\u5b50\u805a\u5408\u7269\u4f1a\u589e\u52a0\u4f53\u7cfb\u7684\u7c98\u5ea6\uff0c\u76f4\u5230\u6750\u6599\u4ece\u7c7b\u6db2\u4f53\u76f8\u5230\u7c7b\u56fa\u4f53\u76f8\u7684\u8f6c\u53d8\uff0c\u8fd9\u79cd\u8f6c\u53d8\u4e5f\u88ab\u79f0\u4e4b\u4e3a\u51dd\u80f6\u8fc7\u7a0b\u3002\u5f53\u6d3b\u6027\u4e2d\u5fc3\u5206\u5b50\u76f8\u4e92\u78b0\u649e\u65f6\uff0c\u5bfc\u81f4\u805a\u5408\u53cd\u5e94\u505c\u6b62\u3002<\/p>\n<p><strong><b>\u00a0<img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243160\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60271718.png\" alt=\"\" width=\"551\" height=\"230\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60271718.png 551w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60271718-300x125.png 300w\" sizes=\"(max-width: 551px) 100vw, 551px\" \/><\/b><\/strong><\/p>\n<p><strong>\u56fe3<\/strong>\u00a0\u805a\u4e59\u70ef\u81ea\u7531\u57fa\u805a\u5408\u53cd\u5e94\u673a\u7406\u793a\u610f\u56fe\u3002<\/p>\n<p><strong><b>\u00a0<\/b><\/strong><\/p>\n<p>\u4e0b\u9762\u7ed9\u5927\u5bb6\u4ecb\u7ecd\u51e0\u79cd\u5173\u4e8e\u81ea\u7531\u57fa\u5728\u5316\u5b66\u4e0e\u751f\u7269\u79d1\u5b66\u4e2d\u53d1\u6325\u7684\u4f5c\u7528\uff1a<\/p>\n<p><strong><b>1\u3001\u5728\u7535\u5316\u5b66CO<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>\u8fd8\u539f\u8fc7\u7a0b\u4e2d\uff0c\u7f9f\u57fa\u81ea\u7531\u57fa\u4e3b\u5bfc\u6c27\u5316\u94dc\u7684\u518d\u6c27\u5316<\/b><\/strong><\/p>\n<p>\u901a\u8fc7\u53ef\u518d\u751f\u7535\u529b\u9a71\u52a8\u7684\u7535\u5316\u5b66CO<sub>2<\/sub>\u8fd8\u539f\u53cd\u5e94\uff08CO<sub>2<\/sub>RR\uff09\u5c06CO<sub>2<\/sub>\u8f6c\u5316\u4e3a\u9644\u52a0\u503c\u9ad8\u7684\u5316\u5b66\u54c1\u5df2\u88ab\u516c\u8ba4\u4e3a\u5b9e\u73b0\u201c\u78b3\u4e2d\u548c\u201d\u7684\u4e00\u79cd\u6709\u524d\u666f\u7684\u7b56\u7565\u3002\u6c27\u5316\u94dc\u884d\u751f\u7269\uff08OD-Cu\uff09\u5df2\u88ab\u8bc1\u660e\u662f\u4e00\u7ec4\u9ad8\u6548\u7684CO<sub>2<\/sub>RR\u7535\u50ac\u5316\u5242\uff0c\u5c24\u5176\u662f\u591a\u78b3\u4ea7\u7269\uff08C<sub>2+<\/sub>\uff09\u7684\u50ac\u5316\u5242\u3002\u7136\u800c\uff0c\u786e\u5207\u7684\u673a\u7406\u5c1a\u4e0d\u6e05\u695a\uff0c\u4eba\u4eec\u63d0\u51fa\u4e86\u4e0d\u540c\u7684\u89c2\u70b9\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u8ba1\u7b97\u5747\u8868\u660e\uff0cCu<sup>\u03b4+<\/sup>\/Cu<sup>0<\/sup>\u754c\u9762\u53ef\u4ee5\u6fc0\u6d3b\u60f0\u6027CO<sub>2<\/sub>\u5206\u5b50\uff0c\u4fc3\u8fdbCO-CO\u5076\u8054\u3002\u4e3a\u4e86\u8c03\u8282C<sub>2+<\/sub>\u4ea7\u7269\u7684\u9009\u62e9\u6027\uff0c\u901a\u8fc7\u6784\u5efa\u5404\u79cd\u6c27\u5316\u9884\u50ac\u5316\u5242\u6216\u91c7\u7528CO<sub>2<\/sub>-\u8109\u51b2\u7535\u89e3\uff0c\u83b7\u5f97\u4e86\u591a\u79cd\u5177\u6709Cu<sup>\u03b4+<\/sup>\u4f4d\u70b9\u7279\u5f81\u7684\u9ad8\u6548OD-Cu\u50ac\u5316\u5242\u3002\u4e86\u89e3OD-Cu\u5728\u5e38\u7528\u7684CO<sub>2<\/sub>\u9971\u548cKHCO<sub>3<\/sub>\u7535\u89e3\u8d28\u4e2d\u7684\u8fd8\u539f\/\u518d\u6c27\u5316\u884c\u4e3a\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\uff0c\u4f46\u5bf9\u786e\u5b9a\u6c27\u5316\u79cd\u7c7b\u81f3\u5173\u91cd\u8981\u3002\u8fd1\u65e5\uff0c<strong><b>\u7535\u5b50\u79d1\u6280\u5927\u5b66\u9686\u6636<\/b><\/strong>\u535a\u58eb\u548c<strong><b>\u5d14\u6625\u534e<\/b><\/strong>\u6559\u6388\u4ee5\u201cHydroxyl radicals dominate reoxidation of oxidederived Cu in electrochemical CO<sub>2<\/sub>\u00a0reduction\u201d\u4e3a\u9898\uff0c\u5728<em>Nat. Commun<\/em>\u4e0a\u53d1\u8868\u3002\u4f5c\u8005\u901a\u8fc7\u7535\u5b50\u987a\u78c1\u5171\u632f\u6280\u672f\uff0c\u8bc1\u5b9e\u4e86HCO<sub>3<\/sub><sup>&#8211;<\/sup>\u6eb6\u6db2\u4e2d\u5f62\u6210\u7684\u5f3a\u6c27\u5316\u6027\u7684\u7f9f\u57fa\u81ea\u7531\u57fa(OH\u2022)\u3002\u6b64\u5916\uff0c\u4ed6\u4eec\u8fd8\u7ed3\u5408\u4e86\u539f\u4f4d\u62c9\u66fc\u5149\u8c31\u3001\u4e8c\u6b21\u79bb\u5b50\u8d28\u8c31\u548c\u540c\u4f4d\u7d20\u6807\u8bb0\uff0c\u5c55\u793a\u4e86OD-Cu\u8868\u9762\u7684\u52a8\u6001\u8fd8\u539f\/\u518d\u6c27\u5316\u884c\u4e3a\uff0c\u63ed\u793a\u4e86HCO<sub>3<\/sub><sup>&#8211;<\/sup>\u548cH<sub>2<\/sub>O\u4e4b\u95f4\u7684\u5feb\u901f\u6c27\u4ea4\u6362\u4e3aOH\u2022\u81ea\u7531\u57fa\u7684\u5f62\u6210\u63d0\u4f9b\u4e86\u6c27\u6e90\uff0c\u8fde\u7eed\u751f\u6210\u4f1a\u5f15\u8d77Cu\u7535\u6781\u7684\u81ea\u53d1\u6c27\u5316\uff0c\u4ea7\u751f\u8868\u9762CuOx\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8fd9\u9879\u5de5\u4f5c\u8868\u660e\uff0c\u9634\u6781\u8fd8\u539f\u548cOH\u2022\u8bf1\u5bfc\u7684\u518d\u6c27\u5316\u4e4b\u95f4\u5b58\u5728\u201c\u8df7\u8df7\u677f\u6548\u5e94\u201d\uff0c\u51b3\u5b9a\u4e86CO2RR\u4e2dCu<sup>\u03b4+<\/sup>\u7269\u79cd\u7684\u5316\u5b66\u72b6\u6001\u548c\u542b\u91cf\u3002\u8fd9\u4e00\u53d1\u73b0\u6709\u671b\u63a8\u52a8\u4eba\u4eec\u7406\u89e3\u7535\u89e3\u8d28\u5728CO<sub>2<\/sub>RR\u4e2d\u7684\u5173\u952e\u4f5c\u7528\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243161\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60272483.png\" alt=\"\" width=\"554\" height=\"295\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60272483.png 554w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60272483-300x160.png 300w\" sizes=\"(max-width: 554px) 100vw, 554px\" \/><\/p>\n<p><strong>\u56fe4<\/strong><strong>\u00a0<\/strong>Ar\u9971\u548c\u76840.5M KHC<sup>16<\/sup>O<sub>3<\/sub>\u00a0H<sub>2<\/sub>\u00a0<sup>18<\/sup>O\u6eb6\u6db2\u4e2d\u6c27\u540c\u4f4d\u7d20\u6807\u8bb0\u6cd5\u6d4b\u5b9aOH\u2022\u6765\u6e90<sup>[8]<\/sup>\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>2\u3001\u787c\u4fc3\u8fdb\u8fc7\u6c27\u5316<\/b><\/strong><strong><b>\u5355<\/b><\/strong><strong><b>\u786b\u9178<\/b><\/strong><strong><b>\u76d0<\/b><\/strong><strong><b>\u7c7b\u82ac\u987f\u6d3b\u5316\u6c34\u51c0\u5316\u7684\u5206\u5b50\u548c\u52a8\u529b\u5b66\u7814\u7a76<\/b><\/strong><\/p>\n<p>\u00a0\u00a0\u00a0\u5728\u9ad8\u7ea7\u6c27\u5316\u8fc7\u7a0b(AOPs)\u4e2d\u4ea7\u751f\u7684\u9ad8\u6d3b\u6027\u6c27(ROS)\uff0c\u5982\u7f9f\u57fa\u81ea\u7531\u57fa(\u2022OH)\u3001\u786b\u9178\u76d0\u81ea\u7531\u57fa(SO<sub>4<\/sub><sup>\u2022-<\/sup>)\u3001\u9ad8\u4ef7\u91d1\u5c5e\u548c\u5355\u6001\u6c27\uff0c\u53ef\u4ee5\u964d\u89e3\u5927\u91cf\u6709\u673a\u6c61\u67d3\u7269\u3002\u56e0\u6b64\uff0c\u5229\u7528\u6700\u5148\u8fdb\u7684\u7b56\u7565\u6301\u7eed\u751f\u4ea7\u6d3b\u6027\u6c27\u662f\u975e\u5e38\u6709\u5229\u4e8e\u6c34\u51c0\u5316\u7684\u3002\u7136\u800c\uff0c\u8fd9\u4e9b\u5177\u6709\u660e\u663e\u6c27\u5316\u8fd8\u539f\u80fd\u529b\u548c\u53cd\u5e94\u9014\u5f84\u7684ROS\u5728\u4e0e\u6709\u673a\u6c61\u67d3\u7269\u53cd\u5e94\u65f6\u8868\u73b0\u51fa\u5e95\u7269\u7279\u5f02\u6027\u53cd\u5e94\u6d3b\u6027\u3002\u4f8b\u5982\uff0c\u2022OH\u4f1a\u901a\u8fc7\u5438\u6c22\u53cd\u5e94\u65e0\u9009\u62e9\u6027\u5730\u653b\u51fb\u6709\u673a\u6c61\u67d3\u7269\u3002\u800c\u2022OH\u53d7\u9ad8pH\u73af\u5883(pKa = 11.9)\u3001\u81ea\u731d\u706d(5.5\u00d710<sup>9<\/sup>\u00a0M<sup>-1<\/sup>\u22c5s<sup>-1<\/sup>)\u3001\u6eb6\u5242\u731d\u706d(1.8\u00d710<sup>6<\/sup>\u00a0M<sup>-1<\/sup>\u22c5s<sup>-1<\/sup>)\u4ee5\u53ca\u771f\u5b9e\u6c34\u57fa\u8d28(\u5982\u78b3\u9178\u76d0\u3001\u5364\u7d20\u3001\u5929\u7136\u6709\u673a\u7269)\u4e2d\u5171\u5b58\u7684\u80cc\u666f\u6709\u673a\/\u65e0\u673a\u7269\u7684\u6e05\u9664\uff0c\u5bfc\u81f4\u6269\u6563\u52a8\u529b\u5b66\u53d7\u9650\u3002\u6b64\u5916\uff0c\u56db\u4ef7\u94c1(Fe(IV)\uff0cFe<sup>IV<\/sup>O<sup>2+<\/sup>)\u662f\u4e00\u79cd\u9ad8\u81ea\u65cb\u6001\u3001\u5e26\u6b63\u7535\u7684\u4eb2\u7535\u7269\u79cd\uff0c\u53ef\u4ee5\u9009\u62e9\u6027\u6c27\u5316\u5bcc\u7535\u5b50\/\u63d0\u4f9b\u7535\u5b50\u7684\u6709\u673a\u7269\u3002\u867d\u7136Fe(IV)\u7684\u6c27\u5316\u7535\u4f4d(2.0 V vs SHE)\u4f4e\u4e8e\u2022OH (2.7 V vs SHE)\u548cSO<sub>4<\/sub><sup>\u2022-<\/sup>\u00a0(2.50 ~ 3.10 V vs SHE)\uff0c\u4f46Fe(IV)\u7684\u6e29\u548c\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\u8f83\u4f4e(IV)\u4fdd\u8bc1\u4e86\u6eb6\u6db2\u4e2d\u66f4\u957f\u7684\u4f20\u8d28\u5bff\u547d\uff0c\u4ee5\u653b\u51fb\u76ee\u6807\u6c61\u67d3\u7269\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u7ec4\u5408\u7684AOP\u7cfb\u7edf\u6765\u4ea7\u751f\u4e0d\u540c\u7684ROS\u53ef\u4ee5\u514b\u670d\u6bcf\u4e2a\u5355\u72ec\u6c27\u5316\u9014\u5f84\u7684\u9650\u5236\u3002\u8fd1\u65e5\uff0c<strong><b>\u56db\u5ddd\u5927\u5b66\u7684\u8d56\u6ce2\u6559\u6388<\/b><\/strong>\u548c<strong><b>\u6fb3\u5927\u5229\u4e9a\u963f\u5fb7\u83b1\u5fb7\u5927\u5b66\u6bb5\u6653\u5149<\/b><\/strong>\u6559\u6388\u5408\u4f5c\uff0c\u4ee5\u201cMolecular and kinetic insights to boron boosted Fenton-like activation of peroxymonosulfate for water decontamination\u201d\u4e3a\u9898\uff0c\u5728<em>Appl. Catal. B Environ.<\/em>\u4e0a\u53d1\u8868\u3002\u4f5c\u8005\u9009\u7528\u6676\u4f53\u787c\u7c07\u4f5c\u4e3a\u7eff\u8272\u5171\u50ac\u5316\u5242\uff0c\u4ee5\u52a0\u901fFe(III)\/PMS\uff08\u8fc7\u6c27\u5355\u786b\u9178\u76d0\uff09\u4f53\u7cfb\u4e2d\u7684\u6c27\u5316\u8fd8\u539f\u8fc7\u7a0b\u3002\u787c\u4e8c\u5341\u9762\u4f53B<sub>12<\/sub>\u5355\u5143\u4e2d\u7684\u534a\u91d1\u5c5eB-B\u952e\u5c06\u8d21\u732e\u7535\u5b50\u6765\u8fd8\u539fFe(III)\uff0c\u4ece\u800c\u542f\u52a8\u7c7b\u4f3cFenton\u7684PMS\u6d3b\u5316\uff0c\u751f\u6210\u7f9f\u57fa\u81ea\u7531\u57fa(\u2022OH)\u3001\u786b\u9178\u6839\u81ea\u7531\u57fa\uff08SO<sub>4<\/sub><sup>\u2022-<\/sup>\u00a0) \u548c\u9ad8\u4ef7Fe(IV)\u3002\u540c\u65f6\uff0c\u8868\u9762\u787c\u539f\u5b50\u53ef\u4ee5\u76f4\u63a5\u88c2\u89e3PMS\u5206\u5b50\u7684\u8fc7\u6c27\u5316\u7269O-O\u952e\uff0c\u751f\u6210\u2022OH\u3002\u81ea\u7531\u57fa\u548cFe(IV)\u7684\u8d21\u732e\u53ef\u4ee5\u901a\u8fc7Fe(III)\u7684\u5242\u91cf\u8fdb\u884c\u8c03\u8282\uff0c\u5e73\u884c\u81ea\u7531\u57fa\u548c\u975e\u81ea\u7531\u57fa\u6c27\u5316\u5c06\u80fd\u591f\u4ee5\u8f83\u9ad8\u7684PMS\u5229\u7528\u6548\u7387\u975e\u9009\u62e9\u6027\u964d\u89e3\u5404\u79cd\u6709\u673a\u6c61\u67d3\u7269\u3002\u6b64\u5916\uff0cFe(III)\u52a0\u901f\u4e86\u787c\u8868\u9762\u7684\u81ea\u6e05\u6d01\uff0c\u5e76\u786e\u4fdd\u6d3b\u6027\u4e2d\u5fc3\u7684\u6301\u7eed\u66b4\u9732\u3002\u787c\u4f1a\u81ea\u53d1\u5730\u7ecf\u5386\u9010\u6b65\u6c27\u5316\u548c\u6c34\u89e3\uff0c\u751f\u6210\u53ef\u6eb6\u6027\u4ea7\u54c1\uff0c\u800c\u4e0d\u4f1a\u4ea7\u751f\u6bd2\u7d20\u3002\u65b0\u578b\u787c\/\u94c1(III)\/PMS\u7cfb\u7edf\u514b\u670d\u4e86\u82ac\u987f\u5316\u5b66\u4e2d\u7684\u9650\u901f\u6b65\u9aa4\uff0c\u5e76\u5728\u957f\u671f\u8fd0\u884c\u4e2d\u5b9e\u73b0\u4e86\u5353\u8d8a\u7684\u6548\u7387\u548c\u7a33\u5b9a\u6027\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243162\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60273623.png\" alt=\"\" width=\"554\" height=\"306\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60273623.png 554w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60273623-300x166.png 300w\" sizes=\"(max-width: 554px) 100vw, 554px\" \/><\/p>\n<p><strong>\u56fe5<\/strong>\u00a05\u6b21\u5faa\u73af\u8bd5\u9a8c\u540e(a, b)\u539f\u59cb\u787c\u548c(c, d)\u6b8b\u7559\u787c\u7684HAADF-STEM\u56fe\u50cf\uff0c(e)\u787c\/\u94c1(III)\/PMS\u4f53\u7cfb\u7684\u673a\u7406<sup>[<\/sup><sup>9]<\/sup>\u3002<\/p>\n<p><strong><b>3\u3001<\/b><\/strong><strong><b>\u6cbb\u7597\u6027\u8d85\u58f0\u8bf1\u5bfc\u8132\u952e\u65ad\u88c2\u91ca\u653e\u751f\u7269\u529f\u80fd\u5206\u5b50<\/b><\/strong><\/p>\n<p>\u53ef\u63a7\u751f\u7269\u529f\u80fd\u5206\u5b50\u91ca\u653e\u5728\u751f\u7269\u5b66\u7814\u7a76\u4e2d\u5177\u6709\u91cd\u8981\u4f5c\u7528\u3002\u5728\u9884\u671f\u7684\u65f6\u95f4\u548c\u4f4d\u7f6e\u91ca\u653e\u611f\u5174\u8da3\u7684\u5206\u5b50\u4e0d\u4ec5\u5bf9\u7814\u7a76\u57fa\u672c\u751f\u7269\u673a\u5236\u4e0d\u53ef\u6216\u7f3a\uff0c\u800c\u4e14\u8fd8\u80fd\u51cf\u5c11\u75be\u75c5(\u5982\u764c\u75c7)\u6cbb\u7597\u4e2d\u7684\u4e0d\u826f\u5f71\u54cd\u548c\u5242\u91cf\u4f9d\u8d56\u6027\u6bd2\u6027\u3002\u4e00\u822c\u6765\u8bf4\uff0c\u4e00\u4e2a\u5178\u578b\u7684\u53ef\u6fc0\u6d3b\u751f\u7269\u529f\u80fd\u7cfb\u7edf\u7531\u56db\u4e2a\u5143\u7d20\u7ec4\u6210:\u751f\u7269\u6d3b\u6027\u5206\u5b50\u3001\u53ef\u88c2\u89e3\u8fde\u63a5\u5242\u3001\u4fdd\u62a4\u57fa\u56e2\u548c\u523a\u6fc0\u56e0\u5b50\u3002\u5f53\u751f\u7269\u6d3b\u6027\u5206\u5b50\u901a\u8fc7\u53ef\u88c2\u89e3\u952e\u4e0e\u4fdd\u62a4\u57fa\u56e2\u7ed3\u5408\u65f6\uff0c\u751f\u7269\u6d3b\u6027\u5206\u5b50\u7684\u529f\u80fd\u5c06\u88ab\u5173\u95ed\uff0c\u800c\u5728\u611f\u77e5\u5230\u7279\u5b9a\u523a\u6fc0\u540e\uff0c\u8fde\u63a5\u5b50\u5c06\u88ab\u65ad\u5f00\uff0c\u6d3b\u6027\u5206\u5b50\u91ca\u653e\uff0c\u751f\u7269\u529f\u80fd\u6062\u590d\u3002\u5728\u5404\u79cd\u53ef\u6fc0\u6d3b\u7cfb\u7edf\u4e2d\uff0c\u5149\u54cd\u5e94\u7684\u4eb2\u751f\u7269\u529f\u80fd\u5206\u5b50\u5177\u6709\u975e\u4fb5\u5165\u6027\u548c\u5b9e\u65f6\u63a7\u5236\u7684\u9ad8\u65f6\u7a7a\u5206\u8fa8\u7387\u7b49\u7a81\u51fa\u4f18\u70b9\uff0c\u5c24\u5176\u5438\u5f15\u4eba\u3002\u7136\u800c\uff0c\u5149\u672c\u8eab\u80fd\u591f\u7a7f\u900f\u7ec4\u7ec7\u7684\u80fd\u529b\u8f83\u4f4e\uff0c\u5927\u5927\u9650\u5236\u4e86\u5b83\u7684\u5b9e\u9645\u5e94\u7528\u3002\u4f5c\u4e3a\u4e00\u79cd\u66ff\u4ee3\u65b9\u6cd5\uff0c\u8d85\u58f0\u4e5f\u5177\u6709\u50cf\u5149\u4e00\u6837\u7684\u9ad8\u65f6\u7a7a\u63a7\u5236\uff0c\u7531\u4e8e\u5176\u6210\u672c\u4f4e\u5ec9\uff0c\u5df2\u88ab\u7528\u4e8e\u4e34\u5e8a\u6210\u50cf\u548c\u6cbb\u7597\u3002\u91cd\u8981\u7684\u662f\uff0c\u4e0e\u9891\u7387\u76f8\u5bf9\u5e94\uff0c\u8d85\u58f0\u6ce2\u53ef\u4ee5\u7a7f\u900f15\u5398\u7c73\u6df1\u7684\u7ec4\u7ec7\u3002\u8d85\u58f0\u6ce2\u89e6\u53d1\u7684\u7ec6\u80de\u751f\u7269\u5206\u5b50\u529f\u80fd\u8fdc\u7a0b\u63a7\u5236\u4e3a\u6211\u4eec\u7814\u7a76\u81ea\u7136\u63d0\u4f9b\u4e86\u72ec\u7279\u7684\u4f18\u52bf\u3002\u7136\u800c\uff0c\u8bbe\u8ba1\u6cbb\u7597\u6027\u8d85\u58f0\u54cd\u5e94\u529f\u80fd\u5206\u5b50\u7684\u7b56\u7565\u4ecd\u7136\u96be\u4ee5\u6349\u6478\uff0c\u8fc4\u4eca\u4e3a\u6b62\u5df2\u7ecf\u5f00\u53d1\u51fa\u4e86\u7f55\u89c1\u7684\u8d85\u58f0\u53ef\u5207\u5272\u5316\u5b66\u952e\u3002\u8fd1\u65e5\uff0c<strong><b>\u5927\u8fde\u7406\u5de5\u5927\u5b66\u5f6d\u5b5d\u519b<\/b><\/strong>\u9662\u58eb\u56e2\u961f\u4ee5\u201cUrea-Bond Scission Induced by Therapeutic Ultrasound for Biofunctional Molecule Release\u201d\u4e3a\u9898\uff0c\u5728<em>J. Am. Chem. Soc<\/em>\u4e0a\u53d1\u8868\u3002\u8be5\u56e2\u961f\u9996\u6b21\u8bc1\u660e\u4e86\u6cbb\u7597\u6027\u8d85\u58f0\uff081MHz\uff09\u8bf1\u5bfc\u8132\u952e\u65ad\u88c2\u7528\u4e8e\u836f\u7269\u91ca\u653e\u3002\u8fd9\u79cd\u8f6c\u53d8\u5df2\u88ab\u8bc1\u5b9e\u662f\u7531\u7a7a\u5316\u6ce1\u5185\u90e8\u4ea7\u751f\u7684\u7f9f\u57fa\u81ea\u7531\u57fa(\u2022OH)\u5f15\u53d1\u7684\uff0c\u7279\u522b\u662f\u5728\u7a7a\u5316\u6ce1\u5904\u2212\u6db2\u4f53\u754c\u9762\u3002\u8be5\u56e2\u961f\u8bbe\u8ba1\u4e86\u4e00\u7cfb\u5217\u57fa\u4e8e\u4e9a\u7532\u84dd\uff08MB\uff09\u7684\u542b\u8132\u952e\u524d\u836f\uff0c\u5373MBU\u3002\u7528\u4f4e\u5f3a\u5ea6\u6cbb\u7597\u8d85\u58f0\u8fdb\u884c\u8d85\u58f0\u5904\u7406\u540e\uff0c\u4e0e\u4f2f\u80fa\u76f8\u8fde\u7684\u8132\u952e\u53ef\u4ee5\u9009\u62e9\u6027\u5730\u88c2\u89e3\uff0c\u5728\u751f\u7406\u76f8\u5173\u7684\u73af\u5883\u4e2d\u91ca\u653e\u6e38\u79bbMB\uff0c\u540c\u65f6\u6062\u590d\u5438\u5149\u5ea6\u3001\u8367\u5149\u548c\u5149\u654f\u6027\u3002\u6b64\u5916\uff0c\u8fd8\u5f00\u53d1\u4e86\u4e00\u79cd\u7ecfFDA\u6279\u51c6\u7684\u542b\u8132\u952e\u7684\u70f7\u57fa\u5316\u5242(MBU-Mel)\uff0c\u6210\u529f\u5730\u5728\u6df1\u5c42\u764c\u7ec6\u80de\u4e2d\u5b9e\u73b0\u4e86\u8d85\u58f0\u89e6\u53d1\u836f\u7269\u91ca\u653e\uff0c\u663e\u793a\u4e86\u8d85\u58f0\u54cd\u5e94\u5206\u5b50\u5e73\u53f0\u5728\u751f\u7269\u6d3b\u6027\u5206\u5b50\u91ca\u653e\u65b9\u9762\u7684\u53ef\u6269\u5c55\u6027\u3002\u8fd9\u53ef\u80fd\u4e3a\u6cbb\u7597\u6027\u8d85\u58f0\u8bf1\u5bfc\u836f\u7269\u91ca\u653e\u5960\u5b9a\u4e86\u8d77\u70b9\uff0c\u4e3a\u201c\u8d85\u58f0\u836f\u7406\u5b66\u201d\u8fc8\u51fa\u4e86\u4e00\u6b65\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-243163\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60274580.png\" alt=\"\" width=\"554\" height=\"415\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60274580.png 554w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/10\/\u88ab\u8a89\u4e3a\u4e07\u6076\u4e4b\u6e90\u7684\u201c\u81ea\u7531\u57fa\u201d\u7684\u4e24\u9762\u60274580-300x225.png 300w\" sizes=\"(max-width: 554px) 100vw, 554px\" \/><\/p>\n<p><strong>\u56fe6<\/strong>\u00a0\u6cbb\u7597\u6027\u8d85\u58f0\u8bf1\u5bfc\u952e\u5206\u88c2\u91ca\u653eMB\u8fc7\u7a0b\u7684\u793a\u610f\u56fe<sup>[<\/sup><sup>10]<\/sup>\u3002<\/p>\n<p><strong>\u53c2\u8003\u6587\u732e<\/strong><\/p>\n<p>1 Cheeseman K H, Slater T F. 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Hydroxyl radicals dominate reoxidation of oxide-derived Cu in electrochemical CO<sub>2<\/sub>\u00a0reduction[J]. Nature communications, 2022, 13(1): 1-8.<\/p>\n<p>9 Zhou P, Yang Y, Ren W, et al. Molecular and kinetic insights to boron boosted Fenton-like activation of peroxymonosulfate for water decontamination[J]. Applied Catalysis B: Environmental, 2022: 121916.<\/p>\n<p>10 Tong Y, Li M, Huang H, et al. Urea-Bond Scission Induced by Therapeutic Ultrasound for Biofunctional Molecule Release[J]. Journal of the American Chemical Society, 2022,\u00a0144, 16799\u221216807.<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u4e00 \u3001\u5565\u662f\u81ea\u7531\u57fa\uff1f \u81ea\u7531\u57fa\u662f\u4e00\u79cd\u5177\u6709\u672a\u914d\u5bf9\u7535\u5b50\u7684\u5316\u5b66\u7269\u8d28\uff0c\u4e5f\u88ab\u79f0\u4e3a\u201c\u6e38\u79bb\u57fa\u201d\u3002\u901a\u5e38\u88ab\u8ba4\u4e3a\u662f\u5206\u5b50\u7684\u788e\u7247\uff0c\u5177\u6709\u975e\u5e38\u6d3b\u6cfc\u7684\u5316\u5b66\u6027\u8d28\u3002\u81ea\u7531\u57fa\u662f\u901a\u8fc7\u5149\u3001\u70ed\u7b49\u5916\u754c\u6761\u4ef6\u4e0b\u5316\u5408&#8230;<\/p>\n","protected":false},"author":35234,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[2],"tags":[],"class_list":["post-243155","post","type-post","status-publish","format-standard","hentry","category-keji"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243155"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/35234"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=243155"}],"version-history":[{"count":1,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243155\/revisions"}],"predecessor-version":[{"id":243164,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/243155\/revisions\/243164"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=243155"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=243155"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=243155"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}