{"id":242086,"date":"2022-09-11T06:41:00","date_gmt":"2022-09-10T22:41:00","guid":{"rendered":"\/\/m.iemloyee.com\/?p=242086"},"modified":"2022-09-10T20:45:50","modified_gmt":"2022-09-10T12:45:50","slug":"%e4%b8%9c%e5%8c%97%e5%b8%88%e8%8c%83%e5%a4%a7%e5%ad%a6%e7%8e%8b%e6%98%a5%e5%88%9a%ef%bc%8c%e6%9d%8e%e9%b9%bf%e8%af%be%e9%a2%98%e7%bb%84chem-sci-%ef%bc%9a%e5%88%a9%e7%94%a8%e5%9b%ba%e6%ba%b6%e5%8f%8d","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=242086","title":{"rendered":"\u4e1c\u5317\u5e08\u8303\u5927\u5b66\u738b\u6625\u521a\uff0c\u674e\u9e7f\u8bfe\u9898\u7ec4Chem. Sci.\uff1a\u5229\u7528\u56fa\u6eb6\u53cd\u5e94\u6291\u5236\u9530\u57fa\u666e\u9c81\u58eb\u84dd\u7c7b\u4f3c\u7269Jahn-Teller\u6548\u5e94"},"content":{"rendered":"<p><strong>\u5bfc\u8bfb<\/strong><\/p>\n<p>\u666e\u9c81\u58eb\u84dd\u7c7b\u4f3c\u7269\uff08PBAs\uff09\u7531\u4e8e\u5176\u62e5\u67093D\u5f00\u653e\u7684\u6846\u67b6\u5e76\u4e14\u6210\u672c\u8f83\u4f4e\u88ab\u8ba4\u4e3a\u662f\u94be\u79bb\u5b50\u7535\u6c60\uff08PIBs\uff09\u7406\u60f3\u7684\u6b63\u6781\u6750\u6599\u3002\u5728\u5404\u79cd\u7c7b\u578b\u7684PBAs\u4e2d\uff0c\u5bcc\u94be\u9530\u57faPBAs\uff08KMnHCF\uff09\u5177\u6709\u6700\u5927\u7684\u53ef\u9006\u5bb9\u91cf\u548c\u6700\u9ad8\u7684\u5de5\u4f5c\u7535\u538b\uff0c\u4ee5\u53ca\u6613\u4e8e\u5408\u6210\u548c\u5143\u7d20\u4e30\u5ea6\u5e7f\u7b49\u4f18\u70b9\uff0c\u4f7f\u5176\u6210\u4e3aPIBs\u6700\u6770\u51fa\u7684\u6b63\u6781\u6750\u6599\u4e4b\u4e00\u3002\u867d\u7136KMnHCF\u6709\u7740\u9ad8\u6bd4\u5bb9\u91cf\u548c\u9ad8\u7535\u538b\u5e73\u53f0\uff0c\u4f46\u662fKMnHCF\u7684\u5faa\u73af\u6027\u80fd\u5f88\u5dee\uff0c\u4e25\u91cd\u5730\u5236\u7ea6\u4e86\u5176\u53d1\u5c55\uff0c\u5176\u4e3b\u8981\u539f\u56e0\u5c31\u662fKMnHCF\u7684Jahn-Teller\u6548\u5e94\u3002\u5728KMnHCF\u4e2d\uff0cJahn-Teller\u6548\u5e94\u8868\u73b0\u4e3a\u56db\u4e2aMn-N\u952e\u7684\u6536\u7f29\u3002\u56e0\u4e3a[MnN<sub>6<\/sub>]<sup>3+<\/sup>\u662fJahn-Teller\u6548\u5e94\u626d\u66f2\u9020\u6210\u7684\uff0c\u800c[MnN<sub>6<\/sub>]<sup>2+<\/sup>\u4e0d\u662f\uff0c\u6240\u4ee5\u8fd9\u4e9b\u516b\u9762\u4f53\u5728\u6bcf\u6b21\u5145\u653e\u7535\u5faa\u73af\u4e2d\u90fd\u4f1a\u7ecf\u5386\u4e0d\u7a33\u5b9a\u7684\u4e0d\u5bf9\u79f0\u6536\u7f29\u548c\u81a8\u80c0\uff0c\u5bfc\u81f4\u7ed3\u6784\u9010\u6e10\u65ad\u88c2\u3002KMnHCF\u7531\u4e8eJahn-Teller\u6548\u5e94\u4ea7\u751f\u7684\u76f8\u53d8\u6240\u9020\u6210\u7684\u4f53\u79ef\u53d8\u5316\u4f1a\u5bfc\u81f4\u5bb9\u91cf\u5267\u70c8\u8870\u51cf\u3002\u56e0\u6b64\uff0c\u6291\u5236Jahn-Teller\u6548\u5e94\u4ece\u800c\u5f00\u53d1\u517c\u5177\u9ad8\u6bd4\u5bb9\u91cf\u548c\u4f18\u5f02\u5faa\u73af\u7a33\u5b9a\u6027\u7684KMnHCF\u6b63\u6781\u7535\u6781\u6750\u6599\u5b9e\u73b0\u9ad8\u6548\u80fd\u6e90\u8f6c\u6362\u6210\u4e3a\u8be5\u9886\u57df\u8feb\u5207\u9700\u8981\u653b\u514b\u7684\u96be\u9898\u4e4b\u4e00\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong>\u6210\u679c\u80cc\u666f<\/strong><\/p>\n<p>\u4e3a\u4e86\u89e3\u51b3\u8fd9\u4e00\u96be\u9898\uff0c\u4e1c\u5317\u5e08\u8303\u5927\u5b66\u738b\u6625\u521a\u6559\u6388\uff0c\u674e\u9e7f\u526f\u6559\u6388\u5728\u201cChemical Science\u201d\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201c<a href=\"https:\/\/www.x-mol.com\/paperRedirect\/1563338589552685056\">Solid-solution reaction suppresses the Jahn\u2013Teller effect of potassium manganese hexacyanoferrate in potassium-ion batteries<\/a>\u201d\u7684\u6587\u7ae0\uff0c\u4ee5PAA\u4e3a\u6a21\u677f\uff0c\u5236\u5907\u4e86\u7531\u8d85\u5c0fKMnHCF\u7eb3\u7c73\u7acb\u65b9\u4f53\u7ec4\u6210\u7684\u7a7a\u5fc3KMnHCF\u7eb3\u7c73\u7403\uff08KMnHCF-S\uff09\uff0c\u901a\u8fc7\u539f\u4f4dXRD\u9a8c\u8bc1\u4e86\u5176\u5145\u653e\u7535\u8fc7\u7a0b\u4e3a\u65e0\u76f8\u53d8\u7684\u56fa\u6eb6\u53cd\u5e94\uff0c\u4e0e\u4f20\u7edf\u76f8\u53d8\u53cd\u5e94\u7684\u5927\u5c3a\u5bf8KMnHCF\uff08KMnHCF-L\uff09\u76f8\u6bd4\uff0cKMnHCF-S\u8868\u73b0\u51fa\u66f4\u9ad8\u7684\u6bd4\u5bb9\u91cf\uff0c\u66f4\u597d\u7684\u500d\u7387\u6027\u80fd\u4ee5\u53ca\u66f4\u7a33\u5b9a\u7684\u5faa\u73af\u5bff\u547d\u3002\u5e76\u901a\u8fc7\u7b2c\u4e00\u539f\u7406\u6027\u8ba1\u7b97\u8bc1\u660e\u4e86\u56fa\u6eb6\u53cd\u5e94\u53ef\u4ee5\u6709\u6548\u5730\u6291\u5236KMnHCF\u7684Jahn-Teller\u6548\u5e94\u3002\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a\u4e1c\u5317\u5e08\u8303\u5927\u5b66\u535a\u58eb\u540e\u5218\u70b3\u6c42\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242087\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image002-1.jpg\" alt=\"\" width=\"693\" height=\"274\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image002-1.jpg 693w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image002-1-300x119.jpg 300w\" sizes=\"(max-width: 693px) 100vw, 693px\" \/> <\/p>\n<p><strong>\u5173\u952e\u521b\u65b0\u70b9<\/strong><\/p>\n<ul>\n<li>\u901a\u8fc7\u4e00\u79cd\u7b80\u4fbf\u7684\u5408\u6210\u65b9\u6cd5\u5236\u5907\u4e86\u7531\u8d85\u5c0fKMnHCF\u7eb3\u7c73\u7acb\u65b9\u4f53\uff089 nm\uff09\u7ec4\u6210\u7684\u7a7a\u5fc3KMnHCF\u7eb3\u7c73\u7403<\/li>\n<li>\u62e5\u6709\u8d85\u5c0f\u7ed3\u6784\u7684\u7a7a\u5fc3KMnHCF\u7eb3\u7c73\u7403\u5728\u5145\u653e\u7535\u8fc7\u7a0b\u4e2d\u5b9e\u73b0\u4e86\u65e0\u76f8\u53d8\u7684\u56fa\u6eb6\u53cd\u5e94\uff0c\u6253\u7834\u4f20\u7edfKMnHCF\u7684\u4e09\u76f8\u8f6c\u53d8\u7684\u76f8\u53d8\u53cd\u5e94\uff0c\u6709\u6548\u5730\u6291\u5236\u4e86KMnHCF\u7684Jahn-Teller\u6548\u5e94\u3002<\/li>\n<\/ul>\n<p>&nbsp;<\/p>\n<p>&nbsp;<\/p>\n<p><strong>\u6570\u636e\u6982\u89c8<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242088\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image004.gif\" alt=\"\" width=\"572\" height=\"306\" \/><\/p>\n<p>\u56fe1\uff1aKMnHCF-S\u7684\u5236\u5907\u8fc7\u7a0b\u6d41\u7a0b\u56fe\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242089\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image006-2.jpg\" alt=\"\" width=\"636\" height=\"627\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image006-2.jpg 636w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image006-2-300x296.jpg 300w\" sizes=\"(max-width: 636px) 100vw, 636px\" \/><\/p>\n<p>\u56fe2\uff1a\u9ad8\u5206\u8fa8\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff1a(a) PAA-K \u7eb3\u7c73\u7403\uff0c(b) PAA-K\/Mn(OH)<sub>2<\/sub>\u7eb3\u7c73\u7403\uff0c(c) KMnHCF-S, (d)\u5355\u4e2aKMnHCF-S\u7eb3\u7c73\u7403\uff0c(g)\u5355\u4e2aKMnHCF-M\u7eb3\u7c73\u7403\uff0c\u626b\u63cf\u7535\u955c\u56fe\u50cf\uff1a(e)\u5355\u4e2aKMnHCF-S \u7eb3\u7c73\u7403, (f) KMnHCF-S\uff0c(h)\u5355\u4e2aKMnHCF-M \u7eb3\u7c73\u7403\uff0c(i) KMnHCF-M\u3002\u5355\u4e2aKMnHCF-S\u7eb3\u7c73\u7403\u7684\u5143\u7d20\u9762\u626b\u63cf\u56fe\u50cf\uff1a(j)\u9ad8\u5206\u8fa8\u900f\u5c04\u7535\u955c\u56fe\u50cf\u548c\u5bf9\u5e94\u7684\u5143\u7d20K\uff0cMn\uff0cFe\uff0cC\uff0cN\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242090\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image008-2.jpg\" alt=\"\" width=\"585\" height=\"237\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image008-2.jpg 585w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image008-2-300x122.jpg 300w\" sizes=\"(max-width: 585px) 100vw, 585px\" \/><\/p>\n<p>\u56fe3\uff1a\u4e0d\u540c\u53cd\u5e94\u65f6\u95f4\u7684KMnHCF-S\uff08a\uff09\u626b\u63cf\u7535\u955c\u56fe\u50cf\u548c\uff08b\uff09\u900f\u5c04\u7535\u955c\u56fe\u50cf\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242091\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image010-2.jpg\" alt=\"\" width=\"681\" height=\"352\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image010-2.jpg 681w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image010-2-300x155.jpg 300w\" sizes=\"(max-width: 681px) 100vw, 681px\" \/><\/p>\n<p>\u56fe4\uff1aKMnHCF-S\u7684\uff08a\uff09XRD\u7cbe\u4fee\u56fe\u8c31\u548c\uff08b\uff09\u6676\u4f53\u7ed3\u6784\u793a\u610f\u56fe\u3002KMnHCF-S\uff0cKMnHCF-M\u548cKMnHCF-L\u7684\uff08c\uff09\u62c9\u66fc\u56fe\u8c31\u548c\uff08d\uff09XPS\u5149\u8c31\u3002KMnHCF-S\u7684XPS\uff08e\uff09Mn 2p\u548c\uff08f\uff09Fe 2p\u62df\u5408\u8c31\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242092\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image012-2.jpg\" alt=\"\" width=\"692\" height=\"508\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image012-2.jpg 692w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image012-2-300x220.jpg 300w\" sizes=\"(max-width: 692px) 100vw, 692px\" \/><\/p>\n<p>\u56fe5\uff1a\uff08a\uff09KMnHCF-S\u57280.1 mV s<sup>-1<\/sup>\u7684\u626b\u901f\u4e0b\u7684CV\u66f2\u7ebf\u3002\uff08b\uff09KMnHCF-S\uff0cKMnHCF-M\u548cKMnHCF-L\u57280.02 A g<sup>-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002\uff08c\uff09KMnHCF-S\u4ece0.02\u52303 A g<sup>-1<\/sup>\u4e0b\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002\uff08d\uff09KMnHCF-S\u7684\u500d\u7387\u6027\u80fd\u56fe\u3002\uff08e\uff09\u4e09\u79cd\u6837\u54c1\u57280.05 A g<sup>-1<\/sup>\u4e0b\u5faa\u73af200\u5708\u3002\uff08f\uff09KMnHCF-S\u57280.05 A g<sup>-1<\/sup>\u4e0b\u5faa\u73af\u4e0d\u540c\u5708\u6570\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002\uff08g\uff09\u4e09\u79cd\u6837\u54c1\u57280.1 A g<sup>-1<\/sup>\u4e0b\u957f\u5faa\u73af1000\u5708\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242093\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image014-2.jpg\" alt=\"\" width=\"659\" height=\"746\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image014-2.jpg 659w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image014-2-265x300.jpg 265w\" sizes=\"(max-width: 659px) 100vw, 659px\" \/><\/p>\n<p>\u56fe6\uff1a\uff08a\uff0cb\uff09KMnHCF-S\u548c\uff08c\uff0cd\uff09KMnHCF-L\u57280.02 A g<sup>-1<\/sup>\u7535\u538b\u57282.0\u548c4.5 V\u4e4b\u95f4\u7684\u539f\u4f4dXRD\u56fe\u8c31\u3002\uff08e\uff09\u56fa\u6eb6\u53cd\u5e94\u548c\u76f8\u53d8\u4e4b\u95f4\u5dee\u5f02\u7684\u673a\u7406\u56fe\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242094\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image016.gif\" alt=\"\" width=\"692\" height=\"592\" \/><\/p>\n<p>\u56fe7\uff1a\uff08a\uff09Mn-N\u952e\u53d8\u5316\u7684\u7406\u8bba\u9884\u6d4b\u548c\uff08b\uff09\u901a\u8fc7\u8ba1\u7b97\u5f97\u5230\u7684\u56fa\u6eb6\u53cd\u5e94\u548c\u76f8\u53d8\u53cd\u5e94\u65f6\u53cd\u5e94\u80fd\u91cf\u548c\u76f8\u5bf9\u4f53\u79ef\u53d8\u5316\u3002\uff08c\uff09\u56fa\u6eb6\u53cd\u5e94\u548c\uff08d\uff09\u76f8\u53d8\u53cd\u5e94\u7684Mn<sup>2+<\/sup>\u548cMn<sup>3+<\/sup>\u7535\u5b50\u6784\u578b\u4ee5\u53caJahn-Teller\u7578\u53d8\u7684\u53ef\u89c6\u5316\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-242095\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image018-1.jpg\" alt=\"\" width=\"672\" height=\"483\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image018-1.jpg 672w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/09\/image018-1-300x216.jpg 300w\" sizes=\"(max-width: 672px) 100vw, 672px\" 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