{"id":242068,"date":"2022-09-11T06:33:13","date_gmt":"2022-09-10T22:33:13","guid":{"rendered":"\/\/m.iemloyee.com\/?p=242068"},"modified":"2022-09-10T21:33:35","modified_gmt":"2022-09-10T13:33:35","slug":"%e8%b0%a2%e5%92%8c%e5%b9%b3%e5%80%aa%e8%90%8c%e9%82%b5%e5%ae%97%e5%b9%b3%ef%bc%8c%e6%9c%80%e6%96%b0nature-energy%ef%bc%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=242068","title":{"rendered":"\u8c22\u548c\u5e73&\u502a\u840c&\u90b5\u5b97\u5e73\uff0c\u6700\u65b0Nature Energy\uff01"},"content":{"rendered":"

\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fa\u4f53\u6c27\u5316\u7269\u71c3\u6599\u7535\u6c60\uff08solid oxide fuel cell, SOFC\uff09\u4f5c\u4e3a\u7eff\u8272\u7535\u5316\u5b66\u5668\u4ef6\u7684\u4ee3\u8868\uff0c\u56e0\u5176\u9ad8\u80fd\u6548\u3001\u4f4e\u6392\u653e\u548c\u71c3\u6599\u7075\u6d3b\u6027\u800c\u5907\u53d7\u5173\u6ce8\u3002\u7136\u800c\uff0c\u9676\u74f7\u71c3\u6599\u7535\u6c60\u6280\u672f\u5546\u4e1a\u5316\u7531\u4e8e\u5176\u9ad8\u5de5\u4f5c\u6e29\u5ea6\uff08800-1000 \u00b0C\uff09\u800c\u53d7\u5230\u5f88\u5927\u963b\u788d\uff0c\u5728\u8be5\u6e29\u5ea6\u4e0b\u5bc6\u5c01\u96be\u3001\u8fd0\u8425\u6210\u672c\u9ad8\u548c\u6750\u6599\u964d\u89e3\u52a0\u901f\u3002\u5728\u4fdd\u6301\u8db3\u591f\u529f\u7387\u8f93\u51fa\u4e0b\uff0c\u540c\u65f6\u964d\u4f4e\u5de5\u4f5c\u6e29\u5ea6\u662f\u5b9e\u73b0\u5176\u66f4\u5e7f\u6cdb\u5e94\u7528\u548c\u4fbf\u643a\u6027\u7684\u5173\u952e\u4e00\u6b65\u3002\u5728\u7406\u8bba\u4e0a\uff0c\u4f53\u76f8\u6c27p-\u5e26\u4e2d\u5fc3\u3001\u4f53\u76f8\u6c27\u7a7a\u4f4d\u5f62\u6210\u80fd\u548c\u7535\u8377\u8f6c\u79fb\u80fd\u4e0e\u5404\u79cd\u6761\u4ef6\u4e0b\u6c27\u8fd8\u539f\/\u6790\u51fa\u53cd\u5e94\uff08ORR\/OER\uff09\u7684\u50ac\u5316\u6d3b\u6027\u5bc6\u5207\u76f8\u5173\u3002\u9ad8\u901a\u91cf\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u65b9\u6cd5\u4e25\u91cd\u4f9d\u8d56\u4e8e\u4e0d\u53ef\u6216\u7f3a\u7684\u590d\u6742\u8ba1\u7b97\u6a21\u62df\u65b9\u6cd5\uff0c\u5176\u9700\u8981\u8017\u65f6\u3001\u6602\u8d35\u7684\u6a21\u62df\u548c\u8ba1\u7b97\u8fc7\u7a0b\uff0c\u56e0\u6b64\u5f71\u54cd\u7b5b\u9009\u6548\u7387\u7684\u5173\u952e\u5236\u7ea6\u56e0\u7d20\u4ecd\u7136\u5b58\u5728\u3002SOFC\u9634\u6781\u5df2\u53d1\u8868\u4e86\u5927\u91cf\u5b9e\u9a8c\u6570\u636e\uff0c\u503c\u5f97\u6536\u96c6\u3001\u6574\u7406\u548c\u4f5c\u4e3a\u884d\u751f\u65b0\u7535\u6781\u5019\u9009\u8005\u7684\u57fa\u77f3\u3002\u7136\u800c\uff0c\u76ee\u524d\u7f3a\u4e4f\u51c6\u786e\u53cd\u6620\u9ad8\u6e29\u4e0bORR\u8fc7\u7a0b\u673a\u7406\u7684\u5177\u6709\u4ee3\u8868\u6027\u7684\u7269\u7406\u63cf\u8ff0\u7b26\u3002\u56e0\u6b64\uff0c\u5fc5\u987b\u5bfb\u627e\u6709\u6548\u7684\u7269\u7406\u63cf\u8ff0\u7b26\uff0c\u660e\u786eORR\u52a8\u529b\u5b66\u7684\u63a7\u5236\u89c4\u5219\uff0c\u5e76\u786e\u5b9a\u7528\u4e8e\u6570\u636e\u6316\u6398\u548c\u91cd\u6784\u7684\u53ef\u9760\u6027\u56de\u5f52\u6a21\u578b\u3002<\/p>\n

\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6df1\u5733\u5927\u5b66\/\u56db\u5ddd\u5927\u5b66\u8c22\u548c\u5e73\u9662\u58eb\u3001\u9999\u6e2f\u7406\u5de5\u5927\u5b66\u502a\u840c\u6559\u6388\u548c\u5357\u4eac\u5de5\u4e1a\u5927\u5b66\u90b5\u5b97\u5e73\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u7ecf\u8fc7\u5b9e\u9a8c\u9a8c\u8bc1\u7684\u673a\u5668\u5b66\u4e60\u9a71\u52a8\u65b9\u6cd5\uff0c\u4ee5\u52a0\u901f\u53d1\u73b0\u6709\u6548\u7684\u6c27\u8fd8\u539f\u7535\u6781\uff0c\u5176\u4e2d\u5f15\u5165\u4e86\u79bb\u5b50\u8def\u6613\u65af\u9178\uff08ionic Lewis acid, ISA\uff09\u5f3a\u5ea6\u4f5c\u4e3a\u9499\u949b\u77ff\u6c27\u5316\u7269\u6c27\u8fd8\u539f\u53cd\u5e94\uff08ORR\uff09\u6d3b\u6027\u7684\u6709\u6548\u7269\u7406\u63cf\u8ff0\u7b26\u3002\u4e3a\u4e86\u9a8c\u8bc1\u9884\u6d4b\uff0c\u4f5c\u8005\u5408\u6210\u4e86\u4ece6871\u79cd\u4e0d\u540c\u6210\u5206\u4e2d\u7b5b\u9009\u51fa\u6765\u7684\u56db\u79cd\u9499\u949b\u77ff\u6c27\u5316\u7269\uff0c\u5e76\u8fdb\u4e00\u6b65\u8fdb\u884c\u8868\u5f81\u548c\u7535\u5316\u5b66\u6d4b\u8bd5\u3002\u7279\u522b\u662fSr0.9<\/sub>Cs0.1<\/sub>Co0.9<\/sub>Nb0.1<\/sub>O3<\/sub>\uff08SCCN\uff09\u8868\u73b0\u51fa\u4f18\u5f02\u7684ORR\u6d3b\u6027\uff0c\u4ee5\u53ca\u6781\u4f4e\u7684\u6bd4\u7535\u963b\uff08area-specific resistance, ASR\uff09\u3002\u901a\u8fc7\u964d\u4f4eA\u4f4d\u70b9ISA\u548c\u589e\u52a0B\u4f4d\u70b9ISA\uff0c\u5b9e\u73b0\u4e86\u63d0\u5347\u7684\u8868\u9762\u4ea4\u6362\u52a8\u529b\u5b66\u901f\u7387\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u8ba1\u7b97\u8868\u660e\uff0cISA\u7684\u6781\u5316\u5206\u5e03\u4e0e\u6700\u4f73\u7ed3\u6784\u6709\u5173\uff0c\u7531\u4e8e\u7535\u5b50\u5bf9\u7684\u504f\u79fb\uff0c\u6c27\u7a7a\u4f4d\uff08VO\uff09\u5f62\u6210\u80fd\u548c\u8fc1\u79fb\u52bf\u5792\u964d\u4f4e\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cA combined ionic Lewis acid descriptor and machine-earning approach to prediction of efficient oxygen reduction electrodes for ceramic fuel cells<\/strong>\u201d\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Energy<\/em>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u3010\u6838\u5fc3\u521b\u65b0\u3011<\/strong><\/p>\n

\u5c06\u673a\u5668\u5b66\u4e60\u3001\u7406\u8bba\u8ba1\u7b97\u4e0e\u9676\u74f7\u56fa\u4f53\u6c27\u5316\u7269\u5f00\u53d1\u76f8\u7ed3\u5408\uff0c\u5f00\u53d1\u4e86\u4e00\u4e2a\u7ecf\u8fc7\u5b9e\u9a8c\u9a8c\u8bc1\u7684\u9634\u6781\u6750\u6599\u673a\u5668\u5b66\u4e60\u7b5b\u9009\u6280\u672f\uff0c\u5b9e\u73b0\u4e86\u5feb\u901f\u3001\u6709\u6548\u7684\u4ece\u5e9e\u5927\u7684\u9499\u949b\u77ff\u7ec4\u5206\u4e2d\u7b5b\u9009\u9ad8\u6d3b\u6027\u56fa\u4f53\u6c27\u5316\u7269\u71c3\u6599\u7535\u6c60\u9634\u6781\u6750\u6599\uff0c\u9610\u660e\u4e86\u9499\u949b\u77ff\u6c27\u5316\u7269\u8def\u6613\u65af\u9178\u6027\u8c03\u63a7\u7b56\u7565\u63d0\u5347\u672c\u5f81\u6d3b\u6027\u673a\u7406\u3002<\/p>\n

\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u6574\u4f53\u5de5\u4f5c\u6d41\u7a0b\u56fe<\/strong>\u00a92022 Springer Nature Limited<\/p>\n

\"\"<\/p>\n

\u56fe\u4e8c\u3001\u6a21\u578b\u8bc4\u4f30\u548c\u63cf\u8ff0\u7b26\u91cd\u8981\u5ea6\u5206\u6790<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a\uff09\u4e00\u7cfb\u5217\u9634\u6781\u6750\u6599\u5728700 \u00b0C\u4e0b\u6781\u5316\u7535\u963b\u7684\u5b9e\u9a8c\u6d4b\u91cf\u503c\u4e0e\u9884\u6d4b\u503c\uff1b<\/p>\n

\uff08b-c\uff09\u57fa\u4e8eANN\u6a21\u578b\u654f\u611f\u6027\u5206\u6790\u7684\u79bb\u5b50\u63cf\u8ff0\u7b26\u7684\u7279\u5f81\u91cd\u8981\u6027\u548c\u7279\u5f81\u7ec4\u5408\u91cd\u8981\u6027\uff08FCI\uff09\uff1b<\/p>\n

\uff08d-g\uff09\u4e0e\u5185\u5728ORR\u6d3b\u6027\uff08log-10(ASR)\uff09\u8d8b\u52bf\u7684\u76f8\u5173\u6027\uff0c\u4f5c\u4e3aAISA\u548cBISA\u3001R<\/em>A<\/sub>\u548cR<\/em>B<\/sub>\u3001AISA\u2009+\u2009BISA\u548cR<\/em>A<\/sub>\u2009+\u2009R<\/em>B<\/sub>\u7684\u51fd\u6570\u3002<\/p>\n

\u56fe\u4e09\u3001\u5408\u6210\u9499\u949b\u77ff\u6c27\u5316\u7269\u6837\u54c1\u7684\u7ed3\u6784\u548c\u7535\u5316\u5b66\u6027\u80fd<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a-b\uff09SCCN\u3001BSCCFM\u3001BSCFN\u548cSPBCFN\u7684XRD\u56fe\u8c31\u53caASR\u503c\u7684Arrhenius\u56fe\uff1b<\/p>\n

\uff08c\uff09\u57fa\u4e8eSDC\u7684\u5bf9\u79f0\u7535\u6c60\u4e2d\uff0cSCCN\u9634\u6781\u7684Nyquist\u56fe\uff1b<\/p>\n

\uff08d\uff09\u5728450-700 \u00b0C\u4e0b\uff0cSCCN\u9634\u6781\u7684\u5f1b\u8c6b\u65f6\u95f4\u5206\u5e03\u5206\u6790\uff1b<\/p>\n

\uff08e\uff09SCCN\u3001BSCCFM\u3001BSCFN\u548cSPBCFN\u9634\u6781\u5728500\u2009 \u00b0C\u548c550 \u2009\u00b0C\u4e0b\u7684\u5f1b\u8c6b\u65f6\u95f4\u5206\u5e03\u5206\u6790\uff1b<\/p>\n

\uff08f\uff09\u6bd4\u8f83SCCN\u3001BSCCFM\u3001BSCFN\u548cSPBCFN\u7684RHF\u548cRIF\u503c\uff0c\u5176\u4e2dCPE\u8868\u793a\u6052\u5b9a\u76f8\u4f4d\u5143\u4ef6\u3002<\/p>\n

\u56fe\u56db\u3001\u57fa\u4e8eSCCN\u9634\u6781\u7684\u5bf9\u79f0\u7535\u6c60\u7a33\u5b9a\u6027\u548c\u5355\u7535\u6c60\u6027\u80fd<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a\uff09\u5728550 \u00b0C\u7a7a\u6c14\u4e2d\u6d4b\u91cf\u7684\u5bf9\u79f0\u7535\u6c60SCCN\u7684ASR\u503c\uff1b<\/p>\n

\uff08b\uff09\u5177\u6709Ni\u2009+\u2009SDC|SDC|SCCN\u6784\u578b\u7684\u5355\u7535\u6c60\u5728450-650 \u00b0C\u4e0b\u7684I-V-P\u66f2\u7ebf\uff1b<\/p>\n

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\u56fe\u4e94\u3001BSCCFM\u7684\u5f62\u6001<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a\uff09BSCCFM\u7684\u626b\u63cf\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff1b<\/p>\n

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\u56fe\u516d\u3001\u6c27-\u8f6c\u79fb\u76f8\u5173\u7684\u8868\u5f81<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a\uff09BSCF73\u548cBSCCFM\u7684X\u5c04\u7ebf\u884d\u5c04\u56fe\uff1b<\/p>\n

\uff08b\uff09BSCCFM\u5728600 \u00b0C\u4e0b\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31\uff1b<\/p>\n

\uff08c\uff09BSCCFM\u548cBSCF73\u5728600\u2009 \u00b0C\u4e0bASR\u4e0e\u6c27\u5206\u538b\u7684\u5173\u7cfb\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09BSCCFM\u548cBSCF73\u7684O 1s XPS\u66f2\u7ebf\u7684\u53cd\u5377\u79ef\uff1b<\/p>\n

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\uff08f\uff09BSCCFM\u548cBSCF73\u7684\u7535\u5b50\u7535\u5bfc\u7387\uff1b<\/p>\n

\uff08g\uff09\u5341\u4e8c\u914d\u4f4d\u7684Cs+<\/sup>\u3001Ba2+<\/sup>\u3001Sr2+<\/sup>\u9633\u79bb\u5b50\u548c\u516d\u914d\u4f4d\u7684Co3+<\/sup>\u3001Co4+<\/sup>\u3001Fe3+<\/sup>\u3001Fe4+<\/sup>\u3001Mo6+<\/sup>\u9633\u79bb\u5b50\u7684\u8def\u6613\u65af\u9178\u5f3a\u5ea6\uff1b<\/p>\n

\uff08h\uff09BSCCFM\u4e2d\u6c27\u7a7a\u4f4d\u5f62\u6210\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e03\u3001\u7535\u5b50\u7ed3\u6784\u6f14\u5316\u7684DFT\u8ba1\u7b97<\/strong>\u00a92022 Springer Nature Limited
\n \"\"\uff08a-b\uff09BSCCFM-m\u7684\u6a21\u578b\u548c\u5dee\u5206\u7535\u8377\u5bc6\u5ea6\uff1b<\/p>\n

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\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aA combined ionic Lewis acid descriptor and machine-learning approach to prediction of efficient oxygen reduction electrodes for ceramic fuel cells<\/a><\/strong>. Nature Energy<\/em>, 2022<\/strong>, DOI: 10.1038\/s41560-022-01098-3.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1\uff1atougao@cailiaoren.com.<\/p>\n

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\u3010\u5bfc\u8bfb\u3011 \u56fa\u4f53\u6c27\u5316\u7269\u71c3\u6599\u7535\u6c60\uff08solid oxide fuel cell, SOFC\uff09\u4f5c\u4e3a\u7eff\u8272\u7535\u5316\u5b66\u5668\u4ef6\u7684\u4ee3\u8868\uff0c\u56e0\u5176\u9ad8\u80fd\u6548\u3001\u4f4e\u6392\u653e\u548c\u71c3\u6599\u7075\u6d3b\u6027\u800c\u5907\u53d7\u5173\u6ce8\u3002\u7136\u800c\uff0c…<\/p>\n","protected":false},"author":7770,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215,2],"tags":[],"class_list":["post-242068","post","type-post","status-publish","format-standard","hentry","category-jiedu","category-keji"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/242068"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/7770"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=242068"}],"version-history":[{"count":2,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/242068\/revisions"}],"predecessor-version":[{"id":242097,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/242068\/revisions\/242097"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=242068"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=242068"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=242068"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}