{"id":236860,"date":"2022-05-12T14:39:23","date_gmt":"2022-05-12T06:39:23","guid":{"rendered":"\/\/m.iemloyee.com\/?p=236860"},"modified":"2022-05-12T14:39:30","modified_gmt":"2022-05-12T06:39:30","slug":"%e3%80%90%e5%b7%b2%e5%ae%a1%e3%80%91%e7%86%8a%e6%99%96%e6%9c%80%e6%96%b0nm%ef%bc%9a%e7%94%a8%e4%ba%8e%e9%94%82%e7%a6%bb%e5%ad%90%e7%94%b5%e6%b1%a0%e7%9a%84%e6%b0%a7%e5%8c%96%e9%93%8c%e7%94%b5%e6%9e%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=236860","title":{"rendered":"\u718a\u6656\u6700\u65b0NM\uff1a\u7528\u4e8e\u9502\u79bb\u5b50\u7535\u6c60\u7684\u6c27\u5316\u94cc\u7535\u6781\u4e2d\u7535\u5316\u5b66\u8bf1\u5bfc\u7684\u65e0\u5b9a\u5f62\u5230\u5ca9\u76d0\u76f8\u53d8"},"content":{"rendered":"<p style=\"text-align: center;\">\u00a0<\/p>\n<p style=\"text-align: center;\"><strong><b>\u00a0\u4e00\u3001[\u5bfc\u8bfb]<\/b><\/strong><\/p>\n<p><strong><span style=\"color: #003366;\">\u63d2\u5c42\u578b\u91d1\u5c5e\u6c27\u5316\u7269<\/span><\/strong>\u7531\u4e8e\u5728\u4f4e\u7535\u538b\u4e0b\u9540\u9502\u7684\u5371\u9669\u6027\u964d\u4f4e\uff0c\u662f\u5b89\u5168\u53ef\u5145\u9502\u79bb\u5b50\u7535\u6c60\u6781\u6709\u524d\u9014\u7684\u8d1f\u6781\u6750\u6599\u3002\u7136\u800c\uff0c\u5176\u8f83\u4f4e\u7684\u80fd\u91cf\u548c\u529f\u7387\u5bc6\u5ea6\u4ee5\u53ca\u5faa\u73af\u4e0d\u7a33\u5b9a\u6027\u4ecd\u7136\u662f\u5236\u7ea6\u5176\u53d1\u5c55\u7684\u74f6\u9888\uff0c\u5c24\u5176\u662f\u5bf9\u4e8e\u5feb\u901f\u5145\u653e\u7535\u8fc7\u7a0b\u3002<\/p>\n<p><strong><b>\u00a0<\/b><\/strong><\/p>\n<p style=\"text-align: center;\"><strong><b>\u4e8c\u3001[\u6210\u679c\u63a0\u5f71]<\/b><\/strong><\/p>\n<p><strong><b>\u7f8e\u56fd\u535a\u4f0a\u897f\u5dde\u7acb\u5927\u5b66<\/b><\/strong><strong><b>\u718a\u6656<\/b><\/strong><strong><b>\u4e0e\u7f8e\u56fd\u52a0\u5dde\u5927\u5b66\u5723\u5730\u4e9a\u54e5\u5206\u6821Shyue Ping Ong\u8bfe\u9898\u7ec4\u5408\u4f5c\uff0c\u62a5\u544a\u4e86\u4e00\u79cd\u7eb3\u7c73\u7ed3\u6784\u7684\u5ca9\u76d0Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\uff0c\u8be5\u7535\u6781\u662f\u5728\u4e0eLi+\u91cd\u590d\u7535\u5316\u5b66\u5faa\u73af\u8fc7\u7a0b\u4e2d\u901a\u8fc7\u975e\u6676\u5411\u6676\u4f53\u7684\u8f6c\u53d8\u800c\u5f62\u6210\u7684\u3002<\/b><\/strong>\u8be5\u7535\u6781\u6bcfNb<sub>2<\/sub>O<sub>5<\/sub>\u53ef\u4ee5\u53ef\u9006\u5faa\u73af\u4e09\u4e2a\u9502\uff0c\u572820 mA g<sup>-1<\/sup>\u65f6\u5177\u6709269 mAh g<sup>-1<\/sup>\u7684\u53ef\u9006\u5bb9\u91cf\uff0c\u5e76\u57281\u2009A\u2009g<sup>-1<\/sup>\u7684\u9ad8\u500d\u7387\u4e0b\u80fd\u91cf\u5bc6\u5ea6\u9ad8\u8fbe191\u2009mAh\u2009g<sup>-1<\/sup>\u3002\u5728200 mA g<sup>-1<\/sup>\u4e0b\u5faa\u73af400\u6b21\uff0c\u5bb9\u91cf\u4e3a225 mAh g<sup>-1<\/sup>\uff0c\u5e93\u4ed1\u6548\u7387\u9ad8\u8fbe99.93%\u3002\u672c\u5de5\u4f5c\u5c06\u589e\u5f3a\u7684\u6027\u80fd\u5f52\u56e0\u4e8e\u7acb\u65b9\u5ca9\u76d0\u6846\u67b6\uff0c\u5b83\u4fc3\u8fdb\u4e86\u4f4e\u80fd\u8fc1\u79fb\u8def\u5f84\u3002\u672c\u5de5\u4f5c\u8868\u660e\uff0c\u901a\u8fc7\u7535\u5316\u5b66\u5faa\u73af\u8bf1\u5bfc\u975e\u6676\u6001\u7eb3\u7c73\u6750\u6599\u7684\u6676\u5316\u662f\u521b\u9020\u975e\u5e38\u89c4\u9ad8\u6027\u80fd\u91d1\u5c5e\u6c27\u5316\u7269\u7535\u6781\u6750\u6599\u7684\u4e00\u4e2a\u5f88\u6709\u524d\u666f\u7684\u9014\u5f84\u3002\u76f8\u5173\u8bba\u6587\u4ee5\u9898\u4e3a\uff1a\u201c<strong><em><i>Electrochemically induced amorphous-to-rock-salt phase transformation in niobium oxide electrode for Li-ion batteries<\/i><\/em><\/strong>\u201d\u53d1\u8868\u5728<strong><em><i>Nature Materials<\/i><\/em><\/strong>\u4e0a\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-236861\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72471-4.png\" alt=\"\" width=\"753\" height=\"452\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72471-4.png 753w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72471-4-300x180.png 300w\" sizes=\"(max-width: 753px) 100vw, 753px\" \/><\/p>\n<p>&nbsp;<\/p>\n<p style=\"text-align: center;\"><strong><b>\u4e09\u3001[\u6838\u5fc3\u521b\u65b0\u70b9]<\/b><\/strong><\/p>\n<ul>\n<li><b><\/b><strong><b>\u4e00\u79cd<\/b><\/strong><strong><b>\u72ec\u7279\u7684\u6c27\u5316\u94cc\u7535\u6781\uff0c\u5176\u53ef\u4ee5\u901a\u8fc7Li<\/b><\/strong><strong><sup><b>+<\/b><\/sup><\/strong><strong><b>\u91cd\u590d\u7535\u5316\u5b66\u5faa\u73af\u671f\u95f4\u7531\u65e0\u5b9a\u5f62\u5230\u6676\u4f53\u7684\u8f6c\u53d8\u83b7\u5f97<\/b><\/strong>\u3002<\/li>\n<li>\u5f53\u7ec4\u6210\u7535\u6c60\u65f6\uff0c\u8be5\u7535\u6781\u5177\u6709\u4f18\u79c0\u7684\u53ef\u9006\u5bb9\u91cf\u548c\u5faa\u73af\u7a33\u5b9a\u6027\uff0c\u8fd9\u53ef\u4ee5\u5f52\u56e0\u4e8e\u8be5\u7535\u6781\u7684\u7acb\u65b9\u5ca9\u76d0\u6846\u67b6\uff0c\u5b83\u4fc3\u8fdb\u4e86\u4f4e\u80fd\u8fc1\u79fb\u8def\u5f84\u3002<\/li>\n<li><b><\/b><strong><b>\u672c\u5de5\u4f5c<\/b><\/strong><strong><b>\u63d0\u51fa<\/b><\/strong><strong><b>\uff0c\u901a\u8fc7\u7535\u5316\u5b66\u5faa\u73af\u8bf1\u5bfc\u975e\u6676\u6001\u7eb3\u7c73\u6750\u6599\u7684\u6676\u5316\u662f\u521b\u9020\u975e\u5e38\u89c4\u9ad8\u6027\u80fd\u91d1\u5c5e\u6c27\u5316\u7269\u7535\u6781\u6750\u6599\u7684\u4e00\u4e2a\u5f88\u6709\u524d\u666f\u7684\u9014\u5f84<\/b><\/strong>\u3002<\/li>\n<\/ul>\n<p><strong><b>\u00a0<\/b><\/strong><\/p>\n<p><strong><b>\u00a0<\/b><\/strong><\/p>\n<p style=\"text-align: center;\"><strong><b>\u56db\u3001[\u6570\u636e\u6982\u89c8]<\/b><\/strong><\/p>\n<p><strong><b>\u5236\u5907\u7684\u7eb3\u7c73\u901a\u9053Nb2O5\u7684\u8868\u5f81<\/b><\/strong><strong><b>\u4ee5\u53ca<\/b><\/strong><strong><b>\u901a\u8fc7\u7535\u5316\u5b66\u5faa\u73af\u5b9e\u73b0NCNO\u7684a-to-c\u8f6c\u5316<\/b><\/strong><\/p>\n<p>\u6837\u54c1\u7531\u7535\u8fde\u63a5\u5230Nb\u96c6\u7535\u5668\u7684\u5782\u76f4\u5b9a\u5411\u7eb3\u7c73\u901a\u9053\u6c27\u5316\u94cc(NCNO)\u7ec4\u6210\uff08<strong>\u56fe1<\/strong>\uff09\u3002\u8fd9\u79cd\u7279\u6b8a\u7684\u7eb3\u7c73\u7ed3\u6784\u6709\u52a9\u4e8e\u7535\u89e3\u8d28\u5feb\u901f\u8fdb\u5165\u6d3b\u6027\u58c1\uff0c\u5e76\u4fc3\u8fdb\u7535\u5b50\u548c\u79bb\u5b50\u4f20\u8f93\u4ee5\u589e\u5f3a\u52a8\u529b\u5b66\u3002\u9009\u533a\u7535\u5b50\u884d\u5c04\uff08SAED\uff1b\u56fe 1d\uff09\u3001X 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loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-236862\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72472-3.png\" alt=\"\" width=\"692\" height=\"435\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72472-3.png 692w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72472-3-300x189.png 300w\" sizes=\"(max-width: 692px) 100vw, 692px\" \/><\/p>\n<p style=\"text-align: center;\"><strong>\u56fe1.<\/strong> \u5236\u5907\u7684NCNO\u7684\u8868\u5f81\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-236863\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72473-3.png\" alt=\"\" width=\"711\" height=\"283\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72473-3.png 711w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72473-3-300x119.png 300w\" sizes=\"(max-width: 711px) 100vw, 711px\" \/><\/p>\n<p style=\"text-align: center;\"><strong>\u56fe2.<\/strong> \u7ecf\u7535\u5316\u5b66\u5faa\u73af\u7684NCNO\u7684\u7535\u538b\u66f2\u7ebf\u548c\u5fae\u5206\u5bb9\u91cf\u56fe\u00a0\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p><strong><b>a-to-c Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u7684\u7ed3\u6784\u8868\u5f81<\/b><\/strong><strong><b>\u4ee5\u53caRS-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u7684\u591a\u7535\u5b50\u6c27\u5316\u8fd8\u539f<\/b><\/strong><\/p>\n<p>\u900f\u5c04\u7535\u955c\u3001\u63a0\u5165\u5c04\u540c\u6b65\u52a0\u901f\u5668 X \u5c04\u7ebf\u884d\u5c04\u548c\u975e\u539f\u4f4d\u6269\u5c55X\u5c04\u7ebf\u5438\u6536\u7cbe\u7ec6\u7ed3\u6784 (EXAFS) \u7528\u4e8e\u9610\u660e Nb<sub>2<\/sub>O<sub>5<\/sub>\u00a0\u7684\u65b0\u5ca9\u76d0\u76f8\uff08\u56fe3\uff09\u3002\u9996\u5148\u901a\u8fc7SAED\u548c\u9ad8\u5206\u8fa8\u7387TEM\u8bc4\u4f303\u2009V\u548c0.5\u2009V\u4e4b\u95f4\u7535\u5316\u5b66\u5faa\u73af\u65f6\u7684\u76f8\u53d8\uff08\u56fe3a-f\uff09\u3002\u539f\u59cb\u6837\u54c1\u5728SAED\u4e2d\u5448\u73b0\u51fa\u6f2b\u5c04\u73af\uff08\u56fe3a\uff09\uff0c\u4e0e\u5728\u9ad8\u5206\u8fa8\u7387TEM\u4e2d\u89c2\u5bdf\u5230\u7684\u65e0\u5b9a\u5f62\u7279\u5f81\u4e00\u81f4\uff08\u56fe3d\uff09\u3002SAED \u56fe\u6848\u5728\u7b2c\u4e00\u4e2a\u5faa\u73af\u540e\u5f00\u59cb\u9510\u5316\uff08\u56fe3b\uff09\uff0c\u8868\u660e\u5728\u65e0\u5b9a\u5f62\u57fa\u8d28\u5185\u5f62\u6210\u4e86\u7eb3\u7c73\u5fae\u6676\uff08\u56fe3e\uff09\u3002\u7b2c20\u6b21\u5faa\u73af\u540e\uff0cSAED\u548c\u9ad8\u5206\u8fa8\u7387TEM\u5747\u663e\u793a\u6c27\u5316\u7269\u5df2\u5b8c\u5168\u7ed3\u6676\uff08\u56fe3c\uff0cf\uff09\u3002\u6b64\u5916\uff0c\u63a0\u5165\u5c04\u540c\u6b65\u8f90\u5c04X\u5c04\u7ebf\u884d\u5c04\u5728\u4e0d\u540c\u5165\u5c04\u89d2\uff0c\u5373\u63a2\u6d4b\u6df1\u5ea6\u4e0b\uff0c\u6837\u54c1\u7684\u5cf0\u5f62\u548c\u5cf0\u4f4d\u6ca1\u6709\u660e\u663e\u53d8\u5316\u3002\u56e0\u6b64\uff0c\u6837\u54c1\u59cb\u7ec8\u4fdd\u6301\u7eb3\u7c73\u6676\uff0c\u8868\u660e\u8584\u819c\u7684\u5747\u5300\u6027\u548c\u5fae\u4e0d\u8db3\u9053\u7684\u8868\u9762\u7d0a\u4e71\u3002<strong><b>\u8fd9\u8fdb\u4e00\u6b65\u8bf4\u660e\u901a\u8fc7\u7535\u5316\u5b66\u5faa\u73af\u5f97\u5230\u7684\u65b0\u6676\u6001\u7ed3\u6784\u76f8\u5bf9\u4e8e\u5176\u521d\u59cb\u975e\u6676\u7ed3\u6784\u7684\u6027\u80fd\u6709\u6240\u6539\u5584<\/b><\/strong>\u3002<\/p>\n<p>\u672c\u5de5\u4f5c\u91c7\u7528\u539f\u4f4dNb K\u8fb9X\u5c04\u7ebf\u5438\u6536\u8fd1\u8fb9\u7ed3\u6784(XANES)\u548cXPS\u5bf9\u6837\u54c1\u4e2dNb\u5728\u5404\u79cd\u653e\u7535\u72b6\u6001(\u56fe4a,b)\u4e0b\u7684\u4ef7\u6001\u8fdb\u884c\u8bc4\u4ef7\u3002\u539f\u59cb\u6837\u54c1\u7684XANES\u8c31\u6700\u63a5\u8fd1\u4e8eH-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6807\u51c6\uff0c\u8868\u660eNb\u5728+5\u5de6\u53f3\u7684\u4f53\u4e2d\u5904\u4e8e\u6c27\u5316\u72b6\u6001\u3002\u5f53\u653e\u7535\u52301 V\u65f6\uff0c\u6837\u54c1\u8fb9\u7f18\u4f4d\u7f6e\u4e0eNbO<sub>2<\/sub>\u6807\u51c6\u63a5\u8fd1\uff0c\u8bf4\u660eNb\u7684\u6c27\u5316\u6001\u964d\u4f4e\u5230+4\u3002\u8fdb\u4e00\u6b65\u653e\u7535\u52300.5 V\u65f6\uff0c\u8c31\u7ebf\u8fb9\u7f18\u79fb\u52a8\u5230\u66f4\u4f4e\u7684\u80fd\u91cf\uff0c\u8868\u660e\u7535\u6781\u672c\u4f53\u4e2d\u5904\u4e8e+4\u4ee5\u4e0b\u7684Nb\u6c27\u5316\u72b6\u6001\u3002\u91c7\u7528DFT\u6a21\u62df\u4e86\u5d4c\u9502\u8fdb\u5165RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7684\u7535\u538b\u5256\u9762\u3002\u7531\u8fd9\u4e9b\u8ba1\u7b97\u6784\u5efa\u7684\u4f2a\u4e8c\u5143RS-Nb<sub>2<\/sub>O<sub>5<\/sub>-Li<sub>3<\/sub>Nb<sub>2<\/sub>O<sub>5<\/sub>\u76f8\u56fe\u5982\u56fe4c\u6240\u793a\uff0c\u8ba1\u7b97\u548c\u5b9e\u9a8c\u7535\u538b\u5206\u5e03\u56fe\u5982\u56fe4d\u6240\u793a\u3002\u603b\u4f53\u800c\u8a00\uff0cPerdew-Burke-Ernzerhof\u7535\u538b\u5e73\u5747\u503c\u4e3a1.76 V\uff0c\u4e0e\u5b9e\u9a8c\u5e73\u5747\u503c1.67 V\u975e\u5e38\u543b\u5408\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-236864 aligncenter\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72474-3.png\" alt=\"\" width=\"555\" height=\"600\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72474-3.png 555w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72474-3-278x300.png 278w\" sizes=\"(max-width: 555px) 100vw, 555px\" \/><\/p>\n<p style=\"text-align: center;\"><strong>\u56fe3.<\/strong> \u7535\u5316\u5b66\u5faa\u73af\u4e2dNCNO\u6837\u54c1\u7684\u7ed3\u6784\u8868\u5f81 \u00a0\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-236865\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72475-1.png\" alt=\"\" width=\"664\" height=\"509\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72475-1.png 664w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72475-1-300x230.png 300w\" sizes=\"(max-width: 664px) 100vw, 664px\" \/><\/p>\n<p><strong>\u56fe4.<\/strong> RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u4e2dNb\u6c27\u5316\u6001\u7684\u8868\u5f81\uff1bPerdew-Burke-Enzerhof\u8ba1\u7b97\u7684\u5316\u5408\u7269\u76f8\u56fe\uff1b\u4ee5\u53caLixNb<sub>2<\/sub>O<sub>5<\/sub>\u7684\u7535\u538b\u5206\u5e03\u00a0\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>N<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O\u4f5c\u4e3aO\u6e90\u5728\u915a\u7c7b\u50ac\u5316\u5408\u6210\u4e2d\u7684\u91cd\u4f30<\/b><\/strong><strong><b>\u4ee5\u53caRS-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7684\u7535\u8377\u5b58\u50a8\u548c\u4f20\u8f93\u52a8\u529b\u5b66<\/b><\/strong><\/p>\n<p>RS-\u548ca-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u572820\u300150\u3001100\u3001200\u548c1,000\u2009mA\u2009g<sup>-1<\/sup>\u7684\u4e0d\u540c\u7535\u6d41\u901f\u7387\u4e0b\u7684\u500d\u7387\u6027\u80fd\u5982\u56fe5a\u6240\u793a\u3002RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u572820\u2009mA\u2009g<sup>-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8868\u73b0\u51fa269\u2009mAh\u2009g<sup>-1<\/sup>\u7684\u9ad8\u53ef\u9006\u5bb9\u91cf\uff0c\u5bf9\u5e94\u4e8e\u6bcfNb\u7ea61.42\u4e2a\u7535\u5b50\u6c27\u5316\u8fd8\u539f\u3002RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7684\u9ad8\u5bb9\u91cf\u662fNb<sub>2<\/sub>O<sub>5<\/sub>\u548c\u94cc\u9178\u76d0\u7535\u6781\u62a5\u544a\u503c\u4e2d\u6700\u597d\u7684\u3002\u6b64\u5916\uff0c\u672c\u5de5\u4f5c\u89c2\u5bdf\u5230\u5728200\u2009mA\u2009g<sup>&#8211;<\/sup><sup>1<\/sup>(243\u2009mAh\u2009g<sup>\u22121<\/sup>)\u7684\u7535\u6d41\u901f\u7387\u589e\u52a0\u65f6\u5bb9\u91cf\u4e0b\u964d&lt;10%\uff0c\u800c\u57281,000\u2009mA\u2009g<sup>&#8211;<\/sup><sup>1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u7535\u6781\u5bb9\u91cf\u5728191\u2009mAh g<sup>-1<\/sup>\u65f6\u7565\u4f4e\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0ca-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u57281,000\u2009mA\u2009g<sup>-1<\/sup>\u7684\u500d\u7387\u4e0b\u663e\u793a\u51fa\u76f8\u5f53\u4f4e\u7684\u5bb9\u91cf\uff0873\u2009mAh\u2009g<sup>-1<\/sup>\uff09\u3002RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u548ca-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u5728200 m A g<sup>-1<\/sup>\u7535\u6d41\u4e0b\u7684\u5faa\u73af\u5bff\u547d\u5982\u56fe5b\u6240\u793a\u3002RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u5728400\u6b21\u5faa\u73af\u4e2d\u8868\u73b0\u51fa224\u2009mAh\u2009g<sup>-1<\/sup>\u7684\u9ad8\u53ef\u9006\u5bb9\u91cf\uff0c\u5bb9\u91cf\u635f\u5931\u4ec50.02 %\u3002\u5728RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u00a0(20 mA g<sup>-1<\/sup>)\u7684\u524d4\u4e2a\u5f62\u6210\u5468\u671f\u4e2d\uff0c\u521d\u59cb\u5e93\u4ed1\u6548\u7387\u4e3a75 %\u3002<strong><b>\u5faa\u73af10\u6b21\u540e\uff0c\u7535\u6781\u5e93\u4ed1\u6548\u7387\u8d85\u8fc799%<\/b><\/strong>\u3002\u5230\u7b2c400\u6b21\u5faa\u73af\u65f6\uff0c\u7535\u6781\u8868\u73b0\u51fa99.93%\u4ee5\u4e0a\u7684\u5e93\u4ed1\u6548\u7387\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u03b1-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7535\u6781\u7684\u5e93\u4ed1\u6548\u7387\u4e3a98.78%\uff0c\u7b2c400\u6b21\u5faa\u73af\u65f6\u5bb9\u91cf\u635f\u5931\u8d85\u8fc715%\u3002<strong><b>RS-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u7a33\u5b9a\u6027\u7684\u63d0\u9ad8\u53ef\u5f52\u56e0\u4e8e\u5176\u7acb\u65b9\u9aa8\u67b6\u53ca\u5176\u7eb3\u7c73\u7ed3\u6784\u5728\u6574\u4e2a\u8131\u5d4c\u9502\u8fc7\u7a0b\u4e2d\u7684\u4fdd\u7559<\/b><\/strong>\u3002<\/p>\n<p>\u4e3a\u4e86\u9610\u660eLi<sub>3<\/sub>Nb<sub>2<\/sub>O<sub>5<\/sub>\u4e2d\u9502\u7684\u8fc1\u79fb\u673a\u5236\uff0c\u672c\u5de5\u4f5c\u8ba1\u7b97\u4e866\u79cd\u4ee3\u8868\u6027\u4f4e\u80fd\u6784\u578b\u4e2d38\u6761Li\u8df3\u8dc3\u8def\u5f84\u7684\u52a8\u529b\u5b66\u5206\u8fa8\u6fc0\u6d3b\u52bf\u5792\uff0c\u4ee5\u8003\u8651\u5c40\u57df\u73af\u5883\u53ef\u80fd\u7684\u5f71\u54cd\u3002\u4e0eDRX\u9502\u8fc7\u6e21\u91d1\u5c5e\u6c27\u5316\u7269\u9634\u6781\u76f8\u6bd4\uff0c\u672c\u5de5\u4f5c\u53d1\u73b0\u76f4\u63a5\u516b\u9762\u4f53-\u516b\u9762\u4f53\u8dc3\u8fc1\u6bd4\u516b\u9762\u4f53-\u56db\u9762\u4f53-\u516b\u9762\u4f53\u8dc3\u8fc1\u66f4\u53d7\u9752\u7750\u3002\u6cbf\u516b\u9762\u4f53-\u516b\u9762\u4f53\u8dc3\u8fc1\u7684\u5c40\u57df\u73af\u5883\u53ef\u4ee5\u7528x-Li\u6765\u8868\u5f81\uff0c\u5176\u4e2d0\u2264x\u22644\u662fLi\u79bb\u5b50\u5360\u636e\u8fc1\u79fb\u8def\u5f84\u76f8\u90bb\u7684\u5171\u8fb9\u516b\u9762\u4f53\u4f4d\u7684\u6570\u76ee\u3002Nb\u5360\u636e\u90bb\u8fd1\u4f4d\u7f6e\u7684\u6570\u91cf\u4e3a4-x\u3002\u5982\u56fe5c\u6240\u793a\uff0c\u4e0eNb<sup>3+\/4+<\/sup>\u76f8\u6bd4\uff0cx-Li\u7684\u589e\u52a0\u663e\u8457\u964d\u4f4e\u4e86Li<sup>+<\/sup>\u7684\u9759\u7535\u65a5\u529b\u5bfc\u81f4\u7684\u8fc1\u79fb\u969c\u788d\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-236866\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72476-1.png\" alt=\"\" width=\"667\" height=\"515\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72476-1.png 667w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72476-1-300x232.png 300w\" sizes=\"(max-width: 667px) 100vw, 667px\" \/><\/p>\n<p><strong>\u56fe5.<\/strong> RS-Li<sub>3<\/sub>Nb<sub>2<\/sub>O<sub>5<\/sub>\u8fc1\u79fb\u52bf\u5792\u7684RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u8ba1\u7b97\u548ca-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6837\u54c1\u7684\u7535\u5316\u5b66\u6027\u80fd\u00a0\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p><strong><b>RS-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7684\u7535<\/b><\/strong><strong><b>\u5b66<\/b><\/strong><strong><b>\u7279\u6027<\/b><\/strong><\/p>\n<p>\u63d2\u5c42\u7535\u6781\u6750\u6599\u4e3a\u6df7\u5408\u79bb\u5b50\u5bfc\u4f53\u548c\u7535\u5b50\u5bfc\u4f53\u3002\u6750\u6599\u7684\u7535\u5bfc\u7387\u5bf9\u5176\u529f\u7387\u6027\u80fd\u6709\u660e\u663e\u5f71\u54cd\u3002\u56e0\u6b64\uff0c\u672c\u5de5\u4f5c\u901a\u8fc7Mott-Schottky\u5206\u6790\u548c\u4e24\u70b9\u63a2\u9488\u7535\u5bfc\u7387\u6d4b\u91cf\uff0c\u4ee5\u53caPF-TUNA\u5bf9\u6bd4a-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6765\u8bc4\u4ef7RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7684\u7535\u5bfc\u7387(\u56fe6)\u3002\u5bf9\u7eaf\u76f8\u3001a-Nb<sub>2<\/sub>O<sub>5<\/sub>\u548cRS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6837\u54c1\u8fdb\u884cMott-Schottky\u5206\u6790(\u56fe6a)\u3002\u56fe6a\u4e2d\u6bcf\u4e2a\u6837\u54c1\u7684\u6b63\u659c\u7387\u8868\u660e\u4e86\u4e00\u4e2an\u578b\u534a\u5bfc\u4f53\u54cd\u5e94\uff0c\u5176\u4e2d\u7535\u5b50\u662f\u4e3b\u8981\u7684\u7535\u8377\u8f7d\u6d41\u5b50\uff0c\u5982\u9884\u671f\u7684Nb<sub>2<\/sub>O<sub>5<\/sub>\u3002Mott-Schottky\u66f2\u7ebf\u4e2d\u659c\u7387\u8d8a\u51f9\u9677\uff0c\u76f8\u5e94\u7684\u8f7d\u6d41\u5b50\u6d53\u5ea6\u8d8a\u9ad8\uff0cRS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7684\u7535\u8377\u8f7d\u6d41\u5b50\u6d53\u5ea6\u6700\u9ad8\u3002\u5bf9\u5faa\u73af\u540e\u7684a-Nb<sub>2<\/sub>O<sub>5<\/sub>\u548cRS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6837\u54c1\u8fdb\u884c\u4e86PF-TUNA\u6210\u50cf(\u56fe6b-d)\uff0c\u540c\u65f6\u7ed8\u5236\u4e86\u5404\u6837\u54c1\u7684\u7535\u5bfc\u7387\u548c\u5f62\u8c8c\u56fe\u3002<strong><b>\u539f\u59cb\u6837\u54c1PF- TUNA\u6210\u50cf\u663e\u793a\u7535\u5bfc\u7387\u53ef\u5ffd\u7565\u4e0d\u8ba1\uff0c\u8868\u660e\u5176\u7edd\u7f18\u6027\u3002<\/b><\/strong>\u800c\u5faa\u73afa-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6837\u54c1(\u56fe6b)\u4e2d\u7684\u7535\u5bfc\u76f8\u5bf9\u4e8e\u539f\u59cb\u6837\u54c1\u6709\u6240\u589e\u52a0\uff0c\u4f46RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u00a0(\u56fe6c)\u7684\u89c2\u6d4b\u5e73\u5747\u7535\u6d41\u6bd4a-Nb<sub>2<\/sub>O<sub>5<\/sub>\u9ad8\u4e24\u4e2a\u6570\u91cf\u7ea7\u3002<strong><b>PF-TUNA\u6210\u50cf\u8868\u660e\uff0c\u5c3d\u7ba1RS-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u76f8\u5bf9a-Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u7684\u7535\u5bfc\u7387\u5927\u5e45\u63d0\u9ad8\uff0c\u4f46\u5728\u7eb3\u7c73\u5c3a\u5ea6\u4e0b\u8868\u9762\u4ecd\u7136\u662f\u5f02\u8d28\u7684<\/b><\/strong>\u3002\u5728\u56fe6d\u6240\u793a\u76845\u00d75\u2009\u03bcm<sup>2<\/sup>\u533a\u57df\u5185\uff0c\u8868\u9762\u4e0a\u89c2\u5bdf\u5230\u7535\u6d41\u5206\u5e03\u4e0d\u5747\u5300\u3002\u672c\u5de5\u4f5c\u5047\u8bbe\u89c2\u5bdf\u5230\u7684\u975e\u5747\u5300\u6027\u4e0e\u76f8\u53d8\u8fc7\u7a0b\u6709\u5173\uff0c\u76f8\u53d8\u8fc7\u7a0b\u81ea\u9002\u5e94\u5730\u4fc3\u8fdb\u79bb\u5b50\u548c\u7535\u5b50\u8f93\u8fd0\u7684\u6700\u4f4e\u8fc1\u79fb\u5792\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-236867 aligncenter\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72477-1.png\" alt=\"\" width=\"668\" height=\"615\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72477-1.png 668w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/05\/\u56fe\u72477-1-300x276.png 300w\" sizes=\"(max-width: 668px) 100vw, 668px\" \/><\/p>\n<p><strong>\u56fe6.<\/strong> RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u548ca-Nb<sub>2<\/sub>O<sub>5<\/sub>\u6837\u54c1\u7684\u7535\u5bfc\u7387\u8868\u5f81 \u00a0\u00a0<span style=\"color: #808080;\">\u00a9 2022 Springer Nature \u00a0<\/span><\/p>\n<p>&nbsp;<\/p>\n<p style=\"text-align: center;\"><strong><b>\u00a0\u4e94\u3001[\u6210\u679c\u542f\u793a]<\/b><\/strong><\/p>\n<p><strong><b>\u00a0<\/b><\/strong><\/p>\n<p><strong><b>\u603b\u4e4b\uff0c<\/b><\/strong><strong><b>\u672c\u5de5\u4f5c<\/b><\/strong><strong><b>\u62a5\u9053\u4e86\u4e00\u79cd\u901a\u8fc7\u7535\u5316\u5b66\u9a71\u52a8\u7684\u975e\u6676\u6001\u7eb3\u7c73\u901a\u9053Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u6676\u5316\u800c\u4ea7\u751f\u7684\u5ca9\u76d0Nb<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><strong><b>O<\/b><\/strong><strong><sub><b>5<\/b><\/sub><\/strong><strong><b>\u7535\u6781\u6750\u6599\u3002<\/b><\/strong>RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u4e3a\u6bcfNb\u591a\u7535\u5b50\u6c27\u5316\u8fd8\u539f\uff0c\u7528\u4e8e\u9502\u79bb\u5b50\u5b58\u50a8\u3002DFT\u8ba1\u7b97\u63ed\u793a\u4e86\u5bfc\u81f4RS-Nb<sub>2<\/sub>O<sub>5<\/sub>\u7279\u6b8a\u7535\u5316\u5b66\u6027\u80fd\u7684\u91cd\u8981\u4f4e\u80fd\u9502\u8fc1\u79fb\u8def\u5f84\u3002\u7acb\u65b9\u7ed3\u6784\u7531\u4e8e\u589e\u52a0\u4e86\u9502\u79bb\u5b50\u6269\u6563\u7cfb\u6570\u548c\u7535\u5bfc\u7387\uff0c\u4ece\u800c\u63d0\u4f9b\u4e86\u5177\u6709\u9ad8\u500d\u7387\u6027\u80fd\u7684\u6750\u6599\u3002\u540c\u65f6\uff0c\u7531\u4e8e\u8131\u5d4c\u9502\u7684\u7ed3\u6784\u5b8c\u6574\u6027\uff0c\u8be5\u6676\u4f53\u8868\u73b0\u51fa\u8f83\u9ad8\u7684\u7a33\u5b9a\u6027\u3002\u7535\u5316\u5b66\u5faa\u73af\u8fc7\u7a0b\u4e2d\u539f\u5b50\u81ea\u7ec4\u7ec7\u8fdb\u5165\u6700\u4f18\u6676\u4f53\u7ed3\u6784\uff0c\u4e3a\u83b7\u5f97\u5177\u6709\u72ec\u7279\u6027\u80fd\u7684\u7a00\u6709\u91d1\u5c5e\u6c27\u5316\u7269\u7ed3\u6784\u63d0\u4f9b\u4e86\u5408\u6210\u9014\u5f84\u3002\u5229\u7528\u7535\u5316\u5b66\u5faa\u73af\u5f62\u6210\u65b0\u9896\u7684\u6676\u6001\u7ed3\u6784\uff0c\u53ef\u4ee5\u6709\u5229\u4e8e\u8bbe\u8ba1\u5176\u4ed6\u589e\u5f3a\u7535\u6781\u6750\u6599\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>&nbsp;<\/p>\n<p>\u7b2c\u4e00\u4f5c\u8005\uff1aPete Barnes<\/p>\n<p>\u901a\u8baf\u4f5c\u8005\uff1a\u718a\u6656\u3001Shyue Ping Ong<\/p>\n<p>\u901a\u8baf\u5355\u4f4d\uff1a\u5fb7\u56fd\u9a6c\u514b\u65af\u666e\u6717\u514b\u7164\u70ad\u7814\u7a76\u6240<\/p>\n<p>\u8bba\u6587doi\uff1a<\/p>\n<p>https:\/\/doi.org\/10.1038\/s41563-022-01242-0<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u00a0 \u00a0\u4e00\u3001[\u5bfc\u8bfb] 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