{"id":236213,"date":"2022-04-25T06:01:41","date_gmt":"2022-04-24T22:01:41","guid":{"rendered":"\/\/m.iemloyee.com\/?p=236213"},"modified":"2022-04-24T16:01:49","modified_gmt":"2022-04-24T08:01:49","slug":"%e6%b1%aa%e6%b7%8f%e7%94%b0-nature-catalysis%ef%bc%9a%e7%ba%af%e5%ba%a6%ef%bc%9e99%e3%80%81%e5%9b%9e%e6%94%b6%e7%8e%8790%ef%bc%81pse%e5%8f%8d%e5%ba%94%e5%99%a8%e5%8a%a9%e5%8a%9bco2rr","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=236213","title":{"rendered":"\u6c6a\u6dcf\u7530 Nature Catalysis\uff1a\u7eaf\u5ea6\uff1e99%\u3001\u56de\u6536\u738790%\uff01PSE\u53cd\u5e94\u5668\u52a9\u529bCO2RR"},"content":{"rendered":"

\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u5229\u7528\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u53cd\u5e94\uff08CO2<\/sub>RR\uff09\u5c06CO2<\/sub>\u7535\u5316\u5b66\u8f6c\u5316\u6210\u57fa\u672c\u7684\u5316\u5b66\u539f\u6599\u662f\u4e00\u79cd\u5728\u7f13\u89e3\u6c14\u5019\u53d8\u5316\u7684\u65b9\u6cd5\uff0c\u540c\u65f6\u50a8\u5b58\u548c\u4f7f\u7528\u53ef\u518d\u751f\u7535\u529b\u3002\u5176\u4e2d\uff0c\u50ac\u5316\u6750\u6599\u8bbe\u8ba1\u548c\u53cd\u5e94\u5668\u5de5\u7a0b\u4e00\u76f4\u662f\u8be5\u9886\u57df\u7684\u4e24\u5927\u91cd\u70b9\u3002\u867d\u7136\u5f00\u53d1\u4e86\u591a\u79cd\u50ac\u5316\u5242\u6765\u63d0\u9ad8\u5bf9C1<\/sub>\uff08CO\u7b49\uff09\u3001C2<\/sub>\uff08\u4e59\u9187\u7b49\uff09\u4ea7\u7269\u7684\u9009\u62e9\u6027\u548c\u6d3b\u6027\uff0c\u4f46CO2<\/sub>\u7535\u89e3\u69fd\u7684\u53d1\u5c55\uff0c\u5c24\u5176\u662f\u5728\u6d41\u901a\u6c60\u548c\u819c\u7535\u6781\u7ec4\u4ef6\uff08MEA\uff09\u7535\u6c60\u53cd\u5e94\u5668\u4e2d\u4f7f\u7528\u6c14\u4f53\u6269\u6563\u5c42\uff08GDL\uff09\u7535\u6781\uff0c\u5728\u8fbe\u5230\u5de5\u4e1a\u76f8\u5173\u6307\u6807\u65b9\u9762\u53d1\u6325\u6838\u5fc3\u4f5c\u7528\u3002\u5c3d\u7ba1CO2<\/sub>RR\u6027\u80fd\u7684\u53d6\u5f97\u4e0d\u9519\u8fdb\u5c55\uff0c\u4f46\u5b58\u5728\u4e00\u4e2a\u57fa\u672c\u4f46\u7ecf\u5e38\u88ab\u5ffd\u89c6\u7684\u6311\u6218\uff0c\u5b83\u53ef\u80fd\u4f1a\u6781\u5927\u5730\u9650\u5236CO2<\/sub>RR\u7684\u5546\u4e1a\u5316\u6f5c\u529b\uff1a\u78b3\u9178\u76d0\u4ea4\u53c9\u5bfc\u81f4\u7684\u5927\u91cf\u78b3\u635f\u5931\u3002\u5728CO2<\/sub>RR\u7535\u89e3\u8fc7\u7a0b\u4e2d\uff0c\u7279\u522b\u662f\u5728\u5927\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u9634\u6781\u7535\u89e3\u8d28\u754c\u9762\u4f1a\u4ea7\u751f\u5927\u91cf\u6c22\u6c27\u6839\u79bb\u5b50\uff08OH–<\/sup>\uff09\uff0c\u4e0eCO2<\/sub>\u5feb\u901f\u53cd\u5e94\u5f62\u6210\u78b3\u9178\u6839\u6216\u78b3\u9178\u6c22\u6839\u79bb\u5b50\u3002\u5728\u7535\u573a\u9a71\u52a8\u4e0b\uff0c\u8fd9\u4e9b\u78b3\u9178\u6839\u79bb\u5b50\u7a7f\u8fc7\u9634\u6781-\u9633\u6781\u754c\u9762\uff08\u6c34\u6eb6\u6db2\u6216\u9634\u79bb\u5b50\u4ea4\u6362\u819c\uff09\u5411\u53cd\u5e94\u5668\u7684\u9633\u6781\u4fa7\u8fc1\u79fb\uff0c\u5e76\u4e0e\u6790\u6c27\u53cd\u5e94\uff08OER\uff09\u4e2d\u5c40\u90e8\u4ea7\u751f\u7684\u8d28\u5b50\uff08H+<\/sup>\uff09\u91cd\u65b0\u7ed3\u5408\uff0c\u518d\u6b21\u5f62\u6210CO2<\/sub>\u6c14\u4f53\u3002\u8fd9\u4e9b\u4ea4\u53c9CO2<\/sub>\u6c14\u4f53\u5206\u5b50\u4e0d\u80fd\u76f4\u63a5\u7528\u4e8eCO2<\/sub>RR\uff0c\u5bfc\u81f4\u663e\u8457\u7684\u78b3\u635f\u5931\uff0c\u4ece\u800c\u964d\u4f4e\u4e86CO2<\/sub>RR\u7684\u6574\u4f53\u80fd\u6e90\u6548\u7387\u3002\u7531\u4e8eCO2<\/sub>\u6d41\u548c\u7535\u89e3\u8d28\u4e4b\u95f4\u7684\u6301\u7eed\u5316\u5b66\u53cd\u5e94\uff0c\u5f53\u4f7f\u7528\u5f3a\u78b1\u6027\u6eb6\u6db2\u65f6\uff0c\u78b3\u635f\u5931\u95ee\u9898\u66f4\u52a0\u4e25\u91cd\u3002
\n \"\"<\/p>\n

\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u83b1\u65af\u5927\u5b66\u6c6a\u6dcf\u7530\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u591a\u5b54\u56fa\u4f53\u7535\u89e3\u8d28\uff08porous solid electrolyte, PSE\uff09\u53cd\u5e94\u5668\uff0c\u4ee5\u6709\u6548\u7684\u5b9e\u73b0\u4e86\u5728CO2<\/sub>RR\u7535\u89e3\u8fc7\u7a0b\u4e2d\u4ea4\u53c9CO2<\/sub>\u7684\u9ad8\u6548\u56de\u6536\u3002\u901a\u8fc7\u5728\u9634\u6781\u548c\u9633\u6781\u4e4b\u95f4\u5f62\u6210\u53ef\u6e17\u900f\u7684\u79bb\u5b50\u4f20\u5bfc\u78fa\u5316\u805a\u5408\u7269\u7535\u89e3\u8d28\u4f5c\u4e3a\u7f13\u51b2\u5c42\uff0c\u4ea4\u53c9\u78b3\u9178\u76d0\uff08CO3<\/sub>2-<\/sup>\uff09\u53ef\u4ee5\u4e0e\u9633\u6781OER\u4ea7\u751f\u7684\u8d28\u5b50\uff08H+<\/sup>\uff09\u7ed3\u5408\uff0c\u91cd\u65b0\u5f62\u6210CO2<\/sub>\u6c14\u4f53\uff0c\u540c\u65f6\u5229\u7528\u53bb\u79bb\u5b50\u6c34\u8fde\u7eed\u51b2\u6d17PSE\u7f13\u51b2\u5c42\uff0c\u53ef\u4ee5\u5f88\u5bb9\u6613\u5730\u91cd\u65b0\u6355\u83b7CO2<\/sub>\u6c14\u4f53\u4ee5\u91cd\u590d\u4f7f\u7528\uff0c\u800c\u65e0\u9700\u4e0e\u9633\u6781O2\u6df7\u5408\u3002\u6b64\u5916\uff0c\u4f5c\u8005\u4f7f\u7528\u94f6\u7eb3\u7c73\u7ebf\uff08Ag NWs\uff09\u50ac\u5316\u5242\u4f5c\u4e3a\u6a21\u578b\uff0c\u5c06CO2<\/sub>\u8fd8\u539f\u4e3aCO\uff0c\u80fd\u591f\u4ee5\u8d85\u9ad8\u7eaf\u5ea6\u5f62\u5f0f\uff08\u6c14\u4f53\u7eaf\u5ea6\u8d85\u8fc799%\uff09\u5b9e\u73b0\u56de\u6536\u7387\u9ad8\u8fbe90%\u7684\u4ea4\u53c9CO2<\/sub>\u6c14\u4f53\uff0c\u540c\u65f6\u5728200 mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u53ef\u4ee5\u63d0\u4f9b\u8d85\u8fc790%\u7684CO\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u3002\u6b64\u5916\uff0c\u4f5c\u8005\u8fd8\u8bc1\u660e\u4e86\u7528\u4e8e\u4ea4\u53c9CO2\u56de\u6536\u7684PSE\u53cd\u5e94\u5668\u53ef\u4ee5\u6210\u529f\u5730\u6269\u5c55\u5230\u4e0d\u540c\u7684CO2RR\u50ac\u5316\u5242\u548c\u4ea7\u54c1\u3002\u5c06\u8fd9\u4e9b\u56de\u6536\u7684CO2<\/sub>\u518d\u5faa\u73af\u56de\u8f93\u5165\u6d41\u4e2d\uff0c\u5728100 mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u83b7\u5f97\u8d85\u8fc790%\u7684\u8fde\u7eedCO2<\/sub>\u8f6c\u5316\u6548\u7387\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cRecovering carbon losses in CO2<\/sub> electrolysis using a solid electrolyte reactor\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Catalysis<\/em>\u4e0a\u3002<\/p>\n

\u672c\u6587\u6240\u6709\u56fe\u6765\u6e90\u4e8e\u00a9 2022 Springer Nature Limited\u3002
\n \"\"
\n \u3010\u6838\u5fc3\u521b\u65b0\u3011<\/strong><\/p>\n

1\u3001\u5229\u7528PSE\u53cd\u5e94\u5668\uff0c\u5b9e\u73b0\u4e86\u5728CO2<\/sub>RR\u7535\u89e3\u8fc7\u7a0b\u4e2d\u4ea4\u53c9CO2<\/sub>\u7684\u9ad8\u6548\u56de\u6536\uff0c\u800c\u65e0\u9700\u4e0e\u9633\u6781O2<\/sub>\u6df7\u5408\u3002<\/p>\n

2\u3001\u5229\u7528Ag NWs\u50ac\u5316\u5242\u5c06CO2<\/sub>\u8fd8\u539f\u4e3aCO\uff0c\u4ee5\u6c14\u4f53\u7eaf\u5ea6\u8d85\u8fc799%\u5f62\u5f0f\u5b9e\u73b0\u56de\u6536\u7387\u9ad8\u8fbe90%\u7684\u4ea4\u53c9CO2<\/sub>\u6c14\u4f53\uff0c\u540c\u65f6\u5728200 mA cm-2<\/sup>\u4e0b\u53ef\u63d0\u4f9b\u8d85\u8fc790%\u7684CO\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u3002<\/p>\n

3\u3001\u5c06\u56de\u6536\u7684CO2<\/sub>\u518d\u5faa\u73af\u56de\u8f93\u5165\u6d41\u4e2d\uff0c\u5728100 mA cm-2<\/sup>\u4e0b\u5b9e\u73b0\u4e86\u8d85\u8fc790%\u7684\u8fde\u7eedCO2<\/sub>\u8f6c\u5316\u6548\u7387<\/p>\n

\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u9634\u79bb\u5b50MEA\u7535\u6c60\u4e2dCO2<\/sub>\u4ea4\u53c9\u73b0\u8c61\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e8c\u3001\u4f20\u7edfCO2<\/sub> MEA\u7535\u89e3\u69fd\u4e2d\u7684\u5927\u91cf\u78b3\u635f\u5931<\/strong>
\n \"\"\uff08a\uff09\u9634\u6781\u4fa7CO2<\/sub>\u6d41\u91cf\u5206\u6790\uff0c\u5176\u4e2d\u5b9eCO2<\/sub>\u6d41\u51fa\u8fdc\u5c0f\u4e8eCO2<\/sub>\u6d41\u91cf\uff0c\u4ec5\u8003\u8651CO2<\/sub>RR\u6d88\u8017\uff1b<\/p>\n

\uff08b\uff09\u9633\u6781\u4fa7\u7684\u603b\u6c14\u4f53\u6d41\u91cf\u5206\u6790\uff0c\u5176\u4e2d\u7535\u5316\u5b66\u8ba1\u7b97\u7684O2<\/sub>\u6d41\u91cf\u548c\u6d4b\u91cf\u7684O2<\/sub>\u6d41\u51fa\u91cf\u8fdc\u8fdc\u8d85\u8fc7\u4ea4\u53c9CO2<\/sub>\u6c14\u4f53\u6d41\u91cf\uff1b<\/p>\n

\uff08c\uff09CO2\u6d41\u91cf\u5206\u6790\uff0c\u663e\u793a\u4ea4\u53c9CO2<\/sub>\u548c\u8f6c\u5316\u7684CO2<\/sub>\uff0c\u52a0\u8d77\u6765\u5339\u914d\u9634\u6781\u4fa7\u7684\u603bCO2<\/sub>\u6d41\u91cf\u53d8\u5316\uff1b<\/p>\n

\uff08d\uff09\u4e0d\u540cCO2<\/sub>RR\u4ea7\u7269\u7684\u4ea4\u53c9CO2<\/sub>\u4e0e\u8f6c\u5316CO2<\/sub>\u7684\u6bd4\u7387\u3002<\/p>\n

\u56fe\u4e09\u3001PSE\u53cd\u5e94\u5668\u53ca\u5176\u6c14\u4f53\u5206\u6790\u7cfb\u7edf<\/strong>
\n \"\"\uff08a\uff09PSE\u53cd\u5e94\u5668\u4e2dCO2<\/sub>RR\u7684\u793a\u610f\u56fe\u4ee5\u53ca\u901a\u8fc7\u4e0ePSE\u7f13\u51b2\u5c42\u4e2d\u7684\u8d28\u5b50\u590d\u5408\u6765\u56de\u6536\u4ea4\u53c9CO3<\/sub>2-<\/sup>\u79bb\u5b50\u7684\u8fc7\u7a0b\uff1b<\/p>\n

\uff08b\uff09PSE\u53cd\u5e94\u5668\u4e2dCO2<\/sub>RR\u8fc7\u7a0b\u4e2dCO2\u56de\u6536\u7387\u6d4b\u91cf\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u56db\u3001Ag NW\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u4e2d\u7684\u4ea4\u53c9CO2<\/sub>\u56de\u6536\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09Ag NW\u7684SEM\u548cHRTEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u4e2d\uff0cAg NW\u50ac\u5316\u5242\u4e0aCO2<\/sub>RR\u7684IV\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u4e2d\uff0c\u4e0d\u540c\u5de5\u4f5c\u7535\u6d41\u4e0bAg NW\u7684CO FE\uff1b<\/p>\n

\uff08d\uff09\u4f7f\u7528Ag NW\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u7684CO2<\/sub>\u56de\u6536\u6027\u80fd\uff1b<\/p>\n

\uff08e\uff09\u4e0eGC\u6d4b\u91cf\u7684\u4ea4\u53c9CO2<\/sub>\u6216\u7406\u8bba\u8ba1\u7b97\u7684\u4ea4\u53c9CO2<\/sub>\u76f8\u6bd4\uff0c\u5728\u4e2d\u95f4\u5c42\u56de\u6536\u7684CO2<\/sub>\u7684\u6bd4\u4f8b\uff1b<\/p>\n

\uff08f\uff09\u6765\u81eaGC\u7684\u70ed\u5bfc\u68c0\u6d4b\u5668\u54cd\u5e94\u663e\u793aH2<\/sub>\u5cf0\u3001O2<\/sub>\u5cf0\u548cCO2<\/sub>\u5cf0\uff0c\u5176\u4e2dCO2<\/sub>\u5bf9\u5e94\u4e8e\u4e00\u7cfb\u5217\u7535\u6d41\u7684\u56de\u6536\u6c14\u4f53\u7eaf\u5ea6\u3002<\/p>\n

\u56fe\u4e94\u3001PSE\u53cd\u5e94\u5668\u56de\u6536\u4ea4\u53c9CO2<\/sub>\u7684\u5e7f\u6cdb\u9002\u7528\u6027<\/strong>
\n \"\"\uff08a-c\uff09Ni-SAC\u30012D-Bi\u548cCu NPs\u7684TEM;<\/p>\n

\uff08d-f\uff09PSE\u53cd\u5e94\u5668\u4e0eNi-SAC\u30012D-Bi\u548cCu NPs\u7684\u7535\u6d41\u548c\u7535\u6d41\u5bc6\u5ea6\u4e0e\u7535\u6c60\u7535\u538b\uff08IV\u66f2\u7ebf\uff09\u7684\u5173\u7cfb\uff1b<\/p>\n

\uff08g-i\uff09CO\u3001\u7532\u9178\u76d0\u548c\u4e03\u79cd\u4e0d\u540c\u7684CO2<\/sub>RR\u4ea7\u7269FE\u5206\u522b\u5728Ni-SAC\u30012D-Bi\u548cCu NPs\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u4e2d\u8fdb\u884c\u7535\u5316\u5b66\u6d4b\u8bd5\uff1b<\/p>\n

\uff08j-l\uff09\u5177\u6709Ni-SAC\u30012D-Bi\u548cCu NPs\u7684PSE\u53cd\u5e94\u5668\u7684CO2<\/sub>\u56de\u6536\u6027\u80fd\u3002<\/p>\n

\u56fe\u516d\u3001\u8fde\u7eedCO2<\/sub>\u6c14\u4f53\u56de\u6536\u7684DI\u6c34\u5faa\u73af\u548c\u7a33\u5b9a\u6027\u6d4b\u8bd5<\/strong>
\n \"\"\uff08a\uff09\u7528\u4e8eCO2\u6c14\u4f53\u56de\u6536\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u53cd\u5e94\u5668\u7cfb\u7edf\u7684\u56fe\u50cf\u548c\u7535\u6c60\u8fd0\u884c\u524dAg NW\u50ac\u5316\u5242\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u7535\u6c60\u5728250\u2009 mA\uff08100\u2009mA\u2009cm-2<\/sup>\uff09\u4e0b\u8fd0\u884c90\u2009 min\u540e\uff0c\u56de\u6536\u7684CO2<\/sub>\u586b\u5145\u4e86\u4e00\u4e2a100 ml\u7684\u6c14\u7403\uff1b<\/p>\n

\uff08c\uff09250 mA\u2009cm-2<\/sup>\u6216100\u2009mA\u2009cm-2<\/sup>\u4e0b750\u2009 h\u7684CO2<\/sub>\u56de\u6536\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002<\/p>\n

\u56fe\u4e03\u3001\u5229\u7528\u56de\u6536\u4ea4\u53c9CO2<\/sub>\u63d0\u9ad8CO2<\/sub>\u8f6c\u5316\u7387<\/strong>
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\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aRecovering carbon losses in CO2<\/sub> electrolysis using a solid electrolyte reactor<\/a><\/strong>. Nature Catalysis<\/em>, 2022<\/strong>, DOI: 10.1038\/s41929-022-00763-w.<\/p>\n

\u56e2\u961f\u4ecb\u7ecd\uff1a<\/strong><\/p>\n

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