{"id":234900,"date":"2022-03-22T06:31:31","date_gmt":"2022-03-21T22:31:31","guid":{"rendered":"\/\/m.iemloyee.com\/?p=234900"},"modified":"2022-03-21T22:47:14","modified_gmt":"2022-03-21T14:47:14","slug":"%e8%a5%bf%e5%ae%89%e5%bb%ba%e5%a4%a7%e5%a7%9a%e5%b0%a7%e5%9b%a2%e9%98%9fchem-eng-j-%ef%bc%9a%e6%9e%84%e5%bb%bag-c3-6n4%e5%9f%ba%e5%8a%9f%e8%83%bd%e6%9f%94%e6%80%a7%e5%85%89%e7%94%b5%e5%ad%90","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=234900","title":{"rendered":"\u897f\u5b89\u5efa\u5927\u59da\u5c27\u56e2\u961fChem. Eng. J.\uff1a\u6784\u5efag-C3.6N4\u57fa\u529f\u80fd\u67d4\u6027\u5149\u7535\u5b50\u8584\u819c\uff0c\u5b9e\u73b0\u4f18\u5f02\u7684\u5149\u6d3b\u6027\u6297\u83cc\u6027\u80fd"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u6162\u6027\u4f24\u53e3\u5df2\u7ecf\u53d1\u5c55\u6210\u4e3a\u5168\u7403\u516c\u4f17\u5065\u5eb7\u95ee\u9898\uff0c\u7ec6\u83cc\u611f\u67d3\u662f\u5bfc\u81f4\u6162\u6027\u4f24\u53e3\u7684\u4e3b\u8981\u56e0\u7d20\u4e4b\u4e00\u3002\u6297\u751f\u7d20\u4f5c\u4e3a\u4e00\u79cd\u6709\u6548\u7684\u3001\u53ef\u5de5\u4e1a\u5316\u7684\u6297\u83cc\u5242\uff0c\u5728\u9632\u6b62\u7ec6\u83cc\u7684\u6e17\u900f\u548c\u5fae\u751f\u7269\u7684\u751f\u957f\u65b9\u9762\u53d1\u6325\u7740\u91cd\u8981\u4f5c\u7528\u3002\u7136\u800c\uff0c\u6700\u8fd1\u7684\u7814\u7a76\u8868\u660e\uff0c\u6297\u751f\u7d20\u4e0d\u4ec5\u53d7\u5230\u6297\u751f\u7d20\u8010\u836f\u6027\u7684\u9650\u5236\uff0c\u800c\u4e14\u96be\u4ee5\u964d\u89e3\uff0c\u5bf9\u4eba\u4f53\u5065\u5eb7\u6784\u6210\u6f5c\u5728\u5a01\u80c1\u3002\u65e0\u91d1\u5c5e\u5149\u50ac\u5316\u5242\u4f5c\u4e3a\u4e00\u79cd\u53ef\u66ff\u4ee3\u7b56\u7565\u5728\u6297\u83cc\u65b9\u9762\u5177\u6709\u5e7f\u9614\u7684\u5e94\u7528\u524d\u666f\uff0c\u4f46\u5e38\u7528\u65e0\u91d1\u5c5e\u5149\u50ac\u5316\u5242\u5982g-C3<\/sub>N4<\/sub>\u5b58\u5728\u5149\u751f\u7535\u5b50-\u7a7a\u7a74\u5bf9\u6613\u590d\u5408\u3001\u53ef\u89c1\u5149\u5438\u6536\u5f31\u7b49\u56fa\u6709\u95ee\u9898\u3002\u56e0\u6b64\uff0c\u5355-\u6709\u673a\u7ec4\u5206\u5149\u50ac\u5316\u5242\u5728\u5149\u50ac\u5316\u6297\u83cc\u65b9\u9762\u4ecd\u662f\u4e00\u4e2a\u91cd\u8981\u7684\u6311\u6218\u3002<\/p>\n

\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u897f\u5b89\u5efa\u7b51\u79d1\u6280\u5927\u5b66\u59da\u5c27\u56e2\u961f\u5728\u300aChemical Engineering Journal\u300b\u671f\u520a\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cSingle-organic component g-C3.6<\/sub>N4<\/sub>\u00a0Achieves Superior Photoactivity Antibacterial\u201d\u7684\u6587\u7ae0\uff08DOI:\u00a010.1016\/j.cej.2022.135873\uff09\u3002\u4e3a\u514b\u670d\u65e0\u91d1\u5c5e\u5149\u50ac\u5316\u5242\u5149\u751f\u7535\u5b50-\u7a7a\u7a74\u5bf9\u6613\u590d\u5408\u3001\u53ef\u89c1\u5149\u5438\u6536\u5f31\u7684\u95ee\u9898\uff0c\u5e76\u5b9e\u73b0\u5149\u50ac\u5316\u6750\u6599\u5728\u4f24\u53e3\u6577\u6599\u9886\u57df\u7684\u5e94\u7528\uff0c\u8be5\u8bfe\u9898\u7ec4\u8bbe\u8ba1\u5236\u5907\u4e86\u4e00\u7c7b\u65b0\u9896\u7ed3\u6784\u5149\u50ac\u5316\u5242g-C3.6<\/sub>N4<\/sub>\uff0c\u5e76\u4ee5PVA\u4e3a\u57fa\u6750\uff0c\u91c7\u7528\u7b80\u5355\u7684\u65b9\u6cd5\u5408\u6210\u4e86g-C3.6<\/sub>N4<\/sub>\/PVA\u67d4\u6027\u5149\u7535\u5b50\u8584\u819c\uff0c\u5b9e\u73b0\u4f18\u5f02\u7684\u5149\u6d3b\u6027\u6297\u83cc\u6027\u80fd\u3002\u897f\u5b89\u5efa\u7b51\u79d1\u6280\u5927\u5b66\u59da\u5c27\u6559\u6388\uff0c\u5218\u864e\u535a\u58eb\u548c\u5f20\u826f\u6559\u6388\u7b49\u4e3a\u8bba\u6587\u7684\u901a\u8baf\u4f5c\u8005\uff0c\u5317\u4eac\u5de5\u5546\u5927\u5b66\u9a6c\u632f\u8f89\u6559\u6388\u548c\u7518\u8083\u4e2d\u533b\u836f\u5927\u5b66\u548c\u5efa\u653f\u535a\u58eb\u5206\u522b\u4e3a\u8bba\u6587\u7684\u7406\u8bba\u8ba1\u7b97\u548c\u751f\u7269\u5b66\u8868\u5f81\u5de5\u4f5c\u63d0\u4f9b\u4e86\u6307\u5bfc\u548c\u5e2e\u52a9\uff0c\u897f\u5b89\u5efa\u7b51\u79d1\u6280\u5927\u5b662020\u7ea7\u7855\u58eb\u751f\u82d7\u82e5\u5ca9\u4e3a\u8bba\u6587\u7684\u7b2c\u4e00\u4f5c\u8005\u3002<\/p>\n

\"\"<\/p>\n

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\u4e09\u3001\u3010\u672c\u6587\u8981\u70b9\u3011<\/strong><\/p>\n

1) \u7406\u8bba\u8ba1\u7b97\u5f15\u5bfc\u7684\u6750\u6599\u8bbe\u8ba1<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe1\u00a0g-C3<\/sub>N4<\/sub>\u548cg-C3.6<\/sub>N4<\/sub>\u7684 (a) PDOS\u8ba1\u7b97\uff1b(b)\u00a0HOMO\u8f68\u9053\u548cLUMO\u8f68\u9053\uff1b(c)\u00a0\u754c\u9762\u7684bader\u7535\u8377\u5206\u6790\u3002<\/p>\n

\u8be5\u7814\u7a76\u9996\u5148\u901a\u8fc7\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba(DFT)\u8ba1\u7b97\u7814\u7a76\u4e86g-C3<\/sub>N4<\/sub>\u548cg-C3.6<\/sub>N4<\/sub>\u754c\u9762\u7684\u7535\u8377\u8f6c\u79fb\u548c\u7535\u8377\u5206\u5e03\u7279\u6027\uff0c\u8fdb\u4e00\u6b65\u6307\u5bfc\u4e86\u6750\u6599\u7684\u6269\u5c55\u5e94\u7528\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u5e2d\u592b\u78b1\u952e\u7684\u5f15\u5165\u4f7fmelem\u73af\u5171\u8f6d\u589e\u5927\uff0c\u4f7fC\u539f\u5b50\u5f62\u6210\u53cc\u952e\uff0c\u5931\u53bb\u7684\u7535\u5b50\u66f4\u5c11\uff0c\u5177\u6709\u660e\u663e\u7684\u975e\u6781\u6027(\u56fe1c)\u3002\u56feg-C3<\/sub>N4<\/sub>\u548cg-C3.6<\/sub>N4<\/sub>\u7684\u6700\u9ad8\u5360\u636e\u5206\u5b50\u8f68\u9053(HOMO)\u548c\u6700\u4f4e\u5360\u636e\u5206\u5b50\u8f68\u9053(LUMO)\u7684\u5206\u5e03\u56fe\u4e5f\u663e\u793a\u4e86\u5728\u5149\u50ac\u5316\u8fc7\u7a0b\u4e2d\uff0c\u4e0eg-C3<\/sub>N4<\/sub>\u76f8\u6bd4\uff0cg-C3.6<\/sub>N4<\/sub>\u7684HOMO\u8f68\u9053\u548cLUMO\u8f68\u9053\u5206\u5e03\u660e\u663e\u79bb\u6563\uff0c\u6709\u5229\u4e8e\u5149\u751f\u7535\u5b50\u7684\u5feb\u901f\u8f6c\u79fb\uff0c\u964d\u4f4e\u5149\u751f\u7535\u5b50-\u7a7a\u7a74\u590d\u5408\u6982\u7387(\u56fe1b)\u3002<\/p>\n

2)\u00a0\u5f62\u8c8c\u8868\u5f81\u53ca\u529b\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe2 (a-b) PVA\u7684\u626b\u9762\u7535\u955c\u56fe\uff1b(c-d) g-C3.6<\/sub>N4<\/sub>\/PVA\u7684\u626b\u63cf\u7535\u955c\u56fe\uff1b(e-h) g-C3.6<\/sub>N4<\/sub>\/PVA\u7684\u5143\u7d20\u5206\u5e03\u56fe\uff1b(i-j) g-C3.6<\/sub>N4<\/sub>\/PVA\u7684\u5149\u5b66\u56fe\u50cf\uff1b(k-l) g-C3.6<\/sub>N4<\/sub>\/PVA\u7684\u9ecf\u9644\u6027\u548c\u67d4\u6027;\u00a0g-C3.6<\/sub>N4<\/sub>\/PVA\u6c34\u51dd\u80f6\u819c\u62c9\u4f38\u8bd5\u9a8c\uff1a(m)\u62c9\u4f38\u524d\uff0c(n)\u62c9\u4f38\u540e\u3002<\/p>\n

\u4e3a\u4e86\u8fdb\u4e00\u6b65\u63a2\u7a76\u6750\u6599\u4f5c\u4e3a\u4f24\u53e3\u6577\u6599\u7684\u5e94\u7528\u6f5c\u529b\uff0c\u901a\u8fc7SEM(\u56fe2a-h)\u53ca\u529b\u5b66\u8868\u5f81(\u56fe2i-n)\u5206\u6790\u4e86\u6750\u6599\u7684\u5f62\u8c8c\u53ca\u7c98\u9644\u529b\u548c\u62c9\u4f38\u80fd\u529b\u3002\u7ed3\u679c\u8868\u660e\uff0cPVA\u6c34\u51dd\u80f6\u758f\u677e\u591a\u5b54\u7684\u7ed3\u6784\u4e3ag-C3.6<\/sub>N4<\/sub>\u7684\u8d1f\u8f7d\u63d0\u4f9b\u4e86\u5e73\u53f0\u3002\u5f62\u6210\u7684g-C3.6<\/sub>N4<\/sub>\/PVA\u6c34\u51dd\u80f6\u53ef\u4ee5\u4e3a\u5149\u50ac\u5316\u8fc7\u7a0b\u63d0\u4f9b\u6c34\u73af\u5883\uff0c\u6709\u5229\u4e8eROS\u7684\u4ea7\u751f\uff0c\u4e14\u5f62\u6210\u7684\u6c34\u51dd\u80f6\u5177\u6709\u4e00\u5b9a\u7684\u7c98\u9644\u529b\u548c\u67d4\u6027\uff0c\u80fd\u591f\u6ee1\u8db3\u5728\u4f24\u53e3\u4e0a\u7684\u5e94\u7528\u3002<\/p>\n

3) \u5149\u50ac\u5316\u673a\u5236<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe3\u00a0(a) UV-vis\uff1b(b)\u00a0Kubelka-Munk\u51fd\u6570\u56fe\uff1b(c)\u00a0Mott-Schottky\uff1b(d)\u00a0\u91c7\u7528\u5149\u5b66\u5438\u6536\u6cd5\u548c\u7535\u5316\u5b66Mott-Schottky\u6cd5\u8ba1\u7b97\u7684g-C3<\/sub>N4<\/sub>\/PVA\u548cg-C3.6<\/sub>N4<\/sub>\/PVA\u7684\u80fd\u5e26\u6c34\u5e73\u3002<\/p>\n

\"\"<\/p>\n

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4) \u5149\u50ac\u5316\u6297\u83cc\u6d3b\u6027<\/strong><\/p>\n

\"\"<\/p>\n

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