{"id":234118,"date":"2022-03-13T06:15:20","date_gmt":"2022-03-12T22:15:20","guid":{"rendered":"\/\/m.iemloyee.com\/?p=234118"},"modified":"2022-03-12T21:31:02","modified_gmt":"2022-03-12T13:31:02","slug":"%e5%94%90%e5%86%9b%e6%97%ba-nature-reviews-materials%ef%bc%9a%e5%85%89%e5%82%ac%e5%8c%96%e7%94%b2%e7%83%b7%e8%bd%ac%e5%8c%96%e6%9c%80%e6%96%b0%e8%bf%9b%e5%b1%95%ef%bc%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=234118","title":{"rendered":"\u5510\u519b\u65fa Nature Reviews Materials\uff1a\u5149\u50ac\u5316\u7532\u70f7\u8f6c\u5316\u6700\u65b0\u8fdb\u5c55\uff01"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u968f\u7740\u539f\u6cb9\u50a8\u91cf\u7684\u4e0b\u964d\uff0c\u9700\u8981\u5229\u7528\u7532\u70f7\u4ee3\u66ff\u77f3\u6cb9\u4f5c\u4e3a\u5316\u5b66\u5408\u6210\u7684\u57fa\u77f3\u3002\u5c06\u7532\u70f7\u53ef\u4ee5\u76f4\u63a5\u8f6c\u5316\u4e3a\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u71c3\u6599\u548c\u5316\u5b66\u54c1\uff0c\u4f46\u5728\u5546\u4e1a\u89c4\u6a21\u4e0a\u5c1a\u4e0d\u80fd\u5b9e\u73b0\u3002\u7531\u4e8e\u7532\u70f7\u7684\u5bf9\u79f0\u6027\u56db\u9762\u4f53\u3001\u4f4e\u6781\u5316\u7387\u548c\u9ad8C-H\u952e\u80fd\uff0c\u5176\u4f20\u7edf\u8f6c\u5316\u6cd5\u9700\u8981\u82db\u523b\u7684\u53cd\u5e94\u6761\u4ef6\u548c\u5f3a\u6c27\u5316\u5242\uff0c\u5e76\u4e14\u4f1a\u4ea7\u751f\u8fc7\u91cf\u7684CO2<\/sub>\u6392\u653e\u3002\u5728\u5982\u6b64\u6076\u52a3\u7684\u6761\u4ef6\u4e0b\uff0c\u7ecf\u5e38\u4f1a\u53d1\u751f\u7126\u70ad\u7684\u5feb\u901f\u5806\u79ef\u548c\u50ac\u5316\u5242\u7684\u70e7\u7ed3<\/strong><\/span>\uff0c\u4ece\u800c\u5bfc\u81f4\u50ac\u5316\u5242\u5931\u6d3b\u3002\u56e0\u6b64\uff0c\u9700\u8981\u5f00\u53d1\u6709\u6548\u548c\u7eff\u8272\u7684\u65b9\u6cd5\uff0c\u5c06\u7532\u70f7\u76f4\u63a5\u8f6c\u5316\u4e3a\u6709\u4ef7\u503c\u7684\u5316\u5b66\u54c1\u3002\u5149\u50ac\u5316\uff08photocatalysis\uff09\u662f\u4f20\u7edf\u70ed\u50ac\u5316\u7684\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u66ff\u4ee3\u65b9\u6cd5\uff0c\u5176\u5229\u7528\u5149\u5b50\u800c\u4e0d\u662f\u70ed\u80fd\u6765\u9a71\u52a8\u5316\u5b66\u8fc7\u7a0b\u3002\u7531\u4e8e\u7532\u70f7\u7684\u60f0\u6027\uff0c\u901a\u8fc7\u70ed\u50ac\u5316\u8f6c\u5316\u7532\u70f7\u9700\u8981\u5f88\u5927\u7684\u6d3b\u5316\u80fd\uff0c\u800c\u5149\u50ac\u5316\u4ea7\u751f\u975e\u5e38\u9ad8\u80fd\u7684\u7535\u8377\u8f7d\u4f53\uff0c\u9884\u6d3b\u5316\u7532\u70f7\u5e76\u5927\u5e45\u964d\u4f4e\u6d3b\u5316\u80fd\u3002\u6b64\u5916\uff0c\u5149\u50ac\u5316\u53cd\u5e94\u7406\u8bba\u4e0a\u53ef\u4ee5\u907f\u514d\u82db\u523b\u7684\u53cd\u5e94\u6761\u4ef6\u3001\u8fc7\u5ea6\u6c27\u5316\u548c\u50ac\u5316\u5242\u5931\u6d3b\uff0c\u53cd\u5e94\u4ea7\u751f\u7684\u70ed\u91cf\u4e5f\u53ef\u4ee5\u5f88\u5bb9\u6613\u5730\u6d88\u6563\u3002\u56e0\u6b64\uff0c\u51e0\u4e4e\u6240\u6709\u70ed\u70b9\u4ea7\u54c1\u90fd\u53ef\u4ee5\u5b9e\u73b0\u9009\u62e9\u6027>90%\u751a\u81f3100%\u7684\u5149\u50ac\u5316\u7cfb\u7edf\u3002
\n \"\"
\n \u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u82f1\u56fd\u4f26\u6566\u5927\u5b66\u5510\u519b\u65fa\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u7bc7\u5173\u4e8e\u5149\u50ac\u5316\u7532\u70f7\u8f6c\u5316\u6700\u65b0\u8fdb\u5c55\u7684\u7efc\u8ff0\u3002\u5728\u6587\u4e2d\uff0c\u4f5c\u8005\u4ecb\u7ecd\u4e86\u5149\u50ac\u5316\u5242\u548c\u52a9\u50ac\u5316\u5242\u7684\u53d1\u5c55\uff0c\u4ee5\u5168\u9762\u7814\u7a76\u63d0\u9ad8\u6240\u9700\u4ea7\u54c1\u7684\u9009\u62e9\u6027\u548c\u4ea7\u7387\u4ee5\u53ca\u50ac\u5316\u5242\u7a33\u5b9a\u6027\u7684\u7b56\u7565\u3002\u63a5\u7740\uff0c\u4f5c\u8005\u89e3\u91ca\u4e86\u95f4\u6b47\u6216\u6d41\u52a8\u53cd\u5e94\u7cfb\u7edf\u7684\u8bbe\u8ba1\u4e0e\u6027\u80fd\uff0c\u4ee5\u53ca\u5982\u4f55\u5f71\u54cd\u53cd\u5e94\u52a8\u529b\u5b66\u548c\u4ea7\u54c1\u9009\u62e9\u6027\uff0c\u5e76\u8ba8\u8bba\u4e86\u7814\u7a76\u5149\u7269\u7406\u548c\u8868\u9762\u5316\u5b66\u53cd\u5e94\u673a\u5236\u53d6\u5f97\u7684\u8fdb\u5c55\u3002\u6700\u540e\uff0c\u4f5c\u8005\u63d0\u51fa\u4e86\u5176\u5bf9\u8be5\u9886\u57df\u9762\u4e34\u7684\u6311\u6218\u7684\u770b\u6cd5\uff0c\u5e76\u63d0\u51fa\u4e86\u6f5c\u5728\u7684\u89e3\u51b3\u65b9\u6848\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cMethane transformation by photocatalysis\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Reviews Materials<\/em>\u4e0a\u3002<\/p>\n

\u672c\u6587\u6240\u6709\u56fe\u6765\u6e90\u4e8e\u00a9 2022 Springer Nature Limited\u3002<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

\u221a\u901a\u8fc7\u4ecb\u7ecd\u65e0\u673a\u6750\u6599\u3001\u805a\u5408\u7269\u534a\u5bfc\u4f53\u7b49\u5149\u50ac\u5316\u5242\u548c\u52a9\u50ac\u5316\u5242\uff0c\u603b\u7ed3\u4e86\u63d0\u9ad8\u9009\u62e9\u6027\u548c\u4ea7\u7387\u3001\u7a33\u5b9a\u6027<\/strong><\/span>\u7684\u7b56\u7565<\/p>\n

\u221a\u89e3\u91ca\u4e86\u95f4\u6b47\u6216\u6d41\u52a8\u53cd\u5e94\u7cfb\u7edf<\/span><\/strong>\u5982\u4f55\u5f71\u54cd\u53cd\u5e94\u52a8\u529b\u5b66\u548c\u4ea7\u54c1\u9009\u62e9\u6027<\/p>\n

\u221a\u5206\u6790\u4e86\u7814\u7a76\u5149\u7269\u7406\u548c\u8868\u9762\u5316\u5b66\u53cd\u5e94\u673a\u5236<\/span><\/strong>\u7684\u8fdb\u5c55<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

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\n \"\"\uff08a\uff09\u5728\u5ba4\u6e29\u4e0b\u8fdb\u884c\u7684\u7532\u70f7\u8f6c\u5316\u7684\u70ed\u529b\u5b66\u4e0d\u5229\uff08\u0394G>0\uff09\u548c\u6709\u5229\uff08\u0394G<0\uff09\u53cd\u5e94\u9014\u5f84\uff1b<\/p>\n

\uff08b\uff09\u5149\u50ac\u5316\u7684\u539f\u7406\u5305\u62ec\u5149\u7167\u3001\u7535\u5b50\u4ece\u4ef7\u5e26\u6fc0\u53d1\u5230\u5bfc\u5e26\u3001\u7535\u8377\u5206\u79bb\u548c\u4f20\u8f93\u5230\u53cd\u5e94\u4f4d\u70b9\u3001\u8868\u9762\u53cd\u5e94\u548c\u8868\u9762\u7535\u8377\u91cd\u7ec4\uff1b<\/p>\n

\uff08c\uff09\u4e0d\u540c\u7684\u5149\u50ac\u5316\u673a\u5236\u6d3b\u5316\u7532\u70f7<\/p>\n

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\"\"<\/p>\n

\u56fe\u4e09\u3001\u5149\u50ac\u5316\u7532\u70f7\u8f6c\u5316\u4e2d\u7684\u4ee3\u8868\u6027\u53cd\u5e94\u4f53\u7cfb<\/strong>
\n \"\"\uff08a\uff09\u5177\u6709\u5faa\u73af\u6cf5\u7684\u95f4\u6b47\u5f0f\u53cd\u5e94\u5668\u6539\u5584\u7532\u70f7\u7684\u4f20\u8d28\uff1b<\/p>\n

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\uff08c\uff09\u6d41\u52a8\u53cd\u5e94\u5668\u88ab\u62a5\u9053\u7528\u4e8e\u7532\u70f7\u53cd\u5e94\u7684\u5149\u50ac\u5316\u6c27\u5316\u5076\u8054\uff1b<\/p>\n

\uff08d\uff09\u91c7\u7528\u4e24\u76f8\u53cd\u5e94\u4f53\u7cfb\uff0c\u901a\u8fc7NaClO2<\/sub>\u5bf9CH4<\/sub>\u8fdb\u884c\u5149\u6c27\u5316\uff1b<\/p>\n

\uff08e\uff09\u5316\u5b66\u56de\u8def\u7528\u4e8e\u901a\u8fc7Ag-H3<\/sub>PW12<\/sub>O40<\/sub>\/TiO2<\/sub>\u5c06\u5316\u5b66\u8ba1\u91cf\u7684\u7532\u70f7\u8f6c\u5316\u4e3a\u4e59\u70f7<\/p>\n

\u56fe\u56db\u3001\u4e92\u8865\u65f6\u95f4\u5206\u8fa8\u5149\u8c31\u63a2\u6d4b\u5149\u50ac\u5316\u5242\u4e2d\u7684\u5149\u7269\u7406\u548c\u5149\u5316\u5b66\u8fc7\u7a0b<\/strong>
\n \"\"\uff08a\uff09\u65f6\u95f4\u5206\u8fa8\u7ea2\u5916\u5149\u8c31\uff08TRIR\uff09\u3001\u77ac\u6001\u5438\u6536\u5149\u8c31\uff08TAS\uff09\u548c\u65f6\u95f4\u5206\u8fa8\u62c9\u66fc\u5149\u8c31\uff08TRRS\uff09\u7684\u64cd\u4f5c\u548c\u89c2\u5bdf\u7a97\u53e3\u3001\u65f6\u95f4\u5c3a\u5ea6\u548c\u4e3b\u9898\uff1b<\/p>\n

\uff08b\uff09\u6fc0\u53d1\u540e\u65f6\u95f4\u5206\u8fa8\u62c9\u66fc\u5149\u8c31\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

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\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aMethane transformation by photocatalysis<\/a><\/strong>. Nature Reviews Materials<\/em>, 2022<\/strong>, DOI: 10.1038\/s41578-022-00422-3.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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