{"id":233003,"date":"2022-02-16T06:18:17","date_gmt":"2022-02-15T22:18:17","guid":{"rendered":"\/\/m.iemloyee.com\/?p=233003"},"modified":"2022-02-15T20:30:21","modified_gmt":"2022-02-15T12:30:21","slug":"nat-chem-%ef%bc%9a%e6%b4%bb%e6%80%a7%e5%8f%af%e4%bf%ae%e5%a4%8d%e7%9a%84%e5%8f%8c%e6%a0%b8%e5%8f%af%e8%a7%81%e5%85%89%e5%82%ac%e5%8c%96%e5%88%b6%e6%b0%a2%e5%82%ac%e5%8c%96%e5%89%82","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=233003","title":{"rendered":"Nat. Chem.\uff1a\u6d3b\u6027\u53ef\u4fee\u590d\u7684\u53cc\u6838\u53ef\u89c1\u5149\u50ac\u5316\u5236\u6c22\u50ac\u5316\u5242"},"content":{"rendered":"<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233180\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/0-6.jpg\" alt=\"\" width=\"600\" height=\"266\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/0-6.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/0-6-300x133.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n<p>\u5c06\u592a\u9633\u80fd\u76f4\u63a5\u8f6c\u6362\u4e3a\u5316\u5b66\u80fd\u7684\u5149\u50ac\u5316\u65b9\u6cd5\uff0c\u53ef\u4ee5\u514b\u670d\u591a\u6b21\u8f6c\u6362\u8fc7\u7a0b\u4e2d\u7684\u80fd\u91cf\u635f\u5931\uff0c\u8fd9\u79cd\u65b9\u6cd5\u662f\u5f88\u6709\u524d\u9014\u7684\u3002\u5229\u7528\u5149\u5316\u5b66\u5206\u5b50\u5668\u4ef6\uff08PMDs\uff09\u5c06\u6c34\u5149\u50ac\u5316\u5206\u89e3\u4e3a\u6c27\u6c14\u548c\u6c22\u6c14\u662f\u4e00\u79cd\u975e\u5e38\u6709\u610f\u4e49\u7684\u65b9\u6cd5\u3002\u5728\u5149\u5408\u4f5c\u7528\u4e2d\uff0c\u592a\u9633\u80fd\u3001\u4e8c\u6c27\u5316\u78b3\u548c\u6c34\u53d1\u751f\u53cd\u5e94\uff0c\u751f\u6210\u6c27\u6c14\u548c\u78b3\u6c34\u5316\u5408\u7269\u3002\u53f6\u7eff\u4f53\u901a\u8fc7\u5149\u7cfb\u7edfI\u548cII\uff08\u5206\u522b\u4e3aPSI\u548cPSII\uff09\u7684\u5149\u5438\u6536\u5355\u5143\u5438\u6536\u5149\u5b50\uff0c\u4ece\u800c\u8bf1\u5bfc\u7535\u5b50\u9010\u7ea7\u8f6c\u79fb\uff0c\u4ece\u653e\u6c27\u590d\u5408\u7269\uff08OEC\uff09\u5230ferredoxin-nicotinamide adenine dinucleotide phosphate oxidoreductase\uff08FNR\uff09\uff0c\u7528\u9ad8\u80fd\u7535\u5b50\u5c06\u70df\u9170\u80fa\u817a\u560c\u5464\u4e8c\u6838\u82f7\u9178\u78f7\u9178\uff08NADP<sup>+<\/sup>\uff09\u8fd8\u539f\u4e3aNADPH\u3002\u5728\u5361\u5c14\u6587-\u672c\u68ee\u5faa\u73af\u4e2d\uff0c\u2009\u5728\u690d\u7269\u548c\u85fb\u7c7b\u5149\u5408\u4f5c\u7528\u671f\u95f4\uff0cNADPH\u5c06\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u4e3a\u7cd6\u5206\uff0c\u6bcf\u5e74\u5c06\u8f6c\u5316440 Gt\u4e8c\u6c27\u5316\u78b3\u3002\u5728\u5149\u5316\u5b66\u53cd\u5e94\u4e2d\uff0c\u86cb\u767d\u8d28D1\u662f\u6784\u6210PSII\u53cd\u5e94\u4e2d\u5fc3\u7684\u4e24\u79cd\u86cb\u767d\u8d28\u4e4b\u4e00\uff0c\u7531\u4e8e\u8fc7\u5ea6\u5149\u7167\u800c\u53d7\u5230\u4e0d\u53ef\u9006\u8f6c\u7684\u635f\u5bb3\u3002\u7136\u800c\uff0c\u53d7\u635f\u7684\u86cb\u767d\u8d28D1\u88abftsH\u548cDeg\u86cb\u767d\u9176\u89e3\u6784\uff0c\u5e76\u88ab\u65b0\u5408\u6210\u7684\u86cb\u767d\u8d28\u53d6\u4ee3\uff0c\u4ee5\u91cd\u5efaPSII\u548c\u6574\u4e2a\u5149\u5408\u4f5c\u7528\u673a\u5236\u3002\u56e0\u6b64\uff0c\u86cb\u767dD1\u7684\u6210\u5206\u727a\u7272\uff0c\u4fdd\u62a4\u6574\u4e2aPSII\u514d\u53d7\u5149\u635f\u4f24\u3002D1\u7684\u6301\u7eed\u4e3b\u52a8\u4fee\u590d\u662f\u662f\u5149\u5408\u4e2d\u5fc3\u80fd\u591f\u7ef4\u6301\u957f\u671f\u5149\u50ac\u5316\u6d3b\u6027\u7684\u539f\u56e0\u3002\u57fa\u4e8e\u81ea\u7136\u7684\u6982\u5ff5\uff0c\u8bb8\u591a\u4eba\u5de5\u7cfb\u7edf\u5df2\u7ecf\u88ab\u5f00\u53d1\u51fa\u6765\uff0c\u5c06\u5149\u5438\u6536\u5355\u5143\u548c\u50ac\u5316\u4e2d\u5fc3\u7ed3\u5408\u8d77\u6765\uff0c\u4ee5\u4fc3\u8fdb\u5149\u9a71\u52a8\u7684\u6c34\u5206\u89e3\u3002\u9664\u4e86\u6c34\u6c27\u5316\u7b56\u7565\u5916\uff0c\u8fd8\u53ef\u4ee5\u901a\u8fc7\u53ef\u89c1\u5149\u5438\u6536\u5c06\u6c34\u5149\u50ac\u5316\u8fd8\u539f\u4e3a\u6c22\u3002\u4f5c\u8005\u4e4b\u524d\u62a5\u9053\u8fc7\u4e00\u79cdPMD\u4ea7\u6c22\uff0c\u5b83\u80fd\u5728\u53ef\u89c1\u5149\uff08470\u2009 nm\uff09\u7167\u5c04\u4e0b\uff0c\u4ece\u6c34\u4e2d\u6709\u6548\u5730\u4ea7\u6c22\u3002\u8be5\u88c5\u7f6e\u57fa\u4e8e\u5206\u5b50\u5185\u65b9\u6cd5\uff0c\u5c06\u4e09\u4e2a\u529f\u80fd\u5355\u5143\u7ec4\u5408\u6210\u4e00\u4e2a\u5206\u5b50\u7269\u79cd\u3002\u8fd9\u79cd\u6a21\u5757\u5316\u6982\u5ff5\u5141\u8bb8\u5bf9\u5355\u4e2a\u7ec4\u4ef6\u8fdb\u884c\u5fae\u8c03\uff0c\u4ee5\u4f18\u5316\u6027\u80fd\uff0c\u800c\u4e0d\u4f1a\u5f71\u54cdPMD\u7684\u4e00\u822c\u529f\u80fd\u3002<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u5fb7\u56fd\u4e4c\u5c14\u59c6\u5927\u5b66<\/strong>\u7684<strong>Sven Rau<\/strong>\u548c<strong>\u8036\u62ff\u5927\u5b66<\/strong>\u7684<strong>Benjamin Dietzek-Ivan\u0161i\u0107<\/strong><strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u53d1\u73b0\u7531\u5149\u4e2d\u5fc3\u3001\u6865\u914d\u4f53\u548c\u50ac\u5316\u4e2d\u5fc3\u7ec4\u6210\u7684\u7528\u4e8e\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u7684\u4eff\u751f\u5206\u5b50\u88c5\u7f6e\uff0c\u5728\u5176\u5355\u4e2a\u6a21\u5757\u7ed3\u6784\u53d7\u635f\u65f6\uff0c\u53ef\u80fd\u4f1a\u53d8\u5f97\u4e0d\u7a33\u5b9a\u5e76\u53d1\u751f\u6545\u969c\uff0c\u4ece\u800c\u505c\u6b62\u5176\u6574\u4f53\u529f\u80fd\u548c\u8fd0\u884c\u3002\u672c\u6587\u62a5\u544a\u4e86\u4e00\u79cd\u4e3b\u52a8\u4fee\u590d\u7684\u4eba\u5de5\u5149\u5408\u5206\u5b50\u88c5\u7f6e\uff0c\u53ef\u4ee5\u5b8c\u5168\u6062\u590d\u50ac\u5316\u6d3b\u6027\u3002\u672c\u6587\u786e\u5b9a\u5931\u6d3b\u673a\u5236\u662f\u6865\u914d\u4f53\u7684\u6c22\u5316\u4f5c\u7528\uff0c\u5b83\u6291\u5236\u5149\u4e2d\u5fc3\u548c\u50ac\u5316\u4e2d\u5fc3\u4e4b\u95f4\u7684\u5149\u9a71\u52a8\u7535\u5b50\u8f6c\u79fb\u3002\u672c\u6587\u91c7\u7528\u5149\u9a71\u52a8\u7684\u5355\u7ebf\u6001\u6c27\u751f\u6210\uff0c\u5728\u5149\u4e2d\u5fc3\u7684\u50ac\u5316\u4e0b\uff0c\u5b9e\u73b0\u6865\u63a5\u5355\u5143\u7684\u6c27\u5316\u8131\u6c22\uff0c\u4ece\u800c\u6062\u590d\u5149\u50ac\u5316\u5236\u6c22\u3002\u76f8\u5173\u6210\u679c\u4ee5<strong>\u201c<\/strong><strong>Active repair of a dinuclear photocatalyst for visible-light-driven hydrogen production<\/strong>\u201d\u53d1\u8868\u5728<em><strong>Nature Chemistry<\/strong><\/em>\u4e0a\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p><strong>\u56fe<\/strong><strong> 1 <\/strong><strong>\u53ef\u89c1\u5149\u9a71\u52a8\u7684<\/strong><strong>PMD<\/strong><strong>\u5236\u6c22\u00a0<\/strong><span style=\"color: #999999;\"><strong>\u00a92022 Springer Nature<\/strong><\/span><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233181\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig1_HTML.webp_.jpg\" alt=\"\" width=\"600\" height=\"1071\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig1_HTML.webp_.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig1_HTML.webp_-168x300.jpg 168w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig1_HTML.webp_-574x1024.jpg 574w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09Ru(tpphz)PtI<sub>2<\/sub>\u5149\u50ac\u5316\u5242\u7684\u5206\u5b50\u7ed3\u6784\uff1b<\/p>\n<p>\uff08b\uff09Ru(tpphz)PtI<sub>2<\/sub>\u5149\u50ac\u5316\u5236\u6c22<\/p>\n<p><strong>\u56fe<\/strong><strong> 2 <\/strong><strong>\u4e0d\u540c\u8f90\u7167\u65f6\u95f4\u4e0b\u50ac\u5316\u6eb6\u6db2\u7684\u7d2b\u5916<\/strong><strong>&#8211;<\/strong><strong>\u53ef\u89c1\u5438\u6536\u5149\u8c31\u00a0<span style=\"color: #999999;\">\u00a92022 Springer Nature<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233182\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig2_HTML.webp_.jpg\" alt=\"\" width=\"600\" height=\"306\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig2_HTML.webp_.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig2_HTML.webp_-300x153.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u56fe<\/strong><strong> 3 <\/strong><strong>\u4e0d\u540c\u8f90\u7167\u65f6\u95f4\u4e0b\u50ac\u5316\u6eb6\u6db2\u7684\u7d2b\u5916<\/strong><strong>&#8211;<\/strong><strong>\u53ef\u89c1\u5149\u8c31\u548c\u8d85\u5feb\u77ac\u6001\u5438\u6536\u5149\u8c31 \u00a0<span style=\"color: #999999;\">\u00a92022 Springer Nature<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233184\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig3_HTML.webp_.jpg\" alt=\"\" width=\"600\" height=\"463\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig3_HTML.webp_.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig3_HTML.webp_-300x232.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a-d\uff090.5\u79d2\u540e\u50ac\u5316\u6eb6\u6db2\u7684\u539f\u4f4d\u77ac\u6001\u5438\u6536\u5149\u8c31\uff1b<\/p>\n<p>\uff08e\uff090.5\u79d2\u540e\u50ac\u5316\u6eb6\u6db2\u7684\u7a33\u6001\u5438\u6536\u5149\u8c31<\/p>\n<p><strong>\u56fe<\/strong><strong> 4 <\/strong><strong>\u5931\u6d3b\u5149\u50ac\u5316\u5242<\/strong><strong>Ru(tpphzH<sub>2<\/sub>)PtI<sub>2<\/sub><\/strong><strong>\u5355\u91cd\u6001\u6c27\u8131\u6c22\u7684\u7d2b\u5916<\/strong><strong>&#8211;<\/strong><strong>\u53ef\u89c1\u5438\u6536\u5149\u8c31 \u00a0<span style=\"color: #999999;\">\u00a92022 Springer Nature<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233185\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig4_HTML.webp_.jpg\" alt=\"\" width=\"600\" height=\"433\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig4_HTML.webp_.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig4_HTML.webp_-300x217.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u56fe<\/strong><strong> 5<\/strong> <strong>Ru(tpphzH<sub>2<\/sub>)PtI<sub>2<\/sub><\/strong><strong>\u5149\u50ac\u5316\u5242\u7684\u6d3b\u6027\u4fee\u590d \u00a0<span style=\"color: #999999;\">\u00a92022 Springer Nature<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-233186\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig5_HTML.webp_.jpg\" alt=\"\" width=\"600\" height=\"1006\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig5_HTML.webp_.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2022\/02\/41557_2021_860_Fig5_HTML.webp_-179x300.jpg 179w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09\u6d3b\u6027\u548c\u975e\u6d3b\u6027\u5f62\u5f0f\u7684\u5149\u50ac\u5316\u5242Ru(bptz)PtCl<sub>2<\/sub>\u7684\u5206\u5b50\u7ed3\u6784\uff1b<\/p>\n<p>\uff08b\uff09\u5728470 nm\u7684LED\u7167\u660e140 h\u65f6\uff0cTONs\u7528\u4e8e\u6c22\u6c14\u7684\u751f\u6210<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>\u672c\u6587\u53d1\u73b0\u4e86\u4e00\u79cd\u76ee\u524d\u8fd8\u672a\u88ab\u62a5\u9053\u8fc7\u7684\u4e3b\u52a8\u4fee\u590d\u673a\u5236\uff0c\u53ef\u4ee5\u663e\u8457\u5ef6\u957f\u4eba\u5de5\u5149\u50ac\u5316\u5242\u7684\u6d3b\u6027\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u56e0\u4e3a\u6865\u8054\u914d\u4f53\u7684\u53ef\u9006\u6c22\u5316\uff0c\u5149\u50ac\u5316\u5242\u4e0d\u4f1a\u56e0\u4e3a\u5316\u5408\u7269\u7684\u5206\u89e3\u800c\u5931\u6d3b\u3002\u539f\u5219\u4e0a\uff0c\u8be5\u4e3b\u52a8\u4fee\u590d\u7a0b\u5e8f\u53ef\u9002\u7528\u4e8e\u6ee1\u8db3\u4ee5\u4e0b\u8981\u6c42\u7684\u6bcf\u4e2a\u5149\u50ac\u5316\u6d3b\u6027PMD\uff1a<span style=\"color: #003366;\"><strong>\uff081\uff09\u5149\u50ac\u5316\u5242\u5fc5\u987b\u5728\u5355\u4e2a\u6a21\u5757\u6216\u7ec4\u4ef6\u7684\u7a33\u5b9a\u8fde\u63a5\u65b9\u9762\u5177\u6709\u5316\u5b66\u7a33\u5b9a\u6027\uff1b\uff082\uff09\u5931\u6d3b\u8fc7\u7a0b\u53ca\u5176\u4ea7\u54c1\u5fc5\u987b\u662f\u53ef\u8bc6\u522b\u7684\uff1b\uff083\uff09\u5931\u6d3b\u8fc7\u7a0b\u5fc5\u987b\u662f\u53ef\u9006\u7684\u3002<\/strong><\/span>\u4e00\u65e6\u6ee1\u8db3\u8fd9\u4e9b\u8981\u6c42\uff0c\u5c31\u53ef\u4ee5\u5236\u5b9a\u9002\u5f53\u7684\u7ef4\u4fee\u7a0b\u5e8f\uff0c\u4f8b\u5982\u901a\u8fc7\u6dfb\u52a0\u6216\u539f\u4f4d\u751f\u6210\u7ef4\u4fee\u5242\u3002\u4f7f\u592a\u9633\u80fd\u9a71\u52a8\u5316\u5b66\u4e2d\u76f8\u5173PMD\u7684\u8bbe\u8ba1\u7b56\u7565\u5f97\u4ee5\u5b9e\u73b0\uff0c\u91cd\u70b9\u5728\u4e8e\u4e3b\u52a8\u4fee\u590d\u7684\u5e94\u7528\uff0c\u540c\u65f6\u5b9e\u73b0\u6700\u5927\u7684\u5149\u50ac\u5316\u6d3b\u6027\u3002\u8fd9\u4e3a\u81ea\u6211\u4fee\u590d\u548c\u63d0\u4f9b\u989d\u5916\u7684\u7ed3\u5408\u7403\u63d0\u4f9b\u4e86\u4e00\u79cd\u66ff\u4ee3\u65b9\u6848\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5<\/strong><a href=\"https:\/\/www.nature.com\/articles\/s41557-021-00860-6\" target=\"_blank\" rel=\"noopener\"><strong>Active repair of a dinuclear photocatalyst for visible-light-driven hydrogen production<\/strong><\/a>\uff08<em>Nature Chemistry<\/em> DOI: 10.1038\/s41557-021-00860-6\uff09\u3002<\/p>\n<p><strong>\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1a<\/strong><strong>cailiaokefu<\/strong><strong>\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n<p>\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002\u672c\u6587\u7531\u6750\u6599\u4ebaMaterials_1219\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>&nbsp; \u3010\u5f15\u8a00\u3011 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