{"id":231901,"date":"2022-01-14T06:24:35","date_gmt":"2022-01-13T22:24:35","guid":{"rendered":"\/\/m.iemloyee.com\/?p=231901"},"modified":"2022-01-13T21:24:54","modified_gmt":"2022-01-13T13:24:54","slug":"%e6%b8%af%e7%a7%91%e5%a4%a7%e9%bb%84%e5%ae%9d%e9%99%b5-sci-adv-%ef%bc%9a%e5%88%9b%e7%ba%aa%e5%bd%95%e5%80%bc%ef%bc%81%e9%9d%9e%e6%b0%b4%e7%b3%bb%e7%a6%bb%e5%ad%90%e5%87%9d%e8%83%b6%e5%ae%9e%e7%8e%b0","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=231901","title":{"rendered":"\u6e2f\u79d1\u5927\u9ec4\u5b9d\u9675 Sci. Adv.\uff1a\u521b\u7eaa\u5f55\u503c\uff01\u975e\u6c34\u7cfb\u79bb\u5b50\u51dd\u80f6\u5b9e\u73b0\u53cc\u5411\u53ef\u8c03\u70ed\u7535\u52bf"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u70ed\u6d41\u548c\u6e29\u5ea6\u7684\u7cbe\u786e\u68c0\u6d4b\u5728\u4ece\u5de5\u4e1a\u5230\u5bb6\u7528\u7684\u4f17\u591a\u5e94\u7528\u4e2d\u8d77\u7740\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u57fa\u4e8eSeebeck\u6548\u5e94\u7684\u70ed\u7535\u5668\u4ef6\uff0c\u5728\u6e29\u5dee\u2206T\u4e0b\u901a\u8fc7\u7535\u8377\u6269\u6563\u4ea7\u751f\u70ed\u7535\u538bV\uff0c\u4e3a\u76f4\u63a5\u5c06\u70ed\u8f6c\u6362\u4e3a\u7535\u63d0\u4f9b\u4e86\u4e00\u79cd\u53ef\u884c\u4e14\u7b80\u5355\u7684\u89e3\u51b3\u65b9\u6848\uff0c\u4f7f\u5176\u5177\u6709\u70ed\u611f\u5e94\u80fd\u529b\u3002\u76ee\u524d\u70ed\u7535\u6750\u6599\u6709\u9650\u7684Seebeck\u7cfb\u6570\u6781\u5927\u5730\u9650\u5236\u4e86\u5176\u70ed\u611f\u6d4b\u7075\u654f\u5ea6\uff0c\u5728\u70ed\u7535\u70ed\u6d41\u4f20\u611f\u5668\u7b49\u70ed\u7535\u5668\u4ef6\u4e2d\uff0c\u5fc5\u987b\u96c6\u6210\u5927\u91cf\u5143\u4ef6\u4ee5\u653e\u5927\u4fe1\u53f7\u8f93\u51fa\uff0c\u4f46\u901a\u5e38\u4f1a\u5bfc\u81f4\u590d\u6742\u7684\u5236\u9020\u548c\u9ad8\u6210\u672c\u3002\u540c\u65f6\uff0cSeebeck\u7cfb\u6570\u8f83\u9ad8\u7684\u7edd\u7f18\u4f53\u5177\u6709\u5f88\u4f4e\u7684\u5bfc\u7535\u7387\uff0c\u5bfc\u81f4\u6d4b\u91cf\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u8f83\u5927\u7684\u566a\u58f0\u3002\u5728\u4e0d\u727a\u7272\u5176\u4ed6\u91cd\u8981\u70ed\u7535\u6027\u80fd\u7684\u60c5\u51b5\u4e0b\u663e\u8457\u63d0\u9ad8Seebeck\u7cfb\u6570\u662f\u4e00\u4e2a\u6311\u6218\uff0c\u56e0\u4e3a\u5b83\u4eec\u5177\u6709\u5f88\u5f3a\u7684\u76f8\u4e92\u8026\u5408\u6027\u3002<\/p>\n

\u8fd1\u4e9b\u5e74\u6765\uff0c\u6c34\u6eb6\u6db2\u548c\u6709\u673a\u6eb6\u6db2\u4e2d\u7684\u79bb\u5b50\u70ed\u7535\u52bf\u5f97\u5230\u4e86\u5e7f\u6cdb\u7684\u7814\u7a76\u3002\u5927\u578b\u79bb\u5b50\u70ed\u7535\u56fa\u4f53\u7535\u89e3\u8d28\uff0c\u5c24\u5176\u662f\u805a\u5408\u7269\u51dd\u80f6\uff0c\u7531\u4e8e\u5176\u5728\u5236\u9020\u548c\u5668\u4ef6\u96c6\u6210\u65b9\u9762\u7684\u4f18\u52bf\u800c\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\u3002\u5f53\u524d\uff0c\u51e0\u4e4e\u6240\u6709\u8c03\u8282\u79bb\u5b50\u70ed\u7535\u52bf\uff08thermopower\uff09\u7b26\u53f7\u548c\u5927\u5c0f\u7684\u7b56\u7565\u90fd\u96c6\u4e2d\u5728\u8c03\u8282\u79bb\u5b50\u4e0e\u57fa\u4f53\u73af\u5883\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u4e0a\u3002\u7136\u800c\uff0c\u7531\u4e8e\u7a33\u5b9a\u6027\u548c\u673a\u68b0\u5f3a\u5ea6\u7b49\u5404\u79cd\u8003\u8651\u56e0\u7d20\uff0c\u9002\u7528\u4e8e\u7535\u89e3\u8d28\u7684\u805a\u5408\u7269\u57fa\u8d28\u53d7\u5230\u9650\u5236\uff0c\u5e76\u4e14\u6240\u9009\u805a\u5408\u7269\u57fa\u8d28\u4e0e\u79bb\u5b50\u4e4b\u95f4\u76f8\u4e92\u4f5c\u7528\u7684\u8c03\u8282\u4e5f\u5177\u6709\u6311\u6218\u6027\u3002\u5c3d\u7ba1\u5728\u5b9e\u73b0\u5de8\u5927\u7684\u79bb\u5b50\u70ed\u7535\u52bf\u65b9\u9762\u53d6\u5f97\u4e86\u91cd\u5927\u8fdb\u5c55\uff0c\u4f46\u662f\u5927\u591a\u6570\u6700\u5148\u8fdb\u7684\u79bb\u5b50\u70ed\u7535\u6750\u6599\u662fp-\u578b\u6216\u5177\u6709\u6b63\u79bb\u5b50\u70ed\u7535\u52bf\u3002\u56e0\u6b64\uff0cn-\u578b\u79bb\u5b50\u70ed\u7535\u6750\u6599\u8fd8\u5f88\u5c11\u89c1\uff0c\u76f8\u5bf9\u8f83\u4f4e\u7684\u70ed\u7535\u529f\u7387\u5f88\u96be\u4e0ep-\u578b\u79bb\u5b50\u70ed\u7535\u6750\u6599\u7684\u6027\u80fd\u76f8\u5339\u914d\u3002
\n \"\"\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u9999\u6e2f\u79d1\u6280\u5927\u5b66\u9ec4\u5b9d\u9675\u526f\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u65b0\u7684\u7b56\u7565\uff0c\u5176\u4e2d\u5c06\u5f3a\u79bb\u5b50-\u79bb\u5b50\u76f8\u4e92\u4f5c\u7528\u9009\u62e9\u6027\u5730\u5f15\u5165\u79bb\u5b50\u70ed\u7535\u6750\u6599\u4e2d\uff0c\u4ee5\u5728\u6240\u9700\u7684\u6b63\u5411\u6216\u8d1f\u5411\u8c03\u8282\u79bb\u5b50\u70ed\u7535\u52bf\uff08thermopower\uff09\u3002\u4f5c\u8005\u91c7\u7528\u57fa\u4e8e\u4e8c\u5143\u79bb\u5b50\u6db2\u4f53\uff08IL\uff09\u7684\u805a\u5408\u7269\u79bb\u5b50\u51dd\u80f6\u4f5c\u4e3a\u8d77\u70b9\uff0c\u5176\u5177\u6709\u7075\u6d3b\u6027\uff0c\u53ef\u4ee5\u4f7f\u7528\u4f4e\u6210\u672c\u7684\u6eb6\u6db2\u5de5\u827a\u5236\u5907\u3002\u5f53\u6dfb\u52a0\u80fd\u4e0e\u539f\u59cb\u79bb\u5b50\u7d27\u5bc6\u76f8\u4e92\u4f5c\u7528\u7684\u79bb\u5b50\u76d0\u5f62\u6210\u4e09\u5143\u805a\u5408\u7269\u79bb\u5b50\u51dd\u80f6\u65f6\uff0c\u79bb\u5b50\u70ed\u7535\u52bf\u53ef\u4ee5\u5728-15\u81f3+17 mV K-1<\/sup>\u8303\u56f4\u5185\uff0c\u5728\u63a5\u8fd1\u5ba4\u6e29\u548c60%\u7684\u76f8\u5bf9\u6e7f\u5ea6\uff08RH\uff09\u6761\u4ef6\u4e0b\uff0c\u5728\u6b63\u5411\u6216\u8d1f\u5411\u6025\u5267\u8c03\u8282\u3002\u4f5c\u8005\u5229\u7528\u8fd9\u79cd\u7b56\u7565\u5b9e\u73b0\u4e86-15 mV K-1<\/sup>\u7684\u8d1f\u70ed\u7535\u52bf\uff0c\u5728\u76f8\u540c\u6761\u4ef6\u4e0b\u8fbe\u5230\u4e86n-\u578b\u79bb\u5b50\u70ed\u7535\u6750\u6599\u7684\u521b\u7eaa\u5f55\u503c<\/strong>\u3002\u901a\u8fc7\u5305\u62ec\u62c9\u66fc\u5149\u8c31\u3001\u7ea2\u5916\u5149\u8c31\u548c\u6838\u78c1\u5171\u632f\uff08NMR\uff09\u5149\u8c31\u5728\u5185\u7684\u5404\u79cd\u8868\u5f81\u6280\u672f\uff0c\u4f5c\u8005\u5f97\u51fa\u4ee5\u4e0b\u7ed3\u8bba\uff1a\u53cc\u5411\u53ef\u8c03\u70ed\u7535\u52bf\u662f\u7531\u76d0\u79bb\u5b50\u548c\u79bb\u5b50\u6db2\u4f53\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u4ea7\u751f\u7684\u3002\u4f5c\u8005\u8fd8\u5c55\u793a\u4e86\u4e00\u79cd\u57fa\u4e8e\u5f00\u53d1\u7684p-\u578b\u548cn-\u578b\u79bb\u5b50\u51dd\u80f6\u7684\u753112\u5bf9p-n\u5bf9\u7ec4\u6210\u7684\u67d4\u6027\u53ef\u7a7f\u6234\u79bb\u5b50\u70ed\u7535\u5668\u4ef6\uff0c\u5b9e\u73b0\u4e86358 mV K-1<\/sup>\u7684\u5668\u4ef6\u70ed\u7535\u52bf\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cGiant and bidirectionally tunable thermopower in nonaqueous ionogels enabled by selective ion doping\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aScience Advances<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u805a\u5408\u7269\u51dd\u80f6\u7684\u70ed\u7535\u52bf<\/strong>
\n \"\"\uff08A\uff09\u6587\u732e\u4e2d\u79bb\u5b50\u70ed\u7535\u6750\u6599\u572860% RH\u4e0b\u7684\u70ed\u7535\u52bf\uff1b<\/p>\n

\uff08B\uff09p-\u578b\u548cn-\u578b\u79bb\u5b50\u51dd\u80f6\u5728\u6db2\u4f53\u7535\u89e3\u8d28\u4e0e\u805a\u5408\u7269\u57fa\u8d28PVDF-HFP\u7684\u4e0d\u540c\u91cd\u91cf\u6bd4\u4e0b\u7684\u70ed\u7535\u52bf\u3002<\/p>\n

\u56fe\u4e8c\u3001LIBF4<\/sub>\u6d53\u5ea6\u5bf9\u79bb\u5b50\u51dd\u80f6\u70ed\u7535\u6027\u80fd\u7684\u5f71\u54cd<\/strong>
\n \"\"\uff08A\uff09LiBF4<\/sub>\/EMIMTFSI\/PVDF-HFP\u79bb\u5b50\u51dd\u80f6\u5728\u4e0d\u540cLiBF4<\/sub>\u6d53\u5ea6\u4e0b\u7684\u70ed\u7535\u52bf\u548c\u79bb\u5b50\u7535\u5bfc\u7387\uff1b<\/p>\n

\uff08B\uff09c(LiBF4)=0\u30010.2\u30010.4\u30010.6\u30010.8\u548c1 M\u65f6\uff0cLiBF4<\/sub>\/EMIMTFSI\/PVDF-HFP\u79bb\u5b50\u51dd\u80f6\u7684\u62c9\u66fc\u5149\u8c31\uff1b<\/p>\n

\uff08C\uff09\u805a\u5408\u7269\u901a\u9053\u79bb\u5b50\u70ed\u6269\u6563\u8fc7\u7a0b\u4e2d\uff0cLi+<\/sup>\u9633\u79bb\u5b50\u548c\u9634\u79bb\u5b50\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08D\uff09EMIMTFSI\/PVDF-HFP\u79bb\u5b50\u51dd\u80f6\u5206\u522b\u5177\u67090.5 M LiBF4<\/sub>\u3001EMIMBF4<\/sub>\u548cLiTFSI\u7684\u70ed\u7535\u52bf\u3002<\/p>\n

\u56fe\u4e09\u3001EMIMCl\u6d53\u5ea6\u5bf9\u79bb\u5b50\u51dd\u80f6\u70ed\u7535\u6027\u80fd\u7684\u5f71\u54cd<\/strong>
\n \"\"\uff08A\uff09EMIMCl\/EMIMTFSI\/PVDF-HFP\u79bb\u5b50\u51dd\u80f6\u5728\u4e0d\u540cEMIMCl\u6d53\u5ea6\u4e0b\u7684\u70ed\u7535\u52bf\u548c\u79bb\u5b50\u7535\u5bfc\u7387\uff1b<\/p>\n

\uff08B\uff09EMIMCl\/EMIMTFSI\u6df7\u5408\u7269\u4e2dC(2)-H\u7684\u5316\u5b66\u4f4d\u79fb\uff1b<\/p>\n

\uff08C\uff09c(EMIMCl)=0\u30010.5\u548c1 M\u65f6\uff0cEMIMCl\/EMIMTFSI\/PVDF-HFP\u79bb\u5b50\u51dd\u80f6\u7684FTIR\u5149\u8c31\uff1b<\/p>\n

\uff08D\uff09\u805a\u5408\u7269\u901a\u9053\u79bb\u5b50\u70ed\u6269\u6563\u8fc7\u7a0b\u4e2d\uff0cCl–<\/sup>\u9634\u79bb\u5b50\u548c\u9633\u79bb\u5b50\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u3002<\/p>\n

\u56fe\u56db\u3001\u67d4\u6027\u70ed\u7535\u5668\u4ef6<\/strong>
\n \"\"\uff08A\uff09\u5e26\u670912\u5bf9p-\u578b\u548cn-\u578b\u79bb\u5b50\u51dd\u80f6\u7684\u8bbe\u8ba1\u793a\u610f\u56fe\u4ee5\u53ca\u5668\u4ef6\u56fe\u7247\uff1b<\/p>\n

\uff08B\uff09\u7535\u538b\u968f\u6e29\u5dee\u53d8\u5316\uff1b<\/p>\n

\uff08C\uff09\u7535\u538b\u4e0e\u6e29\u5dee\u7684\u7ebf\u6027\u62df\u5408\uff1b<\/p>\n

\uff08D\uff09\u572825 \u00b0C\u65f6\uff0c\u5c06\u5668\u4ef6\u653e\u5728\u4eba\u7684\u624b\u81c2\u4e0a\u65f6\u4ea7\u751f\u7684\u7535\u538b\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aGiant and bidirectionally tunable thermopower in nonaqueous ionogels enabled by selective ion doping<\/a><\/strong>. Science Advances<\/em>, 2021<\/strong>, DOI: 10.1126\/sciadv.abj3019.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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