{"id":231322,"date":"2021-12-30T06:08:36","date_gmt":"2021-12-29T22:08:36","guid":{"rendered":"\/\/m.iemloyee.com\/?p=231322"},"modified":"2021-12-29T20:08:49","modified_gmt":"2021-12-29T12:08:49","slug":"%e6%b1%9f%e6%b5%b7%e9%be%99%e5%9b%a2%e9%98%9f-angew-%ef%bc%9apd3cuuio-66%e5%85%89%e8%be%85%e5%8a%a9%e5%82%ac%e5%8c%96co2%e5%8a%a0%e6%b0%a2","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=231322","title":{"rendered":"\u6c5f\u6d77\u9f99\u56e2\u961f Angew.\uff1aPd3Cu@UiO-66\u5149\u8f85\u52a9\u50ac\u5316CO2\u52a0\u6c22"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u968f\u7740\u5de5\u4e1a\u5316\u8fdb\u7a0b\u7684\u5feb\u901f\u63a8\u8fdb\uff0c\u5927\u6c14\u4e2d\u4e8c\u6c27\u5316\u78b3\uff08CO2<\/sub>\uff09\u6d53\u5ea6\u4e0d\u65ad\u589e\u52a0\uff0c\u4ece\u800c\u5f15\u53d1\u4e86\u5168\u7403\u53d8\u6696\u7b49\u5371\u673a\u3002\u5728\u4f17\u591a\u7684CO2<\/sub>\u6355\u96c6\u4e0e\u8f6c\u5316\u6280\u672f\u4e2d\uff0c\u5c06CO2<\/sub>\u52a0\u6c22\u8f6c\u5316\u4e3a\u7532\u9178\uff08HCOOH\uff09\u3001\u7532\u9187\uff08CH3<\/sub>OH\uff09\u548c\u7532\u70f7\uff08CH4<\/sub>\uff09\u7b49\u589e\u503c\u5316\u5b66\u54c1\u88ab\u8ba4\u4e3a\u662f\u884c\u4e4b\u6709\u6548\u7684\u7b56\u7565\u3002\u5176\u4e2d\uff0c\u7532\u9187\u662f\u8fde\u63a5\u4e0a\u6e38C1<\/sub>\u5c0f\u5206\u5b50\u4e0e\u4e0b\u6e38\u5927\u5b97\u5316\u5b66\u54c1\u548c\u71c3\u6599\u7684\u91cd\u8981\u5316\u5de5\u539f\u6599\u3002\u76ee\u524d\uff0c\u901a\u8fc7\u7535\u3001\u5149\u50ac\u5316CO2<\/sub>\u8fd8\u539f\u5f97\u5230\u7532\u9187\u5f80\u5f80\u9762\u4e34\u6548\u7387\u4f4e\uff1b\u70ed\u50ac\u5316CO2<\/sub>\u5f80\u5f80\u9700\u8981\u9ad8\u6e29\u9ad8\u538b\uff0850-100 bar\u3001200-300 \u00b0C\uff09\u7684\u82db\u523b\u6761\u4ef6\uff0c\u800c\u5728\u9ad8\u6e29\u4e0b\u5f80\u5f80\u66f4\u5bb9\u6613\u53d1\u751f\u9006\u6c34\u7164\u6c14\u8f6c\u6362\uff08RWGS\uff09\u526f\u53cd\u5e94\uff0c\u4e0d\u5229\u4e8e\u9ad8\u9009\u62e9\u6027\u7684\u5236\u5907\u7532\u9187\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u4e00\u79cd\u80fd\u591f\u5728\u76f8\u5bf9\u4f4e\u6e29\u4e0b\u9ad8\u6548\uff0c\u9ad8\u9009\u62e9\u6027\u50ac\u5316CO2<\/sub>\u52a0\u6c22\u5236\u7532\u9187\u7684\u50ac\u5316\u5242\u81f3\u5173\u91cd\u8981\u3002\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\uff08MOFs\uff09\u662f\u4e00\u7c7b\u65b0\u578b\u7684\u6676\u6001\u591a\u5b54\u6750\u6599\uff0c\u5177\u6709\u7075\u6d3b\u7684\u7ed3\u6784\u53ef\u88c1\u526a\u6027\uff0c\u662f\u5236\u5907\u8fd9\u79cd\u591a\u529f\u80fd\u50ac\u5316\u5242\u7684\u7406\u60f3\u6750\u6599\u3002\u7136\u800c\uff0c\u57fa\u4e8eMOF\u57fa\u6750\u6599\u4e0a\u5f15\u5165\u592a\u9633\u80fd\u9a71\u52a8\u70ed\u50ac\u5316CO2<\/sub>\u52a0\u6c22\u5236\u7532\u9187\u7684\u7814\u7a76\u5c1a\u672a\u62a5\u9053\u3002
\n \"\"\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u6c5f\u6d77\u9f99\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u5c06\u53cc\u91d1\u5c5ePd3<\/sub>Cu NPs\u5f15\u5165\u5230\u7ecf\u5178\u7684\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\u6750\u6599UiO-66\u4e2d\uff0c\u5f97\u5230Pd3<\/sub>Cu@UiO-66\u590d\u5408\u6750\u6599\uff0c\u5e76\u7528\u4e8e\u5149\u8f85\u52a9\u6761\u4ef6\u4e0b\u7684CO2<\/sub>\u52a0\u6c22\u53cd\u5e94\u3002\u7814\u7a76\u53d1\u73b0\uff0cZr-oxo\u7c07\u4e0a\u7684\u7f3a\u9677\u4f4d\u70b9\u80fd\u591f\u6355\u83b7\u548c\u6d3b\u5316CO2<\/sub>\u5206\u5b50\uff0cPd3<\/sub>Cu NPs\u53ef\u4ee5\u9ad8\u6548\u6d3b\u5316H2<\/sub>\u3002\u540c\u65f6\uff0cMOF\u914d\u4f53\u53ef\u4ee5\u6355\u83b7\u5149\u5b50\u5e76\u5149\u751f\u7535\u5b50\uff0c\u5149\u751f\u7535\u5b50\u901a\u8fc7LCCT\uff08\u914d\u4f53\u5230\u7c07\u7684\u7535\u8377\u8f6c\u79fb\uff09\u8fc7\u7a0b\u5c06\u5149\u751f\u7535\u5b50\u6ce8\u5165\u5230\u5438\u9644\u5728Zr-oxo\u7c07\u4e0a\u7684CO2<\/sub>\u7684\u53cd\u952e\u8f68\u9053\uff0c\u52a0\u901f\u4e86\u4e2d\u95f4\u7269\u79cdHCOO*\u7684\u751f\u6210\uff0c\u4ece\u800c\u663e\u8457\u964d\u4f4e\u4e86\u6574\u4e2a\u53cd\u5e94\u7684\u8868\u89c2\u6d3b\u5316\u80fd\u3002\u57fa\u4e8ePd3<\/sub>Cu@UiO-66\u4e8c\u6c27\u5316\u78b3\u52a0\u6c22\u50ac\u5316\u5242\u4e2d\u6210\u529f\u6784\u7b51\u4e86\u8fd1\u90bb\u7684CO2<\/sub>\u548cH2<\/sub>\u6d3b\u5316\u4f4d\u70b9\uff0c\u5728200 \u00b0C\u548c1.25 MPa\uff0cPd3<\/sub>Cu@UiO-66\u5728\u5149\u8f85\u52a9\u4e0b\u5b9e\u73b0\u4e86340 \u00b5mol g-1<\/sup> h-1<\/sup>\u7684\u7532\u9187\u4ea7\u7387\uff0c\u9ad8\u51fa\u9ed1\u6697\u6761\u4ef6\u4e0b\u50ac\u5316\u6027\u80fd\u76845.6\u500d\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cLight-Assisted CO2<\/sub> Hydrogenation over Pd3<\/sub>Cu@UiO-66 Promoted by Active Sites in Close Proximity\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aAngew. Chem. Int. Ed.<\/strong>\u4e0a\u3002
\n \"\"\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001Pd3<\/sub>Cu@UiO-66\u548cPd3<\/sub>Cu\/UiO-66\u4e0a\u5149\u8f85\u52a9CO2<\/sub>\u52a0\u6c22\u6210CH3<\/sub>OH\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"
\n \u56fe\u4e8c\u3001Pd3<\/sub>Cu@UiO-66\u7684\u7ed3\u6784\u8868\u5f81<\/strong>
\n \"\"\uff08a-b\uff09Pd3<\/sub>Cu@UiO-66 TEM\u56fe\u7247\uff1b<\/p>\n

\uff08c-f\uff09\u9ad8\u5206\u8fa8\u900f\u5c04\u7535\u955c\u56fe\u7247\u548c\u76f8\u5e94\u7684Zr\u3001Pd\u3001Cu\u5143\u7d20\u626b\u63cf\u56fe\u7247\u3002<\/p>\n

\u56fe\u4e09\u3001Pd3<\/sub>Cu@UiO-66\u4e0a\u7684\u5149\u8f85\u52a9CO2<\/sub>\u5408\u6210\u7532\u9187<\/strong>
\n \"\"\uff08a\uff09\u4e0d\u540c\u53cd\u5e94\u6e29\u5ea6\u4e0bCH3<\/sub>OH\u7684\u751f\u4ea7\u901f\u7387\uff1b<\/p>\n

\uff08b-c\uff09Pd3<\/sub>Cu@UiO-66\u7684\u963f\u4f26\u5c3c\u4e4c\u65af\u56fe\u548c\u52a8\u529b\u5b66\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09Pd3<\/sub>Cu@UiO-66\u7684\u50ac\u5316\u5faa\u73af\u6d4b\u8bd5\u3002<\/p>\n

\u56fe\u56db\u3001CO2<\/sub>-TPD\u548cH2<\/sub>-TPD\u6d4b\u8bd5<\/strong>
\n \"\"\uff08a-b\uff09Pd3<\/sub>Cu@UiO-66\u548cUiO-66\u7684CO2<\/sub>-TPD\u548cH2<\/sub>-TPD\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e94\u3001Pd3<\/sub>Cu@UiO-66\u4e0aCO2<\/sub>\u52a0\u6c22\u5236\u7532\u9187\u7684\u6027\u80fd\u6d4b\u8bd5\u4e0e\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09\u4e0d\u540c\u5149\u7167\u5f3a\u5ea6\u4e0b\u7684\u7532\u9187\u5408\u6210\u4ea7\u7387\uff1b<\/p>\n

\uff08b\uff09\u4e0d\u540c\u6ce2\u957f\u4e0b\u7684\u7684\u7532\u9187\u5408\u6210\u4ea7\u7387\uff1b<\/p>\n

\uff08c\uff09UiO-66\u548cPd3<\/sub>Cu@UiO-66\u7684\u7d2b\u5916-\u53ef\u89c1\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09Pd3<\/sub>Cu@UiO-66\u5728\u4e0d\u540c\u6761\u4ef6\u4e0b\u7684ESR\u8c31\u3002<\/p>\n

\u56fe\u516d\u3001\u539f\u4f4dDRIFT\u5149\u8c31<\/strong>
\n \"\"\uff08a\uff09Pd3<\/sub>Cu@UiO-66\u57283500-2700 cm-1<\/sup>\u8303\u56f4\u5185\u7684\u539f\u4f4dDRIFT\u5149\u8c31\uff1b<\/p>\n

\uff08b\uff09\u5438\u9644\u5728\u5f00\u653eZr\u4f4d\u70b9\u4e0a\u7684\u53cc\u9f7f\u7532\u9178\u76d0\u7269\u79cd\u7684\u03bd(C-H)\u3002<\/p>\n

\u56fe\u4e03\u3001DFT\u8ba1\u7b97<\/strong>
\n \"\"\uff08a\uff09\u5438\u9644\u5728\u4e0d\u9971\u548cZr-oxo\u7c07\u4e0a\u7684\u4ea7\u7269\u4e2d\u95f4\u4f53\u6a21\u578b\uff1b<\/p>\n

\uff08b\uff09CO2<\/sub>\u6c22\u5316\u53cd\u5e94\u8def\u5f84\u7684\u81ea\u7531\u80fd\u53d8\u5316\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u901a\u8fc7\u5c06\u8d85\u5c0f\u7684Pd3<\/sub>Cu NPs\u5747\u5300\u5730\u5c01\u88c5\u5728UiO-66\u4e2d\u5f97\u5230\u4e86Pd3<\/sub>Cu@UiO-66\u590d\u5408\u6750\u6599\uff0c\u5728\u5149\u7167\u5c04\u4e0b\u5c06CO2<\/sub>\u52a0\u6c22\u8f6c\u53d8\u4e3a\u7532\u9187\u4e2d\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u50ac\u5316\u6d3b\u6027\u3002\u5149\u7167\u4e0b\uff0cUiO-66\u7684\u914d\u4f53\u6355\u83b7\u5149\u5b50\u5e76\u4ea7\u751f\u5149\u751f\u7535\u5b50\uff0c\u5149\u751f\u7535\u5b50\u901a\u8fc7LCCT\uff08\u914d\u4f53\u5230\u7c07\u7684\u7535\u8377\u8f6c\u79fb\uff09\u8fc7\u7a0b\u5c06\u5149\u751f\u7535\u5b50\u6ce8\u5165\u5230\u5438\u9644\u5728Zr-oxo\u7c07\u4e0a\u7684CO2<\/sub>\u7684\u53cd\u952e\u8f68\u9053\uff0c\u52a0\u901f\u4e86\u4e2d\u95f4\u7269\u79cdHCOO*\u7684\u751f\u6210\uff0c\u4ece\u800c\u663e\u8457\u964d\u4f4e\u4e86\u6574\u4e2a\u53cd\u5e94\u7684\u8868\u89c2\u6d3b\u5316\u80fd\u3002\u6d4b\u8bd5\u7ed3\u679c\u8868\u660e\uff0c\u5f53\u53cd\u5e94\u6761\u4ef6\u4e3a200 \u2103\u30011.25 MPa\uff0c\u5149\u7167\u4e0b\u7532\u9187\u7684\u6700\u5927\u4ea7\u7387\u4e3a340 \u00b5mol g-1<\/sup> h-1<\/sup>\uff0c\u6bd4\u9ed1\u6697\u4e2d\u7684\u4ea7\u7387\u9ad8\u51fa5.6\u500d\u3002\u6b64\u5916\uff0cPd3<\/sub>Cu\u76f8\u5bf9\u4e8eUiO-66\u7684\u7a7a\u95f4\u4f4d\u7f6e\u5728\u50ac\u5316\u4e2d\u8d77\u7740\u5173\u952e\u4f5c\u7528\u3002\u4e0ePd3<\/sub>Cu\/UiO-66\uff08Pd3<\/sub>Cu NPs\u5206\u6563\u5728UiO-66\u5b54\u5916\uff09\u76f8\u6bd4\uff0cPd3<\/sub>Cu@UiO-66\uff08Pd3<\/sub>Cu NPs\u5206\u6563\u5728UiO-66\u5b54\u5185\uff09\u4e2d\u9ad8\u5ea6\u5206\u6563\u7684Pd3<\/sub>Cu NPs\u4f7f\u5f97Zr-oxo\u7c07\u548cPd3<\/sub>Cu NPs\u7684\u6d3b\u6027\u4f4d\u70b9\u5341\u5206\u63a5\u8fd1\uff0c\u4f7fPd3<\/sub>Cu\u5411\u5468\u56f4\u7684Zr-oxo\u7c07\u63d0\u4f9b\u8db3\u591f\u7684\u6ea2\u6d41\u6c22\uff0c\u964d\u4f4e\u53cd\u5e94\u7684\u8868\u89c2\u6d3b\u5316\u80fd\u3002\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u4e3a\u5149\u70ed\u534f\u540c\u50ac\u5316\u63d0\u4f9b\u4e86\u6df1\u5165\u4e86\u89e3\uff0c\u800c\u4e14\u8bc1\u660e\u4e86CO2<\/sub>\u548cH2<\/sub>\u6d3b\u5316\u4f4d\u70b9\u4e4b\u95f4\u7684\u8fd1\u90bb\u4f5c\u7528\u5728CO2<\/sub>\u52a0\u6c22\u4e2d\u7684\u91cd\u8981\u4f5c\u7528\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aLight-Assisted CO2<\/sub> Hydrogenation over Pd3<\/sub>Cu@UiO-66 Promoted by Active Sites in Close Proximity<\/a><\/strong>. Angew. Chem. Int. Ed.<\/em>, 2021<\/strong>, DOI: 10.1002\/anie.202116396.<\/p>\n

\u6c5f\u6d77\u9f99\u6559\u6388\u7b80\u4ecb\uff1a<\/strong><\/p>\n

\u6c5f\u6d77\u9f99\uff0c1981\u5e748\u6708\u751f\u4e8e\u5b89\u5fbd\u5408\u80a5\u5e90\u6c5f\u53bf\u3002\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u6559\u6388\u3001\u535a\u58eb\u751f\u5bfc\u5e08\u3001\u82f1\u56fd\u7687\u5bb6\u5316\u5b66\u4f1a\u4f1a\u58eb\uff08FRSC\uff09\uff0c\u83b7\u5f97\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u57fa\u91d1\u8d44\u52a9\uff0c\u5165\u9009\u7b2c\u56db\u6279\u56fd\u5bb6\u201c\u4e07\u4eba\u8ba1\u5212\u201d\u79d1\u6280\u521b\u65b0\u9886\u519b\u4eba\u624d\uff082019\u5e74\uff09\u3001\u79d1\u6280\u90e8\u4e2d\u9752\u5e74\u79d1\u6280\u521b\u65b0\u9886\u519b\u4eba\u624d\uff082018\u5e74\uff09\u7b49\u3002\u81ea2017\u5e74\u81f3\u4eca\uff0c\u8fde\u7eed\u6bcf\u5e74\u5165\u9009\u79d1\u777f\u552f\u5b89\uff08\u539f\u6c64\u68ee\u8def\u900f\uff09\u5168\u7403\u9ad8\u88ab\u5f15\u79d1\u5b66\u5bb6\uff08\u5316\u5b66\uff09\u548c\u7231\u601d\u552f\u5c14\uff08Elsevier\uff09\u4e2d\u56fd\u9ad8\u88ab\u5f15\u5b66\u8005\u699c\u5355<\/strong>\u3002<\/p>\n

2003\u5e747\u6708\u4e8e\u5b89\u5fbd\u5e08\u8303\u5927\u5b66\u83b7\u5316\u5b66\u5b66\u58eb\u5b66\u4f4d\uff1b2008\u5e747\u6708\u4e8e\u4e2d\u56fd\u79d1\u5b66\u9662\u798f\u5efa\u7269\u8d28\u7ed3\u6784\u7814\u7a76\u6240\u83b7\u65e0\u673a\u5316\u5b66\u535a\u58eb\u5b66\u4f4d\u30022008\u5e748\u6708\u81f32011\u5e748\u6708\u5728\u65e5\u672c\u56fd\u7acb\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\u5de5\u4f5c\uff0c\u5206\u522b\u4efb\u4ea7\u7efc\u7814\u7279\u522b\u7814\u7a76\u5458\u548c\u65e5\u672c\u5b66\u672f\u632f\u5174\u4f1a\u5916\u56fd\u4eba\u7279\u522b\u7814\u7a76\u5458\uff08JSPS fellow\uff09\uff1b2011\u5e749\u6708\u81f32013\u5e741\u6708\u5728\u7f8e\u56fd\u5fb7\u514b\u8428\u65af\u519c\u5de5\u5927\u5b66\u4ece\u4e8b\u535a\u58eb\u540e\u7814\u7a76\u30022013\u5e74\u521d\u5165\u804c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u5316\u5b66\u7cfb\uff08\u73b0\u4efb\u7cfb\u6267\u884c\u4e3b\u4efb\uff09\uff0c\u62c5\u4efb\u6559\u6388\u3001\u535a\u58eb\u751f\u5bfc\u5e08\u30022017\u5e74\u83b7\u5f97\u4e2d\u56fd\u79d1\u5927\u6d77\u5916\u6821\u53cb\u57fa\u91d1\u4f1a\u9752\u5e74\u6559\u5e08\u4e8b\u4e1a\u5956\uff0c2018\u5e74\u83b7\u5f97\u5362\u5609\u9521\u4f18\u79c0\u5bfc\u5e08\u5956\u3001\u592a\u9633\u80fd\u5149\u5316\u5b66\u4e0e\u5149\u50ac\u5316\u7814\u7a76\u9886\u57df\u4f18\u79c0\u9752\u5e74\u5956\uff0c2019\u5e74\u83b7\u5f97\u4e2d\u56fd\u79d1\u5b66\u9662\u4f18\u79c0\u5bfc\u5e08\u5956\u3002<\/p>\n

\u6c5f\u6d77\u9f99\u6559\u6388\u957f\u671f\u4ece\u4e8b\u914d\u4f4d\u5316\u5b66\u3001\u6750\u6599\u5316\u5b66\u548c\u50ac\u5316\u5316\u5b66\u7684\u4ea4\u53c9\u6027\u7814\u7a76\u5de5\u4f5c\uff0c\u7279\u522b\u5728\u57fa\u4e8e\u91d1\u5c5e\u6709\u673a\u6846\u67b6\uff08MOFs\uff09\u7684\u6676\u6001\u591a\u5b54\u529f\u80fd\u6750\u6599\u7684\u8bbe\u8ba1\u3001\u5408\u6210\u4e0e\u50ac\u5316\u65b9\u9762\u5f00\u5c55\u4e86\u7cfb\u7edf\u7684\u7814\u7a76\u5de5\u4f5c<\/strong>\uff0c\u90e8\u5206\u7814\u7a76\u6210\u679c\u83b72020\u5e74\u5ea6\u6559\u80b2\u90e8\u81ea\u7136\u79d1\u5b66\u4e00\u7b49\u5956\uff08\u7b2c\u4e00\u5b8c\u6210\u4eba\uff09\u3002\u7814\u7a76\u7ed3\u679c\u5df2\u5728\u56fd\u9645\u91cd\u8981SCI\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587170\u4f59\u7bc7\uff0c\u5176\u4e2d2013\u5e74\u56de\u56fd\u72ec\u7acb\u5de5\u4f5c\u4ee5\u6765\uff0c\u4ee5\u901a\u8baf\u4f5c\u8005\u8eab\u4efd\u5728Nat. Catal.\uff081\u7bc7\uff09\uff0cJ. Am. Chem. Soc.\uff0810\u7bc7\uff09\uff0cAngew. Chem.\uff0816\u7bc7\uff09\uff0cChem\uff084\u7bc7\uff09\uff0cNat. Commun.\uff082\u7bc7\uff09\uff0cAdv. Mater.\uff087\u7bc7\uff09\uff0cNatl. Sci. Rev.\uff082\u7bc7\uff09\uff0cMatter\uff081\u7bc7\uff09\uff0cAcc. Chem. Res.\uff081\u7bc7\uff09\uff0cAcc. Mater. Res.\uff081\u7bc7\uff09\uff0cChem. Rev.\uff081\u7bc7\uff09\uff0cChem. Soc. Rev.\uff082\u7bc7\uff09\uff0cCoord. Chem. Rev.\uff083\u7bc7\uff09, Mater. Today\uff081\u7bc7\uff09\u7b49\u9ad8\u6c34\u5e73\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587\u3002\u8bba\u6587\u88ab\u5f15\u752830000\u6b21\u4ee5\u4e0a\uff08H\u6307\u6570\uff1a87\uff09\uff0c\u7bc7\u5747\u8bba\u6587\u5f15\u7528\u8fbe170\u6b21\u4ee5\u4e0a\uff0c\u5176\u4e2d58\u7bc7\u5165\u9009ESI\u9ad8\u88ab\u5f15\u8bba\u6587\uff08Highly Cited Papers, Top 1%\uff09\uff1b\u6388\u6743\u4e2d\u56fd\u4e13\u52293\u9879\u3002\u5728\u300aNanoporous Materials: Synthesis and Applications\u300b\u4e2d\u64b0\u5199\u4e66\u7ae0\u4e00\u7ae0\u3002\u62c5\u4efb\u4e2d\u56fd\u5316\u5b66\u4f1a\u6676\u4f53\u5316\u5b66\u4e13\u4e1a\u59d4\u5458\u4f1a\u59d4\u5458\u3001\u4e2d\u56fd\u611f\u5149\u5b66\u4f1a\u5149\u50ac\u5316\u4e13\u4e1a\u59d4\u5458\u4f1a\u59d4\u5458\u3001\u5929\u6d25\u5e02\u80fd\u6e90\u6750\u6599\u5316\u5b66\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u5b66\u672f\u59d4\u5458\u4f1a\u59d4\u5458\u7b49\uff1b\u62c5\u4efbEnergyChem\uff08Elsevier\uff09\u3001Materials\uff08MDPI\uff09\u3001\u4e2d\u56fd\u5316\u5b66\u5feb\u62a5\u3001\u5316\u5b66\u5b66\u62a5\u3001Scientific Reports\uff08NPG\uff09\u3001\u65e0\u673a\u5316\u5b66\u5b66\u62a5\u3001\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u5b66\u62a5\u7b49\u671f\u520a\u7f16\u59d4\u548c\u987e\u95ee\u59d4\u5458\u4f1a\u59d4\u5458\u3002\u627f\u62c5\u57fa\u91d1\u59d4\u3001\u79d1\u6280\u90e8\u3001\u4e2d\u79d1\u9662\u3001\u6559\u80b2\u90e8\u3001\u5b89\u5fbd\u7701\u7b49\u591a\u9879\u91cd\u8981\u79d1\u7814\u4efb\u52a1\u3002<\/p>\n

\u8bfe\u9898\u7ec4\u4e3b\u9875\uff1ahttp:\/\/staff.ustc.edu.cn\/~jianglab\/index.html.<\/strong><\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1\uff1atougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu.<\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011 \u968f\u7740\u5de5\u4e1a\u5316\u8fdb\u7a0b\u7684\u5feb\u901f\u63a8\u8fdb\uff0c\u5927\u6c14\u4e2d\u4e8c\u6c27\u5316\u78b3\uff08CO2\uff09\u6d53\u5ea6\u4e0d\u65ad\u589e\u52a0\uff0c\u4ece\u800c\u5f15\u53d1\u4e86\u5168\u7403\u53d8\u6696\u7b49\u5371\u673a\u3002\u5728\u4f17\u591a\u7684CO2\u6355\u96c6\u4e0e\u8f6c\u5316\u6280\u672f\u4e2d\uff0c\u5c06CO2\u52a0\u6c22\u8f6c\u5316\u4e3a\u7532\u9178\uff08…<\/p>\n","protected":false},"author":7770,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[4781],"class_list":["post-231322","post","type-post","status-publish","format-standard","hentry","category-jiedu","tag-pd3cuuio-66"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231322"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/7770"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=231322"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231322\/revisions"}],"predecessor-version":[{"id":231394,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231322\/revisions\/231394"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=231322"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=231322"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=231322"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}