{"id":231247,"date":"2021-12-26T06:53:04","date_gmt":"2021-12-25T22:53:04","guid":{"rendered":"\/\/m.iemloyee.com\/?p=231247"},"modified":"2021-12-25T18:53:33","modified_gmt":"2021-12-25T10:53:33","slug":"2021%e5%b9%b4mof%e9%a2%86%e5%9f%9f%e5%a4%a7%e4%bd%ac%e4%bb%acyaghi%e3%80%81%e8%b5%b5%e4%b8%b9%e3%80%81%e6%b4%aa%e8%8c%82%e6%a4%bf%e3%80%81%e8%8b%8f%e6%88%90%e5%8b%87%e3%80%81%e9%99%88%e9%82%a6","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=231247","title":{"rendered":"2021\u5e74MOF\u9886\u57df\u5927\u4f6c\u4eecYaghi\u3001\u8d75\u4e39\u3001\u6d2a\u8302\u693f\u3001\u82cf\u6210\u52c7\u3001\u9648\u90a6\u6797\u6210\u679c"},"content":{"rendered":"

1.\u00a0\u00a0\u00a0 Yaghi\uff1a(Angew.Chem.Int.Ed) \u00a0Cu(I)\u548c Ag(I)\u5bf9\u63a5\u7684\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u53ef\u7528\u4e8e\u5438\u9644\u548c\u5206\u79bb\u6c19\u6c14<\/p>\n

\"\"<\/p>\n

Omar M.Yaghi\u6559\u6388\u4e8e2021\u5e741\u6708\u4e8eAngew.Chem.Int.Ed\u53d1\u8868\u4e86\u4e00\u7bc7\u9898\u76ee\u4e3a\u201cDocking of CuI and AgI in Metal\u2010Organic Frameworks for Adsorption and Separation of Xenon\u201d\u7684\u6587\u7ae0\u3002\u8be5\u6587\u7ae0\u4e3b\u8981\u8bb2\u8ff0\u5229\u7528\u591a\u5b54\u5438\u9644\u5242\u4ece\u6c2a\u6c14\u4e2d\u5206\u79bb\u6c19\u6c14\u662f\u4e00\u79cd\u53ef\u6301\u7eed\u751f\u4ea7\u5c0f\u4f53\u79ef\u4f46\u9ad8\u4ef7\u503c\u60f0\u6027\u6c14\u4f53\u7684\u6280\u672f\u3002MOF \u662f\u8bbe\u8ba1\u597d\u7684\u6c19\u6c14\u5438\u9644\u5242\uff0c\u5176\u5438\u9644\u5206\u79bb\u6027\u80fd\u53ef\u4ee5\u901a\u8fc7\u8c03\u6574\u5b54\u9699\u6307\u6807\u3001\u529f\u80fd\u548c\u6297\u8861\u79bb\u5b50\u6765\u589e\u5f3a\u3002Yue-Biao Zhang\u3001Omar M. Yaghi \u548c\u5176\u4ed6\u5408\u4f5c\u8005\u63cf\u8ff0\u4e86\u4e00\u79cd\u65b0\u7684 MOF \u5408\u6210\u540e\u91d1\u5c5e\u5316\u65b9\u6cd5\uff0c\u8be5\u65b9\u6cd5\u901a\u8fc7\u4fdd\u7559\u591a\u4f59\u7684\u91d1\u5c5e\u79bb\u5b50\u548c\u6297\u8861\u79bb\u5b50\u6765\u540c\u65f6\u63d0\u9ad8\u5438\u9644\u9009\u62e9\u6027\u548c\u5438\u6536\u80fd\u529b\u3002<\/p>\n

\u7279\u522b\u662f\uff0cAg-MOF-303 \u5728 298 K \u548c 0.2 bar \u4e0b\u8868\u73b0\u51fa 59 cm3<\/sup>\u2022cm -3<\/sup> \u7684 Xe \u5438\u6536\uff0c\u9009\u62e9\u6027\u4e3a 10.4\uff0c\u4f7f\u5176\u6210\u4e3a\u6027\u80fd\u6700\u9ad8\u7684 MOF\u3002\u4e0e\u539f\u59cb MOF-303 \u76f8\u6bd4\uff0c\u52a8\u6001\u5206\u79bb\u6027\u80fd\u63d0\u9ad8\u4e86 100%\u3002\u8fd9\u79cd\u91d1\u5c5e\u5316\u7b56\u7565\u4ee3\u8868\u4e86\u4e00\u79cd\u8bbe\u8ba1 MOF \u4ee5\u63d0\u4f9b\u9ad8\u6027\u80fd\u6c14\u4f53\u5206\u79bb\u7684\u65b0\u7b56\u7565\u3002<\/p>\n

DOI<\/strong>\uff1a10.1002\/anie.202016907<\/strong><\/a><\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/full\/10.1002\/anie.202016907<\/p>\n

2.Yaghi<\/strong>\uff1a(AM<\/strong>) \u4ece\u5206\u5b50\u5230\u6846\u67b6\u518d\u5230\u8d85\u6846\u67b6\u6676\u4f53<\/p>\n

\"\"<\/p>\n

\u6784\u5efa\u63a5\u8fd1\u751f\u7269\u7cfb\u7edf\u6c34\u5e73\u7684\u590d\u6742\u6027\u548c\u529f\u80fd\u6027\u5316\u5b66\u7ed3\u6784\u59cb\u7ec8\u662f\u4e00\u4e2a\u6301\u7eed\u7684\u6311\u6218\u3002 Yaghi<\/strong>\u6559\u6388\u5e26\u9886\u5176\u56e2\u961f\u63d0\u51fa\u4e86\u4e00\u79cd\u901a\u7528\u7684\u5408\u6210\u7b56\u7565\uff0c\u5229\u7528\u4e00\u4e2a\u6784\u5efa\u5757\u9010\u6b65\u5b9e\u73b0\u4e86\u5230\u8d85\u6846\u67b6\u6676\u4f53\u7684\u8f6c\u53d8\u3002<\/p>\n

\u5177\u4f53\u800c\u8a00\uff0c\u5c31\u662f\u5c06\u91d1\u5c5e\u914d\u5408\u7269\u548c\u6709\u673a\u5206\u5b50\u8fde\u63a5\u6210\u7f51\u72b6\u6846\u67b6\u7684\u77e5\u8bc6\u5e94\u7528\u5230\u5c06\u8fd9\u4e9b\u6846\u67b6\u7684\u6676\u4f53\u8fde\u63a5\u6210\u8d85\u6676\u4f53\uff08\u8d85\u6846\u67b6\uff09\u3002 \u8fd9\u79cd\u7b56\u7565\u5b9e\u73b0\u4e86\u5728\u5206\u5b50\u5c42\u9762\u4e0a\u63a7\u5236\u5206\u5b50\uff0c\u4ee5\u4ea7\u751f\u66f4\u591a\u6bd4\u5f53\u524d\u6750\u6599\u66f4\u5177\u6709\u6f5c\u529b\u7684\u65b0\u578b\u6750\u6599\u3002\u8be5\u7814\u7a76\u4ee5\u201cFrom Molecules to Frameworks to Superframework Crystals\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eAdv Mater\u4e0a\u3002<\/p>\n

DOI<\/strong>\uff1a10.1002\/adma.202103808<\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/abs\/10.1002\/adma.202103808<\/strong><\/a><\/p>\n

3.\u8d75\u4e39\uff1a<\/strong>(AM<\/strong>) \u901a\u8fc7\u7528\u4e8e\u6c14\u4f53\u5206\u79bb\u7684\u591a\u754c\u9762\u5de5\u7a0b\u7b56\u7565\u7684\u8d85\u8584\u5171\u4ef7\u6709\u673a\u9aa8\u67b6\u819c<\/strong><\/p>\n

\"\"<\/p>\n

\u5171\u4ef7\u6709\u673a\u9aa8\u67b6\uff08COFs\uff09\u7531\u4e8e\u5176\u9ad8\u5b54\u9699\u7387\u3001\u6709\u5e8f\u6392\u5217\u548c\u9ad8\u7a33\u5b9a\u6027\u800c\u6210\u4e3a\u6709\u524d\u9014\u7684\u819c\u6750\u6599\u3002\u7136\u800c\uff0cCOFs \u76f8\u5bf9\u8f83\u5927\u7684\u5b54\u5f84\u548c\u590d\u6742\u7684\u819c\u5236\u5907\u5de5\u827a\u9650\u5236\u4e86\u5b83\u4eec\u5728\u7b5b\u5206\u5c0f\u6c14\u4f53\u5206\u5b50\u4e2d\u7684\u5e94\u7528\uff0c\u5373\u4f7f\u5728\u5b9e\u9a8c\u5ba4\u89c4\u6a21\u4e5f\u662f\u5982\u6b64\u3002\u57fa\u4e8e\u6b64\uff0c\u8d75\u4e39<\/strong>\u6559\u6388\u63d0\u51fa\u4e86\u4e00\u79cd\u591a\u754c\u9762\u5de5\u7a0b\u7b56\u7565\uff0c\u5373\u5177\u6709\u4e0d\u540c\u5b54\u5f84\u7684\u4e24\u79cd COF\uff08TpPa-SO3<\/sub>H \u548c TpTG\u00a0Cl<\/sub>\uff09\u76f4\u63a5\u9010\u5c42\u754c\u9762\u53cd\u5e94\uff0c\u5728 COF-COF \u754c\u9762\u9876\u90e8\u5f62\u6210\u72ed\u7a84\u7684\u5b54\u5f84\u76f8\u5bf9\u5927\u5b54\u7684 COF (COF-LZU1) \u8584\u819c\u3002\u5728423 K\uff0c\u4e00\u4e2a\u5236\u9020\u4e3a155nm\u539a\u7684\u8d85\u8584COF\u819c\u663e\u793a\u0127\u00a02<\/sub>\u6e17\u900f\u6027\u9ad8\u8fbe2163\u4e2a\u6c14\u4f53\u6e17\u900f\u5355\u5143\uff08GPU\uff09\u4ee5\u53caH2<\/sub>\u00a0\/CO2<\/sub>\u9009\u62e9\u6027\u4e3a26\uff0c\u8d85\u8d8a\u4e862008 \u5e74 Robeson \u7684\u4e0a\u9650\u3002\u8be5\u7b56\u7565\u4e0d\u4ec5\u4e3a H2<\/sub>\u5206\u79bb\u63d0\u4f9b\u4e86\u9ad8\u6027\u80fd\u7684\u819c\u5019\u9009\u7269\uff0c\u800c\u4e14\u4e3a\u5176\u4ed6 COF\u3001\u591a\u5b54\u805a\u5408\u7269\u53ca\u5176\u819c\u7684\u754c\u9762\u5de5\u7a0b\u548c\u5b54\u5de5\u7a0b\u64cd\u4f5c\u63d0\u4f9b\u4e86\u542f\u793a\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5 \u201cUltrathin covalent organic framework membranes via a multi-interfacial engineering strategy for gas separation\u201d\u4e3a\u9898\u53d1\u8868\u4e8eAdv. Mater.\u00a0\u671f\u520a\u4e0a\u3002<\/strong><\/p>\n

DOI<\/strong>\uff1a\u00a010.1002\/adma.202104946<\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/abs\/10.1002\/adma.202104946<\/a><\/p>\n

4.\u8d75\u4e39\uff1a<\/strong>(AM<\/strong>) \u5177\u6709\u53ef\u53d8\u529f\u80fd\u7684\u53ef\u6eb6\u6db2\u52a0\u5de5\u91d1\u5c5e<\/strong>–<\/strong>\u6709\u673a\u9aa8\u67b6\u7eb3\u7c73\u7247<\/strong><\/p>\n

\"\"<\/p>\n

\u91d1\u5c5e\u6709\u673a\u6846\u67b6\uff08MOF\uff09\u672c\u8d28\u4e0a\u7f3a\u4e4f\u6d41\u52a8\u6027\uff0c\u56e0\u6b64\u7f3a\u4e4f\u6eb6\u6db2\u52a0\u5de5\u6027\u3002\u76f4\u63a5\u5408\u51fa\u50cf\u805a\u5408\u7269\u4e00\u6837\u7684\u5728\u6eb6\u6db2\u4e2d\u53ef\u52a0\u5de5\u6027\u7684MOF\u4ecd\u7136\u5177\u6709\u6311\u6218\u6027\uff0c\u90a3\u6837\u7684MOF\u5728\u4f17\u591a\u5e94\u7528\u4e2d\u5907\u53d7\u8ffd\u6367\u3002\u8be5\u7814\u7a76\u4e2d\uff0c\u4e00\u9505\u6cd5\u3001\u65e0\u8868\u9762\u6d3b\u6027\u5242\u548c\u53ef\u6269\u5c55\u7684\u9ad8\u5ea6\u7a33\u5b9a MOF \u60ac\u6d6e\u6db2\u7531\u5e73\u5747\u9762\u79ef\u5f02\u5e38\u5927\u7684\u5177\u6709\u53ef\u53d8\u529f\u80fd\u7684\uff08\u5e73\u5747\u9762\u79ef > 15000 \u00b5m\u00a02<\/sup>) NUS-8 \u7eb3\u7c73\u7247\u5408\u6210\u3002\u8fd9\u662f\u901a\u8fc7\u5728\u5408\u6210\u8fc7\u7a0b\u4e2d\u6dfb\u52a0\u5c01\u7aef\u5206\u5b50\u4ee5\u53ca\u660e\u667a\u5730\u63a7\u5236\u524d\u4f53\u6d53\u5ea6\u548c MOF \u7eb3\u7c73\u7247-\u6eb6\u5242\u76f8\u4e92\u4f5c\u7528\u6765\u5b9e\u73b0\u7684\u3002\u7531\u6b64\u4ea7\u751f\u7684\u5177\u6709\u53ef\u53d8\u529f\u80fd\u7684 2D NUS-8 \u7eb3\u7c73\u7247\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u6eb6\u6db2\u52a0\u5de5\u6027\u3002\u56e0\u6b64\uff0c\u53ef\u4ee5\u8f7b\u677e\u5236\u9020\u76f8\u5173\u7684\u6574\u4f53\u3001\u6c14\u51dd\u80f6\u548c\u5e72\u51dd\u80f6\u4ee5\u53ca\u5177\u6709\u826f\u597d\u5747\u5300\u6027\u3001\u53ef\u63a7\u539a\u5ea6\u548c\u53ef\u89c2\u673a\u68b0\u6027\u80fd\u7684\u5927\u9762\u79ef\u7eb9\u7406\u8584\u819c\u3002\u6b64\u5916\uff0c\u4ece\u5206\u5b50\u548c\u82af\u7247\u7ea7\u522b\u90fd\u8bc1\u660e\uff0c\u4e0e\u4e0d\u540c\u7aef\u57fa\u5b98\u80fd\u5316\u7684 NUS-8 \u8584\u819c\u96c6\u6210\u7684\u7535\u5bb9\u4f20\u611f\u5668\u7531\u4e8e\u5176\u4e3b\u5ba2\u4f53\u76f8\u4e92\u4f5c\u7528\u800c\u5bf9\u4e19\u916e\u8868\u73b0\u51fa\u53ef\u533a\u5206\u7684\u4f20\u611f\u884c\u4e3a\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u9898\u76ee\u4e3a\u201cSolution-processable metal\u2013organic framework nanosheets with variable functionalities\u201d\u62a5\u9053\u5728Adv. Mater.\u00a0\u671f\u520a\u4e0a\u3002<\/p>\n

DOI<\/strong>\uff1a10.1002\/adma.202101257<\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/abs\/10.1002\/adma.202101257<\/a><\/p>\n

5.\u6d2a\u8302\u693f<\/strong>:<\/strong> (JACS<\/strong>) \u901a\u8fc7<\/strong>\u03c0\u00b7\u00b7\u00b7\u03c0\u5806\u79ef\u548c\u6c22\u952e\u6784\u5efa\u57fa\u4e8e<\/strong>\u03c0\u5806\u79ef\u8d85\u5206\u5b50\u7b3c\u7684\u5206\u5c42\u81ea\u7ec4\u88c5<\/strong><\/p>\n

\"\"<\/p>\n

\u901a\u8fc7\u5f31\u5206\u5b50\u95f4\u76f8\u4e92\u4f5c\u7528\u6784\u5efa\u5177\u6709\u591a\u4e2a\u4e9a\u57fa\u7684\u8d85\u5206\u5b50\u7b3c\u662f\u5316\u5b66\u4e2d\u957f\u671f\u5b58\u5728\u7684\u6311\u6218\u3002\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u03c0-\u5806\u53e0\u8d85\u5206\u5b50\u7b3c\u4ecd\u7136\u6709\u5f85\u63a2\u7d22\u3002\u6d2a\u8302\u693f<\/strong>\u9662\u58eb\u5e26\u9886\u5176\u56e2\u961f\u63d0\u4f9b\u4e86\u4e00\u7cfb\u5217\u57fa\u4e8e\u03c0\u5806\u53e0\u7b3c\u7684\u5206\u5c42\u81ea\u7ec4\u88c5\u3002\u03c0-MX \u7b3c\u5c55\u793a\u4e86\u72ec\u7279\u7684\u591a\u529f\u80fd\u6027\uff0c\u53ef\u5728\u5c42\u7ed3\u6784\u7684\u7ec4\u88c5\u8fc7\u7a0b\u4e2d\u901a\u8fc7\u4e0d\u540c\u7684\u6c22\u952e\u6a21\u5f0f\u7ed3\u5408\u591a\u79cd\u7269\u79cd\u3002\u8be5\u7814\u7a76\u6210\u679c\u4e3a\u8fdb\u4e00\u6b65\u63a2\u7d22\u57fa\u4e8e \u03c0-\u03c0 \u5806\u79ef\u5206\u5b50\u95f4\u76f8\u4e92\u4f5c\u7528\u7684\u8d85\u5206\u5b50\u7b3c\u7684\u5316\u5b66\u548c\u5206\u5c42\u7ec4\u88c5\u63d0\u4f9b\u4e86\u53c2\u8003\u3002\u8be5\u7814\u7a76\u4ee5\u9898\u76ee\u4e3a\u201cConstructing \u03c0\u2011Stacked Supramolecular Cage Based Hierarchical Self-Assemblies via \u03c0\u00b7\u00b7\u00b7\u03c0 Stacking and Hydrogen Bonding\u201d\u53d1\u8868\u4e8eJ. Am. Chem. Soc.\u4e0a\u3002<\/p>\n

DOI<\/strong>\uff1a10.1021\/jacs.1c01161<\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/pubs.acs.org\/doi\/abs\/10.1021\/jacs.1c01161<\/p>\n

6.\u6d2a\u8302\u693f<\/strong>: <\/strong>(Angew. Chem. Int. Ed.)<\/strong> \u540c\u65f6\u5177\u6709<\/strong>\u9ad8<\/strong>C2<\/sub>H2<\/sub><\/strong>\u50a8\u5b58\u91cf\u548c<\/strong>\u4f18\u5f02<\/strong>\u7684<\/strong>C2<\/sub>H2<\/sub> \/ CO2<\/sub><\/strong>\u5206\u79bb\u6027\u80fd\u7684<\/strong>\u7b3c\u72b6\u591a\u5b54\u6750\u6599<\/strong><\/p>\n

\"\"<\/p>\n

\u5438\u9644\u5206\u79bb\u5177\u6709\u73af\u4fdd\u3001\u8282\u80fd\u7b49\u4f18\u70b9\uff0c\u662f\u7eaf\u5316C2<\/sub>H2<\/sub>\u7684\u4e00\u9879\u91cd\u8981\u6280\u672f\u3002\u9664\u4e86C2<\/sub>H2 <\/sub>\/ CO2<\/sub>\u7684\u9ad8\u9009\u62e9\u6027\u4e4b\u5916\uff0c\u5bf9\u4e8eC2<\/sub>H2<\/sub>\u9ad8\u5438\u6536\u5728\u5206\u79bb\u8fc7\u7a0b\u4e2d\u4e5f\u8d77\u7740\u91cd\u8981\u7684\u4f5c\u7528\u3002\u4f46\u662f\uff0c\u5438\u9644\u80fd\u529b\u548c\u5206\u79bb\u6027\u80fd\u4e4b\u95f4\u7684\u6743\u8861\u4ecd\u7136\u662f\u4e00\u4e2a\u96be\u9898\u3002\u6d2a\u8302\u693f\u9662\u58eb\u5e26\u9886\u5176\u56e2\u961f\u5408\u6210\u4e86\u4e00\u7cfb\u5217\u7b3c\u72b6\u591a\u5b54\u6750\u6599\uff0c\u540d\u4e3aFJI-H8-R\uff08R = Me\uff0cEt\uff0cn<\/sup>Pr\u548ciPr\uff09\uff0c\u5b83\u4eec\u57281 bar\u548c298 K\u4e0b\u90fd\u5177\u6709\u8f83\u9ad8\u7684C2<\/sub>H2<\/sub>\u5438\u9644\u80fd\u529b\u3002\u52a8\u6001\u7a81\u7834\u7814\u7a76\u8868\u660e\uff0c\u5b83\u4eec\u90fd\u5177\u6709\u51fa\u8272\u7684C2<\/sub>H2<\/sub>\u00a0\/ CO2<\/sub>\u5206\u79bb\u6027\u80fd\u3002\u6b64\u5916\uff0cGrand Canonical Monte Carlo\uff08GCMC\uff09\u6a21\u62df\u7ed3\u679c\u8868\u660e\uff0c\u5408\u9002\u7684\u5b54\u9699\u7a7a\u95f4\u548c\u51e0\u4f55\u5f62\u72b6\u5bf9\u51fa\u8272\u7684\u5206\u79bb\u6027\u80fd\u8d77\u4e86\u5f88\u5927\u7684\u4f5c\u7528\u3002\u8be5\u7814\u7a76\u4ee5\u9898\u76ee\u4e3a\u201cCage\u2010like Porous Materials with Simultaneous High C2<\/sub>H2 <\/sub>Storage and Excellent C2<\/sub>H2<\/sub>\u00a0\/ CO2 <\/sub>Separation Performance\u201d\u53d1\u8868\u4e8eAngew.Chem.Int.Ed\u4e0a\u3002<\/p>\n

DOI<\/strong>\uff1a10.1002\/anie.202101907<\/strong><\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.202101907<\/p>\n

7.\u00a0\u00a0\u00a0\u00a0 \u82cf\u6210\u52c7: (Angew. Chem. Int. Ed.) \u901a\u8fc7\u9633\u79bb\u5b50\u7b3c\u5728\u6eb6\u6db2\u4e2d\u521b\u5efa\u52a8\u6001\u7eb3\u7c73\u7a7a\u95f4\u4f5c\u4e3a\u8d85\u8d8a\u9176\u6a21\u62df\u7684\u975e\u5e38\u89c4C(sp)-H\u6d3b\u5316\u7684\u591a\u89d2\u8272\u50ac\u5316\u5e73\u53f0<\/p>\n

\"\"<\/p>\n

\u4e2d\u5c71\u5927\u5b66\u7684\u82cf\u6210\u52c7\u6559\u6388\u5e26\u9886\u5176\u56e2\u961f\u7814\u7a76\u53d1\u73b0\u57fa\u4e8e[Pd6<\/sub>(RuL3<\/sub>)8<\/sub>]28+<\/sup>\u7684\u9ad8\u7535\u8377\u6b63\u914d\u4f4d\u7b3c\u5728\u6eb6\u6db2\u4e2d\u521b\u5efa\u52a8\u6001\u7eb3\u7c73\u7a7a\u95f4\uff0c\u501f\u52a9\u4eff\u751f\u7b3c\u6548\u5e94\uff0c\u591a\u89d2\u8272\u3001\u591a\u9014\u5f84\u7b3c\u7ea6\u675f\u50ac\u5316\u53ef\u5b9e\u73b0\u591a\u529f\u80fd\u548c\u5f02\u5e38\u53cd\u5e94\u6027\u3002\u8be5\u7814\u7a76\u5b9e\u73b0\u4e86\u6c34\u4e0d\u6eb6\u6027\u5e95\u7269\/\u4ea7\u7269\/\u5171\u50ac\u5316\u5242\u7684\u76f8\u8f6c\u79fb\uff0c\u4f7f\u975e\u6df7\u6eb6\u76f8\u548c\u53cc\u76f8\u50ac\u5316\u6210\u4e3a\u53ef\u80fd\uff0c\u4ece\u800c\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u7528\u7684\u50ac\u5316\u534f\u8bae\uff0c\u5c06\u5747\u76f8\u3001\u975e\u5747\u76f8\u3001\u9176\u50ac\u5316\u548c\u76f8\u8f6c\u79fb\u50ac\u5316\u7684\u4f18\u70b9\u7ed3\u5408\u8d77\u6765\u3002\u8be5\u7814\u7a76\u4ee5\u9898\u76ee\u4e3a\u201cCreating Dynamic Nanospaces in Solution by Cationic Cages as Multirole Catalytic Platform for Unconventional C(sp)\u2212H Activation Beyond Enzyme Mimics\u201d\u53d1\u8868\u4e8eAngew.Chem.Int.Ed\u4e0a\u3002<\/p>\n

DOI<\/strong>\uff1a10.1002\/anie.202114070<\/strong>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.202114070<\/a><\/p>\n

8.\u9648\u90a6\u6797: (Angew. Chem. Int. Ed.) \u5728\u4e09\u7ef4\u5171\u4ef7\u6709\u673a\u6846\u67b6\u4e2d\u6700\u5927\u5316\u7535\u6d3b\u6027\u4f4d\u70b9\u663e\u8457\u63d0\u9ad8\u7535\u50ac\u5316\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f<\/p>\n

\"\"<\/p>\n

\u8be5\u7814\u7a76\u901a\u8fc7\u915e\u83c1\u57fa\u56db\u9178\u9150\u548c1,3,5,7-\u56db\uff084-\u6c28\u57fa\u82ef\u57fa\uff09\u91d1\u521a\u70f7\u4e4b\u95f4\u7684\u4e9a\u80fa\u5316\u53cd\u5e94\u6784\u5efa\u4e863D\u9170\u4e9a\u80fa\u952e\u5408COFs\uff0c\u5e76\u5c06\u5176\u7528\u4e8e CO2<\/sub>\u8fd8\u539f\u53cd\u5e94\u7535\u50ac\u5316\uff0c\u663e\u793a\u51fa\u9ad8CO2<\/sub>\u5230CO\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u3002\u503c\u5f97\u4e00\u63d0\u7684\u662f\u4e0e\u5177\u6709\u76f8\u540c\u915e\u83c1\u4e9a\u5355\u5143\u7684 2D COF \u7535\u50ac\u5316\u5242\u76f8\u6bd4\uff0c\u8fd9\u79cd 3D COF\u7684\u6d3b\u6027\u7535\u50ac\u5316\u4e2d\u5fc3\u548c\u7535\u6d41\u5bc6\u5ea6\uff08jCO\uff09\u5f97\u5230\u4e86\u663e\u7740\u6539\u5584\u3002\u8be5\u7814\u7a76\u4ee5\u9898\u76ee\u4e3a\u201cMaximizing Electroactive Sites in a Three-Dimensional Covalent Organic Framework for Significantly Improved Carbon Dioxide Reduction Electrocatalysis\u00a0<\/a>\u201d\u53d1\u8868\u4e8eAngew.Chem.Int.Ed\u4e0a\u3002<\/p>\n

DOI:<\/strong>\u00a010.1002\/anie.202114244<\/a>\u00a0<\/p>\n

\u539f\u6587\u94fe\u63a5<\/strong>\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/abs\/10.1002\/anie.202114244<\/p>\n","protected":false},"excerpt":{"rendered":"

1.\u00a0\u00a0\u00a0 Yaghi\uff1a(Angew.Chem.Int.Ed) \u00a0Cu(I)\u548c Ag(I)\u5bf9\u63a5\u7684\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u53ef\u7528\u4e8e\u5438\u9644\u548c\u5206\u79bb\u6c19\u6c14 Omar M.Yaghi\u6559\u6388…<\/p>\n","protected":false},"author":2,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-231247","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231247"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=231247"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231247\/revisions"}],"predecessor-version":[{"id":231275,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/231247\/revisions\/231275"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=231247"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=231247"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=231247"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}