{"id":231138,"date":"2021-12-27T06:24:30","date_gmt":"2021-12-26T22:24:30","guid":{"rendered":"\/\/m.iemloyee.com\/?p=231138"},"modified":"2021-12-26T20:36:35","modified_gmt":"2021-12-26T12:36:35","slug":"nature-%e9%87%91%e5%b1%9e%e5%8c%96%e5%90%88%e7%89%a9%e7%9a%84%e9%80%89%e6%8b%a9%e6%80%a7%e7%a1%ab%e5%8c%96","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=231138","title":{"rendered":"Nature: \u91d1\u5c5e\u5316\u5408\u7269\u7684\u9009\u62e9\u6027\u786b\u5316"},"content":{"rendered":"<p><strong>\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n<p>\u4ee5\u53ef\u518d\u751f\u7535\u529b\u4e3a\u793e\u4f1a\u63d0\u4f9b\u52a8\u529b\u6240\u9700\u7684\u57fa\u7840\u8bbe\u65bd\uff08\u78c1\u94c1\u3001\u7535\u6c60\u3001\u50ac\u5316\u5242\u3001\u7535\u5b50\u8bbe\u5907\uff09\u5bf9\u5173\u952e\u7684\u526f\u4ea7\u54c1\u91d1\u5c5e\u5143\u7d20\u6709\u7740\u524d\u6240\u672a\u6709\u7684\u8feb\u5207\u9700\u6c42\u3002\u7136\u800c\uff0c\u4ece\u77ff\u7269\u548c\u56de\u6536\u6d41\u4e2d\u63d0\u53d6\u8fd9\u4e9bd-\u548cf-\u5d4c\u6bb5\u91d1\u5c5e\u5728\u70ed\u529b\u5b66\u4e0a\u662f\u56f0\u96be\u7684\uff0c\u901a\u5e38\u9700\u8981\u5b8c\u5168\u6eb6\u89e3\u6750\u6599\uff0c\u7136\u540e\u4f7f\u7528\u91d1\u5c5e\u79bb\u5b50\u7edc\u5408\u6216\u87af\u5408\u884c\u4e3a\u8fdb\u884c\u6db2-\u6db2\u5206\u79bb\u3002\u8fd9\u4e9b\u91d1\u5c5e\u7684\u76f8\u4f3c\u7535\u5b50\u7ed3\u6784\u5bfc\u81f4\u5206\u79bb\u7cfb\u6570\u5dee\uff0c\u9700\u8981\u5927\u91cf\u7684\u80fd\u6e90\u3001\u6c34\u548c\u5316\u5b66\u54c1\u6d88\u8017\u3002<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u7f8e\u56fd\u9ebb\u7701\u7406\u5de5\u5b66\u9662Antoine Allanore\u8bfe\u9898\u7ec4\uff0c\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u9009\u62e9\u6027\u9634\u79bb\u5b50\u4ea4\u6362\u7684\u5904\u7406\u65b9\u6cd5\u3002\u901a\u8fc7\u91d1\u5c5e\u5316\u5408\u7269\u7684\u9009\u62e9\u6027\u786b\u5316\uff0c\u5229\u7528\u786b\u5316\u7269\u548c\u6c27\u5316\u7269\u4e4b\u95f4\u7684\u7269\u7406\u548c\u5316\u5b66\u5dee\u5f02(\u5982\u5bc6\u5ea6\u3001\u78c1\u5316\u7387\u3001\u8868\u9762\u5316\u5b66\u7b49)\u53ef\u4ee5\u5927\u5927\u6539\u5584\u6db2\u6db2\u5206\u79bb\u65b9\u6cd5\u3002\u672c\u5de5\u4f5c\u63d0\u4f9b\u4e8656\u79cd\u5143\u7d20\u7684\u786b\u5316\u5de5\u827a\u6761\u4ef6\uff0c\u5e76\u5bf9\u5176\u4e2d15\u79cd\u5143\u7d20\u8fdb\u884c\u4e86\u6f14\u793a\u3002\u5bf9\u73af\u5883\u548c\u7ecf\u6d4e\u5f71\u54cd\u7684\u8bc4\u4f30\u8868\u660e\uff0c\u4e0e\u6db2-\u6db2\u6e7f\u6cd5\u51b6\u91d1\u76f8\u6bd4\uff0c\u6539\u5584\u540e\u7684\u5206\u79bb\u65b9\u6cd5\u53ef\u51cf\u5c1160-90%\u7684\u6e29\u5ba4\u6c14\u4f53\u6392\u653e\uff0c\u540c\u65f6\u663e\u7740\u8282\u7701\u5206\u79bb\u6210\u672c\u3002\u76f8\u5173\u8bba\u6587\u4ee5\u9898\u4e3a\u201cSelective sulfidation of metal compounds\u201d\u4e8e2021\u5e7412\u670817\u65e5\u53d1\u8868\u5728Nature\u4e0a\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u89e3\u6790\u3011<\/strong><\/p>\n<p>\u4e00\u3001\u786b\u5316\u70ed\u529b\u5b66\u548c\u52a8\u529b\u5b66\u3002<\/p>\n<p>\u5982\u56fe1a\u6240\u793a\uff0c\u5316\u5408\u7269\u5206\u79bb\u7684\u96be\u6613\u7a0b\u5ea6\u662f\u7531\u5b83\u4eec\u7684\u76f8\u5bf9\u7a33\u5b9a\u6027\u4e4b\u95f4\u7684\u5dee\u5f02\u5b9a\u4e49\u7684\uff0c\u5bf9\u4e8e\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\uff0c\u901a\u8fc7\u6c27\u548c\u786b\u5206\u538b\uff08[P<sub>O2<\/sub>]<sub>crit<\/sub>\uff0c[P<sub>S2<\/sub>]<sub>crit<\/sub>\uff09\u6765\u63cf\u8ff0 \u8fd8\u539f\u7ed9\u5b9a\u7684\u91d1\u5c5e\u5316\u5408\u7269\u3002\u5728\u706b\u6cd5\u51b6\u91d1\u8fd8\u539f\u8fc7\u7a0b\u4e2d\uff0cPO<sub>2<\/sub>\u548cP<sub>S2<\/sub>\u7684\u5206\u538b\u901a\u5e38\u7531CO\/CO<sub>2<\/sub>\u3001H<sub>2<\/sub>\/H<sub>2<\/sub>O\u6216H<sub>2<\/sub>\/H<sub>2<\/sub>S\u7b49\u6c14\u4f53\u6bd4\u4f8b\u6765\u8bbe\u5b9a\uff0c\u4f46\u7531\u4e8e\u8fd9\u4e9b\u6c14\u4f53\u901a\u5e38\u53cd\u5e94\u751f\u6210\u91d1\u5c5e\u78b3\u5316\u7269\u6216\u6c22\u5316\u7269\uff0c\u8fd9\u4e9b\u6bd4\u4f8b\u5f88\u96be\u63a7\u5236\u3002\u4e0e\u5355\u72ec\u7528\u4e8e\u6c27\u5316\u7269\u8fd8\u539f\u7684P<sub>O2<\/sub>\u548c\u5355\u72ec\u7528\u4e8e\u786b\u5316\u7269\u8fd8\u539f\u7684P<sub>S2<\/sub>\u4e0d\u540c\uff0c\u539f\u5219\u4e0a\u652f\u6301\u91d1\u5c5e\u6c27\u5316\u7269\u7684\u9009\u62e9\u6027\u786b\u5316\uff0c\u53ef\u4ee5\u7cbe\u786e\u63a7\u5236\u6c27\u5316\u7269\u786b\u5316\u7684P<sub>S2<\/sub>\/P<sub>SO2<\/sub>\u6bd4\u503c\u3002\u968f\u7740\u56fa\u4f53\u7269\u6599\u8fdb\u6599\u5185\u90e8\u9009\u62e9\u6027\u5f62\u6210\u786b\u5316\u7269\u76f8\uff0c\u57fa\u4e8e\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\u76f8\u7269\u7406\u6027\u8d28\u5dee\u5f02\u7684\u7269\u7406\u5206\u79bb\u6210\u4e3a\u53ef\u80fd\u3002<\/p>\n<p>[P<sub>S2<\/sub>\/PS<sub>O2<\/sub>]<sub>crit<\/sub>\u00a0\u5728\u5b9a\u4e49\u786b\u5316\u7684\u70ed\u529b\u5b66\u666f\u89c2\u7684\u540c\u65f6\uff0c\u8fd8\u63cf\u8ff0\u4e86\u5728\u53cd\u5e94\u5668\u5185\u53d1\u751f\u786b\u5316\u6240\u5141\u8bb8\u7684S<sub>2<\/sub>\u5165\u53e3\u548cSO<sub>2<\/sub>\u79ef\u7d2f\uff0c\u5141\u8bb8\u8003\u8651\u4f20\u8f93\u548c\u52a8\u529b\u5b66\u6548\u5e94\u3002\u53ef\u4ee5\u533a\u5206\u63a7\u5236P<sub>S2<\/sub>\u548cP<sub>SO2<\/sub>\u7684\u4e09\u79cd\u53ef\u80fd\u6027\uff1ai)\u786b\u5316\u53cd\u5e94\u7684\u56fa\u6709\u901f\u7387\uff0cii)\u8fdb\u51fa\u53cd\u5e94\u5668\u7684\u6c14\u4f53\u7a7a\u95f4\u65f6\u95f4\u548c\u901f\u5ea6\uff0c\u4ee5\u53ca iii)S<sub>2<\/sub>\u548cS<sub>O2<\/sub>\u4e0e\u5185\u90e8\u5176\u4ed6\u7269\u8d28\u7684\u7684\u5316\u5b66\u53cd\u5e94\u3002\u672c\u5de5\u4f5c\u5c55\u793a\u4e86\u7531\u70ed\u6d3b\u5316\u5dee\u5f02\u63d0\u4f9b\u7684\u53ef\u80fd\u6760\u6746\u4f5c\u7528\u6765\u63a7\u5236\u5177\u6709\u4e0d\u540c\u7194\u5316\u6e29\u5ea6\u7684\u6c27\u5316\u7269\u7684\u786b\u5316\u3002\u5728\u6b64\u901a\u8fc7\u5bf9\u94c1\u548c\u7a00\u571f\u6c27\u5316\u7269\uff08Fe<sub>2<\/sub>O<sub>3<\/sub>\u3001Ln<sub>2<\/sub>O<sub>3<\/sub>\uff0c\u7194\u70b9 1597\u00b0C \u548c~2200-2500\u00b0C\uff09\u4e4b\u95f4\u786b\u5316\u9009\u62e9\u6027\u7684\u52a8\u529b\u5b66\u63a7\u5236\u6765\u652f\u6301\u7a00\u571f\u78c1\u4f53\u7684\u56de\u6536\u3002\u901a\u8fc7\u63a7\u5236\u78b3\u6c27\u6bd4\uff0cCDSR\u5bf9\u786b\u5316\u7684\u63a7\u5236\u5982\u56fe1b\u6240\u793a\uff0c\u8fd9\u4f53\u73b0\u5728\u5408\u6210\u7a00\u571f\u77ff\u7269\u52a0\u5de5\u8fc7\u7a0b\u4e2d\u6c27\u786b\u5316\u7269\u548c\u786b\u5316\u7269\u76f8\u7684\u9009\u62e9\u6027\u751f\u6210\u3002<\/p>\n<p>\u56fe1. \u7528\u4e8e\u91d1\u5c5e\u9009\u62e9\u6027\u786b\u5316\u7684\u786b\u4e0e\u4e8c\u6c27\u5316\u786b\u7684\u6bd4\u7387\uff0c\u4ee5\u53ca\u76f8\u5e94\u7684\u6c14\u6001\u65f6\u7a7a\u3001\u7a7a\u901f\u548c\u78b3\u70ed\u9a71\u52a8\u7684\u786b\u56de\u6d41(CDSR)\u6760\u6746<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-231143\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/12\/101.png\" alt=\"\" width=\"1009\" height=\"384\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/12\/101.png 1009w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/12\/101-300x114.png 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/12\/101-768x292.png 768w\" sizes=\"(max-width: 1009px) 100vw, 1009px\" \/><\/p>\n<p>\u4e8c\u3001\u9502\u79bb\u5b50\u7535\u6c60\u3001\u7a00\u571f\u78c1\u94c1\u56de\u6536\u53ca\u7a00\u571f\u5143\u7d20\u9009\u77ff\u3002<\/p>\n<p>\u9996\u5148\uff0c\u672c\u5de5\u4f5c\u4ee5\u9502\u79bb\u5b50\u7535\u6c60(LIBs)\u56de\u6536\u7528\u954d\u9530\u94b4\u6c27\u5316\u7269(NM )\u6b63\u6781\u6750\u6599\u7684\u65e0\u78b3\u9009\u62e9\u6027\u786b\u5316\u4e3a\u4f8b\uff0c\u7814\u7a76\u4e86[P<sub>S2<\/sub>\/P<sub>SO2<\/sub>]<sub>crt<\/sub>\u63a5\u8fd1\u4e8e1\u7684\u6df7\u5408\u91d1\u5c5e\u7684\u9009\u62e9\u6027\u786b\u5316\u548c\u5206\u79bb\uff0c\u4e00\u822c\u9002\u7528\u4e8e\u8fc7\u6e21\u91d1\u5c5e\u5206\u79bb\u3002\u5982\u56fe2a\u6240\u793a\uff0c\u5728\u786b\u5316\u540e\uff0cLIB\u6b63\u6781\u7194\u4f53\u548c\u76f8\u5206\u79bb\u6210\u4e09\u79cd\u4e0d\u6df7\u6eb6\u7684\u6db2\u4f53\uff1a\u5bcc\u954d\u786b\u5316\u7269\u3001\u5bcc\u94b4\u786b\u5316\u7269\u548c\u9530\u6c27\u786b\u5316\u7269\u3002\u540c\u65f6\uff0c\u96be\u4ee5\u4ece\u56de\u6536\u7684\u6db2\u4f53\u4e2d\u5206\u79bb\u7684\u5143\u7d20\uff0c\u5982\u94dd\uff0c\u88ab\u7145\u70e7\u6210\u6c27\u5316\u7269\u3002\u5f53\u7eb3\u5165\u786b\u5316\u7535\u8377\u540e\uff0c\u5916\u52a0S<sub>O2<\/sub>\u8fdb\u5165\u53cd\u5e94\u5668\uff0c\u94dd\u5728\u9009\u62e9\u6027\u786b\u5316\u65f6\u4ecd\u4f5c\u4e3a\u6c27\u5316\u7269\u5b58\u5728\u3002\u7834\u788e\u540e\u786b\u5316\u56fa\u4f53\u7684\u7c97\u6d6e\u9009\u663e\u793a\u954d\u94b4\u4ece\u94dd\u3001\u9502\u3001\u9530\u4e2d\u9009\u62e9\u6027\u5206\u79bb\uff0c\u7eaf\u5ea682.8%\uff0c\u56de\u6536\u738752.8%\u3002\u91c7\u7528\u78c1\u9009\u6cd5\u4ece\u94dd\u3001\u9530\u3001\u9502\u4e2d\u5206\u79bb\u94b4\u3001\u954d\uff0c\u4ea7\u54c1\u7eaf\u5ea6\u4e3a82.1%\uff0c\u56de\u6536\u7387\u4e3a84.8%\u3002\u672c\u5de5\u4f5c\u7684\u7814\u7a76\u7ed3\u679c\u8868\u660e\uff0c\u8fc7\u6e21\u91d1\u5c5e\u5143\u7d20\u4ee5\u524d\u9700\u8981\u4e00\u7cfb\u5217\u82db\u523b\u7684\u706b\u6cd5\u548c\u6e7f\u6cd5\u5206\u79bb\uff0c\u73b0\u5728\u53ef\u4ee5\u901a\u8fc7\u4e00\u4e2a\u5355\u4e00\u7684\u706b\u6cd5\u786b\u5316\u6b65\u9aa4\u5206\u79bb\uff0c\u4ea7\u751f\u4e00\u79cd\u9002\u5408\u7b80\u5355\u7684\u5e38\u89c4\u7269\u7406\u5206\u79bb\u6280\u672f\u7684\u4e2d\u95f4\u54c1\u3002<\/p>\n<p>\u5229\u7528\u786b\u5316\u52a8\u529b\u5b66\u548c\u6eb6\u6db2\u70ed\u529b\u5b66\uff0c\u901a\u8fc7\u9009\u62e9\u6027\u786b\u5316\u4ece\u590d\u6742\u9972\u6599\u4e2d\u6709\u6548\u5206\u79bb\u7269\u6599\u662f\u5fc5\u8981\u7684\u3002\u9009\u62e9\u7a00\u571f\u5143\u7d20(L)\u4ece(Nd, Pr, Dy)-Fe-B\u78c1\u4f53\u4e2d\u8403\u53d6\u5206\u79bb\u4f5c\u4e3a\u5b9e\u9645\u4f53\u7cfb\u4e2d\u786b\u5316\u9009\u62e9\u6027\u52a8\u529b\u5b66\u63a7\u5236\u7684\u6848\u4f8b\u7814\u7a76\u3002(Nd, Pr, Dy)-Fe-B\u7ecf\u9000\u78c1\u3001\u7834\u788e\u3001\u9664\u954d\u548c\u7145\u70e7\u540e\uff0c(Nd, Pr, Dy)-Fe-B\u78c1\u4f53\u6c27\u5316\u7269\u9009\u62e9\u6027\u786b\u5316\uff0c\u5f62\u6210\u5c3a\u5bf8\u7ea620~100\u00a0\u03bcm\u7684(Nd, Pr, B)<sub>2<\/sub>O<sub>3<\/sub>\u5939\u6742FeS (\u56fe2b)\u3002\u8fd9\u79cd\u5c3a\u5bf8\u6709\u671b\u901a\u8fc7\u4f18\u5316\u5f62\u6838\u3001\u957f\u5927\u548c\u7c97\u5316\u73b0\u8c61\u6765\u652f\u6301\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\u76f8\u7684\u7c89\u788e\u548c\u7269\u7406\u5206\u79bb\u3002\u5728\u6b64\uff0c(Nd, Pr, Dy)-Fe-B\u78c1\u4f53\u7684\u9009\u62e9\u6027\u786b\u5316\u56de\u6536\uff0c\u9664\u4e86\u662f\u7a33\u5b9a\u548c\u591a\u6837\u5316Ln\u4f9b\u5e94\u7684\u4e00\u4e2a\u6709\u524d\u666f\u7684\u9014\u5f84\u5916\uff0c\u663e\u793a\u4e86\u672c\u5de5\u4f5c\u65b0\u9896\u3001\u7efc\u5408\u3001\u6df1\u5165\u4e86\u89e3\u6eb6\u6db2\u70ed\u529b\u5b66\u548c\u53cd\u5e94\u52a8\u529b\u5b66\u7684\u80fd\u529b\uff0c\u6709\u52a9\u4e8e\u8bbe\u8ba1\u6709\u6548\u7684\u9009\u62e9\u6027\u786b\u5316\u5206\u79bb\u7cfb\u7edf\u3002<\/p>\n<p>\u5bf9\u4e8e\u9ad8[P<sub>S2<\/sub>\/P<sub>SO2<\/sub>]\u503c\u6750\u6599\u7684\u9009\u62e9\u6027\u786b\u5316\uff0c\u53ef\u4ee5\u901a\u8fc7CDSR\u6765\u63a7\u5236PS<sub>2<\/sub>\/P<sub>SO2<\/sub>\uff0c\u672c\u5de5\u4f5c\u63a5\u4e0b\u6765\u8ba8\u8bba\u4e86\u4ece\u6df7\u5408\u6c27\u5316\u7269\u76f8\u4e2d\u5206\u79bb\u5143\u7d20\u7684\u65b9\u6cd5\u3002\u672c\u5de5\u4f5c\u4ece(Nd, Pr, 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