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2020\u5e749\u670822\u65e5\uff0c\u5728\u7b2c75\u5c4a\u8054\u5408\u56fd\u5927\u4f1a\u4e00\u822c\u6027\u8fa9\u8bba\u4e0a\uff0c\u4e60\u8fd1\u5e73\u4e3b\u5e2d\u63d0\u51fa\uff0c\u4e2d\u56fd\u7684\u4e8c\u6c27\u5316\u78b3\u6392\u653e\u529b\u4e89\u4e8e2030\u5e74\u524d\u8fbe\u5230\u5cf0\u503c\uff0c\u52aa\u529b\u4e89\u53d62060\u5e74\u524d\u5b9e\u73b0\u78b3\u4e2d\u548c\u3002 \u4e3a\u4e2d\u56fd\u4e0b\u4e00\u9636\u6bb5\u7684\u80fd\u6e90\u8f6c\u578b\u548c\u7eff\u8272\u53d1\u5c55\u6307\u660e\u4e86\u65b9\u5411\uff0c\u8fd9\u4e9b\u5e74\u201cC\u201d\u7684C\u4f4d\u9010\u6e10\u4e0d\u4fdd\u3001\u9010\u6b65\u5411\u6e05\u6d01\u80fd\u6e90\u8f6c\u5411\u3002\u672c\u6587\u6c47\u603b\u8fd1\u671fCO2<\/sub>\u3001\u78b3\u6750\u6599\u5728\u8fd9\u79cd\u5927\u80cc\u666f\u4e0b\u5c06\u5982\u4f55\u8f6c\u5316\u7684\u6587\u7ae0\uff0c\u4f9b\u5927\u5bb6\u5b66\u4e60\u53c2\u8003\u3002<\/p>\n Nature<\/strong>\uff1a\u6765\u81ea\u9633\u5149\u548c\u7a7a\u6c14\u7684\u5ec9\u4ef7\u71c3\u6599<\/strong><\/p>\n 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Steinfeld\u3001Philipp Furler\u7b49\u4eba\u62a5\u9053\u4e86\u7528\u9633\u5149\u548c\u7a7a\u6c14\u751f\u4ea7\u71c3\u6599\uff0c\u540c\u65f6\u5b9e\u65bd\u4e86\u8be5\u8ba1\u5212\u7684\u5404\u4e2a\u6b65\u9aa4\uff0c\u6f14\u793a\u4e86\u6574\u4e2a\u70ed\u5316\u5b66\u592a\u9633\u80fd\u71c3\u6599\u751f\u4ea7\u94fe\u7684\u8fd0\u884c\uff0c\u4ece\u76f4\u63a5\u4ece\u73af\u5883\u7a7a\u6c14\u4e2d\u6355\u83b7\u7684H2<\/sub>O\u548cCO2<\/sub>\u5230\u8fd0\u8f93\u71c3\u6599\uff08\u5982\u7532\u9187\u3001\u7164\u6cb9\uff09\u7684\u5408\u6210\uff0c\u91c7\u7528\u6a21\u5757\u5316\u76845\u5343\u74e6\u4e2d\u8bd5\u89c4\u6a21\u592a\u9633\u80fd\u7cfb\u7edf\u5728\u5b9e\u9645\u73b0\u573a\u6761\u4ef6\u4e0b\u8fd0\u884c\uff0c\u5e76\u5c06\u8fdb\u4e00\u6b65\u786e\u5b9a\u7814\u53d1\u5de5\u4f5c\uff0c\u5e76\u8ba8\u8bba\u5c06\u8fd9\u4e9b\u592a\u9633\u80fd\u71c3\u6599\u63a8\u5411\u5e02\u573a\u6240\u9700\u7684\u7ecf\u6d4e\u53ef\u884c\u6027\u548c\u653f\u7b56\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cDrop-in Fuels from Sunlight and Air\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nature\u4e0a\u3002DOI: 10.1038\/s41586-021-04174-y<\/p>\n \u56fe1 \u4e09\u4e2a\u70ed\u5316\u5b66\u8f6c\u6362\u5355\u5143\u4e32\u8054\u5728\u4e00\u8d77\u7684\u592a\u9633\u80fd\u71c3\u6599\u7cfb\u7edf\u7684\u7b80\u5316\u8fc7\u7a0b<\/p>\n Nature Commun.<\/strong>\uff1a\u5355\u4f4d\u70b9\u5bcc\u96c6\u94dc\u7ed3\u6676\u591a\u5b54\u50ac\u5316\u5242\u5728<\/strong>CO2<\/sub><\/strong>\u8fd8\u539f\u4e3a<\/strong>CH4<\/sub><\/strong>\u4e2d\u7684\u914d\u4f4d\u73af\u5883\u9009\u62e9\u6027<\/strong><\/p>\n \u7535\u5316\u5b66CO2<\/sub>\u8fd8\u539f\u9ad8\u9644\u52a0\u503c\u5316\u5b66\u54c1\u662f\u80fd\u6e90\u8f6c\u6362\u9886\u57df\u6700\u6709\u524d\u9014\u548c\u6311\u6218\u6027\u7684\u7814\u7a76\u4e4b\u4e00\u3002\u5357\u4eac\u5e08\u8303\u5927\u5b66\u5170\u4e9a\u4e7e\u6559\u6388\u62a5\u9053\u4e86\u5f00\u53d1\u4e86\u4e00\u79cd\u9ad8\u5ea6\u5171\u8f6d\u7684\u7c7b\u77f3\u58a8\u70ef\u914d\u4f53\u548cCu\u8282\u70b9\u7ec4\u6210\u7684Cu\u57fa\u5bfc\u7535\u91d1\u5c5e-\u6709\u673a\u9aa8\u67b6\uff08cMOF\uff09\u7528\u4e8eCO2<\/sub>\u8fd8\u539f\u7684\u6709\u6548\u7535\u50ac\u5316\u5242\u3002\u57fa\u4e8eCu\u57fa\u5bfc\u7535\u91d1\u5c5e-\u6709\u673a\u9aa8\u67b6(Cu-DBC)\u7684\u9ad8\u6548ECR\u50ac\u5316\u5242\u80fd\u591f\u4ee5\u4f18\u5f02\u7684\u6d3b\u6027\u548c\u9009\u62e9\u6027\u5236\u5907CH4<\/sub>\uff0c\u5176\u6cd5\u62c9\u7b2c\u6548\u7387\u9ad8\u8fbe80%\uff0c\u5728\u22120.9 V \u65f6\u7535\u6d41\u5bc6\u5ea6\u4e3a\u2212203 mA cm\u22122<\/sup>\u3002\u57fa\u4e8e\u7406\u8bba\u8ba1\u7b97\u548c\u5b9e\u9a8c\u7ed3\u679c\u7684\u8fdb\u4e00\u6b65\u7814\u7a76\u8868\u660e\uff0cCu-DBC\u542b\u6c27\u4f4d\u70b9\u5728ECR\u8fc7\u7a0b\u4e2d\u5177\u6709\u8f83\u4f4e\u7684Cu-O4<\/sub>\u4f4d\u80fd\u5792\uff0c\u6bd4\u5176\u4ed6\u4e24\u79cdCu\u914d\u6c2e\u4f4d\u70b9\u5177\u6709\u66f4\u9ad8\u7684\u9009\u62e9\u6027\u548c\u6d3b\u6027\u3002\u8be5\u7814\u7a76\u63ed\u793a\u4e86\u7ed3\u6676\u591a\u5b54\u50ac\u5316\u5242\u4e2dECR\u9009\u62e9\u6027\u5bf9Cu\u4f4d\u914d\u4f4d\u73af\u5883\u7684\u5f3a\u70c8\u4f9d\u8d56\uff0c\u4e3a\u6784\u5efa\u9ad8\u9009\u62e9\u6027ECR\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u5e73\u53f0\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cCoordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2<\/sub> reduction to CH4<\/sub>\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nature Commun.\u4e0a\u3002DOI: 10.1038\/s41467-021-26724-8<\/p>\n \u56fe2 Cu-DBC\u7535\u50ac\u5316\u5242\u7684ECR-CH4<\/sub>\u6027\u80fd<\/p>\n EES<\/strong>\uff1a<\/strong>Janus<\/strong>\u754c\u9762\u5de5\u7a0b\u63a8\u52a8\u592a\u9633\u80fd\u84b8\u6c7d\u5b9e\u73b0\u9ad8\u6548\u96c6\u6c34<\/strong><\/p>\n \u592a\u9633\u80fd\u6e05\u6d01\u6c34\u751f\u4ea7\u88ab\u8ba4\u4e3a\u662f\u89e3\u51b3\u5168\u7403\u6c34\u8d44\u6e90\u77ed\u7f3a\u95ee\u9898\u7684\u4e00\u4e2a\u6709\u5229\u9014\u5f84\u3002\u592a\u9633\u80fd\u6e05\u6d01\u6c34\u751f\u4ea7\u88ab\u8ba4\u4e3a\u662f\u89e3\u51b3\u5168\u7403\u6c34\u8d44\u6e90\u77ed\u7f3a\u95ee\u9898\u7684\u4e00\u4e2a\u6709\u5229\u9014\u5f84\u3002\u7136\u800c\uff0c\u7531\u4e8e\u5165\u5c04\u9633\u5149\u4e0e\u751f\u6210\u7684\u6c34\u6c7d\u4e4b\u95f4\u5b58\u5728\u5f3a\u70c8\u7684\u76f8\u4e92\u5e72\u6270\uff0c\u4f7f\u5f97\u6bd4\u6c34\u751f\u4ea7\u529b(SWP)\u4ecd\u8fdc\u672a\u8fbe\u5230\u4ee4\u4eba\u6ee1\u610f\u7684\u6c34\u5e73\uff0c\u9020\u6210\u4e86\u5de8\u5927\u7684\u80fd\u91cf\u635f\u5931\uff0c\u8fdb\u800c\u5236\u7ea6\u4e86\u6c34\u5206\u84b8\u53d1\u548c\u6536\u96c6\u7684\u6700\u7ec8\u6548\u7387\u3002SWP\u662f\u6bcf\u5c0f\u65f6\u6bcf\u592a\u9633\u8f90\u5c04\u533a\u57df\u7684\u6c34\u6536\u96c6\u91cf\uff0c\u5b83\u53cd\u6620\u4e86\u6c34\u751f\u4ea7\u7684\u5b9e\u9645\u592a\u9633\u80fd\u6548\u7387\uff0c\u4e5f\u662f\u6d77\u6c34\u6de1\u5316\u7684\u4e00\u4e2a\u5173\u952e\u95ee\u9898\u3002\u5728\u6b64\uff0c\u6e05\u534e\u5927\u5b66\u66f2\u826f\u4f53\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cd\u5408\u7406\u7684Janus\u754c\u9762\u592a\u9633\u84b8\u6c7d\u53d1\u751f\u5668(J-SSG)\uff0c\u5b83\u5c06\u6c34\u7684\u84b8\u53d1\u548c\u592a\u9633\u70ed\u8f6c\u6362\u5206\u79bb\u5728\u8584\u819c\u53d1\u751f\u5668\u7684\u4e24\u4fa7\u3002\u8be5J-SSG\u57281\u4e2a\u592a\u9633\u7167\u5c04\u4e0b\uff0c\u5728100\u5e73\u65b9\u5398\u7c73\u7684\u5927\u9762\u79ef\u8303\u56f4\u5185\uff0c\u6c34\u5206\u84b8\u53d1\u7387\u9ad8\u8fbe2.21 kg m-2<\/sup> h-1<\/sup>\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u5728\u4e00\u4e2a\u7b80\u5355\u7684\u7cfb\u7edf\u4e2d\u5b9e\u73b0\u4e861.95 kg m-2<\/sup> h-1<\/sup>\u7684\u9ad8SWP\uff0cSWP\u4e0e\u84b8\u53d1\u7387\u4e4b\u6bd4\u5bf9\u5e94\u7684SWP\u6548\u7387\u9ad8\u8fbe88%\u3002\u5728\u5ba4\u5916\u8bd5\u9a8c(\u5317\u4eac\uff0c\u592a\u9633\u80fd~15 MJ m-2 <\/sup>day-1<\/sup>)\u4e2d\uff0c\u5f88\u5bb9\u6613\u8fbe\u5230\u6bcf\u5e73\u65b9\u7c7310\u5347\u7eaf\u51c0\u6c34\u3002\u592a\u9633\u80fd\u84b8\u6c7d\u53d1\u751f\u5668\u7684Janus\u754c\u9762\u5de5\u7a0b\u4e3a\u592a\u9633\u80fd\u5236\u6c34\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u9896\u7684\u7b56\u7565\u548c\u89e3\u51b3\u65b9\u6848\uff0c\u5177\u6709\u91cd\u8981\u7684\u73b0\u5b9e\u610f\u4e49\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cJanus-interface engineering boosting solar steam towards high-efficiency water collection\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728EES\u4e0a\u3002DOI: 10.1039\/d1ee01381e<\/p>\n \u56fe3 \u592a\u9633\u80fd\u84b8\u6c7d\u53d1\u751f\u5668\u7684\u84b8\u6c7d\u4ea7\u751f\u8fc7\u7a0b\u793a\u610f\u56fe<\/p>\n Angew.<\/strong>\uff1a\u57fa\u4e8e\u805a\u79bb\u5b50\u6db2\u4f53<\/strong>Cu(0)-Cu(I)<\/strong>\u4e32\u8054\u50ac\u5316\u5242\u4e0a\u9ad8\u6548\u7535\u50ac\u5316<\/strong>CO2<\/sub><\/strong>\u8fd8\u539f\u4e3a<\/strong>C2+<\/sub><\/strong>\u4ea7\u7269<\/strong><\/p>\n \u805a\u5408\u7269\u6539\u6027\u94dc\u57fa\u50ac\u5316\u5242\u4e0aCO2<\/sub>\u7684\u7535\u8fd8\u539f\u663e\u793a\u51fa\u9ad8\u7684\u591a\u7535\u5b50\u8fd8\u539f\uff08>2e\u2013<\/sup>\uff09\u9009\u62e9\u6027\uff0c\u800c\u5927\u591a\u6570\u76f8\u5e94\u7684\u7535\u6d41\u5bc6\u5ea6\u4ecd\u7136\u592a\u5c0f\uff0c\u65e0\u6cd5\u652f\u6301\u5de5\u4e1a\u5e94\u7528\u3002\u4e2d\u79d1\u9662\u8fc7\u7a0b\u5de5\u7a0b\u7814\u7a76\u6240\u5f90\u5b9d\u534e\u7b49\u4eba\u8bbe\u8ba1\u4e86\u4e00\u79cd\u57fa\u4e8e\u805a\u79bb\u5b50\u6db2\u4f53\uff08PIL\uff09\u7684Cu(0)-Cu(I)\u4e32\u8054\u50ac\u5316\u5242\uff0c\u7528\u4e8e\u751f\u4ea7\u5177\u6709\u9ad8\u53cd\u5e94\u901f\u7387\u548c\u9ad8\u9009\u62e9\u6027\u7684C2+<\/sub>\u4ea7\u7269\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u83b7\u5f97\u4e8676.1%\u7684\u9ad8C2+<\/sub>\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE C2+<\/sub>\uff09\u548c304.2 mA cm\u20132<\/sup>\u7684\u9ad8\u5206\u7535\u6d41\u5bc6\u5ea6\u3002\u673a\u7406\u7814\u7a76\u8868\u660e\uff0cCu(0)-PIL-Cu(I)\u754c\u9762\u7684\u6570\u91cf\u548c\u9ad8\u5ea6\u5206\u6563\u6027\u5bf9\u8be5\u53cd\u5e94\u6027\u81f3\u5173\u91cd\u8981\u3002\u5177\u4f53\u800c\u8a00\uff0c\u94dc\u7eb3\u7c73\u9897\u7c92\u884d\u751f\u7684Cu(0)-PIL\u754c\u9762\u5177\u6709\u9ad8\u7535\u6d41\u5bc6\u5ea6\u548c\u4e2d\u7b49\u7684C2+<\/sub>\u9009\u62e9\u6027\uff0c\u800cCu(I)\u7269\u79cd\u884d\u751f\u7684PIL-Cu(I)\u754c\u9762\u8868\u73b0\u51fa\u4e0e\u5c40\u90e8\u5bcc\u96c6\u7684*CO\u4e2d\u95f4\u4f53\u7684\u9ad8C\u2013C\u5076\u8054\u6d3b\u6027\u3002\u6b64\u5916\uff0cPIL\u5c42\u7684\u5b58\u5728\u901a\u8fc7\u964d\u4f4eC\u2013C\u8026\u5408\u7684\u52bf\u5792\u4fc3\u8fdb\u4e86C2+<\/sub>\u7684\u9009\u62e9\u6027\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cHighly Efficient Electrocatalytic CO2<\/sub> Reduction to C2+<\/sub> Products on a Poly(ionic liquid)-Based Cu(0)-Cu(I) Tandem Catalyst\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Angew.\u4e0a\u3002DOI: 10.1002\/anie.202110657<\/p>\n \u56fe4 Cu(0)@PIL@Cu(I)-5 \u8868\u5f81\u53caCO2<\/sub>RR\u6027\u80fd<\/p>\n AM<\/strong>\uff1a\u9ad8\u7535\u6d41\u5bc6\u5ea6\u6c34\u5206\u88c2\u7535\u50ac\u5316\u5242\u8bbe\u8ba1\u7684\u6700\u65b0\u8fdb\u5c55<\/strong><\/p>\n \u7535\u5316\u5b66\u6c34\u5206\u88c2\u6280\u672f\u751f\u4ea7\u201c\u7eff\u8272\u6c22\u201d\u662f\u5b9e\u73b0\u5168\u7403\u78b3\u4e2d\u6027\u76ee\u6807\u7684\u91cd\u8981\u6280\u672f\u3002\u5728\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5177\u6709\u826f\u597d\u6027\u80fd\u7684\u7535\u50ac\u5316\u5242\u5728\u8be5\u6280\u672f\u7684\u5de5\u4e1a\u5e94\u7528\u4e2d\u53d1\u6325\u7740\u6838\u5fc3\u4f5c\u7528\u3002\u8fd1\u5e74\u6765\uff0c\u8fd9\u4e00\u9886\u57df\u53d6\u5f97\u4e86\u5de8\u5927\u7684\u8fdb\u6b65\uff0c\u8bb8\u591a\u7c7b\u578b\u7684\u50ac\u5316\u5242\u88ab\u8bbe\u8ba1\u548c\u5408\u6210\u4e3a\u4e0e\u5de5\u4e1a\u76f8\u5173\u7684\u7535\u6d41\u5bc6\u5ea6(> 200 mA cm-2<\/sup>)\u3002\u901a\u8fc7\u8ba8\u8bba\u8fd9\u4e00\u9886\u57df\u7684\u6700\u65b0\u8fdb\u5c55\uff0c\u6e05\u534e\u5927\u5b66Liu Bilu\u3001\u5251\u6865\u5927\u5b66Manish Chhowalla\u7b49\u4eba\u603b\u7ed3\u4e86\u5f71\u54cd\u9ad8\u7535\u6d41\u5bc6\u5ea6\u7535\u50ac\u5316\u6027\u80fd\u7684\u51e0\u4e2a\u5173\u952e\u65b9\u9762\u5305\u62ec\u50ac\u5316\u5242\u7684\u7ef4\u6570\u3001\u8868\u9762\u5316\u5b66\u3001\u7535\u5b50\u4f20\u9012\u8def\u5f84\u3001\u5f62\u6001\u548c\u50ac\u5316\u5242-\u7535\u89e3\u8d28\u7684\u76f8\u4e92\u4f5c\u7528\u3002\u7814\u7a76\u5f3a\u8c03\u4e86\u5728\u5f00\u53d1\u9ad8\u7535\u6d41\u5bc6\u5ea6\u7535\u50ac\u5316\u5242\u65f6\u7efc\u5408\u8003\u8651\u8fd9\u4e9b\u65b9\u9762\u7684\u591a\u5c3a\u5ea6\u8bbe\u8ba1\u7b56\u7565\u3002\u5e76\u5bf9\u8fd9\u4e00\u65b0\u5174\u9886\u57df\u7684\u53d1\u5c55\u65b9\u5411\u63d0\u51fa\u4e86\u81ea\u5df1\u7684\u770b\u6cd5\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cRecent Advances in Design of Electrocatalysts for High-Current-Density Water Splitting\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728AM\u4e0a\u3002DOI: 10.1002\/adma.202108133<\/p>\n \u56fe5 \u9ad8\u7535\u6d41\u5bc6\u5ea6(HCD)\u7535\u50ac\u5316\u5242\u5728\u901a\u8fc7\u7535\u5316\u5b66\u6c34\u5206\u89e3\u6280\u672f\u4e0e\u53ef\u518d\u751f\u7535\u529b\u7ed3\u5408\u751f\u4ea7\u201c\u7eff\u8272\u6c22\u201d\u4e2d\u7684\u5173\u952e\u4f5c\u7528<\/p>\n Chem. Rev.<\/strong>\uff1a\u53ef\u6301\u7eed\u80fd\u6e90\u7684\u5747\u76f8\u50ac\u5316\uff1a\u6c22\u3001\u7532\u9187\u53ca\u751f\u7269\u8d28\u71c3\u6599\u76f8\u5173\u8bfe\u9898<\/strong><\/p>\n \u968f\u7740\u5168\u4e16\u754c\u627f\u8bfa\u5927\u5e45\u51cf\u5c11\u78b3\u6392\u653e\uff0c\u5bf9\u53ef\u6301\u7eed\u548c\u6e05\u6d01\u80fd\u6e90\u7684\u9700\u6c42\u73b0\u5728\u6bd4\u4ee5\u5f80\u4efb\u4f55\u65f6\u5019\u90fd\u66f4\u52a0\u91cd\u8981\u3002\u8fd9\u5305\u62ec\u80fd\u91cf\u8f7d\u4f53\u7684\u751f\u4ea7\u548c\u50a8\u5b58\uff0c\u5176\u4e2d\u5927\u90e8\u5206\u6d89\u53ca\u50ac\u5316\u53cd\u5e94\u3002\u5723\u5b89\u5fb7\u9c81\u65af\u5927\u5b66Amit Kumar\u7b49\u4eba\u7efc\u8ff0\u4e86\u8fd1\u5e74\u6765\u5747\u76f8\u50ac\u5316\u5242\u5728\u53ef\u6301\u7eed\u80fd\u6e90\u65b0\u5174\u5e94\u7528\u4e2d\u7684\u53d1\u5c55\u3002\u6700\u91cd\u8981\u7684\u7126\u70b9\u662f\u6c22\u5b58\u50a8\uff0c\u56e0\u4e3a\u6700\u8fd1\u62a5\u9053\u4e86\u51e0\u79cd\u9ad8\u6548\u7684\u5747\u76f8\u50ac\u5316\u5242\u7528\u4e8e\u6c22\u5316\u8f6c\u5316\uff0c\u6709\u671b\u5b9e\u73b0\u6c22\u7ecf\u6d4e\u3002\u5728\u8fd9\u7bc7\u7efc\u8ff0\u4e2d\u5e7f\u6cdb\u6d89\u53ca\u7684\u53e6\u4e00\u4e2a\u65b9\u5411\u662f\u7532\u9187\u3002\u8be6\u7ec6\u8ba8\u8bba\u4e86\u7528CO2<\/sub>\u3001CO\u548cHCOOH\u5236\u7532\u9187\u7684\u5747\u76f8\u50ac\u5316\u5242\u7684\u7814\u7a76\u60c5\u51b5\u3002\u6b64\u5916\uff0c\u8fd8\u8ba8\u8bba\u4e86\u4ece\u751f\u7269\u8d28\u6216\u4f4e\u70f7\u70c3\u751f\u4ea7\u4f20\u7edf\u71c3\u6599(\u5982\u67f4\u6cb9\u3001\u8721\u7b49\u9ad8\u70f7\u70c3)\u7684\u50ac\u5316\u8fc7\u7a0b\u3002\u8fd8\u6709\u4e00\u90e8\u5206\u4e13\u95e8\u7528\u4e8e\u4f7f\u7528\u5747\u76f8\u50ac\u5316\u5242\u4eceCO\u548cH2<\/sub>\u4e2d\u751f\u4ea7\u4e59\u4e8c\u9187\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cHomogeneous Catalysis for Sustainable Energy: Hydrogen and Methanol Economies, Fuels from Biomass, and Related Topics\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Chem. Rev.\u4e0a\u3002DOI: 10.1021\/acs.chemrev.1c00412<\/p>\n \u56fe6 LOHCs\u5728\u6c22\u7ecf\u6d4e\u4e2d\u7684\u4f7f\u7528\u7684\u6a21\u578b<\/p>\n EES:<\/strong>\u5916\u6e90\u7535\u5b50\u6ce8\u5165\u84dd\u85fb\u5149\u5408\u7cfb\u7edf<\/strong>I<\/strong>\u9a71\u52a8<\/strong>CO2<\/sub><\/strong>\u9ad8\u6548\u8fd8\u539f<\/strong><\/p>\n \u81ea\u7136\u754c\u7684\u751f\u7269\u50ac\u5316\u8fc7\u7a0b\u662f\u7531\u5149\u5408\u4f5c\u7528\u9a71\u52a8\u7684\uff0c\u901a\u8fc7\u5149\u5408\u4f5c\u7528\uff0c\u5149\u7cfb\u7edfI\u548c\u5149\u7cfb\u7edfII\u88ab\u4e32\u8054\u8d77\u6765\uff0c\u4ee5\u5149\u523a\u6fc0\u4ea7\u751f\u71c3\u6599\u4ea7\u54c1\u6216\u7535\u529b\u3002\u5916\u90e8\u76f4\u63a5\u5411\u5149\u5408\u7535\u5b50\u8f6c\u79fb\u94fe(PETC)\u4f9b\u7535\u6709\u8bb8\u591a\u6f5c\u5728\u7684\u597d\u5904\uff0c\u5c3d\u7ba1\u5b9e\u73b0\u8fd9\u4e00\u76ee\u6807\u7684\u7b56\u7565\u4ecd\u7136\u96be\u4ee5\u6349\u6478\u3002\u5728\u8fd9\u91cc\uff0c\u7f8e\u56fd\u56fd\u5bb6\u53ef\u518d\u751f\u80fd\u6e90\u5b9e\u9a8c\u5ba4\u7684Wei Xiong\u3001Jeffrey Blackburn\u7b49\u4eba\u62a5\u544a\u4e86\u4e00\u4e2a\u96c6\u6210\u5149\u7535\u7535\u5316\u5b66\u7ed3\u6784\uff0c\u76f4\u63a5\u7a7f\u68ad\u7535\u5b50\u5230\u751f\u6d3b\u7684\u84dd\u7ec6\u83cc\u7684PETC\u3002\u8be5\u4f53\u7cfb\u7ed3\u6784\u7684\u9634\u6781\u4e0e\u7f3a\u4e4f\u5149\u7cfb\u7edfII\u6d3b\u6027\u4e14\u4e0d\u80fd\u72ec\u7acb\u8fdb\u884c\u5149\u5408\u4f5c\u7528\u7684\u84dd\u85fb\u7ec6\u80de\u7535\u5316\u5b66\u754c\u9762\u3002\u9634\u6781\u7684\u7167\u660e\u901a\u8fc7\u5149\u7cfb\u7edfI\u5c06\u7535\u5b50\u4ece\u5916\u90e8\u7535\u8def\u4f20\u8f93\u5230\u7ec6\u80de\u5185\u7684PETC\uff0c\u6700\u7ec8\u4fc3\u8fdb\u84dd\u85fb\u7ec6\u83cc\u5c06\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u4e3a\u918b\u9178\u76d0\u3002\u5728\u95f4\u6b47\u6761\u4ef6\u4e0b\uff0c\u5373\u5728\u5149\u7167\u548c\u5916\u6e90\u7535\u5b50\u5904\u4e8e30\u79d2\u4f9b\u5e94\u52a030\u5206\u949f\u7684\u95f4\u9694\u6761\u4ef6\u65f6\uff0c\u540c\u65f6\u5411\u7cfb\u7edf\u63d0\u4f9b\u5149\u7167\u548c\u5916\u6e90\u7535\u5b50\u65f6\u624d\u4f1a\u6709\u4e59\u9178\u76d0\u7684\u5f62\u6210\u3002\u5728\u95f4\u6b47LED\u7167\u660e(400\u2013700 nm)\u548c\u5916\u6e90\u7535\u5b50\u4f9b\u5e94\u4e0b\uff0c\u751f\u6210\u4e59\u9178\u76d0\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u53ef\u8fbe9%\u3002\u8fd9\u79cd\u65b9\u6cd5\u9002\u7528\u4e8e\u901a\u8fc7\u4f7f\u7528\u5de5\u7a0b\u84dd\u85fb\u4ea7\u751f\u5404\u79cd CO2<\/sub>\u00a0\u8fd8\u539f\u4ea7\u7269\uff0c\u5176\u4e2d\u4e00\u79cd\u5df2\u7ecf\u5b9e\u73b0\u4e86\u4e59\u70ef\uff08\u4e00\u79cd\u5728\u5316\u5b66\u5de5\u4e1a\u4e2d\u5e7f\u6cdb\u4f7f\u7528\u7684\u78b3\u6c22\u5316\u5408\u7269\uff09\u7684\u5149\u7535\u751f\u4ea7\u3002\u636e\u4f30\u7b97\uff0c\u7b2c8\u5929\u65f6\u4e59\u70ef\u6548\u4ef7\u53ef\u8fbe0.365 mmol L-1<\/sup>OD730<\/sub>-1<\/sup>\uff0c\u5e73\u5747\u5916\u6e90\u7535\u5b50\u5229\u7528\u7387\u4e3a74.9%\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cExogenous electricity flowing through cyanobacterial photosystem I drives CO2<\/sub> valorization with high energy efficiency\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728EES\u4e0a\u3002DOI: 10.1039\/d1ee01526e<\/p>\n \u56fe7 \u5149\u5408\u7cfb\u7edf\u793a\u610f\u56fe<\/p>\n Science<\/strong>\uff1a\u4e8c\u6c27\u5316\u78b3\u65e0\u7ec6\u80de\u5316\u9176\u6dc0\u7c89\u5408\u6210<\/strong><\/p>\n \u6dc0\u7c89\u662f\u78b3\u6c34\u5316\u5408\u7269\u7684\u4e00\u79cd\u50a8\u5b58\u5f62\u5f0f\uff0c\u662f\u4eba\u7c7b\u996e\u98df\u4e2d\u70ed\u91cf\u7684\u4e3b\u8981\u6765\u6e90\uff0c\u4e5f\u662f\u751f\u7269\u5de5\u4e1a\u7684\u4e3b\u8981\u539f\u6599\u3002\u4e2d\u79d1\u9662\u5929\u6d25\u5de5\u4e1a\u751f\u7269\u6280\u672f\u7814\u7a76\u6240\u9a6c\u5ef6\u548c\u7b49\u4eba\u62a5\u9053\u4e86\u5728\u65e0\u7ec6\u80de\u7cfb\u7edf\u4e2d\u7531\u4e8c\u6c27\u5316\u78b3(CO2<\/sub>)\u548c\u6c22\u6c14\u5408\u6210\u6dc0\u7c89\u7684\u5316\u5b66-\u751f\u5316\u6742\u4ea4\u9014\u5f84\u3002\u4eba\u5de5\u6dc0\u7c89\u5408\u6210\u4ee3\u8c22\u9014\u5f84(ASAP)\u753111\u4e2a\u6838\u5fc3\u53cd\u5e94\u7ec4\u6210\uff0c\u901a\u8fc7\u8ba1\u7b97\u9014\u5f84\u8bbe\u8ba1\uff0c\u901a\u8fc7\u6a21\u5757\u5316\u7ec4\u88c5\u548c\u66ff\u4ee3\u5efa\u7acb\uff0c\u5e76\u901a\u8fc7\u4e09\u79cd\u74f6\u9888\u76f8\u5173\u9176\u7684\u86cb\u767d\u8d28\u5de5\u7a0b\u4f18\u5316\u3002\u5728\u4e00\u4e2a\u5177\u6709\u7a7a\u95f4\u548c\u65f6\u95f4\u5206\u79bb\u7684\u5316\u9176\u7cfb\u7edf\u4e2d\uff0c\u5728\u6c22\u7684\u9a71\u52a8\u4e0b\uff0cASAP\u5c06\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u4e3a\u6dc0\u7c89\u7684\u901f\u7387\u4e3a\u6bcf\u5206\u949f22\u7eb3\u7c73\u6469\u5c14\u7684\u4e8c\u6c27\u5316\u78b3\u6bcf\u6beb\u514b\uff0c\u662f\u7389\u7c73\u6dc0\u7c89\u5408\u6210\u901f\u7387\u76848.5\u500d\u3002\u8fd9\u79cd\u65b9\u6cd5\u4e3a\u672a\u6765\u5229\u7528\u4e8c\u6c27\u5316\u78b3\u5408\u6210\u5316\u5b66\u751f\u7269\u6742\u5316\u6dc0\u7c89\u5f00\u8f9f\u4e86\u9053\u8def\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cCell-free 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