{"id":229685,"date":"2021-11-14T06:30:15","date_gmt":"2021-11-13T22:30:15","guid":{"rendered":"\/\/m.iemloyee.com\/?p=229685"},"modified":"2021-11-13T21:12:43","modified_gmt":"2021-11-13T13:12:43","slug":"jacs%e6%bf%80%e5%ad%90%e7%bb%93%e5%90%88%e8%83%bd%e8%b0%83%e6%8e%a7%e5%8a%a9%e5%8a%9b%e6%8f%90%e9%ab%98%e4%ba%8c%e7%bb%b4%e9%92%99%e9%92%9b%e7%9f%bf%e8%87%aa%e6%97%8b%e6%9e%81%e5%8c%96%e5%af%bf","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=229685","title":{"rendered":"JACS:\u6fc0\u5b50\u7ed3\u5408\u80fd\u8c03\u63a7\u52a9\u529b\u63d0\u9ad8\u4e8c\u7ef4\u9499\u949b\u77ff\u81ea\u65cb\u6781\u5316\u5bff\u547d"},"content":{"rendered":"<p><strong>\u5168\u6587\u901f\u89c8<\/strong><\/p>\n<p>\u901a\u8fc7\u5f15\u5165\u4e0d\u540c\u4ecb\u7535\u5e38\u6570\u7684\u6709\u673a\u9633\u79bb\u5b50\uff0c\u53ef\u4ee5\u6709\u6548\u6539\u53d8\u4e8c\u7ef4\u9499\u949b\u77ff\u7684\u6fc0\u5b50\u7ed3\u5408\u80fd\uff0c\u5b9e\u73b0\u4e8c\u7ef4\u9499\u949b\u77ff\u81ea\u65cb\u6781\u5316\u5bff\u547d\u7684\u8c03\u63a7\u3002\u5229\u7528\u77ac\u6001\u5706\u504f\u632f\u53cd\u5c04\u5149\u8c31\uff08Transient Circular Polarization Spectroscopy\uff09\u8ffd\u8e2a\u53cc\u6fc0\u5b50\u4fe1\u53f7\u7684\u53d8\u5316\u89c4\u5f8b\uff0c\u8fdb\u800c\u63d0\u53d6\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u81ea\u65cb\u6781\u5316\u5bff\u547d\u3002\u5f53\u6fc0\u5b50\u7ed3\u5408\u6838\u80fd\uff08EOA<sub>2<\/sub>PbI<sub>4<\/sub>\uff09\u4e3a46 meV\u65f6\uff0c\u81ea\u65cb\u6781\u5316\u5bff\u547d\u53ef\u8fbe26ps\u3002\u8fdb\u4e00\u6b65\u7814\u7a76\u53d1\u73b0\u6fc0\u5b50\u6d53\u5ea6\u662f\u5f71\u54cd\u6fc0\u5b50\u81ea\u65cb\u5f1b\u8c6b\u7684\u91cd\u8981\u56e0\u6570\u3002\u57fa\u4e8e\u5149\u8c31\u5206\u6790\u7ed3\u679c\uff0c\u4f4e\u6fc0\u5b50\u6d53\u5ea6\u6761\u4ef6\u4e0b\uff0c\u4e8c\u7ef4\u9499\u949b\u77ff\u7684\u81ea\u65cb\u5f1b\u8c6b\u884c\u4e3a\u7531D\u2019yakonov-Perel (DP) \u673a\u5236\u8d77\u4e3b\u5bfc\u4f5c\u7528\uff1b\u9ad8\u6fc0\u5b50\u6d53\u5ea6\u6761\u4ef6\u4e3aBir\u2013Aronov\u2013Pikus (BAP) \u673a\u5236\u3002<\/p>\n<p><strong>\u80cc\u666f\u4ecb\u7ecd<\/strong><\/p>\n<p>\u4e8c\u7ef4\u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u5177\u6709\u4f18\u5f02\u7684\u5149\u5438\u6536\u7279\u6027\uff0c\u9ad8\u8367\u5149\u91cf\u5b50\u4ea7\u7387\uff08PLQY\uff09\u548c\u6613\u4e8e\u5316\u5b66\u6539\u6027\uff0c\u5728\u592a\u9633\u80fd\u7535\u6c60\uff0cLED\uff0c\u6fc0\u5149\u548c\u5149\u50ac\u5316\u7b49\u9886\u57df\u5177\u6709\u5f88\u597d\u7684\u5e94\u7528\u524d\u666f\u3002\u7531\u4e8e\u5f3a\u70c8\u7684\u81ea\u65cb\u8f68\u9053\u8026\u5408\u4f5c\u7528\uff08SOC\uff09\u548c\u7ed3\u6784\u5bf9\u79f0\u6027\u7684\u7f3a\u5931\uff0c\u4f7f\u4e8c\u7ef4\u9499\u949b\u77ff\u7684\u80fd\u7ea7\u53d1\u751f\u5288\u88c2\uff08\u4f8b\u5982Rashba-effect\uff09\uff0c\u662f\u7814\u7a76\u5ba4\u6e29\u4f4e\u7ef4\u534a\u5bfc\u4f53\u81ea\u65cb\u6781\u5316\u8fc7\u7a0b\u7684\u7406\u60f3\u5bf9\u8c61\u3002<\/p>\n<p>\u4e8c\u7ef4\u9499\u949b\u77ff\u901a\u5e38\u5177\u6709Ruddlesden-Popper\u7ed3\u6784\uff0c\u5373\u65e0\u673a\u5c42PbI<sub>6<\/sub>\u516b\u9762\u4f53\u501f\u52a9\u6709\u673a\u94f5\u9633\u79bb\u5b50\u6709\u673a\u7269\u901a\u8fc7\u9876\u89d2\u8fde\u63a5\uff08\u89c1\u56fe1a-b\uff09\u3002\u65e0\u673a\u5c42\u548c\u6709\u673a\u5c42\u4e4b\u95f4\u4ecb\u7535\u5e38\u6570\u7684\u4e0d\u5339\u914d\uff0c\u4f7f\u5149\u6fc0\u53d1\u4ea7\u751f\u7684\u6fc0\u5b50\u5c40\u57df\u5728\u65e0\u673a\u5c42\u4e2d\uff0c\u5bfc\u81f4\u5176\u6fc0\u5b50\u7ed3\u5408\u80fd\u901a\u5e38\u5728\u767e\u6beb\u7535\u5b50\u4f0f\u7279\u7684\u7ea7\u522b\u3002\u4f8b\u5982\uff0c\u7528\u975e\u6781\u6027\u7684\u6709\u673a\u7269\u914d\u4f53\uff08BA\u4e01\u80fa\uff09\u7684BA<sub>2<\/sub>PBI<sub>4<\/sub>\u7684\u6fc0\u5b50\u96c6\u5408\u80fd\u4e3a482meV\u3002\u800c\u5f53\u91c7\u7528\u5177\u6709\u8f83\u5927\u4ecb\u7535\u5e38\u6570\uff08\u03b5<sub>r<\/sub>=37.2\uff09\u7684\u4e59\u9187\u80fa\uff08EOA\uff09\u6709\u673a\u914d\u4f53\uff0c\u5176\u6fc0\u5b50\u7ed3\u5408\u53ef\u4ee5\u964d\u4f4e\u523046meV\u3002\u8f83\u4f4e\u7684\u7ed3\u5408\u80fd\u53ef\u4ee5\u6709\u6548\u5c4f\u853d\u6676\u683c\u5bf9\u5149\u751f\u6fc0\u5b50\u675f\u7f1a\uff0c\u8fdb\u800c\u63d0\u9ad8\u8f7d\u6d41\u5b50\u7684\u81ea\u65cb\u6781\u5316\u5bff\u547d\u3002\u56e0\u6b64\u501f\u52a9\u914d\u4f53\u5de5\u7a0b\u5f15\u5165\u5177\u6709\u4e0d\u540c\u4ecb\u7535\u5e38\u6570\u7684\u6709\u673a\u914d\u4f53\u6765\u8c03\u63a7\u4e8c\u7ef4\u9499\u949b\u77ff\u81ea\u65cb\u6781\u5316\u5bff\u547d\uff0c\u5bf9\u7814\u7a76\u8be5\u7c7b\u4f4e\u7ef4\u534a\u5bfc\u4f53\u6750\u6599\u7684\u81ea\u65cb\u5f1b\u8c6b\u7684\u7269\u7406\u673a\u5236\u5177\u6709\u79ef\u6781\u7684\u610f\u4e49\u3002<\/p>\n<p><strong>\u56fe\u6587\u5bfc\u8bfb<\/strong><\/p>\n<p>\u57fa\u4e8e\u6b64\u7b56\u7565\uff0c<strong>\u5357\u65b9\u79d1\u6280\u5927\u5b66\u673a\u68b0\u4e0e\u80fd\u6e90\u5de5\u7a0b\u7cfb\u9648\u71b9\u7ff0\u52a9\u7406\u6559\u6388\uff0c\u7f8e\u56fd\u56fd\u5bb6\u53ef\u518d\u751f\u80fd\u6e90\u5b9e\u9a8c\u5ba4\u7684<\/strong><strong>Matthew C. Beard 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(DP) \u673a\u5236\u8d77\u4e3b\u5bfc\u4f5c\u7528\uff1b\u9ad8\u6fc0\u5b50\u6d53\u5ea6\u6761\u4ef6\u4e3aBir\u2013Aronov\u2013Pikus (BAP) \u673a\u5236\uff0c\u53ef\u901a\u8fc7\u8c03\u63a7\u6fc0\u5b50\u7ed3\u5408\u80fd\u8c03\u63a7\u81ea\u65cb\u5bff\u547d\uff08\u56fe4\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-229686\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/1-7.png\" alt=\"\" width=\"600\" height=\"249\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/1-7.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/1-7-300x125.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe1 BA\u548cEOA\u4e8c\u7ef4\u9499\u949b\u77ff\u5355\u6676\u7684\u7ed3\u6784\u793a\u610f\u56fe\u548c\u7a33\u6001\u5438\u6536\u5149\u8c31\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-229687\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/2-6.png\" alt=\"\" width=\"600\" height=\"354\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/2-6.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/2-6-300x177.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe2 \u81ea\u65cb\u5f1b\u8c6b\u52a8\u529b\u5b66\u6d4b\u8bd5\u793a\u610f\u56fe\u548c\u4ee3\u8868\u6027\u7684TR\u8c31\u56fe\u548c\u81ea\u65cb\u5f1b\u8c6b\u52a8\u529b\u5b66\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-229688\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/3-5.png\" alt=\"\" width=\"600\" height=\"546\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/3-5.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/3-5-300x273.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe3 \u6e29\u5ea6\u548c\u6fc0\u5b50\u6d53\u5ea6\u4f9d\u8d56\u7684\u81ea\u65cb\u5f1b\u8c6b\u5bff\u547d\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-229689\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/4-6.png\" alt=\"\" width=\"600\" height=\"337\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/4-6.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/11\/4-6-300x169.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe4 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C. Beard \u9ad8\u7ea7\u7814\u7a76\u5458\u4e3a\u8be5\u8bba\u6587\u7684\u901a\u8baf\u4f5c\u8005\uff0c\u7f8e\u56fd\u53ef\u518d\u751f\u80fd\u6e90\u5b9e\u9a8c\u5ba4\u53ca\u5357\u65b9\u79d1\u6280\u5927\u5b66\u4e3a\u8bba\u6587\u901a\u8baf\u5355\u4f4d\u3002\u8be5\u7814\u7a76\u5f97\u5230\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u53ca\u7f8e\u56fd\u80fd\u6e90\u90e8\u7684\u652f\u6301\u3002<\/p>\n<p>\u6587\u7ae0\u94fe\u63a5\uff1a<\/p>\n<p>Chen, Xihan* et. al. Tuning Spin-Polarized Lifetime in Two-Dimensional Metal\u2013Halide Perovskite through Exciton Binding Energy, <em>J. Am. Chem. Soc. ASAP<\/em><\/p>\n<p><a href=\"https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.1c08514\">https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.1c08514<\/a><\/p>\n<p>\u672c\u6587\u7531\u4f5c\u8005\u6295\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u5168\u6587\u901f\u89c8 \u901a\u8fc7\u5f15\u5165\u4e0d\u540c\u4ecb\u7535\u5e38\u6570\u7684\u6709\u673a\u9633\u79bb\u5b50\uff0c\u53ef\u4ee5\u6709\u6548\u6539\u53d8\u4e8c\u7ef4\u9499\u949b\u77ff\u7684\u6fc0\u5b50\u7ed3\u5408\u80fd\uff0c\u5b9e\u73b0\u4e8c\u7ef4\u9499\u949b\u77ff\u81ea\u65cb\u6781\u5316\u5bff\u547d\u7684\u8c03\u63a7\u3002\u5229\u7528\u77ac\u6001\u5706\u504f\u632f\u53cd\u5c04\u5149\u8c31\uff08Transient C&#8230;<\/p>\n","protected":false},"author":11454,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-229685","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/229685"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=229685"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/229685\/revisions"}],"predecessor-version":[{"id":229692,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/229685\/revisions\/229692"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=229685"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=229685"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=229685"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}