{"id":227891,"date":"2021-09-30T12:00:43","date_gmt":"2021-09-30T04:00:43","guid":{"rendered":"\/\/m.iemloyee.com\/?p=227891"},"modified":"2021-09-30T11:11:10","modified_gmt":"2021-09-30T03:11:10","slug":"%e4%b8%8a%e4%ba%a4%e5%a4%a7%e7%bd%97%e5%8a%a0%e4%b8%a5adv-mater-%ef%bc%9a%e4%ba%9a5-%c2%b5m%e5%9b%ba%e4%bd%93%e8%81%9a%e5%90%88%e7%89%a9%e7%94%b5%e8%a7%a3%e8%b4%a8%e5%8a%a9%e5%8a%9b%e9%ab%98%e8%83%bd","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=227891","title":{"rendered":"\u4e0a\u4ea4\u5927\u7f57\u52a0\u4e25Adv. Mater.\uff1a\u4e9a5 \u00b5m\u56fa\u4f53\u805a\u5408\u7269\u7535\u89e3\u8d28\u52a9\u529b\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u56fa\u6001\u9502\u91d1\u5c5e\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5728\u9502\u7535\u6c60\u4e2d\uff0c\u9502\u56e0\u5176\u9ad8\u7684\u7406\u8bba\u5bb9\u91cf\uff083860 mA hg-1<\/sup>\uff09\u548c\u4f4e\u7684\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\uff08\u76f8\u5bf9\u4e8e\u6807\u51c6\u6c22\u7535\u6781\u4e3a-3.04 V\uff09\u800c\u88ab\u89c6\u4e3a\u7406\u60f3\u8d1f\u6781\uff0c\u4f46\u662f\u9502\u679d\u6676\u7684\u5f62\u6210\u548c\u751f\u957f\u963b\u788d\u4e86\u5176\u5b9e\u9645\u5e94\u7528\u3002\u56fa\u6001\u7535\u89e3\u8d28\uff08SSEs\uff09\u53ef\u4ee5\u963b\u6b62\u9502\u679d\u6676\u751f\u957f\uff0c\u4fc3\u8fdb\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u5b89\u5168\u6027\u7684\u56fa\u6001\u9502\u91d1\u5c5e\u7535\u6c60\u7684\u53d1\u5c55\u3002\u56e0\u6b64\uff0c\u5408\u7406\u8bbe\u8ba1\u9ad8\u7a33\u5b9a\u6027\u548c\u673a\u68b0\u5f3a\u5ea6\u7684SSEs\u5bf9\u4e8e\u5236\u5907\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u5b89\u5168\u6027\u7684\u9502\u7535\u6c60\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u4e3a\u4e86\u83b7\u5f97\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u957f\u5faa\u73af\u5bff\u547d\u7684\u56fa\u6001\u7535\u6c60\uff0c\u5fc5\u987b\u83b7\u5f97\u9ad8\u5e73\u5747\u5e93\u4ed1\u6548\u7387(CEavg<\/sub>)\u7684\u6709\u9650\u9502\u50a8\u5c42\u3002\u4e0e\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\u7684SSE\u76f8\u6bd4\uff0c\u805a\u5408\u7269SSE\u572811.6 \u00b5m\u7684\u539a\u5ea6\u4e0b\u53ef\u4ee5\u8fbe\u5230500 Wh kg-1<\/sup>\u7684\u80fd\u91cf\u5bc6\u5ea6\u3002\u4f46\u662f\u7531\u4e8e\u5bc6\u5ea6\u7684\u589e\u52a0\uff0c\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\u7684\u539a\u5ea6\u5fc5\u987b\u5728\u76f8\u540c\u6761\u4ef6\u4e0b\u663e\u7740\u964d\u4f4e\uff08\u6c27\u5316\u7269\u548c\u786b\u5316\u7269\u5206\u522b\u4e3a7.6\u548c2.7 \u00b5m\uff09\u3002\u7136\u800c\uff0c\u6709\u9650\u7684SSE\u539a\u5ea6\u5fc5\u7136\u4f1a\u5bfc\u81f4\u673a\u68b0\u5f3a\u5ea6\u53d8\u5dee\uff0c\u5e76\u4e14\u96be\u4ee5\u5728\u5927\u89c4\u6a21\u751f\u4ea7\u4e2d\u63a7\u5236\u4ea7\u54c1\u8d28\u91cf\u3002\u8584SSEs\u673a\u68b0\u5f3a\u5ea6\u7684\u4e0b\u964d\uff0c\u4e5f\u4f1a\u589e\u52a0\u5faa\u73af\u8fc7\u7a0b\u4e2d\u9502\u679d\u6676\u7a7f\u900f\u7684\u98ce\u9669\uff0c\u5e76\u9020\u6210\u4e25\u91cd\u7684\u5b89\u5168\u9690\u60a3\uff0c\u56e0\u6b64\u8feb\u5207\u9700\u8981\u5bf9\u8bbe\u8ba1\u8584\u800c\u575a\u56fa\u7684SSEs\u8fdb\u884c\u66f4\u591a\u7814\u7a76\u3002\u4e3a\u4e86\u89e3\u51b3\u4e0a\u8ff0\u95ee\u9898\uff0c\u4e00\u79cd\u6709\u6548\u7684\u7b56\u7565\u662f\u5c06\u521a\u6027\u9676\u74f7\u586b\u6599\u6dfb\u52a0\u5230\u67d4\u6027\u9502\u79bb\u5b50\u5bfc\u7535\u805a\u5408\u7269\u4e2d\uff0c\u8fd9\u53ef\u4ee5\u540c\u65f6\u63d0\u9ad8SSE\u7684\u79bb\u5b50\u7535\u5bfc\u7387\u3001\u673a\u68b0\u5f3a\u5ea6\u4ee5\u53ca\u70ed\u548c\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u3002\u529f\u80fd\u6027\u586b\u6599\u53ef\u4ee5\u540c\u65f6\u4e0e\u9634\u79bb\u5b50\u548c\u805a\u5408\u7269\u94fe\u6bb5\u76f8\u4e92\u4f5c\u7528\uff0c\u4ece\u800c\u4fc3\u8fdb\u5c40\u90e8\u975e\u6676\u5316\u5e76\u6539\u5584Li+<\/sup>\u4f20\u8f93\u3002\u540c\u65f6\uff0c\u9ad8\u6a21\u91cf\u548c\u7535\u5b50\u7edd\u7f18\u6027\u80fd\u4fdd\u8bc1\u4e86SSEs\u4f18\u5f02\u7684\u673a\u68b0\u548c\u7535\u5316\u5b66\u6027\u80fd\u3002\u5c06\u9502\u91d1\u5c5e\u8d1f\u6781\u4e0e\u9ad8\u538b\u6b63\u6781\u8026\u5408\u662f\u5b9e\u73b0\u9ad8\u80fd\u91cf\u5bc6\u5ea6SSB\u7684\u53e6\u4e00\u4e2a\u6709\u8da3\u7b56\u7565\uff0c\u8fd9\u9700\u8981SSE\u540c\u65f6\u5bf9Li\u7535\u5316\u5b66\u7a33\u5b9a\u5e76\u4e0e\u9ad8\u538b\u6b63\u6781\u517c\u5bb9\u3002\u7136\u800c\uff0c\u7531\u4e8e\u56fa\u6709\u7684\u6709\u9650\u7535\u5316\u5b66\u7a97\u53e3\uff0c\u5f88\u5c11\u6709SSE\u663e\u793a\u51fa\u6709\u5e0c\u671b\u7684\u80fd\u529b\u3002\u5e76\u4e14\u6709\u5fc5\u8981\u8bbe\u8ba1\u4e00\u79cd\u591a\u5c42\u7535\u89e3\u8d28\u4ee5\u540c\u65f6\u8010\u53d7\u8fd8\u539f\u548c\u6c27\u5316\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u56fd\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66<\/strong>\u7684\u7f57\u52a0\u4e25\u6559\u6388\uff08\u901a\u8baf\uff09<\/strong>\u4f5c\u8005\u7b49\u4eba\u63d0\u51fa\u4e86\u4e00\u79cd\u591a\u5b54\u9676\u74f7\u652f\u67b6\u548c\u53cc\u5c42Li+<\/sup>\u5bfc\u7535\u805a\u5408\u7269\u7684\u8d85\u8584(4.2 \u00b5m)\u53cc\u5c42SSEs\u3002\u8010\u706b\u4e14\u575a\u786c\u7684\u9676\u74f7\u652f\u67b6\u63d0\u9ad8\u4e86\u590d\u5408SSEs\u7684\u5b89\u5168\u80fd\u529b\u548c\u673a\u68b0\u5f3a\u5ea6\uff0c\u53cc\u5c42\u805a\u5408\u7269\u7ed3\u6784\u589e\u5f3a\u4e86\u9502\u91d1\u5c5e\u8d1f\u6781\u548c\u9ad8\u538b\u6b63\u6781\u7684\u76f8\u5bb9\u6027\u30023D\u9676\u74f7\u4fc3\u8fdb\u9502\u79bb\u5b50\u4f20\u5bfc\u5e76\u8c03\u8282\u9502\u6c89\u79ef\u3002\u56e0\u6b64\uff0c\u57fa\u4e8e\u5177\u6709\u4f4eN\/P\u6bd4\u548c\u8d85\u8fc73000\u5c0f\u65f6\u957f\u5bff\u547d\u7684LiNi0.8<\/sub>Co0.1<\/sub>Mn0.1<\/sub>O2<\/sub>(NCM811)\u6b63\u6781\uff0c\u5b9e\u73b0\u4e86506 Wh kg-1<\/sup>\u548c1514 Wh L-1<\/sup>\u7684\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>High Energy Density Solid State Lithium Metal Batteries Enabled by Sub-5 \u00b5m Solid Polymer Electrolytes<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Advanced Materials<\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong> 1 <\/strong>\u53cc\u5c42<\/strong>UFF\/PEO\/PAN\/LiTFSI SSE<\/strong>\u7684\u5236\u5907\u548c\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u53cc\u5c42UFF\/PEO\/PAN\/LiTFSI SSE\u7684\u5236\u5907\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u94dd\u7b94\u4e0a\u7684UFF\u7167\u7247\uff1b<\/p>\n

\uff08c\uff09UFF\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09\u53cc\u5c42UFF\/PEO\/PAN\/LiTFSI SSE\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff09F\u3001Si\u548cN\u5143\u7d20\u7684UFF\/PEO\/PAN\/LiTFSI SSE\u548cEDS\u56fe\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09\u6765\u81eaToF-SIMS\u6d4b\u8bd5\u76843D\u89c6\u56fe\u4e2dUFF\/PEO\/PAN\/LiTFSI\u7684F\u3001N\u3001O\u548cSi\u5206\u5e03\uff0c\u4ee5\u53ca\u4f5c\u4e3a\u7b49\u6548\u6df1\u5ea6\u51fd\u6570\u7684\u76f8\u5173\u7269\u79cd\u7684\u5f3a\u5ea6\u6f14\u53d8\u3002<\/p>\n

\u56fe<\/strong> 2 UFF\/PEO\/PAN\/LiTFSI<\/strong>\u7684\u7535\u5316\u5b66\u8868\u5f81\u548c\u9632\u706b\u5b89\u5168\u6d4b\u8bd5<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09DFT\u8ba1\u7b97\u4e86PEO\u548cPAN\u5355\u4f53\u5728UFF\u4e0a\u7684\u5438\u9644\u80fd\uff1b<\/p>\n

\uff08b\uff09\u8fde\u7eedUFF-\u805a\u5408\u7269\u754c\u9762\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08c\uff09SS|SSE|SS\u7535\u6c60\u7684\u963b\u6297\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09\u9ad8\u6e29\u4e0bSSE\u7684Arrhenius\u56fe\uff1b<\/p>\n

\uff08e\uff09UFF\/PEO\/PAN\/LiTFSI\u548cPEO\/PAN\/LiTFSI\u7535\u89e3\u8d28\u7684PEO\u4fa7\u7684\u7eb3\u7c73\u538b\u75d5\u6d4b\u8bd5\uff1b<\/p>\n

\uff08f\uff09PEO\/PAN\/LiTFSI\u8584\u819c\u548c\u86ed\u77f3(VM)\u8584\u819c\u7684\u706b\u7130\u6d4b\u8bd5\u7167\u7247\uff1b<\/p>\n

\uff08g\uff09UFF\/PEO\/PAN\/LiTFSI\u7535\u89e3\u8d28\u7684\u7535\u5316\u5b66\u7a97\u53e3\uff1b<\/p>\n

\uff08h\uff09\u4e0d\u540c\u7535\u89e3\u8d28\u5bf9Li|Cu\u534a\u7535\u6c60\u4e2d\u9502\u91d1\u5c5eCE\u7684Aurbach\u6d4b\u91cf\u3002<\/p>\n

\u56fe<\/strong> 3 <\/strong>\u9ad8\u8d1f\u8f7d<\/strong>NCM SSBs<\/strong>\u7684\u5faa\u73af\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff0cb\uff09Li|UFF\/PEO\/PAN\/LiTFSI|NCM811 SSB\u7684\u957f\u5faa\u73af\u548c\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08c\uff09Li|UFF\/PEO\/PAN\/LiTFSI|NCM622 SSB\u7684\u957f\u5faa\u73af\u548c\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08e\uff09\u56fa\u6001\u9502\u7535\u6c60\u4e0e\u5df2\u62a5\u5230\u7684\u65e0\u673a-\u805a\u5408\u7269\u590d\u5408\u7535\u89e3\u8d28\u7684\u5bb9\u91cf-\u7535\u538b\u6bd4\u8f83\u56fe\u3002<\/p>\n

\u56fe<\/strong> 4 UFF\/PEO\/PAN\/LiTFSI<\/strong>\u7684\u65e0\u8d1f\u6781\u5168\u7535\u6c60\u548c\u8f6f\u5305\u7535\u6c60\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u9ad8\u9762\u79ef\u5bb9\u91cf\uff083.6 mAh cm-2<\/sup>\uff09\u7684NCM811\u6b63\u6781\u3001\u8d85\u8584UFF\/PEO\/PAN\/LiTFSI\u7535\u89e3\u8d28\u4e14\u65e0\u9502\u8d1f\u6781\u7ec4\u6210\u7684\u5168\u7535\u6c60\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u57280.1 C\u5145\u7535\/0.5 C\u653e\u7535\u4e0b\uff0cUFF\/PEO\/PAN\/LiTFSI\u56fa\u4f53\u7535\u89e3\u8d28\u548cLiPF6<\/sub>\/EC\/DEC\u6db2\u4f53\u7535\u89e3\u8d28\u7684\u65e0\u8d1f\u6781\u7535\u6c60\u7684\u5faa\u73af\u6b21\u6570\u4e0e\u5f52\u4e00\u5316\u5bb9\u91cf\u4fdd\u6301\u7387\u548c\u5e93\u4ed1\u6548\u7387\u7684\u5173\u7cfb\u56fe\uff1b<\/p>\n

\uff08c\uff09\u6db2\u4f53\u7535\u89e3\u8d28LiPF6<\/sub>\/EC\/DEC\u7684\u65e0\u8d1f\u6781Cu|NMC811(3.6 mAh cm-2<\/sup>)\u7535\u6c60\u5faa\u73af10\u6b21\u540e\u7684Li\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff0ce\uff09UFF\/PEO\/PAN\/LiTFSI SSE\u7684\u65e0\u8d1f\u6781Cu|NMC811(3.6 mAh cm-2<\/sup>)\u7535\u6c60\u5faa\u73af10\u6b21\u7684Li\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09\u57280.35 mA cm-2<\/sup>\u4e0b\uff0cUFF\/PEO\/PAN\/LiTFSI SSE\u4e2d\u9502\u79bb\u5b50\u68af\u5ea6\u7684\u6a21\u62df\u56fe\uff1b<\/p>\n

\uff08g\uff09\u57280.35\u548c3.5 mA cm-2<\/sup>\u65f6\uff0c\u6a21\u62dfSSE\u4e2d\u6cbfY\u8f74\u7684\u9502\u79bb\u5b50\u6d53\u5ea6\uff1b<\/p>\n

\uff08h\uff09\u57280.45 mAcm-2<\/sup>\u4e0b\uff0cLi|UFF\/PEO\/PAN\/LiTFSI|NCM811\u8f6f\u5305\u7535\u6c60\u7b2c\u4e8c\u5708\u7684\u5145\u7535\/\u653e\u7535\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08i\uff09\u5728\u6b63\u5e38\u3001\u5f2f\u66f2\u548c\u5207\u5272\u72b6\u6001\u4e0b\uff0c\u6ee1\u7535\u7684Li|UFF\/PEO\/PAN\/LiTFSI|NCM811\u8f6f\u5305\u7535\u6c60\u70b9\u4eae\u53d1\u5149\u4e8c\u6781\u7ba1\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>High Energy Density Solid State Lithium Metal Batteries Enabled by Sub-5 \u00b5m Solid Polymer Electrolytes<\/a>\uff08Advanced Materials, 2020, 10.1002\/adma.202105329\uff09\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1a<\/strong>cailiaokefu<\/strong>\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n

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 <\/p>\n","protected":false},"excerpt":{"rendered":"

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