{"id":227412,"date":"2021-09-18T06:30:05","date_gmt":"2021-09-17T22:30:05","guid":{"rendered":"\/\/m.iemloyee.com\/?p=227412"},"modified":"2021-09-17T21:50:20","modified_gmt":"2021-09-17T13:50:20","slug":"2021%e5%b9%b49%e7%af%87nature%e7%b3%bb%e5%88%97%e7%9b%98%e7%82%b9%ef%bc%8c%e5%9b%ba%e6%80%81%e7%94%b5%e6%b1%a0%e9%a2%86%e5%9f%9f%e8%83%bd%e5%90%a6%e5%bc%95%e5%af%bc%e6%96%b0%e7%9a%84%e8%83%bd%e6%ba%90","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=227412","title":{"rendered":"2021\u5e749\u7bc7Nature\u7cfb\u5217\u76d8\u70b9\uff0c\u56fa\u6001\u7535\u6c60\u9886\u57df\u80fd\u5426\u5f15\u5bfc\u65b0\u7684\u80fd\u6e90\u9769\u547d"},"content":{"rendered":"

\u56fa\u6001\u7535\u6c60\u4f5c\u4e3a\u4e00\u79cd\u96c6\u9ad8\u80fd\u91cf\u9ad8\u529f\u7387\u5bc6\u5ea6\uff0c\u9ad8\u5b89\u5168\u6027\u7b49\u8bf8\u591a\u4f18\u70b9\u4e8e\u4e00\u8eab\u7684\u50a8\u80fd\u65b0\u4f53\u7cfb\uff0c\u4e00\u76f4\u53d7\u5230\u4e1a\u754c\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u7279\u522b\u662f\u65b0\u80fd\u6e90\u6c7d\u8f66\u9886\u57df\u3002\u4eca\u5e74\u4e5d\u6708\u4e03\u65e5\uff0c\u65e5\u672c\u4e30\u7530\u516c\u53f8\u53ec\u5f00\u4e86\u7535\u6c60\u4e0e\u78b3\u4e2d\u548c\u53d1\u5e03\u4f1a\uff0c\u4f1a\u4e0a\u5c55\u793a\u4e86\u5176\u6700\u65b0\u7814\u53d1\u7684\u56fa\u6001\u7535\u6c60\u65b0\u80fd\u6e90\u8f66\uff0c\u5f15\u8d77\u4e86\u5de8\u5927\u7684\u8f70\u52a8\u3002\u7531\u6b64\u53ef\u89c1\uff0c\u56fa\u6001\u7535\u6c60\u53ef\u80fd\u662f\u4e0b\u4e00\u4ee3\u65b0\u80fd\u6e90\u6c7d\u8f66\u6280\u672f\u5b9e\u73b0\u98a0\u8986\u6027\u9769\u65b0\u7684\u5173\u952e\u3002\u4f46\u662f\uff0c\u5168\u56fa\u6001\u7535\u6c60\u7684\u5546\u4e1a\u5316\u4ecd\u7136\u5b58\u5728\u7406\u8bba\u548c\u5b9e\u9645\u4e0a\u7684\u6311\u6218\uff0c\u5982\u79bb\u5b50\u4f20\u8f93\u52a8\u529b\u5b66\u8fdf\u7f13\uff0c\u754c\u9762\u7a33\u5b9a\u6027\u5dee\uff0c\u7ec4\u88c5\u96be\u5ea6\u5927\uff0c\u6210\u672c\u9ad8\u7b49\u95ee\u9898\u3002\u9488\u5bf9\u8fd9\u4e9b\u56fa\u6709\u6311\u6218\uff0c\u5927\u91cf\u5b66\u8005\u653b\u575a\u514b\u96be\uff0c\u53d6\u5f97\u4e86\u4e00\u7cfb\u5217\u91cd\u5927\u7a81\u7834\uff0c\u63a8\u52a8\u4e86\u56fa\u6001\u7535\u6c60\u7684\u957f\u8db3\u53d1\u5c55\u3002\u63a5\u4e0b\u6765\uff0c\u672c\u6587\u5c06\u70b9\u8bc42021\u5e74Nature\u53ca\u5176\u5b50\u520a\u5728\u56fa\u6001\u7535\u6c60\u9886\u57df\u62a5\u9053\u7684\u4e00\u4e9b\u7a81\u7834\u6027\u8fdb\u5c55\uff0c\u4ee5\u5e2e\u52a9\u5927\u5bb6\u66f4\u597d\u5730\u7406\u89e3\u8fd9\u95e8\u65b0\u578b\u50a8\u80fd\u6280\u672f\u3002<\/p>\n

Nature(IF<\/b><\/strong>\uff1a<\/b><\/strong>49.962)<\/b><\/strong>\uff1a\u9502\u91d1\u5c5e\u56fa\u6001\u7535\u6c60\u7684\u52a8\u6001\u7a33\u5b9a\u6027\u8bbe\u8ba1\u7b56\u7565<\/b><\/strong><\/p>\n

\u56fa\u6001\u7535\u89e3\u8d28\u5177\u6709\u9ad8\u673a\u68b0\u5f3a\u5ea6\uff0c\u6709\u671b\u6291\u5236\u9502\uff08Li\uff09\u679d\u6676\u6e17\u900f\u3002\u7136\u800c\uff0c\u5728\u5b9e\u9645\u4e2d\uff0c\u5b9e\u73b0\u65e0\u679d\u6676\u9502\u91d1\u5c5e\u8d1f\u6781\u4ecd\u7136\u5177\u6709\u6311\u6218\u6027\uff0c\u56e0\u4e3a\u5728\u7535\u6c60\u7ec4\u88c5\u6216\u957f\u5faa\u73af\u8fc7\u7a0b\u4e2d\u7ecf\u5e38\u4f1a\u5728\u9676\u74f7\u9897\u7c92\u4e2d\u4ea7\u751f\u5fae\u7c73\u6216\u4e9a\u5fae\u7c73\u7ea7\u7684\u88c2\u7eb9\u3002\u4e00\u65e6\u88c2\u7eb9\u5f62\u6210\uff0c\u9502\u679d\u6676\u6e17\u900f\u4e0d\u53ef\u907f\u514d\u3002\u5728\u8fd9\u7bc7Nature\u4e2d\uff0c\u54c8\u4f5b\u5927\u5b66\u674e\u946b\u6559\u6388\u8bbe\u8ba1\u4e86\u4e00\u79cd\u5177\u6709\u591a\u5c42\u56fa\u6001\u7535\u89e3\u8d28\u7ed3\u6784\u7684\u56fa\u6001\u7535\u6c60\uff0c\u4ee5\u5b9e\u73b0\u8d85\u9ad8\u7535\u6d41\u5bc6\u5ea6\u5e76\u6291\u5236\u9502\u679d\u6676\u6e17\u900f\u3002\u591a\u5c42\u7ed3\u6784\u4e3a\u5c06\u4e0d\u592a\u7a33\u5b9a\u7684\u7535\u89e3\u8d28\u5939\u5728\u7a33\u5b9a\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u4e4b\u95f4\uff0c\u901a\u8fc7\u4e2d\u95f4\u5c42\u7535\u89e3\u8d28\u7684\u5c40\u90e8\u5206\u89e3\u6765\u9632\u6b62\u9502\u679d\u6676\u751f\u957f\u3002\u8fd9\u79cd\u673a\u5236\u7c7b\u4f3c\u4e8e\u81a8\u80c0\u87ba\u6746\u6548\u5e94\uff0c\u5176\u4e2d\u4efb\u4f55\u88c2\u7f1d\u90fd\u4f1a\u88ab\u52a8\u6001\u4ea7\u751f\u7684\u5206\u89e3\u7269\u586b\u5145\uff0c\u8fd9\u4e9b\u5206\u89e3\u4e5f\u53d7\u5230\u5f88\u597d\u7684\u7ea6\u675f\uff0c\u53ef\u80fd\u662f\u901a\u8fc7\u5206\u89e3\u5f15\u8d77\u7684\u201c\u951a\u5b9a\u201d\u6548\u5e94\u3002\u9502\u91d1\u5c5e\u8d1f\u6781\u4e0eLiNi0.8<\/sub>Mn0.1<\/sub>Co0.1<\/sub>O2<\/sub>\u6b63\u6781\u914d\u5bf9\u7ec4\u88c5\u7684\u5168\u56fa\u6001\u7535\u6c60\u5faa\u73af\u6027\u80fd\u975e\u5e38\u7a33\u5b9a\uff0c\u4ee520C\u500d\u7387\uff088.6 mA\u00a0cm-2<\/sup>\uff09\u5faa\u73af10000\u6b21\u540e\u5bb9\u91cf\u4fdd\u6301\u7387\u4e3a82%\uff0c\u4ee51.5C\u7684\u500d\u7387\uff080.64\u00a0mA\u00a0cm-2<\/sup>\uff09\u5faa\u73af2000\u5708\u540e\u5bb9\u91cf\u4fdd\u6301\u7387\u4e3a81.3%\u3002\u591a\u5c42\u8bbe\u8ba1\u8fd8\u5b9e\u73b0\u4e86110.6kW\u00a0kg-1<\/sup>\u7684\u6bd4\u529f\u7387\u548c\u9ad8\u8fbe631.1 Wh kg-1<\/sup>\u7684\u6bd4\u80fd\u91cf\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cA dynamic stability design strategy for lithium metal solid state batteries\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature\u4e0a\u3002DOI: 10.1038\/s41586-021-03486-3<\/p>\n

\"\"<\/p>\n

\u56fe 1\u3001\u591a\u5c42\u8bbe\u8ba1\u56fa\u6001\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

Nature(IF<\/b><\/strong>\uff1a<\/b><\/strong>49.962)<\/b><\/strong>\uff1a\u4e00\u79cd\u9ad8\u5ea6\u7a33\u5b9a\u4e14\u67d4\u6027\u7684\u6cb8\u77f3\u7535\u89e3\u8d28\u56fa\u6001\u9502\u7a7a\u6c14\u7535\u6c60\u3002<\/b><\/strong><\/p>\n

\u56fa\u6001\u9502\uff08Li\uff09-\u7a7a\u6c14\u7535\u6c60\u6709\u671b\u89e3\u51b3\u6db2\u4f53\u7535\u6c60\u4f53\u7cfb\u4e2d\u7684\u5b89\u5168\u6027\u548c\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u95ee\u9898\u3002\u7136\u800c\uff0c\u4f20\u7edf\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u4e0d\u9002\u7528\u4e8e\u56fa\u6001\u9502\u7a7a\u6c14\u7535\u6c60\u4f53\u7cfb\uff0c\u56e0\u4e3a\u5b83\u4eec\u5bf9\u9502\u91d1\u5c5e\u548c\u7a7a\u6c14\u4e0d\u7a33\u5b9a\uff0c\u5e76\u4e14\u96be\u4ee5\u6784\u5efa\u4f4e\u7684\u754c\u9762\u7535\u963b\u3002\u5728\u8fd9\u91cc\uff0c\u5409\u6797\u5927\u5b66\u4e8e\u5409\u7ea2\u9662\u58eb\u548c\u5f90\u5409\u9759\u6559\u6388\u8bbe\u8ba1\u4e86\u4e00\u79cd\u96c6\u6210\u7684\u56fa\u6001\u9502\u7a7a\u6c14\u7535\u6c60\uff0c\u8be5\u7535\u6c60\u5305\u542b\u8d85\u8584\u3001\u9ad8\u79bb\u5b50\u5bfc\u7535\u6027\u7684\u9502\u79bb\u5b50\u4ea4\u6362\u6cb8\u77f3X(LiX)\u819c\u4f5c\u4e3a\u56fa\u4f53\u7535\u89e3\u8d28\u3002\u8fd9\u79cd\u7535\u89e3\u8d28\u4f7f\u7528\u539f\u4f4d\u7ec4\u88c5\u7b56\u7565\u4e0e\u9502\u8d1f\u6781\u548c\u78b3\u7eb3\u7c73\u7ba1\u6b63\u6781\u96c6\u6210\u5728\u4e00\u8d77\u3002\u7531\u4e8e\u6cb8\u77f3\u56fa\u6709\u7684\u5316\u5b66\u7a33\u5b9a\u6027\uff0c\u6709\u6548\u6291\u5236\u4e86\u7535\u89e3\u8d28\u56e0\u9502\u6216\u7a7a\u6c14\u7684\u4f5c\u7528\u800c\u53d8\u8d28\u3002\u8be5\u7535\u6c60\u5bb9\u91cf\u4e3a12020 mAh g-1<\/sup>\uff0c\u5728500 mA g-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u548c1000 mAh g-1<\/sup>\u7684\u5bb9\u91cf\u4e0b\u5faa\u73af\u5bff\u547d\u4e3a149\u6b21\u3002\u5728\u76f8\u540c\u6761\u4ef6\u4e0b\uff0c\u8fd9\u79cd\u5faa\u73af\u5bff\u547d\u5927\u4e8e\u57fa\u4e8e\u78f7\u9178\u94dd\u9517\u9502\uff0812\u6b21\u5faa\u73af\uff09\u548c\u6709\u673a\u7535\u89e3\u8d28\uff08102\u6b21\u5faa\u73af\uff09\u7684\u7535\u6c60\u3002\u6cb8\u77f3\u57fa\u9502\u7a7a\u6c14\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd\u3001\u67d4\u6027\u548c\u7a33\u5b9a\u6027\u8d4b\u4e88\u5176\u5b9e\u9645\u9002\u7528\u6027\uff0c\u53ef\u4ee5\u6269\u5c55\u5230\u5176\u4ed6\u50a8\u80fd\u4f53\u7cfb\uff0c\u5982\u9502\u79bb\u5b50\u3001\u94a0\u7a7a\u6c14\u548c\u94a0\u79bb\u5b50\u7535\u6c60\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cA highly stable and flexible zeolite electrolyte solid-state Li\u2013air battery\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature\u4e0a\u3002DOI: 10.1038\/s41586-021-03410-9<\/p>\n

\"\"<\/p>\n

\u56fe 2\u3001\u6cb8\u77f3\u56fa\u4f53\u7535\u89e3\u8d28\u7684\u793a\u610f\u56fe\u548c\u8868\u5f81\u3002<\/p>\n

Na<\/b><\/strong>ture Materials(IF: 43.841):<\/b><\/strong>\u00a0<\/b><\/strong>\u7535\u89e3\u8d28\u7194\u4f53\u6e17\u900f\u7528\u4e8e\u65e0\u673a\u5168\u56fa\u6001\u9502\u79bb\u5b50\u7535\u6c60\u7684\u53ef\u6269\u5c55\u5236\u9020<\/b><\/strong><\/p>\n

\u5177\u6709\u65e0\u673a\u56fa\u6001\u7535\u89e3\u8d28\u7684\u5168\u56fa\u6001\u9502(Li)\u91d1\u5c5e\u548c\u9502\u79bb\u5b50\u7535\u6c60(ASSLB)\u53ef\u4e3a\u7535\u52a8\u6c7d\u8f66\u548c\u5176\u4ed6\u5e94\u7528\u63d0\u4f9b\u66f4\u9ad8\u7684\u5b89\u5168\u6027\u3002\u7136\u800c\uff0c\u76ee\u524d\u7684\u65e0\u673aASSLB\u5236\u9020\u6280\u672f\u5b58\u5728\u6210\u672c\u9ad8\u3001\u56fa\u6001\u7535\u89e3\u8d28\u548c\u5bfc\u7535\u6dfb\u52a0\u5242\u8fc7\u591a\u3001\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u4f4e\u7b49\u95ee\u9898\u3002\u76ee\u524d\u7684\u5236\u9020\u65b9\u6cd5\u6d89\u53ca\u5355\u72ec\u5236\u9020\u70e7\u7ed3\u9676\u74f7\u56fa\u6001\u7535\u89e3\u8d28\u819c\u548cASSLB\u7535\u6781\uff0c\u7136\u540e\u5728\u7cbe\u786e\u63a7\u5236\u7684\u73af\u5883\u4e2d\u5c0f\u5fc3\u5730\u5806\u53e0\u548c\u70e7\u7ed3\u5728\u4e00\u8d77\u3002\u5728\u8fd9\u91cc\uff0c\u4f50\u6cbb\u4e9a\u7406\u5de5\u5b66\u9662Gleb Yushin\u62a5\u544a\u4e86\u4e00\u79cd\u98a0\u8986\u6027\u7684\u5236\u9020\u6280\u672f\uff0c\u8be5\u6280\u672f\u53ef\u964d\u4f4e\u6240\u6709\u56fa\u4f53\u7535\u6c60\u7684\u5236\u9020\u6210\u672c\u5e76\u63d0\u9ad8\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u3002\u8be5\u65b9\u6cd5\u6a21\u4eff\u4e86\u5546\u4e1a\u9502\u79bb\u5b50\u7535\u6c60\u7684\u5236\u9020\u8fc7\u7a0b\uff0c\u4e0d\u540c\u4e4b\u5904\u5728\u4e8e\u4f7f\u7528\u5177\u6709\u4f4e\u7194\u70b9\u7684\u56fa\u6001\u7535\u89e3\u8d28\u4ee3\u66ff\u7535\u89e3\u6db2\uff0c\u8fd9\u4e9b\u7535\u89e3\u8d28\u5728\u9002\u5ea6\u5347\u9ad8\u7684\u6e29\u5ea6\uff08~300 \u00b0C\u6216\u66f4\u4f4e\uff09\u4e0b\u6e17\u900f\u5230\u81f4\u5bc6\u3001\u70ed\u7a33\u5b9a\u7684\u7535\u6781\u4e2d\uff0c\u7136\u540e\u5728\u51b7\u5374\u8fc7\u7a0b\u4e2d\u56fa\u5316\u3002\u73b0\u6709\u7684\u5546\u4e1a\u8bbe\u5907\u53ef\u76f4\u63a5\u7528\u4e8e\u7535\u6781\u548c\u7535\u6c60\u5236\u9020\uff0c\u5927\u5927\u964d\u4f4e\u4e86\u4ea7\u4e1a\u94fe\u5347\u7ea7\u7684\u969c\u788d\u3002\u8fd9\u79cd\u65b9\u6cd5\u6210\u529f\u7528\u4e8e\u5236\u9020\u5177\u6709 LiNi0.33<\/sub>Mn0.33<\/sub>Co0.33<\/sub>O2<\/sub>\u6b63\u6781\u548cLi4<\/sub>Ti5<\/sub>O12<\/sub>\/\u77f3\u58a8\u8d1f\u6781\u7684\u65e0\u673aASSLB\uff0c\u4e3a\u52a0\u901fASSLB\u7684\u5e94\u7528\u4ee5\u5b9e\u73b0\u66f4\u5b89\u5168\u7684\u7535\u52a8\u6c7d\u8f66\u5f00\u8f9f\u4e86\u65b0\u7684\u673a\u4f1a\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cElectrolyte melt infiltration for scalable manufacturing of inorganic all-solid-state lithium-ion batteries\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002DOI: 10.1038\/s41563-021-00943-2<\/p>\n

\"\"<\/p>\n

\u56fe 3\u3001\u56fa\u6001\u7535\u89e3\u8d28\u7194\u76d0\u6e17\u900f\u793a\u610f\u56fe\u3002<\/p>\n

Na<\/b><\/strong>ture Materials(IF: 43.841):<\/b><\/strong>\u00a0\u5177\u6709\u7eb3\u7c73\u6676\u9502\u79bb\u5b50\u901a\u8def\u7684\u56fa\u6001\u805a\u5408\u7269\u590d\u5408\u7535\u89e3\u8d28<\/b><\/strong><\/p>\n

\u4e0b\u4e00\u4ee3\u9502\u57fa\u7535\u6c60\u7684\u4e00\u4e2a\u5173\u952e\u6311\u6218\u5728\u4e8e\u5f00\u53d1\u80fd\u591f\u5b9e\u73b0\u70ed\u5b89\u5168\u7684\u7535\u89e3\u8d28\u4ee5\u53ca\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7535\u6781\u7684\u4f7f\u7528\u3002\u4e3a\u6b64\uff0c\u5f17\u5409\u5c3c\u4e9a\u7406\u5de5Louis A. Madsen\u4ecb\u7ecd\u4e86\u4e00\u79cd\u5177\u6709\u9635\u5217\u7ed3\u6784\u7684\u6db2\u6676\u805a\u5408\u7269\u4e0e\u79bb\u5b50\u6db2\u4f53\u548c\u6d53\u7f29\u9502\u76d0\u76f8\u7ed3\u5408\u7684\u5206\u5b50\u79bb\u5b50\u590d\u5408\u7535\u89e3\u8d28\u3002\u8fd9\u79cd\u9ad8\u5f3a\u5ea6(200 MPa)\u4e14\u4e0d\u53ef\u71c3\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u5177\u6709\u51fa\u8272\u7684Li+<\/sup>\u7535\u5bfc\u7387\uff0825 \u00b0C\u65f6\u4e3a1 mS cm-1<\/sup>\uff09\u548c\u7535\u5316\u5b66\u7a33\u5b9a\u6027\uff085.6 V vs\u00a0Li|Li+<\/sup>\uff09\uff0c\u540c\u65f6\u6291\u5236\u679d\u6676\u751f\u957f\u5e76\u8868\u73b0\u51fa\u4f4e\u7684\u754c\u9762\u7535\u963b\uff0832 \u03a9 cm2<\/sup>\uff09\u548c\u9502\u5bf9\u79f0\u7535\u6c60\u8fc7\u7535\u4f4d\uff08\u2264120 mV at 1 mA cm\u22122<\/sup>\uff09\u3002\u76d0\u63ba\u6742\u8fc7\u7a0b\u6539\u53d8\u4e86\u5c40\u90e8\u6709\u5e8f\u7684\u805a\u5408\u7269-\u79bb\u5b50\u914d\u4f4d\u7ed3\u6784\uff0c\u4ee5\u6784\u5efa\u586b\u5145LiFSI\u548cLiBF4<\/sub>\u7eb3\u7c73\u6676\u4f53\u7684\u6676\u95f4\u7f51\u7edc\uff0c\u4ece\u800c\u5927\u5927\u589e\u5f3a\u4e86Li+<\/sup>\u7535\u5bfc\u7387\u3002\u5c06\u9676\u74f7\u7c7b\u5bfc\u4f53\u7684\u5feb\u901f\u79bb\u5b50\u4f20\u8f93\u4e0e\u805a\u5408\u7269\u7535\u89e3\u8d28\u7684\u67d4\u6027\u76f8\u7ed3\u5408\uff0c\u8fd9\u79cd\u6a21\u5757\u5316\u6750\u6599\u5236\u9020\u5e73\u53f0\u6709\u671b\u7528\u4e8e\u5b89\u5168\u548c\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u50a8\u80fd\u548c\u8f6c\u6362\u5e94\u7528\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cSolid-state rigid-rod polymer composite electrolytes with nanocrystalline lithium ion pathways\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002DOI: 10.1038\/s41563-021-00995-4<\/p>\n

\"\"<\/p>\n

\u56fe 4\u3001a\uff0c\u5206\u5b50\u79bb\u5b50\u590d\u5408\u7535\u89e3\u8d28\u7684\u5236\u9020\u6d41\u7a0b\u3002b\uff0c\u7b2c\u4e8c\u4e2a\u79bb\u5b50\u4ea4\u6362\u8fc7\u7a0b\u3002c\u3001d\uff0cRMIC-5 (c) \u548c RMIC-15 (d) \u7684 SEM \u56fe\u50cf\u3002e-g\uff0c\u7eb3\u7c73\u6676\u5bfc\u7535\u7f51\u7edc\u793a\u610f\u56fe\u3002<\/p>\n

Na<\/b><\/strong>ture Materials(IF: 43.841):<\/b><\/strong>\u00a0\u63ed\u793a\u6b63\u6781<\/b><\/strong>-\u7535\u89e3\u8d28\u754c\u9762\u5bf9\u56fa\u6001\u7535\u6c60\u7684\u4f5c\u7528<\/b><\/strong><\/p>\n

\u754c\u9762\u5728\u4e8c\u6b21\u56fa\u6001\u7535\u6c60\u7684\u6027\u80fd\u4e2d\u5177\u6709\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u5728\u8fd9\u91cc\uff0c\u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u5384\u5df4\u7eb3\u9999\u69df\u5206\u6821Paul V. Braun\u4f7f\u7528\u6676\u4f53\u5b66\u9ad8\u5ea6\u53d6\u5411\u5316\u7684\u539a\u6b63\u6781\uff0c\u76f4\u63a5\u8bc4\u4f30\u6b63\u6781\u6676\u4f53\u5b66\u53d6\u5411\u548c\u5f62\u6001\u5bf9\u56fa\u6001\u7535\u6c60\u957f\u5faa\u73af\u6027\u80fd\u7684\u5f71\u54cd\u3002\u8fd9\u4e9b\u6b63\u6781\u7684\u754c\u9762\u6676\u4f53\u5b66\u3001\u9762\u79ef\u548c\u5fae\u89c2\u7ed3\u6784\u53ef\u63a7\uff0c\u4f7f\u4eba\u4eec\u80fd\u591f\u4e86\u89e3\u4f20\u7edf\u8584\u819c\u548c\u590d\u5408\u56fa\u6001\u7535\u6781\u4e2d\u672a\u77e5\u7684\u754c\u9762\u4e0d\u7a33\u5b9a\u6027\u3002\u5bf9\u4e8e\u5404\u79cd\u9502\u57fa\u548c\u94a0\u57fa\u6b63\u6781\u548c\u56fa\u4f53\u7535\u89e3\u8d28\uff0c\u63ed\u793a\u4e86\u7535\u6c60\u6027\u80fd\u548c\u754c\u9762\u7a33\u5b9a\u6027\u4e4b\u95f4\u7684\u76f4\u63a5\u76f8\u5173\u6027\u3002\u7814\u7a76\u7ed3\u679c\u663e\u793a\uff0c\u6700\u5c0f\u5316\u754c\u9762\u9762\u79ef\uff0c\u800c\u4e0d\u662f\u50cf\u4f20\u7edf\u590d\u5408\u6b63\u6781\u90a3\u6837\u6269\u5927\u754c\u9762\u9762\u79ef\uff0c\u662f\u7406\u89e3\u754c\u9762\u4e0d\u7a33\u5b9a\u6027\u7684\u672c\u8d28\u548c\u63d0\u9ad8\u7535\u6c60\u6027\u80fd\u7684\u5173\u952e\u3002\u7814\u7a76\u7ed3\u679c\u8fd8\u6307\u51fa\u4f7f\u7528\u81f4\u5bc6\u548c\u539a\u7684\u6b63\u6781\u80fd\u591f\u63d0\u9ad8\u56fa\u6001\u7535\u6c60\u80fd\u91cf\u5bc6\u5ea6\u548c\u7a33\u5b9a\u6027\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cRevealing the role of the cathode\u2013electrolyte interface on solid-state batteries\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002DOI: 10.1038\/s41563-021-01016-0<\/p>\n

\"\"<\/p>\n

\u56fe 5\u3001\u81f4\u5bc6\u4e14\u9ad8\u5ea6\u53d6\u5411\u5316\u7684\u6b63\u6781\u8c03\u8282\u754c\u9762\u9762\u79ef\u548c\u754c\u9762\u6676\u4f53\u5b66\u7684\u793a\u610f\u56fe\u3002<\/p>\n

Na<\/b><\/strong>ture Materials(IF: 43.841):<\/b><\/strong>\u00a0\u53ef\u89c6\u5316\u9502\u8d1f\u6781\u56fa\u4f53\u7535\u89e3\u8d28\u7535\u6c60\u4e2d\u7535\u9540\u5f15\u8d77\u7684\u5f00\u88c2<\/b><\/strong><\/p>\n

\u9502\u679d\u6676\u901a\u8fc7\u9676\u74f7\u7535\u89e3\u8d28\u4f20\u64ad\uff0c\u5bfc\u81f4\u5728\u9ad8\u5145\u7535\u901f\u7387\u4e0b\u77ed\u8def\uff0c\u662f\u5b9e\u73b0\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u5168\u56fa\u6001\u9502\u8d1f\u6781\u7535\u6c60\u7684\u6700\u5927\u969c\u788d\u4e4b\u4e00\u3002\u5728\u8fd9\u91cc\uff0c\u725b\u6d25\u5927\u5b66Peter G. Bruce\u5229\u7528\u539f\u4f4dX\u5c04\u7ebf\u8ba1\u7b97\u673a\u65ad\u5c42\u626b\u63cf\u4e0e\u7a7a\u95f4\u6620\u5c04X\u5c04\u7ebf\u884d\u5c04\u76f8\u7ed3\u5408\uff0c\u5728Li\/Li6<\/sub>PS5<\/sub>Cl\/Li\u7535\u6c60\u4e2d\u8ddf\u8e2a\u88c2\u7eb9\u548c\u9502\u679d\u6676\u5728\u56fa\u4f53\u7535\u89e3\u8d28\u4e2d\u7684\u4f20\u64ad\u3002\u5728\u7535\u9540\u8fc7\u7a0b\u4e2d\uff0c\u5f00\u88c2\u4ee5\u6563\u88c2\u5f00\u59cb\uff0c\u5706\u9525\u5f62\u201c\u5751\u6d1e\u201d\u72b6\u88c2\u7eb9\u5728\u9676\u74f7\u7535\u89e3\u8d28\u4e2d\u5f62\u6210\uff0c\u9760\u8fd1\u7535\u9540\u7535\u6781\u7684\u8868\u9762\u3002\u6563\u88c2\u4e3b\u8981\u5f62\u6210\u4e8e\u9502\u7535\u6781\u8fb9\u7f18\u7684\u5c40\u90e8\u7535\u573a\u8f83\u9ad8\u7684\u5730\u65b9\u3002\u7136\u540e\u6a2a\u5411\u88c2\u7eb9\u4ece\u7535\u9540\u7535\u6781\u5411\u5265\u79bb\u7535\u6781\u4f20\u64ad\uff0c\u7a7f\u8fc7\u7535\u89e3\u8d28\u3002\u9502\u7684\u8fdb\u5165\u4f7f\u88c2\u7eb9\u53d8\u5bbd\uff0c\u5e76\u9a71\u52a8\u6563\u88c2\u548c\u6a2a\u5411\u88c2\u7eb9\u7684\u4f20\u64ad\uff1b\u4e5f\u5c31\u662f\u8bf4\uff0c\u88c2\u7eb9\u5728Li\u4f20\u64ad\u4e4b\u524d\u5c31\u5df2\u6269\u5c55\u3002\u7ed3\u679c\uff0c\u5728\u9502\u5230\u8fbe\u53e6\u4e00\u4e2a\u7535\u6781\u4e4b\u524d\uff0c\u88c2\u7f1d\u5c31\u7a7f\u8fc7\u6574\u4e2a\u7535\u89e3\u8d28\uff0c\u56e0\u6b64\u53d1\u751f\u5728\u77ed\u8def\u4e4b\u524d\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cVisualizing plating-induced cracking in lithium-anode solid-electrolyte cells\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002DOI: 10.1038\/s41563-021-00967-8<\/p>\n

\"\"<\/p>\n

\u56fe 6\u3001a\uff0c\u5bf9\u79f0Li\/Li6<\/sub>PS5<\/sub>Cl\/Li\u7535\u6c60\u57287 MPa\u548c1.25 mA cm-2<\/sup>\u4e0b\u5faa\u73af\u7684\u7535\u538b\u66f2\u7ebf\uff1bb\uff0c\u6cbf\u7740\u5e73\u884c\u4e8e\u9502\u7535\u6781\u4e0b\u65b95\u4e2a\u50cf\u7d20\u7684\u5e73\u9762\u62cd\u6444\u7684\u865a\u62df\u56fe\u50cf\u5207\u7247\u3002c,\u6a2a\u622a\u9762\u56fe\u50cf\u5207\u7247\u7684\u653e\u5927\u56fe\u50cf\u3002d\uff0c\u5faa\u73afLi\/Li3<\/sub>N\/Li\u5bf9\u79f0\u7535\u6c60XCT\u626b\u63cf\u6a2a\u622a\u9762\u56fe\u50cf\u5207\u7247\u3002<\/p>\n

Na<\/b><\/strong>ture Materials(IF: 43.841):<\/b><\/strong>\u00a0\u4f7f\u7528\u539f\u4f4d<\/b><\/strong>X\u5c04\u7ebf\u65ad\u5c42\u626b\u63cf\u5c06\u7a7a\u9699\u548c\u76f8\u95f4\u6f14\u5316\u4e0e\u56fa\u6001\u7535\u6c60\u4e2d\u7684\u7535\u5316\u5b66\u8054\u7cfb\u8d77\u6765<\/b><\/strong><\/p>\n

\u5c3d\u7ba1\u56fa\u6001\u7535\u6c60\u5de5\u7a0b\u53d6\u5f97\u4e86\u8fdb\u5c55\uff0c\u4f46\u4e0e\u56fa\u6db2\u754c\u9762\u76f8\u6bd4\uff0c\u5bf9\u63a7\u5236\u56fa\u56fa\u754c\u9762\u7535\u5316\u5b66\u884c\u4e3a\u548c\u7a33\u5b9a\u6027\u7684\u5316\u5b66\u673a\u68b0\u73b0\u8c61\u7684\u7406\u89e3\u4ecd\u7136\u6709\u9650\u3002\u5728\u8fd9\u91cc\uff0c\u4f50\u6cbb\u4e9a\u7406\u5de5\u5b66\u9662Matthew T. McDowell\u4f7f\u7528\u539f\u4f4d\u540c\u6b65\u52a0\u901f\u5668X\u5c04\u7ebf\u8ba1\u7b97\u673a\u663e\u5fae\u65ad\u5c42\u626b\u63cf\u6765\u7814\u7a76\u7535\u6c60\u5faa\u73af\u8fc7\u7a0b\u4e2d\u9502\/\u56fa\u6001\u7535\u89e3\u8d28\u754c\u9762\u7684\u6f14\u53d8\uff0c\u63ed\u793a\u7a7a\u9699\u5f62\u6210\u3001\u76f8\u95f4\u751f\u957f\u548c\u4f53\u79ef\u53d8\u5316\u4e4b\u95f4\u590d\u6742\u7684\u76f8\u4e92\u4f5c\u7528\u5982\u4f55\u5f71\u54cd\u7535\u6c60\u884c\u4e3a\u3002\u5728\u5bf9\u79f0\u7535\u6c60\u4e2d\u53ef\u4ee5\u76f4\u63a5\u770b\u5230\u9502\u5265\u79bb\u8fc7\u7a0b\u4e2d\u7684\u7a7a\u9699\u5f62\u6210\uff0c\u5e76\u4e14\u91cf\u5316\u4e86\u9502\u548c\u56fa\u6001\u7535\u89e3\u8d28(Li10<\/sub>SnP2<\/sub>S12<\/sub>)\u4e4b\u95f4\u754c\u9762\u5904\u5bfc\u81f4\u7535\u6d41\u6536\u7f29\u7684\u63a5\u89e6\u635f\u5931\uff0c\u5e76\u53d1\u73b0\u8fd9\u662f\u7535\u6c60\u6545\u969c\u7684\u4e3b\u8981\u539f\u56e0\u3002\u53d1\u73b0\u754c\u9762\u5728\u5145\u7535\u65f6\u5177\u6709\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\uff0c\u5e76\u4e14\u7531\u4e8e\u4efb\u4e00\u7535\u6781\u7684\u504f\u6469\u5c14\u4f53\u79ef\u4e0d\u5339\u914d\u800c\u53d1\u751f\u6574\u4f53\u4f53\u79ef\u53d8\u5316\u3002\u8fd9\u4e9b\u7ed3\u679c\u63d0\u4f9b\u4e86\u5bf9\u5316\u5b66\u673a\u68b0\u73b0\u8c61\u5982\u4f55\u5f71\u54cd\u7535\u6c60\u6027\u80fd\u7684\u6df1\u5165\u4e86\u89e3\uff0c\u4ece\u800c\u4fc3\u8fdb\u4e86\u56fa\u6001\u7535\u6c60\u7684\u53d1\u5c55\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cLinking void and interphase evolution to electrochemistry in solid-state batteries using operando X-ray tomography\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Materials\u4e0a\u3002DOI: 10.1038\/s41563-020-00903-2<\/p>\n

\"\"<\/p>\n

\u56fe 7\u3001a\uff0cLi\/LSPS\/Li\u7535\u6c60\u7684\u539f\u4f4dX\u5c04\u7ebf\u65ad\u5c42\u626b\u63cf\u7535\u6c60\u793a\u610f\u56fe\u3002\u57284 mA cm-2<\/sup>(b)\u548c1 mA cm-2<\/sup>\u00a0(c)\u4e0b\u6d4b\u91cf\u7684\u7535\u538b\u66f2\u7ebf\u3002\u57284 mA cm-2(d)\u548c1 mA cm-2(e)\u5faa\u73af\u4e4b\u524d\u91cd\u6784\u7684\u6a2a\u622a\u9762\u56fe\u50cf\u3002f\uff0c\u57281 mA cm\u22122<\/sup>\u5faa\u73af\u4e4b\u524dLi\/LSPS\u754c\u9762\u7684\u653e\u5927\u6a2a\u622a\u9762\u3002g\uff0ch\uff0c\u5faa\u73af\u540e\u7684\u6a2a\u622a\u9762\u56fe\u50cf\u3002i\uff0c\u57281 mA cm\u22122<\/sup>\u5904\u7ecf\u8fc7\u4e00\u4e2a\u5b8c\u6574\u5faa\u73af\u540e\uff0c\u754c\u9762\u7684\u6a2a\u622a\u9762\u3002<\/p>\n

Nature<\/b><\/strong>\u00a0<\/b><\/strong>Communications<\/b><\/strong>(IF<\/b><\/strong>\uff1a<\/b><\/strong>14.919): <\/b><\/strong>\u4e00\u79cd\u7528\u4e8e\u9502\u7535\u6c60\u7684\u7ecf\u6d4e\u9ad8\u6548\u4e14\u8010\u6e7f\u7684\u6c2f\u5316\u7269\u56fa\u4f53\u7535\u89e3\u8d28<\/b><\/strong><\/p>\n

\u6c2f\u5316\u7269\u56fa\u4f53\u7535\u89e3\u8d28\u56e0\u5176\u9ad8\u79bb\u5b50\u7535\u5bfc\u7387\u3001\u53ef\u53d8\u5f62\u6027\u548c\u6c27\u5316\u7a33\u5b9a\u6027\u7b49\u7269\u7406\u5316\u5b66\u7279\u6027\u800c\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\u3002\u7136\u800c\uff0c\u539f\u6750\u6599\u6602\u8d35\uff0c\u5927\u89c4\u6a21\u4f7f\u7528\u8fd9\u7c7b\u65e0\u673a\u8d85\u79bb\u5b50\u5bfc\u4f53\u4f3c\u4e4e\u4e0d\u592a\u53ef\u80fd\u3002\u5728\u8fd9\u91cc\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u9a6c\u9a8b\u6559\u6388\u62a5\u9053\u4e86\u4e00\u79cd\u5177\u6709\u6210\u672c\u6548\u76ca\u7684\u6c2f\u5316\u7269\u56fa\u4f53\u7535\u89e3\u8d28Li2<\/sub>ZrCl6<\/sub>\u3002\u5b83\u7684\u539f\u6750\u6599\u6bd4\u6700\u5148\u8fdb\u7684\u6c2f\u5316\u7269\u56fa\u4f53\u7535\u89e3\u8d28\u4fbf\u5b9c\u51e0\u4e2a\u6570\u91cf\u7ea7\uff0c\u4f46\u79bb\u5b50\u7535\u5bfc\u7387\u9ad8\uff08\u5ba4\u6e29\u4e0b\u4e3a0.81 mS cm-1<\/sup>\uff09\u3001\u53ef\u53d8\u5f62\u6027\u548c4V\u7684\u6c27\u5316\u7535\u538b\u3002\u6b64\u5916\uff0cLi2<\/sub>ZrCl6<\/sub>\u5bf9\u6c34\u5206\u4e0d\u654f\u611f\uff0c\u5728\u66b4\u9732\u4e8e5%\u76f8\u5bf9\u6e7f\u5ea6\u7684\u5927\u6c14\u4e2d\u540e\uff0c\u6ca1\u6709\u5438\u6e7f\u6216\u7535\u5bfc\u7387\u4e0b\u964d\u7684\u8ff9\u8c61\u3002\u901a\u8fc7\u5c06Li2<\/sub>ZrCl6<\/sub>\u4e0eLi-In\u8d1f\u6781\u548c\u5355\u6676LiNi0.8<\/sub>Mn0.1<\/sub>Co0.1<\/sub>O2<\/sub>\u6b63\u6781\u76f8\u7ed3\u5408\uff0c\u83b7\u5f97\u4e86\u4e00\u79cd\u5ba4\u6e29\u5168\u56fa\u6001\u7535\u6c60\uff0c\u5176\u6bd4\u5bb9\u91cf\u7ea6\u4e3a150 mAh g-1<\/sup>\uff0c\u53ef\u5728200 mA g\u20131<\/sup>\u7a33\u5b9a\u5faa\u73af200\u6b21\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cA cost-effective and humidity-tolerant chloride solid electrolyte for lithium batteries\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Communications\u4e0a\u3002DOI: 10.1038\/s41467-021-24697-2<\/p>\n

\"\"<\/p>\n

\u56fe 8\u3001Li2<\/sub>ZrCl6<\/sub>\u548c\u6700\u5148\u8fdb\u7684\u6c2f\u5316\u7269\u56fa\u4f53\u7535\u89e3\u8d28\u7684\u539f\u6750\u6599\u6210\u672c\u3002<\/p>\n

Nature<\/b><\/strong>\u00a0<\/b><\/strong>Communications<\/b><\/strong>(IF<\/b><\/strong>\uff1a<\/b><\/strong>14.919): <\/b><\/strong>\u4e00\u79cd\u7528\u4e8e\u65e0\u679d\u6676\u56fa\u4f53\u9502\u91d1\u5c5e\u7535\u6c60\u7684\u67d4\u6027\u7535\u5b50\u963b\u6321\u754c\u9762\u5c4f\u853d\u5c42<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

\u56fe 9\u3001LLZTO\u8868\u9762PAA\u5c42\u7684\u7269\u7406\u7279\u6027\u3002<\/p>\n

\u672c\u6587\u7531micro\u7136\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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