{"id":227144,"date":"2021-09-13T06:12:00","date_gmt":"2021-09-12T22:12:00","guid":{"rendered":"\/\/m.iemloyee.com\/?p=227144"},"modified":"2021-09-12T20:12:13","modified_gmt":"2021-09-12T12:12:13","slug":"%e8%83%bd%e6%ba%90%e5%82%ac%e5%8c%96%e6%96%b0%e6%9d%90%e6%96%99%e9%a2%91%e5%87%ba%ef%bc%8c%e5%8d%95%e5%8e%9f%e5%ad%90%e6%9c%aa%e6%9d%a5%e4%b9%8b%e8%b7%af%e4%bd%95%e5%8e%bb%e4%bd%95%e4%bb%8e%ef%bc%9f","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=227144","title":{"rendered":"\u80fd\u6e90\u50ac\u5316\u65b0\u6750\u6599\u9891\u51fa\uff0c\u5355\u539f\u5b50\u672a\u6765\u4e4b\u8def\u4f55\u53bb\u4f55\u4ece\uff1f"},"content":{"rendered":"

\u4e2d\u56fd\u79d1\u5b66\u62a5\u62a5\u9053\uff0c\u57282020\u5e74\uff0c\u4e2d\u56fd\u79d1\u5b66\u9662\u5927\u8fde\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u63d0\u4f9b\u5173\u952e\u6280\u672f\u7684\u201c5\u4e07\u5428\/\u5e74\u4e59\u70ef\u6c22\u7532\u9170\u5316\u751f\u4ea7\u6b63\u4e19\u9187\u5de5\u4e1a\u5316\u88c5\u7f6e\u201d\u5728\u5b81\u6ce2\u5b9e\u73b0\u5168\u6d41\u7a0b\u4e00\u6b21\u6295\u4ea7\u6210\u529f\u3002\u88ab\u8ba4\u4e3a\u662f\u5355\u539f\u5b50\u50ac\u5316\u9886\u57df\u7814\u7a76\u7684\u91cd\u8981\u91cc\u7a0b\u7891\uff0c\u7834\u89e3\u4e86\u56f0\u6270\u50ac\u5316\u754c80\u591a\u5e74\u7684\u96be\u9898\uff0c\u800c\u5728\u540c\u5e74\u768410\u670813\u65e5\uff0c\u5728\u5317\u4eac\u53ec\u5f00\u7684\u201d\u5355\u539f\u5b50\u50ac\u5316\u201c\u9999\u5c71\u79d1\u5b66\u4f1a\u8bae\u4e0a\uff0c\u4e0e\u4f1a\u4e13\u5bb6\u8ba4\u4e3a\uff0c\u4f5c\u4e3a\u4e00\u4e2a\u7531\u4e2d\u56fd\u79d1\u5b66\u5bb6\u9996\u6b21\u63d0\u51fa\u7684\u65b0\u6982\u5ff5\uff0c\u201c\u5355\u539f\u5b50\u50ac\u5316\u201d\u5df2\u7ecf\u6210\u4e3a\u50ac\u5316\u548c\u6750\u6599\u79d1\u5b66\u9886\u57df\u65b0\u7684\u7814\u7a76\u524d\u6cbf\u548c\u70ed\u70b9\uff0c\u5e94\u5c3d\u65e9\u5e03\u5c40\uff0c\u4ee5\u5e94\u5bf9\u8be5\u9886\u57df\u57fa\u7840\u79d1\u5b66\u3001\u5de5\u4e1a\u5e94\u7528\u4e0a\u9762\u4e34\u7684\u6311\u6218\u3002\u90a3\u4e48\uff0c\u5355\u539f\u5b50\u5728\u5927\u725b\u624b\u4e2d\u53c8\u662f\u5982\u4f55\u7ee7\u7eed\u53d1\u5149\u53d1\u70ed\u7684\uff1f<\/p>\n

\"\"<\/b><\/strong><\/p>\n

1. Nature\u00a0<\/b><\/strong><\/b>Catalysis<\/b><\/strong>\uff1a\u4e00\u79cd\u975e\u5747\u76f8\u94f1\u5355\u539f\u5b50\u4f4d\u70b9\u50ac\u5316\u5242\u7528\u4e8e\u9ad8\u533a\u57df\u9009\u62e9\u6027\u7684\u7c7b\u5361\u5bbe<\/b><\/strong>O<\/b><\/strong>–<\/b><\/strong>H<\/b><\/strong>\u952e\u63d2\u5165<\/b><\/strong><\/p>\n

\u5728\u8fc7\u6e21\u91d1\u5c5e\u50ac\u5316\u5242\u7684\u5408\u6210\u4e2d\uff0c\u7c7b\u5361\u5bbe\u7f9f\u57fa\u63d2\u5165\u6cd5\u662f\u4e00\u79cd\u6709\u6548\u4e14\u901a\u7528\u7684\u78b3\u6c27\u952e\u5f62\u6210\u9014\u5f84\uff0c\u800c\u78b3\u6c27\u952e\u7684\u5f62\u6210\u53ef\u4ee5\u589e\u5f3a\u9187\u7c7b\u4f4d\u70b9\u7684\u9009\u62e9\u6027\u529f\u80fd\u5316\uff0c\u867d\u7136\u8fd9\u79cd\u5408\u6210\u65b9\u6cd5\u5177\u6709\u5f88\u5927\u7684\u6f5c\u529b\uff0c\u4f46\u4e5f\u540c\u65f6\u5b58\u5728\u8f83\u5927\u7684\u6311\u6218\u6027\u3002\u4ee5\u8fd9\u79cd\u5408\u6210\u65b9\u6cd5\u4e3a\u57fa\u70b9\uff0c\u534e\u4e1c\u7406\u5de5\u8d75\u6770\u7279\u8058\u526f\u7814\u7a76\u5458\uff0c\u6e05\u534e\u5927\u5b66\u738b\u5b9a\u80dc\u6559\u6388\u548c\u7f8e\u56fd\u52b3\u4f26\u65af\u4f2f\u514b\u5229\u56fd\u5bb6\u5b9e\u9a8c\u5ba4F. Dean\u00a0Toste\u5171\u540c\u63d0\u51fa\u4e86\u4e00\u79cd\u9009\u62e9\u6027\u7c7b\u5361\u5bbeO-H\u63d2\u5165\u7b56\u7565\uff0c\u7814\u7a76\u4eba\u5458\u5c06\u5747\u5300\u5206\u6563\u5728\u7532\u9187\u6eb6\u6db2\u4e2d\u7684\u54aa\u5511\u9aa8\u67b6-8\u6cb8\u77f3\u5f15\u5165\u5230\u542b\u6709\u6c2f\u5316\u94f1\u548c\u5355\u4f53PZS\u7684\u6eb6\u6db2\u4e2d\uff0c\u5728\u4e09\u7532\u80fa\u7684\u5f15\u53d1\u4e0b\uff0c\u4e24\u79cd\u524d\u9a71\u4f53\u5728ZIF-8\u8868\u9762\u8fdb\u884c\u805a\u5408\uff0c\u5f97\u5230\u4e09\u5143\u590d\u5408\u6750\u6599\uff0c\u5e76\u5177\u6709\u591a\u9762\u4f53\u5f62\u8c8c\u3002\u4e4b\u540e\u901a\u8fc7\u70ed\u89e3\u624b\u6bb5\u83b7\u5f97\u4e86\u8d1f\u8f7d\u5728\u6742\u539f\u5b50\u63ba\u6742\u7684\u78b3\u4e0a\u7684Ir\u5355\u539f\u5b50\u50ac\u5316\u5242\u3002\u8be5\u50ac\u5316\u5242\u5bf9\u4e8e\u915a\u7c7bO-H\u952e\u4e0a\u7684\u8102\u80aa\u65cf\u5b98\u80fd\u5316\u7684\u9009\u62e9\u6027\u9ad8\u8fbe99:1\u3002\u672c\u5de5\u4f5c\u5c06\u6709\u673a\u5408\u6210\u7b56\u7565\u4e0e\u7eb3\u7c73\u6750\u6599\u50ac\u5316\u5242\u6709\u6548\u7684\u7ed3\u5408\uff0c\u5de7\u5999\u7684\u5f15\u5165\u4e86\u5de5\u7a0b\u5316\u7684\u975e\u5747\u76f8\u94f1\u5355\u539f\u5b50\u50ac\u5316\u5242\uff0c\u4e3a\u6709\u673a\u8f6c\u5316\u65b9\u5411\u63d0\u4f9b\u4e86\u673a\u4f1a\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cA<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>heterogeneous<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>iridium<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>single<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>atom<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>site<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalyst<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>for<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>highly<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>regioselective<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>carbenoid<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>O<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>H<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>bond<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>insertion<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Catalysis<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 1\u00a0\u94f1\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5408\u6210\u53ca\u5f62\u8c8c\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41929-021-00637-7<\/p>\n

2. Nature\u00a0<\/b><\/strong><\/b>Chemistry<\/b><\/strong>\uff1a<\/b><\/strong>\u57fa\u4e8e\u78b3\u57fa\u5e95\u7684\u9ad8\u8f7d\u91cf\u8fc7\u6e21\u91d1\u5c5e\u5355\u539f\u5b50\u6750\u6599\u7684\u666e\u9002\u6027\u5408\u6210\u7b56\u7565<\/b><\/strong><\/p>\n

\u8fc7\u6e21\u91d1\u5c5e\u5355\u539f\u5b50\u6750\u6599\u5177\u6709\u8f83\u9ad8\u7684\u539f\u5b50\u5229\u7528\u7387\u548c\u50ac\u5316\u6d3b\u6027\u4e2d\u5fc3\u4f4d\u70b9\uff0c\u5176\u72ec\u7279\u7684\u7535\u5b50\u7ed3\u6784\u548c\u53ef\u8c03\u914d\u7684\u914d\u4f4d\u7ed3\u6784\uff0c\u5728\u5404\u79cd\u7535\u50ac\u5316\u53cd\u5e94\u4e2d\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u6d3b\u6027\u3002\u73b0\u6709\u7684\u5408\u6210\u65b9\u6cd5\u4e3b\u8981\u5305\u62ec\u201c\u81ea\u4e0a\u800c\u4e0b\u201d\u6cd5\u548c\u201c\u81ea\u4e0b\u800c\u4e0a\u201d\u6cd5\uff0c\u5355\u539f\u5b50\u6750\u6599\u4e2d\u7684\u91d1\u5c5e\u539f\u5b50\u5bc6\u5ea6\u8f83\u4f4e\uff0c\u9650\u5236\u4e86\u5176\u5de5\u4e1a\u5e94\u7528\u524d\u666f\u3002\u672c\u5de5\u4f5c\u4e2d\uff0c\u7535\u5b50\u79d1\u6280\u5927\u5b66\u3001\u52a0\u62ff\u5927\u5149\u6e90\u548c\u7f8e\u56fd\u83b1\u65af\u5927\u5b66\u4e09\u4e2a\u5355\u4f4d\u5171\u540c\u5408\u4f5c\uff0c\u7535\u5b50\u79d1\u6280\u5927\u5b66\u7684\u590f\u5ddd\u6559\u6388\u4e3a\u7b2c\u4e00\u4f5c\u8005\u548c\u901a\u8baf\u4f5c\u8005\u3002\u8be5\u56e2\u961f\u521b\u65b0\u6027\u5730\u4f7f\u7528\u6bd4\u8868\u9762\u5927\u3001\u70ed\u7a33\u5b9a\u6027\u9ad8\u7684\u77f3\u58a8\u70ef\u91cf\u5b50\u70b9\u4f5c\u4e3a\u78b3\u57fa\u5e95\uff0c\u5bf9\u5176\u8fdb\u884c-NH2<\/sub>\u57fa\u56e2\u4fee\u9970\uff0c\u4f7f\u5176\u5bf9\u91d1\u5c5e\u79bb\u5b50\u5177\u6709\u9ad8\u914d\u4f4d\u6d3b\u6027\u3002\u5f15\u5165\u91d1\u5c5e\u79bb\u5b50\u540e\u53ef\u5f97\u5230\u4ee5\u91d1\u5c5e\u79bb\u5b50\u4f5c\u4e3a\u8282\u70b9\u3001\u529f\u80fd\u5316\u77f3\u58a8\u70ef\u91cf\u5b50\u70b9\u4f5c\u4e3a\u7ed3\u6784\u5355\u5143\u7684\u4ea4\u8054\u7f51\u7edc\uff0c\u6700\u540e\u70ed\u89e3\u5373\u53ef\u5f97\u5230\u9ad8\u8f7d\u91cf\u7684\u91d1\u5c5e\u5355\u539f\u5b50\u6750\u6599\u3002\u76f8\u8f83\u4e8e\u4f20\u7edf\u201c\u81ea\u4e0a\u800c\u4e0b\u201d\u548c\u201c\u81ea\u4e0b\u800c\u4e0a\u201d\u7684\u5355\u539f\u5b50\u50ac\u5316\u5242\u5408\u6210\u65b9\u6cd5\uff0c\u8be5\u7814\u7a76\u62a5\u9053\u7684\u65b9\u6cd5\u65e2\u4fdd\u8bc1\u4e86\u9ad8\u542b\u91cf\u91d1\u5c5e\u79bb\u5b50\u521d\u59cb\u951a\u5b9a\u65f6\u7684\u9ad8\u5206\u6563\u6027\u53c8\u80fd\u6709\u6548\u6291\u5236\u540e\u7eed\u70ed\u89e3\u8fc7\u7a0b\u57fa\u5e95\u70e7\u7ed3\u91cd\u6784\u5f15\u8d77\u7684\u91d1\u5c5e\u539f\u5b50\u56e2\u805a\u3002\u6b64\u65b9\u6cd5\u53ef\u4ee5\u666e\u9002\u6027\u7684\u7528\u4e8e\u591a\u79cd\u8fc7\u6e21\u91d1\u5c5e\u5355\u539f\u5b50\u6750\u6599\u5408\u6210\uff0c\u5b9e\u73b0\u4e86\u9ad8\u8fbe 40\u00a0wt.% \u6216 3.8\u00a0at.% \u7684\u9ad8\u8fc7\u6e21\u91d1\u5c5e\u539f\u5b50\u8d1f\u8f7d\uff0c\u6bd4\u76ee\u524d\u62a5\u9053\u7684\u5355\u539f\u5b50\u8d1f\u8f7d\u91cf\u63d0\u5347\u4e86\u51e0\u500d\u751a\u81f3\u6570\u5341\u500d\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cG<\/i><\/b><\/em><\/strong>eneral<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>synthesis<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>of<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>single<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>atom<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalysts<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>with<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>high<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>metal<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>loading<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>using<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>graphene<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>quantum<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>dots<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Chemistry<\/i><\/b><\/em><\/strong>\u3002<\/p>\n

\"\"<\/p>\n

\u56fe 2\u00a0\u77f3\u58a8\u70ef\u91cf\u5b50\u70b9\u57fa\u5e95\u7684\u5355\u539f\u5b50\u50ac\u5316\u5242\u5408\u6210\u7b56\u7565<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41557-021-00734-x<\/p>\n

<\/b>3. Nature\u00a0<\/b><\/strong><\/b>Communications<\/b><\/strong>\uff1a<\/b><\/strong>\u901a\u8fc7\u91d1\u5c5e-\u8f7d\u4f53\u7535\u5b50\u76f8\u4e92\u4f5c\u7528\u8c03\u63a7\u5355\u539f\u5b50\u50ac\u5316\u5242\u6790\u6c22\u53cd\u5e94<\/b><\/strong><\/p>\n

\u5355\u539f\u5b50\u50ac\u5316\u5242\u7ecf\u8fc7\u591a\u5e74\u7684\u53d1\u5c55\u521b\u65b0\uff0c\u5176\u5de5\u4f5c\u91cd\u70b9\u9010\u6e10\u4ece\u6700\u521d\u7684\u5236\u5907\u8f6c\u79fb\u81f3\u673a\u7406\u6027\u63a2\u7a76\uff0c\u800c\u76ee\u524d\u5bf9\u4e8e\u5355\u539f\u5b50\u50ac\u5316\u53cd\u5e94\u7684\u6b65\u9aa4\u8fc7\u7a0b\u548c\u53cd\u5e94\u673a\u7406\u4ecd\u5728\u521d\u6b65\u63a2\u7d22\u9636\u6bb5\u3002\u6784\u5efa\u53ef\u9760\u7684\u50ac\u5316\u53cd\u5e94\u6784\u6548\u5173\u7cfb\uff0c\u5bf9\u8bbe\u8ba1\u9ad8\u6027\u80fd\u5355\u539f\u5b50\u50ac\u5316\u5242\u81f3\u5173\u91cd\u8981\u3002\u800c\u7814\u7a76\u8868\u660e\uff0c\u5355\u539f\u5b50\u4e0d\u53ef\u4ee5\u8131\u79bb\u8f7d\u4f53\u800c\u72ec\u81ea\u5b58\u5728\uff0c\u5176\u8f7d\u4f53\u5bf9\u5176\u50ac\u5316\u6027\u80fd\u7684\u5f71\u54cd\u4e5f\u81f3\u5173\u91cd\u8981\uff0c\u91d1\u5c5e-\u8f7d\u4f53\u7535\u5b50\u76f8\u4e92\u4f5c\u7528\uff08EMSI\uff09\u662f\u4e00\u79cd\u53ef\u4ee5\u8c03\u63a7\u91d1\u5c5e\u548c\u8f7d\u4f53\u4e4b\u95f4\u7684\u7535\u5b50\u8f6c\u79fb\u8c03\u8282\u8d1f\u8f7d\u91d1\u5c5e\u7535\u5b50\u6001\u7684\u76f4\u63a5\u65b9\u6cd5\u3002\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66\uff08NUS\uff09\u9648\u4f1f\u6559\u6388\u3001\u65bd\u6bc5\u535a\u58eb\u548c\u5357\u4eac\u5927\u5b66\u590f\u5174\u534e\u6559\u6388\u7b49\u4eba\u63d0\u51fa\u901a\u8fc7EMSI\u5bf9\u5355\u539f\u5b50Pt\u50ac\u5316\u5242\u7684\u7535\u5b50\u7ed3\u6784\u8fdb\u884c\u8c03\u63a7\uff0c\u6784\u5efa\u9178\u6027\u548c\u78b1\u6027\u6c22\u6c14\u6790\u51fa\u53cd\u5e94\u6784\u6548\u5173\u7cfb\u3002\u5229\u7528\u6b64\u524d\u62a5\u9053\u8fc7\u7684\u7279\u5f02\u6027\u4f4d\u70b9\u6b20\u7535\u4f4d\u6c89\u79ef\u6cd5\uff08Nat.Commun.,2020,11,4558\uff09,\u5236\u5907\u51fa\u4e8c\u7ef4\u6750\u6599\u8fc7\u6e21\u91d1\u5c5e\u786b\/\u7852\u5316\u7269\uff08MoS2<\/sub>\u3001WS2<\/sub>\u3001MoSe2<\/sub>\u548cWSe2<\/sub>\uff09\u8d1f\u8f7d\u7684\u5355\u539f\u5b50Pt\u50ac\u5316\u5242\u3002\u8f7d\u4f53\u4e0a\u7684\u4e2d\u5fc3\u951a\u5b9a\u786b\u65cf\u539f\u5b50\uff08S\u548cSe\uff09\u548c\u5468\u56f4\u8fc7\u6e21\u91d1\u5c5e\u539f\u5b50\uff08W\u548cMo\uff09\u901a\u8fc7EMSI\u5171\u540c\u8c03\u63a7\u5355\u539f\u5b50Pt\u7535\u5b50\u7ed3\u6784\uff0c\u8fdb\u800c\u5f71\u54cd\u5176HER\u7535\u50ac\u5316\u8fc7\u7a0b\u4e2d\u95f4\u7269\u79cd\u7684\u5438\u9644\u80fd\u548c\u50ac\u5316\u6d3b\u6027\u3002\u4f5c\u8005\u5229\u7528HAADF-STEM\u8868\u5f81\u6e05\u6670\u7684\u89c2\u6d4b \u5230\u4e86Pt\u539f\u5b50\u5728\u4e8c\u7ef4\u57fa\u5e95\u4e0a\u7684\u539f\u5b50\u7ea7\u5206\u6563\u3002\u540c\u65f6\u5229\u7528DFT\u7406\u8bba\u6a21\u62df\uff0c\u63a2\u7a76\u4e86\u50ac\u5316\u53cd\u5e94\u4e2d\u95f4\u7269\u79cd\u7684\u5438\u9644\u80fd\uff0c\u6784\u5efa\u4e86\u9178\u6027\u548c\u78b1\u6027HER\u7684\u6784\u6548\u5173\u7cfb\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cElectronic<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>metal<\/i><\/b><\/em><\/strong>\u2013<\/i><\/b><\/em><\/strong>support<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>interaction<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>modulates<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>single<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>atom<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>platinum<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalysis<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>for<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>hydrogen<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>evolution<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>reaction<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Communications<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 3\u00a0Pt\/MoS2<\/sub>\u3001Pt\/WS2<\/sub>\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5408\u6210\u53ca\u5f62\u8c8c\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41467-021-23306-6<\/p>\n

4. Nature<\/b><\/strong><\/b>Materials<\/b><\/strong>\uff1a<\/b><\/strong>\u975e\u5f3a\u914d\u4f4d\u9ad8\u6d3b\u6027\u5355\u539f\u5b50<\/b><\/strong>OER<\/b><\/strong>\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\u5927\u91cf\u7684\u7814\u7a76\u8868\u660e\uff0c\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u6027\u80fd\u5f88\u5927\u7a0b\u5ea6\u7684\u4f9d\u8d56\u5176\u8f7d\u4f53\uff0c\u8d1f\u8f7d\u5728\u6c27\u5316\u7269\u6216\u78b3\u8d28\u6750\u6599\u4e0a\u7684\u91d1\u5c5e\u50ac\u5316\u4f4d\u70b9\u901a\u5e38\u4e0e\u6c27\u6216\u5176\u4ed6\u6742\u539f\u5b50\u53d1\u751f\u5f3a\u914d\u4f4d\uff0c\u4ece\u800c\u6539\u53d8\u5176\u7535\u5b50\u7ed3\u6784\u800c\u5f71\u54cd\u50ac\u5316\u5242\u6d3b\u6027\u3002\u9a6c\u514b\u65af\u666e\u6717\u514b\u534f\u4f1a\u56fa\u4f53\u7814\u7a76\u6240\u7684\u738b\u6bc5\u7814\u7a76\u5458\u3001\u56db\u5ddd\u5927\u5b66\u7684\u7a0b\u51b2\u7814\u7a76\u5458\u3001\u67cf\u6797\u5de5\u4e1a\u5927\u5b66\u7684Arne\u00a0Thomas\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u5c06WCx<\/sub>\u4f5c\u4e3a\u8f7d\u4f53\uff0c\u7528\u4e8e\u7a33\u5b9a\u91d1\u5c5e\u50ac\u5316\u4e2d\u5fc3\uff0c\u4ece\u800c\u6709\u6548\u5730\u4fc3\u8fdb\u4e86\u6790\u6c27\u53cd\u5e94(OER)\u3002\u901a\u8fc7\u6c89\u6dc0\u53cd\u5e94\u5408\u6210\u4e86\u542b\u6709\u5fae\u91cfFe\u3001Ni\u6216FeNi\u7684\u591a\u5df4\u80fa\u94a8\u9178\u76d0\u590d\u5408\u7269\uff0c\u5c06\u524d\u9a71\u4f53\u70ed\u5904\u7406\u540e\u5f97\u5230\u4e86WCx<\/sub>-Fe\u3001WCx<\/sub>-Ni\u548cWCx<\/sub>-FeNi\u50ac\u5316\u5242\u3002\u6240\u5f97\u5230\u7684\u6750\u6599\u5177\u6709\u4e00\u5c42\u8584\u8584\u7684\u3001\u8d1f\u8f7d\u5728WCx<\/sub>\u4e0a\u7684\u539f\u5b50\u7ea7Fe\/Ni\u91d1\u5c5e\u4e2d\u5fc3\uff0c\u8868\u73b0\u51fa\u4f18\u8d8a\u7684\u50ac\u5316\u6d3b\u6027\u548c\u8010\u4e45\u6027\u3002\u5176\u4e2dWCx<\/sub>-FeNi\u50ac\u5316\u5242\u572810\u00a0mA\u00a0cm\u2212<\/sup>2<\/sup>\u4e0b\u5177\u6709\u8f83\u4f4e\u7684\u8fc7\u7535\u4f4d\uff0c\u4e3a237\u00a0mV\u3002\u5728\u8fc7\u7535\u4f4d\u4e3a300\u00a0mV\u65f6\uff0cTOF\u503c\u9ad8\u8fbe4.96\u00a0s\u2212<\/sup>1<\/sup>\uff0c\u5e76\u5728\u4e0d\u540c\u7684\u5de5\u4f5c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5747\u4fdd\u6301\u826f\u597d\u7684\u7a33\u5b9a\u6027\uff08>1000\u00a0h\uff09\u3002\u5f53\u91d1\u5c5eFeNi\u542b\u91cf\u589e\u52a0\u65f6\uff0c10\u00a0mA\u00a0cm\u2212<\/sup>2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u8fc7\u7535\u4f4d\u53ef\u8fdb\u4e00\u6b65\u964d\u4f4e\u5230211\u00a0mV\u3002\u540c\u65f6\u5229\u7528DFT\u7406\u8bba\u6a21\u62df\u63ed\u793a\u4e86\u91d1\u5c5eFe\/Ni\u539f\u5b50\u6216(\u6c22)\u6c27\u5316\u7269FeNi\u7269\u79cd\u662f\u5176\u9ad8OER\u6d3b\u6027\u7684\u6839\u672c\u539f\u56e0\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cOxygen<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>evolving<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalytic<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>atoms<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>on<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>metal<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>carbides<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Materials<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 4\u00a0Fe\/Ni\u539f\u5b50\u7ea7\u50ac\u5316\u5242\u7684\u5408\u6210\u53ca\u7ed3\u6784\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41563-021-01006-2<\/p>\n

5. Nature\u00a0<\/b><\/strong><\/b>Energy<\/b><\/strong>\uff1a<\/b><\/strong>\u5177\u6709<\/b><\/strong>Pt<\/b><\/strong>–<\/b><\/strong>Fe<\/b><\/strong>\u5bf9\u4f4d\u70b9\u7684<\/b><\/strong>Pt<\/b><\/strong>\/<\/b><\/strong>Fe<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>3<\/b><\/sub><\/strong>\u4f5c\u4e3a\u8d85\u4f4e<\/b><\/strong>Pt<\/b><\/strong>\u6c27\u8fd8\u539f\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\u5929\u6d25\u5927\u5b66\u90b9\u5409\u519b\u6559\u6388\u3001\u6f58\u4f26\u526f\u6559\u6388\u56e2\u961f\u8054\u5408\u97e9\u56fd\u9996\u5c14\u5927\u5b66Jongwoo\u00a0Lim\u526f\u6559\u6388\u56e2\u961f\uff0c\u5408\u6210\u4e86\u65b0\u578b\u7684\u542b\u6709Pt-Fe\u539f\u5b50\u5bf9\u7684\u8d85\u4f4e\u94c2\u542b\u91cf\u7684Pt\/Fe2<\/sub>O3<\/sub>\u6c27\u8fd8\u539f\u50ac\u5316\u5242\u3002\u6c27\u8fd8\u539f\u662f\u71c3\u6599\u7535\u6c60\u548c\u950c\u7a7a\u7535\u6c60\u7684\u5173\u952e\u53cd\u5e94\uff0c\u8be5\u53cd\u5e94\u7684\u50ac\u5316\u5242\u4e3b\u8981\u4e3a\u8d35\u91d1\u5c5ePt\u3002\u964d\u4f4ePt\u7684\u7528\u91cf\u5bf9\u71c3\u6599\u7535\u6c60\u7684\u5927\u89c4\u6a21\u5e94\u7528\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u5355\u4f4d\u70b9Pt\u5177\u6709\u6700\u9ad8\u7684Pt\u5229\u7528\u7387\uff0c\u4f46\u5176\u5bf9\u6c27\u5206\u5b50\u7684\u89e3\u79bb\u6d3b\u5316\u6027\u80fd\u4e0d\u4f73\uff0c\u901a\u5e38\u8868\u73b0\u51fa\u8f83\u4f4e\u7684\u6d3b\u6027\u548c\u9009\u62e9\u6027\u3002\u7814\u7a76\u4eba\u5458\u5c06Pt\u539f\u5b50\u8d1f\u8f7d\u5728Fe2<\/sub>O3<\/sub>\uff08012\uff09\u6676\u9762\uff0cPt\u7684\u8d1f\u8f7d\u91cf\u4ec5\u4e3a0.13wt%\uff0c\u4e0e\u8868\u9762\u7684Fe\u539f\u5b50\u6784\u5efa\u4e86Pt-Fe\u539f\u5b50\u5bf9\u3002\u7814\u7a76\u8868\u660e\u5728\u5f3a\u7535\u5b50\u8026\u5408\u4f5c\u7528\u4e0bFe\u7684\u7535\u5b50\u8f6c\u79fb\u81f3Pt\uff0c\u5f62\u6210\u4e86\u90e8\u5206\u5360\u636ed\u8f68\u9053\uff0c\u5782\u76f4\u57fa\u9762\u7684dz2<\/sub>\u8f68\u9053\u4f7fPt-Fe\u548cO\u7684\u8f68\u9053\u91cd\u53e0\u6700\u5927\u5316\uff0c\u9ad8\u6548\u534f\u540c\u50ac\u5316O-O\u89e3\u79bb\uff0c\u540c\u65f6OH*\u4e2d\u95f4\u4f53\u5728Pt\u4f4d\u5feb\u901f\u89e3\u5438\uff0c\u514b\u670d\u4e86\u6c27\u8fd8\u539f\u50ac\u5316\u53cd\u5e94\u4e2d\u7684\u5438\u9644\u80fd\u6bd4\u4f8b\u5173\u7cfb\u7684\u9650\u5236\u3002\u5728\u78b1\u6027\u6761\u4ef6\u4e0b\uff0c\u8be5\u50ac\u5316\u5242\u7684\u8d77\u59cb\u7535\u4f4d\u548c\u534a\u6ce2\u7535\u4f4d\u5206\u522b\u4e3a1.15V\u548c1.05V\uff0c\u8d28\u91cf\u6d3b\u6027\u8fbe14.9\u00a0A\u00a0mg–<\/sup>1<\/sup>Pt<\/sub>@0.95\u00a0V\u3002\u5728\u950c\u7a7a\u6c14\u7535\u6c60\u548cH2<\/sub>-O2<\/sub>\u71c3\u6599\u7535\u6c60\u6d4b\u8bd5\u4e2d\uff0c\u8be5\u50ac\u5316\u5242\u5728\u80fd\u91cf\u5bc6\u5ea6\u548cPt\u5229\u7528\u7387\u65b9\u9762\u4e5f\u660e\u663e\u4f18\u4e8e20% Pt\/C\u50ac\u5316\u5242\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cPt<\/i><\/b><\/em><\/strong>\/<\/i><\/b><\/em><\/strong>Fe<\/i><\/b><\/em><\/strong>2<\/i><\/b><\/sub><\/em><\/strong>O<\/i><\/b><\/em><\/strong>3<\/i><\/b><\/sub><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>with<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Pt<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>Fe<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>sites<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>as<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>a<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalyst<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>for<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>oxygen<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>reduction<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>with<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>ultralow<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Pt<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>loading<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Energy<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 5\u00a0Pt\/Fe2<\/sub>O3<\/sub>\u50ac\u5316\u5242\u7684\u5f62\u8c8c\u53ca\u7ed3\u6784\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41560-021-00826-5<\/p>\n

6. Nature\u00a0<\/b><\/strong><\/b>Communications<\/b><\/strong>\uff1a<\/b><\/strong>\u5355\u539f\u5b50<\/b><\/strong>Te<\/b><\/strong>\u7a7a\u4f4d\u7684\u6709\u5e8f\u8c03\u63a7\u63d0\u5347\u539f\u5b50\u7ea7\u8584\u7684<\/b><\/strong>PtTe<\/b><\/strong>2<\/b><\/sub><\/strong>\u7535\u50ac\u5316\u4ea7\u6c22\u6027\u80fd<\/b><\/strong><\/p>\n

\u76ee\u524d\u5730\u7403\u4e0a\u7684\u5f88\u591a\u95ee\u9898\uff0c\u6bd4\u5982\u80fd\u6e90\u9700\u6c42\u589e\u52a0\u3001\u73af\u5883\u6c61\u67d3\u4e25\u91cd\u548c\u5730\u7403\u8d44\u6e90\u6709\u9650\u7b49\u90fd\u5a01\u80c1\u7740\u4eba\u7c7b\u7684\u53ef\u6301\u7eed\u53d1\u5c55\u3002\u800c\u5229\u7528\u5148\u8fdb\u7684\u65b0\u80fd\u6e90\u6280\u672f\uff0c\u53ef\u6301\u7eed\u53d1\u5c55\u7684\u80fd\u6e90\u6750\u6599\u548c\u7eff\u8272\u6280\u672f\u53ef\u4ee5\u6709\u6548\u7684\u5c06\u65b0\u578b\u53ef\u6301\u7eed\u8d44\u6e90\uff08\u4f8b\u5982\u6c34\u3001\u4e8c\u6c27\u5316\u78b3\u3001\u6c2e\u6c14\u548c\u592a\u9633\u80fd\uff09\u8f6c\u6362\u4e3a\u9ad8\u9644\u52a0\u503c\u4ea7\u54c1\uff0c\u6709\u671b\u89e3\u51b3\u76ee\u524d\u7684\u80fd\u6e90\u5371\u673a\u3002\u8fd1\u65e5\uff0c\u4e2d\u56fd\u6df1\u5733\u5927\u5b66\u82cf\u9648\u826f\u6559\u6388\u3001\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66Jiong\u00a0Lu\u6559\u6388\u4ee5\u53ca\u65b0\u52a0\u5761\u5357\u6d0b\u7406\u5de5\u5927\u5b66Bin\u00a0Liu\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba\u5236\u5907\u4e86\u4e8c\u7ef4\u539f\u5b50\u7ea7PtTe2<\/sub>\u8584\u7eb3\u7c73\u7247\uff0c\u5176\u5177\u6709\u5206\u6563\u7684\u5355\u539f\u5b50Te\u7a7a\u4f4d\uff08Te-SAVs\uff09\u548c\u539f\u5b50\u7ea7\u914d\u4f4d\u4e0d\u8db3\u7684Pt\u4f4d\u4f5c\u4e3a\u7535\u50ac\u5316\u5242\u3002\u53d7\u70ed\u5904\u7406\u9a71\u52a8\u7684Te-SAVs\u8fc1\u79fb\uff0c\u4ee5\u5f62\u6210\u70ed\u529b\u5b66\u7a33\u5b9a\u7684\u6709\u5e8fTe-SAV\u7c07\uff0c\u65e2\u964d\u4f4e\u4e86\u8d39\u7c73\u80fd\u7ea7\u9644\u8fd1\u672a\u914d\u4f4d\u7684Pt\u4f4d\u70b9\u7684\u6001\u5bc6\u5ea6\uff0c\u53c8\u964d\u4f4e\u4e86Pt\u4f4d\u70b9\u7684\u76f8\u4e92\u4f5c\u7528\u8f68\u9053\u533a\u57df\u3002\u6709\u6548\u5730\u964d\u4f4e\u4e86\u539f\u5b50\u7ea7Pt\u6d3b\u6027\u4f4d\u70b9\u4e0eH\u4e2d\u95f4\u4f53\u7684\u7ed3\u5408\u5f3a\u5ea6\uff0c\u8fd9\u4f7f\u5f97PtTe2<\/sub>\u7eb3\u7c73\u7247\u5728\u7535\u50ac\u5316\u6790\u6c22\u53cd\u5e94\u4e2d\u5177\u6709\u5f88\u9ad8\u7684\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cOrdered<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>clustering<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>of<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>single<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>atomic<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Te<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>vacancies<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>in<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>atomically<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>thin<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>PtTe<\/i><\/b><\/em><\/strong>2<\/i><\/b><\/sub><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>promotes<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>hydrogen<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>evolution<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalysis<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Communications<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 6\u00a0PtTe2<\/sub>\u7535\u50ac\u5316\u5242\u7684\u5236\u5907\u53ca\u5f62\u8c8c\u7ed3\u6784\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41467-021-22681-4<\/p>\n

7. Nature<\/b><\/strong><\/b>Communications<\/b><\/strong>\uff1a<\/b><\/strong>\u94c1\u915e\u83c1\u5206\u5b50\u7684\u65b0\u578b\u914d\u4f4d\u7535\u8377\u8c03\u63a7\u7b56\u7565\u63d0\u5347\u50ac\u5316\u6d3b\u6027<\/b><\/strong><\/p>\n

\u5f00\u53d1\u4f4e\u6210\u672c\u9ad8\u6d3b\u6027\u7684\u6c27\u8fd8\u539f\u50ac\u5316\u5242\u5bf9\u71c3\u6599\u548c\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\u7684\u5feb\u901f\u53d1\u5c55\u81f3\u5173\u91cd\u8981\u3002\u4e2d\u5357\u5927\u5b66\u7269\u7406\u4e0e\u7535\u5b50\u5b66\u9662\u5218\u654f\u6559\u6388\u56e2\u961f\u9488\u5bf9\u94c1\u915e\u83c1\u5206\u5b50\u8fdb\u884c\u4e86\u6df1\u5165\u7814\u7a76\uff0c\u5176\u5de5\u4f5c\u8868\u660e\u914d\u4f4d\u8bf1\u5bfc\u94c1\u539f\u5b50\u7684\u7535\u8377\u5c40\u57df\u5316\u53ef\u4ee5\u6709\u6548\u7684\u63d0\u9ad8\u5206\u5b50\u50ac\u5316\u5242\u7684\u6c27\u8fd8\u539f\u6d3b\u6027\u3002\u94c1\u915e\u83c1\u5206\u5b50\u50ac\u5316\u5242\u5177\u6709\u72ec\u7279\u7684Fe-N4<\/sub>\u6d3b\u6027\u548c\u8f83\u4f4e\u7684\u6c27\u8fd8\u539f\u53cd\u5e94\u80fd\u5792\uff0c\u57fa\u4e8e\u6b64\u79cd\u7279\u8d28\uff0c\u4ece\u5176\u88ab\u53d1\u73b0\u5f00\u59cb\u5c31\u5f15\u8d77\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\u548c\u7814\u7a76\u3002\u7136\u800c\uff0c\u94c1\u915e\u83c1\u7684\u4e8c\u7ef4\u5e73\u9762\u7ed3\u6784\u4f7f\u5f97\u5176\u7535\u5b50\u7ed3\u6784\u6781\u5176\u5bf9\u79f0\uff0c\u5e76\u4e14\u8fd9\u79cd\u7535\u5b50\u7ed3\u6784\u9650\u5236\u4e86\u5176\u5bf9\u6c27\u6c14\u7684\u5438\u9644\u548c\u6d3b\u5316\uff0c\u56e0\u6b64\u8c03\u63a7\u6d3b\u6027\u4e2d\u5fc3\u7684\u7535\u5b50\u7ed3\u6784\u63d0\u9ad8\u53cd\u5e94\u6d3b\u6027\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u5218\u654f\u6559\u6388\u56e2\u961f\u63d0\u51fa\u4e86\u4e00\u79cd\u8f74\u5411Fe-O\u914d\u4f4d\u8bf1\u5bfc\u7684\u7535\u5b50\u91cd\u5206\u5e03\u7b56\u7565\uff0c\u901a\u8fc7\u914d\u4f4d\u8bf1\u5bfc\u7535\u8377\u5c40\u57df\u5316\uff0c\u6253\u7834\u6d3b\u6027\u4e2d\u5fc3\u7684\u7535\u8377\u5bf9\u79f0\u6027\uff0c\u63d0\u9ad8\u4e86\u5206\u5b50\u50ac\u5316\u5242\u7684\u6c27\u8fd8\u539f\u6d3b\u6027\u3002\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u914d\u4f4d\u53ef\u6709\u6548\u8c03\u8282\u94c1\u915e\u83c1\u7684\u7535\u5b50\u7ed3\u6784\uff0c\u4f7f\u5f97\u5176\u50ac\u5316\u6027\u80fd\u589e\u5f3a\u3002\u540c\u6b65X\u5c04\u7ebf\u548c\u83ab\u65af\u5821\u5c14\u8c31\u7684\u6d4b\u8bd5\u7ed3\u679c\u8868\u660e\u4e86\u914d\u4f4d\u7684\u6709\u6548\u6784\u5efa\u5e76\u63d0\u9ad8\u4e86\u6c27\u6c14\u7684\u5438\u9644\u80fd\u529b\u3002\u5b9e\u9a8c\u6240\u83b7\u5f97\u7684\u6700\u4f18\u50ac\u5316\u5242\uff0c\u663e\u793a\u51fa\u6781\u5176\u4f18\u5f02\u7684\u6c27\u8fd8\u539f\u6027\u80fd\uff0c\u534a\u6ce2\u7535\u4f4d\u4e3a0.90\u00a0V\uff0c\u5854\u83f2\u513f\u659c\u7387\u4e3a\u521b\u7eaa\u5f55\u768427.5\u00a0mV\u00a0dec\u2212<\/sup>1<\/sup>\uff0c\u8fd9\u9879\u5de5\u4f5c\u4e3a\u6784\u5efa\u9ad8\u6548\u7684\u5206\u5b50\u50ac\u5316\u5242\u6253\u5f00\u4e86\u65b0\u601d\u8def\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cIron<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>phthalocyanine<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>with<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>coordination<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>induced<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>electronic<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>localization<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>to<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>boost<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>oxygen<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>reduction<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>reaction<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u4e8eNature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Communications<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 7\u00a0\u94c1\u915e\u83c1\u5206\u5b50\u7ed3\u6784\u3001\u50ac\u5316\u53cd\u5e94\u7535\u8377\u8f6c\u79fb\u548c\u53cd\u5e94\u81ea\u7531\u80fd\u80fd\u5792\u793a\u610f\u56fe<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41467-020-18062-y<\/p>\n

8. Nature\u00a0<\/b><\/strong><\/b>Catalysis<\/b><\/strong>\uff1a<\/b><\/strong>\u5355\u4f4d\u70b9<\/b><\/strong>Co<\/b><\/strong>\u9ad8\u6548\u6c34\u6c27\u5316\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\u7535\u89e3\u6c34\u5728\u80fd\u6e90\u5229\u7528\u4e2d\u6709\u7740\u8f83\u91cd\u8981\u7684\u5730\u4f4d\uff0c\u7531\u4e8e\u591a\u7535\u5b50\u53cd\u5e94\uff0c\u6790\u6c27\u53cd\u5e94\u4f5c\u4e3a\u7535\u89e3\u6c34\u7684\u9633\u6781\u53cd\u5e94\u5bf9\u6574\u4e2a\u7535\u89e3\u8fc7\u7a0b\u6548\u7387\u8d77\u5230\u4e86\u51b3\u5b9a\u6027\u7684\u4f5c\u7528\u3002\u76ee\u524d\u6240\u4f7f\u7528\u7684\u7535\u50ac\u5316\u5242\u4e3b\u8981\u5305\u62ec\u9499\u949b\u77ff\u6750\u6599\u3001\u5c16\u6676\u77f3\u91d1\u5c5e\u6c27\u5316\u7269\u4ee5\u53ca\u5c42\u72b6\u53cc\u91d1\u5c5e\u6c22\u6c27\u5316\u7269\uff0c\u90fd\u53ef\u4ee5\u6709\u6548\u7684\u63d0\u5347\u6790\u6c27\u53cd\u5e94\u5728\u78b1\u6027\u7535\u89e3\u8d28\u4e2d\u7684\u53cd\u5e94\u6548\u7387\u3002\u4f46\u662f\u5927\u90e8\u5206\u5f02\u76f8\u50ac\u5316\u5242\u8868\u9762\u7ed3\u6784\u7684\u4e0d\u786e\u5b9a\u6027\u5bfc\u81f4\u4e86\u5bf9\u4e8e\u7535\u50ac\u5316\u53cd\u5e94\u6d3b\u6027\u4f4d\u70b9\u548c\u672c\u5f81\u6d3b\u6027\u7684\u8ba4\u77e5\u6bd4\u8f83\u6a21\u7cca\uff0c\u4ee5\u81f3\u4e8e\u50ac\u5316\u53cd\u5e94\u673a\u7406\u7684\u7814\u7a76\u65e0\u6cd5\u660e\u786e\u3002\u56e0\u6b64\uff0c\u7cbe\u51c6\u7684\u50ac\u5316\u4f4d\u70b9\u63a7\u5236\u5bf9\u4e8e\u9ad8\u6027\u80fd\u7684\u7535\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u548c\u6790\u6c27\u53cd\u5e94\u7684\u53cd\u5e94\u673a\u7406\u7684\u7814\u7a76\u663e\u5f97\u5c24\u4e3a\u91cd\u8981\u3002\u7f8e\u56fd\u5f17\u5409\u5c3c\u4e9a\u5927\u5b66\u5316\u5b66\u7cfb\u5f20\u68ee\u6559\u6388\u8bfe\u9898\u7ec4\u548c\u52a0\u5dde\u7406\u5de5\u5b66\u9662 William\u00a0A. Goddard\u00a0III\u6559\u6388\u8bfe\u9898\u7ec4\u901a\u8fc7\u53ef\u63a7\u80f6\u4f53\u5408\u6210\u6cd5\u6210\u529f\u5f97\u5230\u5747\u4e00\u5206\u6563\u5728\u677f\u949b\u77ffTiO2<\/sub>\u7eb3\u7c73\u68d2\u4e0a\u7684\u5177\u6709\u7cbe\u51c6\u7ed3\u6784\u7684\u94b4\u5355\u539f\u5b50\u7535\u50ac\u5316\u5242\uff0c\u5e76\u4e14\u5bf9\u7cbe\u786e\u7684\u94b4\u5355\u539f\u5b50\u7ed3\u6784\u8fdb\u884c\u4e86\u91cf\u5b50\u529b\u5b66\u7406\u8bba\u6a21\u62df\uff0c\u4ece\u800c\u5bf9\u6790\u6c27\u53cd\u5e94\u5728\u5355\u6d3b\u6027\u4f4d\u70b9\u7684\u53cd\u5e94\u673a\u7406\u6df1\u5165\u7406\u89e3\u3002\u8be5\u5de5\u4f5c\u4ee5\u201cOxygen<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>evolution<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>reaction<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>over<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>catalytic<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>single<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>site<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Co<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>in<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>a<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>well<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>defined<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>brookite<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>TiO<\/i><\/b><\/em><\/strong>2<\/i><\/b><\/sub><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>nanorod<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>surface<\/i><\/b><\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature<\/i><\/b><\/em><\/strong>\u00a0<\/i><\/b><\/em><\/strong>Catalysis<\/i><\/b><\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u56fe 8\u00a0Co\/TiO2<\/sub>\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5f62\u8c8c\u8868\u5f81<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41929-020-00550-5<\/p>\n

9. Nature\u00a0<\/b><\/strong><\/b>Communications<\/b><\/strong>\uff1a<\/b><\/strong>\u591a\u5c42\u56fa\u5b9a\u91d1\u5c5e\u524d\u9a71\u4f53\u7b56\u7565\u5236\u5907\u8d85\u9ad8\u8d1f\u8f7d\u91cf\u7684\u5355\u539f\u5b50\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

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\"\"<\/b><\/strong><\/p>\n

\u56fe 9\u00a0Fe\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5408\u6210\u793a\u610f\u56fe\u53ca\u5f62\u8c8c\u8868\u5f81\u56fe<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41467-020-19599-8<\/p>\n

\u672c\u6587\u7531\u63d0\u7434\u8537\u8587\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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