{"id":224677,"date":"2021-07-21T06:34:42","date_gmt":"2021-07-20T22:34:42","guid":{"rendered":"\/\/m.iemloyee.com\/?p=224677"},"modified":"2021-07-20T21:34:57","modified_gmt":"2021-07-20T13:34:57","slug":"ff%e5%80%bc%e7%aa%81%e7%a0%b40-8%ef%bc%8cpscs%e5%8f%88%e5%8f%91%e4%b8%80%e7%af%87science%e5%ad%90%e5%88%8a%ef%bc%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=224677","title":{"rendered":"FF\u503c\u7a81\u78340.8\uff0cPSCs\u53c8\u53d1\u4e00\u7bc7Science\u5b50\u520a\uff01"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u6742\u5316\u6709\u673a-\u65e0\u673a\u5364\u5316\u7269\u9499\u949b\u77ff\u662f\u4e00\u79cd\u5f88\u6709\u5438\u5f15\u529b\u7684\u5149\u7535\u6750\u6599\uff0c\u5177\u6709\u6210\u672c\u4f4e\u3001\u6613\u5236\u9020\u3001\u5168\u8272\u5438\u6536\u592a\u9633\u5149\u5f3a\u3001\u8f7d\u6d41\u5b50\u6269\u6563\u957f\u5ea6\u957f\u7b49\u4f18\u70b9\u3002\u5177\u6709\u5e38\u89c4\uff08n-i-p\uff09\u7ed3\u6784\u7684\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\uff08PSCs\uff09\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387\uff08PCEs\uff09\u6700\u9ad8\u5df2\u8fbe\u523025.5%\u3002\u4f46\u662f\uff0c\u5012\u7f6e\uff08p-i-n\uff09PSCs\u7684PCE\u660e\u663e\u4f4e\u4e8e\u5e38\u89c4\u7ed3\u6784\u5668\u4ef6\u3002\u5c3d\u7ba1\u5f00\u8def\u7535\u538b\uff08V<\/em>oc<\/sub>\uff09\u3001\u77ed\u8def\u7535\u6d41\uff08J<\/em>sc<\/sub>\uff09\u548c\u586b\u5145\u56e0\u5b50\uff08FF\uff09\u5bf9PCE\u6709\u7740\u9ad8\u5ea6\u7684\u76f8\u5173\u6027\u548c\u534f\u540c\u4f5c\u7528\uff0c\u4f46\u5927\u591a\u6570\u7814\u7a76\u8005\u4e3b\u8981\u81f4\u529b\u4e8e\u4f18\u5316V<\/em>oc<\/sub>\u548cJ<\/em>sc<\/sub>\uff0c\u800c\u4e0d\u662f\u7406\u89e3\u548c\u4f18\u5316FF\u503c\u3002\u901a\u5e38\uff0cPSCs\u7684FF\u503c\u57280.7\u52300.8\u4e4b\u95f4\uff0c\u5373\u4f7fPCEs\u572822.7%\u523023.3%\u7684\u5668\u4ef6\uff0c\u5176FF\u503c\u4e5f\u4f4e\u4e8e0.8\u3002\u4f18\u5316FF\uff0c\u901a\u5e38\u9700\u8981\u4f4e\u4e32\u8054\u7535\u963b\uff08R<\/em>s<\/sub>\uff09\u548c\u9ad8\u5e76\u8054\u7535\u963b\uff08R<\/em>sh<\/sub>\uff09\u3002PSCs\u4e2d\u7684R<\/em>s<\/sub>\u7531\u5bfc\u7535\u57fa\u5e95\u3001\u7535\u5b50\u548c\u7a7a\u7a74\u4f20\u8f93\u5c42\uff08ETL\u548cHTL\uff09\u7b49\u786e\u5b9a\uff0c\u56e0\u6b64\u63d0\u9ad8ETL\u548cHTL\u7684\u7535\u5bfc\u7387\u548c\u8fc1\u79fb\u7387\u6709\u52a9\u4e8e\u4f18\u5316FF\u503c\u3002\u4e3a\u63d0\u9ad8R<\/em>sh<\/sub>\u503c\uff0c\u5e94\u5c3d\u53ef\u80fd\u51cf\u5c0f\u8f7d\u6d41\u5b50\u590d\u5408\u5f15\u8d77\u7684\u6f0f\u7535\u6d41\u3002\u867d\u7136\u5df2\u63d0\u51fa\u4e86\u8bb8\u591a\u949d\u5316\u65b9\u6cd5\u6765\u964d\u4f4e\u7f3a\u9677\u5bc6\u5ea6\uff0c\u663e\u8457\u63d0\u9ad8Rsh\u548c\u51cf\u5c11\u7f3a\u9677\u8bf1\u5bfc\u7684\u590d\u5408\u3002\u5f53\u5c0f\u5206\u5b50\u4f5c\u6dfb\u52a0\u5242\u65f6\uff0c\u5176\u9ad8\u6325\u53d1\u6027\u548c\u9ad8\u6269\u6563\u7cfb\u6570\u53ef\u80fd\u4f7fPSCs\u5728\u6781\u7aef\u6761\u4ef6\u4e0b\u96be\u4ee5\u4fdd\u6301\u957f\u671f\u7a33\u5b9a\u6027\u3002\u5f53\u4f7f\u7528\u805a\u5408\u7269\u4f5c\u4e3a\u6dfb\u52a0\u5242\u65f6\uff0c\u5176\u5177\u6709\u4e00\u7ef4\uff081D\uff09\u7ebf\u6027\u7ed3\u6784\uff0c\u5728\u4fee\u9970\u9499\u949b\u77ff\u8584\u819c\u7684\u8868\u9762\u65f6\u53ea\u80fd\u8868\u73b0\u51fa\u5355\u4e00\u7684\u949d\u5316\u6548\u5e94\u3002\u5f88\u5c11\u6709\u7814\u7a76\u8005\u901a\u8fc7\u5177\u6709\u591a\u4e2a\u5206\u652f\u548c\u6bcf\u4e2a\u5206\u652f\u4e0a\u6709\u591a\u4e2a\u5b98\u80fd\u56e2\u7684\u4e09\u7ef4\uff083D\uff09\u805a\u5408\u7269\u76f4\u63a5\u949d\u5316\u9499\u949b\u77ff\u8584\u819c\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u674e\u70ab\u534e\u6559\u6388\u548c\u745e\u58eb\u6d1b\u6851\u8054\u90a6\u7406\u5de5\u5927\u5b66Michael Gr\u00e4tzel\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd3D\u661f\u5f62\u591a\u9762\u4f53\u4f4e\u805a\u500d\u534a\u7845\u6c27\u70f7-\u805a\u7532\u57fa\u4e19\u70ef\u9178\u4e09\u6c1f\u4e59\u916f-b-\u805a\u7532\u57fa\u4e19\u70ef\u9178\u7532\u916f\uff08PPP\uff09\u805a\u5408\u7269\u4f5c\u4e3a\u8c03\u8282\u9499\u949b\u77ff\u8584\u819c\u7ed3\u6676\u7684\u65b0\u578b\u8c03\u8282\u5242\u3002\u661f\u5f62PPP\u6750\u6599\u4e2d\u4f5c\u4e3a\u6838\u5fc3\u7684\u591a\u9762\u4f53\u4f4e\u805a\u500d\u534a\u7845\u6c27\u70f7\u88ab\u516b\u4e2a\u652f\u94fe\u5305\u56f4\uff0c\u5305\u62ec\u805a\u7532\u57fa\u4e19\u70ef\u9178\u4e09\u6c1f\u4e59\u916f\u548c\u805a\u7532\u57fa\u4e19\u70ef\u9178\u7532\u916f\u5206\u5b50\u94fe\u3002\u6838\u5fc3\u662f\u4e00\u79cd\u6709\u673a-\u65e0\u673a\u5206\u5b50\u5185\u6742\u5316\u6750\u6599\uff0c\u5177\u6709\u9ad8\u5ea6\u5bf9\u79f0\u7684\u521a\u6027Si-O-Si\u7acb\u65b9\u7b3c\u9aa8\u67b6\uff0c\u53ef\u4ee5\u63d0\u4f9bPPP\u6750\u6599\u76843D\u7ed3\u6784\u7a33\u5b9a\u6027\u3002\u5728PPP\u805a\u5408\u7269\u5206\u652f\u4e0a\uff0c\u6709\u591a\u4e2a\u5316\u5b66\u951a\u5b9a\u4f4d\u70b9\uff0c\u5305\u62ec\u7fb0\u57fa\uff08C=O\uff09\u548c-CF3<\/sub>\uff0c\u5b83\u4eec\u4f5c\u4e3a3D\u9aa8\u67b6\u6a21\u677f\u949d\u5316\u6676\u754c\u548c\u754c\u9762\u8868\u9762\u7684\u7f3a\u9677\uff0c\u6291\u5236\u975e\u8f90\u5c04\u590d\u5408\u548c\u7535\u8377\u8f93\u8fd0\u635f\u5931\uff0c\u5e76\u6539\u5584\u5728\u6c34\u5206\u3001\u70ed\uff0c\u5149\u7167\u5e94\u529b\u3002\u6d4b\u8bd5\u7ed3\u679c\u8868\u660e\uff0cPPP\u6539\u6027\u7684\u5012\u7f6e\u5668\u4ef6\u83b7\u5f97\u4e86\u6700\u4f73\u768422.1%\u7684PCEs\u548c\u9ad8\u8fbe0.862\u7684FF\u503c\u3002\u5728\u5927\u6c14\u73af\u5883\u4e0b\uff0840% RH\u300125 \u2103\uff09\u66b4\u97326000 h\u540e\uff0c\u975e\u5c01\u88c5\u6539\u6027\u5668\u4ef6\u663e\u793a\u51fa\u663e\u8457\u589e\u5f3a\u7684\u73af\u5883\u7a33\u5b9a\u6027\uff0c\u4fdd\u6301\u8d85\u8fc793%\u7684\u521d\u59cb\u6548\u7387\u3002\u5c01\u88c5\u540e\u7684\u6539\u8fdb\u578b\u5668\u4ef6\u5177\u6709\u826f\u597d\u7684\u5de5\u4f5c\u7a33\u5b9a\u6027\uff0c\u572845 \u2103\u4e00\u6b21\u592a\u9633\u5149\u7167\u4e0b\u6700\u5927\u529f\u7387\u70b9\u8ddf\u8e2a1000 h\u540e\uff0c\u6548\u7387\u51e0\u4e4e\u6ca1\u6709\u53d8\u5316\uff1b\u572875 \u2103\u4e00\u6b21\u592a\u9633\u5149\u7167\u4e0b\u8fde\u7eed1000 h\uff0c\u70ed\u7a33\u5b9a\u6027\u4ecd\u65e7\u975e\u5e38\u597d\uff0c\u521d\u59cb\u6548\u7387\u4fdd\u6301\u572891%\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cEfficient and stable inverted perovskite solar cells with very high fill factors via incorporation of star-shaped polymer\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aScience Advances<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001PPP\u805a\u5408\u7269\u548c\u9499\u949b\u77ff\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528<\/strong>
\n \"\"\uff08A\uff09PPP\u805a\u5408\u7269\u7684\u7ed3\u6784\u5f0f\uff1b<\/p>\n

\uff08B\uff09PPP\u805a\u5408\u7269\u4e0e\u9499\u949b\u77ff\u76f8\u4e92\u4f5c\u7528\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08C\uff09PPP\u805a\u5408\u7269\u3001PbI2<\/sub>\u548cPPP-PbI2<\/sub>\u7684FTIR\u5149\u8c31\uff1b<\/p>\n

\uff08D\uff09C=O\u7684\u6307\u7eb9\u533a\uff1b<\/p>\n

\uff08E-F\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u6027\u9499\u949b\u77ff\u8584\u819c\u4e2dPb 4f\u548cN 1s\u7684XPS\u5149\u8c31\uff1b<\/p>\n

\uff08G\uff09FAI\u548cFAI-PPP\u6df7\u5408\u7269\u76841<\/sup>H NMR\u5149\u8c31\uff1b<\/p>\n

\uff08H\uff09MABr\u548cMABr-PPP \u6df7\u5408\u7269\u76841<\/sup>H NMR\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e8c\u3001\u9499\u949b\u77ff\u8584\u819c\u7684\u5f62\u6001\u548c\u7ed3\u6784\u7279\u6027<\/strong>
\n \"\"\uff08A-B\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u6027\u9499\u949b\u77ff\u8584\u819c\u7684\u4fef\u89c6SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08C-D\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u6027\u9499\u949b\u77ff\u8584\u819c\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08E\uff09PPP\u6539\u6027\u9499\u949b\u77ff\u6676\u4f53\u7684\u9ad8\u5206\u8fa8\u7387TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08F\uff09\uff08E\uff09\u4e2d\u7ea2\u8272\u6846\u7684\u653e\u5927TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08G\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u6027\u9499\u949b\u77ff\u8584\u819c\u7684XRD\u8c31\u3002<\/p>\n

\u56fe\u4e09\u3001\u5149\u4f0f\u6027\u80fd<\/strong>
\n \"\"\uff08A\uff09PP\u6539\u8fdbPSCs\u7684\u5668\u4ef6\u7ed3\u6784\uff1b<\/p>\n

\uff08B\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u8fdb\u5668\u4ef6\u7684\u6b63\u5411\u548c\u53cd\u5411\u626b\u63cf\u4e2d\u83b7\u5f97\u7684J-V<\/em>\u66f2\u7ebf\uff1b<\/p>\n

\uff08C\uff09\u57280.91\u548c0.97 V\u4e0b\uff0c\u5bf9\u7167\u7ec4\u548cPPP\u6539\u8fdb\u5668\u4ef6\u7684\u5149\u7535\u6d41\u548cSPO\uff1b<\/p>\n

\uff08D\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u8fdb\u5668\u4ef6\u7684EQE\u8c31\u548c\u79ef\u5206\u7535\u6d41\uff1b<\/p>\n

\uff08E\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u8fdb\u8bbe\u5907\u768420\u4e2aPSCs\u7684PCE\u76f4\u65b9\u56fe\uff1b<\/p>\n

\uff08F\uff09\u6536\u96c6FFs\u4e0ePCE\uff0c\u62a5\u9053\u5012\u7f6ePSCs\u3002<\/p>\n

\u56fe\u56db\u3001PPP\u6539\u6027\u5bf9\u9499\u949b\u77ff\u8584\u819c\u7535\u6548\u5e94\u7684\u5f71\u54cd<\/strong>
\n \"\"\uff08A-B\uff09SSPL\u3001\u5bf9\u7167\u7ec4\u548cPPP\u6539\u6027\u9499\u949b\u77ff\u8584\u819c\u7684TRPL\u5149\u8c31\uff1b<\/p>\n

\uff08C\uff091\/C2<\/sup>\u4e0e\u63a7\u5236\u548cPPP\u6539\u8fdbPSCs\u4e2d\u65bd\u52a0\u7684\u7535\u538b\u56fe\uff08Mott-Schottky\uff09\uff1b<\/p>\n

\uff08D\uff09\u5668\u4ef6\u4e2dV<\/em>oc<\/sub>\u4e0eJ<\/em>sc<\/sub>\u7684\u5bf9\u6570\u4f5c\u56fe\uff1b<\/p>\n

\uff08E\uff09\u5bf9\u7167\u7ec4\u548cPPP \u6539\u8fdbPSCs\u7684J-V\u66f2\u7ebf\uff1b<\/p>\n

\uff08F\uff09\u5668\u4ef6FF S-Q\u9650\u5236\u5305\u62ec\u7535\u8377\u4f20\u8f93\u635f\u8017\u548c\u975e\u8f90\u5c04\u635f\u8017\u3002<\/p>\n

\u56fe\u4e94\u3001\u7a33\u5b9a\u6027<\/strong>
\n \"\"\uff08A\uff09\u975e\u5c01\u88c5\u5bf9\u7167\u7ec4\u5668\u4ef6\u548cPPP\u6539\u8fdb\u5668\u4ef6\u7684\u7a7a\u6c14\u7a33\u5b9a\u6027\uff1b<\/p>\n

\uff08B\uff09\u572845 \u00b0C\u4e00\u6b21\u592a\u9633\u5149\u7167\u4e0b\uff0c\u5728\u7a7a\u6c14\u4e2d\u6709\u65e0PPP\u6539\u8fdb\u7684\u5c01\u88c5PSCs\u7684\u6700\u5927\u529f\u7387\u70b9\uff08MPP\uff09\u8ddf\u8e2a\uff1b<\/p>\n

\uff08C\uff09\u5c01\u88c5\u5bf9\u7167\u7ec4\u5668\u4ef6\u548cPPP\u6539\u8fdb\u5668\u4ef6\u7684\u70ed\u7a33\u5b9a\u6027\uff1b<\/p>\n

\uff08D-E\uff09\u5bf9\u7167\u7ec4\u548cPPP\u6539\u8fdb\u7684\u65e0\u7535\u6781PSCs\u5668\u4ef6\u572875 \u00b0C\u548c\u5168\u8c31\u592a\u9633\u5149\u7167\u4e0b\u3001N2<\/sub>\u6c14\u6c1b\u4e2d\u70ed\u8001\u5316300 h\u524d\u540e\u7684ToF-SIMS\u6df1\u5ea6\u66f2\u7ebf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aEfficient and stable inverted perovskite solar cells with very high fill factors via incorporation of star-shaped polymer<\/a><\/strong>. Science Advances<\/em>, 2021<\/strong>, DOI: 10.1126\/sciadv.abg0633.<\/p>\n

\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

\u674e\u70ab\u534e\uff0c\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u6559\u6388\uff0c\u4f26\u6566\u739b\u4e3d\u5973\u738b\u5927\u5b66\u5ba2\u5ea7\u6559\u6388<\/strong>\uff0c\u201c\u9986\u85cf\u58c1\u753b\u4fdd\u62a4\u4fee\u590d\u4e0e\u6750\u6599\u79d1\u5b66\u7814\u7a76\u201d\u56fd\u5bb6\u6587\u7269\u5c40\u91cd\u70b9\u79d1\u7814\u57fa\u5730\u526f\u4e3b\u4efb\uff0c\u9999\u6e2f\u5927\u5b66\u7535\u5b50\u5de5\u7a0b\u7cfb\uff08\u5149\u7535\u5b50\u5b66\uff09\u535a\u58eb\uff0c\u7eb3\u7c73\u80fd\u6e90\u6750\u6599\u7814\u7a76\u4e2d\u5fc3\u6838\u5fc3\u6210\u5458\u3002\u4ece\u4e8b\u7eb3\u7c73\u5149\u7535\u6750\u6599\u4e0e\u6587\u7269\u4fdd\u62a4\u6750\u6599\u76f8\u5173\u7814\u7a76\u3002\u4e3b\u6301\u56fd\u5bb6\u3001\u7701\u90e8\u7ea7\u7b49\u5404\u7c7b\u9879\u76ee10\u4f59\u9879\uff0c\u6388\u6743\u56fd\u5bb6\u53d1\u660e\u4e13\u522919\u9879\uff0c\u4ee5\u7b2c\u4e00\u4f5c\u8005\u6216\u901a\u8baf\u4f5c\u8005\u5728Sci. Adv., Nature Commun., Chem.Soc. Rev., Energy Environ. Sci., Adv. Mater., Adv. Energy. Mater., Adv. Funct. Mater., \u7b49\u56fd\u9645\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u658765\u7bc7\uff0c\u5f71\u54cd\u56e0\u5b50\u5927\u4e8e15\u7684\u8bba\u658723\u7bc7\uff0c 11 \u7bc7\u6587\u7ae0\u88ab\u9009\u4e3a\u5c01\u9762\u3002 \u5165\u9009\u56fd\u5bb6\u4e07\u4eba\u8ba1\u5212\u201c\u9752\u5e74\u62d4\u5c16\u4eba\u624d\u201d\uff0c\u9655\u897f\u7701\u79d1\u6280\u91cd\u70b9\u521b\u65b0\u56e2\u961f\u8d1f\u8d23\u4eba\uff0c\u9655\u897f\u7701\u9ad8\u5c42\u6b21\u4eba\u624d\u201c\u7279\u652f\u8ba1\u5212\u201c\u9752\u5e74\u62d4\u5c16\u4eba\u624d\uff0c\u9655\u897f\u7701\u9752\u5e74\u79d1\u6280\u65b0\u661f\uff0c\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u7ff1\u7fd4\u9752\u5e74\u5b66\u8005\u7b49\u3002<\/p>\n

https:\/\/teacher.nwpu.edu.cn\/lixuanhua<\/a><\/p>\n

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\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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