{"id":223407,"date":"2021-06-16T06:37:39","date_gmt":"2021-06-15T22:37:39","guid":{"rendered":"\/\/m.iemloyee.com\/?p=223407"},"modified":"2021-06-15T21:37:54","modified_gmt":"2021-06-15T13:37:54","slug":"%e9%92%99%e9%92%9b%e7%9f%bf%e5%a4%a7%e7%89%9b%ef%bc%9asang-il-seok%e3%80%81tae-woo-lee%e3%80%81michael-d-mcgehee%e3%80%81edward-h-sargent%e3%80%81michael-gratzel%e8%bf%91%e6%9c%9f%e6%88%90%e6%9e%9c","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=223407","title":{"rendered":"\u9499\u949b\u77ff\u5927\u725b\uff1aSang Il Seok\u3001Tae-Woo Lee\u3001Michael D. McGehee\u3001Edward H. Sargent\u3001Michael Gratzel\u8fd1\u671f\u6210\u679c\u4e00\u89c8\u00a0"},"content":{"rendered":"

Nature Photonics\uff1a\u9ad8\u6548\u53d1\u5149\u4e8c\u6781\u7ba1\u4e2d\u9499\u949b\u77ff\u7eb3\u7c73\u6676\u4f53\u7f3a\u9677\u7684\u7efc\u5408\u6291\u5236<\/b><\/strong><\/p>\n

\u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u7eb3\u7c73\u6676\u4f53(PNCs)\u7684\u7535\u81f4\u53d1\u5149\u6548\u7387\u53d7\u5230\u9650\u5236\uff0c\u56e0\u4e3a\u7f3a\u4e4f\u65e2\u80fd\u6291\u5236\u7f3a\u9677\u5f62\u6210\u53c8\u80fd\u589e\u5f3a\u8f7d\u6d41\u5b50\u7ea6\u675f\u7684\u6750\u6599\u7b56\u7565\u3002\u5728\u8fd9\u91cc\uff0c\u97e9\u56fd\u56fd\u7acb\u9996\u5c14\u5927\u5b66Tae-Woo Lee\u8054\u5408\u5bbe\u5915\u6cd5\u5c3c\u4e9a\u5927\u5b66Andrew M. Rappe\u7b49\u4eba\u62a5\u544a\u4e86\u4e00\u79cd\u5355\u63ba\u6742\u7684\u5408\u91d1\u5316\u7b56\u7565\uff0c\u5b83\u53ef\u4ee5\u4ea7\u751f\u66f4\u5c0f\u7684\u3001\u5355\u5206\u6563\u7684\u80f6\u4f53\u7c92\u5b50(\u9650\u5236\u7535\u5b50\u548c\u7a7a\u7a74\uff0c\u5e76\u4fc3\u8fdb\u8f90\u5c04\u590d\u5408)\uff0c\u540c\u65f6\u51cf\u5c11\u8868\u9762\u7f3a\u9677(\u51cf\u5c11\u975e\u8f90\u5c04\u590d\u5408)\u3002\u80cd\u63ba\u6742\u7532\u919b\u8112\u6eb4\u5316\u94c5PNCs\u4ea7\u751f\u6709\u9650\u7684\u4f53\u79ef\u6eb6\u89e3\u5ea6\uff0c\u540c\u65f6\u5728PNCs\u4e2d\u4ea7\u751f\u4e00\u4e2a\u71b5\u7a33\u5b9a\u76f8\uff0c\u5bfc\u81f4\u66f4\u5c0f\u7684PNC\u548c\u66f4\u591a\u7684\u8f7d\u6d41\u5b50\u7ea6\u675f\u3002\u989d\u5916\u7684\u80cd\u5206\u79bb\u5230\u8868\u9762\u5e76\u7a33\u5b9a\u4e86\u4e0d\u534f\u8c03\u4f4d\u70b9\u3002\u6b64\u5916\uff0c\u8fd8\u5e94\u7528\u4e86\u4e00\u79cd\u8868\u9762\u7a33\u5b9a\u76841,3,5-\u4e09(\u6eb4\u4e59\u57fa)-2,4,6-\u4e09\u4e59\u82ef\u4f5c\u4e3a\u6eb4\u5316\u7a7a\u4f4d\u6108\u5408\u5242\u3002\u7ed3\u679c\u8868\u660e\uff0c\u5728\u534a\u7403\u5f62\u900f\u955c\u4e0b\uff0c\u7535\u6d41\u6548\u7387\u4e3a108 cd A\u2212<\/sup>1<\/sup>(\u5916\u91cf\u5b50\u6548\u7387\u4e3a23.4%)\u7684\u9ad8\u6548PNC\u57fa\u53d1\u5149\u4e8c\u6781\u7ba1\uff0c\u5176\u7535\u6d41\u6548\u7387\u4e3a205 cd A\u2212<\/sup>1<\/sup>(\u5916\u91cf\u5b50\u6548\u7387\u4e3a45.5%)\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cComprehensive defect suppression in perovskite nanocrystals for high-efficiency light-emitting diodes\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nature\u00a0Photonics\u4e0a\u3002DOI:\u00a010.1038\/s41566-020-00732-4<\/p>\n

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\u6c27\u5316\u954d(NiOx<\/sub>)\u7a7a\u7a74\u4f20\u8f93\u5c42(HTLs)\u662f\u9499\u949b\u77ff\u5149\u4f0f\u7684\u7406\u60f3\u63a5\u89e6\u70b9\uff0c\u56e0\u4e3a\u5b83\u4eec\u6210\u672c\u4f4e\uff0c\u7a33\u5b9a\uff0c\u6613\u4e8e\u6269\u5c55\uff1b\u7136\u800c\uff0c\u4e0e\u6709\u673a\u9ad8\u6e29\u9ad8\u538b\u76f8\u6bd4\uff0c\u5b83\u4eec\u63d0\u4f9b\u66f4\u4f4e\u7684\u5f00\u8def\u7535\u538b(VOCs)\u3002\u5728\u8fd9\u91cc\uff0c\u79d1\u7f57\u62c9\u591a\u5927\u5b66\u6ce2\u5fb7\u5206\u6821Michael D. McGehee\u3001\u4e9a\u5229\u6851\u90a3\u5927\u5b66Neal R. Armstrong\u7b49\u4eba\u8868\u5f81\u548c\u51cf\u7f13\u4e86\u7535\u5b50\u8f6c\u79fb-\u8d28\u5b50\u8f6c\u79fb\u53cd\u5e94\u4e4b\u95f4\u7684NiOx <\/sub>HTLs\u548c\u9499\u949b\u77ff\u524d\u4f53\u3002\u901a\u8fc7XPS\u548cUPS\u8868\u5f81\uff0c\u53d1\u73b0NiOx<\/sub>\u8584\u819c\u4e2d\u7684Ni\u2265<\/sup>3+<\/sup>\u91d1\u5c5e\u9633\u79bb\u5b50\u4f4d\u540c\u65f6\u4f5c\u4e3aBr\u00f8nsted\u8d28\u5b50\u53d7\u4f53\u548cLewis\u7535\u5b50\u53d7\u4f53\u3002\u53bb\u8d28\u5b50\u5316\u9633\u79bb\u5b50\u80fa\u548c\u6c27\u5316\u7898\u5316\u7269\uff0c\u5728\u9499\u949b\u77ff-NiOx<\/sub>\u754c\u9762\u5f62\u6210\u5bcc\u542bPbI2-x<\/sub>Brx<\/sub>\u7684\u7a7a\u7a74\u8403\u53d6\u5c4f\u969c\u3002\u5728\u9499\u949b\u77ff\u6d3b\u6027\u5c42\u6c89\u79ef\u8fc7\u7a0b\u4e2d\uff0c\u7528\u8fc7\u91cf\u7684A\u4f4d\u9633\u79bb\u5b50\u76d0\u6ef4\u5b9a\u53cd\u5e94\u6027Ni\u2265<\/sup>3+<\/sup>\u8868\u9762\u6001\uff0c\u53ef\u4f7fVOC<\/sub>\u503c\u589e\u52a0\u52301.15 V\uff0c\u529f\u7387\u8f6c\u6362\u6548\u7387\u63d0\u9ad820%\u3002\u8fd9\u53ef\u80fd\u662f\u91d1\u5c5e\u6c27\u5316\u7269\u63a5\u89e6\u7684\u666e\u904d\u53d1\u73b0\uff0c\u4f5c\u4e3aBr\u00f8nsted\u548cLewis\u9178\u78b1\u53cd\u5e94\u7269\u5bf9\u9499\u949b\u77ff\u524d\u4f53\uff0c\u8fd9\u4e5f\u662f\u6700\u8fd1\u7684\u4e00\u9879\u89c2\u5bdfTiO2<\/sub>\u548cSnO2<\/sub>\u63a5\u89e6\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cOvercoming Redox Reactions at Perovskite-Nickel\u00a0Oxide Interfaces to Boost Voltages\u00a0in Perovskite Solar Cells\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Joule\u4e0a\u3002DOI: 10.1016\/j.joule.2020.06.004<\/p>\n

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\u56fe4\u00a0\u9634\u5f71\u533a\u57df\u7535\u6d41-\u7535\u538b\u53c2\u6570\u7684\u663e\u8457\u53d8\u5316<\/p>\n

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AE<\/b><\/strong>n<\/b><\/strong>M<\/b><\/strong>\uff1a<\/b><\/strong>\u03b4-CsPbI<\/b><\/strong>3<\/b><\/sub><\/strong>\/\u03b4-RbPbI<\/b><\/strong>3<\/b><\/sub><\/strong>\u79cd\u5b50\u8f85\u52a9\u5f02\u76f8\u6210\u6838<\/b><\/strong>\u7528\u4e8e<\/b><\/strong>\u9ad8\u6027\u80fd\u591a\u9633\u79bb\u5b50\u5364\u5316\u7269\u7684\u9499\u949b\u77ff\u5149\u4f0f<\/b><\/strong><\/p>\n

\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u6027\u80fd\u4e0e\u5236\u5907\u65b9\u6cd5\u5bc6\u5207\u76f8\u5173\uff1b\u56e0\u6b64\uff0c\u63a7\u5236\u9499\u949b\u77ff\u6676\u4f53\u7684\u751f\u957f\u673a\u5236\u662f\u63d0\u9ad8\u9499\u949b\u77ff\u6676\u4f53\u6548\u7387\u548c\u7a33\u5b9a\u6027\u7684\u6709\u6548\u9014\u5f84\u3002\u5728\u6b64\uff0c\u6d1b\u6851\u8054\u90a6\u7406\u5de5\u5b66\u9662Michael Gr\u00e4tzel\u7b49\u4eba\u901a\u8fc7\u4e24\u6b65\u987a\u5e8f\u6c89\u79ef\u65b9\u6cd5\u8bbe\u8ba1\u4e86\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u591a\u5364\u5316\u7269\u7ec4\u5408\u7269\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u5728PbI2<\/sub>\u524d\u9a71\u4f53\u6eb6\u6db2\u4e2d\u52a0\u5165\u4e00\u7ef4\u591a\u6676\u03b4-RbPbI3<\/sub>\u548c\u03b4-CsPbI3<\/sub>\u7684\u6df7\u5408\u7269\uff0c\u53ef\u8bf1\u5bfc\u5f62\u6210\u591a\u5b54\u4ecb\u5b54\u516d\u65b9\u819c\u3002\u8fd9\u79cd\u5b54\u9699\u7387\u6781\u5927\u5730\u4fc3\u8fdb\u4e86FA(\u7532\u9170\u80fa)\/MA(\u7532\u57fa\u94f5)\u9633\u79bb\u5b50\u5728PbI2<\/sub>\u819c\u4e2d\u7684\u5f02\u76f8\u6210\u6838\u548c\u6e17\u900f\u3002\u56e0\u6b64\uff0c\u968f\u540e\u7684PbI2<\/sub>\u8f6c\u6362\u4e3a\u6240\u9700\u7684\u591a\u7ec4\u7acb\u65b9\u03b1-\u7ed3\u6784\u66b4\u9732\u4e8e\u7532\u9170\u80fa\u7532\u57fa\u5364\u5316\u94f5\u6eb6\u6db2\u4e2d\u5927\u5927\u589e\u5f3a\u3002\u5728\u8f6c\u5316\u8fc7\u7a0b\u4e2d\uff0c\u03b4-CsPbI3<\/sub>\u4e5f\u5b8c\u5168\u96c6\u6210\u5230\u4e09\u7ef4\u6df7\u5408\u9633\u79bb\u5b50\u9499\u949b\u77ff\u6676\u683c\u4e2d\uff0c\u8868\u73b0\u51fa\u9ad8\u7ed3\u6676\u5ea6\u548c\u4f18\u8d8a\u7684\u5149\u7535\u6027\u80fd\u3002\u51a0\u519b\u8bbe\u5907\u663e\u793a\u4e86\u8d85\u8fc722%\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387(PCE)\u3002\u6b64\u5916\uff0c\u8fd9\u4e9b\u5668\u4ef6\u8868\u73b0\u51fa\u66f4\u5f3a\u7684\u8fd0\u884c\u7a33\u5b9a\u6027\uff0c\u57281\u4e2a\u592a\u9633\u5149\u7167\u4e0b\uff0c\u6700\u5927\u529f\u7387\u70b9\u8ddf\u8e2a400 h\uff0c\u6700\u4f73\u5668\u4ef6\u80fd\u4fdd\u6301PCE\u521d\u59cb\u503c\u768490%\u4ee5\u4e0a\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cFormation of High-Performance Multi-Cation Halide\u00a0Perovskites Photovoltaics by \u03b4-CsPbI3\/\u03b4-RbPbI3 Seed-Assisted\u00a0Heterogeneous Nucleation\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728AEnM\u4e0a\u3002DOI: 10.1002\/aenm.202003785<\/p>\n

\u56fe5\u00a0\u4e0d\u540c\u7684\u9499\u949b\u77ff\u8584\u819ca)\u5438\u6536\u5149\u8c31\uff0cb)\u7a33\u6001\u5149\u81f4\u53d1\u5149(PL)\uff0c c)\u65f6\u95f4\u5206\u8fa8\u5149\u81f4\u53d1\u5149(TRPL)<\/p>\n

\"\"<\/p>\n

A<\/b><\/strong>FM<\/b><\/strong>\uff1a\u5b9a\u5411\u5de5\u7a0b\u5c0f\u5206\u5b50\u534a\u5bfc\u4f53\u4f5c\u4e3a\u9ad8\u6548\u7a33\u5b9a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u65e0\u63ba\u6742\u7a7a\u7a74\u4f20\u8f93\u6750\u6599<\/b><\/strong><\/p>\n

\u7ed3\u6676p\u578b\u5c0f\u5206\u5b50\u534a\u5bfc\u4f53\u7531\u4e8e\u5177\u6709\u8f83\u9ad8\u7684\u7a7a\u7a74\u8fc1\u79fb\u7387\u3001\u826f\u597d\u7684\u7a33\u5b9a\u6027\u548c\u53ef\u8c03\u7684\u6700\u9ad8\u5206\u5b50\u8f68\u9053\uff0c\u5728\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60(PSCs)\u4e2d\u4f5c\u4e3a\u9ad8\u6548\u7a33\u5b9a\u7684\u7a7a\u7a74\u4f20\u8f93\u6750\u6599(HTMs)\u5177\u6709\u5f88\u5927\u7684\u6f5c\u529b\u3002\u5728\u8fd9\u91cc\uff0c\u9999\u6e2f\u5927\u5b66Paddy Kwok Leung Chan\u3001Shien-Ping Feng\u8054\u5408\u6d1b\u6851\u8054\u90a6\u7406\u5de5\u5b66\u9662Michael Gr\u00e4tzel\u7b49\u4eba\u5c06\u4e00\u4e2a\u57fa\u4e8e\u786b\u70ef\u7684\u6709\u673a\u534a\u5bfc\u4f53\uff0cDPh-DNTT\uff0c\u88ab\u70ed\u84b8\u53d1\u5e76\u88ab\u7528\u4f5c\u65e0\u63ba\u6742\u7684HTM\uff0c\u53ef\u4ee5\u88ab\u653e\u5927\u7528\u4e8e\u5927\u9762\u79ef\u7684\u5236\u9020\u3002\u901a\u8fc7\u63a7\u5236\u6c89\u79ef\u6e29\u5ea6\uff0c\u5c06\u5206\u5b50\u53d6\u5411\u8c03\u6574\u4e3a\u5782\u76f4\u4e8e\u886c\u5e95\u8868\u9762\u7684\u03c0 -\u03c0\u5806\u79ef\u65b9\u5411\uff0c\u4f7f\u5e73\u9762\u5916\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u6700\u5927\u5316\u3002\u901a\u8fc7\u8bbe\u8ba1\u7684\u9762\u5411\u53d6\u5411\uff0cDPh-DNTT\u8584\u819c\u7684\u9762\u5916\u8fc1\u79fb\u7387\u63d0\u9ad8\u4e863.3 \u00d7 10\u22122<\/sup>\u00a0cm2<\/sup>\u00a0V\u22121<\/sup>\u00a0s\u22121<\/sup>\uff0c\u4f18\u4e8e\u8fc4\u4eca\u4e3a\u6b62\u62a5\u9053\u7684HTMs\u3002\u8fd9\u79cd\u53d6\u5411\u589e\u5f3a\u7684\u8fc1\u79fb\u7387\u4f7fCH3<\/sub>NH3<\/sub>PbI3<\/sub>\u5012\u7f6e\u6548\u7387\u8fbe\u5230\u4e8620.2%\u3002\u672c\u6587\u62a5\u544a\u7684\u7ed3\u679c\u4e3a\u65e0\u63ba\u6742\u6709\u673a\u5206\u5b50\u7684\u5b9a\u5411\u5de5\u7a0b\u63d0\u4f9b\u4e86\u89c1\u89e3\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cOrientation-Engineered Small-Molecule Semiconductors\u00a0as Dopant-Free Hole Transporting Materials for Efficient\u00a0and Stable Perovskite Solar Cells\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728AFM\u4e0a\u3002DOI: 10.1002\/adfm.202011270<\/p>\n

\u56fe6\u00a0a) DNTT\u3001C10-DNTT\u3001DPh-DNTT\u7684\u5206\u5b50\u7ed3\u6784\u3002b)\u57fa\u4e8ep\u578b\u534a\u5bfc\u4f53\u7684OFET\u5668\u4ef6\u539f\u7406\u7ed3\u6784\u3002c)\u5177\u6709\u7535\u5b50\/\u7a7a\u7a74\u4f20\u8f93\u5c42(ETL\/HTL)\u7684\u5e73\u9762\u5012\u7f6ePSC\u5668\u4ef6\u793a\u610f\u56fe\u7ed3\u6784\u3002d-f)\u6709\u673a\u534a\u5bfc\u4f53\u7684\u9762\u5bf9\u3001\u89d2\u5bf9\u548c\u94fe\u5bf9\u65b9\u5411\u793a\u610f\u56fe\u3002<\/p>\n

\"\"<\/p>\n

A<\/b><\/strong>M<\/b><\/strong>\uff1a\u7b2c\u56db\u7cfb\u9499\u949b\u77ff\u4e2d\u7684\u6eb6\u5242\u8f85\u52a9\u52a8\u529b\u5b66\u6355\u83b7<\/b><\/strong><\/p>\n

\u901a\u8fc7\u5408\u91d1\u5316\u5de5\u7a0b\u5364\u5316\u9499\u949b\u77ff\u53ef\u4ee5\u5408\u6210\u5177\u6709\u8c03\u8c10\u7535\u5b50\u548c\u5149\u5b66\u7279\u6027\u7684\u6750\u6599;\u7136\u800c\uff0c\u7531\u4e8e\u6676\u4f53\u7ed3\u6784\u7684\u70ed\u529b\u5b66\u4e0d\u7a33\u5b9a\u800c\u4ea7\u751f\u7684\u5206\u79bb\u76f8\u963b\u788d\u4e86\u8fd9\u4e9b\u5408\u91d1\u7684\u5408\u6210\u3002\u4eba\u4eec\u5df2\u7ecf\u5f00\u53d1\u4e86\u5236\u9020\u8fd9\u79cd\u5408\u91d1\u7684\u65b9\u6cd5\uff0c\u5982\u56fa\u76f8\u53cd\u5e94\u3001\u5316\u5b66\u6c14\u76f8\u6c89\u79ef\u548c\u673a\u68b0\u78e8\u524a;\u4f46\u8fd9\u4e9b\u6750\u6599\u4e0e\u4f4e\u6e29\u6eb6\u6db2\u5904\u7406\u548c\u5355\u7247\u96c6\u6210\u4e0d\u76f8\u5bb9\uff0c\u59a8\u788d\u4e86\u8fd9\u4e9b\u6750\u6599\u7684\u4e00\u4e9b\u91cd\u8981\u5e94\u7528\u3002\u5728\u6b64\uff0c\u52a0\u62ff\u5927\u591a\u4f26\u591a\u5927\u5b66Edward H. Sargent\u7b49\u4eba\u5f00\u53d1\u4e86\u4e00\u79cd\u80fd\u591f\u5408\u6210\u65b0\u578b\u70ed\u529b\u5b66\u4e0d\u5229\u9499\u949b\u77ff\u5408\u91d1\u7684\u65b9\u6cd5—-\u6eb6\u5242\u76f8\u52a8\u529b\u5b66\u6355\u83b7(SPKT)\u3002\u5229\u7528SPKT\u5408\u6210\u4e86Cs1\u2212x<\/sub>Rbx<\/sub>PbCl3<\/sub>\uff0c\u5e76\u9996\u6b21\u62a5\u9053\u4e86\u591a\u6676\u9499\u949b\u77ff\u8584\u819c\u7684\u7d2b\u5916\u5149\u53d1\u5c04\u3002\u4e0e\u76f8\u540c\u524d\u9a71\u4f53\u7684\u975e\u52a8\u529b\u5b66\u6355\u83b7\u6750\u6599\u76f8\u6bd4\uff0cSPKT\u5bfc\u81f4\u6750\u6599\u8868\u73b0\u51fa\u4f18\u8d8a\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u5149\u7a33\u5b9a\u6027\u3002\u52a8\u6001\u6355\u83b7\u6750\u6599\u7684\u77ac\u6001\u5438\u6536\u5149\u8c31\u663e\u793a\u4e86\u6539\u8fdb\u7684\u5149\u5b66\u7279\u6027\uff1a\u66f4\u5927\u7684\u5438\u6536\uff0c\u66f4\u957f\u7684\u57fa\u6001\u6f02\u767d\u5bff\u547d\u3002SPKT\u53ef\u5e94\u7528\u4e8e\u5176\u4ed6\u9499\u949b\u77ff\uff0c\u4ee5\u6539\u5584\u6750\u6599\u6027\u80fd\uff0c\u540c\u65f6\u53d7\u76ca\u4e8e\u6613\u4e8e\u6eb6\u6db2\u5904\u7406\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cSolvent-Assisted Kinetic Trapping in Quaternary Perovskites\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728AM\u4e0a\u3002DOI: 10.1002\/adma.202008690<\/p>\n

\u56fe7\u00a0A)\u6eb6\u5242\u76f8\u52a8\u529b\u5b66\u4fd8\u83b7\u6cd5\u539f\u7406\u56fe\u3002B) Cs1\u2212x<\/sub>Rbx<\/sub>PbCl3<\/sub>\u7b49\u4ef7\u7269\u5728\u5347\u9ad8\u6e29\u5ea6\u65f6\u65cb\u8f6c\u6d82\u8986\u7684Tauc\u56fe\u5438\u6536\u5149\u8c31\u3002C) CRPC\u7684\u7c89\u672bx\u5c04\u7ebf\u884d\u5c04\u56fe(\u6a59\u8272)\u4ee5\u53ca\u76f8\u5e94\u7684CsPbCl3<\/sub>\u5cf0(\u7eff\u8272)\u3002<\/p>\n

\"\"<\/p>\n

Nature<\/b><\/strong>\u00a0Energy<\/b><\/strong>\uff1a<\/b><\/strong>\u9ad8\u6548\u53cc\u9762\u5355\u7247\u9499\u949b\u77ff\/\u7845\u4e32\u8054\u592a\u9633\u80fd\u7535\u6c60\u7684\u5e26\u9699\u5de5\u7a0b<\/b><\/strong><\/p>\n

\u53cc\u9762\u5355\u7247\u9499\u949b\u77ff\/\u7845\u4e32\u8054\u592a\u9633\u80fd\u7535\u6c60\u5229\u7528\u53cd\u5c04\u5149\u2014\u2014\u6765\u81ea\u73af\u5883\u7684\u6f2b\u53cd\u5c04\u5149\u2014\u2014\u63d0\u9ad8\u5176\u6027\u80fd\u9ad8\u4e8e\u5355\u9762\u9499\u949b\u77ff\/\u7845\u4e32\u8054\u592a\u9633\u80fd\u7535\u6c60\u3002\u5728\u8fd9\u91cc\uff0c\u52a0\u62ff\u5927\u591a\u4f26\u591a\u5927\u5b66Edward H. Sargent\u200a\u7b49\u4eba\u62a5\u9053\u4e86\u53cc\u9762\u4e32\u8054\uff0c\u5728\u5355\u9762AM1.5G 1\u592a\u9633\u5149\u7167\u4e0b\uff0c\u7ecf\u8ba4\u8bc1\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387>25%\uff0c\u5728\u5ba4\u5916\u6d4b\u8bd5\u4e2d\u53d1\u7535\u5bc6\u5ea6\u9ad8\u8fbe~26 mW cm-2<\/sup>\u3002\u7814\u7a76\u4e86\u9499\u949b\u77ff\u5e26\u9699\u5728\u5404\u79cd\u73b0\u5b9e\u7167\u660e\u548c\u53cd\u7167\u7387\u6761\u4ef6\u4e0b\u83b7\u5f97\u6700\u4f73\u7535\u6d41\u5339\u914d\u6240\u9700\u7684\u3002\u7136\u540e\uff0c\u6bd4\u8f83\u4e86\u8fd9\u4e9b\u53cc\u9762\u4e32\u8054\u66b4\u9732\u5728\u4e0d\u540c\u53cd\u7167\u7387\u4e0b\u7684\u7279\u6027\uff0c\u5e76\u63d0\u4f9b\u4e86\u4e24\u4e2a\u5730\u70b9\u4e0d\u540c\u73af\u5883\u6761\u4ef6\u4e0b\u7684\u80fd\u6e90\u4ea7\u91cf\u8ba1\u7b97\u3002\u6700\u540e\uff0c\u7ed9\u51fa\u4e86\u5355\u9762\u548c\u53cc\u9762\u9499\u949b\u77ff\/\u7845\u4e32\u8054\u7684\u5ba4\u5916\u6d4b\u8bd5\u573a\u7684\u6bd4\u8f83\uff0c\u4ee5\u8bc1\u660e\u4e32\u8054\u53cc\u9762\u5bf9\u4e8e\u5177\u6709\u5b9e\u9645\u76f8\u5173\u6027\u7684\u4f4d\u7f6e\u7684\u9644\u52a0\u4ef7\u503c\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cEfficient bifacial monolithic perovskite\/silicon\u00a0tandem solar cells via bandgap engineering\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nature\u00a0Energy\u4e0a\u3002DOI: 10.1038\/s41560-020-00756-8<\/p>\n

\u56fe8\u00a0\u9499\u949b\u77ff\/\u7845\u4e32\u8054\u5de5\u4f5c\u7ec4\"\"<\/p>\n

Science:\u57fa\u4e8e\u03b1\u76f8\u7532\u9170\u4e9a\u80fa\u7898\u5316\u94c5\u7684\u9ad8\u6548\u7a33\u5b9a\u592a\u9633\u80fd\u7535\u6c60<\/b><\/strong><\/p>\n

\u79bb\u5b50\u63ba\u6742\u662f\u7a33\u5b9a\u03b1-FAPbI3<\/sub>\u9499\u949b\u77ff\u7684\u91cd\u8981\u65b9\u6cd5\uff0c\u5728\u5f15\u5165\u5176\u4ed6\u79bb\u5b50\u540e\uff0c\u901a\u5e38\u4f1a\u5bf9\u5e26\u9699\u3001\u8f7d\u6d41\u5b50\u52a8\u529b\u5b66\u3001\u7a33\u5b9a\u6027\u4ee5\u53ca\u6676\u683c\u5fae\u5e94\u529b\u4ea7\u751f\u975e\u5e38\u5927\u7684\u5f71\u54cd\uff0c\u751a\u81f3\u5bfc\u81f4\u7f3a\u9677\u4f4d\u70b9\u7684\u4ea7\u751f\u3002\u97e9\u56fd\u851a\u5c71\u56fd\u7acb\u79d1\u6280\u5b66\u9662Sang Il Seok\u7b49\u4eba\u901a\u8fc7\u5728A\u4f4d\u5f15\u5165Cs+<\/sup>\u548cMDA+<\/sup>\u79bb\u5b50\uff0c\u53d1\u73b0\u5728\u63ba\u6742\u4e00\u5b9a\u91cf\u7684\u60c5\u51b5\u4e0b\uff0c\u6676\u683c\u5e94\u529b\u51cf\u5c0f\uff0c\u8f7d\u6d41\u5b50\u5bff\u547d\u5ef6\u957f\uff0c\u4e4c\u5c14\u5df4\u8d6b\u80fd\u548c\u7f3a\u9677\u5bc6\u5ea6\u964d\u4f4e\u3002\u6700\u7ec8\u83b7\u5f97\u4e86\u8ba4\u8bc1\u6548\u7387\u8fbe\u523024.4%\u7684FAPbI3<\/sub>\u57fa\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\uff0c\u672a\u5c01\u88c5\u7684\u7535\u6c60\u5668\u4ef6\u572885\u2103\u7684\u70ed\u7a33\u5b9a\u6d4b\u8bd5\u8fc7\u7a0b\u4e2d\uff08\u907f\u5149\uff09\uff0c\u57281300h\u4e4b\u540e\u4ecd\u80fd\u4fdd\u6301\u521d\u59cb\u6548\u7387\u768480%\u4ee5\u4e0a\u3002\u76f8\u5173\u7814\u7a76\u201cImpact of strain relaxation on performance of\u00a0\u03b1-formamidinium lead iodide perovskite solar cells\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Science\u4e0a\u3002DOI: 10.1126\/science.abc4417<\/p>\n

\u56fe9 \u6c89\u79ef\u9499\u949b\u77ff\u8584\u819c\u7684\u7f3a\u9677\u5206\u6790<\/p>\n

\"\"<\/p>\n

ACS Appl. Mater. Interfaces<\/b><\/strong>\uff1a\u5316\u5b66\u7a33\u5b9a\u7684\u94df\u9521\u6c27\u5316\u7269<\/b><\/strong>\/\u77f3\u58a8\u70ef\u9633\u6781\u9ad8\u6548<\/b><\/strong>\u9499\u949b\u77ff\u53d1\u5149\u4e8c\u6781\u7ba1<\/b><\/strong><\/p>\n

\u77f3\u58a8\u70ef\u5177\u6709\u4f18\u5f02\u7684\u6297\u6e17\u6027\u548c\u5316\u5b66\u9c81\u68d2\u6027\uff0c\u662f\u4e00\u79cd\u7406\u60f3\u7684\u79bb\u5b50\u6269\u6563\u5c4f\u969c\u6750\u6599\u3002\u94df\u9521\u6c27\u5316\u7269(ITO)\u5e38\u7528\u4e8e\u9499\u949b\u77ff\u53d1\u5149\u4e8c\u6781\u7ba1(PeLEDs)\u4e2d\uff0c\u5176\u66b4\u9732\u4e8e\u9178\u6027\u7a7a\u7a74\u6ce8\u5165\u5c42\u65f6\u5bb9\u6613\u91ca\u653e\u51fa\u94df\uff0c\u4ece\u800c\u4f7f\u53d1\u5149\u660e\u663e\u731d\u706d\u3002\u5728\u8fd9\u91cc\uff0c\u97e9\u56fd\u56fd\u7acb\u9996\u5c14\u5927\u5b66Tae-Woo Lee\u7b49\u4eba\u5229\u7528\u77f3\u58a8\u70ef\u4f18\u5f02\u7684\u6e17\u900f\u6027\uff0c\u5e76\u5c06\u5176\u4f5c\u4e3a\u5316\u5b66\u5c4f\u969c\u6765\u963b\u6b62ITO\u66b4\u9732\u5728PeLEDs\u7684\u9178\u6027\u7a7a\u7a74\u6ce8\u5165\u5c42\u4e2d\u53ef\u80fd\u53d1\u751f\u7684\u8680\u523b\u3002\u8fd9\u4e00\u963b\u6321\u5c42\u964d\u4f4e\u4e86\u8fd9\u4e9b\u91d1\u5c5e\u7269\u79cd\u6240\u5f15\u8d77\u7684\u53d1\u5149\u731d\u706d\uff0c\u56e0\u6b64\u5728ITO\u548c\u77f3\u58a8\u70ef\u5c42\u7684\u5668\u4ef6\u4e2d\u9499\u949b\u77ff\u8584\u819c\u7684\u5149\u81f4\u53d1\u5149\u5bff\u547d(87.9 ns)\u660e\u663e\u9ad8\u4e8e\u53ea\u6709ITO\u9633\u6781\u7684\u5668\u4ef6(22.1 ns)\u3002\u6709\u77f3\u58a8\u70ef\u5c4f\u969c\u7684PeLEDs\u7684\u5149\u7535\u6d41\u6548\u7387(16.4 cd\/A)\u4e5f\u9ad8\u4e8e\u6ca1\u6709\u77f3\u58a8\u70ef\u5c4f\u969c\u7684PeLEDs (9.02 cd\/A)\u3002\u7814\u7a76\u8868\u660e\uff0c\u5728\u5149\u7535\u5668\u4ef6\u4e2d\uff0c\u77f3\u58a8\u70ef\u53ef\u4ee5\u4f5c\u4e3a\u4e00\u79cd\u5c4f\u969c\uff0c\u901a\u8fc7\u5316\u5b66\u8680\u523b\u6765\u51cf\u5c11\u900f\u660e\u7535\u6781\u7684\u964d\u89e3\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cChemically Robust Indium Tin Oxide\/Graphene Anode for Efficient\u00a0Perovskite Light-Emitting Diodes\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728ACS Appl. Mater. Interfaces\u4e0a\u3002DOI:\u00a010.1021\/acsami.0c12939<\/p>\n

\u56fe10 \u539f\u59cb\u900f\u660e\u5bfc\u7535\u6c27\u5316\u7269\u53ca\u5e26\u6709\u77f3\u58a8\u70ef\u7684\u900f\u660e\u5bfc\u7535\u6750\u6599\u7684\u7a33\u5b9a\u6027<\/p>\n

\"\"<\/p>\n

\u6587\u4e2d\u6240\u8ff0\u5982\u6709\u4e0d\u59a5\u4e4b\u5904\uff0c\u6b22\u8fce\u8bc4\u8bba\u533a\u7559\u8a00~<\/p>\n

\u672c\u6587\u7531Junas\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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Nature Photonics\uff1a\u9ad8\u6548\u53d1\u5149\u4e8c\u6781\u7ba1\u4e2d\u9499\u949b\u77ff\u7eb3\u7c73\u6676\u4f53\u7f3a\u9677\u7684\u7efc\u5408\u6291\u5236 \u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u7eb3\u7c73\u6676\u4f53(PNCs)\u7684\u7535\u81f4\u53d1\u5149\u6548\u7387\u53d7\u5230\u9650\u5236\uff0c\u56e0\u4e3a\u7f3a\u4e4f\u65e2\u80fd\u6291\u5236\u7f3a\u9677…<\/p>\n","protected":false},"author":11454,"featured_media":223419,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1187],"tags":[],"class_list":["post-223407","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-zhuanlan"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/223407"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=223407"}],"version-history":[{"count":1,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/223407\/revisions"}],"predecessor-version":[{"id":223418,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/223407\/revisions\/223418"}],"wp:featuredmedia":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/media\/223419"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=223407"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=223407"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=223407"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}