{"id":220792,"date":"2021-05-04T06:02:11","date_gmt":"2021-05-03T22:02:11","guid":{"rendered":"\/\/m.iemloyee.com\/?p=220792"},"modified":"2021-05-03T19:02:20","modified_gmt":"2021-05-03T11:02:20","slug":"%e7%be%8e%e5%9b%bd%e8%a5%bf%e5%8c%97%e5%a4%a7%e5%ad%a6j-fraser-stoddart-acc-chem-res-%e6%96%b0%e7%9a%84%e5%a4%a7%e7%8e%af-%e5%88%86%e5%ad%90%e4%b8%89%e8%a7%92%e5%bd%a2","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=220792","title":{"rendered":"\u7f8e\u56fd\u897f\u5317\u5927\u5b66J. Fraser Stoddart Acc. Chem. Res.:\u65b0\u7684\u5927\u73af\u2014\u2014\u5206\u5b50\u4e09\u89d2\u5f62"},"content":{"rendered":"<p>\u3010<strong><b>\u5f15\u8a00<\/b><\/strong>\u3011<\/p>\n<p>\u5927\u73af\u5316\u5408\u7269\u7531\u4e8e\u5176\u4e30\u5bcc\u7684\u5206\u5b50\u8bc6\u522b\u548c\u81ea\u7ec4\u88c5\u7279\u6027\uff0c\u5bf9\u5efa\u7acb\u8d85\u5206\u5b50\u5316\u5b66\u5177\u6709\u6df1\u8fdc\u7684\u5f71\u54cd\u3002\u53ef\u4ee5\u901a\u8fc7\u5408\u6210\u5b9a\u5236\u4ee5\u663e\u793a\u65b0\u5947\u7279\u5f02\u6027\u8d28\u7684\u65b0\u5927\u73af\u53d7\u4f53\u7684\u8bbe\u8ba1\uff0c\u5bf9\u4e8e\u5316\u5b66\u5bb6\u548c\u6750\u6599\u79d1\u5b66\u5bb6\u800c\u8a00\u662f\u91cd\u8981\u7684\u7814\u7a76\u76ee\u6807\u3002\u4e0e\u67d4\u97e7\u7684\u5927\u73af\u76f8\u6bd4\uff0c\u5177\u6709\u03c0\u5171\u8f6d\u82b3\u65cf\u5355\u5143\u7684\u521a\u6027\u5927\u73af\u9664\u4e86\u5177\u6709\u6301\u4e45\u7684\u5f62\u72b6\u5916\uff0c\u8fd8\u503e\u5411\u4e8e\u5177\u6709\u8f83\u5927\u7684\u5185\u90e8\u548c\u5916\u90e8\u03c0\u8868\u9762\u3002\u8fd9\u4e9b\u529f\u80fd\u4e0d\u4ec5\u4f7f\u8fd9\u4e9b\u5927\u73af\u5177\u6709\u5e7f\u6cdb\u7684\u5bbf\u4e3b\u5ba2\u4f53\u7279\u6027\uff0c\u800c\u4e14\u4f7f\u5b83\u4eec\u6210\u4e3a\u6784\u5efa\u5404\u79cd\u8d85\u5206\u5b50\u4f53\u7cfb\u7ed3\u6784\u7684\u7406\u60f3\u6784\u5efa\u57fa\u5757\u3002\u5c06\u03c0-\u5171\u8f6d\u5355\u5143\u7ed3\u5408\u5230\u5927\u73af\u4e2d\u8fd8\u4f7f\u5176\u5177\u6709\u4e30\u5bcc\u7684\u5149\u5b66\uff0c\u7535\u5b50\u548c\u78c1\u6027\u6027\u8d28\uff0c\u4ece\u800c\u4f7f\u5176\u5728\u6750\u6599\u79d1\u5b66\u548c\u5206\u5b50\u7eb3\u7c73\u6280\u672f\u4e2d\u5f97\u5230\u5e7f\u6cdb\u5e94\u7528\u3002\u6700\u8fd1\uff0c\u4f5c\u8005\u8bbe\u8ba1\u5e76\u5408\u6210\u4e86\u4e00\u7c7b\u65b0\u7684\u5927\u73af\uff0c\u5373\u5206\u5b50\u4e09\u89d2\u5f62\uff0c\u5b83\u5177\u6709\u5177\u6709\u4e09\u89d2\u5f62\u51e0\u4f55\u5f62\u72b6\u7684\u521a\u6027\u7ed3\u6784\u3002\u5b83\u4eec\u7531\u4e09\u4e2a\u624b\u6027\u53cd\u5f0f1,2-\u73af\u5df1\u916e\u9876\u70b9\u548c\u4e09\u4e2a\u82b3\u65cf\u56db\u7fa7\u9178\u4e8c\u9170\u4e9a\u80fa\u8fde\u63a5\u57fa\u7ec4\u6210\uff0c\u4f8b\u5982\u5747\u82ef\u56db\u7532\u9178\u4e8c\u9170\u4e9a\u80fa\uff0c\u8418\u4e8c\u9170\u4e9a\u80fa\u7b49\u3002\u4ece\u5bb9\u6613\u83b7\u5f97\u7684\u5408\u6210\u65b9\u6848\u4e2d\u53d7\u76ca\uff0c\u8fd9\u4e9b\u521a\u6027\u5206\u5b50\u4e09\u89d2\u5f62\u7684\u51e0\u4f55\u5f62\u72b6\u548c\u6027\u8d28\u53ef\u4ee5\u4efb\u610f\u6539\u53d8\u3002\u901a\u8fc7\u7ed3\u5408\u8fd9\u4e9b\u56db\u7fa7\u9178\u4e8c\u9170\u4e9a\u80fa\u8fde\u63a5\u4f53\uff0c\u4f5c\u8005\u5df2\u7ecf\u80fd\u591f\u5408\u6210\u5206\u5b50\u7b49\u8fb9\u4e09\u89d2\u5f62\u548c\u7b49\u8170\u4e09\u89d2\u5f62\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5e74\u4e2d\uff0c\u4f5c\u8005\u5bf9\u8fd9\u4e9b\u5206\u5b50\u4e09\u89d2\u5f62\u7684\u7ed3\u6784\u7279\u5f81\u548c\u81ea\u7ec4\u88c5\u7279\u5f81\u8fdb\u884c\u4e86\u7cfb\u7edf\u7684\u7814\u7a76\u3002\u5173\u4e8e\u8fd9\u4e9b\u5206\u5b50\u4e09\u89d2\u5f62\uff0c\u4ee5\u4e0b\u51e0\u70b9\u503c\u5f97\u6ce8\u610f\uff1a\uff08i\uff09\u5b83\u4eec\u5177\u6709\u5f62\u72b6\u6301\u4e45\u7684\u5185\u8154\uff0c\u5177\u6709\u9ad8\u5ea6\u7535\u5b50\u7f3a\u9677\u7684\u6027\u8d28\u3002\u8fd9\u4e9b\u7279\u5f81\u4f7f\u5b83\u4eec\u5177\u6709\u4e0e\u9634\u79bb\u5b50\u548c\u5bcc\u7535\u5b50\u5206\u5b50\u7edc\u5408\u7684\u80fd\u529b\uff0c\u5f62\u6210\u8d85\u5206\u5b50\u7eb3\u7c73\u7ba1\u548c\u4e8c\u7ef4\u5e73\u94fa\u3002\uff08ii\uff09\u5177\u6709\u56fa\u6709\u624b\u6027\u7684\u5206\u5b50\u80fd\u591f\u81ea\u7ec4\u88c5\u6210\u56fa\u6001\u975e\u87ba\u65cb\u6216\u5355\u624b\u87ba\u65cb\u8d85\u7ed3\u6784\uff0c\u4ece\u800c\u5f15\u8d77\u4ece\u5927\u73af\u5316\u5408\u7269\u5230\u5176\u6676\u4f53\u8d85\u5206\u5b50\u7ec4\u88c5\u4f53\u7684\u9009\u62e9\u6027\u624b\u6027\u8f6c\u79fb\u3002\uff08iii\uff09\u82b3\u65cf\u56db\u7fa7\u9178\u4e8c\u9170\u4e9a\u80fa\u8fde\u63a5\u4f53\u7684\u4e09\u89d2\u5f62\u6392\u5217\u6709\u52a9\u4e8e\u6574\u4e2a\u7a7a\u95f4\u5927\u73af\u7a7a\u95f4\u7535\u5b50\u7684\u79bb\u57df\u5316\uff0c\u4ece\u800c\u8d4b\u4e88\u5f02\u4e4e\u5bfb\u5e38\u7684\u7535\u5b50\u548c\u81ea\u65cb\u7279\u6027\u3002\u8fc4\u4eca\u4e3a\u6b62\uff0c\u5206\u5b50\u4e09\u89d2\u5f62\u5bb6\u65cf\u5df2\u5c55\u73b0\u51fa\u4e00\u7cfb\u5217\u7684\u7406\u5316\u7279\u6027\uff0c\u4f8b\u5982\u9634\u79bb\u5b50\u8bc6\u522b\uff0c\u624b\u6027\u7ec4\u88c5\uff0c\u8d85\u5206\u5b50\u51dd\u80f6\u5316\uff0c\u80fd\u91cf\u5b58\u50a8\uff0c\u56fa\u6001\u53d1\u5149\u548c\u975e\u7ebf\u6027\u5149\u5b66\u54cd\u5e94\u3002<\/p>\n<p>\u3010<strong><b>\u6210\u679c\u7b80\u4ecb<\/b><\/strong>\u3011<\/p>\n<p><strong><b>\u00a0<\/b><\/strong><strong><b>\u00a0\u00a0\u00a0\u00a0\u00a0<\/b><\/strong><strong><b>\u00a0\u00a0<\/b><\/strong>\u00a0<strong><b>\u7f8e\u56fd\u897f\u5317\u5927\u5b66J. Fraser Stoddart<\/b><\/strong>\u603b\u7ed3\u4e86\u6700\u8fd1\u5bf9\u8fd9\u4e9b\u5206\u5b50\u4e09\u89d2\u5f62\u7684\u7814\u7a76\u8fdb\u5c55\u3002\u4f5c\u8005\u5bf9\u5b83\u4eec\u7684\u8bbe\u8ba1\u548c\u7efc\u5408\u8fdb\u884c\u4e86\u6982\u8ff0\uff0c\u5e76\u5bf9\u5176\u7ed3\u6784\u7279\u5f81\u8fdb\u884c\u4e86\u603b\u4f53\u603b\u7ed3\u3002\u4f5c\u8005\u63a5\u7740\u8ba8\u8bba\u6709\u5173\u5176\u5206\u5b50\u8bc6\u522b\u7279\u6027\u548c\u7ec4\u88c5\u7279\u6027\u7684\u6700\u65b0\u53d1\u5c55\u3002\u6b64\u5916\uff0c\u4f5c\u8005\u91cd\u70b9\u4ecb\u7ecd\u4e86\u8fd9\u4e9b\u5206\u5b50\u4e09\u89d2\u5f62\u53ca\u5176\u4e0e\u4e00\u7cfb\u5217\u6eb6\u5242\u548c\u5bcc\u7535\u5b50\u5206\u5b50\u7684\u914d\u5408\u7269\u7684\u6f5c\u5728\u5e94\u7528\u3002\u6700\u540e\uff0c\u4f5c\u8005\u63a8\u6d4b\u57fa\u4e8e\u6b64\u7c7b\u5206\u5b50\u4e09\u89d2\u5f62\u7684\u8fdb\u4e00\u6b65\u7ed3\u6784\u4fee\u9970\u548c\u9762\u5411\u5e94\u7528\u7684\u63a2\u7d22\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a<strong>\u201c<\/strong><strong>Molecular Triangles: A New Class of Macrocycles<\/strong><strong>\u201d<\/strong>\u53d1\u8868\u5728<strong><b>Acc. Chem. Res.<\/b><\/strong><strong>\u4e0a<\/strong>\u3002<\/p>\n<p><strong><b>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n<p><strong><b>Fig<\/b><\/strong><strong>u<\/strong><strong><b>re 1.\u5404\u7c7b\u4e09\u89d2\u5206\u5b50\u7684\u7ed3\u6784\u5f0f<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220793\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r1-4.jpg\" alt=\"\" width=\"600\" height=\"848\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r1-4.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r1-4-212x300.jpg 212w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 2.\u7269\u7406\u6027\u8d28\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220794\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r2-4.jpg\" alt=\"\" width=\"600\" height=\"365\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r2-4.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r2-4-300x183.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09\u5355\u6676X\u5c04\u7ebf\u7ed3\u6784\uff08b\uff09DFT\u8ba1\u7b97\u7684\u6700\u4f4e\u672a\u5360\u7528\u5206\u5b50\u8f68\u9053\uff08LUMO\uff09\uff08c\uff09CD\u5149\u8c31 \uff08d\uff09CV\u00a0\uff08e-f\uff09EPR\u548cENDOR\u5149\u8c31<\/p>\n<p><strong><b>Figure 3.\u7ed3\u6784\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220795\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r3-4.jpg\" alt=\"\" width=\"600\" height=\"430\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r3-4.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r3-4-300x215.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 4.\u5355\u6676\u8d85\u7ed3\u6784<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220796\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r4-3.jpg\" alt=\"\" width=\"600\" height=\"708\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r4-3.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r4-3-254x300.jpg 254w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 5.\u56fa\u6001\u8d85\u7ed3\u6784<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220797\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r5-3.jpg\" alt=\"\" width=\"600\" height=\"248\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r5-3.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r5-3-300x124.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 6.\u57fa\u4e8ePMDI\u7684\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\u5316\u5408\u7269\u7684\u6052\u7535\u6d41\u6d4b\u91cf<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220798\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r6-1.jpg\" alt=\"\" width=\"600\" height=\"305\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r6-1.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r6-1-300x153.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 7.\u53d1\u5149\u6027\u80fd<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220799\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r7-1.jpg\" alt=\"\" width=\"600\" height=\"458\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r7-1.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r7-1-300x229.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 8.\u5355\u6676\u8d85\u7ed3\u6784\u548c\u53cc\u5149\u5b50\u6210\u50cf<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220800\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r8-1.jpg\" alt=\"\" width=\"600\" height=\"317\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r8-1.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r8-1-300x159.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Figure 9.\u8d85\u5206\u5b50\u51dd\u80f6\u7684\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-220801\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r9-1.jpg\" alt=\"\" width=\"600\" height=\"402\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r9-1.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/04\/r9-1-300x201.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>\u3010<\/b><\/strong><strong><b>\u5c0f\u7ed3<\/b><\/strong><strong><b>\u3011<\/b><\/strong><\/p>\n<p>\u4f5c\u4e3a\u65b0\u5174\u7684\u5927\u73af\u5316\u5408\u7269\uff0c\u5206\u5b50\u4e09\u89d2\u5f62\u7531\u4e8e\u5176\u72ec\u7279\u7684\u7279\u5f81\uff08\u5305\u62ec\u7ed3\u6784\u521a\u5ea6\uff0c\u7535\u5b50\u4e0d\u8db3\uff0c\u7a7a\u95f4\u7535\u5b50\u901a\u4fe1\u548c\u56fa\u6709\u624b\u5f81\u6027\uff09\u800c\u5438\u5f15\u4e86\u8d8a\u6765\u8d8a\u591a\u7684\u5173\u6ce8\u3002\u5728\u8fc7\u53bb\u7684\u516b\u5e74\u4e2d\uff0c\u5bf9\u5176\u6027\u80fd\u7684\u7814\u7a76\u6d89\u53ca\u591a\u4e2a\u65b9\u9762\uff0c\u4f8b\u5982\u9634\u79bb\u5b50\u8bc6\u522b\uff0c\u624b\u6027\u7ec4\u88c5\uff0c\u8d85\u5206\u5b50\u51dd\u80f6\u5316\uff0c\u80fd\u91cf\u5b58\u50a8\uff0c\u56fa\u6001\u53d1\u5149\u548c\u975e\u7ebf\u6027\u5149\u5b66\u54cd\u5e94\u3002 \u5728\u8fd9\u4e2a\u7efc\u8ff0\u4e2d\uff0c\u4f5c\u8005\u603b\u7ed3\u4e86\u8fd9\u4e9b\u5206\u5b50\u4e09\u89d2\u5f62\u5316\u5b66\u7684\u6700\u65b0\u8fdb\u5c55\uff0c\u5305\u62ec\u5b83\u4eec\u7684\u5206\u5b50\u8bbe\u8ba1\uff0c\u5408\u6210\uff0c\u7ec4\u88c5\uff0c\u6027\u8d28\u548c\u5e94\u7528\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5<\/b><\/strong>\uff1aMolecular Triangles: A New Class of Macrocycles, <strong><b>Acc. Chem. 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