{"id":218668,"date":"2021-03-07T06:30:35","date_gmt":"2021-03-06T22:30:35","guid":{"rendered":"\/\/m.iemloyee.com\/?p=218668"},"modified":"2021-03-07T11:32:34","modified_gmt":"2021-03-07T03:32:34","slug":"%ef%bc%88%e5%b7%b2%e6%a0%a1%e7%a8%bf%e4%bb%b6%ef%bc%89%e6%b5%99%e5%a4%a7%e9%ab%98%e8%b6%85%e3%80%81%e5%be%90%e5%bf%97%e5%ba%b7-%e9%a9%ac%e9%87%8c%e5%85%b0%e5%a4%a7%e5%ad%a6%e7%8e%8b%e6%98%a5%e7%94%9f","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=218668","title":{"rendered":"\u6d59\u5927\u9ad8\u8d85\u3001\u5f90\u5fd7\u5eb7\/\u9a6c\u91cc\u5170\u5927\u5b66\u738b\u6625\u751f Adv. Mater.\uff1a\u7a81\u7834\u6781\u9650\uff01\u8d85\u6d53\u6c34\u7cfb\u7535\u89e3\u8d28\u52a9\u529b\u9ad8\u6027\u80fd\u6c34\u7cfb\u7535\u6c60"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u4f17\u6240\u5468\u77e5\uff0c\u6c34\u7cfb\u7535\u89e3\u8d28\u7684\u4f7f\u7528\u6709\u6548\u7f13\u89e3\u4e86\u7535\u6c60\u7684\u5b89\u5168\u6027\u3001\u6210\u672c\u548c\u73af\u5883\u5f71\u54cd\u7684\u95ee\u9898\u3002\u4f46\u662f\uff0c\u5f53\u524d\u6c34\u7cfb\u7535\u89e3\u8d28\u7684\u53d1\u5c55\u4e3b\u8981\u53d7\u9650\u4e8e\u5176\u72ed\u7a84\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u7a97\u53e3\uff08\u7ea61.23 V\uff09\u548c\u7f3a\u5c11\u53ef\u4e0e\u8be5\u7a97\u53e3\u76f8\u517c\u5bb9\u7684\u9ad8\u6bd4\u5bb9\u91cf\u7535\u5316\u5b66\u53cd\u5e94\u7c7b\u578b\u3002\u89e3\u51b3\u6b64\u95ee\u9898\u7684\u6709\u6548\u65b9\u6cd5\u662f\u8c03\u89e3\u7535\u89e3\u8d28\u79bb\u5b50\u4e0e\u6c34\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\uff0c\u5bf9\u7535\u89e3\u8d28\u7684\u7c98\u5ea6\u3001\u6eb6\u89e3\u5ea6\u3001\u5316\u5b66\u53cd\u5e94\u6027\u548c\u7a33\u5b9a\u6027\u7b49\u53c2\u6570\u5177\u6709\u91cd\u5927\u5f71\u54cd\u3002\u5bf9\u6bd4\u4f20\u7edf\u7684\u6c34\u7cfb\u7535\u89e3\u8d28\uff08\u7ea61 mol L-1<\/sup>\uff09\uff0c\u4ee520-30 mol kg-1<\/sup>\uff08m\uff09\u7684\u76d0\u6d53\u5ea6\u4e3a\u7279\u5f81\u201c\u76d0\u5305\u6c34\u201d\u578b\u7535\u89e3\u8d28\u53ef\u4ee5\u6709\u6548\u62d3\u5bbd\u7535\u5316\u5b66\u7a33\u5b9a\u7a97\u53e3\u81f33.0 V\uff0c\u6781\u5927\u5730\u63d0\u5347\u4e86\u6c34\u7cfb\u7535\u5316\u5b66\u50a8\u80fd\u5668\u4ef6\u7684\u80fd\u91cf\u5bc6\u5ea6\u3002\u540c\u65f6\uff0c\u53ef\u4ee5\u6eb6\u89e3\u5177\u6709\u76f8\u4f3c\u5316\u5b66\u6027\u8d28\u7684\u53e6\u4e00\u79cd\u76d0\u800c\u5f62\u6210\u4f4e\u5171\u7194\u878d\u4f53\u7cfb\uff0c\u56e0\u6b64\u83b7\u5f97\u5177\u6709\u66f4\u9ad8\u76d0\u6d53\u5ea6\u4ee5\u53ca\u66f4\u5bbd\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u7a97\u53e3\u7684\uff08\u53cc\uff09\u76d0\u5305\u6c34\/\u6c34\u5408\u5171\u7194\u76d0\u7535\u89e3\u8d28\uff0c\u8fdb\u800c\u4f7f\u6c34\u7cfb\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6\u66f4\u63a5\u8fd1\u4e8e\u5176\u975e\u6c34\u5bf9\u5e94\u7269\u3002\u7136\u800c\uff0c\u968f\u7740\uff08\u53cc\uff09\u76d0\u5305\u6c34\u7535\u89e3\u8d28\u4e2d\u7684\u6c34\u8fbe\u5230\u5176\u7269\u7406\u6eb6\u89e3\u5ea6\u6781\u9650\uff0c\u8fdb\u4e00\u6b65\u589e\u52a0\u6c34\u4e2d\u7535\u89e3\u8d28\u7684\u542b\u91cf\u9762\u4e34\u5de8\u5927\u7684\u6311\u6218\u3002\u6b64\u5916\uff0c\u5f88\u5c11\u62a5\u9053\u4f7f\u7528\u6d53\u7f29\u7684\u7535\u89e3\u8d28\u6765\u589e\u52a0\u6c34\u7cfb\u80fd\u91cf\u5b58\u50a8\u88c5\u7f6e\u7684\u6bd4\u5bb9\u91cf\uff0c\u7279\u522b\u662f\u57fa\u4e8e\u975e\u9502\uff08Li\uff09\u5143\u7d20\u7684\u6c34\u7cfb\u80fd\u91cf\u5b58\u50a8\u88c5\u7f6e\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6d59\u6c5f\u5927\u5b66\u9ad8\u8d85\u6559\u6388\u548c\u5f90\u5fd7\u5eb7\u6559\u6388\u4ee5\u53ca\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u738b\u6625\u751f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u8054\u5408\u62a5\u9053\u4e86\u4e00\u79cd\u7531ZnCl2<\/sub>\/ZnBr2<\/sub>\/Zn(OAc)2<\/sub>\u7ec4\u6210\u7684\u6c34\u7cfb\u7535\u89e3\u8d28\uff0c\u5176\u6eb6\u89e3\u5ea6\u9ad8\u8fbe75 mol kg-1<\/sup>\uff08m\uff09\uff0c\u7a81\u7834\u4e86\u7269\u7406\u6eb6\u89e3\u5ea6\u6781\u9650\u3002\u5176\u539f\u56e0\u662fBr–<\/sup>\/Cl–<\/sup>-H\u548cBr–<\/sup>\/Cl–<\/sup>\/O-Zn2+<\/sup>\u76f8\u4e92\u4f5c\u7528\uff0c\u6865\u8054\u5f62\u6210\u4e86\u918b\u9178\u76d0\u5c01\u7aef\u7684\u6c34-\u76d0\u4f4e\u805a\u7269\u3002\u901a\u8fc7\u8d28\u8c31\u5206\u6790\u8868\u660e\uff0c\u542b\u6709\u975e\u6781\u6027\u8d28\u5b50\u7684\u918b\u9178\u76d0\u9634\u79bb\u5b50\u963b\u6b62\u4e86\u79bb\u5b50\u4f4e\u805a\u7269\u7684\u8fc7\u5ea6\u751f\u957f\u548c\u6c89\u6dc0\u3002\u8fd9\u79cd\u65e0\u673a\u7535\u89e3\u8d28\u7684\u7c7b\u805a\u5408\u7269\u73bb\u7483\u5316\u8f6c\u53d8\u6e29\u5ea6\u7ea6\u4e3a-70\u81f3-60 \u2103\uff0c\u5728\u6e29\u5ea6\u4ece40\u81f3-80\u2103\u53d8\u5316\u8303\u56f4\u5185\u6ca1\u6709\u89c2\u5bdf\u5230\u76d0\u7ed3\u6676\u548c\u6c34\u51bb\u7ed3\u5cf0\u3002\u8fd9\u79cd\u8d85\u6d53\u548c\u53ef\u6eb6\u6027\u7535\u89e3\u8d28\u4f7f\u9ad8\u6027\u80fd\u6c34\u7cfb\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u53ef\u9006\u5bb9\u91cf\u8fbe\u5230\u4e86605.7 mAh g-1<\/sup>\uff0c\u76f8\u5f53\u4e8e\u80fd\u91cf\u5bc6\u5ea6\u4e3a908.5 Wh kg-1<\/sup>\uff0c\u540c\u65f6\u5176\u5e93\u4ed1\u6548\u7387\u4e3a98.07%\u3001\u622a\u6b62\u7535\u538b\u4e3a1.85 V\u548c\u4f7f\u7528\u5bff\u547d\u5728500\u6b21\u4ee5\u4e0a\u3002\u6b64\u5916\uff0c\u901a\u8fc7\u539f\u4f4dX\u5c04\u7ebf\u884d\u5c04\u548c\u62c9\u66fc\u5149\u8c31\u6280\u672f\u8868\u660e\uff0c\u8fd9\u79cd\u9ad8\u79bb\u5b50\u6d53\u5ea6\u7684\u8d85\u53ef\u6eb6\u6027\u7535\u89e3\u8d28\u4f7f\u5f97\u6eb4\u80fd\u591f\u57281\u9636\u6bb5\u63d2\u5165\u5b8f\u89c2\u7ec4\u88c5\u7684\u77f3\u58a8\u70ef\u6b63\u6781\u4e2d\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cWater-Salt Oligomers Enable Supersoluble Electrolytes for High-Performance Aqueous Batteries\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aAdv. Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a\u9ad8\u8d85\u6559\u6388\u56e2\u961f\u7684\u535a\u58eb\u751f\u8521\u76db\u8d62\u3001\u672c\u79d1\u751f\u891a\u661f\u8fdc\u4e3a\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u3002<\/strong><\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u7535\u89e3\u8d28\u7ed3\u6784\u8868\u5f81<\/strong>
\n \"\"a\uff09\u7531\u5316\u5b66\u8ba1\u91cf\u6bd4\u7684ZnCl2<\/sub>\u3001ZnBr2<\/sub>\u3001Zn(OAc)2<\/sub>\u548c\u6c34\u5236\u5907\u7684WSOE45<\/sub>-1\uff1b<\/p>\n

b\uff09\u7531\u5316\u5b66\u8ba1\u91cf\u6bd4\u7684ZnCl2<\/sub>\u3001ZnBr2<\/sub>\u548c\u6c34\u5236\u590740 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u60ac\u6d6e\u6db2\uff1b<\/p>\n

c\uff09\u753120 m ZnCl2<\/sub>\u300120 m ZnBr2<\/sub>\u548c20 m Zn(OAc)2<\/sub>\u7ec4\u6210\u7684WSOE40<\/sub>-20\uff1b<\/p>\n

d\uff09\u753125 m ZnCl2<\/sub>\u300125 m ZnBr2<\/sub>\u548c25 m Zn(OAc)2<\/sub>\u7ec4\u6210WSOE50<\/sub>-25\uff1b<\/p>\n

e\uff09\u7535\u89e3\u8d28\u4e2dZn\u884d\u751f\u7269\u7684\u62c9\u66fc\u5149\u8c31\uff1b<\/p>\n

f\uff09Zn(H2<\/sub>O)6<\/sub>2+<\/sup>\u548c1-46 m\u7535\u89e3\u8d28\u4e2d\u805a\u5408\u7269\u79cd\u7c7b\u542b\u91cf\u7684\u53d8\u5316\u8d8b\u52bf\uff1b<\/p>\n

g\uff091 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u6c34\u6eb6\u6db2\uff08\u66f2\u7ebf1\uff09\u300140 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u60ac\u6d6e\u6db2\uff08\u4e0a\u6e05\u6db2\uff0c\u66f2\u7ebf2\uff09\u3001WSOE45<\/sub>-1\uff08\u66f2\u7ebf3\uff09\u3001WSOE45<\/sub>-2\uff08\u66f2\u7ebf4\uff09\u548cWSOE45<\/sub>-10\uff08\u66f2\u7ebf5\uff09\u7684\u8d28\u8c31\u56fe\uff1b<\/p>\n

h\uff09WSOE45<\/sub>-1\uff08\u66f2\u7ebf1\uff09\u3001WSOE45<\/sub>-2\uff08\u66f2\u7ebf2\uff09\u3001WSOE45<\/sub>-4\uff08\u66f2\u7ebf3\uff09\u3001WSOE45<\/sub>-6\uff08\u66f2\u7ebf4\uff09\u3001WSOE45<\/sub>-8\uff08\u66f2\u7ebf5\uff09\u3001WSOE45<\/sub>-10\uff08\u66f2\u7ebf6\uff09WSOE45<\/sub>-15\uff08\u66f2\u7ebf7\uff09\uff0cWSOE45<\/sub>-20\uff08\u66f2\u7ebf8\uff09\u548cWSOE45<\/sub>-30\uff08\u66f2\u7ebf9\uff09\u7684DSC\u7ed3\u679c\uff1b<\/p>\n

i-j\uff09\u7535\u89e3\u8d28\u4e2d\u6c34\u5206\u5b50\u7684\u62c9\u66fc\u5149\u8c31\u548cFTIR\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e8c\u3001\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df<\/strong>
\n \"\"a-b\uff09WSOE45<\/sub>-1\u548c5 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u6c34\u6eb6\u6db2\u7684MD\u6a21\u62df\u622a\u56fe\uff1b<\/p>\n

c-d\uff09\u4ece\u6a21\u5f0fa\u548cb\u4e2d\u63d0\u53d6\u7684\u5178\u578b\u5206\u5b50\u6784\u8c61\uff1b<\/p>\n

e-g\uff095 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u6c34\u7cfb\u7535\u89e3\u8d28\u548cWSOE45<\/sub>-1\u4e2dH\u539f\u5b50\u7684\u5f84\u5411\u5206\u5e03\u51fd\u6570\u548c\u79ef\u5206\u66f2\u7ebf\uff1b<\/p>\n

h-j\uff095 m ZnBr0.5<\/sub>Cl1.5<\/sub>\u6c34\u7cfb\u7535\u89e3\u8d28\u548cWSOE45<\/sub>-1\u4e2dZn\u539f\u5b50\u7684\u5f84\u5411\u5206\u5e03\u51fd\u6570\u548c\u79ef\u5206\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e09\u3001\u57fa\u4e8eWSOE45<\/sub>-1\u7684\u9ad8\u6bd4\u5bb9\u91cf\u6c34\u7cfb\u53cc\u79bb\u5b50\u7535\u6c60<\/strong>
\n \"\"a\uff09\u7531WSOE45<\/sub>-1\u3001PGA\u6b63\u6781\u548cZn\/GFF\u8d1f\u6781\u6784\u6210\u7684\u53cc\u79bb\u5b50\u7535\u6c60\u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n

b\uff09\u4f7f\u7528WSOE45<\/sub>-1\u4f5c\u4e3a\u7535\u89e3\u8d28\u7684\u8d1f\u6781\u3001\u6b63\u6781\u3001\u96c6\u7535\u5668\u548c\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u5faa\u73af\u4f0f\u5b89\u66f2\u7ebf\uff1b<\/p>\n

c-d\uff09\u5728\u4e0d\u540c\u622a\u6b62\u7535\u538b\u4e0b\uff0cZn\/GFF|WSOE45<\/sub>-1|PGA\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u5145\/\u653e\u7535\u6bd4\u5bb9\u91cf\uff1b<\/p>\n

e-f\uff09\u4f7f\u75285-46 m\u7535\u89e3\u8d28\u7ec4\u88c5\u7684\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u653e\u7535\u6bd4\u5bb9\u91cf\uff1b<\/p>\n

g\uff09\u4f7f\u75285-46 m\u7535\u89e3\u8d28\u7ec4\u88c5\u7684\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u5e93\u4ed1\u6548\u7387\u3002<\/p>\n

\u56fe\u56db\u3001\u53cc\u79bb\u5b50\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong>
\n \"\"a\uff09\u53cc\u79bb\u5b50\u7535\u6c60\u5728\u4e0d\u540c\u500d\u7387\u4e0b\u7684\u6052\u7535\u6d41\u5145\/\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

b\uff09\u53cc\u79bb\u5b50\u7535\u6c60\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a1 A g-1<\/sup>\u4e0b\u7684\u5faa\u73af\u7a33\u5b9a\u6027\uff1b<\/p>\n

c\uff09\u901a\u8fc7\u4e09\u7535\u6781\u8bbe\u7f6e\u83b7\u5f97\u7684WSOE45<\/sub>-1\u4e2d\u5404\u79cdSOCs\u4e0bPGA\u6b63\u6781\u7684Nyquist\u56fe\uff1b<\/p>\n

d\uff09\u5bf9\u6bd4\u4f7f\u7528\u975e\u6c34\u548c\u6c34\u7cfb\u7535\u89e3\u8d28\u7684\u5404\u79cd\u5148\u8fdb\u6b63\u6781\uff0c\u63d2\u6709Br\u7684PGA\u6b63\u6781\u7684\u80fd\u91cf\u5bc6\u5ea6\uff1b<\/p>\n

e\uff09\u5d4c\u5165Br\u7684PGA\u6b63\u6781\u4e0e\u5404\u79cd\u975e\u6c34\u548c\u6c34\u6b63\u6781\u7684Ragone\u56fe\u3002<\/p>\n

\u56fe\u4e94\u3001\u80fd\u91cf\u5b58\u50a8\u673a\u7406<\/strong>
\n \"\"a-b\uff09\u5728\u5145\/\u653e\u7535\u5faa\u73af\u4e2d\uff0c\u539f\u4f4d\u5d4c\u5165Br\u7684PGA\u6b63\u6781\u7684\u62c9\u66fc\u5149\u8c31\uff1b<\/p>\n

c\uff09\u5728\u5145\u7535\u524d\uff0c\u539f\u59cbPGA\u6b63\u6781\u7684\u62c9\u66fc\u5149\u8c31\u56fe\u548c\u76f8\u5e94\u7684\u5cf0\uff1b<\/p>\n

d\uff09\u5728\u5145\u7535\u671f\u95f4\uff0c2\u9636\u6bb5Br-\u5d4c\u5165PGA\u6b63\u6781\u7684\u62c9\u66fc\u5149\u8c31\u56fe\u548c\u76f8\u5e94\u7684\u5cf0\uff1b<\/p>\n

e\uff09\u5728\u5145\u7535\u540e\uff0c1\u9636\u6bb5Br-\u5d4c\u5165PGA\u6b63\u6781\u7684\u62c9\u66fc\u5149\u8c31\u56fe\u548c\u76f8\u5e94\u7684\u5cf0\uff1b<\/p>\n

f\uff09\u5728\u5145\/\u653e\u7535\u5faa\u73af\u4e2d\uff0c\u539f\u4f4d\u83b7\u5f97\u7684Br-\u5d4c\u5165PGA\u6b63\u6781\u7684XRD\u66f2\u7ebf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aWater-Salt Oligomers Enable Supersoluble Electrolytes for High-Performance Aqueous Batteries<\/a><\/strong>. Adv. Mater.<\/em>, 2021<\/strong>, DOI: 10.1002\/adma.202007470.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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