{"id":218398,"date":"2021-03-01T06:35:35","date_gmt":"2021-02-28T22:35:35","guid":{"rendered":"\/\/m.iemloyee.com\/?p=218398"},"modified":"2021-02-28T20:35:50","modified_gmt":"2021-02-28T12:35:50","slug":"%e7%8e%8b%e6%98%a5%e7%94%9f%e5%a7%9a%e9%9c%9e%e9%93%b6-acs-energy-lett-%ef%bc%9a%e5%9f%ba%e4%ba%8e%e5%8f%8c%e5%8a%9f%e8%83%bdlgps-li%e7%95%8c%e9%9d%a2%e7%9a%84%e5%85%a8%e5%9b%ba%e6%80%81%e9%94%82","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=218398","title":{"rendered":"\u738b\u6625\u751f&\u59da\u971e\u94f6 ACS Energy Lett.\uff1a\u57fa\u4e8e\u53cc\u529f\u80fdLGPS\/Li\u754c\u9762\u7684\u5168\u56fa\u6001\u9502\u786b\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u738b\u6625\u751f\u6559\u6388<\/strong>\u548c\u4e2d\u56fd\u79d1\u5b66\u9662\u5b81\u6ce2\u6750\u6599\u6280\u672f\u4e0e\u5de5\u7a0b\u7814\u7a76\u6240\u59da\u971e\u94f6\u7814\u7a76\u5458<\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u5728LGPS\/Li\u754c\u9762\u4e0a\uff0c\u4f9d\u6b21\u8fd8\u539fMg(TFSI)2<\/sub>-LiTFSI-DME\uff08TFSI\uff1a\u53cc\uff08\u4e09\u6c1f\u7532\u57fa\u78fa\u9170\uff09\u4e9a\u80fa\uff1bDME\uff1a\u4e8c\u7532\u6c27\u57fa\u4e59\u70f7\uff09\u6db2\u6001\u7535\u89e3\u6db2\u4e2d\u7684\u76d0\u548c\u6eb6\u5242\uff0c\u5728Li\u548cLGPS\u4e4b\u95f4\u5f62\u6210\u4e86\u4eb2\u9502-\u758f\u9502\u68af\u5ea6\u7684\u4e2d\u95f4\u5c42\uff0c\u4ece\u800c\u89e3\u51b3\u4e86Li\u679d\u6676\u7684\u751f\u957f\u548cLGPS\u7684\u5206\u89e3\u3002Mg(TFSI)2<\/sub>-LiTFSI\u9996\u5148\u88ab\u8fd8\u539f\uff0c\u7531\u4e8e\u758f\u9502\u6027\u5dee\u5f02\uff0c\u5728Li\u8868\u9762\u4e0a\u5f62\u6210\u4e86\u4eb2\u9502\u7684\u5bccLix<\/sub><\/em>Mg\u5408\u91d1\u5c42\uff0c\u5728Lix<\/sub><\/em>Mg\u4e0a\u90e8\u5f62\u6210\u4e86\u758f\u9502\u7684\u5bccLiF\u5c42\uff0c\u800cDME\u6eb6\u5242\u7684\u8fd8\u539f\u4f1a\u5728\u5bccLiF\u5c42\u548cLGPS\u4e4b\u95f4\u5f62\u6210\u67d4\u6027\u6709\u673a\u805a\u5408\u7269\u3002\u5728DME\u6eb6\u5242\u84b8\u53d1\u540e\uff0cLi\/LGPS\/Ni-Li2<\/sub>S-LiTiS2<\/sub>\u5168\u56fa\u6001\u7535\u6c60\u7684\u9996\u5708\u53ef\u9006\u5bb9\u91cf\u4e3a699.7 mAh g-1<\/sup>\uff081.07 mAh cm-2<\/sup>\uff0c\u57fa\u4e8eNi-Li2<\/sub>S-LiTiS2<\/sub>\u7684\u8d28\u91cf\uff09\u3002Li\u8d1f\u6781\u548cLGPS\u7535\u89e3\u8d28\u4e4b\u95f4\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762\u7684\u5408\u7406\u8bbe\u8ba1\u4e3a\u5f00\u53d1\u9ad8\u6027\u80fd\u5168\u56fa\u6001\u9502\u7535\u6c60\u63d0\u4f9b\u4e86\u65b0\u7684\u673a\u4f1a\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>Bifunctional Interphase-Enabled Li10<\/sub>GeP2<\/sub>S12<\/sub> Electrolytes for Lithium-Sulfur Battery<\/strong>\u201d\u53d1\u8868\u5728ACS Energy Letters<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong> 1 <\/strong>\u56fa\u6001\u7535\u89e3\u8d28\u7684\u5236\u5907\u793a\u610f\u56fe\u53ca\u5176\u5e94\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5728LGPS\u8868\u9762\u4e0a\u6ef4\u52a01.0 M LiTFSI-Mg(TFSI)2<\/sub>-DME\u6db2\u4f53\u7535\u89e3\u6db2\u540e\uff0cLi\u548cLGPS\u4e4b\u95f4\u539f\u4f4d\u5f62\u6210\u7684Lix<\/sub><\/em>Mg\/LiF\/\u805a\u5408\u7269\uff08\u4eb2\u9502-\u758f\u9502\uff09\u754c\u9762\u76f8\u7684\u56fe\u793a \uff1b<\/p>\n

\uff08b\uff09\u57280.2 mA cm-2<\/sup>\u548c0.2 mAh cm-2<\/sup>\u4e0b\uff0c\u4e0d\u540cLiTFSI-Mg(TFSI)2<\/sub>-DME\u6db2\u6001\u7535\u89e3\u6db2\u5904\u7406\u540e\u7684Li\/LGPS\/Li\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

\u56fe<\/strong> 2<\/strong>\u5728<\/strong>LiTFSI-Mg(TFSI)2<\/sub>-DME<\/strong>\u6db2\u4f53\u7535\u89e3\u6db2\u4e2d\u5faa\u73af\u540e\u7684<\/strong>Li<\/strong>\u8d1f\u6781\u4e0a<\/strong>SEI<\/strong>\u7684\u6210\u5206\u5206\u5e03\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 3 <\/strong>\u5faa\u73af\u540e\uff0c<\/strong>Li\/Mg(TFSI)2<\/sub>-LiTFSI-DME@LGPS\/Li<\/strong>\u7535\u6c60\u7684\u754c\u9762\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Li\/Mg(TFSI)2<\/sub>-LiTFSI-DME@LGPS\/Li\u7535\u6c60\u4e2dLGPS\u7684Ga+<\/sup>\u79bb\u5b50\u675f\u6e85\u5c04\u56fe\uff1b<\/p>\n

\uff08b\uff09Li\/Mg(TFSI)2<\/sub>-LiTFSI-DME@LGPS\/Li\u7535\u6c60\u4e2d\u5faa\u73af\u540eLi\u8868\u9762\u7684F\u5143\u7d20\u7684ToF-SIMS\u5206\u6790\u56fe\uff1b<\/p>\n

\uff08c\uff09Li\/Mg(TFSI)2<\/sub>-LiTFSI-DME@LGPS\/Li\u7535\u6c60\u4e2d\u5faa\u73af\u540eLi\u8868\u9762\u7684F\u5143\u7d20\u5206\u5e03\u56fe\u3002<\/p>\n

\u56fe<\/strong> 4 LiMg22<\/strong>\u5904\u7406\u5bf9\u7535\u6c60\u5faa\u73af\u6027\u80fd\u7684\u5f71\u54cd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u57282 mAh cm-2<\/sup>\u548c0.05 mA cm-2<\/sup>\u4e0b\uff0cLi\/LGPS\/Li\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08b\uff09\u57281 mAh cm-2<\/sup>\u548c\u9010\u6e10\u589e\u52a0\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0cLi\/LGPS\/Li\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08c\uff09\u5728\u7535\u6d41\u5bc6\u5ea6\u9010\u6b65\u589e\u52a0\u7684\u60c5\u51b5\u4e0b\uff0c\u7eafLGPS\u548cLiMg22\u5904\u7406\u540e\u7684Li\/LGPS\/Li\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

\u56fe<\/strong> 5<\/strong> \u7535\u6c60\u5faa\u73af\u524d\u540e\uff0c<\/strong>LiMg22<\/strong>\u6db2\u6001\u7535\u89e3\u6db2\u5bf9<\/strong>LGPS<\/strong>\u754c\u9762\u7684\u5f71\u54cd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5faa\u73af\u540e\uff0cLi\/LGPS\/Li\u7535\u6c60\u4e2d\u4f53\u76f8LGPS\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff0cc\uff09\u5faa\u73af\u524d\u540e\uff0cLi\/LGPS-LiMg22\/Li\u7535\u6c60\u4e2d\u4f53\u76f8LGPS\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09\u5faa\u73af\u540e\uff0cLi\/LGPS\/Li\u7535\u6c60\u754c\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff0cf\uff09\u5faa\u73af\u524d\u540e\uff0cLi\/LGPS-LiMg22\/Li\u7535\u6c60\u4e2dLGPS\/Li\u754c\u9762\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/strong> 6 <\/strong>\u5faa\u73af\u540e\uff0c<\/strong>LGPS\/Li<\/strong>\u7684\u754c\u9762\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5faa\u73af\u540e\uff0cLi\/LGPS\/Li\u7535\u6c60\u4e2dLGPS\/Li\u754c\u9762\u7684\u5143\u7d20Mapping\u56fe\uff1b<\/p>\n

\uff08b\uff09\u5faa\u73af\u540e\uff0cLi\/LGPS-LiMg22\/Li\u7535\u6c60\u4e2dLGPS\/Li\u754c\u9762\u7684\u5143\u7d20Mapping\u56fe\u3002<\/p>\n

\u56fe<\/strong> 7 Ni-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS-LiMg22\/Li<\/strong>\u5168\u56fa\u6001\u7535\u6c60\u7684\u6027\u80fd<\/strong><\/p>\n

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\uff08a\uff0cb\uff09Ni-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS\/Li\u548cNi-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS-LiMg22\/Li\u7535\u6c60\u7684\u5bb9\u91cf-\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u5728100 mA g-1<\/sup>\u65f6\uff0cNi-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS-LiMg22\/Li\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08d\uff09Ni-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS-LiMg22\/Li\u7535\u6c60\u7684\u500d\u7387\u6027\u80fd\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u5728LGPS\u56fa\u4f53\u7535\u89e3\u8d28\u548cLi\u8d1f\u6781\u4e4b\u95f4\u6dfb\u52a0LiTFSI-Mg(TFSI)2<\/sub>-DME\u6db2\u4f53\u7535\u89e3\u6db2\u53ef\u4ee5\u6709\u6548\u6291\u5236\u679d\u6676\u751f\u957f\u548cLGPS\u8fd8\u539f\uff0c\u56e0\u4e3aLi\u548cLGPS\u4e4b\u95f4\u5f62\u6210\u4e86Lix<\/sub><\/em>Mg\/LiF\/\u805a\u5408\u7269\u4eb2\u9502-\u758f\u9502\u590d\u5408\u754c\u9762\u3002\u901a\u8fc7LiTFSI-Mg(TFSI)2<\/sub>-DME\u6db2\u4f53\u7535\u89e3\u6db2\u6539\u6027LGPS\uff0c\u4f7fLGPS\u7684\u4e34\u754c\u7535\u6d41\u5bc6\u5ea6\u4ece0.6 mA cm-2<\/sup>\uff08\u5bb9\u91cf\u4e3a0.6 mAh cm-2<\/sup>\uff09\u663e\u8457\u63d0\u9ad8\u52301.3 mA cm-2<\/sup>\uff08\u5bb9\u91cf\u4e3a1.3 mAh cm-2<\/sup>\uff09\u3002\u5168\u56fa\u6001Ni-Li2<\/sub>S-LiTiS2<\/sub>\/LGPS-LiMg22\/Li\u7535\u6c60\u5728100 mA g-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u663e\u793a\u51fa699.7 mAh g-1<\/sup>\uff081.07 mAh cm-2<\/sup>\uff09\u7684\u9ad8\u53ef\u9006\u5bb9\u91cf\uff0c\u5faa\u73af\u5bff\u547d>120\u4e2a\u5faa\u73af\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5<\/strong>Bifunctional Interphase-Enabled Li10<\/sub>GeP2<\/sub>S12<\/sub> Electrolytes for Lithium\u2013Sulfur Battery<\/strong><\/a>\uff08ACS Energy Letters DOI: 10.1021\/acsenergylett.0c02617\uff09\u3002<\/p>\n

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