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Nat. Biotechnol.\uff1a\u8fd1\u7ea2\u5916<\/b><\/strong>IIb<\/b><\/strong>\u533a\u7a00\u571f\u7eb3\u7c73\u9897\u7c92\u7684\u6d3b\u4f53\u5206\u5b50\u6210\u50cf\u52a9\u529b\u514d\u75ab\u6cbb\u7597<\/b><\/strong><\/p>\n

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\u65af\u5766\u798f\u5927\u5b66\u7684\u6234\u5b8f\u6770<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u4e00\u79cd\u5177\u6709\u6838\u58f3\u7ed3\u6784\uff08NaYbF4<\/sub>:2%Er,2%Ce,10%Zn@NaYF4<\/sub>\uff09\u7684\u950c\u63ba\u6742\u03b1\u76f8\u94d2\u57fa\u7a00\u571f\u7eb3\u7c73\u9897\u7c92\uff08\u03b1-ErNPs\uff09\u3002\u5728\u8fd9\u4e00\u9897\u7c92\u4e2d\uff0c\u7814\u7a76\u4eba\u5458\u53ef\u589e\u5f3a\u591a\u5149\u5b50\u5f1b\u8c6b\u5e76\u901a\u8fc7\u950c\u79bb\u5b50\u63ba\u6742\u51cf\u5c11\u6676\u4f53\u573a\u5bf9\u79f0\u6027\uff0c\u4ece\u800c\u5b9e\u73b0\u76f8\u5bf9\u6700\u4eae\u03b2-ErNPs\u589e\u5f3a11\u500d\u7684\u4e0b\u8f6c\u6362\u53d1\u5149\u6027\u80fd\u3002\u6b64\u5916\uff0c\u6750\u6599\u4e2d\u7684\u4eb2\u6c34\u4ea4\u8054\u805a\u5408\u7269\u7f51\u7edc\u53ef\u8d4b\u4e88\u7eb3\u7c73\u9897\u7c92\u826f\u597d\u7684\u6c34\u6eb6\u6027\u548c\u751f\u7269\u76f8\u5bb9\u6027\uff0c\u53ef\u5728\u4e24\u5468\u5185\u5b9e\u73b0\u5feb\u901f\u7684\u80c6\u6c41\u6392\u6cc4\u3002\u8fdb\u4e00\u6b65\u5229\u7528anti-PD-L1\u5355\u6297\u8fdb\u884c\u6807\u8bb0\uff0cErNPs\u5728\u7ed3\u80a0\u764c\u6a21\u578b\u5c0f\u9f20\u4e2d\u5b9e\u73b0\u4e86\u80bf\u7624\/\u6b63\u5e38\u7ec4\u7ec7\u4fe1\u566a\u6bd4\u9ad8\u8fbe40\u5de6\u53f3\u7684\u6210\u50cf\u3002\u8fdb\u4e00\u6b65\u5bf9PD-L1\u548cCD8\u8fdb\u884c\u6210\u50cf\u63ed\u793a\u4e86\u514d\u75ab\u7597\u6cd5\u4e2d\u5728\u80bf\u7624\u5fae\u73af\u5883\u4e2d\u51fa\u73b0\u7684\u6bd2\u6027T\u7ec6\u80de\u4ee5\u53caCD8\u7684\u4fe1\u53f7\u6539\u53d8\uff0c\u4e3a\u66f4\u52a0\u7cbe\u51c6\u9884\u6d4b\u514d\u75ab\u6cbb\u7597\u53cd\u5e94\u63d0\u4f9b\u4e86\u6709\u6548\u7684\u7b56\u7565\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/www.nature.com\/articles\/s41587-019-0262-4<\/p>\n

AM\uff1a\u5177\u6709\u8fd1\u7ea2\u5916\u538b\u81f4\u53d1\u5149\u6027\u80fd\u7684\u94c1\u7535\u7a00\u571f\u6750\u6599<\/b><\/strong><\/p>\n

\u5f3a\u538b\u7535\u6750\u6599\u5f88\u5c11\u80fd\u5c55\u73b0\u51fa\u538b\u81f4\u53d1\u5149\u73b0\u8c61\uff0c\u56e0\u6b64\u5236\u5907\u540c\u65f6\u5177\u6709\u538b\u7535\u6548\u5e94\u548c\u538b\u81f4\u53d1\u5149\u6027\u80fd\u7684\u591a\u538b\u7535\uff08multipiezo\uff09\u6750\u6599\u6781\u5177\u6311\u6218\u3002\u800c\u5177\u6709\u5fae\u5e94\u53d8\u6c34\u5e73\u538b\u529b\u63a2\u6d4b\u80fd\u529b\u7684\u9ad8\u538b\u81f4\u53d1\u5149\u6750\u6599\u5728\u9ad8\u7cbe\u5ea6\u538b\u529b\u68c0\u6d4b\u548c\u9ad8\u5206\u8fa8\u751f\u7269\u529b\u5b66\u6210\u50cf\u7b49\u9886\u57df\u5177\u6709\u91cd\u5927\u7684\u5e94\u7528\u4ef7\u503c\u3002\u56e0\u6b64\uff0c\u5177\u6709\u9ad8\u529b\u81f4\u53d1\u5149\u7075\u654f\u5ea6\u7684\u4f4e\u538b\u529b\u89e6\u53d1NIR\u538b\u81f4\u53d1\u5149\u6750\u6599\u7684\u7814\u53d1\u5b58\u5728\u91cd\u8981\u7684\u610f\u4e49\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

SSN\u7684\u538b\u81f4\u53d1\u5149\u6027\u80fd<\/b><\/strong><\/p>\n

\u65e5\u672c\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\u7684Chao-Nan Xu<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cd\u5728\u9521\u9178\u9536\uff08Sr3<\/sub>Sn2<\/sub>O7<\/sub>\uff09\u94c1\u7535\u57fa\u8d28\u4e2d\u63ba\u6742\u7a00\u571f\u9495\u79bb\u5b50\u7684\u65b0\u578b\u591a\u538b\u7535\u6750\u6599SSN\uff0c\u5176\u80fd\u5728800-1500nm\u7684\u533a\u57df\u5c55\u73b0\u51fa\u8d85\u7075\u654f\u3001\u53ef\u6301\u7eed\u7684\u9ad8\u6027\u80fdNIR\u538b\u81f4\u53d1\u5149\u3002\u7814\u7a76\u8868\u793a\uff0c\u4e09\u4ef7\u7684\u9495\u79bb\u5b50\u80fd\u591f\u53d6\u4ee3\u6750\u6599\u4e2d\u4e8c\u4ef7\u9536\u79bb\u5b50\u4f4d\u70b9\uff0c\u4ece\u800c\u626e\u6f14NIR\u53d1\u5c04\u7684\u53d1\u5149\u4e2d\u5fc3\u3002\u4f5c\u4e3a\u538b\u81f4\u53d1\u5149\u7684\u9ad8\u6548\u53d1\u5c04\u4f53\uff0c\u9521\u9178\u9536\u4e2d\u4e24\u79cd\u7c7b\u578b\u7684\u516b\u9762\u4f53\u65cb\u8f6c\u7684\u4e09\u7ebf\u8026\u5408\u80fd\u591f\u6253\u7834\u5bf9\u79f0\uff0c\u4ece\u800c\u5bfc\u81f4\u81ea\u53d1\u6781\u5316\u7684\u51fa\u73b0\uff1b\u800cSSN\u7684\u6742\u5316\u6027\u8d28\u5219\u80fd\u591f\u63d0\u5347\u52a8\u6001\u6676\u683c\u626d\u66f2\u4e0b\u9495\u79bb\u5b50\u4f4d\u70b9\u9644\u8fd1\u8f7d\u6d41\u5b50\u7684\u8f90\u5c04\u590d\u5408\uff0c\u5b9e\u73b0\u589e\u5f3a\u7684NIR\u53d1\u5c04\u3002\u6b64\u5916\uff0c\u7814\u7a76\u8fd8\u8ba8\u8bba\u4e86\u57fa\u4e8eSSN\u7684\u538b\u81f4\u53d1\u5149\u6a21\u578b\uff0c\u9610\u91ca\u4e86\u5176\u5b9e\u73b0\u65e0\u5149\u6fc0\u53d1\u6210\u50cf\u80fd\u529b\u3002\u7efc\u5408\u4ee5\u4e0a\u7814\u7a76\u6210\u679c\uff0c\u6587\u7ae0\u8ba4\u4e3a\u8be5NIR\u538b\u81f4\u53d1\u5149\u6750\u6599\u53ef\u4ee5\u4f5c\u4e3a\u6df1\u5c42\u6210\u50cf\u548c\u529b\u5b66\u63a2\u6d4b\u7684\u63a2\u9488\u8fdb\u884c\u4f7f\u7528\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/full\/10.1002\/adma.201908083<\/p>\n

Angew\uff1a\u8d85\u8584\u6c27\u5316\u9486\u7eb3\u7c73\u5377\u8f74\u7528\u4e8e\u78c1\u5171\u632f\u6210\u50cf<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

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\u53d1\u5c55\u5177\u6709\u80bf\u7624\u5fae\u73af\u5883\u6fc0\u6d3b\u6cbb\u7597\u6a21\u5f0f\u7684\u751f\u7269\u53ef\u964d\u89e3\u65e0\u673a\u7eb3\u7c73\u9897\u7c92\u5bf9\u4e8e\u7cbe\u51c6\u764c\u75c7\u533b\u5b66\u6765\u8bf4\u662f\u4e9f\u5f85\u89e3\u51b3\u7684\u9700\u6c42\u548c\u6311\u6218\u3002\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u7684\u96f7\u6ce2\u548c\u5357\u5f00\u5927\u5b66\u7684\u675c\u4e9a\u5e73<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba\u8054\u5408\u62a5\u9053\u5408\u6210\u4e86\u8d85\u8584\u6c27\u5316\u9486\u7eb3\u7c73\u5377\u8f74\u3002\u8fd9\u4e00\u7eb3\u7c73\u6750\u6599\u5177\u6709\u9ad8\u5ea6\u53ef\u63a7\u7684\u78c1\u5b66\u6027\u80fd\uff0c\u80fd\u591f\u5b9e\u73b0\u9ad8\u5206\u8fa8\u7684\u78c1\u5171\u632f\u6210\u50cf\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u6c27\u5316\u9486\u7eb3\u7c73\u5377\u8f74\u53ef\u54cd\u5e94\u80bf\u7624pH\u8fdb\u884c\u964d\u89e3\u5e76\u9009\u62e9\u6027\u6e17\u900f\u80bf\u7624\u7ec4\u7ec7\uff0c\u4ece\u800c\u5b9e\u73b0\u6297\u764c\u836f\u7269\u7684\u9776\u5411\u91ca\u653e\u3002\u4e0d\u4ec5\u5982\u6b64\uff0c\u901a\u8fc710%\u7684\u94d5\u79bb\u5b50\u63ba\u6742\uff0c\u7eb3\u7c73\u5377\u8f74\u8fd8\u53ef\u5b9e\u73b0\u4f18\u5f02\u7684\u5149\u81f4\u53d1\u5149\u6027\u80fd\u3002\u51ed\u501f\u5de8\u5927\u7684\u6bd4\u8868\u9762\u79ef\uff0c\u7eb3\u7c73\u5377\u8f74\u53ef\u4ee5\u9ad8\u6548\u88c5\u8f7d\u6297\u764c\u836f\u7269DOX\uff0880%\u5de6\u53f3\uff09\uff0c\u5728\u7ec6\u80de\u548c\u7ec4\u7ec7\u6bd2\u6027\u51e0\u4e4e\u53ef\u4ee5\u5ffd\u7565\u4e0d\u8ba1\u7684\u524d\u63d0\u4e0b\u5c55\u73b0\u51fa\u4e86\u663e\u8457\u7684\u80bf\u7624\u751f\u957f\u6291\u5236\u80fd\u529b\u3002\u6587\u7ae0\u8ba4\u4e3a\uff0c\u8fd9\u4e00\u7814\u7a76\u53ef\u4ee5\u4e3a\u8bbe\u8ba1\u7528\u4e8e\u751f\u7269\u6210\u50cf\u548c\u751f\u7269\u964d\u89e3\u589e\u5f3a\u578b\u764c\u75c7\u6cbb\u7597\u7684\u80bf\u7624\u5fae\u73af\u5883\u54cd\u5e94\u65e0\u673a\u7eb3\u7c73\u6750\u6599\u63d0\u4f9b\u65b0\u7684\u601d\u8def\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/www.onlinelibrary.wiley.com\/doi\/full\/10.1002\/anie.201812972\u00a0<\/b><\/strong><\/p>\n

JACS\uff1a\u5728\u94dc-\u6c27\u5316\u94c8\u7eb3\u7c73\u68d2\u50ac\u5316\u5242\u4e2d\u6784\u5efa\u6d3b\u6027\u4f4d\u70b9<\/b><\/strong><\/p>\n

\u5927\u91cf\u7684\u7814\u7a76\u8868\u660e\uff0c\u5728\u6c27\u5316\u94c8\u4e0a\u8d1f\u8f7d\u9ad8\u542b\u91cf\u94dc\u53ef\u88ab\u7528\u4e8e\u4e00\u6c27\u5316\u78b3\u7684\u6e05\u9664\u548c\u5229\u7528\u3002\u7136\u800c\uff0c\u8fd9\u7c7b\u6750\u6599\u7684\u9ad8\u6d3b\u6027\u548c\u70ed\u7a33\u5b9a\u6027\u4e00\u76f4\u65e0\u6cd5\u5171\u5b58\uff0c\u4e25\u91cd\u9650\u5236\u4e86\u94dc-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u7684\u5b9e\u9645\u5e94\u7528\u3002\u540c\u65f6\uff0c\u94dc-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u4e2d\u6d3b\u6027\u4f4d\u70b9\u7684\u539f\u5b50\u7ed3\u6784\u4f9d\u7136\u65e0\u6cd5\u8fa8\u6790\u4e14\u5b58\u5728\u4e89\u8bae\uff0c\u59cb\u7ec8\u963b\u788d\u7740\u6750\u6599\u50ac\u5316\u673a\u5236\u53ca\u5176\u5e94\u7528\u7814\u7a76\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u94dc-\u6c27\u5316\u94c8\u7684\u50ac\u5316\u4e00\u6c27\u5316\u78b3\u6c27\u5316\u673a\u7406<\/b><\/strong><\/p>\n

\u9488\u5bf9\u8fd9\u4e9b\u95ee\u9898\uff0c\u5317\u4eac\u5927\u5b66\u7684\u4e25\u7eaf\u534e\u3001\u5c71\u4e1c\u5927\u5b66\u7684\u8d3e\u6625\u6c5f\u548c\u4e2d\u79d1\u9662\u4e0a\u6d77\u5e94\u7528\u7269\u7406\u7814\u7a76\u6240\u7684Rui Si<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba\u901a\u8fc7800\u6444\u6c0f\u5ea6\u7684\u7a7a\u6c14\u7145\u70e7\u5728\u70e7\u7ed3\u7684\u94dc-\u6c27\u5316\u94c8\u4e0a\u610f\u5916\u6784\u5efa\u4e86\u914d\u4f4d\u4e0d\u9971\u548c\u3001\u539f\u5b50\u7ea7\u5206\u6563\u7684\u94dc\u7269\u79cd\u3002\u8fd9\u4e00\u94dc-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u5bf9\u4e00\u6c27\u5316\u78b3\u6c27\u5316\u8868\u73b0\u51fa\u4e86\u6781\u9ad8\u7684\u6d3b\u6027\uff0c\u5728120\u6444\u6c0f\u5ea6\u65f6\u4e00\u6c27\u5316\u78b3\u7684\u6d88\u8017\u901f\u5ea6\u53ef\u8fbe\u52306100 \u03bcmolCO<\/sub>\u00b7gCu<\/sub>\u22121<\/sup>\u00b7s\u22121<\/sup>\uff0c\u81f3\u5c11\u6bd4\u5df2\u62a5\u9053\u7684\u94dc\u50ac\u5316\u5242\u9ad820\u500d\u3002\u6b64\u5916\uff0c\u5728\u4e25\u82db\u7684\u5faa\u73af\u53cd\u5e94\u6761\u4ef6\u4e2d\uff0c\u8be5\u50ac\u5316\u5242\u4f9d\u7136\u5c55\u73b0\u51fa\u4e86\u4f18\u5f02\u7684\u957f\u671f\u7a33\u5b9a\u6027\u3002\u57fa\u4e8e\u7efc\u5408\u7684\u7ed3\u6784\u8868\u5f81\u548c\u673a\u5236\u7814\u7a76\uff0c\u7814\u7a76\u53d1\u73b0\u5355\u4e2a\u4f4d\u70b9\u5904\u7684\u975e\u9971\u548c\u914d\u4f4d\u94dc\u539f\u5b50\u4ee5Cu1<\/sub>O3<\/sub>\u7684\u5f62\u5f0f\u5b58\u5728\uff0c\u4f7f\u4e00\u6c27\u5316\u78b3\u548c\u6c27\u6c14\u5206\u5b50\u53ef\u5747\u5728\u8be5\u4f4d\u70b9\u5904\u6d3b\u5316\uff0c\u4ece\u800c\u5728\u4f4e\u94dc\u8d1f\u8f7d\u91cf\uff081wt%\uff09\u7684\u6761\u4ef6\u4e0b\u5b9e\u73b0\u53ef\u89c2\u7684\u4e00\u6c27\u5316\u78b3\u6c27\u5316\u6d3b\u6027\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.9b05419<\/p>\n

JACS\uff1a\u76f4\u63a5\u8fa8\u6790\u91d1-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u4e0a\u7528\u4e8e\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u7684\u6d3b\u6027\u8868\u9762\u79cd<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u91d1-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u5728\u50ac\u5316\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u4e2d\u7684\u7ed3\u6784\u8868\u5f81<\/b><\/strong><\/p>\n

\u5927\u91cf\u7684\u5de5\u4f5c\u5df2\u7ecf\u9610\u660e\u4e86\u91d1\u5c5e-\u6c27\u5316\u7269\u754c\u9762\u5728\u50ac\u5316\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u4e2d\u626e\u6f14\u7684\u5173\u952e\u89d2\u8272\uff0c\u7136\u800c\u5bf9\u754c\u9762\u4f4d\u70b9\u5904\u7684\u5185\u5728\u53cd\u5e94\u76ee\u524d\u8fd8\u9c9c\u6709\u6df1\u5165\u7684\u7814\u7a76\u3002\u800c\u5317\u4eac\u5927\u5b66\u7684\u4e25\u7eaf\u534e\u3001\u5c71\u4e1c\u5927\u5b66\u7684\u8d3e\u6625\u6c5f\u548c\u4e2d\u79d1\u9662\u4e0a\u6d77\u5e94\u7528\u7269\u7406\u7814\u7a76\u6240\u7684Rui Si<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba\u4e3a\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u5236\u5907\u4e86\u4e24\u79cd\u5177\u6709\u4e0d\u540c\u91d1\u79cd\uff08gold species\uff09\u7684\u91d1-\u6c27\u5316\u94c8\u50ac\u5316\u5242\uff0c\u5176\u4e2d\u4e00\u79cd\u7684\u91d1\u79cd\u4e3a\u5c3a\u5bf8\u5c0f\u4e8e2\u7eb3\u7c73\u7684\u91d1\u7c07\uff0c\u800c\u53e6\u5916\u4e00\u79cd\u5219\u4e3a3-4\u7eb3\u7c73\u7684\u91d1\u7eb3\u7c73\u9897\u7c92\u3002\u7814\u7a76\u663e\u793a\uff0c\u4e0e\u91d1\u7eb3\u7c73\u9897\u7c92\u76f8\u6bd4\uff0c\u91d1\u7c07\u50ac\u5316\u5242\u5c55\u73b0\u51fa\u4e86\u66f4\u52a0\u4f18\u5f02\u7684\u53cd\u5e94\u6d3b\u6027\u3002\u5728\u539f\u4f4d\u8868\u5f81\u6280\u672f\u7684\u5e2e\u52a9\u4e0b\uff0c\u7814\u7a76\u4eba\u5458\u5206\u6790\u4e86\u91d1-\u6c27\u5316\u94c8\u50ac\u5316\u5242\u4e2d\u7684\u6570\u79cd\u8868\u9762\u6c22\u6c27\u6839\uff0c\u53d1\u73b0\u6c27\u5316\u94c8\u57fa\u8d28\u8868\u9762\u6c27\u7a7a\u4f4d\u4e0a\u5f62\u6210\u7684\u6865\u8fde\u7f9f\u57fa\u57fa\u56e2\u5177\u6709\u5355\u4f4d\u70b9\u6d3b\u6027\u6784\u8c61\u3002\u540c\u4f4d\u7d20\u793a\u8e2a\u7ed3\u679c\u4e5f\u8fdb\u4e00\u6b65\u8bc1\u660e\u6865\u8fde\u8868\u9762\u7f9f\u57fa\u4e0e\u5438\u9644\u5728\u754c\u9762\u91d1\u539f\u5b50\u4e0a\u7684\u4e00\u6c27\u5316\u78b3\u4e4b\u95f4\u7684\u53cd\u5e94\u8d21\u732e\u4e86\u5927\u90e8\u5206\u7684\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u6d3b\u6027\u3002\u56e0\u6b64\uff0c\u76f8\u6bd4\u8d77\u91d1\u7eb3\u7c73\u9897\u7c92\uff0c\u91d1\u7c07\u4e2d\u4e30\u5bcc\u7684\u754c\u9762\u4f4d\u70b9\u80fd\u591f\u8fdb\u4e00\u6b65\u5f15\u53d1\u50ac\u5316\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u7684\u53cd\u5e94\u6d3b\u6027\u3002\u8fd9\u4e9b\u7ed3\u679c\u6709\u5229\u4e8e\u5728\u539f\u5b50\u6c34\u5e73\u6df1\u5165\u7406\u89e3\u50ac\u5316\u5242\u50ac\u5316\u7684\u6c34\u7164\u6c14\u4ea4\u6362\u53cd\u5e94\u7684\u53cd\u5e94\u673a\u5236\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.8b09306<\/p>\n

Nat. Commun.\uff1a\u6c27\u5316\u94c8\u4e0a\u94dc\u4f4d\u70b9\u5438\u9644\u6d3b\u5316\u5206\u5b50\u6c27<\/b><\/strong><\/p>\n

\u76f8\u6bd4\u8d77\u91d1\u5c5e\u7c07\u4e2d\u53d1\u73b0\u7684\u8fde\u7eed\u80fd\u5e26\u7ed3\u6784\uff0c\u8868\u9762\u539f\u5b50\u7ea7\u91d1\u5c5e\u4f4d\u70b9\u5219\u5177\u6709\u79bb\u6563\u7684\u7535\u5b50\u7ed3\u6784\uff0c\u56e0\u6b64\u8fd9\u7c7b\u539f\u5b50\u7ea7\u91d1\u5c5e\u4f4d\u70b9\u4e0e\u53cd\u5e94\u7269\u7684\u4f5c\u7528\u5747\u662f\u57fa\u4e8e\u7ed3\u6784\u548c\u80fd\u91cf\u5339\u914d\u3002\u8fd9\u6837\u4e00\u6765\uff0c\u5bf9\u8fd9\u7c7b\u539f\u5b50\u7ea7\u4f4d\u70b9\u7684\u7535\u5b50\u7ed3\u6784\u8fdb\u884c\u7cbe\u786e\u8c03\u63a7\u5bf9\u4e8e\u5b9e\u73b0\u53ef\u63a7\u7684\u53cd\u5e94\u8def\u5f84\u5c31\u663e\u5f97\u683c\u5916\u91cd\u8981\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u94c8\u79bb\u5b50\u7684\u7535\u5b50\u62bd\u51fa\u6548\u5e94\uff08electron withdrawing effect\uff09\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\u4f26\u6566\u5927\u5b66\u5b66\u9662\u7684Bolun Wang\u548cFeng Ryan Wang<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u62a5\u9053\u4e86\u901a\u8fc7\u6c27\u5316\u94c8\u8868\u9762\u5bf9\u539f\u5b50\u7ea7Cu(I)\/Cu(II)\u4f4d\u70b9\u7684\u7535\u5b50\u7ed3\u6784\u8fdb\u884c\u8c03\u63a7\u3002\u7814\u7a76\u8868\u793a\uff0c\u90bb\u8fd1\u7684\u56db\u4ef7\u94c8\u79bb\u5b50\u80fd\u591f\u5c06Cu(II)\u7684\u5360\u636e3d<\/i><\/em>\u80fd\u91cf\u964d\u4f4e0.7eV\uff0c\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u4ece\u6c27\u5316\u94dc\u7c07\u5230\u539f\u5b50\u7ea7Cu(II)\u4f4d\u70b9\uff0c\u672a\u5360\u636e\u76844p<\/i><\/em>z<\/i><\/sub><\/em>\u8f68\u9053\u80fd\u91cf\u5219\u589e\u52a0\u4e862.2eV\u3002\u62c9\u66fc\u8c31\u5b66\u7b49\u8868\u5f81\u53d1\u73b0\uff0c\u8fd9\u4e00\u7535\u5b50\u7ed3\u6784\u4e0a\u7684\u53d8\u5316\u5728\u6c27\u6c14\u5438\u9644\u65f6\u80fd\u591f\u5f62\u6210\u4eb2\u7535\u7684[Cu(II)O2<\/sub>(\u03b72<\/sup>\u2013O2<\/sub>)]4\u2212<\/sup>\u4f4d\u70b9\u3002\u901a\u8fc7\u5bf9\u8868\u9762\u539f\u5b50\u7ea7Cu(II)\u4f4d\u70b9\u8fdb\u884c\u91cf\u5316\uff0c\u7814\u7a76\u8fdb\u4e00\u6b65\u8bc1\u5b9e\u4e86\u4e00\u6c27\u5316\u78b3\u6c27\u5316\u53cd\u5e94\u4e2dCu(I\/II)\u4f4d\u70b9\u7684\u6d3b\u6027\u4e0e\u5b9a\u91cf\u7684\u7535\u5b50\u7ed3\u6784\u9ad8\u5ea6\u76f8\u5173\u3002\u7ed3\u5408\u8fd9\u4e9b\u6210\u679c\uff0c\u8be5\u9879\u7814\u7a76\u5de5\u4f5c\u4e3a\u5229\u7528\u539f\u5b50\u7ea7\u91d1\u5c5e\u548c\u57fa\u8d28\u9633\u79bb\u5b50\u4e4b\u95f4\u7684\u4f5c\u7528\u4ee5\u8c03\u63a7\u6d3b\u6027\u4f4d\u70b9\u7684\u7535\u5b50\u7ed3\u6784\u63d0\u4f9b\u4e86\u666e\u9002\u7684\u7b56\u7565\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/www.nature.com\/articles\/s41467-020-17852-8<\/p>\n

Science\uff1a<\/b><\/strong>\u94d5\u79bb\u5b50\u5bf9<\/b><\/strong>\u63d0\u5347\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u5bff\u547d<\/b><\/strong><\/p>\n

\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u662f\u5e7f\u53d7\u5173\u6ce8\u7684\u65b0\u4e00\u4ee3\u5149\u4f0f\u6280\u672f\uff0c\u800c\u5176\u5de5\u4f5c\u7a33\u5b9a\u6027\u662f\u76ee\u524d\u4ea7\u4e1a\u5316\u7684\u4e3b\u8981\u969c\u788d\u3002\u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u5438\u6536\u5c42\u4e2d\u5e38\u5e38\u542b\u6709\u8f6f\u6027\u6210\u5206\uff0c\u4f1a\u5728\u5668\u4ef6\u5236\u5907\u548c\u8fd0\u884c\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u94c5\uff08Pb0<\/sup>\uff09\u548c\u7898\uff08I0<\/sup>\uff09\u7f3a\u9677\u3002\u8fd9\u4e9b\u7f3a\u9677\u4e0d\u4ec5\u662f\u964d\u4f4e\u5668\u4ef6\u6548\u7387\u7684\u590d\u5408\u4e2d\u5fc3\uff0c\u8fd8\u80fd\u964d\u89e3\u5f15\u53d1\u5242\u6765\u635f\u5bb3\u5668\u4ef6\u5bff\u547d\u3002\u5927\u91cf\u7684\u7814\u7a76\u805a\u7126\u4e8e\u901a\u8fc7\u7ec4\u5206\u4f18\u5316\u3001\u5c01\u88c5\u3001\u754c\u9762\u6539\u6027\u7b49\u6765\u51cf\u7f13\u6027\u80fd\u4e0b\u964d\u3001\u63d0\u5347\u5668\u4ef6\u7a33\u5b9a\u6027\u3002\u7136\u800c\u8981\u8fdb\u4e00\u6b65\u63d0\u9ad8\u5668\u4ef6\u7684\u5bff\u547d\uff0c\u9700\u8981\u53d1\u5c55\u4e00\u79cd\u957f\u671f\u6709\u6548\u7684\u65b9\u6cd5\u4ee5\u6291\u5236\u4f7f\u5f79\u8fc7\u7a0b\u4e2d\u6750\u6599\u7684\u672c\u5f81\u7f3a\u9677\u3002<\/p>\n

\"\"<\/b><\/strong><\/p>\n

Eu<\/b><\/strong>3+<\/b><\/sup><\/strong>-Eu<\/b><\/strong>2+<\/b><\/sup><\/strong>\u79bb\u5b50\u5bf9\u4fc3\u8fdb<\/b><\/strong>Pb<\/b><\/strong>0<\/b><\/sup><\/strong>\u00a0<\/b><\/strong>\u548c<\/b><\/strong>I<\/b><\/strong>0<\/b><\/sup><\/strong>\u00a0<\/b><\/strong>\u5411<\/b><\/strong>Pb<\/b><\/strong>2+<\/b><\/sup><\/strong>\u00a0<\/b><\/strong>\u548c<\/b><\/strong>I<\/b><\/strong>\u2013<\/b><\/sup><\/strong>\u8f6c\u53d8<\/b><\/strong><\/p>\n

\u4e3a\u63d0\u9ad8\u672c\u5f81\u7a33\u5b9a\u6027\uff0c\u5317\u4eac\u5927\u5b66\u5468\u6b22\u840d\u3001\u5b59\u8046\u4e1c<\/b><\/strong>\u4ee5\u53ca<\/b><\/strong>\u4e25\u7eaf\u534e<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u5408\u4f5c\u63d0\u51fa\u5728\u9499\u949b\u77ff\u6d3b\u6027\u5c42\u4e2d\u5f15\u5165\u94d5\u79bb\u5b50\u5bf9\uff08Eu3+<\/sup>\/Eu2+<\/sup>\uff09\u7684\u7b56\u7565\u3002\u94d5\u79bb\u5b50\u5bf9\u53ef\u4f5c\u4e3a\u201c\u6c27\u5316\u8fd8\u539f\u68ad\u201d\uff0c\u53ef\u9009\u62e9\u6027\u5730\u540c\u65f6\u6c27\u5316Pb0<\/sup>\u548c\u8fd8\u539fI0<\/sup>\u7f3a\u9677\u3002\u8be5\u79bb\u5b50\u5bf9\u5728\u5668\u4ef6\u4f7f\u7528\u8fc7\u7a0b\u4e2d\u6ca1\u6709\u660e\u663e\u6d88\u8017\uff0c\u57fa\u4e8e\u6b64\u7b56\u7565\u5236\u5907\u7684\u5668\u4ef6\u80fd\u91cf\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\u6700\u9ad8\u53ef\u8fbe21.52\uff05\uff08\u8ba4\u8bc1\u503c\u4e3a20.52\uff05\uff09\uff0c\u5176\u957f\u671f\u7a33\u5b9a\u8010\u7528\u6027\u4e5f\u5f97\u5230\u4e86\u5927\u5e45\u6539\u5584\u3002\u540c\u65f6\uff0c\u5f15\u5165\u94d5\u79bb\u5b50\u5bf9\u7684\u8584\u819c\u5668\u4ef6\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u5149\u7a33\u5b9a\u6027\uff0c\u5728\u8fde\u7eed\u592a\u9633\u5149\u529f\u7387\u8f90\u7167\u621685\u2103\u52a0\u70ed1500\u5c0f\u65f6\u540e\uff0c\u5668\u4ef6\u4ecd\u53ef\u5206\u522b\u4fdd\u6301\u539f\u6709\u5cf0\u503cPCE\u768492\uff05\u548c89\uff05\uff1b\u5728\u6700\u5927\u529f\u7387\u70b9\u8fde\u7eed\u5de5\u4f5c500\u5c0f\u65f6\u540e\u4fdd\u6301\u539f\u6709\u7a33\u5b9aPCE\u768491%\u3002\u8be5\u7b56\u7565\u7684\u63d0\u51fa\u514b\u670d\u4e86\u5f71\u54cd\u94c5\u5364\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7a33\u5b9a\u6027\u7684\u91cd\u8981\u672c\u5f81\u56e0\u7d20\uff0c\u63d0\u5347\u4e86\u9499\u949b\u77ff\u5149\u7535\u5668\u4ef6\u6027\u80fd\uff0c\u5bf9\u4e8e\u65e0\u673a\u534a\u5bfc\u4f53\u5668\u4ef6\u6027\u80fd\u7684\u4f18\u5316\u6539\u5584\u5177\u6709\u6df1\u523b\u7684\u53c2\u8003\u610f\u4e49\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>https:\/\/science.sciencemag.org\/content\/363\/6424\/265<\/p>\n

\u672c\u6587\u7531NanoCJ\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

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