{"id":215623,"date":"2021-01-11T06:37:23","date_gmt":"2021-01-10T22:37:23","guid":{"rendered":"\/\/m.iemloyee.com\/?p=215623"},"modified":"2021-01-10T19:37:39","modified_gmt":"2021-01-10T11:37:39","slug":"%e4%b8%ad%e7%a7%91%e9%99%a2%e5%8c%96%e5%ad%a6%e6%89%80jacs%ef%bc%9a%e5%8e%9f%e4%bd%8dafm%e6%8f%ad%e7%a4%ba%e4%ba%86%e7%ba%b3%e7%b1%b3%e7%ba%a7%e9%94%82%e6%b2%89%e7%a7%af-%e6%ba%b6%e8%a7%a3%e5%9c%a8","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=215623","title":{"rendered":"\u4e2d\u79d1\u9662\u5316\u5b66\u6240JACS\uff1a\u539f\u4f4dAFM\u63ed\u793a\u4e86\u7eb3\u7c73\u7ea7\u9502\u6c89\u79ef\/\u6eb6\u89e3\u5728\u5168\u56fa\u6001\u7535\u6c60\u7684\u5f62\u6001\u6f14\u5316"},"content":{"rendered":"<p>\u4e3a\u4e86\u63d0\u9ad8\u786b\u5316\u7269\u57faASSLMBs\u7684\u6027\u80fd\uff0c\u5728\u4f20\u7edf\u786b\u5316\u7269\u7535\u89e3\u8d28\u7684\u57fa\u7840\u4e0a\u5f15\u5165\u4e86\u5143\u7d20\u63ba\u6742\uff1a\u7528\u5408\u91d1\u9633\u6781\u4ee3\u66ff\u539f\u59cb\u9502\u6765\u7a33\u5b9a\u9502\u548cSSE\u7684\u754c\u9762\uff0c\u8bbe\u8ba1\u4e86\u590d\u5408\u9634\u6781\u7b56\u7565\u6765\u8fdb\u4e00\u6b65\u6539\u5584\u9634\u6781\/SSE\u754c\u9762\uff0c\u5e76\u901a\u8fc7\u6dfb\u52a0\u754c\u9762\u6d82\u5c42\uff0c\u6709\u6548\u5730\u9632\u6b62\u4e86\u6709\u5bb3\u7684\u526f\u53cd\u5e94\u3002\u5c3d\u7ba1\u8fd9\u4e9b\u65b9\u6cd5\u786e\u5b9e\u53ef\u4ee5\u4f18\u5316\u9633\u6781\u7684\u7535\u5316\u5b66\u6027\u80fd\u548c\u754c\u9762\u7684\u5efa\u7acb\uff0c\u4f46\u662f\u957f\u671f\u7684\u4e0d\u7a33\u5b9a\u6027\u548c\u5267\u70c8\u7684\u7ed3\u6784\u9000\u5316\u4ecd\u7136\u9700\u8981\u6df1\u5165\u4e86\u89e3\u9633\u6781\u7684\u754c\u9762\u673a\u7406\u3002\u5f53\u8003\u8651\u5230\u9502\u91d1\u5c5e\u548c\u7535\u6781\/\u7535\u89e3\u8d28\u754c\u9762\u5728SSE\u7cfb\u7edf\u4e2d\u7684\uff08\u7535\uff09\u5316\u5b66\u6d3b\u6027\u65f6\uff0c\u53ea\u6709\u975e\u5e38\u6709\u9650\u7684\u6280\u672f\u624d\u80fd\u83b7\u5f97SSE\u4e2d\u9502\u9633\u6781\u53ca\u5176SEI\u819c\u7684\u7279\u5f81\u3002\u56e0\u6b64\uff0c\u8fd9\u5f3a\u8c03\u4e86\u4ece\u5fae\u89c2\u89d2\u5ea6\u5bf9Li\u6c89\u79ef\/\u6eb6\u89e3\u7684\u52a8\u6001\u53ef\u89c6\u5316\u548cSEI\u6f14\u5316\u7684\u754c\u9762\u673a\u5236\u7684\u539f\u4f4d\u89c1\u89e3\u7684\u91cd\u8981\u6027\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215625 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-5-2.png\" alt=\"\" width=\"600\" height=\"235\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-5-2.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-5-2-300x118.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u8fd1\u65e5\uff0c\u4e2d\u56fd\u79d1\u5b66\u9662\u5316\u5b66\u7814\u7a76\u6240<strong><b>\u6587\u9510<\/b><\/strong>\u8bfe\u9898\u7ec4\u7814\u7a76\u56e2\u961f\uff0c\u4ee5\u201cMicromechanism in All-Solid-State Alloy-Metal Batteries: Regulating Homogeneous Lithium Precipitation and Flexible Solid Electrolyte Interphase Evolution\u201d\u4e3a\u9898\u5728<em><i>J. Am. Chem. Soc.<\/i><\/em>\u671f\u520a\u4e0a\u53d1\u8868\u91cd\u8981\u7814\u7a76\u6210\u679c\u3002\u5728\u6b64\uff0c\u4f5c\u8005\u901a\u8fc7\u539f\u4f4d\u539f\u5b50\u529b\u663e\u5fae\u955c\u63ed\u793a\u4e86\u5728\u9502\u7535\u6781\u4e0a\u9502\u6c89\u6dc0\u7684\u5757\u72b6\u5f62\u6210\u548c\u5806\u79ef\u884c\u4e3a\uff0c\u63ed\u793a\u4e86\u7eb3\u7c73\u7ea7\u9502\u6c89\u79ef\/\u6eb6\u89e3\u5728ASSBs\u4e2d\u7684\u5f62\u6001\u6f14\u5316\u3002\u6b64\u5916\uff0c\u94df\u7535\u6781\u4e0a\u7684\u4e8c\u7ef4Li-In\u5408\u91d1\u7247\u5c42\u548c\u5747\u76f8\u56fa\u6001\u7535\u89e3\u8d28\u754c\u9762(SEI)\u58f3\u5c42\u53cd\u6620\u4e86\u5408\u91d1\u9633\u6781\u5fae\u89c2\u8c03\u63a7\u7684\u6c89\u6dc0\u673a\u7406\u3002\u67d4\u6027\u548c\u8936\u76b1\u7ed3\u6784\u7684SEI\u58f3\u8fdb\u4e00\u6b65\u4f7f\u7535\u6781\u4fdd\u62a4\u548c\u5185\u90e8\u9502\u8c03\u8282\u5faa\u73af\uff0c\u9610\u660e\u4e86SEI\u58f3\u5bf9\u5faa\u73af\u884c\u4e3a\u7684\u529f\u80fd\u5f71\u54cd\u3002\u8fd9\u79cd\u5bf9\u5f62\u6001\u6f14\u5316\u548c\u52a8\u529b\u5b66\u673a\u5236\u7684\u539f\u4f4d\u8ddf\u8e2a\u63d0\u4f9b\u4e86\u6df1\u5165\u7684\u7406\u89e3\uff0c\u4ece\u800c\u6709\u5229\u4e8e\u5408\u91d1\u57faASSBs\u7684\u4f18\u5316\u3002<\/p>\n<p>\u4f5c\u8005\u91c7\u7528\u539f\u4f4d\u539f\u5b50\u529b\u663e\u5fae\u955c(AFM)\u5bf9Li\u7535\u6781\u7684\u7535\u9540\/\u5265\u79bb\u8fc7\u7a0b\u8fdb\u884c\u4e86\u5b9e\u65f6\u76d1\u6d4b\u3002\u5b9e\u9a8c\u7535\u5316\u5b66\u7535\u6c60\u7684\u793a\u610f\u56fe\u5982\u56fe1a\u6240\u793a\uff0c\u5c06\u4e0a\u8ff0LGPS 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V\u65f6\uff0c\u5c11\u91cf\u7684\u5757\u7ed3\u6784\u4ea7\u7269\u51fa\u73b0\u5728\u7535\u6781\u8868\u9762\uff0c\u5e76\u9644\u7740\u4e86\u4e00\u4e9b\u7eb3\u7c73\u7c92\u5b50(NPs)(\u5982\u56fe1c\u4e2d\u9ec4\u8272\u7bad\u5934\u6240\u793a)\u3002\u8fd9\u4e9b\u5c0f\u5757\u4f53\u751f\u957f\u5e76\u5806\u79ef(\u56fe1d)\uff0c\u8fd9\u53ef\u80fd\u4e0eLi\u6c89\u79ef\u7684\u521d\u59cb\u9636\u6bb5\u6709\u5173\u3002\u540c\u65f6\uff0c\u5728Li\u7535\u6781\u4e0a\u6355\u6349\u5230\u9ad8\u4eae\u663e\u793a\u7684\u5916\u89c2\uff0c\u5982\u56fe1d\u4e2d\u7ea2\u8272\u7bad\u5934\u6240\u793a\u3002\u7a81\u7136\uff0c\u4e00\u5c0f\u5757\u53ea\u51fa\u73b0\u5728\u9ec4\u8272\u865a\u7ebf\u8fb9\u7f18\u7684\u533a\u57df(\u56fe1e)\uff0c\u8bf4\u660e\u4e86Li\/LGPS\u7cfb\u7edf\u4e2d\u4e0d\u5747\u5300\u7684\u9502\u6c89\u79ef\u884c\u4e3a\u3002<\/p>\n<p><strong><b>\u56fe<\/b><\/strong><strong><b>1.<\/b><\/strong>\u00a0<strong><b>\u5728<\/b><\/strong><strong><b>Li\u7535\u6781<\/b><\/strong><strong><b>\u4e0a\u7535<\/b><\/strong><strong><b>\u9540\/\u5265<\/b><\/strong><strong><b>\u79bb<\/b><\/strong><strong><b>Li\u8fc7\u7a0b\u7684\u539f\u5b50\u529b\u663e\u5fae\u955c\u539f\u4f4d\u76d1\u6d4b\u3002<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215626 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-6-2.png\" alt=\"\" width=\"600\" height=\"374\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-6-2.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2021\/01\/\u56fe\u7247-6-2-300x187.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u4e3a\u4e86\u8fdb\u4e00\u6b65\u63a2\u7d22\u5408\u91d1\u9633\u6781\u5728ASSLMBs\u4e2d\u7684\u884c\u4e3a\u548c\u89c4\u5f8b\uff0c\u4f5c\u8005\u9996\u5148\u91c7\u7528In\u7535\u6781\u4f5c\u4e3aWE\uff0cLGPS\u4f5c\u4e3aSSE\uff0c\u5bf9\u9502\u5316\/\u8131\u9502\u8fc7\u7a0b\u8fdb\u884c\u4e86\u73b0\u573a\u76d1\u6d4b\u3002\u56fe2a\u663e\u793a\u4e86\u4ee5\u9502\u4e3aCE\u7684\u57fa\u4e8eLGPS\u7684ASSLMB\u4e2dIn\u9633\u6781\u7684\u5178\u578b\u5faa\u73af\u4f0f\u5b89\u56fe\uff08CV\uff09\uff0c\u5176\u4e2d\u7535\u538b\u8303\u56f4\u4e3a\u22120.1\u81f33 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in All-Solid-State Alloy-Metal Batteries: Regulating Homogeneous Lithium Precipitation and Flexible Solid Electrolyte Interphase Evolution,\u00a0<strong><em><b><i>J. Am. Chem. Soc.<\/i><\/b><\/em><\/strong>\u00a02020. 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