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\"\"<\/p>\n

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\u674e\u707f\u9662\u58eb\u5df2\u53d1\u8868800\u591a\u7bc7\u8bba\u6587\uff0c\u7ea632,000\u6b21\u5f15\u7528\uff0c\u7ea680\u9879\u6388\u6743\u4e13\u5229\u4ee5\u53ca\u5728\u56fd\u9645\u4f1a\u8bae\u4e0a\u8d85\u8fc7100\u6b21\u4e3b\u9898\u62a5\u544a\u3002\u5728\u4ed6\u7684\u6307\u5bfc\u4e0b\uff0c\u8d85\u8fc7150\u540d\u7814\u7a76\u751f\u83b7\u5f97\u4e86\u535a\u58eb\u5b66\u4f4d\u3002<\/p>\n

\u53d1\u8868\u6210\u679c\u4e00\u89c8<\/b><\/strong><\/p>\n

\u4e00\u3001\u5149\u50ac\u5316\u6c34\u5206\u89e3<\/b><\/strong><\/p>\n

(1) Angew:\u8868\u9762\u6781\u6027\u8bf1\u5bfc\u7684\u7a7a\u95f4\u7535\u8377\u5206\u79bb\u4fc3\u8fdbGaN\u7eb3\u7c73\u68d2\u9635\u5217\u4e0a\u7684\u5149\u50ac\u5316\u5168\u6c34\u89e3<\/strong><\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.201912844<\/p>\n

(2) Nature communications:<\/b><\/strong>\u00a0<\/b><\/strong>\u68af\u5ea6\u94bd\u63ba\u6742\u7684\u8d64\u94c1\u77ff\u540c\u8d28\u7ed3\u5149\u7535\u9633\u6781\u53ef\u540c\u65f6\u6539\u5584\u5149\u50ac\u5316\u6c34\u5206\u89e3\u7684\u5149\u7535\u6d41\u548c\u5f00\u542f\u7535\u538b<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1038\/s41467-020-18484-8<\/p>\n

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\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1039\/C9EE02247C<\/u><\/a><\/p>\n

\u4e09\u3001C<\/b><\/strong>O<\/b><\/strong>2<\/b><\/sub><\/strong>\u52a0\u6c22\u5236\u7532\u9187<\/b><\/strong><\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1016\/j.jcat.2020.06.018<\/p>\n

\u56db\u3001\u5149\/\u7535\u50ac\u5316CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f<\/b><\/strong><\/p>\n

(1) Nature communications:<\/b><\/strong>\u00a0\u76f4\u63a5\u548c\u95f4\u63a5Z\u578b\u5f02\u8d28\u7ed3\u6784\u8026\u5408\u5149\u7cfb\u7edf\uff0c\u53ef\u5b9e\u73b0CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f\u548cH<\/b><\/strong>2<\/b><\/sub><\/strong>O\u6c27\u5316<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u5927\u8fde\u5316\u7269\u6240\u674e\u707f\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u901a\u8fc7\u63a7\u5236\u5149\u6c89\u79ef\u6784\u5efa\u4e86Cu2<\/sub>O-Pt\/SiC\/IrOx<\/sub>\u590d\u5408\u6750\u6599\u7136\u540e\u4ee5Nafion\u819c\u5c06\u8fd8\u539f\u548c\u6c27\u5316\u534a\u53cd\u5e94\u5206\u9694\u5f00\u3002\u8be5\u4eba\u9020\u7cfb\u7edf\u5728\u53ef\u89c1\u5149\u7167\u5c04\u4e0b\u5177\u6709\u51fa\u8272\u7684\u5149\u50ac\u5316\u6027\u80fd\uff0c\u53ef\u5c06CO2<\/sub>\u8fd8\u539f\u4e3aHCOOH\uff0c\u5e76\u5c06H2<\/sub>O\u6c27\u5316\u4e3aO2<\/sub>\u3002HCOOH\u548cO2<\/sub>\u7684\u4ea7\u7387\u51e0\u4e4e\u8fbe\u5230\u5316\u5b66\u8ba1\u91cf\u6bd4\uff0c\u5206\u522b\u9ad8\u8fbe896.7\u548c440.7 \u03bcmol\u00b7g-1<\/sup>h-1<\/sup>\u3002\u4eba\u9020\u7cfb\u7edf\u4e2dCO2<\/sub>\u8fd8\u539f\u548cH2<\/sub>O\u6c27\u5316\u7684\u9ad8\u6548\u7387\u5f52\u56e0\u4e8eCu2<\/sub>O-Pt\/SiC\/IrOx<\/sub>\u7684\u76f4\u63a5Z\u578b\u7535\u5b50\u7ed3\u6784\u4ee5\u53ca\u95f4\u63a5Z\u578b\u5206\u79bb\u7684\u8fd8\u539f\u548c\u6c27\u5316\u5355\u5143\uff0c\u4ece\u800c\u5927\u5927\u5ef6\u957f\u4e86\u5149\u751f\u7535\u5b50\u548c\u7a7a\u7a74\u7684\u5bff\u547d\uff0c\u5e76\u9632\u6b62\u4e86\u4ea7\u7269\u7684\u540e\u53cd\u5e94\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u63d0\u9ad8\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u7684\u6548\u7387\u63d0\u4f9b\u4e86\u6709\u6548\u53ef\u884c\u7684\u7b56\u7565\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1038\/s41467-020-16742-3<\/u><\/a><\/p>\n

(2) Applied Catalysis B: Environmental:<\/b><\/strong>\u00a0\u5d4c\u5165\u8fc7\u6e21\u91d1\u5c5e\u7684\u6c2e\u5316\u78b3\u7528\u4e8e\u9009\u62e9\u6027\u7535\u50ac\u5316\u8fd8\u539fCO<\/b><\/strong>2<\/b><\/sub><\/strong><\/p>\n

\"\"<\/p>\n

\u9ad8\u6548CO2<\/sub>\u8fd8\u539f\u50ac\u5316\u5242\u7684\u5f00\u53d1\u5bf9\u4e8e\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u662f\u4e00\u4e2a\u6311\u6218\u3002\u9274\u4e8e\u6b64\uff0c\u5927\u8fde\u5316\u7269\u6240\u674e\u707f\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u62a5\u9053\u4e86\u5d4c\u5165\u8fc7\u6e21\u91d1\u5c5e\u7684\u77f3\u58a8\u6c2e\u5316\u78b3\uff08g-C3<\/sub>N4<\/sub>\uff09\uff0c\u53ef\u4ee5\u4f5c\u4e3a\u6c34\u6027\u73af\u5883\u4e2d\u4e00\u7c7b\u65b0\u7684CO2<\/sub>\u8fd8\u539f\u50ac\u5316\u5242\u3002\u7531\u4e8e\u91d1\u5c5e\u7684\u534f\u540c\u4f5c\u7528\uff0c\u53d1\u73b0\u53cc\u91d1\u5c5e\uff08NiMn\u6216NiCu\uff09-C3<\/sub>N4<\/sub>\u50ac\u5316\u5242\u6bd4\u5355\u91d1\u5c5e\u50ac\u5316\u5242\u66f4\u6709\u6548\uff0c\u5728\u5f88\u5bbd\u7684\u7535\u4f4d\u8303\u56f4\uff08-0.6 V\u81f3-0.9 V\uff09\u4e0b\uff0c0.39 V\u7684\u4f4e\u8d85\u7535\u52bf\u4e0b\u4ea7\u751fCO\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u4e3a90\uff05\u5de6\u53f3\u3002\u9ad8\u6d3b\u6027\u6e90\u81eag-C3<\/sub>N4<\/sub>\u57fa\u8d28\u5bf9\u91d1\u5c5e\u539f\u5b50\u7684\u539f\u5b50\u4fee\u9970\u3002g-C3<\/sub>N4<\/sub>\u4e0d\u4ec5\u5145\u5f53\u914d\u4f4d\u6846\u67b6\uff0c\u800c\u4e14\u4e3aCO2<\/sub>\u8fd8\u539f\u63d0\u4f9b\u4e86\u826f\u597d\u7684\u5c40\u90e8\u73af\u5883\u3002\u672c\u7814\u7a76\u6709\u52a9\u4e8e\u6211\u4eec\u5bf9\u8fd9\u79cd\u6750\u6599\u7684\u7ed3\u6784\u548c\u6d3b\u6027\u8d8b\u52bf\u7684\u7406\u89e3\uff0c\u5e76\u6307\u51fa\u5408\u7406\u8bbe\u8ba1\u66f4\u6709\u6548\u7684CO2<\/sub>\u8fd8\u539f\u50ac\u5316\u5242\u7684\u7b56\u7565\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1016\/j.apcatb.2019.118391<\/p>\n

\u4e94\u3001\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60<\/b><\/strong><\/p>\n

AEM:<\/b><\/strong>\u00a0H-\u952e\u8f85\u52a9\u7684\u975e\u5bcc\u52d2\u70ef\u53d7\u4f53\u7684\u5206\u5b50\u987a\u5e8f\u8c03\u63a7\uff0c\u7528\u4e8e\u9ad8\u6548\u7684\u975e\u9000\u706b\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/aenm.201903650<\/p>\n

\"\"<\/p>\n

\u5f20\u6d9b\uff0c1963\u5e74\u751f\u4e8e\u9655\u897f\u5b89\u5eb7\u3002\u4e2d\u5171\u515a\u5458\uff0c\u535a\u58eb\uff0c\u7814\u7a76\u5458\u30022013\u5e74\u5f53\u9009\u4e3a\u4e2d\u56fd\u79d1\u5b66\u9662\u9662\u58eb\u3002<\/p>\n

1989\u5e74\u5728\u4e2d\u56fd\u79d1\u5b66\u9662\u5927\u8fde\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u83b7\u535a\u58eb\u5b66\u4f4d\uff0c1989\u5e74\u81f31990\u5e74\u5728\u82f1\u56fd\u4f2f\u660e\u7ff0\u5927\u5b66\u505a\u8bbf\u95ee\u5b66\u8005\uff0c\u56de\u56fd\u540e\uff0c\u5386\u4efb\u5927\u8fde\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u7814\u7a76\u7ec4\u526f\u7ec4\u957f\u3001\u7ec4\u957f\u3001\u5ba4\u4e3b\u4efb\u3001\u526f\u6240\u957f\u3001\u515a\u59d4\u4e66\u8bb0\u7b49\u804c\u52a1\uff0c\u66fe\u517c\u4efb\u56fd\u5bb6\u50ac\u5316\u5de5\u7a0b\u6280\u672f\u7814\u7a76\u4e2d\u5fc3\u4e3b\u4efb\uff0c2007\u5e742\u6708\u81f32017\u5e742\u6708\u4efb\u5927\u8fde\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u6240\u957f\u3002\u957f\u671f\u4ece\u4e8b\u5316\u5b66\u5316\u5de5\u9886\u57df\u7684\u7814\u7a76\uff0c\u8d1f\u8d23\u7814\u5236\u7684\u65b0\u578b\u50ac\u5316\u5242\u5e7f\u6cdb\u5e94\u7528\u4e8e\u6211\u77f3\u6cb9\u5316\u5de5\u7b49\u9886\u57df\uff0c\u4e09\u6b21\u4ee5\u7b2c\u4e00\u5b8c\u6210\u4eba\u83b7\u56fd\u5bb6\u6280\u672f\u53d1\u660e\u4e8c\u7b49\u5956\u3002\u8fd1\u671f\u4e3b\u8981\u4ece\u4e8b\u65e0\u6bd2\u63a8\u8fdb\u5242\u50ac\u5316\u5206\u89e3\u6280\u672f\u3001\u751f\u7269\u8d28\u50ac\u5316\u8f6c\u5316\u3001\u5355\u539f\u5b50\u50ac\u5316\u548c\u7eb3\u7c73\u50ac\u5316\u7b49\u65b9\u9762\u7684\u7814\u7a76\uff1b\u6240\u7387\u9886\u7684\u56e2\u961f\u5728\u56fd\u9645\u4e0a\u9996\u6b21\u53d1\u73b0\u7ea4\u7ef4\u7d20\u4e00\u6b65\u6cd5\u50ac\u5316\u8f6c\u5316\u5236\u4e59\u4e8c\u9187\u7684\u65b0\u53cd\u5e94\uff1b\u7387\u5148\u63d0\u51fa\u201c\u5355\u539f\u5b50\u50ac\u5316(Single-Atom Catalysis)\u201d\u7684\u6982\u5ff5\uff0c\u5df2\u5728\u56fd\u9645\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587\u56db\u767e\u4f59\u7bc7\uff0c\u7533\u8bf7\u53d1\u660e\u4e13\u5229\u4e24\u767e\u4f59\u4ef6\u3002<\/p>\n

\u4e00\u3001<\/b><\/strong>\u5355\u539f\u5b50\u5927\u89c4\u6a21\u5408\u6210<\/b><\/strong><\/p>\n

Nature communications: \u5f3a\u91d1\u5c5e-\u8f7d\u4f53\u76f8\u4e92\u4f5c\u7528\u4fc3\u8fdb\u5927\u89c4\u6a21\u751f\u4ea7\u70ed\u7a33\u5b9a<\/b><\/strong>\u6027<\/b><\/strong>\u5355\u539f\u5b50\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u5355\u539f\u5b50\u50ac\u5316\u5242\uff08SAC\uff09\u5728\u8bb8\u591a\u5f02\u76f8\u53cd\u5e94\u4e2d\u5747\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u50ac\u5316\u6027\u80fd\u3002\u7136\u800c\uff0c\u4ee5\u7b80\u5355\u4e14\u5927\u89c4\u6a21\u7684\u5236\u5907\u70ed\u7a33\u5b9a\u7684SAC\u4ecd\u7136\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002\u9274\u4e8e\u6b64\uff0c\u5f20\u6d9b\u9662\u58eb\u56e2\u961f\u7b49\u4eba<\/b><\/strong>\u62a5\u9053\u4e86\u901a\u8fc7\u5c06\u4e9a\u5fae\u7c73RuO2<\/sub>\u805a\u96c6\u4f53\u4e0eMgAl1.2<\/sub>Fe0.8<\/sub>O4<\/sub>\u5c16\u6676\u77f3\u8fdb\u884c\u7269\u7406\u6df7\u5408\uff0c\u4ece\u5546\u4e1aRuO2<\/sub>\u7c89\u672b\u5408\u6210Ru SAC\u3002\u901a\u8fc7\u7403\u5dee\u6821\u6b63\u626b\u63cf\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u548cX\u5c04\u7ebf\u5438\u6536\u5149\u8c31\u786e\u8ba4\u4e86\u539f\u5b50\u5206\u6563\u7684Ru\u3002\u8be6\u7ec6\u7684\u7814\u7a76\u8868\u660e\uff0c\u5206\u6563\u8fc7\u7a0b\u4e0d\u662f\u7531\u6c14\u4f53\u539f\u5b50\u7684\u6355\u83b7\u673a\u5236\u5f15\u8d77\u7684\uff0c\u800c\u662f\u7531\u5f3a\u5171\u4ef7\u91d1\u5c5e-\u8f7d\u4f53\u76f8\u4e92\u4f5c\u7528\u4fc3\u8fdb\u7684\u53cd\u5965\u65af\u7279\u74e6\u5c14\u5fb7\u719f\u5316\u3002\u8fd9\u79cd\u5408\u6210\u7b56\u7565\u7b80\u5355\u6613\u884c\uff0c\u9002\u5408\u5927\u89c4\u6a21\u751f\u4ea7\u7528\u4e8e\u5de5\u4e1a\u5e94\u7528\u7684\u70ed\u7a33\u5b9aSAC\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1038\/s41467-020-14984-9<\/u><\/a><\/p>\n

\u4e8c\u3001CH<\/b><\/strong>4<\/b><\/sub><\/strong>\u71c3\u70e7\u53cd\u5e94<\/b><\/strong><\/p>\n

Angew: \u6c34\u70ed\u7a33\u5b9a\u7684\u4e0d\u53ef\u8fd8\u539f\u6c27\u5316\u7269\u6539\u6027\u7684Pd\/MgAl<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>4<\/b><\/sub><\/strong>\u7532\u70f7\u71c3\u70e7\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.202009050<\/u><\/a>.<\/p>\n

\u4e09\u3001\u6c34\u7164\u6c14\u8f6c\u6362\u53cd\u5e94<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.201914867<\/p>\n

\u56db\u3001\u5149\u70ed\u50ac\u5316\u53cd\u5e94<\/b><\/strong><\/p>\n

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\"\"<\/b><\/strong><\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.202001701<\/u><\/a><\/p>\n

\u4e94\u3001\u751f\u7269\u8d28\u50ac\u5316\u8f6c\u5316<\/b><\/strong><\/p>\n

Green Chemistry: \u6e29\u548c\u6761\u4ef6\u4e0b\u5728\u56fa\u5b9a\u5e8a\u7cfb\u7edf\u4e2d\u7531\u7ce0\u919b\u50ac\u5316\u751f\u4ea71,4-\u620a\u4e8c\u9187<\/b><\/strong><\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1039\/D0GC00233J<\/p>\n

\u516d\u3001CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u52a0\u6c22\u5236\u7532\u9187<\/b><\/strong><\/p>\n

Chem Soc Rev: CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u52a0\u6c22\u5408\u6210\u7532\u9187\u7684\u73b0\u6709\u6280\u672f\u548c\u89c2\u70b9<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1039\/C9CS00614A<\/u><\/a><\/p>\n

\"\"<\/p>\n

\u674e\u4e9a\u680b\uff0c1964\u5e7411\u6708\u751f\u4e8e\u5b89\u5fbd\u7701\u5bbf\u677e\u53bf\u30021986\u5e74\u6bd5\u4e1a\u4e8e\u5b89\u5fbd\u5e08\u8303\u5927\u5b66\u5316\u5b66\u7cfb\uff0c1991\u5e74\u30011998\u5e74\u5148\u540e\u83b7\u7855\u58eb\u3001\u535a\u58eb\u5b66\u4f4d\u3002\u6e05\u534e\u5927\u5b66\u5316\u5b66\u7cfb\u6559\u6388\u3002\u66fe\u5148\u540e\u4e8e2001\u5e74\u30012008\u5e74\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u5956\u4e8c\u7b49\u5956\u30022011\u5e74\u5f53\u9009\u4e3a\u4e2d\u56fd\u79d1\u5b66\u9662\u9662\u58eb\uff0c2014\u5e74\u5f53\u9009\u53d1\u5c55\u4e2d\u56fd\u5bb6\u79d1\u5b66\u9662\u9662\u58eb\u3002\u4e3b\u8981\u4ece\u4e8b\u65e0\u673a\u7eb3\u7c73\u6750\u6599\u5408\u6210\u5316\u5b66\u7814\u7a76\uff0c\u76ee\u524d\u81f4\u529b\u4e8e\u6311\u6218\u91d1\u5c5e\u56e2\u7c07\u3001\u5355\u539f\u5b50\u50ac\u5316\u5242\u4ee5\u671f\u5b9e\u73b0\u975e\u8d35\u91d1\u5c5e\u66ff\u4ee3\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u3001\u63a2\u7d22\u5b9e\u73b0\u50ac\u5316\u65b0\u53cd\u5e94\uff0c\u89e3\u51b3\u50ac\u5316\u5242\u5747\u76f8\u50ac\u5316\u5f02\u9879\u5316\u5b9e\u9a8c\u5ba4\u4e0e\u5de5\u4e1a\u5316\u6280\u672f\u96be\u9898\u3002\u5728\u56fd\u9645\u5b66\u672f\u671f\u520a\u5305\u62ecScience, Nature\uff08\u53ca\u5176\u5b50\u520a\uff09\uff0cJACS, Angew, Chem, PRL, Adv Mater., Nano Letters\u7b49\u53d1\u8868\u5b66\u672f\u8bba\u6587300\u4f59\u7bc7\uff0c\u88ab\u4ed6\u5f15\u8d8540000\u6b21\uff08H-index \u8d85100\uff09\u3002\u5df2\u5148\u540e\u57f9\u517b\u535a\u58eb\u751f\u3001\u535a\u58eb\u540e\u9ad8\u7ea7\u7814\u7a76\u4eba\u545830\u4f59\u540d\uff0c1\u4eba\u83b7\u56fd\u9645\u201cIUPAC\u9752\u5e74\u5316\u5b66\u5bb6\u5956\u201d\uff082005\u5e74\uff09\uff0c4\u4eba\u83b7\u5f97\u201c\u5168\u56fd\u4f18\u79c0\u535a\u58eb\u5b66\u4f4d\u8bba\u6587\u5956\u201d\uff082\u4eba\u83b7\u63d0\u540d\uff09\uff0c6\u4eba\u5df2\u83b7\u5f97\u201c\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u201d\u8d44\u52a9\uff0c8\u4eba\u83b7\u201c\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u201d\u7b49\u4eba\u624d\u79f0\u53f7\u3002<\/p>\n

\u4e00<\/b><\/strong>\u3001<\/b><\/strong>\u5355\u539f\u5b50<\/b><\/strong>\u7535\u50ac\u5316\u6c27\u8fd8\u539fORR<\/b><\/strong><\/p>\n

JACS: \u5177\u6709\u589e\u5f3a\u7684\u8fc7\u6c27\u5316\u6c22\u8010\u53d7\u6027\u7684\u5355\u539f\u5b50Co-N<\/b><\/strong>4<\/b><\/sub><\/strong>\u7535\u50ac\u5316\u5242\u53ef\u5b9e\u73b0\u56db\u7535\u5b50\u6c27\u8fd8\u539f\uff0c\u4ece\u800c\u5b9e\u73b0\u9009\u62e9\u6027\u4f20\u611f<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u56db\u7535\u5b50\u6c27\u8fd8\u539f\u53cd\u5e94\uff08ORR\uff09\u4e3a\u7535\u50ac\u5316\u80fd\u91cf\u8f6c\u6362\uff0c\u5b58\u50a8\u548c\u6c27\u76d1\u6d4b\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u524d\u9014\u7684\u65b9\u6cd5\u3002\u7136\u800c\uff0c\u5728\u5927\u591a\u6570\u4f7f\u7528\u7684\u50ac\u5316\u5242\u4e0a\uff0c\u603b\u4f34\u968f\u7740\u8fc7\u6c27\u5316\u6c22\uff08H2<\/sub>O2<\/sub>\uff09\u7684\u8fd8\u539f\uff0c\u8fd9\u964d\u4f4e\u4e86\u7535\u50ac\u5316\u9009\u62e9\u6027\u3002\u56e0\u6b64\uff0c\u674e\u4e9a\u680b\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u62a5\u9053\u4e86\u5728\u4e2d\u6027\u4ecb\u8d28\u4e2d\u5177\u67090.62 V\uff08vs RHE\uff09\u7684\u8d77\u59cb\u7535\u52bf\u7684\u56db\u7535\u5b50ORR\u7684\u5355\u539f\u5b50Co-N4<\/sub>\u7535\u50ac\u5316\u5242\uff0c\u540c\u65f6\u5177\u6709\u8f83\u9ad8\u7684H2<\/sub>O2<\/sub>\u8010\u53d7\u6027\uff0c\u4f18\u4e8e\u5546\u7528Pt\u7535\u50ac\u5316\u5242\u3002\u7535\u5316\u5b66\u52a8\u529b\u5b66\u5206\u6790\u8bc1\u5b9e\uff0cCo-N4<\/sub>\u50ac\u5316\u4f4d\u70b9\u4e3b\u8981\u4fc3\u8fdbORR\u7684\u76f4\u63a5\u56db\u7535\u5b50\u9014\u5f84\uff0c\u800c\u4e0d\u662f\u4ee5H2<\/sub>O2<\/sub>\u4e3a\u4e2d\u95f4\u7269\u79cd\u7684\u4e24\u4e2a\u8fde\u7eed\u7684\u4e24\u7535\u5b50\u8fd8\u539f\u9014\u5f84\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0cH2<\/sub>O2<\/sub>\u7684\u8fd8\u539f\u53d7\u5230H2<\/sub>O2<\/sub>\u5728\u535f\u5549Co\u4f4d\u70b9\u4e0a\u7684\u5f31\u5438\u9644\u7684\u963b\u788d\u3002\u8fd9\u4f7f\u7535\u50ac\u5316\u5242\u5177\u6709\u66f4\u597d\u7684\u6297H2<\/sub>O2<\/sub>\u7535\u6d41\u5e72\u6270\u7684\u80fd\u529b\uff0c\u4ece\u800c\u5b9e\u73b0\u4e86\u9ad8\u9009\u62e9\u6027\u7684O2<\/sub>\u4f20\u611f\u68c0\u6d4b\u3002\u8be5\u7814\u7a76\u8868\u660e\uff0c\u9ad8\u5bb9\u91cf\u7684\u5355\u539f\u5b50\u50ac\u5316\u5242\u5177\u6709\u8c03\u63a7\u91d1\u5c5e-\u5438\u9644\u7269\u76f8\u4e92\u4f5c\u7528\u7684\u4f18\u52bf\uff0c\u4ece\u800c\u62d3\u5bbd\u4e86\u5176\u5728\u73af\u5883\u548c\u5bff\u547d\u76d1\u6d4b\u4e2d\u7684\u5e94\u7528\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1021\/jacs.0c07790<\/a><\/p>\n

\u4e8c<\/b><\/strong>\u3001\u5355\u539f\u5b50\u7535\u50ac\u5316CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f<\/b><\/strong><\/p>\n

Angew: \u901a\u8fc7\u70ed\u8f6c\u6362\u548c\u8868\u9762\u91cd\u6784\u5408\u6210\u7528\u4e8e\u9ad8\u6548\u7535\u5316\u5b66\u8fd8\u539fCO<\/b><\/strong>2<\/b><\/sub><\/strong>\u7684Ag\u5355\u539f\u5b50\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u6e05\u534e\u5927\u5b66\u738b\u5b9a\u80dc\u548c\u674e\u4e9a\u680b\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u62a5\u9053\u4e86\u4e00\u79cdAg1<\/sub>\u5355\u539f\u5b50\u50ac\u5316\u5242\uff08Ag1<\/sub>\/MnO2<\/sub>\uff09\uff0c\u8be5\u50ac\u5316\u5242\u662f\u901a\u8fc7Ag\u7eb3\u7c73\u9897\u7c92\uff08NPs\uff09\u7684\u70ed\u8f6c\u6362\u548cMnO2<\/sub>\u7684\u8868\u9762\u91cd\u6784\u5408\u6210\u7684\u3002\u901a\u8fc7\u539f\u4f4dETEM\uff0c\u539f\u4f4dXRD\u548cDFT\u8ba1\u7b97\u63ed\u793a\u4e86\u94f6\u7eb3\u7c73\u9897\u7c92\u5411\u5355\u539f\u5b50\u7684\u6f14\u5316\u8fc7\u7a0b\u3002MnO2<\/sub>\u7684\u70ed\u5904\u7406\u548c\u8868\u9762\u91cd\u6784\u662f\u5f62\u6210Ag\u5355\u539f\u5b50\u7684\u9a71\u52a8\u529b\u3002\u6240\u83b7\u5f97\u7684Ag1<\/sub>\/MnO2<\/sub>\u5728-0.85 V vs. RHE\u65f6\u8fbe\u5230\u4e8695.7\uff05\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff0c\u5e76\u4e14\u5177\u6709\u7535\u5316\u5b66CO2<\/sub>\u8fd8\u539f\u53cd\u5e94\uff08CO2<\/sub>RR\uff09\u7684\u957f\u671f\u7a33\u5b9a\u6027\u3002DFT\u8ba1\u7b97\u8868\u660e\uff0c\u5355\u4e2aAg\u4f4d\u70b9\u5177\u6709\u63a5\u8fd1\u8d39\u7c73\u80fd\u7ea7\u7684\u9ad8\u7535\u5b50\u5bc6\u5ea6\uff0c\u5e76\u4e14\u53ef\u4ee5\u5145\u5f53CO2<\/sub>RR\u4e2d\u552f\u4e00\u7684\u6d3b\u6027\u4f4d\u70b9\u3002\u7ed3\u679c\uff0cAg1<\/sub>\/MnO2<\/sub>\u50ac\u5316\u5242\u8868\u73b0\u51fa\u4e86\u51fa\u8272\u7684CO2<\/sub>RR\u6027\u80fd\uff0c\u8fdc\u8fdc\u8d85\u8fc7\u4e86\u4f20\u7edf\u7684Ag\u7eb3\u7c73\u50ac\u5316\u5242\uff08AgNP \/ MnO2<\/sub>\uff09\u548c\u5176\u4ed6\u5df2\u62a5\u9053\u7684\u57fa\u4e8eAg\u7684\u50ac\u5316\u5242\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.202014718<\/p>\n

\u4e09<\/b><\/strong>\u3001\u5355\u539f\u5b50\u7535\u50ac\u5316\u7532\u9178\u6c27\u5316<\/b><\/strong><\/p>\n

\uff081\uff09<\/b><\/strong>Nature Chemistry\uff1a\u901a\u7528\u4e3b\u5ba2\u4f53\u7b56\u7565\u5408\u6210\u6c2e\u63ba\u6742\u78b3\u8d1f\u8f7d\u94f1\u5355\u539f\u5b50\u50ac\u5316\u5242\u7528\u4e8e\u7532\u9178\u6c27\u5316<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u5355\u539f\u5b50\u50ac\u5316\u5242\u4e0d\u4ec5\u53ef\u4ee5\u6700\u5927\u7a0b\u5ea6\u5730\u63d0\u9ad8\u91d1\u5c5e\u539f\u5b50\u6548\u7387\uff0c\u800c\u4e14\u8fd8\u663e\u793a\u51fa\u4e0e\u5e38\u89c4\u7eb3\u7c73\u7c92\u5b50\u76f8\u5f53\u7684\u7279\u6027\uff0c\u8fd9\u4f7f\u5176\u6210\u4e3a\u4e00\u79cd\u6709\u524d\u9014\u7684\u7814\u7a76\u6750\u6599\u3002\u9274\u4e8e\u6b64\uff0c\u674e\u4e9a\u680b\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u5f00\u53d1\u4e86\u4e00\u79cd\u901a\u7528\u7684\u4e3b\u5ba2\u4f53\u7b56\u7565\uff0c\u53ef\u4ee5\u5728\u6c2e\u63ba\u6742\u78b3\uff08M1<\/sub>\/CN\uff0cM = Pt\uff0cIr\uff0cPd\uff0cRu\uff0cMo\uff0cGa\uff0cCu\uff0cNi\uff0cMn\uff09\u4e0a\u5236\u5907\u5404\u79cd\u91d1\u5c5e\u5355\u539f\u5b50\u50ac\u5316\u5242\u3002\u94f1Ir1<\/sub>\/CN\u7535\u50ac\u5316\u7532\u9178\u6c27\u5316\u7684\u8d28\u91cf\u6d3b\u6027\u4e3a12.9 Amg-1<\/sup>Ir<\/sub>\u53cd\u5e94\uff0c\u800cIr\/C\u7eb3\u7c73\u7c92\u5b50\u50ac\u5316\u5242\u51e0\u4e4e\u662f\u60f0\u6027\u7684\uff08\u301c4.8\u00d710-3<\/sup>\u00a0Amg-1<\/sup>Ir<\/sub>\uff09\u3002Ir1<\/sub>\/CN\u7684\u6d3b\u6027\u4e5f\u5206\u522b\u662fPd\/C\u548cPt\/C\u768416\u548c19\u500d\u3002\u6b64\u5916\uff0cIr1<\/sub>\/CN\u8868\u73b0\u51fa\u5bf9CO\u4e2d\u6bd2\u9ad8\u7684\u8010\u53d7\u6027\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u76f8\u5bf9\u4e8e\u5e38\u89c4\u94f1\u7eb3\u7c73\u7c92\u5b50\u50ac\u5316\u5242\u800c\u8a00\uff0cIr1<\/sub>\/CN\u7684\u6027\u8d28\u6e90\u4e8e\u5b64\u7acb\u7684\u94f1\u5355\u4f4d\u70b9\u8c03\u63a7\u4e86\u7535\u5b50\u7ed3\u6784\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41557-020-0473-9<\/u><\/a><\/p>\n

\uff082\uff09Nature Nanotechnology\uff1a\u5355\u539f\u5b50\u94d1\/\u6c2e\u63ba\u6742\u78b3\u7535\u50ac\u5316\u5242\u7528\u4e8e\u7532\u9178\u6c27\u5316<\/strong><\/p>\n

\"\"<\/p>\n

\u4e3a\u4e86\u6ee1\u8db3\u6f5c\u5728\u5e94\u7528\u7684\u8981\u6c42\uff0c\u63a2\u7d22\u5177\u6709\u8d85\u9ad8\u8d28\u91cf\u6d3b\u6027\u548c\u6297CO\u7684\u65b0\u7684\u7532\u9178\u6c27\u5316\u50ac\u5316\u5242\u975e\u5e38\u91cd\u8981\u3002\u56e0\u6b64\uff0c\u6e05\u534e\u5927\u5b66\u674e\u4e9a\u680b\u9662\u58eb\uff0c\u738b\u5b9a\u80dc\u6559\u6388\u7b49\u4eba<\/b><\/strong>\u6210\u529f\u5730\u5728N\u63ba\u6742\u78b3\uff08SA-Rh\/CN\uff09\u4e0a\u5408\u6210\u4e86\u539f\u5b50\u5206\u6563\u7684Rh\uff0c\u5e76\u53d1\u73b0SA-Rh\/CN\u5bf9\u7532\u9178\u6c27\u5316\u8868\u73b0\u51fa\u6709\u5e0c\u671b\u7684\u7535\u50ac\u5316\u6027\u80fd\u3002\u5c3d\u7ba1Rh\/C\u7684\u6d3b\u6027\u8f83\u4f4e\uff0c\u4f46\u4e0e\u73b0\u6709\u7684Pd\/C\u548cPt\/C\u76f8\u6bd4\uff0c\u5176\u8d28\u91cf\u6d3b\u6027\u5206\u522b\u63d0\u9ad8\u4e8628\u500d\u548c67\u500d\u3002\u6709\u8da3\u7684\u662f\uff0cSA-Rh\/CN\u5bf9CO\u4e2d\u6bd2\u7684\u8010\u53d7\u6027\u5927\u5927\u589e\u5f3a\uff0c\u5e76\u4e14SA-Rh\/CN\u4e2d\u7684Rh\u539f\u5b50\u7ecf\u8fc7\u957f\u671f\u6d4b\u8bd5\u540e\u4ecd\u80fd\u62b5\u6297\u70e7\u7ed3\uff0c\u4ece\u800c\u5177\u6709\u51fa\u8272\u7684\u50ac\u5316\u7a33\u5b9a\u6027\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u7532\u9178\u76d0\u8def\u7ebf\u5bf9SA-Rh\/CN\u66f4\u6709\u5229\u3002 \u6839\u636e\u8ba1\u7b97\uff0c\u4ea7\u751fCO\u7684\u9ad8\u58c1\u5792\u4ee5\u53ca\u4e0eCO\u7684\u76f8\u5bf9\u4e0d\u5229\u7684\u7ed3\u5408\u5171\u540c\u5bfc\u81f4\u5176\u5bf9CO\u7684\u8010\u53d7\u6027\u3002<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1038\/s41565-020-0665-x<\/p>\n

\u56db\u3001<\/b><\/strong>\u5149\u50ac\u5316CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u8fd8\u539f<\/b><\/strong><\/p>\n

JACS: UiO-66-NH<\/b><\/strong>2<\/b><\/sub><\/strong>\u4e0a\u4fee\u9970\u7684Cu\u5355\u539f\u5b50\u7684\u5149\u8bf1\u5bfc\u4f5c\u7528\uff0c\u4ee5\u589e\u5f3a\u5149\u50ac\u5316\u8fd8\u539fCO<\/b><\/strong>2<\/b><\/sub><\/strong>\u4e3a\u6db2\u6001\u71c3\u6599<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1021\/jacs.0c09599<\/u><\/a><\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1016\/j.nanoen.2020.105467<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/ange.202004966<\/p>\n

\u672c\u6587\u7531\u82d2\u82d2\u7b03\u884c\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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