{"id":214870,"date":"2020-12-23T06:39:15","date_gmt":"2020-12-22T22:39:15","guid":{"rendered":"\/\/m.iemloyee.com\/?p=214870"},"modified":"2020-12-22T20:39:41","modified_gmt":"2020-12-22T12:39:41","slug":"nature-materials%ef%bc%9a%e5%85%b1%e8%bd%ad%e7%a3%ba%e9%85%b0%e8%83%ba%e7%b1%bb%e6%9c%89%e6%9c%ba%e9%94%82%e7%a6%bb%e5%ad%90%e6%ad%a3%e6%9e%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=214870","title":{"rendered":"Nature Materials\uff1a\u5171\u8f6d\u78fa\u9170\u80fa\u7c7b\u6709\u673a\u9502\u79bb\u5b50\u6b63\u6781"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

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\u8fd1\u65e5\uff0c\u6bd4\u5229\u65f6\u9c81\u6c76\u5927\u5b66Alexandru Vlad\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u7c7b\u65b0\u578b\u7684\u5171\u8f6d\u78fa\u9170\u80fa\uff08CSAs\uff09\u6709\u673a\u5316\u5408\u7269\uff0c\u5176\u6269\u5c55\u4e86\u6709\u673a\u9502\u79bb\u5b50\u6b63\u6781\u6750\u6599\u7684\u5316\u5b66\u7a7a\u95f4\u3002\u540c\u65f6\uff0c\u5728\u73af\u5883\u7a7a\u6c14\u4e2d\u5904\u7406\u65f6\uff0c\u78fa\u9170\u57fa\u4e0a\u7684\u7535\u5b50\u79bb\u57df\u4f7f\u6240\u5f97CSAs\u5177\u6709\u56fa\u6709\u7684\u6297\u6c27\u5316\u6027\u548c\u6297\u6c34\u89e3\u6027\uff0c\u5e76\u4e14\u8fd8\u663e\u793a\u51fa\u53ef\u9006\u7684\u7535\u5316\u5b66\u7535\u8377\u5b58\u50a8\u3002\u672a\u8986\u76d6\u7684CSA\u5316\u5b66\u7269\u8d28\u7684\u5f62\u5f0f\u6c27\u5316\u8fd8\u539f\u7535\u52bf\u57282.85 V\u81f33.45 V\u4e4b\u95f4\uff08\u76f8\u5bf9\u4e8eLi+<\/sup>\/Li0<\/sup>\u800c\u8a00\uff09\uff0c\u53ef\u901a\u8fc7\u9759\u7535\u6216\u611f\u5e94\u5206\u5b50\u8bbe\u8ba1\u8fdb\u884c\u5fae\u8c03\u3002\u603b\u4e4b\uff0c\u8fd9\u7c7b\u6709\u673a\u9502\u79bb\u5b50\u6b63\u7535\u6781\u6750\u6599\u6311\u6218\u4e86\u65e0\u673a\u7535\u6c60\u6b63\u6781\u7684\u9886\u57df\uff0c\u56e0\u4e3a\u8fd9\u7b2c\u4e00\u4ee3CSA\u5316\u5b66\u7269\u8d28\u5df2\u663e\u793a\u51fa\u4e0e\u5b9a\u578bLiFePO4<\/sub>\u76f8\u5f53\u7684\u91cd\u91cf\u50a8\u80fd\u6307\u6807\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cConjugated sulfonamides as a class of organic lithium-ion positive electrodes\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Materials<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

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\n \"\"
\n \uff08a\uff09\u9502\u79bb\u5b50\u6280\u672f\u4f9d\u8d56\u4e8e\u5bf9\u73af\u5883\u7a7a\u6c14\u672c\u8d28\u4e0a\u7a33\u5b9a\u7684\u9502\u50a8\u5c42\u6b63\u6781\u548c\u65e0\u9502\u8d1f\u6781\u6750\u6599\uff1b<\/p>\n

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\u56fe\u4e8c\u3001\u6c27\u5316\u8fd8\u539f\u673a\u7406\u5206\u6790<\/strong>
\n \"\"\uff08a\uff09\u5728\u4e8c\u95021, 4-\u4e9a\u82ef\u57fa\u53cc\uff08\uff08\u7532\u78fa\u9170\u57fa\uff09\u9170\u80fa\uff09\u4e2d\u53ef\u9006\u7684\u4e24\u7535\u5b50\u6c27\u5316\u8fd8\u539f\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

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\n \"\"\uff08a-c\uff09\u5f02\u6784\u6548\u5e94\u3001\u5176\u4ed6\u78fa\u9170\u80fa\u57fa\u56e2\u7684\u5f71\u54cd\u548c\u53d6\u4ee3\u57fa\u7535\u5b50\u6548\u5e94\u3002\u4e0a\u6392\uff1a\u5faa\u73af\u4f0f\u5b89\u56fe\uff0c\u57282 mM\u7684\u6d3b\u6027CSA\u30010.1 M LiCl\u5728DMSO\u4e2d\uff0cPt\u5706\u76d8\u5de5\u4f5c\u7535\u6781\u7684\u6d53\u5ea6\u4e3a100 mV s-1<\/sup>\u65f6\u6d4b\u5f97\uff1b\u4e0b\u6392\uff1a\u5728\u56fa\u76f8\u4e2d\u4ee55 h\u6216C\/10\u4e2d\u4e00\u4e2aLi+<\/sup>\uff08e–<\/sup>\uff09\u7684\u901f\u7387\u5728\u56fa\u76f8\u4e2d\u6d4b\u5f97CSA\u7684\u7b2c\u4e00\u5468\u671f\u6052\u5b9a\u7535\u6d41\u7535\u4f4d\u5206\u5e03\u56fe\u3002<\/p>\n

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\"\"<\/p>\n

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\n \"\"\uff08a-d\uff09Li2<\/sub>-p-PDSA\u548cLi4-PTtSA\u7535\u6781\u57281Li+<\/sup>\/5 h\u7684\u5faa\u73af\u901f\u7387\u4e0b\u7684\u7535\u52bf\u7ec4\u6210\u66f2\u7ebf\u548c\u76f8\u5e94\u7684\u5bb9\u91cf\u4fdd\u6301\u7387\uff1b<\/p>\n

\uff08e\uff09\u4ee52Li+<\/sup>\/1 h\u7684\u5faa\u73af\u901f\u7387\u4e0b\u83b7\u5f97\u76842 mg cm-2<\/sup> Li4<\/sub>-PTtSA\/Li\u7535\u6c60\u4f4e\u8d28\u91cf\u8d1f\u8f7d\u7684\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\uff1b<\/p>\n

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\n \"\"\uff08a\uff09\u4f7f\u7528Li4<\/sub>-PTtSA\u4f5c\u4e3a\u4ee3\u8868\u6027CSA\u6b63\u6781\u6750\u6599\uff0cLi4<\/sub>Ti5<\/sub>O12<\/sub>\u30012, 6-\u8418\u4e8c\u7532\u9178\u4e8c\u9502\u3001\u5076\u6c2e\u82ef-4, 4′-\u4e8c\u7fa7\u9178\u9502\u76d0\u548c\u77f3\u58a8\u4f5c\u4e3a\u8d1f\u6781\u6750\u6599\u5206\u522b\u6784\u5efaCSA-LION_1\u3001CSA-LION_2\u3001CSA-LION_3\u548cCSA-LION_4\u539f\u578b\u7535\u6c60\u7684\u539f\u7406\u56fe\u548c\u6c27\u5316\u8fd8\u539f\u8fc7\u7a0b\uff1b<\/p>\n

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\uff08c\uff09\u5177\u6709\u66f4\u9ad8\u8d28\u91cf\u8d1f\u8f7d\uff087 \u03bcg\/cm2<\/sup> Li4<\/sub>-PTtSA\uff09\u7684\u6027\u80fd\u4f18\u5316\u7684CSA-LION_1\u7535\u6c60\u63d0\u9ad8\u4e86\u500d\u7387\u80fd\u529b\uff0c\u5e76\u63d0\u9ad8\u4e862 C\u65f6\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aConjugated sulfonamides as a class of organic lithium-ion positive electrodes<\/a><\/strong>. Nature Materials<\/em>, 2020<\/strong>, DOI: 10.1038\/s41563-020-00869-1.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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