{"id":214319,"date":"2020-12-09T06:10:28","date_gmt":"2020-12-08T22:10:28","guid":{"rendered":"\/\/m.iemloyee.com\/?p=214319"},"modified":"2020-12-08T21:10:40","modified_gmt":"2020-12-08T13:10:40","slug":"nature-energy%ef%bc%9a%e5%85%b7%e6%9c%89%e8%b6%85%e9%ab%98%e6%af%94%e5%8a%9f%e7%8e%87%e7%9a%84%e9%95%81%e7%94%b5%e6%b1%a0%ef%bc%8c%e6%af%94%e7%9b%ae%e5%89%8d%e6%9c%80%e4%bd%b3%e6%80%a7%e8%83%bd","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=214319","title":{"rendered":"Nature Energy\uff1a\u5177\u6709\u8d85\u9ad8\u6bd4\u529f\u7387\u7684\u9541\u7535\u6c60\uff0c\u6bd4\u76ee\u524d\u6700\u4f73\u6027\u80fd\u8fd8\u9ad8\u51fa\u4e24\u4e2a\u6570\u91cf\u7ea7!"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u4f17\u6240\u5468\u77e5\uff0c\u5177\u6709\u9ad8\u4e30\u5bcc\u5ea6\uff0c\u9ad8\u5bb9\u91cf\u548c\u65e0\u679d\u6676\u7684\u9541\u7535\u6c60\u4e00\u76f4\u662f\u9502\u79bb\u5b50\u7535\u6c60\u6f5c\u5728\u7684\u66ff\u4ee3\u54c1\uff0c\u5c06\u6781\u5927\u63d0\u9ad8\u7535\u6c60\u7684\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u3002\u7136\u800c\uff0cMg2+<\/sup>\u9633\u79bb\u5b50\u7684\u9ad8\u79bb\u5b50\u7535\u4f4d\u4f7f\u5b83\u5728\u9634\u6781\u4e2d\u7684\u6269\u6563\u7f13\u6162\u3002\u540c\u65f6\u8fd8\u5e26\u6765\u4e86\u7535\u89e3\u8d28\u4e2d\u5f3a\u79bb\u5b50\u7f14\u5408\u7684\u95ee\u9898\uff0c\u5bfc\u81f4\u6eb6\u5242\u5206\u5b50\u6216\u9634\u79bb\u5b50\u4e0eMg2+<\/sup>\u4e00\u8d77\u63d2\u5165\u9634\u6781\u3002\u6b64\u5916\uff0c\u91d1\u5c5eMg\u7684\u6709\u6548\u5229\u7528\u53d7\u5230\u7535\u89e3\u8d28\u79bb\u5b50\u7535\u5bfc\u7387\u4f4e\u548c\u6c89\u79ef\/\u5265\u79bb\u6548\u7387\u5dee\u7684\u963b\u788d\uff0c\u7279\u522b\u662f\u5728\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u4f7f\u7528\u3002\u7ed3\u679c\u8868\u660e\uff0c\u9541\u7535\u6c60\u5177\u6709\u8f83\u4f4e\u7684\u529f\u7387\u548c\u80fd\u91cf\u6027\u80fd\u3002\u867d\u7136\u4e4b\u524d\u4e00\u4e9b\u7814\u7a76\u62a5\u544a\u4e86Mg\u7535\u6c60\u5177\u6709\u901a\u8fc7\u50a8\u5b58MgCl+<\/sup>\u800c\u4e0d\u662fMg2+<\/sup>\u7684\u5feb\u901f\u52a8\u529b\u5b66\uff0c\u4f46\u8fd9\u5f80\u5f80\u662f\u4ee5\u727a\u7272\u80fd\u91cf\u5bc6\u5ea6\u548c\u5faa\u73af\u5bff\u547d\u4e3a\u4ee3\u4ef7\u7684\u3002\u5c3d\u7ba1\u5230\u76ee\u524d\u4e3a\u6b62\u8fdb\u884c\u4e86\u8bb8\u591a\u52aa\u529b\uff0c\u4f46\u6700\u5148\u8fdb\u7684\u9541\u7535\u6c60\u4ecd\u7136\u4e0d\u80fd\u63d0\u4f9b\u5177\u6709\u5438\u5f15\u529b\u7684\u6027\u80fd\u3002<\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u4f11\u65af\u6566\u5927\u5b66\u59da\u5f66<\/b><\/strong>\u6559\u6388\u548c\u4e30\u7530\u5317\u7f8e\u7814\u7a76\u6240(TRINA) Rana Mohtadi\u6559\u6388<\/b><\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u63d0\u51fa\u4e86\u4e00\u79cd\u53cc\u7ba1\u9f50\u4e0b\u7684\u7b56\u7565\uff0c\u89e3\u51b3\u4e86\u4e00\u76f4\u4ee5\u6765\u9541\u7535\u6c60\u5b9e\u9645\u529f\u7387\u5bc6\u5ea6\u8f83\u4f4e\u7684\u96be\u9898\uff01\u6bd4\u76ee\u524d\u6700\u4f73\u6027\u80fd\u8fd8\u9ad8\u51fa\u4e24\u4e2a\u6570\u91cf\u7ea7\u3002\u4e00\u65b9\u9762\uff0c\u901a\u8fc7\u7ed5\u5f00\u5e38\u89c4Mg\u9634\u6781\u96be\u4ee5\u89e3\u51b3\u7684\u9ad8\u56fa\u6001\u6269\u6563\u52bf\u5792\u96be\u9898\uff0c\u901a\u8fc7\u5f02\u76f8\u70ef\u9187\u5316\u6c27\u5316\u8fd8\u539f\u5316\u5b66\uff08\u4e0d\u53d1\u751f\u952e\u65ad\u88c2\/\u91cd\u65b0\u5f62\u6210\uff09\uff0c\u6765\u5b9e\u73b0\u5feb\u901f\u7684\u6b63\u6781\u6c27\u5316\u8fd8\u539f\u52a8\u529b\u5b66\uff1b\u53e6\u4e00\u65b9\u9762\uff0c\u901a\u8fc7\u5728\u919a\u7c7b\u6df7\u5408\u6eb6\u5242\u4e2d\u4f7f\u7528\u7531\u5f31\u914d\u4f4d\u9634\u79bb\u5b50\u7ec4\u6210\u7684\u7535\u89e3\u8d28\uff0c\u6539\u5584\u7535\u89e3\u6db2\u7684\u79bb\u5b50\u5bfc\u7535\u7387\u548cMg2+<\/sup>\u7684\u8131\u6eb6\u3002\u5177\u4f53\u6765\u8bb2\uff0c\u901a\u8fc7\u5229\u7528\u6709\u673a\u6b63\u6781\u6750\u6599Pyrene-4,5,9,10-\u56db\u916e\uff08PTO\uff09\u4e0e\u6539\u6027\u7684MMC\u7535\u89e3\u8d28\u6eb6\u6db2\uff0c\u5728\u72ec\u7279\u7684\u919a\u6df7\u5408\u7269\u4e2d\u800c\u5177\u6709\u9ad8\u6eb6\u89e3\u5ea6\u7684\u6539\u6027MMC\u7535\u89e3\u8d28\u6eb6\u6db2\u76f8\u7ed3\u5408\u3002\u7ed3\u679c\u8868\u660e\uff0c\u8fd9\u4e24\u79cd\u6750\u6599\u90fd\u8868\u73b0\u51fa\u4e86\u4f18\u5f02\u7684\u6027\u80fd\u3002\u76f8\u5bf9\u4e8eMg2+<\/sup>\/Mg\uff0c\u57282.1 V\u7535\u538b\u4e0b\u6d4b\u8bd5\u7684PTO\u6bd4\u5bb9\u91cf\u4e3a315 mAh g\u2212<\/sup>1<\/sup>\uff0c\u8fd8\u53ef\u4ee5\u572820 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8fdb\u884c\u65e0\u679d\u6676\u7684Mg\u6c89\u79ef\/\u5265\u79bb\u3002\u6b64\u5916\uff0c\u57fa\u4e8e\u8fd9\u79cd\u7b56\u7565\uff0c\u7814\u7a76\u4eba\u5458\u6700\u7ec8\u6240\u5236\u5907\u7684\u9ad8\u529f\u7387\u9541\u7535\u6c60\uff0c\u5176\u5177\u6709\u9ad8\u8fbe20 A g\u2212<\/sup>1<\/sup>\u7684\u5145\u653e\u7535\u529f\u7387\uff0c\u63d0\u4f9b30.4 kW kg\u2212<\/sup>1<\/sup>\u7684\u8d85\u9ad8\u6bd4\u529f\u7387\uff0c\u8fdc\u8d85\u4e8e\u76ee\u524d\u6700\u5148\u8fdb\u7684\u9541\u7535\u6c60\uff080.45 kW kg\u2212<\/sup>1<\/sup>\uff09\u8fd1\u4e24\u4e2a\u6570\u91cf\u7ea7\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cHigh-power Mg batteries enabled by heterogeneous enolization redox chemistry and weakly coordinating electrolytes<\/b><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Energy<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe\u4e00\u3001\u63d0\u51fa\u7684\u9634\u6781\u5f02\u76f8\u70ef\u9187\u5316\u6c27\u5316\u8fd8\u539f\u5316\u5b66<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09\u5177\u6709MMC\/G4\u7684Mg-PTO\u7535\u6c60\u57280.2C\u65f6\u7684\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09\u5c06PTO\u8fd8\u539f\u6210Mg1<\/sub>PTO\u548cMg2<\/sub>PTO\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08c\uff0cd\uff090.5mM PTO\u548cS8<\/sub>\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

\uff08e\uff09\u5177\u6709MMC\/G4\u7684Mg-PTO\u7535\u6c60\u57280.2\u30011\u548c5C\u65f6\u7684\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u4e8c<\/b><\/strong>\u3001\u975e\u5747\u76f8\u70ef\u9187\u5316\u6c27\u5316\u8fd8\u539f\u5316\u5b66\u5bf9\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u9633\u6781\u53ef\u9006\u6027<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09\u8584(~2\u03bcm)\u548c\u8f7b\u8d28(0.48\u00a0mg\u00a0cm–<\/sup>2<\/sup>)GO\u819c\u7684Mg-PTO\u7535\u6c60\u539f\u7406\u56fe\uff1b<\/p>\n

\uff08b\uff09\u7535\u6d41\u5bc6\u5ea6\u4e3a0.2C\u65f6\u5faa\u73af\u7684Mg-PTO\u7535\u6c60\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u5e93\u4ed1\u6548\u7387\uff1b<\/p>\n

\uff08c\uff0cd\uff09\u5728\u539f\u59cb\u7684MMC\/G4\u7535\u89e3\u6db2\u4e2d\uff0c\u5728\u5206\u522b\u542b\u6709Mg1<\/sub>PTO \u548cMgS8<\/sub>\u7684\u60c5\u5f62\u4e0b\u7684\u7535\u538b\u5206\u5e03\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001MMC\/(DME-G2)\u7535\u89e3\u6db2\u7684\u8bbe\u8ba1\u8fc7\u7a0b\u53ca\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09\u57281:1(v\/v)\u6eb6\u5242\u5171\u6df7\u7269\u4e2d\uff0cMMC\u57280.3\u00a0mol\u00a0kg–<\/sup>1<\/sup>\u4e2d\u7684\u6eb6\u89e3\u5ea6\u56fe\uff1b<\/p>\n

\uff08b\uff09MMC\u5728DME\/G2\u6df7\u5408\u7269\u4e2d\u7684\u6eb6\u89e3\u5ea6\u56fe\uff1b<\/p>\n

\uff08c\uff09\u572825\u00b0C\u4e0b\uff0cG4\u548cDME\/G2\u6df7\u5408\u7269\u4e2dMMC\u6eb6\u6db2\u6d53\u5ea6\u548c\u79bb\u5b50\u7535\u5bfc\u7387\u7684\u5173\u7cfb\uff1b<\/p>\n

\uff08d\uff09MMC\/(DME-G2)\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

\uff08e\uff09\u5728\u7535\u6d41\u5bc6\u5ea6\u4ece0.5\u523050 mA cm-2<\/sup>\u65f6\uff0cMg|Cu\u4e0d\u5bf9\u79f0\u7535\u6c60\u7684\u6781\u5316\u66f2\u7ebf\uff1b<\/p>\n

\uff08f\uff09\u572820 mA cm-2<\/sup>\u7684\u6761\u4ef6\u4e0b\uff0c\u5728Cu\u886c\u5e95\u4e0a\u6c89\u79efMg\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08g\uff09\u572820 mA cm-2<\/sup>\u7684\u6761\u4ef6\u4e0b\uff0cMg|Mg\u5bf9\u79f0\u7535\u6c60\u7684\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001Mg-PTO\u5168\u7535\u6c60\u57280.5 mol kg<\/b><\/strong>–<\/b><\/sup><\/strong>1<\/b><\/sup><\/strong>\u00a0<\/b><\/sup><\/strong>MMC\/(DME-G2)\u7535\u89e3\u6db2\u4e2d\u7684\u7535\u5316\u5b66\u884c\u4e3a<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09\u4f7f\u7528CC-CV\u5145\u7535\u548cCC\u653e\u7535\u6a21\u5f0f\uff0cMg-PTO\u7535\u6c60\u57281\u81f350C\u7684\u6761\u4ef6\u4e0b\u7684\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09\u57285C\u6761\u4ef6\u4e0b\u5faa\u73af\u7684\u5305\u542bGO\/GN\u7684Mg-PTO\u7535\u6c60\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u5e93\u4ed1\u6548\u7387\uff1b<\/p>\n

\uff08c\uff09\u4e0e\u62a5\u9053\u7684\u6700\u5148\u8fdbMg\u91d1\u5c5e\u7535\u6c60\u7684\u6bd4\u8f83\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u5f00\u53d1\u4e86\u4e00\u79cd\u9ad8\u529f\u7387Mg\u7535\u6c60\uff0c\u5176\u7279\u70b9\u662f\u91c7\u7528\u6709\u673a\u918c\u6b63\u6781\u4e0e\u57fa\u4e8e\u787c\u56e2\u7c07\u7684\u5f31\u914d\u4f4d\u7535\u89e3\u8d28\uff0c\u975e\u5747\u76f8\u70ef\u9187\u5316\u6c27\u5316\u8fd8\u539f\u5316\u5b66\u662f\u5feb\u901f\u50a8\u5b58Mg2<\/sup>+<\/sup>\u7684\u5173\u952e\uff0c\u5728\u6df7\u5408\u6eb6\u5242\u4e2d\u57fa\u4e8e\u5f31\u914d\u4f4d\u9634\u79bb\u5b50\u7684\u7535\u89e3\u8d28\u6253\u5f00\u4e86\u9ad8\u500d\u7387\u548c\u65e0\u679d\u6676Mg\u6c89\u79ef\u7684\u6f5c\u529b\u3002\u4e3a\u4eca\u540e\u66f4\u597d\u7684\u7269\u7406\/\u5316\u5b66\u6027\u8d28\u548c\u66f4\u597d\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u6253\u4e0b\u4e86\u575a\u5b9e\u7684\u57fa\u7840\uff0c\u540c\u65f6\u672c\u6587\u7684\u7ed3\u679c\u4e3a\u5f00\u53d1\u9ad8\u6027\u80fd\u7684\u9541\u7535\u6c60\u6b63\u6781\u6750\u6599\u548c\u7535\u89e3\u8d28\u6eb6\u6db2\u63d0\u4f9b\u4e86\u65b9\u5411\uff0c\u5e76\u63ed\u793a\u4e86\u4f7f\u7528\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u91d1\u5c5e\u8fdb\u884c\u5feb\u901f\u50a8\u80fd\u7684\u53ef\u80fd\u6027\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/b><\/strong>High-power Mg batteries enabled by heterogeneous enolization redox chemistry and weakly coordinating electrolytes<\/b><\/u><\/strong><\/a>\u201d(<\/b><\/strong>Nature Energy\uff0c<\/b><\/strong>2020\uff0c10.1038\/s41560-020-00734-0)<\/b><\/strong><\/p>\n

\u00a0<\/b><\/strong>\uff081\uff09\u59da\u5f66\u6559\u6388\u4ecb\u7ecd\uff1b<\/p>\n

\u7f8e\u56fd\u4f11\u65af\u6566\u5927\u5b66\u7535\u5b50\u4e0e\u8ba1\u7b97\u673a\u5de5\u7a0b\u7cfb\u8bb2\u5e2d\u6559\u6388\uff0c\u82f1\u56fd\u7687\u5bb6\u5316\u5b66\u4f1a\u4f1a\u58eb\uff0c\u4f11\u65af\u6566\u5927\u5b66\u80fd\u6e90\u5b58\u50a8\u5fae\u7535\u7f51\u4e2d\u5fc3\u526f\u4e3b\u4efb\u548c\u5fb7\u5dde\u8d85\u5bfc\u4e2d\u5fc3\u6210\u5458\u3002\u66fe\u83b7\u5f97\u6d77\u519b\u9752\u5e74\u79d1\u5b66\u5bb6\u5956\u3001\u79d1\u777f\u552f\u5b89\u201c\u9ad8\u88ab\u5f15\u79d1\u5b66\u5bb6\u201d\u3001\u7f8e\u56fd\u53d1\u660e\u5bb6\u5bb6\u5b66\u9662\u9ad8\u7ea7\u4f1a\u5458\u3001\u5de5\u7a0b\u5b66\u9662\u8bb2\u5e2d\u6559\u6388\u7b49\u5956\u52b1\u3002\u8bfe\u9898\u7ec4\u76ee\u524d\u4e3b\u8981\u4ece\u4e8b\u5168\u56fa\u6001\u7535\u6c60\u3001\u6c34\u7cfb\u7535\u6c60\u3001\u591a\u4ef7\u79bb\u5b50\u7535\u6c60\u7b49\u65b9\u9762\u7684\u7814\u7a76\u3002\u8bfe\u9898\u7ec4\u7f51\u9875: yaoyangroup.com<\/p>\n

\uff082\uff09\u56e2\u961f\u5728\u8be5\u9886\u57df\u5de5\u4f5c\u6c47\u603b\u00a0<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u591a\u4ef7\u6001\u79bb\u5b50\u7535\u6c60\u7684\u73b0\u72b6\u548c\u672a\u6765\u8d8b\u52bf Nature Energy\u00a0<\/i><\/em>2020<\/b><\/strong>,\u00a05, 646\u2013656<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u63a7\u5236\u50a8\u9541\u673a\u5236\u6784\u5efa\u9ad8\u80fd\u6709\u673a\u805a\u5408\u7269\u9541\u7535\u6c60\u00a0Joule<\/i><\/em>\u00a02019<\/b><\/strong>, 3, 782-793<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u50a8\u5b58\u9541\u6c2f\u79bb\u5b50\u7684\u6269\u5c42\u4e8c\u786b\u5316\u949b\u7535\u6c60 Nature Communications\u00a0<\/i><\/em>2017<\/b><\/strong>, 8,\u00a0339<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u9ad8\u7535\u538b\u9541\u94a0\u6df7\u5408\u79bb\u5b50\u7535\u6c60 Nano Energy\u00a0<\/i><\/em>2017<\/b><\/strong>, 34, 188-194<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u77f3\u58a8\u70ef\u4fee\u9970\u7684\u6c27\u5316\u9492\u7eb3\u7c73\u7ebf\u6c14\u51dd\u80f6\u9541\u7535\u6c60\u6b63\u6781\u6750\u6599 Nano Energy\u00a0<\/i><\/em>2015<\/b><\/strong>, 18, 265-272<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u6269\u5c42\u4e8c\u786b\u5316\u94bc\u7eb3\u7c73\u590d\u5408\u6750\u6599\u9541\u7535\u6c60Nano Lett.<\/i><\/em>\u00a02015<\/b><\/strong>, 15, 2194-2202<\/p>\n

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