{"id":214250,"date":"2020-12-10T11:30:41","date_gmt":"2020-12-10T03:30:41","guid":{"rendered":"\/\/m.iemloyee.com\/?p=214250"},"modified":"2020-12-10T11:10:41","modified_gmt":"2020-12-10T03:10:41","slug":"%e5%af%bc%e7%94%b5mof%e7%bb%bc%e8%bf%b0%e5%a4%a7%e9%9b%86%e9%94%a6","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=214250","title":{"rendered":"\u5bfc\u7535MOF\u7efc\u8ff0\u5927\u96c6\u9526"},"content":{"rendered":"<p>\u4ec5\u7ecf\u8fc7\u77ed\u77ed\u4e8c\u5341\u5e74\u7684\u53d1\u5c55\uff0c\u7ed3\u6784\u3001\u529f\u80fd\u4e0a\u5177\u6709\u6781\u5927\u591a\u6837\u6027\u7684\u91d1\u5c5e\u6709\u673a\u6846\u67b6\uff08MOF\uff09\u6750\u6599\u5df2\u7ecf\u6210\u4e3a\u80fd\u6e90\u548c\u73af\u5883\u76f8\u5173\u5e94\u7528\u7684\u70ed\u70b9\u6750\u6599\u3002\u4f46\u662f\u5927\u591a\u6570MOF\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u8f83\u5dee\uff0c\u7535\u5bfc\u7387\u5f88\u4f4e\uff0c\u4e25\u91cd\u5730\u9650\u5236\u4e86\u5b83\u4eec\u7684\u5b9e\u7528\u6027\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5e74\u95f4\uff0c\u5177\u6709\u9ad8\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u548c\u51fa\u8272\u7535\u5bfc\u7387\u7684MOF\u6750\u6599\u5728\u5168\u4e16\u754c\u6380\u8d77\u4e86\u7814\u7a76\u70ed\u6f6e\uff0c\u8fd9\u79cdMOF\u88ab\u79f0\u4e3a\u5bfc\u7535MOF\u3002\u672c\u6587\u4e2d\uff0c\u6211\u4eec\u6311\u9009\u4e86\u4e94\u7bc7\u6709\u5173\u5bfc\u7535MOF\u7684\u91cd\u8981\u7efc\u8ff0\uff0c\u6bcf\u7bc7\u7efc\u8ff0\u90fd\u6709\u5176\u4fa7\u91cd\u70b9\uff0c\u6db5\u76d6\u4e86\u5bfc\u7535MOF\u7684\u7406\u8bba\u548c\u5b9e\u9a8c\u8bbe\u8ba1\u7b56\u7565\uff0c\u5236\u5907\u65b9\u6cd5\uff0c\u5bfc\u7535\u673a\u5236\uff0c\u8f7d\u6d41\u5b50\u4f20\u8f93\uff0c\u7535\u5bfc\u7387\u53ca\u76f8\u5173\u53c2\u6570\u7684\u6d4b\u91cf\u4ee5\u53ca\u5bfc\u7535MOF\u5404\u7c7b\u5e94\u7528\u7b49\u3002<\/p>\n<p>\u4e00\u3001. Electrical conductive coordination polymers<sup>[1]<\/sup><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214251 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/1-2.png\" alt=\"\" width=\"599\" height=\"498\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/1-2.png 599w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/1-2-300x249.png 300w\" sizes=\"(max-width: 599px) 100vw, 599px\" \/><\/p>\n<p>\u672c\u7efc\u8ff0\u6587\u7ae0\u4e8e2012\u5e74\u53d1\u8868\u5728Chemical Society Reviews\u4e0a\uff0c\u662f\u5728\u5bfc\u7535MOF\u521a\u5f00\u59cb\u53d1\u5c55\u7684\u65f6\u5019\u5bf9\u5176\u5bfc\u7535\u673a\u7406\u548c\u6784\u5efa\u624b\u6bb5\u8fdb\u884c\u6df1\u5ea6\u89e3\u8bfb\u7684\u4e00\u7bc7\u7efc\u8ff0\uff0c\u867d\u7136\u9898\u76ee\u662f\u5bfc\u7535\u914d\u4f4d\u805a\u5408\u7269\uff0c\u4f46\u662f\u5176\u6587\u4e2d\u7279\u522b\u8bf4\u660e\u4e86\u7531\u4e8e\u5bf9\u5b54\u9699\u7387\u548c\u50ac\u5316\u6027\u80fd\u7684\u8ffd\u6c42\uff0cMOF\u662f\u5728\u7ed3\u6784\u4e2d\u5177\u6709\u5927\u7a7a\u8154\u7684\u914d\u4f4d\u805a\u5408\u7269\uff0c\u5373\u591a\u5b54\u914d\u4f4d\u805a\u5408\u7269\u3002<\/p>\n<p>\u672c\u6587\u9996\u5148\u5bf9\u7535\u5bfc\u673a\u5236\u548c\u7535\u5bfc\u7387\u6d4b\u91cf\u624b\u6bb5\u8fdb\u884c\u4e86\u5168\u9762\u7684\u6982\u62ec\uff0c\u5bf9\u5b66\u6750\u6599\u4f46\u662f\u7f3a\u4e4f\u7269\u7406\u80cc\u666f\u7684\u79d1\u7814\u4eba\u5458\u6709\u5f88\u5927\u5e2e\u52a9\u3002\u7136\u540e\u4e3b\u8981\u5185\u5bb9\u662f\u5bf9\u5bfc\u7535\u914d\u4f4d\u805a\u5408\u7269\u7684\u5206\u7c7b\u548c\u89e3\u8bfb\uff0c\u5176\u5206\u7c7b\u662f\u662f\u57fa\u4e8e\u4e24\u4e2a\u7ed3\u6784\u6807\u51c6\uff1a\u7ef4\u6570\u548c\u6865\u8054\u914d\u4f53\u3002\u7740\u91cd\u7814\u7a76\u67d0\u4e2a\u7ef4\u5ea6\u7684\u6750\u6599\u7684\u7814\u7a76\u4eba\u5458\u9605\u8bfb\u8d77\u6765\u975e\u5e38\u65b9\u4fbf\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214252 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/2-1.png\" alt=\"\" width=\"426\" height=\"370\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/2-1.png 426w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/2-1-300x261.png 300w\" sizes=\"(max-width: 426px) 100vw, 426px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe1. \u4e00\u7ef4\u548c\u4e8c\u7ef4MOF\u4e2d\u586b\u5145\u5e26\u548c\u534a\u586b\u5145\u5e26\u89c2\u5bdf\u5230\u7684\u7535\u5b50\u72b6\u6001<\/p>\n<p>\u4e8c\u3001Coordination polymer-based conductive materials: ionic conductivity vs. electronic conductivity<sup>[2]<\/sup><\/p>\n<p>\u672c\u7efc\u8ff0\u57fa\u4e8e\u63d0\u9ad8\u7535\u5bfc\u7387\u7684\u4e24\u79cd\u4e3b\u8981\u7b56\u7565\uff1a\u5411\u6846\u67b6\u4e2d\u5f15\u5165\u5ba2\u4f53\u5206\u5b50\uff1b\u91d1\u5c5e\u6216\u6709\u673a\u6210\u5206\u7684\u540e\u4fee\u9970\/\u5b98\u80fd\u56e2\u7684\u5f15\u5165\uff0c\u5c06\u5bfc\u7535\u914d\u4f4d\u805a\u5408\u7269\u5206\u6210\u79bb\u5b50\u5bfc\u7535\u548c\u7535\u5b50\u5bfc\u7535\u4e24\u5927\u7c7b\u3002\u7136\u540e\u4ece\u8fd9\u4e2a\u89d2\u5ea6\u51fa\u53d1\u96c6\u4e2d\u8ba8\u8bba\u4e86\u8fc7\u53bb\u51e0\u5e74\u4e2d\u672a\u6539\u6027\u53ca\u6539\u6027CP\u53ca\u5176\u590d\u5408\u7269\u5728\u79bb\u5b50\u5bfc\u7535\u548c\u7535\u5b50\u5bfc\u7684\u6784\u5efa\u53ca\u5e94\u7528\u65b9\u9762\u7684\u91cd\u8981\u6210\u5c31\u3002<\/p>\n<p>\u6587\u7ae0\u63d0\u51fa\u4e86\u6750\u6599\u8bbe\u8ba1\u548c\u5e94\u7528\u89d2\u5ea6\u8981\u89e3\u51b3\u7684\u4e3b\u8981\u57fa\u672c\u95ee\u9898\uff0c\u901a\u8fc7\u9610\u8ff0CPs\u5728\u79bb\u5b50\/\u7535\u5bfc\u7387\u65b9\u9762\u7684\u4f18\u52bf\u548c\u6311\u6218\uff0c\u63d0\u4f9b\u4e86\u4e00\u4e9b\u6709\u7528\u7684\u5efa\u8bae\uff0c\u4ee5\u9610\u660e\u5b83\u4eec\u7684\u53d1\u5c55\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214253 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/3-1.png\" alt=\"\" width=\"410\" height=\"532\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/3-1.png 410w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/3-1-231x300.png 231w\" sizes=\"(max-width: 410px) 100vw, 410px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe2. \u4e24\u79cd\u63d0\u9ad8\u7535\u5bfc\u7387\u7684\u7b56\u7565<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214254 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/4-1.png\" alt=\"\" width=\"387\" height=\"295\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/4-1.png 387w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/4-1-300x229.png 300w\" sizes=\"(max-width: 387px) 100vw, 387px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe3. \u5404\u79cd\u7c7b\u578b\u7684\u79bb\u5b50\u5bfc\u7535<\/p>\n<p>\u4e09\u3001Recent development and applications of electrical conductive MOFs<sup>[3]<\/sup><\/p>\n<p>\u8fd9\u7bc7\u7efc\u8ff0\u7684\u4e3b\u8981\u4f18\u70b9\u5728\u4e8e\u5185\u5bb9\u5168\u9762\uff0c\u628a\u5bfc\u7535MOF\u7684\u7406\u8bba\u548c\u5b9e\u9a8c\u8bbe\u8ba1\u7b56\u7565\uff0c\u5236\u5907\u65b9\u6cd5\uff0c\u5bfc\u7535\u673a\u5236\uff0c\u8f7d\u6d41\u5b50\u4f20\u8f93\uff0c\u7535\u5bfc\u7387\u53ca\u76f8\u5173\u53c2\u6570\u7684\u6d4b\u91cf\u4ee5\u53ca\u5bfc\u7535MOF\u5404\u7c7b\u5e94\u7528\u90fd\u7cfb\u7edf\u5730\u603b\u7ed3\u5728\u4e00\u8d77\uff0c\u53ef\u4ee5\u65b9\u4fbf\u521a\u5f00\u59cb\u8fdb\u5165\u5bfc\u7535MOF\u9886\u57df\u7684\u7814\u7a76\u4eba\u5458\u5feb\u901f\u6293\u4f4f\u8be5\u9886\u57df\u7684\u6838\u5fc3\u77e5\u8bc6\u5e76\u638c\u63e1\u57fa\u672c\u8981\u70b9\uff0c\u800c\u4e14\u8fd9\u7bc7\u7efc\u8ff0\u662f2020\u5e7411\u6708\u4efd\u521a\u53d1\u8868\u7684\uff0c\u4e0d\u4ec5\u5bf9\u7ecf\u5178\u7684\u5bfc\u7535MOF\u6750\u6599\u8fdb\u884c\u4e86\u603b\u7ed3\uff0c\u5bf9\u4e8e\u8fd1\u4e24\u5e74\u5bfc\u7535MOF\u65b0\u7684\u53d1\u5c55\u6210\u679c\u4e5f\u505a\u4e86\u603b\u7ed3\uff0c\u6709\u5229\u4e8e\u8bfb\u8005\u6e05\u6670\u5730\u4e86\u89e3\u6700\u65b0\u7684\u7814\u7a76\u6210\u679c\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214274 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/\u56fe\u72471-6.png\" alt=\"\" width=\"600\" height=\"266\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/\u56fe\u72471-6.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/\u56fe\u72471-6-300x133.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe4. \u57fa\u4e8e\u4e09\u4e9a\u82ef\u57fa\u884d\u751f\u7684\u914d\u4f53\u7684\u516d\u89d2\u5f62\u4e8c\u7ef4MOF\u7684\u793a\u610f\u7ed3\u6784<\/p>\n<p>\u56db\u3001Conductive two-dimensional metal\u2013organic frameworks as multifunctional materials<sup>[4]<\/sup><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214255 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/5-1.png\" alt=\"\" width=\"600\" height=\"157\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/5-1.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/5-1-300x79.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe5. \u4ee3\u8868\u6027\u4e8c\u7ef4\u6750\u6599\u7684\u7ed3\u6784\u793a\u610f\u56fe<\/p>\n<p>\u8fd9\u7bc7\u7efc\u8ff0\u603b\u7ed3\u4e862D\u5bfc\u7535MOF\u7684\u7814\u7a76\u8fdb\u5c55\uff0c\u4e0e\u524d\u51e0\u7bc7\u8ba8\u8bba\u6784\u5efa\u7b56\u7565\u548c\u5236\u5907\u624b\u6bb5\u7684\u7efc\u8ff0\u4e0d\u540c\uff0c\u8fd9\u7bc7\u7efc\u8ff0\u7684\u91cd\u70b9\u662fMOF\u7684\u5408\u6210\u6a21\u5757\u5316\uff0c\u5668\u4ef6\u96c6\u6210\u7b56\u7565\u548c\u591a\u529f\u80fd\u7279\u6027\u3002\u8ba8\u8bba\u4e86\u6d89\u53ca\u4f20\u611f\uff0c\u50ac\u5316\uff0c\u7535\u5b50\uff0c\u80fd\u91cf\u8f6c\u6362\u548c\u5b58\u50a8\u7684\u5e94\u7528\u3002\u5bf9\u5206\u5b50\u5de5\u7a0b\u548c2D\u5bfc\u7535MOF\u5b9e\u9645\u5f00\u53d1\u8fdb\u884c\u4e86\u6df1\u5ea6\u8ba8\u8bba\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214256 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/6-1.png\" alt=\"\" width=\"492\" height=\"327\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/6-1.png 492w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/6-1-300x199.png 300w\" sizes=\"(max-width: 492px) 100vw, 492px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe6. \u5c062D\u5bfc\u7535MOF\u96c6\u6210\u5230\u8bbe\u5907\u4e2d\u7684\u4e00\u822c\u65b9\u6cd5<\/p>\n<p>\u4e94\u3001Electrically Conductive Porous Metal\u2013Organic Frameworks <sup>[5]<\/sup><\/p>\n<p>\u672c\u6587\u662f\u7531MOF\u8d44\u6df1\u4e13\u5bb6\u9ebb\u7701\u7406\u5de5\u7684Mircea Dinca\u6559\u6388\u4e0e2016\u5e74\u53d1\u8868\u5728Angew. Chem. Int. Ed\u4e0a\u7684\u7efc\u8ff0\uff0c\u6bd4\u8f83\u8be6\u7ec6\u5730\u4ece\u6784\u5efa\u65b9\u5f0f\u4e0a\u89e3\u91ca\u4e86\u589e\u5f3aMOF\u7535\u5bfc\u7387\u7684\u673a\u7406\uff0c\u4ece\u57fa\u672c\u6784\u5efa\u5355\u5143\u51fa\u53d1\uff0c\u6307\u51fa\u6709\u673a\u914d\u4f53\u5e94\u8be5\u662f\u7a33\u5b9a\u7684\u81ea\u7531\u57fa\uff08\u63d0\u4f9b\u4e0d\u6210\u5bf9\u7684\u7535\u5b50\uff09\uff0c\u6216\u8005\u662f\u5177\u6709\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\u7684<sup>[5]<\/sup>\u5206\u5b50\uff0c\u4ee5\u5b9e\u73b0\u5728\u91d1\u5c5e\u79bb\u5b50\u6216\u8282\u70b9\u4e4b\u95f4\u7684\u4fbf\u6377\u7535\u8377\u8f6c\u79fb\uff1b\u800c\u91d1\u5c5e\u79bb\u5b50\u5e94\u5177\u6709\u9ad8\u80fd\u91cf\u7684\u7535\u5b50\u6216\u7a7a\u7a74\u3002\u603b\u7ed3\u4e86\u5f71\u54cd\u7535\u5bfc\u7387\u7684\u5404\u79cd\u7269\u7406\u56e0\u7d20\u53ca\u6d4b\u91cf\u65b9\u6cd5\uff0c\u4ee5\u53ca\u5404\u7c7b\u6d4b\u91cf\u65b9\u6cd5\u7684\u4f7f\u7528\u6761\u4ef6\u548c\u9650\u5236\uff0c\u5bf9\u4e8e\u540c\u65f6\u4ece\u5316\u5b66\u548c\u7269\u7406\u89d2\u5ea6\u5236\u5b9a\u63d0\u9ad8MOF\u7535\u5bfc\u7387\u7684\u7b56\u7565\u6709\u91cd\u8981\u5e2e\u52a9\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-214257 size-full\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/7-1.png\" alt=\"\" width=\"526\" height=\"421\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/7-1.png 526w, \/\/m.iemloyee.com\/wp-content\/uploads\/2020\/12\/7-1-300x240.png 300w\" sizes=\"(max-width: 526px) 100vw, 526px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe7. \u6d4b\u91cf\u7535\u5bfc\u7387\u7684\u4e0d\u540c\u65b9\u5f0f<\/p>\n<p>\u53c2\u8003\u6587\u732e\uff1a<\/p>\n<p>[1]Gonzalo Givaja, Pilar Amo-Ochoa, Carlos J. G\u00f3mez-Garc\u00eda, F\u00e9lix Zamora, Electrical conductive coordination polymers, Chemical Society Reviews, 2012 (41) 115-147.<\/p>\n<p>[2]Hai-Ning Wang, Xing Meng, Long-Zhang Dong, Yifa Chen, Shun-Li Li, Ya-Qian Lan, Coordination polymer-based conductive materials: ionic conductivity vs. electronic conductivity, Journal of Materials Chemistry A, 2019 (7) 24059-24091.<\/p>\n<p>[3]Chun Li, Lili Zhang, Jiaqi Chen, Xuelian Li, Jingwen Sun, Junwu Zhu, Xin Wang, Yongsheng Fu, Recent development and applications of electrical conductive MOFs, Nanoscale, 2020.<\/p>\n<p>[4]Michael Ko, Lukasz Mendecki, Katherine A. Mirica, Conductive two-dimensional metal\u2013organic frameworks as multifunctional materials, Chemical Communications, 2018 (54) 7873-7891.<\/p>\n<p>[5]Lei Sun, Michael G. 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