{"id":213881,"date":"2020-12-01T06:30:42","date_gmt":"2020-11-30T22:30:42","guid":{"rendered":"\/\/m.iemloyee.com\/?p=213881"},"modified":"2020-11-30T22:14:57","modified_gmt":"2020-11-30T14:14:57","slug":"%e3%80%90%e6%8a%95%e7%a8%bf%e3%80%91%e5%8d%97%e5%bc%80%e5%a4%a7%e5%ad%a6%e5%90%91%e4%b8%9c%e6%9d%8e%e8%b7%83%e9%be%99nano-letters-%e6%b6%b2%e6%80%81%e9%87%91%e5%b1%9e%e7%94%b5%e6%9e%81%e7%a0%94","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=213881","title":{"rendered":"\u5357\u5f00\u5927\u5b66\u5411\u4e1c&\u674e\u8dc3\u9f99Nano Letters: \u6db2\u6001\u91d1\u5c5e\u7535\u6781\u7814\u7a76\u9499\u949b\u77ff\u6676\u4f53\u7684\u8f7d\u6d41\u5b50\u8f93\u8fd0\u7279\u6027"},"content":{"rendered":"
<\/p>\n
\u4e00\u3001\u5168\u6587\u901f\u89c8<\/b><\/strong><\/p>\n \u5728\u5149\u7535\u5668\u4ef6\u5fae\u578b\u5316\u8fc7\u7a0b\u4e2d\uff0c\u63a2\u7a76\u6750\u6599\u7684\u5c3a\u5bf8\u5927\u5c0f\u5bf9\u8f7d\u6d41\u5b50\u4f20\u8f93\u7279\u6027\u7684\u5f71\u54cd\u6781\u4e3a\u91cd\u8981\u3002\u5357\u5f00\u5927\u5b66\u5411\u4e1c\u6559\u6388\u548c\u674e\u8dc3\u9f99\u526f\u6559\u6388<\/b><\/strong>\u5408\u4f5c\u5229\u7528\u6db2\u6001\u91d1\u5c5e\u7535\u6781\u6784\u5efa\u201c\u7535\u6781-\u9499\u949b\u77ff\u6676\u4f53-\u7535\u6781\u7ed3\u201d\uff0c\u5728\u5fae\u89c2\u5c3a\u5ea6\u4e0b\u7814\u7a76\u4e86\u9499\u949b\u77ff\u6676\u4f53\u5c3a\u5bf8\u5927\u5c0f\u5bf9\u8f7d\u6d41\u5b50\u4f20\u8f93\u7279\u6027\u7684\u5f71\u54cd\uff0c\u63ed\u793a\u4e86\u57fa\u4e8e\u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u5355\u6676\u7684\u5ba4\u6e29\u8d1f\u5fae\u5206\u7535\u963b\u73b0\u8c61\u53ca\u5176\u673a\u7406\u3002<\/p>\n \u4e8c\u3001\u80cc\u666f\u4ecb\u7ecd<\/b><\/strong><\/p>\n \u5728\u8fc7\u53bb\u5341\u5e74\u4e2d\uff0c\u6742\u5316\u6709\u673a-\u65e0\u673a\u9499\u949b\u77ff\u6750\u6599\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\uff0c\u5176\u4e2d\u7532\u80fa\u94c5\u5364\u9499\u949b\u77ff\u6750\u6599\uff08MAPbX3<\/sub>\uff0c\u5176\u4e2dMA = CH3<\/sub>NH3<\/sub>\uff0cX = I\uff0cBr\u6216Cl\uff09\u7531\u4e8e\u5176\u5e26\u9699\u53ef\u8c03\uff0c\u9ad8\u5438\u6536\u7cfb\u6570\uff0c\u4f4e\u7f3a\u9677\u5bc6\u5ea6\uff0c\u957f\u8f7d\u6d41\u5b50\u5bff\u547d\u548c\u6269\u6563\u957f\u5ea6\u7b49\u4f18\u5f02\u7279\u6027\u4f7fMAPbX3<\/sub>\u6750\u6599\u5e7f\u6cdb\u5e94\u7528\u4e8e\u6fc0\u5149\u5668\uff0c\u53d1\u5149\u4e8c\u6781\u7ba1\uff0c\u592a\u9633\u7535\u6c60\uff0c\u4f20\u611f\u5668\uff0c\u5149\u7535\u63a2\u6d4b\u5668\u7b49\u5149\u7535\u5668\u4ef6\uff0c\u5e76\u53d6\u5f97\u4f18\u5f02\u7684\u5668\u4ef6\u6027\u80fd\u3002\u4e0e\u5b8f\u89c2\u9499\u949b\u77ff\uff08mm\u6216cm\uff09\u591a\u6676\u819c\u76f8\u6bd4\uff0c\u9499\u949b\u77ff\u5c0f\u5355\u6676\u6750\u6599\uff08\u00b5m\u6216nm\uff09\u5177\u6709\u66f4\u4f18\u5f02\u72ec\u7279\u7684\u5149\u7535\u7279\u6027\uff0c\u4f46\u662f\u57fa\u4e8e\u5fae\u7eb3\u9499\u949b\u77ff\u5355\u6676\u7684\u5149\u7535\u7279\u6027\u7814\u7a76\u9c9c\u6709\u62a5\u9053\uff0c\u56e0\u4e3a\u5176\u5728\u7535\u6781\u7684\u5236\u5907\u4e0a\u9762\u4e34\u6311\u6218\u3002<\/p>\n \u5f53\u6d4b\u91cf\u7684\u5bf9\u8c61\u4e3a\u5fae\u7c73\u7ea7\u522b\u7684\u6676\u4f53\u65f6\uff0c\u7528\u4e8e\u7814\u7a76\u5757\u72b6\/\u8584\u819c\u7269\u4f53\u7684\u7535\u6781\u5236\u5907\u65b9\u6cd5\uff08\u84b8\u53d1\u91d1\u5c5e\u5c42\u6216\u65cb\u6d82\u5bfc\u7535\u80f6\uff09\u5df2\u7ecf\u4e0d\u518d\u9002\u5408 (\u56e0\u4e3a\u5f88\u96be\u907f\u514d\u77ed\u8def\u73b0\u8c61)\u3002\u4e3a\u4e86\u7814\u7a76\u5fae\u7c73\u7ea7\u9499\u949b\u77ff\u6676\u4f53\u7684\u7279\u6027\uff0c\u5bf9\u7535\u6781\u6709\u5982\u4e0b\u8981\u6c42\uff1a1\uff09\u7535\u6781\u7684\u5c3a\u5bf8\u5e94\u51cf\u5c0f\u81f3\u5fae\u7c73\u7ea7\u4ee5\u5339\u914d\u9499\u949b\u77ff\u6676\u4f53\u7684\u5c3a\u5bf8\uff0c\u5e76\u4e14\u7535\u6781\u95f4\u8ddd\u5e94\u7cbe\u786e\u53ef\u8c03\u4ee5\u83b7\u5f97\u7535\u6781-\u9499\u949b\u77ff\u6676\u4f53-\u7535\u6781\u7ed3\uff1b2\uff09\u9499\u949b\u77ff\u548c\u7535\u6781\u4e4b\u95f4\u7684\u529b\u53ef\u8c03\uff0c\u53ef\u4ee5\u5f62\u6210\u7d27\u5bc6\u7684\u63a5\u89e6\uff0c\u540c\u65f6\u907f\u514d\u673a\u68b0\u635f\u4f24\uff1b3\uff09\u53ef\u91cd\u590d\u63a5\u89e6\uff0c\u4ee5\u63a2\u6d4b\u8f7d\u6d41\u5b50\u4f20\u8f93\u7279\u6027\u662f\u5426\u53ef\u518d\u73b0\u3002<\/p>\n \u8d1f\u5fae\u5206\u7535\u963b\uff08NDR\uff09\u7684\u7279\u5f81\u662f\u7535\u6d41\u968f\u7535\u538b\u7684\u5347\u9ad8\u800c\u51cf\u5c0f\uff0c\u56e0\u800c\u53d7\u5230\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\uff0c\u5e76\u88ab\u8ba4\u4e3a\u662f\u4f4e\u529f\u7387\u5b58\u50a8\u5668\uff0c\u9ad8\u9891\u632f\u8361\u5668\u548c\u903b\u8f91\u7535\u8def\u7b49\u7eb3\u7c73\u7535\u5b50\u5e94\u7528\u7684\u91cd\u8981\u5143\u7d20\u3002\u901a\u5e38\uff0cNDR\u7531\u53cc\u52bf\u5792\u548c\u4e00\u4e2a\u52bf\u9631\u7ec4\u6210\u7684\u7ed3\u6784\u6765\u5b9e\u73b0\uff0c\u4f46\u662f\u6b64\u65b9\u6cd5\u53d7\u5230\u52a0\u5de5\u5de5\u827a\u7684\u9650\u5236\u3002\u00a0\u8fd9\u91cc\uff0c\u6211\u4eec\u5728\u7535\u6781-\u9499\u949b\u77ff-\u7535\u6781\u7ed3\u4e2d\u4e5f\u89c2\u5bdf\u5230\u4e86NDR \u73b0\u8c61\uff0c\u6b64\u7ed3\u6784\u4e0e\u53cc\u52bf\u5792\u7ed3\u6784\u65e0\u5173\uff0c\u5e76\u4e14\u65e0\u9700\u590d\u6742\u7684\u5fae\u7eb3\u52a0\u5de5\u5de5\u827a\u3002<\/p>\n \u4e09\u3001\u672c\u6587\u4eae\u70b9<\/b><\/strong><\/p>\n \uff081\uff09\u53d1\u5c55\u4e86\u4e00\u79cd\u8f6f\u63a5\u89e6\u7535\u6781\u5236\u5907\u65b9\u6cd5\uff0c\u8be5\u65b9\u6cd5\u91c7\u7528\u6db2\u6001EGaIn\uff08\u9553\u94df\u5408\u91d1\uff09\u4f5c\u4e3a\u9876\u90e8\u7535\u6781\uff0c\u5e76\u91c7\u7528\u5e73\u5766\u7684AgTS<\/sup>\uff08\u6a21\u677f\u5265\u79bb\u5236\u4f5c\u7684\u94f6\u5c42\uff09\u6216\u77f3\u58a8\u70ef\u5c42\u4f5c\u4e3a\u5e95\u90e8\u7535\u6781\u3002 \u8fd9\u79cd\u8f6f\u63a5\u89e6\u7b56\u7565\u9002\u7528\u4e8e\u6784\u9020\u7a33\u5b9a\u7684\u9499\u949b\u77ff\u7ed3\uff0c\u5373\u5c06CH3<\/sub>NH3<\/sub>PbBr3<\/sub>\uff08MAPbBr3<\/sub>\uff09\u6676\u4f53\u5939\u5728\u9876\u90e8\u548c\u5e95\u90e8\u7535\u6781\u4e4b\u95f4\u3002 \u6db2\u6001\u91d1\u5c5e\u7535\u6781 (EGaIn) \u7684\u81ea\u9002\u5e94\u53d8\u5f62\u7279\u6027\u907f\u514d\u4e86\u5bf9\u6837\u54c1\u7684\u673a\u68b0\u635f\u4f24\uff0c\u4ece\u800c\u5efa\u7acb\u7a33\u5b9a\u4e14\u7d27\u5bc6\u7684\u7535\u6781-\u9499\u949b\u77ff\u5355\u6676\u63a5\u89e6\u3002<\/p>\n \uff082\uff09\u7814\u7a76\u4e86MAPbBr3<\/sub>\u5355\u6676\u5fae\u7247\uff08MP\uff09\u548cMAPbBr3<\/sub>\u91cf\u5b50\u70b9\uff08QD\uff09\u8584\u819c\u7684\u5149\u7535\u6027\u80fd\u3002\u4e0e\u91cf\u5b50\u70b9\uff08\u226410 nm\uff09\u8584\u819c\u76f8\u6bd4\uff0c\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\u5728\u5149\u7167\u5c04\u4e0b\u663e\u793a\u51fa\u66f4\u5feb\u7684\u5149\u7535\u6d41\u54cd\u5e94\u548c\u66f4\u9ad8\u7684\u5f00\/\u5173\u6bd4\u3002<\/p>\n \uff083\uff09\u5c0f\u5c3a\u5bf8\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\u7ed3\uff08< 30 \u03bcm\uff09\u8868\u73b0\u51fa\u5ba4\u6e29\u8d1f\u5fae\u5206\u7535\u963b\uff08NDR\uff09\u73b0\u8c61\uff0c\u800c\u5728\u76f8\u540c\u504f\u538b\u8303\u56f4\u5185\u7684\u5927\u9499\u949b\u77ff\u7ed3\uff08> 50 \u03bcm\uff09\u4e2d\u4e0d\u5b58\u5728NDR\u73b0\u8c61\u3002\u5efa\u7acb\u4e86\u9499\u949b\u77ff\u6750\u6599\u57fa\u4e8e\u79bb\u5b50\u8fc1\u79fb\u548c\u589e\u5f3a\u8f7d\u6d41\u5b50\u590d\u5408\u7b49\u6a21\u578b\uff0c\u5c1d\u8bd5\u63ed\u793a\u4e86\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\u7684\u5c3a\u5bf8\u4f9d\u8d56\u6027NDR\u884c\u4e3a\u3002<\/p>\n \u56db\u3001\u56fe\u6587\u89e3\u6790<\/b><\/strong><\/p>\n Figure 1. <\/b><\/strong>Optoelectrical measurement system and images of the perovskite\u00a0crystals.<\/p>\n \u901a\u8fc7\u65a9\u6ce2\u5668\u7684\u8c03\u5236\uff0c\u6fc0\u5149\u7167\u5c04\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\uff08\u6216\u91cf\u5b50\u70b9\u5f62\u6210\u7684\u8584\u819c\uff09\u3002\u00a0\u9499\u949b\u77ff\u6676\u4f53\u5939\u5728\u9876\u90e8EGaIn\u5c16\u7aef\u548c\u5e95\u90e8AgTS<\/sup>\u886c\u5e95\u4e4b\u95f4\uff08\u56fe1a\uff09\u3002 MAPbBr3<\/sub>\u5355\u6676\u5fae\u7247\u7684\u626b\u63cf\u7535\u955c\u56fe\u50cf\uff08\u56fe1b\uff09\u53caMAPbBr3<\/sub>\u91cf\u5b50\u70b9\u7684\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff08\u56fe1c\uff09\u8868\u660e\u4e86\u5355\u6676\u5fae\u7247\u548c\u91cf\u5b50\u70b9\u819c\u7684\u5c3a\u5bf8\u7279\u5f81\u3002\u901a\u8fc7\u538b\u7535\u63a7\u5236\uff0c\u57fa\u677f\u4ee5\u7eb3\u7c73\u7ea7\u7684\u7cbe\u5ea6\u5411\u4e0a\u8fd0\u52a8\u4ee5\u5f62\u6210\u7535\u6781-\u9499\u949b\u77ff\u6676\u4f53-\u7535\u6781\u7ed3\u3002\u4e3a\u4e86\u786e\u4fdd\u9488\u5c16\u76f4\u63a5\u63a5\u89e6\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\uff0c\u4f7f\u7528\u4e24\u4e2a\u6b63\u4ea4\u6570\u5b57\u663e\u5fae\u955c\u6765\u76d1\u63a7\u63a5\u89e6\u8fc7\u7a0b\uff08\u56fe1d-1f\uff09\u3002\u5728\u5e95\u90e8AgTS<\/sup>\u57fa\u677f\u7684\u8868\u9762\u4e0a\u53ef\u4ee5\u660e\u663e\u89c2\u5bdf\u5230\u9876\u90e8EGaIn\u5c16\u7aef\u7684\u955c\u50cf\u3002<\/p>\n Figure 2. <\/b><\/strong>Schematics of two types of junctions and the photodynamic\u00a0responses.<\/p>\n EGaIn-MP-AgTS<\/sup>\u7ed3\u7684\u793a\u610f\u56fe\u5982\u56fe2a\u6240\u793a\uff0c\u5728\u5149\u7167\u4e0b\u89c2\u5bdf\u5230MP\u7ed3\u7684\u5149\u7535\u6d41\u51fa\u73b0\u5c16\u5cf0(\u56fe2b),\u00a0\u5927\u91cf\u5149\u751f\u8f7d\u6d41\u5b50\u5bfc\u81f4\u5728\u5149\u7167\u4e0b\u7535\u6d41\u5feb\u901f\u589e\u52a0\uff0c\u968f\u540e\u8f7d\u6d41\u5b50\u7684\u590d\u5408\u5bfc\u81f4\u7535\u6d41\u7684\u7f13\u6162\u8870\u51cf\uff08\u56fe2c\uff09\u3002EGaIn-QDs-AgTS<\/sup>\u7ed3\u7684\u793a\u610f\u56fe\u5982\u56fe2d\u6240\u793a\uff0c\u5728QD\u8584\u819c\u7ed3\u5904\uff0c\u5149\u7535\u6d41\u5728\u5149\u7167\u4e0b\u7f13\u6162\u589e\u52a0\uff0c\u800c\u5728\u5149\u5173\u95ed\u65f6\u7f13\u6162\u964d\u4f4e\uff08\u56fe2e\uff09\uff0c\u7531\u7f3a\u9677\u5bf9\u8f7d\u6d41\u5b50\u7684\u6355\u83b7\u5bfc\u81f4\u5728\u5149\u7167\u4e0b\u7535\u6d41\u7f13\u6162\u589e\u52a0\uff0c\u800c\u5f53\u5149\u5173\u95ed\u65f6\uff0c\u7f3a\u9677\u6355\u83b7\u7684\u8f7d\u6d41\u5b50\u91ca\u653e\u5bfc\u81f4\u7535\u6d41\u7f13\u6162\u964d\u4f4e\uff08\u56fe2f\uff09\u3002<\/p>\n Figure 3.<\/b><\/strong>\u00a0The I-V curves and the mechanism for the NDR observations.<\/p>\n \u5927\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247(~ 80 \u03bcm)\u5728\u5149\u7167\u4e0b\u6d4b\u5f97\u7684I-V\u66f2\u7ebf\u59823a\u6240\u793a\uff0c\uff081\uff09\u548c\uff082\uff09\u8868\u793a\u6b63\u5411\u626b\u63cf\u548c\u53cd\u5411\u626b\u63cf\uff0c\u63d2\u56fe\u4e3aEGaIn-Perovskite-Graphene\u7ed3\u7684\u793a\u610f\u56fe\uff0c\u5f53\u5411EGaIn\u7535\u6781\u65bd\u52a0\u6b63\u7535\u538b\uff08Vbi<\/sub>\uff09\u65f6\uff0c\u5176\u80fd\u5e26\u7ed3\u6784\u5173\u7cfb\u5982\u56fe3b\u6240\u793a\uff0c\u9499\u949b\u77ff\u5c42\u5185\u90e8\u7684\u7535\u52bf\u5747\u5300\u4e0b\u964d\u3002\u5c0f\u9499\u949b\u77ff\u5355\u6676\u5fae\u7247\uff08~30 \u03bcm\uff09\u5728\u5149\u7167\u4e0b\u7684I-V\u66f2\u7ebf\u5982\u56fe3c\u6240\u793a\uff0c\u5728\u6b63\u504f\u538b\u4e0b\u89c2\u5bdf\u5230\u660e\u663e\u7684NDR\u884c\u4e3a\uff0c\u53ef\u7531\u80fd\u5e26\u5173\u7cfb\u56fe3d\u89e3\u91ca\uff1a\u5728\u5f3a\u5916\u90e8\u7535\u573a\u4e0b\uff0c\u6b63\u8d1f\u79bb\u5b50\u53cd\u65b9\u5411\u79fb\u52a8\u5e76\u5728\u5728\u7535\u6781\/\u9499\u949b\u77ff\u754c\u9762\u5904\u7d2f\u79ef\u4ea7\u751f\u8865\u507f\u573a\uff08Vcom<\/sub>\uff09\uff0c\u8fdb\u800c\u5c4f\u853d\u5916\u90e8\u65bd\u52a0\u7684\u7535\u573a\uff0c\u4ece\u800c\u589e\u5f3a\u4e86\u5185\u90e8\u8f7d\u6d41\u5b50\u7684\u590d\u5408\uff0c\u6700\u7ec8\u5bfc\u81f4NDR\u73b0\u8c61\u7684\u4ea7\u751f\u3002<\/p>\n \u8be5\u8bba\u6587\u4e2d\uff0c\u5357\u5f00\u5927\u5b66\u674e\u8dc3\u9f99\u526f\u6559\u6388\u548c\u5411\u4e1c\u6559\u6388\u4e3a\u8bba\u6587\u7684\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff0c\u5357\u5f00\u5927\u5b66\u535a\u58eb\u751f\u8d75\u667a\u5bbe\u548c2017\u7ea7\u672c\u79d1\u751f\u738b\u6587\u94ce\u4e3a\u8bba\u6587\u7684\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u3002<\/p>\n
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