{"id":206650,"date":"2020-08-05T06:47:51","date_gmt":"2020-08-04T22:47:51","guid":{"rendered":"\/\/m.iemloyee.com\/?p=206650"},"modified":"2020-08-04T21:48:16","modified_gmt":"2020-08-04T13:48:16","slug":"energy-environ-sci-%e6%8a%a5%e9%81%93%ef%bc%9an-n-%e4%ba%8c%e7%94%b2%e5%9f%ba%e4%b9%99%e9%85%b0%e8%83%ba%e5%9f%ba%e7%94%b5%e8%a7%a3%e8%b4%a8%e5%8a%a9%e5%8a%9bli-o2%e7%94%b5%e6%b1%a0%e7%9a%84","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=206650","title":{"rendered":"Energy Environ. Sci. \u62a5\u9053\uff1aN, N-\u4e8c\u7532\u57fa\u4e59\u9170\u80fa\u57fa\u7535\u89e3\u8d28\u52a9\u529bLi-O2\u7535\u6c60\u7684\u5faa\u73af\u7a33\u5b9a\u6027"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u5982\u4eca\uff0c\u65b0\u80fd\u6e90\u6c7d\u8f66\u7b49\u5bf9\u5177\u6709\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u7535\u6c60\u9700\u6c42\u662f\u8d8a\u6765\u8d8a\u9ad8\u3002\u5728\u6240\u6709\u53ef\u7528\u7684\u80fd\u91cf\u5b58\u50a8\u8bbe\u5907\u4e2d\uff0c\u53ef\u5145\u7535\u975e\u6c34\u7cfbLi-O2<\/sub>\u7535\u6c60\u5177\u67093500 Wh\/kg\u7684\u9ad8\u7406\u8bba\u80fd\u91cf\u5bc6\u5ea6\uff0c\u662f\u4e00\u79cd\u5f88\u6709\u524d\u666f\u7684\u5019\u9009\u8005\u3002\u7136\u800c\uff0c\u76ee\u524d\u6ca1\u6709\u7535\u89e3\u8d28\u80fd\u591f\u5728\u4e0eLi\u91d1\u5c5e\u8d1f\u6781\u517c\u5bb9\u7684\u60c5\u51b5\u4e0b\uff0c\u627f\u53d7\u8fd8\u539f\u6c27\uff08O2<\/sub>–<\/sup>\u3001O2<\/sub>2-<\/sup>\u3001HOO–<\/sup>\u548cHO–<\/sup>\uff09\u7684\u4eb2\u6838\u653b\u51fb\uff0c\u56e0\u6b64Li-O2<\/sub>\u7535\u6c60\u5728\u957f\u5faa\u73af\u548c\u5b9e\u9645\u5e94\u7528\u4e2d\u5145\u6ee1\u6311\u6218\u3002\u867d\u7136\u57fa\u4e8e\u6781\u6027\u975e\u8d28\u5b50\u7684N, N\u4e8c\u7532\u57fa\u4e59\u9170\u80fa\uff08DMA\uff09\u7535\u89e3\u8d28\u80fd\u8010\u53d7Li-O2<\/sub>\u7535\u6c60\u7684\u82db\u523b\u6c27\u5316\u73af\u5883\uff0c\u4f46\u662fLi\u91d1\u5c5e\u7684\u4e25\u91cd\u4e0d\u7a33\u5b9a\u6027\uff0c\u4e0d\u4ec5\u4f1a\u8fde\u7eed\u5206\u89e3\u7535\u89e3\u8d28\uff0c\u800c\u4e14\u8fd8\u4f1a\u635f\u8017Li\u91d1\u5c5e\u3002\u540c\u65f6\uff0c\u8fd8\u5b58\u5728Li\u91d1\u5c5e\u8d1f\u6781\u751f\u957f\u679d\u6676\u7684\u95ee\u9898\u3002\u5229\u7528\u7535\u89e3\u8d28\u6dfb\u52a0\u5242\u5728Li\u91d1\u5c5e\u8d1f\u6781\u4e0a\u5f62\u6210\u4fdd\u62a4\u5c42\u53ef\u4ee5\u63d0\u9ad8\u6027\u80fd\uff0c\u4f46\u662f\u8fd9\u4e9b\u4fdd\u62a4\u5c42\u5728\u957f\u5faa\u73af\u4e2d\u6613\u7834\u88c2\u800c\u5931\u53bb\u4f5c\u7528\u3002\u56e0\u6b64\uff0c\u8feb\u5207\u9700\u8981\u8bbe\u8ba1\u4e00\u79cd\u65b0\u7684\u7535\u89e3\u8d28\u4ee5\u514b\u670dDMA\u57fa\u7535\u89e3\u8d28\u7684\u7f3a\u70b9\uff0c\u540c\u65f6\u4fdd\u6301\u5176\u4f18\u52bf\uff0c\u4ece\u800c\u83b7\u5f97\u5177\u6709\u9ad8\u7535\u5316\u5b66\u6027\u80fd\u7684DMA\u57faLi-O2<\/sub>\u7535\u6c60\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u57fa\u4e8e\u6b64\uff0c\u4e2d\u79d1\u9662\u957f\u6625\u5e94\u7528\u5316\u5b66\u7814\u7a76\u6240\u7684\u5f20\u65b0\u6ce2\u7814\u7a76\u5458\uff08\u901a\u8baf\u4f5c\u8005\uff09\u56e2\u961f<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u65b0\u7684\u7535\u89e3\u8d28\u8bbe\u8ba1\u7b56\u7565\uff0c\u57fa\u4e8eDMA\u7535\u89e3\u8d28\u6765\u5b9e\u73b0Li-O2<\/sub>\u7535\u6c60\u7684\u957f\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u4f5c\u8005\u901a\u8fc7\u8c03\u8282Li+<\/sup>\u6eb6\u5242\u5316\u7ed3\u6784\u6765\u8c03\u63a7\u4e2d\u7b49\u7535\u89e3\u8d28\u6d53\u5ea6\u7684SEI\u819c\u548c\u6e38\u79bb\u6eb6\u5242\u5206\u5b50\uff0c\u514b\u670d\u4e86\u7535\u89e3\u8d28\u6d53\u5ea6\u7684\u7f3a\u70b9\uff0c\u751a\u81f3\u8d85\u8fc7\u5176\u4f18\u70b9\u3002\u5229\u7528ab initio\u5206\u5b50\u52a8\u529b\u5b66\uff08AIMD\uff09\u6a21\u62df\u548c\u7535\u5316\u5b66\u5206\u6790\u53d1\u73b0\uff0c\u5728DMA\u4e2d\u4f7f\u75282 M LiTFSI\u548c1 M LiNO3<\/sub>\u6765\u4f18\u5316\u7535\u89e3\u8d28\uff0c\u4f7f\u5f97Li\u8d1f\u6781\u5177\u6709\u4f18\u5f02\u7684\u6291\u5236\u679d\u6676\u548c\u8150\u8680\u7684\u4f5c\u7528\uff0c\u5e76\u4e14\u8868\u73b0\u51fa\u589e\u5f3a\u7684\u52a8\u529b\u5b66\u548c\u4f20\u8d28\u8fc7\u7a0b\u3002\u5b9e\u9a8c\u7ed3\u679c\u8868\u660e\uff0cLi\/Li\u5bf9\u79f0\u7535\u6c60\u548cLi-O2<\/sub>\u7535\u6c60\u7684\u5faa\u73af\u5bff\u547d\u5206\u522b\u5ef6\u957f\u52301800 h\u548c180\u6b21\u5faa\u73af\uff0c\u662f\u5df2\u62a5\u9053\u7684DMA\u57fa\u7535\u6c60\u7684\u6700\u4f73\u7535\u5316\u5b66\u6027\u80fd\u3002\u8be5\u7814\u7a76\u4e3a\u7535\u89e3\u8d28\u8c03\u8282\u7b56\u7565\u6ce8\u5165\u4e86\u65b0\u7684\u6d3b\u529b\uff0c\u5e76\u4e3a\u78b1\u91d1\u5c5e-O2<\/sub>\u7535\u6c60\u7684\u5f00\u53d1\u63d0\u4f9b\u6765\u65b0\u4e1d\u8def\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cA Renaissance of N,N-Dimethylacetamide-Based Electrolyte to Promote the Cycling Stability of Li-O2<\/sub> Batteries<\/strong> \u201d\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aEnergy Environ. Sci.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001Li\u91d1\u5c5e\u8d1f\u6781\u5728\u4e0d\u540c\u79cd\u7c7b\u7684DMA\u57fa\u7535\u89e3\u8d28\u4e2d\u7684\u7a33\u5b9a\u6027<\/strong>
\n \"\"\uff08a\uff09\u5177\u6709\u4e0d\u540c\u6d53\u5ea6LiTFSI\u7535\u89e3\u8d28\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u8d85\u7535\u52bf-\u5faa\u73af\u6b21\u6570\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09\u5177\u6709\u4e0d\u540c\u6d53\u5ea6LiNO3<\/sub>\u7535\u89e3\u8d28\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u8d85\u7535\u52bf-\u5faa\u73af\u6b21\u6570\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u5177\u6709\u4e0d\u540c\u6d53\u5ea6LiNO3<\/sub>\u548cLiTFSI\u7ec4\u6210\u7535\u89e3\u8d28\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u8d85\u7535\u52bf-\u5faa\u73af\u6b21\u6570\u66f2\u7ebf\uff1b<\/p>\n

\uff08d-f\uff09\u4e0d\u540c\u6d53\u5ea6\u7684LiTFSI\u7535\u89e3\u8d28\u3001LiNO3<\/sub>\u7535\u89e3\u8d28\u548c3 M\u7535\u89e3\u8d28\u7ec4\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u5faa\u73af\u5bff\u547d\u7684\u76f4\u65b9\u56fe\uff1b<\/p>\n

\uff08g-i\uff09\u5177\u67094 M LiTFSI\u30015 M LiNO3<\/sub>\u548c2 M LiTFSI 1 M LiNO3<\/sub>\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u6027\u80fd\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e8c\u3001Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong>
\n \"\"\uff08a-b\uff09\u5177\u6709\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a0.1 mA cm-2<\/sup>\u548c1 mA cm-2<\/sup>\u65f6\u7684\u957f\u671f\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08c\uff09Li\/Li\u5bf9\u79f0\u7535\u6c60\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u901f\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08d\uff09\u6bd4\u8f83DMA\u57faLi\/Li\u5bf9\u79f0\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08e-f\uff09Li\/Li\u5bf9\u79f0\u7535\u6c60\u5728\u5faa\u73af\u524d\u548c\u5faa\u73af80 h\u540e\u7684\u5948\u594e\u65af\u7279\u56fe\uff1b<\/p>\n

\uff08g\uff09\u4e0d\u540c\u79cd\u7c7b\u7684\u7535\u89e3\u8d28\u7684\u963f\u7d2f\u5c3c\u4e4c\u65af\uff08Arrhenius\uff09\u66f2\u7ebf\uff1b<\/p>\n

\uff08h\uff09Li\/Li\u5bf9\u79f0\u7535\u6c60\u4e2d\u7684Rct\u7684Arrhenius\u56fe\u548c\u76f8\u5e94\u7684\u6fc0\u6d3b\u80fd\uff1b<\/p>\n

\uff08i\uff09\u5177\u6709\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684Li\/Li\u5bf9\u79f0\u7535\u6c60\u7684CV\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e09\u3001Li\u6c89\u79ef\u5f62\u6001\u548cSEI\u819c\u6210\u5206\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08a-c\uff095 M LiNO3<\/sub>\u30014 M LiTFSI\u548c2 M LiTFSI 1 M LiNO3<\/sub>\u4e2dLi\u6c89\u79ef\u5f62\u6001\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d-i\uff09\u5206\u522b\u57284 M LiTFSI\u30015M LiNO3<\/sub>\u548c2 M LiTFSI 1M LiNO3<\/sub>\u4e2d\u6c89\u79ef0\u548c30 min\u540e\uff0cLi\u5f62\u6001\u6f14\u53d8\u7684\u539f\u4f4d\u5149\u5b66\u663e\u5fae\u955c\u56fe\u50cf\uff1b<\/p>\n

\uff08j\uff09\u5728\u4e0d\u540c\u79cd\u7c7b\u7684\u7535\u89e3\u8d28\u4e2dLi\u6c89\u79ef\u6f14\u53d8\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08k-m\uff09\u8680\u523b5 min\u524d\u540e\uff0c\u57284 M LiTFSI\u30015 M LiNO3<\/sub>\u548c2 M LiTFSI 1 M LiNO3<\/sub>\u4e2d\u8fdb\u884c40\u6b21\u5faa\u73af\u540e\uff0cLi\u7684Li 1s XPS\u5149\u8c31\u3002<\/p>\n

\u56fe\u56db\u3001AIMD\u6a21\u62df\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u4e2d\u7684\u7535\u89e3\u8d28\u6eb6\u5242\u7ed3\u6784<\/strong>
\n \"\"\uff08a-d\uff09AIMD\u6a21\u62df\u76d2\u7684\u5feb\u7167\uff0c\u5176\u4e2d\u5305\u542b3 M LiTFSI\u30012 M LiTFSI 1 M LiNO3<\/sub>\u30014 M LiTFSI\u548c5 M LiNO3<\/sub>\u7535\u89e3\u8d28\uff1b<\/p>\n

\uff08e-f\uff093 M LiTFSI\u548c2 M LiTFSI 1 M LiNO3<\/sub>\u7535\u89e3\u8d28\u4e2d\u7684\u6eb6\u5242\u5316\u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08g-h\uff09Li-O\u548cLi-N\u5728\u4e0d\u540c\u79cd\u7c7b\u7684\u7535\u89e3\u8d28\u4e2d\u7684\u81ea\u7531\u57fa\u5206\u5e03\u51fd\u6570\uff1b<\/p>\n

\uff08i\uff09\u4f5c\u4e3a\u6a21\u62df\u65f6\u95f4\u7684\u51fd\u6570\u7684\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684MSD\u3002<\/p>\n

\u56fe\u4e94\u3001Li-O2<\/sub>\u7535\u6c60\u7684\u7535\u5316\u5b66\u7279\u6027<\/strong>
\n \"\"\uff08a\uff09\u542b2 M LiTFSI 1 M LiNO3<\/sub> DMA\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u5177\u6709\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684Li-O2<\/sub>\u7535\u6c60\u5728\u7b2c1\u6b21\u5faa\u73af\u3001\u7b2c50\u6b21\u5faa\u73af\u7684\u653e\/\u5145\u7535\u66f2\u7ebf\uff0c\u4ee5\u53ca\u8fc7\u7535\u52bf\u6bd4\u8f83\u7684\u76f8\u5e94\u76f4\u65b9\u56fe\uff1b<\/p>\n

\uff08e\uff09\u5e26\u6709\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u901f\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08f\uff09\u4f7f\u7528\u4e0d\u540c\u79cd\u7c7b\u7535\u89e3\u8d28\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u957f\u671f\u5faa\u73af\u5bff\u547d\uff1b<\/p>\n

\uff08g\uff09\u672c\u6587\u548c\u5df2\u62a5\u9053\u7684\u57fa\u4e8eDMA\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u6982\u8ff0\u3002<\/p>\n

\uff08h-i\uff09\u572850\u6b21\u5faa\u73af\u540e\uff0c\u4f7f\u75282 M LiTFSI 1 M LiNO3<\/sub> DMA\u57faLi-O2<\/sub>\u7535\u6c60\u4e2dLi\u91d1\u5c5e\u8d1f\u6781\u7684SEM\u56fe\u548cXRD\u56fe\uff1b<\/p>\n

\uff08j\uff09\u6bd4\u8f83\u4e09\u79cd\u57fa\u4e8e\u7535\u89e3\u8d28\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u6027\u80fd\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aA Renaissance of N, N-Dimethylacetamide-Based Electrolyte to Promote the Cycling Stability of Li-O2<\/sub> Batteries<\/a><\/strong> .\uff08Energy Environ. Sci.<\/em>, 2020<\/strong>, DOI: 10.1039\/D0EE01897J\uff09<\/p>\n

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