{"id":205864,"date":"2020-07-22T06:30:50","date_gmt":"2020-07-21T22:30:50","guid":{"rendered":"\/\/m.iemloyee.com\/?p=205864"},"modified":"2020-07-22T10:39:09","modified_gmt":"2020-07-22T02:39:09","slug":"%e3%80%90%e6%8a%95%e7%a8%bf%e3%80%91%e4%b8%ad%e5%8d%97%e5%a4%a7%e5%ad%a6mte%e5%b0%81%e9%9d%a2%e9%94%8c%e7%94%b5%e6%b1%a0%e6%96%87%e7%ab%a0-%e6%b0%b4%e7%b3%bbzn-mno2%e7%94%b5%e6%b1%a0%e6%ba%b6","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=205864","title":{"rendered":"\u4e2d\u5357\u5927\u5b66MTE\u5c01\u9762\u950c\u7535\u6c60\u6587\u7ae0:\u00a0\u6c34\u7cfbZn\/MnO2\u7535\u6c60\u6eb6\u89e3-\u6c89\u79ef\u673a\u7406"},"content":{"rendered":"

\"\"<\/b><\/strong><\/p>\n

MTE\u5c01\u9762\uff0c2020\u5e746\u6708<\/b><\/strong>\u7b2c<\/b><\/strong>16\u671f<\/b><\/strong>\u3002<\/b><\/strong><\/p>\n

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\u4e00\u7f15\u66d9\u5149\uff0c\u9ece\u660e\u5c31\u8981\u5230\u6765\uff01<\/b><\/strong><\/p>\n

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u5357\u5927\u5b66\u5468\u6c5f\u3001\u6881\u53d4\u5168\u6559\u6388<\/b><\/strong>\u7b49\u4eba\u5728\u56fd\u9645\u671f\u520aMaterials Today Energy\u4e0a\u53d1\u8868\u9898\u4e3a\u201cZn\/MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0Battery Chemistry with Dissolution-Deposition Mechanism<\/b><\/strong>\u201d\u7684\u6700\u65b0\u7814\u7a76\u6210\u679c\u3002\u8be5\u6587\u7ae0\u63d0\u51fa\u4e86\u5728\u5fae\u9178\u6027\u7535\u89e3\u6db2\u4e0bZn\/MnO2<\/sub>\u7535\u6c60\u4e2d\u5360\u636e\u4e3b\u5bfc\u5730\u4f4d\u7684\u6eb6\u89e3-\u6c89\u79ef\u673a\u7406\u3002\u4f5c\u8005\u5408\u6210\u4e86\u03b1-MnO2<\/sub>\uff0c\u03b4-MnO2<\/sub>\u00a0\u548cZn4<\/sub>SO4<\/sub>(OH)6<\/sub>\u00b74H2<\/sub>O (ZHS)\uff0c\u901a\u8fc7\u8868\u5f81\u4ed6\u4eec\u7684\u7535\u5316\u5b66\u884c\u4e3a\u548c\u53cd\u5e94\u4ea7\u7269\uff0c\u8bc1\u660e\u4ed6\u4eec\u5747\u9075\u5faa\u76f8\u540c\u7684\u6eb6\u89e3-\u6c89\u79ef\u673a\u7406\uff0c\u5e76\u5bf9\u9996\u5708\u5e93\u4f26\u6548\u7387\u548c\u5bb9\u91cf\u8870\u51cf\u8fdb\u884c\u4e86\u5408\u7406\u89e3\u91ca\u3002\u63a5\u4e0b\u6765\u4ee5\u63a7\u5236\u5355\u4e00\u53d8\u91cf\u4e3a\u6838\u5fc3\u6307\u5bfc\u601d\u60f3\u3002\u901a\u8fc7\u5bf9\u653e\u7535\u540e\u7535\u89e3\u6db2\u4e2dMn2+<\/sup>\u542b\u91cf\u7684\u68af\u5ea6\u8c03\u63a7\uff0c\u89c2\u5bdf\u63a5\u4e0b\u6765\u5145\u7535\u8fc7\u7a0b\u4e2d\u7684\u7535\u5316\u5b66\u884c\u4e3a\uff0c\u8bc1\u5b9e\u4e86\u6eb6\u89e3-\u6c89\u79ef\u673a\u7406\u5728\u50a8\u80fd\u8fc7\u7a0b\u4e2d\u5360\u636e\u7684\u4e3b\u5bfc\u4f5c\u7528\u3002\u5bf9\u653e\u7535\u53cd\u5e94\u526f\u53cd\u5e94\u4ea7\u7269ZHS\u4e0d\u540c\u7a0b\u5ea6\u7684\u53bb\u9664\uff0c\u4ee5\u8fdb\u884c\u4e0d\u540c\u7684\u6d4b\u8bd5\uff0c\u4f5c\u8005\u8bc1\u660e\u4e86ZHS\u901a\u8fc7\u63a7\u5236\u6d3b\u6027\u6c34\u7684\u65b9\u5f0f\u6291\u5236\u4e86\u6eb6\u89e3\u53cd\u5e94\u7684\u8fdb\u884c\uff0c\u4f7f\u5f97\u6574\u4e2a\u7cfb\u7edf\u96be\u4ee5\u8fbe\u5230\u7406\u8bba\u5bb9\u91cf\u3002\u4f46\u540c\u65f6ZHS\u4e5f\u5438\u6536\u4e86\u6eb6\u6db2\u4e2d\u5927\u91cf\u751f\u6210\u7684OH–<\/sup>\u79bb\u5b50\uff0c\u5bf9\u6574\u4e2a\u53cd\u5e94\u52a8\u529b\u5b66\u8d77\u5230\u4e86\u590d\u6742\u800c\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u4e0a\u8ff0\u52a8\u529b\u5b66\u9650\u5236\u56e0\u7d20\u7684\u63a2\u7a76\u4e3a\u5b9e\u73b0\u7406\u8bba\u5bb9\u91cf\u63d0\u4f9b\u4e86\u5408\u7406\u7684\u6307\u5bfc\u601d\u8def\u3002<\/p>\n

\u3010\u7814\u7a76\u521b\u65b0\u70b9\u3011<\/b><\/strong><\/p>\n

1. \u6df1\u5165\u7814\u7a76Zn\/MnO2<\/sub>\u7535\u6c60\u6eb6\u89e3\/\u6c89\u79ef\u50a8\u80fd\u673a\u7406\uff0c\u5e76\u8bc1\u5b9e\u4e86\u6eb6\u89e3\/\u6c89\u79ef\u673a\u7406\u5728\u50a8\u80fd\u8fc7\u7a0b\u4e2d\u5360\u636e\u7684\u4e3b\u5bfc\u5730\u4f4d\uff1b<\/p>\n

2. \u9530\u6eb6\u89e3\uff0cpH\u6539\u53d8\uff0c\u521d\u59cb\u5e93\u4f26\u6548\u7387\u548c\u5bb9\u91cf\u8870\u51cf\u673a\u7406\u7b49\u96be\u4ee5\u7406\u89e3\u7684\u5b9e\u9a8c\u73b0\u8c61\u5728\u6b64\u5f97\u5230\u4e86\u6b63\u786e\u7684\u8ba4\u8bc6\u548c\u5408\u7406\u7684\u89e3\u91ca\uff1b<\/p>\n

3. \u57fa\u4e8e\u6eb6\u89e3\/\u6c89\u79ef\u673a\u7406\uff0c\u8be6\u7ec6\u63a2\u8ba8\u4e86\u53cd\u5e94\u52a8\u529b\u5b66\u7684\u4e3b\u8981\u9650\u5236\u56e0\u7d20\uff0c\u4f8b\u5982ZHS\u548c\u6d3b\u6027H2<\/sub>O\uff1b<\/p>\n

4. \u5bf9\u4e8e\u50a8\u80fd\u673a\u7406\u7684\u6df1\u523b\u8ba4\u8bc6\u4e3a\u4ee5\u540e\u8fbe\u5230\u7406\u8bba\u5bb9\u91cf\u63d0\u4f9b\u4e86\u575a\u5b9e\u7684\u7406\u8bba\u57fa\u7840\uff0c\u5e76\u9488\u5bf9\u672a\u6765\u7684Zn\/MnO2<\/sub>\u7535\u6c60\u53d1\u5c55\u63d0\u51fa\u4e86\u76f8\u5e94\u7684\u4f18\u5316\u7b56\u7565\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe\u4e00\u3001MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u548cZHS\u7684\u53cd\u5e94\u4ea7\u7269\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a) \u03b1-MnO2<\/sub>\u7684\u975e\u539f\u4f4dXRD\u56fe\uff1b<\/p>\n

(b) \u03b4-MnO2<\/sub>\u7684\u975e\u539f\u4f4dXRD\u56fe\uff1b<\/p>\n

(c) ZHS\u5728\u4e0d\u540c\u7535\u89e3\u6db2\u6d53\u5ea6\u4e0b\u9996\u5708\u7684\u5145\u653e\u7535\u5bb9\u91cf\u548c\u5e93\u4f26\u6548\u7387\u3002<\/p>\n

(d) ZHS\u7684\u975e\u539f\u4f4dXRD\u56fe\uff1b<\/p>\n

(e) ZHS\u7535\u6781\u9996\u5708\u5145\u7535\u540e\u7684SEM\u56fe\u3002<\/p>\n

(f) ZHS\u7535\u6781\u9996\u5708\u653e\u7535\u540e\u7684SEM\u56fe\u3002<\/p>\n

\u56fe\u4e8c\u3001\u5bf9\u653e\u7535\u540e\u7535\u89e3\u6db2\u4f53\u7cfb\u4e2dMn<\/b><\/strong>2+<\/b><\/sup><\/strong>\u542b\u91cf\u7684\u68af\u5ea6\u8c03\u63a7\uff0c\u7814\u7a76\u540e\u7eed\u5145\u7535\u8fc7\u7a0b\u4e2d\u7684\u7535\u5316\u5b66\u884c\u4e3a<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

(a)\u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u57282M ZnSO4<\/sub>\u7535\u89e3\u6db2\u4e2d\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

(b)\u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u57282M ZnSO4<\/sub>\u7535\u89e3\u6db2\u4e2d\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

(c)\u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u57282M ZnSO4<\/sub>+x<\/i><\/em>M MnSO4<\/sub>\u7b49\u4e0d\u540c\u7535\u89e3\u6db2\u4e2d\u7684\u5bb9\u91cf\u548c\u5e93\u4f26\u6548\u7387\uff1b<\/p>\n

(d)\u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u57282M ZnSO4<\/sub>+x<\/i><\/em>M MnSO4<\/sub>\u7b49\u4e0d\u540c\u7535\u89e3\u6db2\u4e2d\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e09\u3001<\/b><\/strong>\u5bf9ZHS\u4e0d\u540c\u7a0b\u5ea6\u7684\u53bb\u9664\uff0c\u8bc1\u660eZHS\u5bf9\u53cd\u5e94\u52a8\u529b\u5b66\u8d77\u5230\u4e86\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u8fdb\u4e00\u6b65\u5728\u918b\u9178\u7f13\u51b2\u6db2\u4e2d\u6e05\u6d1720\u5206\u949f\u540e,\u4ee5\u53bb\u9664\u8868\u9762\u5305\u8986\u7684ZHS\u3002\u5c06\u5f97\u5230\u7684\u7535\u6781\u7247\u57282M ZnSO4<\/sub>\u7535\u89e3\u6db2\u4e2d\u7ec4\u88c5\u6210\u7535\u6c60\uff0c\u6d4b\u8bd5\u5f97\u5230<\/p>\n

(a) \u5faa\u73af\u6027\u80fd<\/p>\n

(b) \u5145\u653e\u7535\u66f2\u7ebf<\/p>\n

(c) ZHS\u5bf9\u53cd\u5e94\u8d77\u5230\u4f5c\u7528\u7684\u56fe\u89e3<\/p>\n

(d) \u5904\u7406\u540e\u7684\u03b1-MnO2<\/sub>(D0.8V) \u7535\u6781\u8fdb\u4e00\u6b65\u5728\u918b\u9178\u7f13\u51b2\u6db2\u4e2d\u6e05\u6d17\u4e0d\u540c\u65f6\u95f4,\u4ee5\u5f97\u5230\u8868\u9762\u5305\u8986\u4e0d\u540c\u7684ZHS\u3002\u5c06\u5f97\u5230\u7684\u7535\u6781\u7247\u57282M ZnSO4<\/sub>\u7535\u89e3\u6db2\u4e2d\u7ec4\u88c5\u6210\u7535\u6c60\uff0c\u518d\u6b21\u653e\u7535\u6d4b\u8bd5\u5f97\u5230\u6027\u80fd\u3002<\/p>\n

(e) \u03b1-MnO2<\/sub>\u00a0\u5728\u4e0d\u540c\u653e\u7535\u9636\u6bb5\u7684EIS\u56fe\u3002<\/p>\n

\u56fe\u56db\u3001Zn\/MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0\u7535\u6c60\u50a8\u80fd\u673a\u7406\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5: Zn\/MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0Battery Chemistry with Dissolution-Deposition Mechanism<\/b><\/strong>, Materials Today Energy,\u00a02020, 16, 100396.<\/p>\n

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