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\u4eba\u7269\u4ecb\u7ecd\uff1a<\/b><\/strong><\/p>\n

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1<\/b><\/strong>\u3001Nat.<\/b><\/strong>\u00a0Com<\/b><\/strong>mun<\/b><\/strong>. <\/b><\/strong>\u4e8c\u6c27\u5316\u7845\u7eb3\u7c73\u94f8\u5165M<\/b><\/strong>OF<\/b><\/strong>s\u4e2d\u5bf9\u9ad8\u8d1f\u8f7d\u94c1\u5355\u539f\u5b50\u7535\u50ac\u5316\u5242\u5b9e\u73b0\u53cc\u91cd\u4fdd\u62a4\u4f5c\u7528<\/b><\/strong>[1]<\/b><\/sup><\/strong><\/p>\n

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2<\/b><\/strong>\u3001<\/b><\/strong>Nat<\/b><\/strong>.<\/b><\/strong>\u00a0Nanotechnol.<\/b><\/strong>\u00a0\u65b0\u578b\u78c1\u5149\u7eb3\u7c73\u6750\u6599\u8bf1\u5bfc\u624b\u6027\u5149\u5b66\u6d3b\u6027<\/b><\/strong>[<\/b><\/sup><\/strong>2<\/b><\/sup><\/strong>]<\/b><\/sup><\/strong><\/p>\n

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3<\/b><\/strong>\u3001Sci.<\/b><\/strong>\u00a0Adv. <\/b><\/strong>\u5de5\u7a0b\u5851\u6599\u66ff\u4ee3\u54c1\uff1a\u7c7b\u5929\u7136\u7eb3\u7c73\u7ea4\u7ef4\u7d20\u9ad8\u6027\u80fd\u7ed3\u6784\u6750\u6599<\/b><\/strong>[<\/b><\/sup><\/strong>3<\/b><\/sup><\/strong>]<\/b><\/sup><\/strong><\/p>\n

\u5851\u6599\u7684\u4f7f\u7528\u7ed9\u4eba\u7c7b\u5e26\u6765\u4e86\u5f88\u591a\u4fbf\u6377\u4e4b\u5904\uff0c\u4f46\u5374\u5f15\u53d1\u4e86\u5851\u6599\u707e\u96be\u3002\u56e0\u6b64\u5f00\u53d1\u53ef\u751f\u7269\u964d\u89e3\u3001\u91cd\u91cf\u8f7b\u3001\u70ed\u5c3a\u5bf8\u7a33\u5b9a\u6027\u597d\u3001\u529b\u5b66\u6027\u80fd\u4f18\u826f\u7684\u53ef\u6301\u7eed\u6750\u6599\u81f3\u5173\u91cd\u8981\uff0c\u4f46\u6750\u6599\u67d0\u4e9b\u6027\u80fd\uff08\u5982\u5f3a\u5ea6\u3001\u97e7\u6027\uff09\u5f88\u96be\u540c\u65f6\u517c\u5f97\u3002\u57fa\u4e8e\u6b64\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u4fde\u4e66\u5b8f\u9662\u58eb\u56e2\u961f<\/b><\/strong>\u7814\u53d1\u4e86\u4e00\u79cd\u65b0\u578b\u7eb3\u7c73\u7ea4\u7ef4\u4eff\u751f\u6750\u6599\u7684\u5236\u5907\u65b9\u6cd5\uff0c\u901a\u8fc7\u751f\u7269\u5408\u6210\u4ece\u8461\u8404\u7cd6\u4e2d\u4ea7\u751f\u575a\u56fa\u7684\u4e09\u7ef4\u7eb3\u7c73\u7ea4\u7ef4\u7f51\u7edcCNF\u6c34\u51dd\u80f6\uff0c\u7136\u540e\u5229\u7528\u4e0d\u540c\u805a\u5408\u7269\u6eb6\u6db2\u5904\u7406\u6216\u8868\u9762\u4fee\u9970\uff0c\u7136\u540e\u591a\u5c42\u538b\u5236\u6210\u9ad8\u6027\u80fd\u5757\u72b6\u7ed3\u6784\u6750\u6599\uff08CNFP\uff09\u3002\u6240\u5236\u5907\u7684\u9ad8\u6027\u80fd\u5757\u72b6\u7ed3\u6784\u6750\u6599\uff08CNFP\uff09\u5177\u6709\u4f18\u5f02\u7684\u7efc\u5408\u6027\u80fd\u2014\u6781\u4f4e\u7684\u5bc6\u5ea6\uff0c\u4f18\u5f02\u7684\u5f3a\u5ea6\u548c\u97e7\u6027\uff0c\u826f\u597d\u7684\u70ed\u5c3a\u5bf8\u7a33\u5b9a\u6027\u3002\u4e0e\u5178\u578b\u7684\u805a\u5408\u7269\u3001\u91d1\u5c5e\u548c\u9676\u74f7\u76f8\u6bd4\uff0c\u5b83\u8868\u73b0\u51fa\u72ec\u7279\u800c\u4f18\u8d8a\u7684\u6027\u80fd\uff0c\u4f7f\u5176\u6210\u4e3a\u6ee1\u8db3\u5de5\u7a0b\u8981\u6c42\uff08\u5c24\u5176\u662f\u822a\u5929\u5668\u6750\u6599\uff09\u7684\u4f4e\u6210\u672c\uff0c\u9ad8\u6027\u80fd\u548c\u73af\u5883\u53cb\u597d\u578b\u66ff\u4ee3\u4ea7\u54c1\u3002\u800c\u4e14CNFP\u5177\u6709\u6781\u9ad8\u7684\u6297\u51b2\u51fb\u6027\u80fd\u3001\u9ad8\u635f\u4f24\u5bb9\u9650\u548c\u9ad8\u80fd\u91cf\u5438\u6536\u6027\u80fd\uff0c\u53ef\u4ee5\u4ee5\u4f4e\u6210\u672c\u5b9e\u73b0\u5176\u5927\u89c4\u6a21\u751f\u4ea7\u3002CNFP\u6709\u671b\u6210\u4e3a\u8fc7\u7a0b\u5851\u6599\u7684\u66ff\u4ee3\u54c1\uff0c\u5177\u6709\u6781\u5176\u5e7f\u9614\u7684\u524d\u666f\u3002<\/p>\n

\"\"<\/p>\n

\u56fe3<\/b><\/strong>. <\/b><\/strong>\u7ea4\u7ef4\u7d20\u7eb3\u7c73\u7ea4\u7ef4\u7ed3\u6784\u6750\u6599\uff08CNFP\uff09\u7684\u5236\u5907\u8fc7\u7a0b\u3001\u7ed3\u6784\u793a\u610f\u56fe\u3001\u6837\u54c1\u7167\u7247\u548c\u53ef\u52a0\u5de5\u6027\u80fd\u5c55\u793a\u3002<\/p>\n

4<\/b><\/strong>\u3001<\/b><\/strong>S<\/b><\/strong>ci<\/b><\/strong>. Adv<\/b><\/strong>.<\/b><\/strong>\u00a0<\/b><\/strong>\u57fa\u4e8e\u94c1\u78b3\u9178\u9499\u7eb3\u7c73\u836f\u7269\u8bf1\u5bfc\u80bf\u7624\u7ec6\u80de\u9776\u5411\u94c1\u6b7b\u4ea1<\/b><\/strong>[<\/b><\/sup><\/strong>4<\/b><\/sup><\/strong>]<\/b><\/sup><\/strong><\/p>\n

\u80bf\u7624\u8010\u836f\u6027\u7684\u8fc5\u901f\u53d1\u5c55\u6210\u4e3a\u4e34\u5e8a\u80bf\u7624\u6cbb\u7597\u7684\u6280\u672f\u74f6\u9888\u3002\u94c1\u6b7b\u4ea1\uff08ferroptosis\uff09\u662f\u4e00\u79cd\u5177\u6709\u4e34\u5e8a\u8f6c\u5316\u6f5c\u529b\u7684\u8c03\u63a7\u7ec6\u80de\u6b7b\u4ea1\u5f62\u5f0f\uff0c\u4f46\u5355\u72ec\u4f7f\u7528\u94c1\u8bf1\u5bfc\u5242\u7684\u7597\u6548\u6613\u53d7\u8bb8\u591a\u5185\u6e90\u6027\u56e0\u7d20\u7684\u5f71\u54cd\uff0c\u5e76\u4e14\u5982\u4f55\u5b9e\u73b0\u764c\u7ec6\u80de\u9776\u5411\u94c1\u6b7b\u4ea1\u4ecd\u7136\u662f\u4e9f\u5f85\u89e3\u51b3\u7684\u96be\u9898\u3002\u4e3a\u4e86\u89e3\u51b3\u4ee5\u4e0a\u95ee\u9898\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u4fde\u4e66\u5b8f\u9662\u58eb\u56e2\u961f\u4e0e\u91cd\u5e86\u5927\u5b66\u7f57\u5fe0\u6559\u6388\u8bfe\u9898\u7ec4<\/b><\/strong>\u5408\u4f5c\u901a\u8fc7\u4e00\u6b65\u539f\u4f4d\u751f\u957f\u5236\u5907\u65e0\u5b9a\u5f62\u542b\u94c1\u78b3\u9178\u9499\u7eb3\u7c73\u836f\u7269\u7ec4\u88c5\u4f53\uff08ACC@DOX.Fe2+-CaSi-PAMAM-FA\/mPEG\uff09\u3002Fe2+<\/sup>\u548c\u963f\u9709\u7d20\u4e4b\u95f4\u7edc\u5408\u4f5c\u7528\u6700\u5927\u7a0b\u5ea6\u51cf\u5c11\u4e86\u836f\u7269\u8fc7\u65e9\u91ca\u653e\uff0c\u7eb3\u7c73\u836f\u7269\u8868\u9762\u4fee\u9970PEG\u548c\u53f6\u9178\u5206\u5b50\uff0c\u63d0\u9ad8\u4e86\u6750\u6599\u7684\u8840\u6db2\u5faa\u73af\u65f6\u95f4\u548c\u80bf\u7624\u9776\u5411\u6027\u3002\u7eb3\u7c73\u836f\u7269\u5728\u80bf\u7624\u7ec6\u80de\u5fae\u73af\u5883\u7684\u523a\u6fc0\u4e0b\u53d1\u751f\u964d\u89e3\uff0c\u963f\u9709\u7d20\u4e0eFe2+<\/sup>\u7684\u914d\u4f4d\u5171\u4f20\u8f93\u80fd\u6700\u5927\u7a0b\u5ea6\u589e\u5f3a\u5176\u7597\u6548\uff0c\u901a\u8fc7\u534f\u540c\u4f5c\u7528\u5b9e\u73b0\u764c\u7ec6\u80de\u94c1\u6b7b\u4ea1\u548c\u5316\u7597\uff0c\u7eb3\u7c73\u836f\u7269\u7ec4\u88c5\u4f53\u7684\u6297\u80bf\u7624\u6548\u679c\u5728\u6d3b\u4f53\u5b9e\u9a8c\u4e5f\u5f97\u5230\u8bc1\u5b9e\u5e76\u4e14\u964d\u4f4e\u963f\u9709\u7d20\u7684\u6bd2\u526f\u4f5c\u7528\u3002\u6b64\u7814\u7a76\u4e2d\u6240\u63d0\u51fa\u7684\u4eff\u751f\u81ea\u7ec4\u88c5\u6280\u672f\u5b9e\u73b0\u9776\u5411\u94c1\u6b7b\u4ea1\u548c\u5316\u7597\u7684\u7b56\u7565\u4e3a\u5f00\u53d1\u65b0\u7684\u80bf\u7624\u4e34\u5e8a\u6cbb\u7597\u65b9\u6cd5\u63d0\u4f9b\u4e86\u65b0\u601d\u8def\uff0c\u5177\u6709\u5e7f\u9614\u7684\u5e94\u7528\u524d\u666f\u3002<\/p>\n

\"\"<\/p>\n

\u56fe4<\/b><\/strong>. <\/b><\/strong>\u7eb3\u7c73\u836f\u7269\u7ec4\u88c5\u4f53\uff08ACC@DOX.Fe2+-CaSi-PAMAM-FA\/mPEG\uff09\u7684\u5408\u6210\u53ca\u5176\u5f15\u53d1\u764c\u7ec6\u80de\u94c1\u6b7b\u4ea1\u3001\u51cb\u4ea1\u793a\u610f\u56fe\u3002<\/p>\n

5<\/b><\/strong>\u3001J.<\/b><\/strong>\u00a0Am. Chem. Soc. <\/b><\/strong>\u901a\u8fc7\u4e2d\u95f4\u9650\u5236\u4fdd\u62a4\u94dc\u7684\u6c27\u5316\u72b6\u6001\u4ee5\u62e9\u6027\u7684\u4e8c\u6c27\u5316\u78b3\u7535\u8fd8\u539f\u4e3aC<\/b><\/strong>2+<\/b><\/sub><\/strong>\u71c3\u6599<\/b><\/strong>[<\/b><\/sup><\/strong>5<\/b><\/sup><\/strong>]<\/b><\/sup><\/strong><\/p>\n

\u4e8c\u6c27\u5316\u78b3\uff08CO2<\/sub>\uff09\u7535\u5316\u5b66\u50ac\u5316\u8f6c\u5316\u4e3a\u71c3\u6599\u548c\u6709\u4ef7\u503c\u7684\u539f\u6599\u662f\u5f53\u524d\u5e94\u5bf9\u4e8c\u6c27\u5316\u78b3\u9010\u5e74\u5347\u9ad8\u548c\u80fd\u6e90\u5371\u673a\u7684\u6709\u6548\u9014\u5f84\u3002\u7406\u60f3\u60c5\u51b5\u4e0b\uff0c\u5982\u679c\u7531\u53ef\u518d\u751f\u7535\u529b\u63d0\u4f9b\u52a8\u529b\uff0c\u5c31\u80fd\u51cf\u5c11\u6e29\u5ba4\u6c14\u4f53\u6392\u653e\uff0c\u540c\u65f6\u5b9e\u73b0\u4eba\u4e3a\u5c01\u95ed\u78b3\u5faa\u73af\u3002\u8bbe\u8ba1\u66f4\u52a0\u9ad8\u6548\u7684\u50ac\u5316\u5242\u662f\u6781\u5177\u524d\u666f\u7684\u7814\u7a76\uff0c\u7136\u800c\u4e8c\u6c27\u5316\u78b3\u6df1\u5ea6\u8fd8\u539f\u6c27\u5316\u7269\u548c\u78b3\u6c22\u5316\u5408\u7269\u7684\u969c\u788d\u662f\u5982\u4f55\u6709\u6548\u6d3b\u5316\u78b3\u78b3\u952e\u3002\u57fa\u4e8e\u6b64\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u4fde\u4e66\u5b8f\u9662\u58eb\u548c\u9ad8\u654f\u9510\u6559\u6388\u56e2\u961f<\/b><\/strong>\u8bbe\u8ba1\u4e86\u4e00\u79cd\u5229\u7528\u7eb3\u7c73\u7a7a\u8154\u7684\u201c\u9650\u57df\u6548\u5e94\u201d\u5728\u539f\u4f4d\u5f62\u6210\u78b3\u7684\u4e2d\u95f4\u4f53\uff0c\u4ece\u800c\u8986\u76d6\u5c40\u90e8\u50ac\u5316\u5242\u8868\u9762\uff0c\u4ece\u800c\u7a33\u5b9aCu+<\/sup>\u7269\u79cd\uff0c\u5b9e\u73b0CO2<\/sub>\u5230\u591a\u78b3\u71c3\u6599\u7684\u9ad8\u6548\u7387\u8f6c\u5316\u3002\u591a\u5b54\u7ed3\u6784\u53ef\u4ee5\u901a\u8fc7\u9650\u57df\u6548\u5e94\u6765\u5bcc\u96c6\u7535\u50ac\u5316\u4e8c\u6c27\u5316\u78b3\u5230\u53cd\u5e94\u4e2d\u95f4\u4f53\uff0c\u4ece\u800c\u4fc3\u8fdb\u66f4\u591a\u78b3\u4ea7\u7269\u7684\u751f\u6210\u3002\u6d41\u52a8\u7535\u6c60\u6d4b\u8bd5\u8868\u9762\u591a\u5b54\u6c27\u5316\u4e9a\u94dc\u5728C2+<\/sub>\u90e8\u5206\u7535\u6d41\u5bc6\u5ea6\u4e3a267\u00b113 mA cm -2<\/sup>\u7684\u6761\u4ef6\u4e0b\uff0cC2+<\/sub>\u4e0eC1<\/sub>\u4e4b\u6bd4\u4e3a7.2\uff0cC2+<\/sub>\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u4e3a75.2\u00b12.7%\uff0c\u6027\u80fd\u660e\u663e\u9ad8\u4e8e\u5176\u4ed6\u7ed3\u6784\u7684\u6c27\u5316\u4e9a\u94dc\u50ac\u5316\u5242\u3002\u539f\u4f4d\u62c9\u66fc\u5149\u8c31\u4e0e\u540c\u6b65X\u5c04\u7ebf\u5438\u6536\u5b9e\u9a8c\u8bc1\u5b9e\uff0c\u5728CO2<\/sub>\u8fd8\u539f\u8fc7\u7a0b\u4e2d\uff0c\u6240\u8bbe\u8ba1\u7684\u50ac\u5316\u5242\u4e2d\u7684\u88ab\u9650\u57df\u7684\u53cd\u5e94\u4e2d\u95f4\u4f53\u80fd\u591f\u6291\u5236Cu+<\/sup>\u7684\u8fd8\u539f\uff0c\u5bfc\u81f4\u4e8c\u6c27\u5316\u78b3\u5230C2<\/sub>+<\/sub>\u8f83\u9ad8\u7684\u8f6c\u5316\u7387\u3002\u8fd9\u79cd\u65b0\u7684\u8bbe\u8ba1\u7406\u5ff5\u4e3a\u4eca\u540e\u76f8\u5173\u7535\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u548c\u9ad8\u9644\u52a0\u503c\u78b3\u57fa\u71c3\u6599\u7684\u5408\u6210\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u3002<\/p>\n

\"\"<\/p>\n

\u56fe5<\/b><\/strong>. <\/b><\/strong>\u591a\u5b54\u8154\u6c27\u5316\u4e9a\u94dc\u9650\u57df\u53cd\u5e94\u4e2d\u95f4\u4f53\u4fc3\u8fdbC2+<\/sub>\u9009\u62e9\u6027\u751f\u6210\u793a\u610f\u56fe\u3002<\/p>\n

6<\/b><\/strong>\u3001J.<\/b><\/strong>\u00a0Am. Chem. Soc. <\/b><\/strong>\u5355\u5c42\u7eb3\u7c73\u7ebf\u4e0a\u56fa\u76f8\u79bb\u5b50\u8fc1\u79fb\u52a8\u529b\u5b66\u7684\u5b9e\u65f6\u53ef\u89c6\u5316<\/b><\/strong>[<\/b><\/sup><\/strong>6<\/b><\/sup><\/strong>]<\/b><\/sup><\/strong><\/p>\n

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\"\"<\/p>\n

\u56fe6<\/b><\/strong>. <\/b><\/strong>\u539f\u4f4d\u8868\u5f81\u6709\u5e8f\u7eb3\u7c73\u7ebf\u7684Ag\u79bb\u5b50\u8fc1\u79fb\u8fc7\u7a0b\u548c\u5176\u8868\u5f81\u3002<\/p>\n

\u53c2\u8003\u6587\u732e\uff1a<\/b><\/strong><\/p>\n

[1]\u00a0Jiao L, Zhang R, Wan G, et al. Nanocasting SiO2<\/sub>\u00a0into metal-organic frameworks imparts dual protection to high-loading Fe single-atom electrocatalysts[J]. Nat. Commun.<\/i><\/b><\/em><\/strong>,\u00a02020<\/b><\/strong>, 11(1): 2831.<\/p>\n

[2]\u00a0Zhuang T, Li Y, Gao X, et al. Regioselective magnetization in semiconducting nanorods[J]. Nat. Nanotechnol.<\/i><\/b><\/em><\/strong>, 2020<\/b><\/strong>, 15(3): 192-197.<\/p>\n

[3]\u00a0Guan Q, Yang H, Han Z, et al. Lightweight, tough, and sustainable cellulose nanofiber-derived bulk structural materials with low thermal expansion coefficient[J]. Sci. Adv.<\/i><\/b><\/em><\/strong>, 2020<\/b><\/strong>, 6: eaaz1114.<\/p>\n

[4]\u00a0Xue C, Li M, Yang Z, et al. Tumor microenvironment-activatable Fe-doxorubici preloaded amorphous CaCO3<\/sub>\u00a0nanoformulation triggers ferroptosis in target tumor cells[J]. Sci. Adv.<\/i><\/b><\/em><\/strong>, 2020<\/b><\/strong>, 6: eaax1346.<\/p>\n

[5]\u00a0Yang P, Zhang X, Gao F, et al. Protecting copper oxidation state via intermediate confinement for selective CO2<\/sub>\u00a0electroreduction to C2+<\/sub>\u00a0fuels[J]. J. Am. Chem. Soc.<\/i><\/b><\/em><\/strong>, 2020<\/b><\/strong>, 142(13): 6400-6408.<\/p>\n

[6]\u00a0He Z, Chang L, Lin Y, et al. Real-time visualization of solid-phase ion migration kinetics on nanowire monolayer[J]. J. Am. Chem. Soc.<\/i><\/b><\/em><\/strong>, 2020<\/b><\/strong>, 142(17): 7968-7975.<\/p>\n

\u672c\u6587\u7531zlq1213\u4f9b\u7a3f\u3002<\/p>\n

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\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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